See discussions, stats, and author profiles for this publication at: https://www.researchgate.net/publication/353024965 Paper-based Electronics: Passive Components and Low Pass Filters Using Solvent-free Eco-friendly Fabrication Conference Paper · June 2021 DOI: 10.1109/FLEPS51544.2021.9469750 CITATION READS 1 1,992 6 authors, including: Muhammad Hamza Zulfiqar Umer Hassan Information Technology University Information Technology University 34 PUBLICATIONS 180 CITATIONS 3 PUBLICATIONS 15 CITATIONS SEE PROFILE SEE PROFILE Aftab Alam Muhammad Zubair Harbin University of Science and Technology Information Technology University 2 PUBLICATIONS 9 CITATIONS 239 PUBLICATIONS 4,316 CITATIONS SEE PROFILE All content following this page was uploaded by Kashif Riaz on 27 October 2021. The user has requested enhancement of the downloaded file. SEE PROFILE Paper-based Electronics: Passive Components and Low Pass Filters Using Solvent-free Eco-friendly Fabrication Muhammad Hamza Zulfiqar, Umer Hassan, Aftab Alam, Muhammad Zubair, Muhammad Qasim Mehmood, Kashif Riaz* Department of Electrical Engineering, Information Technology University (ITU), Lahore 54600, Pakistan. *kashif.riaz@itu.edu.pk Abstract— We report an eco-friendly and easy-going way of fabricating a vast range of passive electronic components and low pass filters. This is achieved by directly writing graphite on paper and cutting and pasting aluminum foil and copper tape on different substrates. Resistance was achieved from 4 kΩ to MΩ(s) by penciling several sustainable layers of different graphite to clay content pencils. Capacitors of capacitance from 2 pF to 10 μF are fabricated using graphite, aluminum foil, and copper tape as conductive materials on printing A4, baking, and butter paper as substrate and dielectric materials as for parallel plate capacitors. Pencil on paper-based interdigitated capacitors is reported to achieve lower capacitance and higher cut-off frequency values of low pass filters. Resistors and capacitors of different values are fabricated in a plane to design low pass filters with 100 Hz – 2 MHz cut-off frequency range. All the components and circuits are fabricated from foldable, eco-friendly, and readily available paper materials as substrates. These paper-based components are helpful for foldable electronics, foldable printed circuit boards, and soft robotics. Keywords—filter circuits; passive components; eco-friendly; paper electronics; solvent-free fabrication I. INTRODUCTION Electronic systems play a vital role in the daily life of humans. The researcher community takes a reasonable interest in developing cheaper, eco-friendly, and biodegradable electronics in the past few years. In this way, the base of development and production was set by the research community, of less-weight, easy design, and foldable electronics, ease in production and its usage in complex applications, e.g., flexible filters and passive components [1], monitoring devices in biomedical applications [2], flexible sensors [3], wearable electronic circuitry [4], and flexible storage of energy [5]. Flexible electronics is a favourable issue for traditional transportation and conventional large area electronics [6]. Flexible and foldable electronics based on rollable and bendable substrates require a stable conductor with a flexible substrate [7]. Folding makes an edge at the point of the fold, which develops the wrinkles, deformation and this deformation remains even after unfolding. Therefore, flexible substrates and conductors are good options, maintaining contact with each other, even in folded conditions [8]. Paper-based substrate offers many advantages like excessive availability, low cost, portability, lightweight, biodegradability, and eco-friendly [9]. These advantages make the paper an inevitable substrate for a wide range of electronic devices, including transistors [10], solar cells [11], radio frequency identification (RFID) tags [12], microfluidic glucose sensors [13], flexible displays [14], micro-electromechanical systems (MEMS) [15], touch sensors [16], foldable passive components and circuits [1] and energy storage devices [5]. Vast availability and realization of paper substrate-based electronics can activate electronic applications to be reached out to the existing electronics. The fabrication technique is one of the vital factors, especially for the design of flexible electronics. In fabrication techniques, economically cheap and high-performance fabrication techniques are more suitable than costly and high-performance