Energy Efficient Thermally Induced Switching by Tailoring the Electron and Phonon Dynamics T. Ostler1, U. Atxitia2,3, O. Chubykalo-Fesenko4 and R.W. Chantrell1 1 - Dept. of Physics, The University of York, York, United Kingdom. 2 - Fachbereich Physik, Universität Konstanz, D-78457 Konstanz, Germany 3 - Zukunftskolleg, Universität Konstanz, D-78457 Konstanz, Germany 4 - Instituto de Ciencia de Materiales de Madrid, CSIC, Cantoblanco, 28049 Madrid, Spain Tuesday 31st March 2015 Background: Thermally Induced Magnetization Switching • Single linearly polarised femtosecond laser pulse. • Linearly polarised = no induced magnetism from E-field (inverse Faraday effect). Material: Amorphous Ferrimagnetic GdFeCo Ostler et al., Nature Comms, 3, 666 (2012). • (left) Time and element resolved dynamics (XMCD). • Switching complete after <2ps. Radu et al., Nature, 472, 205-208 (2011). Tuesday 31st March 2015 2/11 Challenges Size Confinement Ostler et al., Nature Comms, 3, 666 (2012). Heat dissipation Magnetic storage Thermally Induced Switching Application s Materials Mechanism Azim et al., IEEE Electron Device Letters, 35, Issue 12, 13171319 (2014). AFM Exchange Tuesday 31st March 2015 Composition Optical arxiv: 1409.1280 Energy transfer to magnetic interconnects system 3/11 Controlling energy transfer to the spin system Kaganov et al., JETP 1957 Anisimov et al., JETP 1974 Tuesday 31st March 2015 4/11 Range of values of electron-phonon coupling Max and min values 100 • Order of magnitude range in values. • Can be calculated from electronic structure calculations or fitted from reflectivity measurements. Ge− ph [×1017W/ m3K ] Co/Pt Koopmans GdFeCo (simulations) FePt 10 Fe alloys FePt 1 Koopmans 0.1 Ni Co Fe Pt Gd Tb Important consideration when looking for new materials Tuesday 31st March 2015 References Koopmans Nat Mat 9, 259-265 (2010) Mendil Sci Rep 4, 3980 (2014) Verstraete J.Phys: Cond Matt 25, 136001 (2013) Ostler Nat Comm 3, 666 (2012) Radu Nature 472, 205-208 (2011) Radu PRL 91, 22 (2003) Kimling PRB 90, 224408 (2014) Koopmans Nat Mater (2009) Caffrey Thermoscale Thermophys. Eng. 2005 Beaurepaire PRL 1996 Wellershof 1998 Proc. SPIE Bovensiepen J. Phys.: Cond. Mat 19 083201 (2007) 5/11 Magnetic model • Energetics based on the Heisenberg Hamiltonian combined with the stochastic LandauLifshitz-Gilbert equation. Heisenberg parameters fitted to experimental measurements [1]. Damping Precession describes rate of transfer of energy into (below) and out of (above) the system Noise Thermal effects Tuesday 31st March 2015 [1] - Ostler et al. Phys Rev B 84, 024407 (2011) 6/11 Composition Optimisation Barker et al. Nature Scientific Reports, 3, 3262 (2013). Tuesday 31st March 2015 7/11 Mechanism for Switching – requirement for AFM exchange • Data shown 25% (switches) and 35% (does not switch) Gd, both ferrimagnetic. Overlapping bands allows for efficient transfer of energy. Large band gap precludes efficient energy transfer. Barker et al. Nature Scientific Reports, 3, 3262 (2013). Tuesday 31st March 2015 8/11 The role of e-ph coupling on thermal switching Switching favours high peak temperatures and longer pulse durations (more heat to magnetic system) Tuesday 31st March 2015 9/11 Damping and Summary • • Attempts to incorporate the detailed mechanism of energy transfer from subsystems. Extremely difficult to quantify the exact mechanism. Optimisation of composition/thickness of multilayers Low e-p coupling gives more efficient heating effect High thermal bath coupling More efficient switching Tuesday 31st March 2015 10/11 Acknowledgements • Funding from the EU FP7 project FemtoSpin, grant agreement no. 281043. • • Zukunftskolleg Incoming FellowshipProgramme Marie Curie (ZIF-MC). This work made use of the facilities of N8 HPC provided and funded by the N8 consortium and EPSRC (Grant No.EP/K000225/1). The Centre is coordinated by the Universities of Leeds and Manchester. Tuesday 31st March 2015 [1] - Barker et al. Scientific Reports, 3, 3262 (2013). 11/11