SUPPLEMENTARY MATERIAL Background on the Superposed Epoch Analysis The Superposed Epoch Analysis (SEA) technique is a statistical method used to resolve significant signal to noise problems. This is especially desired in cases where the responses to particular events (in our case large radiative forcing from explosive volcanic eruptions) may be obfuscated by noise from other competing influences that operate at similar time scales (internal El Nino variation). Through simple compositing, the SEA method involves sorting data into categories dependent on a ‘key-date’ for synchronization and then comparing the means of those categories. Given sufficient data, a common underlying (causal) response to a forcing event should theoretically emerge in the average (composite) while other noise in the data should cancel. Examples of applications of the SEA method are widespread in various scientific fields of study. For example, the SEA has been employed in studies on the relationship between climate and fire histories (Swetnam and Betancourt, 1990), magnetospheric physics (Lühr et al., 1998), the lunar cycle and rainfall (Brier and Bradley, 1964), and the relationship between volcanic activity and climate variations (Mass and Portman, 1989). Compositing can also lend insight into periodic responses that, because of the relative magnitude of the signal and associated noise, are not detected by spectral analysis. The SEA method is simple and involves basic arithmetic calculations (averaging). However, the randomization procedure used to determine statistical significance, depending on the number of iterations performed, can be computationally demanding. The method requires a random number generator for the Monte Carlo randomization procedure. We used the commercially available Matlab™ statistical software package to perform our SEA. As with any statistical method, care must be taken in the application and interpretation of SEA results. For instance, the SEA can be vulnerable to leveraging resulting from the influence of a single large anomaly. This problem typically arises when the ‘key date’ sample size is small. To deal with this explicitly, our approach embraces proxy data to considerably increase the number of climatically-relevant eruptions incorporated into the SEA. We also include a normalization step in our SEA in order to provide a methodological safeguard to leveraging. Applying the SEA to the ‘Volcano-ENSO Hypothesis’ We employ the SEA method to determine the response (if any) of the El Niño-Southern Oscillation ocean-atmospheric system to negative radiative forcing resulting from volcanic dust veils following large explosive eruptions in the tropics. Such a response to explosive volcanism was proposed from observations by Handler (see references in main text) and was discussed in early model simulations (Hirono, see main text; and MacCrackan and Luther). Because the details of the SEA method can be specifically tailored to each individual application, a detailed description of the basic structure of our statistical approach is included below. This supplements the information provided in the ‘Methods’ section. First, SEA forcing events are selected based on physical criteria and typically referred to as ‘key dates’. For our application, the forcing component determining the selection of ‘key dates’ are years in which explosive eruptions took place in low-latitude (20 N to 20 S). Data sources included both the Ice-core Volcanic Index (IVI) and/or the Volcanic Explosivity Index (see ‘Methods’ sections for selection criteria and references). Given an array of key dates, we then sampled the time series that we analyze for a possible impact (NINO3 or SOI) using a window of data points centered on each key date. For each key date, the typical window used in our analysis is 21 years with 10 data points on either side of the key date. The extracted windows are then stacked in what we refer to as the ‘eruption matrix’. This symmetrical matrix contains before- and after-event information for all selected eruptions (key dates). Thus, for an 18eruption key date list, for example, the accompanying eruption matrix would contain 18 rows and 21 columns of data. Before analyzing the data, an adjustment intended to remove any disproportionate weight any extreme case could have on the overall composite is applied. This involves normalizing the individual data in each key date window by dividing each value in that row by the maximum absolute value of