1.1 Report on Work Package 3 : Applications of Cavity Soliton Lasers The milestone of this workpackage for the year concerns Task 1: Milestone M3.1.1 (month 12) : Observation of drifting CS in optical delay line, or identification of limiting inhomogeneities. 1.1.1 Considerations on the state-of-the art of all-optical delay lines All-optical delay lines are considered to be key component in future all-optical photonic networks, because they are needed for buffering information flow through all-optical routers (e.g., Tucker et al., Electron. Lett. 41, 208, 2005; Gauthier, Physics World, Dec. 2005, p. 30). Task 1 of WP3 is devoted to the demonstration of an all-optical delay line using cavity solitons. The basic idea behind our approach is that a serial bit stream is injected at one location within the transverse aperture of a broad-area CS device (see Fig. 3.1). The ignited CS drift with an adjustable speed determined by a controlled parameter gradient towards a selected part of the device where a time-delayed version of the original bit stream can be recovered by a local detector. Figure 3.1: Scheme illustrating the CS-based all-optical delay line in a rectangular CS-supporting photonic device: Solitons are written at the left by “1” pulses of an incoming optical bit-stream, drift rightwards on a uniform parameter gradient and a time-delayed version is read out at the side. The two lines show two frames from a simulation and illustrate the spatial shift of the bit pattern with increasing time. We remark that there is a lot of recent activity on realizing delay lines by using “slow light” in photonic crystal waveguides, resonators, semiconductor media as well as in optical fibers. Most of these schemes rely on the reduction of the group velocity of light in the vicinity of a resonance. Hence, it appears to be fruitful to explore the possibilities of using a quite different mechanism as the drift of a soliton for creating the delay. In particular, it appears that the soliton based delay line is particularly suited to produce large delays including ones which are longer than the pulse width. The record for delay seems to be about four pulse widths (Kasapi et al. Phys. Rev. Lett. 74, 2447, 1995; Boyd et al. Phys. Rev. A 71, 023801, 2005). However, this experiment is based on electromagnetically induced transparency in an atomic vapor and needs very complex and expensive laser systems to operate. More recent experiments yielding delays in the tens of ns range were performed using stimulated Brillouin scattering in optical fibers (Gonsalez-Herraez et al., Appl. Phys. Lett. 87, 081113, 2005), however the bandwidth is rather limited. Often the product of bandwidth times delay is taken as a figure of merit for an optical delay line ( e.g. Tucker et al., Electron. Lett. 41, 208, 2005). The currently anticipated value of about 5 with the potential for an increase in future devices places the CS-based systems favourable among the currently investigated schemes. In addition, we see advantages for our scheme due to the fact that the integration of routing (packet switching) and delay functions should be feasible due to the bistable character of CS and the cascadability brought about by the active character of the devices. Due to the experimental and theoretical advances made the WP has achieved its goal of demonstrating the feasibility of drifting structures in the first year and is on a good track for a demonstrator of an all-optical delay line. Details on the activities are reported below. 1.1.2 Observation and preliminary analysis of dynamic and drifting structures in devices of improved homogeneity (CNRS-INLN, UP, INFM, deliverable 3.1.1.a) UP investigated parameters of the crystal growth to optimize the layer thickness homogeneity. The most important parameter was identified to be the temperature offset between the lower and upper heater filaments of the Gallium effusions cells. Several epitaxial growth runs were needed to determine the ideal temperature offset. After optimization, the homogeneity of the dip in the reflectance spectrum was improved from +/- 0.8% to +/- 0.3% over a 3 inch wafer (see Fig. 3.2). This homogeneity provides a great advantage to generate optical cavity solitons, is of importance for all WPs, and in particular for WP3. Figure 3.2: Variation of resonance wavelength on wafer in tangential and radial directions after optimisation by UP. UP fabricated large area bottom-emitting VCSELs for optical cavity soliton generation. Devices with two different active diameters were shipped to the partners INLN and USTRAT. The first type was a bottomemitting VCSEL with 80µm active