Fuel 331 (2023) 125695 Contents lists available at ScienceDirect Fuel journal homepage: www.elsevier.com/locate/fuel Multi-timescale and control-perceptive scheduling approach for flexible operation of power plant-carbon capture system Han Xi a, Mingjuan Zhu a, Kwang Y. Lee b, Xiao Wu a, * a b National Engineering Research Center of Power Generation Control and Safety, School of Energy and Environment, Southeast University, Nanjing 210096, China Department of Electrical and Computer Engineering, Baylor University, One Bear Place #97356, Waco, TX 76798-7356, USA A R T I C L E I N F O A B S T R A C T Keywords: Solvent-based carbon capture Coal-fired power plant Multi-timescale scheduling Control-perceptive scheduling Flexible operation A carbon-capture system is required for coal-fired power plants to meet environmental regulation and provide support for grid penetration of renewable energy sources, when the integrated power plant-carbon capture system must operate in a highly flexible manner to accommodate the need for intermittent renewable power. To this end, this paper proposes a hierarchical scheduling scheme for the operation of integrated power plant-carbon capture system to fully exploit the decarbonization and flexibility of carbon capture technology in multiple timescales. The upper layer of the hierarchy implements a day-ahead stochastic scheduling to provide hourly operating instructions in the next 24 h so that the overall economic performance of the plant can be best ach­ ieved, including fuel consumption, load following and carbon trading. A novel index is then introduced to reflect the power adjustment contribution of carbon capture in the intraday scheduling layer and enhance the load ramping performance of power plant by flexible operation of the post-combustion carbon capture in minute timescale. In the lower layer of the hierarchy, control-perceptive scheduling based on close-loop dynamic model is proposed to coordinate the scheduling and underlying control, making the scheduling feasible for the oper­ ating practice. In addition, a new control system, which uses the reboiler steam flowrate to control the CO2 production rate and solvent circulation flowrate to control reboiler temperature is proposed to achieve superior flexibility support role of carbon capture. The case study shows that the proposed scheduling approach can improve the load tracking performance by 36.7% with satisfactory performance in carbon capture, which verifies the efficacy of the proposed scheduling approach in the power system. The impact of the proposed control system is also investigated, providing a broad insight on the flexible operation of carbon capture technology integrated with the power plant. 1. Introduction The CO2 emission from power sector reached a record high of 14.1 Gt in 2019, accounting for over 41 % of global emissions according to the statistical data published by the International Energy Agency (IEA) [1]. While greatly promoting the development of renewable energy sources (RESs), retrofitting existing fossil fuel-fired power plants (FFPPs) with carbon capture technologies is also a direct solution to alleviate the carbon emissions [2]. The reason is the high share of power generation from fossil fuels due to the continual rising of power demand [3]. This trend is particularly evident in developing economies since most of the coal-fired power plants (CFPPs) were built in recent years and could run for another three to four decades [4]. Solvent-based post-combustion carbon capture (PCC) has been confirmed as the most mature and feasible carbon capture technology for the FFPPs [5]. However, it has a lower energy return ratio consid­ ering the high operating and investment costs [6]. For PCC technology, much effort has been made on developing advanced solvent [7] and modifying process configurations [8]. Utilization of CO2 has also drawn much attention, offering different pathways to convert the captured CO2 into valuable fuels, chemicals, and materials [9]. With the increasing penetration of RESs in the power grid, the CFPPs need to shift its operating mode from undertaking the base load to load following frequently over a wide range to ease the integration of inter­ mittent RESs. Such a functional transformation of CFPP brings both challenges and opportunities for the integrated PCC system. On the one hand, the PCC must adapt to the strong fluctuations in flue gas due to the load variations of the CFPP [10]. On the other hand, if the steam used for solvent regeneration can be properly withdrawn from the steam turbine, * Corresponding author. E-mail address: wux@seu.edu.cn (X. Wu). https://doi.org/10.1016/j.fuel.2022.125695 Received 