Particle and Particle Systems Characterization – To appear August 99 Droplet Sizing by Mie Scattering Interferometry in S.I engine. Christine Mounaïm-Rousselle, Olivier Pajot Ass. Prof. Christine Mounaïm-Rousselle and PhD Stud. Olivier Pajot Laboratoire de Mécanique et d’Energétique Université d’Orléans 45072 Orléans cédex 2 (France) Particle and Particle Systems Characterization – To appear August 99 Abstract In this paper, we explain theoretically a technique based on Mie scattering interferometry (M.S.I.), obtained by a defocusing of the collecting optics, to size droplets. The originality of this study is the development of a droplet sizing method by planar laser light scattering for the case of a scattering angle range close to 90°. The feasibility of this method and its limitations are fully described. The dependence on intensity levels and refractive index variations can be neglected. After discussion of some practical details about particle size, imaging and camera constraints, the results obtained in the combustion chamber of a Spark Ignition engine, near the spark plug, prior to ignition and for different injection timings are described and discussed. It can be concluded that the implementation of the M.S.I. method in our experimental setup has been realised successfully to provide droplet distributions in an S.I. engine. To enable easier use of the technique, image processing software is going to be developed in the Matlab environment. Particle and Particle Systems Characterization – To appear August 99 1. Introduction To reduce fuel consumption and pollutants emissions in Spark Ignition engine, one working mode can be the lean burn one. Unfortunately, this mode is prone to misfires. To reduce this problem, the air-fuel mixture must be correctly prepared around the spark plug. For a better understanding of mixture preparation effects, experimental data are needed. One way is to determine the influence of the presence of fuel droplets inside the combustion chamber before the ignition. Indeed, it has been shown by Ballal and Lefebvre [1], and, Singh and Polymeropoulos [2], that the ignition of vapour fuel is affected by the presence of fuel droplets. They have studied the ignition phenomena for different droplet diameters and different liquid/vapor fuel ratios. Moreover, spark ignition affects strongly the initiation of the flame kernel, its propagation and finally formation of pollutants. Therefore the knowledge of the droplet life time near the spark plug and prior to ignition in engines is relevant. As in most experimental devices, the use of optical diagnostics is limited by optical accesses. The final purpose is to estimate fuel droplets diameter distribution in a “transparent” Internal Combustion engine, where the light scattering angle is orthogonal. This collection angle is commonly used and available in the majority of experimental set-ups, designed for planar imaging techniques. To record experimental data in engine environments is relatively difficult and one needs to choose the most appropriate technique. The advantage of optical diagnostics is evident due to their non-intrusivity and because they can provide the spatial evolution of droplet diameter distributions. In S.I. engines, information on the spatial distribution of droplets near the spark plug is sparse. Droplet sizing techniques can be divided in two classes : Local measurement techniques, provide temporal local histories of particle size for particles passing trough a spatial measurement volume, but spatial distribution can only be obtained by mapping out the whole flow field. For example, Kadota et al. [3] have Particle and Particle Systems Characterization – To appear August 99 successfully shown the feasibility of local fuel droplet diameter measurements in engine by using laser Mie scattering. One HeNe laser beam was focused inside the chamber and the scattered light due to the interaction between the ray and the droplet was collected via a photomultiplier placed at 90°. The limitation was related to the quantitative sizing of droplets : a calibration was required or a complex Mie theory simulation. The best developed diagnostics is the Phase Doppler Anemometer. Vannobel et al. [4] and Posylkin et al. [5] have done preliminary studies on optical engines with PDA. It seems to be attractive due to simultaneous droplet size and velocity measurements. Unfortunately, this technique needs a collection optics located in the scattering plane at scattering angles from 25 to 75 degrees and provides temporal data but spatial data have to be mapped out