diameter whereas the second type has an active area of 200 µm. Both types were mounted on a TO56 header with a diamond heat spreader. Delay-line experiments were started at INLN in December 2005, when the new 200 micron diameter VCSEL structure was made available by UP, because these investigations naturally require a sufficient transverse extension of the amplifier structure. The first step was to set-up a spatio-temporal measurement system with sufficient bandwidth and spatial resolution. This was achieved thanks to an array of photodiodes and careful synchronization (and the characterization thereof) of several digital oscilloscopes. At present, the apparatus has a temporal bandwidth of 300 MHz with a spatial resolution of the order of 10 micrometer, on six channels simultaneously. Improvements are currently under way in order to add two channels to the previous ones. Preliminary investigations yielded first signs of complex spatio-temporal dynamics and demonstrated that in a certain parameter region, the dynamics of the system cannot be reduced to a spatially extended pattern evolving in time in a fully correlated way. While some indications for propagating structures were found at that stage, the interpretation of the time series proved to be rather difficult due to the two-dimensional nature of the system. Therefore, the experiment was modified in order to reduce the number of degrees of freedom of drifting cavity solitons. A Michelson interferometer was inserted into the optical path of the holding beam in order to inject a spatially modulated beam into the amplifier. A typical image of the near field intensity distribution is shown in Fig. 3.3. Figure 3.3: Typical near field intensity distribution obtained in the VCSEL under operating conditions with a modulated holding beam. The stripes are running along the diagonal (lower left to upper right). The circles indicate the positions of the photodetectors. INLN demonstrated that stationary CS lock at extrema of a fringe pattern (even of low modulation depth) superimposed on the homogenous holding beam. Moving this fringe pattern, the CS can be dragged around. If the contrast of the resulting fringes is close to unity, an eventual drifting cavity soliton should be forced to travel along the line defined by an interference maximum. In this configuration, INLN was able to demonstrate the propagation of a periodic wave in the transverse dimension of the system. This wave has a period of the order of 10 nanoseconds and a wavelength of the order of 40 micrometers, but these numbers clearly depend on parameters. While the propagation is naturally oriented along the line defined by the holding beam spatial modulation, the origin of the direction of propagation is still to be clarified. Under very similar experimental conditions, INLN was also able to show the motion of a single structure, oscillating around a fixed center (see Figs. 3.3 and 3.4). Applying an external perturbation, it was possible to trigger the departure of this structure from its initial position and to observe its motion over a distance of more than 30 micrometers. This structure appeared to be drifting along the line defined by the spatial modulation of the holding beam at an average speed of about 2 µm/ns. As for the case of wave propagation, the parameters controlling the direction and speed of motion are under investigation. Figure 3.4: Time series of local detectors (vertically offset for clarity). The traces from top to bottom correspond to the detectors indicated in Fig. 3.3 from left to right. The two upper lines indicate the oscillation of a structure around some equilibrium position, which detaches and drifts downstream (lower lines) after a perturbation. INLN demonstrated also a further step towards the realization of an all-optical delay line: the controlled excitation of a CS by a localized optical perturbations, which then drifts away from the ignition point. For this purpose, an addressing system with a beam diameter of 10 micrometers, a pulse duration of 100 nanoseconds and rising and falling edges below 1 nanosecond was set-up. Fig. 3.5 shows the excitation and subsequent drift of a CS using this system. The distance covered amounts to 25 m with a delay of 12 ns. This yields a velocity of about 2.1 m/ns. Figure 3.5: Optical ignition and subsequent drift of a CS. The time series of local detectors are vertically offset for clarity, where the uppermost trace monitors the ignition point and the following ones monitor points progressively downstream. The rising and falling edges of the addressing pulse (and possibly of the drifting structure) are limited by