all anomalies in that window. This scales the magnitudes in each row of the eruption matrix so that the chance that a single anomaly may unduly influence the composite analysis is restricted. The overall mean of the eruption matrix is then removed. As an aside, we additionally employed a ranked approach to account for potential leveraging (results not shown). A ranked SEA is a version of SEA where the ENSO diagnostic anomalies extracted for each eruption are first ranked prior to insertion into the eruption matrix. This is one way of protecting against the undue influence of anomalously large-magnitude events. Results from the ranked SEA method are in good agreement with both normalized and traditional SEA analyses that we performed. Thus we have taken every step possible to protect against this potential bias. For those eruption matrices that exhibit statistically significant cooling in the post-eruption decade compared to the pre-eruption decade due to large scale volcanic cooling, the mean difference between pre- and post-eruption decades is removed (see ‘Methods’ for more discussion on the removal of the surface cooling expected). The significance of post-eruption cooling is determined using the non-parametric Mann-Whitney difference-of-mean test. The composite (or averaged) results of the SEA are simply calculated by averaging down each column in the eruption matrix (e.g. the ‘year –10’ column is averaged for all eruptions yielding the composite value for ten years before explosive eruptions). This compositing of the eruption matrix yields what we call the ‘composite matrix’. The composite matrix contains 21 years of averaged NINO3 or SOI anomalies ranging from ten years before to ten years after the selected explosive eruptions (key dates). It is this averaging procedure that allows us to compare the average values of the NINO3 or SOI in any particular year before and after large eruptions. It is the stated goal here to determine if a systematic post-key date response emerges. In order to compare these composite years and to evaluate the significance of an average anomaly determined in each composite year, several further statistical steps are required. First, the probability of occurrence for each composite value based on chance alone must be determined. To do this, we employ a Monte Carlo randomization procedure that reshuffles blocks of values inside each row of the ‘eruption matrix’ with equal weight given to each eruption. This block resampling procedure generates a randomly generated eruption matrix from the actual eruption matrix that is subsequently averaged to create a new, random composite matrix. Block resampling is based on the fact that serial correlation must be taken into account in estimating null distributions with time series with autocorrelation, or else the resulting confidence limits will be too liberal. The most straightforward way to do this is simply to resample the series in effectively independent blocks, rather than individual values. For a first order autoregressive process, the size of effectively independent blocks is given by the formula we specified (see ‘Methods’). This is repeated 10,000 times to create 10,000 randomly generated composite matrices. These 10,000 randomized composite values are then sorted and a random composite distribution is created for each column (i.e. year relative to the key year 0). These 21 distributions are used to statistically judge how anomalous the actual composites are. We use these distributions to test the significance of the actual composites at the 90%, 95%, and 99% confidence levels. Other Applications of the Superposed Epoch Analysis Brier, G.W., and Donald A. Bradley, 1964: The lunar synodic period and precipitation in the US. J. Atmos. Sci. 21, 386-395. Lühr, H., M. Rother, T. Iyemori, T. L. Hansen, R. P. Lepping. 1998. Superposed epoch analysis applied to large-amplitude travelling convection vortices. Annales Geophysicae 16(7): 743-753. MacCracken, M.C. and Luther, F.M., 1984: Preliminary estimate of the radiative and climatic effects of the El Cichon eruption. Geofisica Internacional 23(3), 385-401. Mass, C. F. and D. A. Portman, 1989: Major volcanic eruptions and climate: A critical evaluation. J. Climate 2, 566-593. Swetnam, T.W. and J.L. Betancourt. 