10 May 2022; Received in revised form 7 August 2022; Accepted 17 August 2022 Available online 26 August 2022 0016-2361/© 2022 Elsevier Ltd. All rights reserved. H. Xi et al. Fuel 331 (2023) 125695 Nomenclature Symbols mCO2 CCFPP CPCC CCO2 Cimb Abbreviations IEA International Energy Agency FFPPs Fossil Fuel-fired Power Plants CFPPs Coal Fired Power Plants RES Renewable energy source PCC Post-combustion Carbon Capture CCUS Carbon capture, Utilization and Storage PV Photovoltaic MEA Monoethanolamine LP Low pressure steam turbine Index L1 L2 L3 t s Day-ahead scheduling Intraday scheduling Control perceptive dynamic scheduling Index of time Index of scenarios Symbols PCFPP Power output of CFPP without integration with PCC, MW PQPCC PCFPP− PCPCC PPV Prate PV PWT Prate WT Pbuy Pcut Pload mcoal mfg mstPCC mscf mpro CO2 PCC αcoal αCO2 αbuy αcut βopex PCC βopex CFPP ηCFPP ηLP ηPV QLHV coal μcut ΔhLP φfg CL Treb TSTC GSTC The power loss due to reboiler steam extraction of PCC, MW Power output of integrated CFPP-PCC system, MW Power consumptions of PCC for solvent circulation and CO2 compression, MW Power output of PV, MW Rated power output of PV, MW Power output of wind turbine, MW Rated power output of wind turbine, MW The purchased power, MW The curtailment of renewable power, MW Power load demands, MW Mass flowrate of pulverized coal, kg/s Mass flowrate of flue gas, kg/s Mass flowrate of reboiler steam, kg/s Mass flowrate of solvent circulation, kg/s Mass flowrate of CO2 production, kg/s Tc ν νr νci νco GT σ J πs γ Np Ns the PCC is able to enhance the flexibility of the upstream CFPP to manage deeper and faster load following [11]. As a result, carbon cap­ ture can become beneficial for accommodating RES in the grid, while the excess power from RESs can also be fully used to reduce the operating cost of carbon capture [12]. The flexible operation of integrated coalfired power plant-post-combustion carbon capture (CFPP-PCC) system thus has great potential in the context of high penetration of RESs. In-depth studies are required to understand the potentials and dif­ ficulties of the CFPP-PCC system, starting from dynamic modeling to the optimal scheduling and real-time control [2]. First principle models [13] and models identified with data-driven approaches [14] were developed to gain knowledge of the interactions between the PCC and CFPP, and followed by the design of conventional [15] and advanced controllers [16], which make the PCC to better adapt to the flue gas variation [17] and run in a power-carbon cooperative manner with the upstream CFPP [18]. Recently, many efforts have also highlighted the value of flexible operation in scheduling the PCC systems under changing power demand and electricity price. Husebye et al. [19] evaluated the flexibility of PCC in a market with cyclical electricity price based on solvent regeneration and storage models, where storage tank levels were optimized to maximize the weekly profit, showing a positive correlation between the optimal storage tank level and electricity price. A better economic Mass flowrate of carbon emission, kg/s Operating cost of CFPP, $ Operating cost of PCC, $ CO2 trading cost, $ Penalties on the imbalance between electricity supply and demand, $ Unitary price of coal, $/kg Unitary trading price of CO2, $/kg Electricity price, $/MWh Penalty coefficient of renewable electricity curtailment, $/MWh Maintenance cost of CFPP, $/MWh Maintenance cost of PCC, $/kg CO2 Power generation efficiency of CFPP Power generation efficiency of the LP turbine Power attenuation coefficient of PV Low calorific value of coal, kJ/kg CO2 emission factor of coal, kg/kg Enthalpy drop of LP, kJ/kg CO2 concentration of flue gas, wt.% CO2 capture level, % Reboiler temperature, K Temperature of PV array under standard test condition, K Insolation at the surface of PV array under standard test condition, kW/m2 Temperature of PV array, K Wind speed, m/s Rated wind speed, m/s Cut-in wind speed, m/s Cut-out wind speed, m/s Insolation at the surface of PV array, kW/m2 Carbon quota allocation of CFPP Objective function Occurrence probability of scenario s Power adjustment contribution rate of PCC Rolling horizon of intraday scheduling Rolling horizon of control perceptive dynamic scheduling performance can be achieved by storing the solvent rich in CO2 during the periods of high-electricity price and regenerating it during the lowelectricity price. Zaman and Lee [20] evaluated the economic perfor­ mance of a CFPP-PCC system under two flexible operating modes, including variant capture level and solvent storage. The results showed that significant cost savings can be attained by implementing the two flexible operating