the detection bandwidth of 300 MHz. These results demonstrate the principle of an embryonic all-optical delay line fully satisfying the milestone. Details are currently under investigation, but obviously the CS-based delay line has the potential to create large delays, i.e. delays considerably larger than the pulse widths at reasonable speeds/bit rates. For a more flexible control of phase and intensity gradients an optically addressable spatial light modulator operating at 980 nanometers is currently set-up. It is addressed by a 650 nanometer beam, whose intensity is in turn prepared by a computer-controlled liquid crystal display. Motivated by these exciting experimental results, INFM performed numerical calculation on the drift of CS in vertical-cavity amplifiers with a uniform phase gradient on the injection field. Velocities around 1.5 m/ns were found in qualitative agreement with the preliminary experimental measurements. Future work will address the specific experimental situation. 1.1.3 Theoretical analysis of the motion of CS and effects of spatial variations of the background (USTRAT, deliverable 3.1.1.a) The utilisation of CS in VCSEL and VECSEL for practical applications in information technology such as those proposed in WP3 crucially depends on the possibility of controlling their spatial position and an understanding of the effects of intentional and parasitic spatial variation of the background state on selforganization and CS. In any real device, some spatial variations will be unavoidable due to growth imperfections. Previous theories and numerical simulations have shown that CS move upward in phase gradients and can be located at maxima of phase modulated backgrounds (W.J. Firth and A.J. Scroggie, Phys. Rev. Lett. 76, 1623, 1996; T. Maggipinto et al., Phys. Rev. E 62, 8726, 2000). These predictions have been experimentally verified in vertical-cavity amplifiers within the project by INLN. A general theory was developed and verified on several models where optical CS have been predicted (Scroggie, et. al., Phys. Rev. E 71, 046602, 2005). At difference with previous approaches, we found that CS can either climb or descend background modulations depending on the parameter values and crucially on the wave-vector of the background modulation. This has obvious consequences for the design of corresponding experiments. The theory is so general that it can also be applied to other spatial structures such as patterns (Scroggie et al., App. Phys. B 81, 963, 2005). By expanding these ideas, we have also formulated a general theory of the spatial response of cavity systems to input pump modulations (Scroggie et al., Phys. Rev. A 72, 023824, 2005). Finally, modulations due to photonic crystals inside the optical cavity have been shown to strongly modify the output spatial structure of nonlinear optical devices and to create novel localised structures (D. Gomila and G.-L. Oppo, Phys. Rev. E 72, 016614, 2005). The theoretical and numerical approach developed to study the motion of CS in modulated background can be extended to investigate the behaviour of CS in presence of inhomogeneities due to material fabrication being a superposition of many Fourier components. This represents essential work for the utilisation of drifting CS in a delay-line and for the development of a CS microscope. Preliminary work performed on Kerr cavities clearly shows that the CS velocity field induced by spatial noise of different bandwidths filters out high spatial frequency components. The determination of the cut-off condition is presently under investigation. At the same time, a theoretical formalism is pursued, by which the motion of a CS under the influence of irregular, noisy backgrounds can be described, which is the typical experimental situation. One important aspect of the dynamics of photonic devices based on semiconductor materials is that the carrier lifetime is considerably longer than the photon lifetime in the cavity and thus the limiting time constant for dynamical phenomena. Hence, it is likely to be also the limiting factor for the drift velocity (see, e.g. Tissoni et al., J. Opt. Soc. Am. B 16, 2095, 1999). Indeed, calculations performed for a model medium with a Kerr nonlinearity with a non-instantaneous response yield that the drift velocity per unit gradient is inversely proportional to the time constant in the perturbative limit. This shows that the speed of the CS and thus the bit-rate in a delay line can be enhanced compared to the current values by reducing the carrier lifetime. These results need to be analysed more systematically and extended to the non-perturbative case in