with multiple measurements. Another technique to size droplets developed by Massoli et al. [6] is based on the polarization properties of light. The quality of the light detectors is important because it needs to compare measured polarized intensities ratios with those computed by Mie theory simulation. Two dimensional planar configurations provide instantaneous spatial resolution. Nowadays, due to the extensive development of CCD cameras, image grabbers and processing systems, these techniques have become very attractive. Peters [7] has estimated droplets size distribution during intake and compression strokes with a basic imaging technique based on Mie light scattering. The difficulties were that to estimate droplet diameter, it was necessary to assume a predetermined droplet density and size range. Moreover, the analysis was not easy due to out-of-focus droplets. Hofeldt et al. [8] have followed the same idea and developed successfully their imaging configuration, providing spatially resolved measurements of particle size for hundreds of droplets in essentially real time ; but with the same difficulties discussed above : necessity to calculate particle scattering intensities with Lorenz-Mie theory, and to perform accurate intensity measurements with intensified CCD cameras. Recently, Skippon et al. [9] have applied another imaging technique in an optical accesses engine : Particle and Particle Systems Characterization – To appear August 99 interferometry based on Mie scattering. Glover et al. [10] initiated this method based on the interference between light reflected from and refracted through individual droplets in the wide-angle forward-scatter region. The advantage is the independence on the absolute scattering intensities : out-of-focus images of laser scattering droplets from the 45° direction consist of a set of lighted spots with fringes. They showed that due to geometrical analysis, the diameter can be easily determined from the number of fringes. They first applied this technique in sparse calibrated sprays and showed a good agreement between their results and those measured with a Malvern sizer. To perform droplet sizing and distribution data in an S.I. engine, Mie Scattering Interferometry (M.S.I.) has been selected in this study, but in our configuration a unique scattering collection angle of 90° was chosen. In this case, not only the scattered intensity is very low but the geometrical analysis must be performed carefully. Ragucci et al. [11] have tested the Mie Scattering Interferometry method in this particular case, but their analysis has been done with only one drop although their conclusion was very promising, indicating the possibility to develop the planar configuration. The emphasis of this paper is on the development of this diagnostic technique. Firstly we will remind its theoretical basis to express clearly the relation between number of fringes and droplet diameter by using a geometrical hypothesis. The experimental setup will be described and advice about experimental constraints will be given. The final section presents and discusses results of preliminary experiments performed near the spark plug in an engine working under different conditions during the compression stroke, prior to ignition. 2. Theoretical bases of the M.S.I. In this part, the basic phenomena and hypothesis will be clearly described in order to get the simple relation between the number of fringes and the droplet diameter. Particle and Particle Systems Characterization – To appear August 99 One of the most important results of Lorenz-Mie theory is that the light scattered by a spherical particle is inhomogeneously distributed in space, depending on droplet diameter, refractive index and incident light characteristics. By using the Generalised Lorenz-Mie theory as in Gouesbet et al. [12], it can be shown that the scattered light intensity is an oscillating function of the angle in the range of 0<. These oscillations, due to interference between diffracted, refracted and reflected rays emanating from the particles, are the bases of the Mie Scattering Interferometry. Van de Hulst [13] has demonstrated that for large size parameter x where x = d/, with d, the droplet diameter and the incident light wavelength, the scattering of light by a spherical particle illuminated by planar wave fronts can be described by geometrical optics rules, simpler than the complex Mie theory. In our case droplet diameters lie within the range from a few micrometers up to 100 µm. So for a 532 nm wavelength, x ranges from 5.9 up to 590. Ungut et