0 400 -250 V1 (0.5m) -500 V2 (1.0m) 300 -750 V3 (1.5m) -1000 V4 (2.0m) -1250 Sg (W/m2) -1500 200 -1750 -2000 100 -2250 -2500 Results Figure 1a) shows the time series of potential and solar radiation for a day with fair weather conditions (average windspeed at 3m was 1.9ms-1, aerosol mass concentration M = 38 μgm-3, few clouds). During the day the potential increases with height and the mean value at 1m is about 180V between 15:00 and 20:00 (British Summer Time). Fluctuations are correlated at different heights and increase in magnitude with height. 1 600 0.75 0.5 0.25 0 00:00 02:00 04:00 06:00 08:00 10:00 12:00 14:00 16:00 18:00 20:00 22:00 00:00 -0.25 potential (volts) -0.5 -0.75 -1 -1.25 -1.5 -1.75 -2 time (BST) Figure 1b) gradient Richardson number for 7th August 1998. Values of -Ri < 1 indicate moderately unstable conditions. 600 1000 750 500 500 250 0 -250 400 -500 V1 (0.5m) -750 300 V2 (1.0m) -1000 V3 (1.5m) -1250 -1500 V4 (2.0m) 200 -1750 Sg (W/m2) -2000 100 -2250 -2500 -2750 0 00:00 02:00 04:00 06:00 08:00 10:00 12:00 14:00 16:00 18:00 20:00 22:00 00:00-3000 -3250 -100 -3500 time (BST) Figure 2a): Solar radiation and time series of potential profile for day 11th August 1998, fair weather conditions. Figure 1b) shows the gradient Richardson number stability parameter 1.00 g T where T is temperature and U is wind speed. It represents the relative importance of buoyancy and wind shear in producing turbulence. Onset of turbulence in unstable conditions occurs when Ri<0.25. Turbulence is supressed in stable conditions when Ri>1. It can be seen from figures 1a) and 1b) that the potential starts to increase within an hour of the onset of turbulence. Values of potential reduce dramatically shortly before 21:00 BST when the atmosphere has returned to stable conditions (Ri >1). This suggests a strong link between the diurnal variation of potential in the surface layer and local atmospheric stability. 0.75 gradient Richardson number z Ri T 2 U z 1000 750 500 250 0 -250 400 -500 -750 V1 (0.5m) 300 -1000 V2 (1.0m) -1250 V3 (1.5m) -1500 200 V4 (2.0m) -1750 Sg (W/m2) -2000 100 -2250 -2500 -2750 0 -3000 00:00 02:00 04:00 06:00 08:00 10:00 12:00 14:00 16:00 18:00 20:00 22:00 00:00 -3250 -100 -3500 500 0.50 0.25 0.00 00:00 02:00 04:00 06:00 08:00 10:00 12:00 14:00 16:00 18:00 20:00 22:00 00:00 -0.25 -0.50 time (BST) Figure 3 a) Solar radiation and potential profile for 20th August 1998. It has been observed that clouds have an effect on surface electrical parameters (Whitlock and Chalmers, 1956) assumed to be due to their charge. Figure 3a) shows solar radiation and potential profile for 12 th August 1998. The sharp minimum in solar radiation was due to a band of altocumulus cloud that passed over the Sonning measurement site. It can be seen that the potential at all heights was considerably reduced in the presence of the cloud. 400 1000 750 500 250 300 0 -250 250 -500 -750 V1 (0.5m) 200 -1000 V2 (1.0m) -1250 V3 (1.5m) 150 -1500 -1750 Sg (W/m2) 100 -2000 -2250 50 -2500 -2750 0 -3000 00:00 02:00 04:00 06:00 08:00 10:00 12:00 14:00 16:00 18:00 20:00 22:00 00:00-3250 -50 -3500 350 time (BST) Figure 3a) solar radiation and potential profile time series for 12th August 1998. Altocumulus cloud causes large reduction in potential. 100 95 90 23 potential gradient 22 temperature 85 21 80 75 20 70 1.00 19 65 0.75 gradient Richardson number An electrostatic fieldmill (Chubb Instruments, UK) was used to make fast response measurements of potential gradient at 2.85m. It was mounted adjacent to a sonic anemometer and platinum resistance thermometer. All three instruments were logged at 4Hz and the data was used to perform eddy correlation and calculate turbulence statistics. Figure 1a) Solar radiation and potential profile time series for 7 th August 1998. Fair weather conditions prevailed. solar radiation (W/m2) Instrumentation Passive wire antennas of length 20m were used to sense atmospheric potential. Electrometers (Harrison, 1997) were used to measure the potential on each wire. Four antennas were mounted in a vertical array at heights 0.5, 1, 1.5 and 2m above the surface. Vertical profiles of temperature and wind were measured using fine wire platinum resistance thermometers and cup anemometers. Aerosol mass concentration in the size range 0.1 to 15 μm was monitored using an optical counter. Solar radiation was measured using a solarimeter and wind speed and direction at 3m were measured using a cup anemometer and a wind vane. All instruments were logged at 1Hz and data was averaged and stored every 5 minutes. -3500 time (BST) gradient Richardson number Field Campaign Measurements were made in the U.K.at Sonning Farm, a semi-rural site near to Reading, during July and August 1998. Surrounding terrain consisted of gently sloping fields divided by shrubs and low trees. Traffic on a busy road to the south of the site presented a considerable source of particulate pollution with semi-diurnal fluctuation. Anti-cyclonic conditions prevailed for most of the measurement period. -100 potential (volts) These results underline the need to treat electrical and micrometeorological parameters as a coupled system in the atmospheric surface layer. This poster presents some results from a field campaign where the effects of