strategies. Flue gas bypass operation mode was also studied for the PCC during the power plant start-up to alleviate the impact of steam extraction on the turbine by venting partial flue gas to the atmosphere [21]. Mac Dowell and Shah [22] presented another operation mode of PCC called time-varying solvent regeneration, which exhibited superior daily economic performance in the scheduling compared with other operating modes. In fact, all these operating modes share a common idea of changing the energy consumption of PCC flexibly according to the load demands and market conditions. Alie et al. [23] compared the scheduling results of PCC process under flexible and fixed CO2 capture level requirements. A reduced-order model with fewer variables was used in the optimal scheduling instead of the original high-fidelity Aspen Plus® model to reduce the computational complexity. The results showed that, flexibly changing the CO2 capture level can markedly enhance the economic performance of the integrated system by providing more reserve power, although the CO2 emission is slightly higher than the fixed capture level case. Khalilpour [24] 2 H. Xi et al. Fuel 331 (2023) 125695 Fig. 1. The schematic diagram of a regional power system consisting of CFPP-PCC and RESs. developed a multi-period mixed integer linear program (MILP) to opti­ mize the operation of PCC trains integrated with CFPP under the pro­ jected carbon and electricity markets. The results showed that, the operating profit can be increased by ramping down or even shutting down the PCC process during the periods with high electricity price. Generally, the scheduling only provides the process with the optimal operating points, and the tracking of these operating points is still dependent on the underlying control system. To this end, Arce et al. [25] presented an optimal operation framework for the solvent regeneration system of PCC. The upper layer calculated the hourly-based optimal CO2 production by solving an economic scheduling problem. Lower control layer was then designed to regulate the plant dynamically towards the operating point issued by the scheduling layer. Abdul Manaf et al. [26] developed similar optimization framework for an integrated CFPP-PCC system, in which economic scheduling was applied to find the future power output and CO2 capture level set-points; while model predictive control (MPC) was implemented in the control layer to achieve fast tracking of the scheduling results. All the aforementioned studies indicate the advantages of flexible scheduling to improve the economic performance of the PCC system. Some studies also gave insights into the mutual benefits between the PCC and RESs through effective scheduling. Chen et al. [12] carried out the scheduling study of a low carbon energy system consisting of su­ percritical CFPP-PCC, wind turbines and photovoltaic panels. They used artificial intelligence approaches of deep belief neural network [27] and particle swarm optimization [28] for model development and sched­ uling optimization. The results showed that by flexible operation of PCC, 51 % more renewable power can be accommodated in the grid to pro­ vide 35 % of the energy required for carbon capture. Similar results were also observed by Zhang and Zhang [29] through scheduling of an electricity-heat-gas energy mix integrated with carbon capture, utiliza­ tion and storage. Both of these studies expounded the views on the low carbon transformation of the energy system that there should be a symbiotic relationship between PCC and renewable power rather than a competitive one. Although the scheduling of CFPP-PCC system has been extensively studied, all of them focused on the day-ahead scheduling, which aims to find the hourly optimal operating points of power generation and CO2 capture in the next day. Although the CFPPs are required to follow the load frequently in real time, such a scheduling cannot deal with the unavoidable uncertainties of day-ahead predictions of electricity price, load demand or renewable generation [30]. In addition, the hourly scheduling is unable to make full use of the flexibility of carbon capture to manage faster load ramping of the power plant in a smaller timescale, and provide more dispatchable energy to the power grid. Moreover, because simplified steady-state model representing the couplings among fuel, electricity and CO2 emission are often used, the day-ahead sched­ uling cannot consider the closed-loop dynamic control performance of the CFPP-PCC system. The lack of coordination between scheduling and control could be a threat to the economic or even stable operation of the integrated plant, because the set-points issued by the