techniques. Recently, many fabrication techniques reported in the literature, such as inkjet printing [17], screen printing [18], bench-top [19], and direct writing [20], have been developed for flexible electronics. In the fabrication of flexible electronics, substrate, conductive, and adhesive (if required) materials are necessary raw components. The fabricated circuits are required to be disposed of after their use. Fabricated components and circuits passed from the recycling stages to recycle the substrate and conductive materials. In this work, broad range resistors and capacitors have been fabricated to obtain the wide cut-off frequency of low pass filter (LPF) circuits. RC filters from pencil-trace on paper were reported at RCS PCCP 2013 [21], passive RC filters on paper were reported at RSC Advances 2016 [22], and pen/pencil-written circuits were reported at Advanced Electronic Materials 2018 [23]. Our work differs from all the above reported in capacitor designs and materials used to ensure the required capacitance, foldability, and circuits' flexibility. The range of resistance, capacitance, and filter circuits is very vast in our work. Different electrode and substrate materials are used to obtain the required characteristics of capacitors and RC filters. II. FABRICATION PROCESS Passive components as resistor and capacitor and passive circuits as low pass filter circuits were fabricated using solvent-free, non-expensive, and non-energy consuming fabrication process as direct writing of pencil-on-paper. Standard A4 photocopier paper was used as a substrate for the resistors, capacitors, filter circuits, and a dielectric material for parallel plate capacitors. Commercially available pencils of different graphite to clay contents as HB (68 ± 2%), 2B (74 ± 2%), 4B (79 ± 2 %), and 8B (90 ± 2 %) purchased from the local bookstore were used to fabricate pencil-on-paper components and circuits. Fig. 1 (a) shows the process of pencil on the paper-based fabrication process. Commercially available Al-foils from a local grocery store were used to fabricate Al-foil on paper-based parallel plate capacitors using solvent-free adhesive. The cut and paste fabrication process for the fabrication of parallel plate capacitors is shown in Fig. 1 (b). III. RESULTS AND DISCUSSION Resistors have been fabricated using four different types of commercial pencils and Fig. 2 shows the relationship between the sheet resistances of resistors and the graphite content used to fabricate the resistors. The evaluation of sheet resistance of resistors fabricated through direct writing of pencil-on-paper was done using a set of devices of different areas for each graphite content. Resistors fabricated from direct writing of pencils with lower graphite-to-clay ratio to higher graphite-to-clay ratio exhibits sheet resistances from higher to lower values, as shown in Fig. 2. Capacitance having a direct effect on the area of parallel plates of a capacitor and dielectric constant. We achieved capacitance according to the requirement by varying the electrode areas of different materials and dielectric materials like simple printer paper, baking paper, butter paper, tissue paper, and Teflon tape. Fig. 3 presents the average capacitance/cm2 of ten different parallel plate capacitors having electrodes of graphite, aluminium, and copper with four different types of papers as printer paper, baking paper, butter paper, and tissue paper substrate, and dielectric materials. Fig. 3. The capacitance of capacitors fabricated from graphite, aluminum, and copper electrodes on four different substrates as a printer, baking, butter, and tissue paper. Fig. 1. Fabrication process. (a) Direct writing of pencil-on-paper-based fabrication process for resistors, capacitors, and filter circuits. (b) Cut and paste fabrication process for deposition of al-foil and copper tape on paper. Capacitance is directly proportionate to the dielectric constant. We fabricated the capacitor on different substrates to achieve a vast capacitance range, with different electrode areas and different electrode materials. In the case of comb and interdigitated capacitors, the capacitance is as follow for single fringe [24][25] C = Ԑ×lo×t / d Fig. 2. The average sheet resistance of 2cm2 resistor patches in Ω's fabricated using pencils with different percentages of graphite content. Capacitors have been fabricated using pencil, aluminum foil and copper tape as electrodes with different paper-based substrates. To achieve additional capacitance ranges from