turbulence and aerosol concentration on measurements of potential were investigated. -2750 0 -3000 00:00 02:00 04:00 06:00 08:00 10:00 12:00 14:00 16:00 18:00 20:00 22:00 00:00 -3250 Effect of clouds on surface layer parameters 60 18 0.50 55 0.25 0.00 00:00 02:00 04:00 06:00 08:00 10:00 12:00 14:00 16:00 18:00 20:00 22:00 00:00 -0.25 solar radiation (W/m2) 250 Figure 2a) shows solar radiation and potential profile time series for the 11th August 1998. There were few clouds, mean 3m windspeed was 1.5 ms-1 and aerosol mass concentration was 8 μgm-3. The average potential at 1m is approximately 100 Vm-1 between 14:00 and 22:00 which is lower than for the 7th August 1998. As there is less aerosol this may be due to increased conductivity. Figure 2b) shows large negative values of Ri during the day. This indicates strong convection and thermal plumes can occur for values of Ri < -1 (Lumley and Panofsky, 1964). Quasi-periodic fluctuations in potential occur at each height between approximately 13:00 and 17:00. Similar fluctuations were observed in temperature and wind at the same time. They coincide with a period of strong convective activity. The fluctuations in potential may be due to thermal plumes transporting space charge upwards. If this is the case then true fair weather conditions are not occuring as the plumes represent a local charge generator. The definition of fair weather should therefore be extended to exclude strongly convective periods. 50 11:30 11:40 11:50 12:00 12:10 12:20 temperature (degrees Celsius) 500 potential (volts) 750 potential gradient (V/m) 1000 500 solar radiation (W/m2) 600 potential (volts) Introduction Turbulent transport of space charge in the surface layer is established as important in determining profiles of electrical parameters. Any realistic model of the electrode effect (Hoppel,1967) has to include the effects of turbulence and aerosol. Law (1963) deduced that there was a considerable convection current when examining measured profiles of ions. In addition, the nature of the turbulent transport of space charge is dependent on its composition (Anderson,1977), whether it is particulate or ionic. solar radiation (W/m2) Turbulent transfer of space charge in the atmospheric surface layer J.F.Barlow and R.G.Harrison Department of Meteorology, University of Reading, PO Box 243, Earley Gate, Reading, RG6 6BB, U.K. 17 12:30 time (BST) -0.50 -0.75 -1.00 time (BST) Figure 3 b) gradient Richardson number for 20th August 1998. Low values show near neutral stability. Figure 3a) shows potential and solar radiation for a non fair weather day. From the solar trace it can be seen there was considerable cloud, the mean windspeed at 3m was 3.9 ms-1 and aerosol mass concentration was moderate (M = 35μgm-3). Figure 3 b) shows that the gradient Richardson number was small (|Ri|0.03) from 07:00 onwards. This indicates that atmospheric conditions were near neutral meaning that turbulence was predominantly mechanical in origin. Figure 3b) 4 Hz measurements of potential gradient and temperature between 11:30 and 12:30 on 12th August 1998. As the cloud passes both temperature and potential gradient are markedly reduced. Figure 3b shows fast response measurements of temperature and potential gradient made at 2.85m. The minimum in temperature occurs roughly 4 minutes before the minimum in potential gradient. The reduction in "noise" in the temperature trace shows that turbulence strength was reduced considerably. The gradient Richardson number was also observed to decrease during this time, indicating a change from unstable to near neutral conditions. Although the cloud could have been electrified, the reduction in the turbulent flux of surface charge associated with the thermal effects of the cloud is considered much more likely to have caused the potential gradient changes. -0.75 -1.00 -1.25 -1.50 -1.75 -2.00 time (BST) Figure 2b): gradient Richardson number for 11th August 1998, fair weather conditions. Large negative values indicate strong convection. The potential decreases at all heights between 19:00 and 20:00 but later increases. This behaviour was only observed when conditions at night were not stable (Ri < 1). Under such conditions mechanical production of turbulence is not supressed by buoyancy. Therefore the overnight increase in potential is probably due to the turbulent mixing of space charge. References Anderson, R.V. (1977) Atmospheric electricity in the real world in "Electrical processes in Atmospheres",ed. H. Dolezalek and R. Reiter, Steinkopf Verlag, Darmstadt Harrison, R.G.(1997) An antenna electrometer system for atmospheric electrical measurements, Rev. Sci. Ins., 68 (3), 1599-1603 Hoppel, W.A.(1967) Theory of the electrode effect, J.A.T.P., 29, 709-721 Law, J (1963) The ionisation of the atmosphere near the ground in fair weather, Q.J.R.M.S., 89, 107-121 Lumley, J.L. and Panofsky, H.A. (1964) The structure of atmospheric turbulence, John Wiley, New York. Whitlock, W.S. and Chalmers, J.A.(1956) Short-period variations in the atmospheric potential gradient, Q.J.R.M.S., 82, 325-336 Turbulent transfer of space charge in the atmospheric surface layer J.F.Barlow and R.G.Harrison Department of Meteorology, University of Reading, PO Box 243, Earley Gate, Reading, RG6 6BB, U.K.