NUCLEAR MODELS In the absence of a detailed theory of nuclear structure, attempts have been made to correlate nuclear data in terms of rough pictures or "models" of the nucleus. Several models have been proposed, each of which is useful in a limited way. Each is used to explain some nuclear phenomena but fails when applied to data outside its range. The models we shall discuss are : the "liquid drop" model which accounts for the nuclear binding energy ; the "shell model" which accounts for the existence of stable isotopes and describes their energy states and their angular momenta ; and also the "collective model" including some rotational and vibrational states. 1. LIQUID - DROP MODEL 1-1 Liquid-drop Model A nucleus may be considered to be analogous to a drop of incompressible fluid of very high density —1014 g/ cm3). This is encouraged by the fact that some of the properties of nuclear forces (saturation and short-range) are analogous to the properties of 1 forces which hold a liquid drop together. The essential assumptions are (i) the nucleus consists of incompressible matter so that R ∝A1/3 (ii) the nuclear force is the same for every nucleon and does not depend on whether it is a neutron or a proton. (iii) the nuclear force saturates This idea has been used together with other classical ideas such as electrostatic repulsion and surface tension to set a semi-empirical formula for the mass or binding energy of a nucleus in its ground state. 1-2 Semi-empirical Mass Formula The formula has been developed by considering the different factors which affect the binding energy, and weighting these factors with constants derived from theory when possible and from experimental data where theory cannot help. Contributions to the total binding energy of the nucleus : (l) Volume energy: The main contribution to Bt comes from a term proportional to the mass no. A, since the volume of the nucleus is 2 also proportional to A , this term is regarded as a "volume energy". π©π = ππ π¨ (7-1) (2) Surface energy: Eq. (7-1) is the binding energy for an "infinitely" large nucleus. Actual nuclei are finite and are usually spherical in shape; hence nucleons on the surface are not attracted as much as estimated. A term proportional to the surface area must be subtracted from the infinite nucleus expression. (3) Coulomb energy between the protons tends to lower Bt and it is given as a negative term. It can be shown that the total Coulomb energy of a nucleus of charge Z is given by . 3 (4) Asymmetry energy: The greatest Bt occurs for symmetric nuclei where Z= N. The asymmetry energy is the difference between the Bt of a nucleus A (Z,N) and the Bt of the symmetric isobar with Z=N=1/2A. To find the difference in b-e . Let us start with the identical energy states of neutrons and protons in the symmetric nucleus. Now, transfer some n protons to neutrons in order to reach the asymmetric case. Now, 4 (5) Pairing energy: Experimental results showed that nuclei with even no. of protons and neutrons (even-even nuclei) are the most stable and have greatest values of Bt . The "odd-odd" nuclei are least stable and have the least values of Bt, while the "odd-A" nuclei are intermediate. A correction term "ο€' is added to Bt to account for these differences. +ο ο€ is added to the Bt in case of even-even nuclei -ο ο€ is added to the Bt in case of odd-odd ο€ is considered zero for odd-A nuclei. 5 (6) Shell effects: An extra tem ο¨ is added to Bt expression to show the effect of the shell structure on Bt . ο¨ has a positive value when N or Z approaches a "magic number", i.e. approaches a closed shell configurations. (Magic numbers are 2, 8, 20, 28, 50, 126) . The total binding energy of a nucleus (Bt) can now take the form The constants of the semi-empirical mass formula can be determined by comparison with available data. The "fit" is never perfect, and hence several sets of coefficients have been used- One such set is (in MeV) The contributions of the various terms to the average b.e. per nucleon, Bave is shown in the figure and it fits with the experimental curve for Bave . 6 7-3 Abundance Systematics of Stable Nuclides The nuclides found on the earth are either stable or are radioactive with half-lives longer than 5×109 years (the age of earth) . The figure below presents an N, Z plot for the known stable nuclides 7 For light nuclides, the average "line of stability" clusters around N=Z; for heavier ones, it deviates from this because the increasing effect of the Coulomb repulsion between protons. We notice that Particularly high stability and high abundance with respect to neighboring nuclides is associated with nuclides for which N or Z is equal to 2, 8, 20, 28, 50, 82 and 126. These "magic numbers" reflect the effects of closed shells (like closing of electronic shells in atoms) 7-4 Mass Parabolas 7-5:Closing Remarks (l) Although we have applied the liquid-drop model only to ground states of nuclei, it can also be used for excited states. These would be produced by oscillations of the nuclear "drop" or by ripples traveling over its surface. This idea is particularly useful in explaining nuclear fission. 