order to access systematically the limits for the drift velocity. Figure 3.6: Drift velocity per unit gradient of a CS (in normalized units) versus , the ratio between the decay rate of the medium and the one of the intracavity field ( 0.01 for a semiconductor mircrocavity. The existence of a scaling region with slope 1 in a double-logarithmic plot shows that the medium controls the drift velocity for small . For large (corresponding to an instantaneously responding medium) the velocity saturates at a value related to the cavity response time. 1.1.4 Long-Term Spatio-Temporal Dynamics of Lasers and VCSELs (USTRAT, deliverable 3.1.1b) Several numerical models describing the generation and dynamics of cavity solitons (CS) in semiconductor lasers suffer of so-called ‘stiffness’. ‘Stiffness’ means that dynamical variables (here the optical field inside the cavity, the carrier density and the dielectric polarization) evolve on very different time scales so that the numerical implementation is very inefficient. Ten years ago the USTRAT group discovered that the straightforward elimination of fast variables in laser models with diffraction can lead to spurious instabilities and that more advanced techniques are needed for a correct description (Oppo et al., Phys. Rev. A 44, 4712, 1991) of lasers’ spatio-temporal dynamics. Semiconductor laser modelling is more complex than the one for ‘standard’ laser devices (e.g. based on solid-state materials). The difficulty of obtaining simple reduced models for broad ranges of parameter values appeared to be insurmountable for a long time. In fact, during the first part of the FunFACS collaboration several groups have used VCSEL models where the dynamics of fast variables had to be simulated in spite of the large separation of the time scales. Recently, USTRAT established that one of the main difficulties in applying the Centre Manifold (CM) technique to the elimination of fast variables can be circumvented by using higher order expansions and non-trivial terms coming from the CM theory. New models for standard two-level (e.g. solid-state) lasers and VCSELs have been derived and tested. With typical decay times of the polarization, the cavity field and the population differences being of around 100 fs, 10 ps and 1 ns, respectively, a carefully reduced model can achieve the same asymptotic result as the original simulation but 1000 times faster. Because of the much larger number of operations per step required in the reduced model, we have achieved a gain factor of 400 in the simulation time of the same spatial structures for both standard lasers and VCSELs. The final equations of the reduced models are quite complicated and are not amenable of analytic manipulations. However they represent a powerful tool for future numerical investigation of CS in a variety of experimental laser configurations ranging from injected signals to saturable absorbers relevant for WP1 and WP3. Fig 3.7 illustrates the power of the method for calculating the switch-on transient of a laser. a) b) Figure 3.7: Time evolution of snapshots after the switch-on of a laser using the full equations (a) and the reduced equations (b). The latter show a remarkable agreement with the former ones with a computational effort reduced by a factor of 400. A similar system of reduced equations was obtained by an independent method by INFM and is reported in WP1. The comparison between the two approaches and the resulting systems of equations is ongoing and will lead to a joint deliverable about this issue in the report for the second year. 1.1.5 Advancing cavity soliton manipulation towards applications by incoherent writing and erasure of cavity solitons (CNRS-LPN, deliverable 3.1.1c) The possibility to excite a CS with an incoherent beam is appealing since it eliminates the need for a controlled phase matching between the excitation and the driving field. It also constitutes a first step in the manipulation of cavity solitons. In the following, we report on the incoherent and coherent writing and erasure of CS in a broad-area, optically-pumped, vertical-cavity semiconductor optical amplifier. This result has been obtained in an optically pumped microresonator thanks to a novel cavity design. The cavity is composed of two aperiodic AlAs/AlGaAs mirrors designed for efficient optical pumping at 800nm. As a result, a pump window created on the high energy side of the multilayer mirror stop-band allows optical pumping over a 20 nm spectral width with a maximum of pump absorption. The active zone is composed of a bulk GaAs layer, surrounded by two AlGaAs absorbing spacers. The total cavity has a resonance