1990. Fire-Southern Oscillation relations in the southwestern United States. Science 249:1017-1020. Time Period 1649-1979 1649-1868 1706-1868 1706-1977 1649-1979 1706-1977 1649-1979 1869 - 1979 1649-1868 1706-1977 1706-1868 1649-1979 1869 - 1979 1869 - 1979 1649-1868 1706-1868 1706-1977 1649-1979 1706-1977 1706-1868 Eruption Criteria IVI Moderate-Large IVI Moderate-Large IVI Moderate-Large IVI Moderate-Large IVI Large Only IVI Large Only VEI >= 4 * VEI >= 4 * VEI >= 4 * VEI >= 4 * VEI >= 4 * VEI moderate-large Handler List VEI moderate-large VEI moderate-large VEI moderate-large VEI moderate-large VEI large VEI large VEI large pre-event mean (A) 0.032 0.031 0.030 0.030 0.031 0.042 0.018 0.006 0.021 0.028 0.055 0.005 -0.006 0.006 -0.001 0.004 0.006 0.029 0.055 0.055 post-event mean (B) -0.035 -0.034 -0.033 -0.033 -0.034 -0.046 -0.020 -0.001 -0.024 -0.030 -0.061 -0.006 0.006 -0.007 0.001 -0.004 -0.006 -0.032 -0.061 -0.061 B-A -0.067 -0.065 -0.063 -0.063 -0.065 -0.088 -0.038 -0.007 -0.045 -0.058 -0.116 -0.011 0.012 -0.013 0.002 -0.008 -0.012 -0.061 -0.116 -0.116 P-value 0.03 0.09 0.09 0.03 0.09 0.03 0.20 0.47 0.18 0.17 0.03 0.42 0.61 0.47 0.5 0.36 0.47 0.09 0.03 0.03 Table S1. Results of the non-parametric Mann-Whitney difference-of-mean test for pre- and post- eruption periods for composite NINO3 reconstruction data. Significance values (bold) show composites that exhibit a pre-eruption mean (A) significantly greater than the post-eruption mean (B) at the p<0 .10 level according to a one sided test. The * marks eruption lists whose selection criteria require that no other eruptions of magnitude VEI>=4 occur in the 12 months before or 12 months after the chosen eruption. Eruption Criteria IVI Moderate-Large IVI Moderate-Large IVI Moderate-Large IVI Moderate-Large IVI Large Only IVI Large Only VEI >= 4, +/- 12m sep. VEI >= 4, +/- 12m sep. VEI >= 4, +/- 12m sep. VEI >= 4, +/- 12m sep. VEI >= 4, +/- 12m sep. VEI moderate-large Handler List VEI moderate-large VEI moderate-large VEI moderate-large VEI moderate-large VEI large VEI large VEI large Time Period # of events 1649-1979 25 1649-1868 18 1706-1868 13 1706-1977 19 1649-1979 12 1706-1977 8 1649-1979 20 1869 - 1979 9 1649-1868 10 1706-1977 16 1706-1868 7 1649-1979 31 1869 - 1979 10 1869 - 1979 9 1649-1868 22 1706-1868 18 1706-1977 26 1649-1979 13 1706-1977 10 1706-1868 7 Total > positive 95% Total > positive 95% Total < negative 95% Total < negative 95% Combined total significant @ 95% Total > positive 99% Total > positive 99% Total < negative 99% Total < negative 99% Combined total significant @ 99% -9 -8 -7 -6 -5 -4 -3 -2 -1 0 1 2 3 4 5 6 7 8 9 N P P N N N P P P* P P P P P N P N* P N N N N* P* N P P N N P P N P N P N P P P P P N N N P* 4 0 0 3 0 0 1 0 0 8 0 0 0 0 0 1 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 1 10 0 2 6 0 0 3 0 0 0 0 0 0 0 0 0 0 0 1 0 0 1 0 0 36 0 0 0 1 0 19 9 0 0 9 17 1 0 7 N 0 3 0 0 0 2 0 5 Table S2. Normalized, Mean-adjusted Annual NINO3 Reconstruction S.E.A Results. Years with positive composite values at the 95 and 99% confidence level are marked by P and P*, respectively; years with negative composite values at the 95 and 99% confidence level are marked by N and N*, respectively. Eruption Criteria IVI Moderate-Large IVI Moderate-Large IVI Large Only VEI >= 4, +/- 12m sep. VEI >= 4, +/- 12m sep. VEI >= 4, +/- 12m sep. Handler List VEI moderate-large VEI moderate-large VEI moderate-large VEI large VEI large Time Period # of events -8 -7 -6 -5 -4 -3 1706-1868 13 1706-1977 19 N 1706-1977 8 1869 - 1979 9 N 1706-1977 16 N 1706-1868 7 Handler List 10 P 1869 - 1979 9 N 1706-1868 18 P P 1706-1977 26 N 1706-1977 10 1706-1868 7 Total > positive 95% 1 1 0 0 1 0 Total > positive 95% 5 Total < negative 95% 0 1 0 0 0 4 Total < negative 95% 5 Total > positive 99% 0 0 0 0 0 0 Total > positive 99% 0 Total < negative 99% 0 0 0 0 0 0 Total < negative 99% 0 -2 -1 0 1 2 3 4 5 6 7 8 N N* P N* P N N* P N N* 0 2 0 0 0 0 0 0 0 1 0 1 0 0 1 6 0 0 0 0 0 0 0 7 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 4 0 0 0 0 0 0 0 4 Table S3. Normalized, Annual Winter SOI Reconstruction S.E.A Results. Years with positive composite values at the 95 and 99% confidence level are marked by P and P*, respectively; years with negative composite values at the 95 and 99% confidence level are marked by N and N*, respectively. Time Period 1856-2001 1856-2001 1856-2001 1856-2001 Eruption Criteria Largest IVI/VEI VEI >= 4, +/- 12m sep. VEI Moderate-Large IVI Moderate-Large Total > positive 90% Total > positive 90% Total < negative 90% Total < negative 90% Total > positive 95% Total > positive 95% Total < negative 95% Total < negative 95% # of events -7 -6 -5 -4 -3 -2 -1 6 10 N n p 11 N N 9 0 