al. [14] have shown that this approximation is valid for droplets as small as 1 µm for forward scattering angle (0-20°). In Fig.1, we compare the scattered light in the plane perpendicular to the incident polarisation, estimated by Mie theory and geometrical analysis for two droplet diameters : 50 µm and 10 µm, with a real refraction index of 1.39 (iso-octane droplet). One can see that a very good agreement occurs when the scattering angle range is 30°<<70°. Figure 1…. Therefore it is possible to use a geometrical analysis to apply M.S.I.. However, if we make a similar comparison for a scattering angle range centred around 90° as in Fig.2, one can note that the intensity value and shape are not in good agreement. But, the number of oscillations, for instance for an angle range of 10° are nearly similar. The geometrical analysis can be inappropriate therefore in our application but it does provide a simple relation to estimate droplet size. Particle and Particle Systems Characterization – To appear August 99 Figure 2…. 2.1 Geometrical analysis All droplets are considered perfectly spherical and homogeneous. The interaction between a light ray (i.e. here a laser beam) and a droplet is shown schematically in Fig. 3. The total scattering light intensity is due to the sum of reflection and successive refractions. For the interferometric Mie scattering method, only the reflection and first refraction rays are considered. The reflection ray is not attenuated by absorption but the first refracted one is : the difference of both optical paths, which form dark and bright fringes, is a function of the droplet diameter. The advantage is that this sizing method is totally independent of the intensity of the illuminating light source. The droplet itself acts as an interferometer. Figure 3… o and 1 are the incidence angles of reflected and refracted beams respectively and ’1 the refraction angle. By the Snell’s law, the relation between ’1 and 1 can be expressed as below, with m the real part of the refractive index: cos 1 1 cos 1 m (1) The scattering angle from the incident ray is, for pure reflection, o=2o and for one refraction, 1=2( 1 -1). There exist only two rays for which these scattering angles are the same. Table [1] shows that for a scattering angle of 90° and for droplets with a range of refractive indices m, the value of 1 is very low. So only very few rays can be reflected once and leave the droplet with a 90° scattering angle. Table 1… The phase difference between both rays can be easily expressed via the phase term determined by simple geometry (Mounaïm-Rousselle and Pajot [15], Golombok et al.(16]) Particle and Particle Systems Characterization – To appear August 99 2d 2d sin 0 (sin 1 m sin 1' ) 2d (sin m 2 1 2m cos ) 2 2 0 1 (2) As Ungut et al.[14] have shown, the phase difference is taken account in total scattered light intensity expression via a cosine. Therefore, an infinitesimal variation of the scattering angle induces a maximum or minimum light intensity variation and occurs when an infinitesimal phase difference is equal to 2. These considerations allow one to write : m sin d (0 1 ) (cos 2 2 m 2 1 2m cos 2 ) 2 (3) So as Van de Hulst [14] and Roth et al. [17] indicated, the angular inter-fringe spacing is linked to the droplet diameter by : 2 d 1 cos 2 m sin 2 m 2 1 2m cos (4) 2 Glover et al. [10] have used a simplified formula (Eq. 5), based on the assumption that the angle of incidence of the refracted ray on the droplet is close to zero. In fact, it is not appropriate for a scattering angle of 45° (in their application) but can be used for a scattering angle of 90°, as shown Golombok et al. [16]. 2 1 d 1 1 m (5) 2.2 Comparison between Mie theory and geometrical analysis In Fig. 4, the angular inter-fringe spacing, obtained by Mie theory, general geometrical analysis (via Eq.4) and the approximation (via Eq.5) is plotted versus (iso-octane) droplet diameter, for a 90° scattering angle. Particle and Particle Systems Characterization – To appear August 99 Figure 4 … The trends are globally the same but an overestimate of approximately 14% appears with the geometrical analysis, for droplets smaller than 10 µm. In fact, we will see below that experimentally, by counting integer numbers of fringes, the droplet size is not an absolute value but is classified with a size class as probability function. 