8 (2) The liquid-drop model stresses cooperative effects between many nucleons and is the basic idea for the "collective" models. 7-6. SHELL MODEL An Impressive amount of experimental material has been accumulated which show periodic variations in many nuclear properties (similar to the regularities in the chemical and physical properties of atoms as shown in the periodic table of the elements). These properties showed marked discontinuities which point to shell closures at certain even values of proton and neutron numbers. These numbers, called the "magic numbers" are: 2, 8, 20, 28, 50, 82 and 126 7-7 Experimental Basis of the Shell Model (l) The abundance data of stable isotones (nuclides of the same N and different Z) show that the number of stable isotones is particularly high when N is a magic number 9 (2) The separation energy for a neutron Sn is very high when N is a magic number (because it is very hard to separate a neutron from a closed shell). On the other hand, Sn becomes very low when N=(magic no. + l). (3) Magic nuclei, being more tightly bound, require more energy to be excited than non-magic nuclei. (4) Magic N nuclei have smaller fast-neutron capture sections. (The cross section is proportional to the probability of a nuclear reaction). This can be explained by the saturation of the neutron closed shells. 10 7-8 Basic Assumptions of Shell Model (1) In spite of the strong interactions between nucleons, each nucleon is assumed to move in its orbit Independent of that of other nucleons. The orbit is determined by the potential energy function V(r) which represents the average effect of all interactions with 11 other nucleons. If all inter-nucleon couplings (called residual interactions) are ignored, we call the model the "single-particle shell model" (2) Neutrons and protons are arranged in separate shells and each shell has a certain maximum number of neutrons or protons. (3) When a shell is completely filled, the resulting configuration is particularly stable and has a lower value of energy. (4) Pauli exclusion principle is applied to both protons and neutrons. It excludes two protons or two neutrons from occupying the same quantum state, i.e., two identical nucleons cannot have the same set of quantum numbers. 7-9 Theoretical Solutions The aim of theoretical studies is to solve the Schrodinger equation for a particle moving in a spherically symmetric central field of force- In this case, we can show that the general wave function can be separated in spherical coordinates r, ο± andο ο¦ 12 13 14 15 16 7-9C Spin - Orbit Coupling (π΅ − πΊ coupling) The successful trial was done independently by Mayer and Haxel in 1949. They proposed a non-central component to the nuclear force. It is the strong interaction existing between the orbital angular momentum π΅β and the intrinsic spin angular momentum sβ, the two angular momenta couple to form the total angular momentum jβ. In terms of quantum numbers, we get that J= π΅ ± π π (6-26) Due to this strong interaction, a different energy is associated with each value of j , giving rise to the splitting of the levels due to spinorbit coupling. Remarks. (i) The term with the higher j value is more stable so it has a lower energy value. (ii) The energy separation of the two levels is roughly proportional to the value of π΅ Sometimes the levels with high j values are lowered very much so that they appear with levels of lower N value (lower shell) (iii) Each state is occupied by a number of nucleons equal to (2j+1) 17 (iv) In spectroscopic notation, the j value is placed as a subscript to the (n, π΅) symbol. For example, for the 1p shell, the splitting produces 1p1/2 and 1p3/2 levels . We can see from the figure that when the value of the spin-orbit coupling is properly adjusted; the major shell breaks occur at the experimentally determined magic numbers. 