0 0 0 0 1 0 1 2 2 0 0 0 0 0 4 0 0 0 0 0 0 0 0 2 1 0 0 0 0 0 3 0 1 2 3 4 5 6 7 p p n P n 0 3 0 2 0 1 0 0 3 0 0 0 0 0 0 0 0 0 0 0 2 0 1 0 0 0 0 0 0 0 0 0 0 0 0 0 Table S4. Normalized, 3-yr Instrumental (Kaplan) Boreal Cold-season NINO3 S.E.A Results. Years with positive composite values at the 90 and 95% confidence level are marked by p and P, respectively; years with negative composite values at the 90 and 95% confidence level are marked by n and N, respectively. Eruption Criteria Time Period # of events -6 -5 -4 -3 -2 -1 0 Largest IVI/VEI 1869-2001 6 N VEI >= 4, +/- 12m sep. 1869-2001 9 N n VEI Moderate-Large 1869-2001 11 N N IVI Moderate-Large 1869-2001 9 p n 0 0 0 0 0 1 0 Total > positive 90% Total > positive 90% 1 0 0 0 0 2 0 0 4 Total < negative 90% Total < negative 90% 2 4 0 0 0 0 0 0 0 Total > positive 95% Total > positive 95% 0 0 0 0 0 2 0 0 2 Total < negative 95% Total < negative 95% 2 2 1 2 3 4 5 6 7 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 0 Table S5. Normalized, 3-yr Instrumental Winter SOI S.E.A Results. Years with positive composite values at the 90 and 95% confidence level are marked by p and P, respectively; years with negative composite values at the 90 and 95% confidence level are marked by n and N, respectively. Eruption Criteria Time Period # of eruptions Eruption Years IVI M-L IVI M-L IVI M-L IVI M-L IVI Large IVI Large 1650-1980 1650-1868 1706-1868 1706-1980 1650-1980 1706-1980 25 18 13 19 12 8 1660 1665 1674 1694 1712 1721 1728 1747 1753 1775 1789 1795 1808 1813 1815 1824 1831 1835 1862 1884 1890 1903 1929 1963 1969 1660 1665 1674 1694 1712 1721 1728 1747 1753 1775 1789 1795 1808 1813 1815 1824 1831 1835 1721 1728 1747 1753 1775 1789 1795 1808 1813 1815 1824 1831 1835 1721 1728 1747 1753 1775 1789 1795 1808 1813 1815 1824 1831 1835 1862 1884 1890 1903 1929 1963 1665 1674 1694 1712 1747 1808 1815 1831 1835 1884 1903 1963 1747 1808 1815 1831 1835 1884 1903 1963 Table S6. IVI-based Eruption Lists. M-L denotes lists containing moderate and large explosive eruptions. Eruption Criteria Largest IVI/VEI VEI >= 4* VEI M-L IVI M-L Time Period 1856-2001 1856-2001 1856-2001 1856-2001 # of eruptions 6 10 11 9 Eruption Years 1884 1903 1951 1963 1982 1991 1869 1884 1899 1902 1911 1917 1943 1951 1963 1968 1884 1899 1902 1911 1917 1943 1951 1963 1968 1982 1991 1884 1890 1903 1929 1963 1969 1975 1982 1991 Table S7. Full Instrumental Period Eruption Lists. M-L denotes lists containing moderate and large explosive eruptions. The * marks lists that require eruptions to be separated from any other VEI>=4 eruptions by at least 12 months. Eruption VEI M-L Handler VEI M-L VEI M-L VEI M-L VEI M-L VEI Large VEI Large VEI Large Criteria Time Period 1650-1980 1869 - 1980 1869 - 1980 1650-1868 1706-1868 1706-1980 1650-1980 1706-1980 1706-1868 31 10 9 22 18 26 13 10 7 # eruptions Eruption Years 1661 1665 1674 1680 1720 1745 1756 1760 1761 1764 1768 1791 1793 1803 1808 1812 1813 1814 1815 1818 1823 1835 1884 1899 1902 1911 1917 1943 1951 1963 1968 1869 1883 1899 1902 1911 1917 1937 1950 1952 1963 1869 1884 1899 1902 1911 1917 1943 1951 1963 1661 1665 1674 1680 1720 1745 1756 1760 1761 1764 1768 1791 1793 1803 1808 1812 1813 1814 1815 1818 1823 1835 1720 1745 1756 1760 1761 1764 1768 1791 1793 1803 1808 1812 1813 1814 1815 1818 1823 1835 1720 1745 1756 1760 1761 1764 1768 1791 1793 1803 1808 1812 1813 1814 1815 1818 1823 1835 1884 1899 1902 1911 1917 1943 1951 1963 1671 1673 1680 1745 1768 1772 1812 1814 1815 1835 1869 1884 1951 1745 1768 1772 1812 1814 1815 1835 1869 1884 1951 Table S8. VEI-based Eruption Lists. M-L denotes lists containing moderate and large explosive eruptions. 1745 1768 1772 1812 1814 1815 1835 Eruption Criteria Time Period # of eruptions Eruption Years Used VEI >= 4 * VEI >= 4 * VEI >= 4 * VEI >= 4 * VEI >= 4 * 1650-1980 1869 - 1980 1650-1868 1706-1980 1706-1868 7 20 9 10 16 1671 1673 1680 1745 1768 1772 1812 1814 1815 1835 1869 1884 1899 1902 1911 1917 1943 1951 1963 1968 1869 1884 1899 1902 1911 1917 1943 1951 1963 1671 1673 1680 1745 1768 1772 1812 1814 1815 1835 1745 1768 1772 1812 1814 1815 1835 1869 1884 1899 1902 1911 1917 1943 1951 1963 1745 1768 1772 1812 1814 1815 1835 Table S9. VEI>=4 Eruption Lists. M-L denotes lists containing moderate and large explosive eruptions. The * denotes that the selection criterion requires eruptions to be separated from any other VEI>=4 eruptions by at least 12 months. The criterion for selection used in these lists is the same as that used by Handler and colleagues.