2.3 Influence of refractive index variations. As all techniques based on Mie scattering, the refraction index changes play an important role on droplet sizing. From Eq.5, it is possible to estimate this effect. As it can be seen below in Fig.5, for iso-octane droplets the refraction index ranges between1.3 and 1.5, due to the temperature field, we can evaluate that this 6% variation around the standard value of 1.39 only induces an angular inter-fringe frequency variation of 0.07 % ! It is clear that one of the advantages of this technique is that the refractive index variation does not sharply affect droplet sizing. Figure 5… 3. Experimental considerations The Planar Mie Scattering Interferometry set-up is simple as can be seen in Fig. 6 : a laser sheet illuminates the droplets and a light collection lens images the droplets onto a CCD or photographic camera. However, to visualise the fringes inside the droplet the camera needs to be positioned out of the focal plane. At the focal plane, the fringes are superimposed and droplet images uniformly lighted are obtained. For a scattering plane at 90°, the main drawback is the low scattered intensity; however with modern CCD cameras, intensifiers are not necessary. Figure 6…. Particle and Particle Systems Characterization – To appear August 99 One important experimental parameter is the collection angle : it must allow to get a number of fringes sufficiently high to distinguish them. is equal to the number of fringes N multiplied by the angular fringe spacing . This angle can be also approximated as function of the magnification ratio G, defined as the ratio between the image size and the object size, and the numerical aperture N.A. : 2 arcsin( G 1 . ) G 1 2 N.A. (6) Finally, from Eq.5 and Eq.6, the droplet diameter can be expressed as : d N 1 G 1 1 arcsin( . ) 1 G 1 2 N.A. m (7) 3.1 Influence of the collection angle The importance of the collection angle is shown in Fig. 7 where the number of fringes in the image is plotted against the droplet diameter for different collection angles. It is evident that for a given diameter, the number of fringes inside the droplet image increases with increasing value of this angle. Therefore, for example a collecting angle of 20° allows a good estimate of droplet diameters range of 5-20 µm, which generates a number of fringes from 3 to 11. A bad knowledge of the collecting angle can add also other errors. Figure 7…. In general experimental geometric constraints may limit the collection angle. So there is a compromise between the possible choice of this angle, linked to the magnification ratio and the lens-object distance, and the more appropriate angle to determine a given droplet diameter range. On the other hand, in most applications, as in engine environment, it is easier to use a CCD camera than photographic one, to follow cycle-by-cycle a phenomena but the current CCD size is not more than 100 mm2. This implies that the image area will be sharply restricted, involving a low magnification ratio. So the useful parameter becomes the number Particle and Particle Systems Characterization – To appear August 99 of aperture : in conclusion, with CCD camera, a good collecting system is an objective which enables a large aperture with a large lens diameter. 3.2 Imaging constraints The droplet image with out-of focus technique is a disk with fringes superimposed. The centre of the disk corresponds to the droplet position in the planar laser sheet. So, with M.S.I. images as in Fig. 8, it is possible to measure simultaneously the droplet spatial distribution and droplet size. Figure 8… We have underlined that to image fringes on the CCD pixels, the camera must be defocused. In fact, this defocusing distance must not be too large in order to allow a sufficient visualisation area. It is evident also that the measurable maximum droplet size is limited by the minimum distinguishable angular inter-fringe spacing. This problem can be seen in Fig. 8 : the biggest droplet, i.e. the brightest image, can not be sized due to the too large number of fringes. So the fringes contrast does not allow an easy count. On the other hand, droplets with one fringe are also difficult to evaluate : it is not possible to know if there is only one fringe or if the droplet is not totally in the laser sheet. As it can also be seen on this image, two interference images can overlap, due to droplets very near to each other and after defocusing they overlap. It is clear that in the case of a fixed out-of focus distance, dense sprays can not be sized. The unique solution would be to increase the magnification but then the image area becomes smaller generating less droplet images. An example of M.S.I. image, taken in an alcohol dense spray (Bissonnier [18]), but with a Nikkon F4S camera, is shown in Fig.9. In