Mineralogical Analyses of Surface Sediments in the Antarctic Dry Valleys: Coordinated Analyses of Raman Spectra, Reflectance Spectra and Elemental Abundances Janice L. Bishop1,2, Peter A. J. Englert3, Shital Patel1,3, Daniela Tirsch5, Alex J. Roy6, Christian Koeberl7, Ute Böttger5, Franziska Hanke5,8, and Ralf Jaumann5. 1 Carl Sagan Center, SETI Institute, 189 Bernardo Avenue, Mountain View, CA, USA (jbishop@seti.org). 2 NASA Ames Research Center, Moffett Field, CA, USA. 3 University of Hawaii at Mānoa, HI, USA. 4 San Jose State University, San Jose, CA, USA. 5 German Aerospace Center (DLR), Berlin, Germany. 6 Department of Land and Natural Resources, Honolulu, HI, USA. 7 Department of Lithospheric Research, University of Vienna, Vienna, Althanstrasse 14, 1090 Austria, and Natural History Museum, Burgring 7, 1010 Vienna, Austria. 8 Technische Universität Berlin, Berlin, Germany. Keywords: Antarctic Dry Valleys, sediments, Raman spectra, reflectance spectra, chemistry Submitted June 2014 to Philosophical Transactions A, Special Issue “Raman spectroscopy meets extremophiles on Earth and Mars – studies for successful search of life” Revised August 2014 Short title: Antarctic Dry Valleys Sediments Electronic Supplementary Material Digital Raman spectra and images of the sediment grains are provided for the data shown in Figures 4, 6 and 8. The Raman spectra are grouped by lake and the spectrum numbers in the digital file are the same as those used in the figures. Figure S1 (filename = Bishop et al LFR-1 sediment grains) This view of several grains from sediment 1 from Lake Fryxell (sample JB 651) illustrates the variety of grain shapes, sizes and colors. The yellow dishes are ~0.5 cm in diameter. All spectra shown were collected on grains from position 1 (yellow dish marked by 1). Figure S2 (filename = Bishop et al LVA-9 sediment grains) This view of several grains from sediment 9 from Lake Vanda (sample JB 669) illustrates the variety of grain shapes, sizes and colors. The yellow dishes are ~0.5 cm in diameter. Spectra 1 and 2 were collected on grains in position 10, while spectra 3 and 4 were collected on dark grains in position 3. Figure S3 (filename = Bishop et al LBR-2 sediment grains) This view of several grains from sediment 2 from Lake Brownworth (sample JB 671) illustrates the variety of grain shapes, sizes and colors. The yellow dishes are ~0.5 cm in diameter. Spectra 1 and 2 were collected on different locations of the same particle in position 2, while spectrum 3 was collected on a dark grain in position 3, and spectrum 4 was collected on a light grain at position 11.