around 880nm. The cavity is first grown upside-down and then bonded onto a SiC substrate. The sample temperature is controlled by a Peltier element and a feedback loop at temperatures close to 275K. A 800nm high-power fiber-coupled laser diode array provides a uniform pump intensity of several Watts. The near-field of the sample is re-imaged on a CCD camera and a fast detector (90 ps risetime) is used for local dynamical measurements. We first set the system in a parameter region where bistable localized spots exist. Bistability is observed by varying either the holding beam intensity or the pump beam intensity. By setting the system at the center of the hysteresis cycle, we are able to excite a cavity soliton by sending a short (60 ps) pulse on the sample, whose wavelength is different from those of the pump and the holding beam. Triggerable writing of cavity solitons by a single pulse has been demonstrated (see Fig. 3.8). A closer look at the switch-on dynamics showed that the transient consists of a ‘lethargic time’, where the system remains close to its initial state, and a ‘switching time’, where abrupt switching occurs. The first one can be of the order of hundreds of nanoseconds while the second is much faster, of the order of 1 ns. The physical origin of the lethargic time is currently under investigation, but we mention that, in this type of excitation, the pulse creates carriers at high energy that cascade very rapidly to the bottom of the bands. In contrast to the case of coherent excitation, writing is initiated by a local excess of carriers. Surprisingly, we could also erase incoherently the CS. However, in that case switch-off is obtained by setting the pump bias apart from the centre of the hysteresis cycle, closer to the switch-off threshold, and we could not in the same experiment repeatedly switch-on and off CS. The exact mechanism by which switching-off occurs is not completely understood at the moment. a) b) a) a) Figure 3.8: Time evolution of the power emitted by a vertical-cavity amplifier (black line) after being perturbed a short pulse of a Ti:Sa laser (red curve). Panel a) shows the switch-on of a CS, panel b) the switch-down. The localized spots generally appear in the central zone of the cavity, where a pump-induced transverse thermal gradient is present. The center of the pumped zone, where heating is more pronounced, has thus a red shifted cavity resonance which translates into a maximum of the field-cavity detuning, attracting the localized spot. We could independently excite two nearby localized spots in sequence by an incoherent excitation, thus demonstrating their CS character. However, the cavity resonance gradient present in the sample combined with the relatively narrow interval in parameter space where CS exist, presently does not the writing and erasure of CS at arbitrary transverse positions of the cavity. In conclusion, we have shown the fast incoherent switch-on and switch-off of cavity solitons in a vertical-cavity optical amplifier. Incoherent writing and erasure of CS opens new perspectives for optical information processing with CS as it greatly reduces the requirements on the writing beam. It also permits a wavelength conversion associated with the writing process, since the CS has a wavelength imposed by the holding beam wavelength while writing of a CS can occur in a very broad range of wavelengths. 1.1.6 Technology for top-emitting devices and design of optimised structures for current injection (CNRS-LAAS in collaboration with CNRS-LPN, CNRS-INLN and USTRAT) LAAS performed technological work on wafer growth and homogeneity of current injection in VCSELs, which is described in detail here, but which is also of high importance for WP 1. Epitaxial growth of an optically-pumped VCSEL structure designed by LPN was planned to be performed during the first year. This could not be achieved, yet, due to a failure of one of the aluminium effusion cells. For the structures grown after careful calibrations, one could not get a reasonable agreement between the measured reflectivity spectra and those calculated for the designed VCSEL structures. Furthermore, one observed a lack of reproducibility of the growth process, which prevented us from any improvement. After a thorough reverse analysis by scanning electron microscopy, a failure of the Al cell was detected. The vacuum chamber was opened which confirmed this analysis and led to the change of the defective cell. Growth will then be performed again in view of providing the optically-pumped VCSEL structures to LPN. Regarding the growth and processing of electrically driven structures, after a