this case, the magnification ratio is unity, so the image area is 24 x 36 mm. The focal length is 136 mm with a out-of-focus of 5 mm, so the defocus distance is around 4 %. When the film plane is normal to the lens axis, the size of the droplet image varies with position across the film, so with the defocus distance. When the Particle and Particle Systems Characterization – To appear August 99 Scheimpflug condition is satisfied, the size of individual out-of-focus images from different droplets is the same. Experimentally, it is verified only when the defocusing is sufficiently at least of 4% of the focal length. This characteristic becomes very relevant to develop an automatic image analysis software. Figure 9… We have shown theoretically that the maximum drop size is determined by the angular inter-fringe spacing but experimentally, also by the imaging area, the magnification ratio and the objective lens characteristics. We have previously verified the accuracy obtained by this technique with a 90° scattering angle in sparse sprays of water (Mounaïm-Rousselle and Pajot [15]). For example, a spray of droplets of mean classical Sauter diameter of 10 µm, measured by a Malvern sizer was used. To get the size distribution by M.S.I., 100 images have been taken, and 500 droplets were counted. The mean Sauter diameter estimated by MSI was 12.91 µm at a scattering angle of 45° and 12.97 µm at 90°. Agreement between the two techniques was reasonable, mainly due to the non evaluation of small droplets (below than 4 µm for the experimental set-up used in this case) with the M.S.I., and also due to the inherent differences in spatial and temporal sampling. Moreover, the results obtained with both scattering angles are very close. 4 Experimental set-up Optical engine. A schematic of the engine and optical system is shown in Fig.10. This optical accessed spark-ignition engine is derived from a standard 4 cylinder-2 litre engine. A single cylinder head is mounted on top of an elongated crankcase. This raised cylinder houses a piston with a transparent quartz crown, allowing optical access to the 4 valve pentroof combustion chamber. Two quartz windows enable access through the cylinder head. Figure 10… Particle and Particle Systems Characterization – To appear August 99 An optical shaft encoder with 3600 pulses per revolution provides the crank angle position to a timer card, which generates pulses for injection, ignition, laser triggering and video capture. The engine was driven at 2000 revolutions per minute by an electrical motor. Iso-octane was the fuel. The mean admission pressure is fixed at 500 mbar and the injection duration at 5 ms. The global equivalence ratio of air/fuel mixture was maintained, for all cases, at stoichiometric level. Three modes of injection were studied : mode 1 corresponding to an injection at the beginning of the intake valves opening ; mode 2, just after the intake valves closing and ; mode 3, at the middle of the intake valves opening. Planar Mie Scattering Interferometry set-up. To implement this technique, a frequency doubled YAG laser beam (532 nm, 200 mJ) passes through a set of cylindrical and spherical lenses to form a sheet with a minimum thickness of 0.5 mm (the sheet thickness must be larger than maximum droplet diameter). This 40 mm width vertical sheet enters in the combustion chamber via the transparent piston head as it can be seen on Fig.10. The location for visualisation of droplets location inside the combustion chamber is just below the spark plug. A laser pulse was triggered once per engine cycle, the light scattered by the fuel droplets was collected at 90° and imaged into a KPM2 Hitachi CCD camera. The CCD resolution is 768 by 568 pixels and its size 6.47mm by 4.83 mm. However, due to the asynchronous trigger, only 768 by 284 pixels were used. The camera was aligned to have the maximum pixel number in the direction of the fringes. The resolution seems to be too low as discussed by Glover et al. [10]. They used a photographic film to get a better resolution. But high resolution is not essential to provide quantitative results which depend on the diameter resolution and the diameter range required : the camera objective is also one of the most important component to select the appropriate droplet diameter range. In our case, several camera objectives have been tested to optimise the collection angle. The best choice in our configuration was the Nikkor AF80-200f/2.8 ; it allows large aperture collection with its non standard lens diameter of 77 mm. For this study, the visualisation area in