18 7-10 Applications of Shell Model (l) Assuming that the angular momentum of odd-A nuclei is determined by the odd-nucleon, a remarkable agreement is obtained between the ground state spins (and parities) of these nuclei and the predictions of the spin-orbit coupling (2) The long-lived isomers (having half-lives greater than one second) are found to exist at mass numbers just below magic numbers, and when the shell is completely filled the isomer states disappear. These long-lived states are caused by large angular momentum differences and small energy differences which make the transitions highly forbidden (having very small probability thus very long half-lives). (3) Experimental magnetic moment values and electric quadrupole measurements are in good agreement with the calculations based on the shell model. Some large quadrupole moment values indicate that the nucleus is not spherical but rather spheroidal in shape, which 19 led to developing the ideas of the "collective" motion of nucleons. 7-11 Angular Momenta of G.S. For even-even nuclei: (1) For even-even nuclei: It is found experimentally that all eveneven nuclei have zero g.s., spins. -It follows that in the g.s. of any nucleus, the net angular momentum associated with an even N or Z is equal to zero. (2) For odd-A nuclei, the angular momentum of the nucleus is determined solely by that of the last odd nucleon. Example: For 7Li3 nucleus, the odd proton lies in the 1p3/2 state- The angular momentum of Li nucleus is I=3/2 (3) For odd-odd nuclei, the angular momentum of the odd proton, Ip , couples with that of the odd neutron, In , where I= Ip + In (Vector addition) (7-27) In terms of quantum numbers, we have I= (Ip+In) , (Ip+In-1), ………..|π°π + π°π | (7-28) Ground states of nuclei are usually formed when the intrinsic spins of the proton and the neutron are parallel - 20 Example: In the case of the deuteron, Ip = ½ and In = ½ the total ang. momentum I=0 or I=1 The g.s. of deuteron has I = 1 , because the g.s. favors the parallel spins (and this is confirmed experimentally) 7-12 Parities of G.S. The parity of the wave function describing a nuclear state is determined by the orbital motion of the nucleon. Since the angular part of the wave function is proportional to the associated Legendre polynomial of the order π΅ in cosο±ο , π·π΅ (cos ο±) , the parity is given ο° is given by π = (−π)π΅ (7-29) (l) For even-even nuclei , all the g.s. have I=0 , thus π΅ = 0 and they all have even parities (ο°ο½ + l) (2) For odd-A nuclei, the parity for the nucleus is determined by the parity of the last odd nucleon. Example : For 15N7 nucleus, the odd proton lies in the 1pl/2 state, it has an odd parity- thus π΅ = π and ο° =-1, it has an odd parity (3) For odd-odd nuclei , the parity of g.s. of the nucleus is the product of the parities of the odd proton (ο°p) and that of the odd neutron (ο° n) , thus 21 ο ο ο ο ο ο ο ο ο ο ο ο ο ο° (total) =ο ο°p + ο° n (7-30) Example: For 6Li3 , the odd proton and the odd neutron both lie in the 1p3/2 state . they both have π΅ = π thus ο°p = -1 and also ο°n =-1 . The parity of g.s. of 6Li is even (ο°ο ο½ο ο«l) 7-13 Closing Remarks (l) Although the shell model explains successfully many aspects of the nuclear structure yet it is not sufficient to explain other aspects. There is mounting evidence that there are other residual forces between nucleons, forces other than that already taken into account in the shell model potential. (2) One of the residual forces is the nucleon-nucleon Interaction that favors the paring of nucleons with opposing angular momenta. An attractive force must be added to the single nucleon spin-orbit interaction, which gives rise to the pairing energy. The magnitude of the pairing energy increases with the π΅ value of the pair. For this reason, the high-spin states like h11/2 and i13/2 predicted by the model are not found in g.s. of odd-A nuclei. For example, the energy of six nucleons in 2d5/2 plus one in 1hl1/2 is higher than the energy of five nucleons in 2d5/2 plus two paired in h11/2 , the latter system is lower in energy and is favored in nature. 22 iii. COLLECTIVE MODEL For heavy nuclei, many predictions of the single-particle shell model do not agree quantitatively with experiment. The discrepancies are particularly severed for magnetic dipole moments. Also, the shell model predicts vanishingly small quadrupole moments for closed shells, and quadrupole moments of opposite sign for neighboring nuclei with atomic numbers π ± π.although this agrees qualitatively with experiment, the measured values of quadrupole moments are very different from the predictions. In fact some heavy nuclei appear to have large permanent electric quadrupole moments, suggesting a nonsphericity in the shape of these nuclei. This is certainly not consistent with the assumptions of the shell model, where rotational symmetry plays a crucial role. 23 In a revival of the liquid drop model, Aage Bohr noted that many properties of heavy nuclei could be attributed to a surface motion of the nuclear liquid