discussion, the Consortium has decided that LAAS would get standard VCSEL structures from UP. These wafers will be processed in LAAS using the novel techniques described below in order to improve carrier injection in topemitting VCSELs. The electrical characteristics of these multilayer structures will be also better than the ones which could be grown currently at LAAS because they use a Beryllium effusion cell for p-type doping which causes diffusion. These problems could be addressed by the use of a Carbon effusion cell installed in a new MBE chamber of which the acquisition is in discussion in LAAS. The carrier injection non-uniformity into the active zone remains the major problem for a large part of microcavity devices and a great challenge for research. Its solution would also open the way to new possibilities for this class of devices. This problem is particularly critical in the case of the large area topemitting VCSELs as those used in FunFACS. Within the FunFACS project, the main contribution of LAAS is to work on the alternative ways to improve this characteristic on standard epitaxial structures. The upper semiconductor layer and the metallic deposit must be thus optimised. -3 carrier density (cm ) A modelling study has been performed using Silvaco ATLAS software. The use of an Esaki junction or a transparent metallic ITO layer has been compared to standard annular contact on a P+ cap layer. The nonuniformity in the carrier density at the QWs between the edge and the center of a 100µm diameter VCSEL structure with an annular metallic contact on the upper P+ DBR layer has been found to be of the order of 2 (see Fig. 3.9, black line). An Esaki junction has been shown to improve this parameter to 1.56, but simultaneously has been measured on test-structures to degrade the series resistance by a factor of 2.65; therefore, this solution does not seem to be the most appropriate to solve the electrical problem in VCSEL devices. Modelling of an ITO electrode leads to a non-uniformity of the same order: 1.6 (see Fig. 3.9, blue line). This solution has been retained. We have equipped a sputtering reactor with an ITO target and performed our first ITO deposits. Up to now, the calibrations of growth rate and layer uniformity have been carried out. The optical (transmission of 98% around 850nm) and electrical characteristics of the ITO have been obtained. Next, these conducting layers will be applied onto test-structures, and the improvement in the carrier injection will be finally characterized. 1x10 19 9x10 18 8x10 18 7x10 18 6x10 18 5x10 18 4x10 18 3x10 18 Figure 3.9: Variation of carrier density along the radial coordinate of a VCSEL with an aperture of diameter of 100 m. Black line: standard top-emitter with a P+ cap laye, blue line: ITO layer, red line: patterned injection. 0 10 20 30 40 50 60 radial position ( m) In order to further improve the carrier injection uniformity, we have modelled a novel contact design. This consists of a mesh for carrier injection, which is a continuous ITO deposit upon a semiconductor layer with localized conducting apertures with predetermined sizes. These conducting apertures can be obtained thanks to localized distributed dielectric patterns on the surface. The preliminary modelling study of this solution shows a clear improvement of the carrier density uniformity (1.06, see Fig. 3.9, red line). This work will be pursued by applying this geometry to test-structures to experimentally validate its positive effect. LAAS proposed a VCSEL structure with a rectangular gain region which would be optimal for the realization of a delay-line due to the channelling of CS motion. This is supported by the latest experiments of INLN. Electrodes along the long sides of the aperture will enable quite homogenous current injection. These devices will be fabricated during the second year of the project. 1.2 WP3 Deliverables Deliverable D3.1.1: Report on status of delay line experiments and theoretical analysis. It is composed of several subparts: Deliverable D3.1.1a A. Scroggie, G.-L. Oppo, W. J. Firth, T. Ackemann, G. Tissoni, F. Prati, M. Brambilla, L.A. Lugiato, F. Pedaci, S. Barland, M. Giudici, J. R. Tredicce, R. Jäger. Report on the status of all-optical delay line: Experiments and theoretical analysis Deliverable D3.1.1b G.-L. Oppo, Long-Term Spatio-Temporal Spatio-Temporal Dynamics Dynamics of Lasers and of Lasers and VCSELs Deliverable D3.1.1c S. Barbay, Y. Menesguen, X. Hachair, L. Leroy, I. Sagnes and R. Kuszelewicz, Incoherent and coherent writing and erasure of cavity solitons in an optically pumped semiconductor amplifier, Opt. Lett. 31, 1504-1507 (2006)