the focal plane is 10 Particle and Particle Systems Characterization – To appear August 99 x 13 mm which gives a magnification ratio of 1:2 and the distance between the laser sheet and the objective lens is 150 mm at 80 mm macro position. To achieve an approximate sufficient number of distinguishable fringes, the out-of-focus distance used was 11 mm, corresponding to 7% of the objective-object distance. In this case, the size of the area visualised becomes 9 x 12 mm. With this set-up, a droplet with a diameter of 3.5 µm gives one fringe image. For this study, we were particularly interested on a droplet diameter range between 10 µm to 50 µm. 5 Results and discussion Firstly we studied the injection mode, i.e. the injection is made at the beginning of the intake valve opening, to analyse the presence of droplets and their diameter distribution. Some of the images do not allow fringe detection due to too small droplet size and also droplets out of the field of view. So some images were not considered; on average, about 75 images from 100 images taken were validated. The images in Fig.11 have been taken at different crank angles relative of the ignition timing (which is 45° before T.D.C.) but not during the same cycle. It is not easy to draw a conclusion concerning the droplet field. It can be noted first that 15° before start of ignition droplets are more at the top of the image, i.e. nearer the spark plug location. Indeed, during this compression stroke, droplets are pushed to the cylinder head, by the piston itself. We can see, also that 5° after the ignition, droplets are still present in this area Figure 11… . To analyse the droplet diameter is difficult, as it can be seen on Fig. 12 where droplet diameter distributions are plotted. It seems that just after the start of ignition, droplets still exist, certainly also due to the piston rise. It can be concluded that larger number of droplets occurs far from ignition due to piston rise and also to the liquid deposits on the piston head. During the rise, with pressure and temperature effects, these droplets due to the deposit vaporise and fewer droplets are found just prior to ignition. After ignition, certainly droplets at Particle and Particle Systems Characterization – To appear August 99 spark plug location have been pushed away by the flame kernel and they appear on the image area. The mean Sauter diameter is about 20 µm in this imaging area and for this injection case. Figure 12 … To emphasise the feasibility of the Planar Mie Scattering Interferometry technique for engine applications, we have visualised droplets for the two other injection modes, 5° prior to ignition. Mode 2 corresponds to an injection when the valves are closed at the beginning of the compression stroke so the liquid droplets stay in the intake pipe for 540° crankrotation. In mode 3, the injection is done 120° after the beginning of intake valves opening. The droplets size distribution for the modes 1 and 3 are plotted on Fig.13. In fact, in mode 2, usually called closed valve injection mode, only two images contain one discernible droplet. This result can be explained by the vaporisation process occurring in the intake pipe itself. Figure 13… For mode 3, the average number of droplets per image is higher than for mode 1 : 2.26 and 1.72 respectively and also the mean Sauter diameter, 23 µm. In fact, for mode 1, the intake flow velocity is lower at the beginning of the intake. Then it can be expected that deposits on the intake wall are more important, introducing less droplets in the combustion chamber. Moreover, the injection is done during the back flow of exhaust gases, where an increase of temperature may induce earlier droplet vaporisation. 6 Conclusion and perspectives The Planar Mie Scattering Interferometry has been applied in an engine environment where optical access is limited but allowing a collecting plane perpendicular to the laser sheet. The theoretical bases of this technique were clearly exposed to illustrate fundamental concepts and assumptions. The experimental arrangement for P.M.S.I. was described and the technical Particle and Particle Systems Characterization – To appear August 99 problems for implementing it was discussed in detail. This technique was used successfully to investigate the distribution of iso-octane droplets as function of engine crank angle during the compression stroke around the spark ignition and just below the spark plug. Three injection modes were also studied to achieve an idea of the droplets life in this area. These results will be used to study the