drop. Furthermore, James Rainwater showed that excellent agreement between the expected and measured values of magnetic dipole and electric quadrupole moments could be obtained under the assumption that the liquid drop had an aspherical shape. These successes presented some- what of a dilemma because the liquid drop model and the single-particle shell model had fundamentally opposite viewpoints about the nature of nuclear structure. Individual particle characteristics, such as intrinsic spin and orbital angular momentum, play no role in a liquid drop picture, where collective motion that involves the entire nucleus has prime importance. On the other hand, individual nucleon properties, especially of the valence nucleons, are crucial to the success of the independent-particle shell model. The shell model had yielded too many important nuclear features to be abandoned outright, and reconciliation between the two extreme views was needed. The reconciliation was brought about by Aage Bohr, Ben Mottelson and James Rainwater who proposed a collective model for the nucleus that provided many features that were not present in either the shell or the liquid drop model. In what follows, we describe this model only qualitatively. Its basic assumption is that 24 1. a nucleus consists of a hard core of nucleons in the filled shells, and outer valence nucleons that behave like the surface molecules in a liquid drop. 2. The surface motion (rotation) of the valence nucleons introduces a nonsphericity in the central core, which in turn affects the quantum states of the valence nucleons. In other words, one can think of the surface motion as a perturbation that causes the quantum states of the valence nucleons to change from the unperturbed states of the shell model. This adjustment accounts for the difference in predictions for dipole and quadrupole moments from those given by the shell model. Physically, one can view the collective model as a shell model with a potential that is not spherically symmetric. Spherically symmetric nuclei are, of course, insensitive to rotations, and consequently rotational motion cannot produce additional (rotational) energy levels in such nuclei. Aspherical nuclei, on the other hand, can have additional energy levels because of the presence of rotational and vibrational degrees of freedom. These types of effects modify the predictions of the simple shell model. In particular, large nonsphericity in nuclei can provide large permanent dipole and quadrupole moments. Mathematically, these ideas can be incorporated as follows. For 25 simplicity, we assume the nucleus to be an ellipsoid defined by the form Where a and b are parameters related to the deformation from a spherical shape of radius R and fixed volume 4/3 ο°R3. The mean potential for nuclear motion can then be chosen as Needless to say, more realistic calculations in the collective model provide even better descriptions of nuclear properties, but they also become far more complicated. One of the important predictions of the collective model is the existence of rotational and vibrational levels in a nucleus. These levels can be derived much the same way as is done for the case of molecules. Thus, we can choose the Hamiltonian for rotations to be with eigenvalues π΅(π΅+π) ππ βπ where the effective moment of inertia I is a function of the nuclear shape. If there is rotation about an axis 26 perpendicular to the symmetry axis of the ellipsoid, it can then be shown that the angular momentum of the rotational levels can only be even. Thus, we see that rotational and vibrational levels in a nucleus are predicted with specific values of angular momentum and parity. Such excitations have indeed been found through the observation of photon quadrupole transitions (π«π΅ = π) between levels. Finally, the collective model accommodates quite naturally the decrease, with increasing A, of the spacing between the first excited state and the ground level in even-even nuclei, as well as the fact that the spacing is largest for nuclei with closed shells. The first follows simply because the moment of inertia grows with A, which decreases the energy eigenvalue of the first excited rotational state. The latter is due to the fact that a nucleus with a closed shell should not have a rotational level because such a nucleus would tend to be spherical. On the other hand, such a nucleus can have vibrational excitations. However, vibrational excitations involve the entire core and not just the surface. The core being much more massive implies that the energy level for vibration will lie far higher, and the spacing between the ground state and the first excited state will be much greater. 27