μF to pF, we tested different designs like a comb, sandwich, and in-plane capacitors. For a parallel plate or sandwiched capacitors, the capacitance C depends upon the area A of electrodes, the distance d between the electrodes, and dielectric constant Ԑ, which is the product of relative permittivity Ԑr and absolute permittivity Ԑo as given in the equation (1). C = ԐA/d (1) (2) where lo is the length of fringe, t is the thickness of fingers, d is the distance between fingers, ɛ is the dielectric constant between the fingers of the comb. The capacitance of comb capacitance has been varied by thickness of fingers, the distance between fingers, and length of fingers of the comb capacitor. Resistors have been fabricated by direct writing of pencil on paper. The required resistance of resistors is achieved by fabricating different graphite to clay content pencils for different patch areas. These components are useful for the development of the diversity of circuits. Resistors and capacitors have been fabricated in a plane in series to fabricate the filter circuits as a low pass filter circuit. Fig. 4 shows the fabricated circuit and the circuit diagram of the RC low pass filter circuit. Fig. 4. Foldable resistor-capacitor (RC) circuit. (a) Paper-based RC low pass filter circuit. (b) Circuit diagram of low pass filter. The paper-based low pass filters have been fabricated by pencilling a capacitor and resistor in series as shown in Fig. 4 (a). Fig. 4 (b) shows the circuit diagram of the RC low pass filter circuit. The cut-off frequency Fc of low pass filters depends upon the capacitance C and resistance R, as described in equation 3. Fc = 1 / 2 𝝅 R C from the 600 kHz low pass foldable resistance capacitor circuit. (3) Resistors and capacitors have been designed to achieve a cut-off frequency range from 160 Hz to 2 MHz. For this, we tested capacitors in the range from 5 pF to 10 μF along with resistors in series from 4 kΩ to 1 MΩ. Here we presented a 6 kHz low pass filter. Fig. 4 (a). shows the low pass fabricated circuit. The circuit comprises five pairs of fringes, and a resistor is designed by using 8B pencil on paper. Fig. 6. The measured and calculated output response of a 600 kHz low pass filter circuit. The cross-section lines denote the points of the cut-off at -3dB gain. At these points, the output is 70.7 % of the input. It shows the cut-off frequency as 150 Hz and 600 kHz, respectively. Table I includes the comparison table of RC low pass filter circuits. Fig. 7. Output responses of paper-based RC low pass filter circuits for 150 Hz and 600 kHz cut-off frequency. TABLE I. COMPARISON OF RC FILTER CIRCUITS. Materials Fig. 5. Input and output waveforms of low pass filter circuit at different frequencies. (a) 100 Hz (b) 100 kHz (c) 600 kHz and (d) 1 MHz. The RC filter circuit consists of a comb capacitor and resistor. Fig. 4 (b) shows the circuit diagram of the RC low pass filter. The 2 Vp-p is applied as an input to the RC circuit. Fig. 5 (a, b, c, d) shows the output waveform of fabricated low pass filter at 100 Hz, 100 kHz, 600 kHz, and 1 MHz frequency, respectively. The applied input is shown as a red waveform and output as a yellow waveform. Fig. 6 shows the graph comprised of the output response of the low pass filter for 0 Hz - 10 MHz frequency. The blue line represents the out gain obtained from the foldable resistance capacitor circuit, and the orange line represents the calculated values. The cross-section lines represent the cutoff point at -3dB gain, where the output is 70.7% of the input. It shows the cut-off frequency as 600 kHz. Fig. 7. shows the graph comprised of the output response of 150 Hz and 600 kHz low pass filter for 0 Hz – 10 MHz frequency. Blueline represents the output gain obtained from the 150 Hz, and the orange line represents the gain obtained Cut-off Frequency (fc) Graphite and Ion 9 kHz Gel [1] Graphite [22] 6 kHz Silver, Nickel, 3 kHz & 60 and Graphite Ink kHz [23] Graphite and 9 kHz NaCl Salt [26] Graphite 150 Hz & [This Work] 600 kHz SolventFree Process Cost Biodegradable No Low Partially Yes Very Low Yes Yes Moderate Yes No Low Yes Yes Very Low Yes IV. CONCLUSION In this work, we proposed low-cost, foldable, and ecofriendly passive components and filter circuits. All the fabricated components and filter circuits are paper-based and are foldable. The proposed passive components are used to design a wide range of low pass filter circuits, with a wide range (100 Hz to 2 MHZ) cut-off frequency. 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