earliest flame kernel in Spark Ignition engine. It can be concluded from this work that the Planar Mie Scattering Interferometry technique is an easy and simple optical diagnostic. It can provide good resolved spatial information about droplet location and size. The simple geometrical analysis is sufficient to establish the relation between optical characteristics of the collecting system, number of fringes detected and droplet diameter. Compromise must be found in terms of droplets size range, maximum distinguishable number of fringes, image area and also the required diameter precision. To avoid the manual fringe count, we are developing an automated image processing software in Matlab environment. Finally, it would be interesting to develop this technique in parallel with Particles Imaging Velocimetry to perform simultaneously, planar measurements of droplet distribution, size and velocity. Acknowledgements The authors wish to thank G. Grehan, CORIA Rouen, for his theoretical help and C. Preterre, Renault S.A., for providing access to a transparent engine during this work. Particle and Particle Systems Characterization – To appear August 99 References [1] Ballal D.R., Lefebvre A.H. : A General Model of Spark Ignition for Gaseous and Liquid Fuel-Air Mixtures, Eighteen Symposium (International) on Combustion, (1981), pp. 17371776. [2] Singh A.K., Polymeropoulos C.E. : Spark Ignition of Aerosols, Twenty-first Symposium (International) on Combustion, (1987), pp. 513-519. [3] Kadota T., Mizutani S., Wu C.Y., Hoshino M. : Fuel Droplet Size Measurements in the Combustion Chamber of a Motored SI Engine via Laser Mie Scattering , (1990), SAE paper 900477. [4] Vannobel F., Dementhon J.B., Robard D. : Phase Doppler Anemometry Measurements on a Gasoline Spray Inside the Inlet Port and Downstream of the Induction Valve ; Steady and Unsteady Conditions, Applications of Laser Techniques in Fluid Mechanics, Edited by Adrian R J, Durao D F G, Durst F, Heitor M, Maeda M and Whitelaw J H,6, 507, (1993), Springer Verlag. [5] Posylkin M., Taylor K.P., Vannobel F. and Whitelaw J.H. : Fuel Droplets Inside a Firing Spark-Ignition Engine, (1994), SAE paper 941989. [6] Massoli P., Beretta F., and D’Alessio A. : Single droplet size, velocity , and optical characteristics by the polarisation properties of scattered light. Applied Optics, vol 28, (1989), p1200-1205 [7] Peters B.D. : Fuel Droplets Inside the Cylinder of a Spark Ignition Engine with Axial Stratification, (1982), SAE paper 820132. [8] Hofeldt D.L. and Hanson R.K. : Instantaneous imaging of particle size and spatial distribution in two phase flows, Applied Optics, Vol 30 n°33, (1991), pp 4936 – 4948. Particle and Particle Systems Characterization – To appear August 99 [9] Skippon S.M. and Tagaki Y. : ILIDS measurements of the evaporation of fuel droplets during the intake and compression strokes in a firing lean burn engine, (1996), SAE paper 960830. [10] Glover A.R., Skippon S.M. and Doyle R.D. : Interferometric Laser Imaging for Droplet Sizing : A Method for Droplet-Size Measurement in a Firing Lean Burn Engine, Applied Optics, vol.34 n°36, (1995), pp. 8409-8421. [11] Ragucci R., Cavaliere A. and Massoli P. : Drop Sizing by Laser Light Scattering Exploiting Intensity Angular Oscillation in the Mie Regime, Part. Part. Syst. Charact. 7, (1990), pp. 221-225. [12] Gouesbet G., Gréhan G. and Maheu B. : Generalized Lorenz-Mie theory and applications to optical sizing, (1991), N. Chigier (ed.) Hemisphere. [13] Van de Hulst H.C. : Light Scattering by Small Particles, (1957), Willey, New York. [14] Ungut A., Grehan G. and Gouesbet G. : Comparisons Between Geometrical Optics and Lorenz-Mie Theory, Applied Optics, Vol. 20 n°17, (1981), pp. 2911-2918. [15] Mounaïm-Rousselle C. and Pajot O. : Droplet Sizing by Interferometric Mie Scattering in Engine Environment, Optical Technology in Fluid, Thermal and Combustion III, ed.SPIE, vol. 3172, (1997), pp. 700-707. [16] Golombok M., Morin V. and Mounaïm-Rousselle C. : Droplet diameter and the interference fringes between reflected and refracted light., J. Phys. D: Applied Physics, vol 31, n°18, (1998), pL59-pL62. [17] Roth N., Anders K. and Frohn A. : Refractive-Index Measurements for Correction of Particle Sizing Methods, Applied optics, Vol 30 n°33, (1991), pp. 4960-4965. [18] Bissonnier A. : Etude expérimentale du TétraChloroBenzene-Applications à l’incinération, PhD Thesis, University of Orléans, Nov. 1998. Particle and Particle Systems Characterization – To appear August 99 Symbols and Abbreviations x : size parameter d : droplet diameter m : real part of the refractive index G : magnification ratio M.S.I. : Mie Scattering Interferometry N : number of fringes N.A. : numerical aperture P.M.S.I : Planar Mie Scattering Interferometry T.D.C. : Top Dead Center incident light wavelength scattering angle : incidence angle ’: refraction angle angular inter-fringe spacing : phase term collection angle subscript 0 : relative to reflected ray 1 : relative to refracted ray Particle and Particle Systems Characterization – To appear August 99 Legends of Illustrations Figure 1. Comparison of the scattered intensity, Ip, in the plane perpendicular to the incident polarisation, estimated by Mie theory and geometrical approximations for droplet diameters of 50 µm and 10 µm (real refractive index of 1.33). Figure 2. Comparison of Ip estimated by Mie theory and geometrical approximations around a scattering angle = 90°, for a droplet of 50 µm (real refractive index of 1.33). Figure 3. Light ray patterns through a droplet. Figure 4. Angular inter-fringe spacing obtained via Mie and geometrical analysis, at 90° scattering angle versus droplet diameter. (m = 1.39, = 532 nm). Figure 5. Effect of the refractive index on the angular inter-fringes spacing for two droplet diameters : 20µm and 60 µm. (m = 1.39, = 90°, = 532 nm). Figure 6. The Planar Mie Scattering Interferometry experimental set-up. Figure 7. Effect of the collecting angle on droplet diameter. (m = 1.39, = 90°, = 532 nm). Figure 8. Defocussed CCD image for a sparse droplet distribution. Figure 9. P.M.S.I. image obtained in dense spray with photographic camera. (Courtesy of Buissonnier [18]). Figure 10. Schematic view of the experimental set-up around the optical accesses engine. Figure 11. Instantaneous P.M.S.I. images at different crank angles for injection mode 1. Figure 12. Droplets diameter distribution for injection mode 1 at different crank angles Figure 13. Droplets diameter distribution for three injection modes, 15° prior ignition. Particle and Particle Systems Characterization – To appear August 99 Tables m 1 (°) ’1 (°) Real refractive index Incidence angle Refraction angle 1,2 2,53 33,64 1,3 2,16 39,76 1,33 2,07 41,29 1,39 1,94 44,03 1,45 1,83 46,42 1,5 1,76 48,21 Table 1. Refracted incidence and refraction angles values for different refractive index with a scattering angle of 90°. Particle and Particle Systems Characterization – To appear August 99 1000000 Mie theory, d = 10 µm Geometrical analysis Mie theory, d = 50 µm Geometrical analysis Scattering light intensity (a.u.) d = 50 µm 100000 10000 1000 100 d = 10 µm 10 1 30 35 40 45 50 55 Scattering angle (°) Figure 1 60 65 70 Particle and Particle Systems Characterization – To appear August 99 Scattered light intensity (a.u.) 1,E+04 1,E+03 1,E+02 Mie theory 1,E+01 Geometrical analysis 1,E+00 80 82 84 86 88 90 92 Scattering angle (°) Figure 2 94 96 98 100 Particle and Particle Systems Characterization – To appear August 99 ’ ’ Spherical droplet on racti f al re Figure 3 n inter n lectio al ref n Exter Incident wave One Particle and Particle Systems Characterization – To appear August 99 Angular inter-fringe spacing (°) 4 3,5 Mie theory 3 Simplified geometrical analysis 2,5 Geometrical analysis 2 1,5 1 0,5 0 5 10 15 20 25 30 35 40 45 50 55 60 65 70 75 80 85 90 95 100 105 Droplet diameter (µm) Figure 4 Particle and Particle Systems Characterization – To appear August 99 Angular inter-fringes spacing (°) 1,9 1,6 d = 60 µm d = 20 µm 1,3 1 0,7 0,4 1,15 1,25 1,35 Mean refractive index m Figure 5 1,45 1,55 Particle and Particle Systems Characterization – To appear August 99 Figure 6 Particle and Particle Systems Characterization – To appear August 99 Influence of the collecting angle Number of fringes 24 alpha = 5° alpha = 10° alpha = 15° alpha = 20° 20 16 12 8 4 0 0 10 20 30 40 50 Droplet diameter (µm) Figure 7 60 70 80 Particle and Particle Systems Characterization – To appear August 99 Figure 8 Particle and Particle System Characterisation – To appear August 99 90 75° before S.I. Ds = 18 µm 55° before S.I., Ds = 19 µm 35° before S.I., Ds = 21 µm 15° before S.I., Ds = 20 µm 5° before S.I., Ds = 20 µm 5° after S.I., Ds = 23 µm 80 Number of droplets 70 60 50 40 30 20 10 0 7 11 14 18 21 25 28 32 Droplet diameter class (µm) 35 Particle and Particle System Characterisation – To appear August 99 Figure 12 Particle and Particle System Characterisation – To appear August 99 Mean number of droplets 0,31 Mode 1 Mode 3 0,21 0,10 0,00 7,00 10,51 14,01 17,51 21,01 24,52 28,02 31,52 35,02 38,52 Droplet diameter (µm) Particle and Particle System Characterisation – To appear August 99 Figure 13