scheduling can be infeasible to the underlying control [31]. These limitations make the standalone day-ahead scheduling method impossible to be directly used in the real operation of integrated CFPP-PCC system. Therefore, it is imperative to develop a comprehensive scheduling framework, which is closely related to the control practice and is capable of exerting the decarbonization and flexibility of carbon capture in multiple timescales. For these reasons, this paper proposes a novel hierarchical sched­ uling structure consisted by three layers of scheduling with different timescale features to achieve an economic, flexible and low carbon operation of the integrated CFPP-PCC system. The upper layer imple­ ments a day-ahead stochastic scheduling, in which hourly operating instructions are optimized to enhance the overall economic performance of the plant involving fuel consumption, electricity load following and carbon trading in the entire next day. The middle layer conducts a rolling horizon intraday scheduling to modify day-ahead power outputs according to the ultra-short-term forecast data. A novel index reflecting the power adjustment contribution of PCC is introduced to improve power ramping performance of CFPP by promoting the flexible opera­ tion of PCC in a small timescale. The lower layer offers a controlperceptive close-loop dynamic scheduling to further refine the intraday scheduling results, so that more feasible results can be issued to underlying control. To our best knowledge, this paper is the first study to propose a complete and practical scheduling scheme for the integrated CFPP-PCC system to fully exploit the decarbonisation and flexibility of carbon capture. Case study using real data of weather condition and load demand demonstrates that the proposed scheduling scheme can improve the power load tracking performance by 36.7 % with satisfactory per­ formance in carbon capture. Further discussions are also presented to identify the roles of each scheduling layer and to understand the influ­ ence of underlying control on the scheduling. The novel contributions of this study are as follows: 3 H. Xi et al. Fuel 331 (2023) 125695 Fig. 2. The diagram of 660 MW CFPP-PCC model [32]. 1) A hierarchical scheduling scheme is proposed for the integrated CFPP-PCC system to fulfill the decarbonization and flexibility sup­ port functions of PCC in multiple timescales; 2) A novel index reflecting power adjustment contribution of PCC is introduced in the scheduling to offer additional dispatchable power for the CFPP by promoting the flexible operation of PCC in a small timescale; 3) A control-perceptive scheduling is developed to bridge the gap be­ tween the optimality of the scheduling and the feasibility of the underlying control; 4) A novel PCC control system is proposed in coordination with scheduling scheme, which can further improve the power ramping performance of the connected CFPP; 5) The superiority of proposed scheduling scheme is demonstrated based on real-time operating simulation. Comprehensive discussions are also presented to identify the roles of each scheduling layer. power output of the CFPP. Therefore, developing a model that can well reflect the relationships between coal, heat, power and carbon within the CFPP-PCC system is the prerequisite to the optimal scheduling study. Considering that optimal scheduling based on a detailed firstprinciple model is highly complex and time consuming, a surrogate model which focuses on the interactions between key variables of the CFPP-PCC will be developed first. Based on the energy conservation principle, the power output of standalone CFPP can be calculated by: 2. System description and model development mfg = ffg (mcoal ) (2) To validate the effectiveness of the proposed scheduling approach in accommodating the intermittent RESs, a regional power grid is consid­ ered as shown in Fig. 1. The regional power demand is met by a su­ percritical CFPP-PCC plant and RESs of wind turbines and photovoltaic (PV) arrays. Given the lack of additional adjustable energy devices, it is of great significance to exploit the flexibility of the integrated CFPP-PCC system in meeting the supply–demand as fast as possible in the context of uncertain load demands and intermittent RESs. φCO2 = μCO2 mcoal /mfg (3) (1) PCFPP = ηCFPP mcoal QLHV coal where mcoal is the mass flowrate of pulverized coal; is the low calorific value of coal; ηCFPP denotes the power generation efficiency of CFPP. The flue gas flowrate mfg and CO2 concentration φCO2 can be esti­ mated by: QLHV coal where ffg is the function between coal flowrate and flue gas flowrate; μCO2 is the CO2 emission factor of coal, which is constant since the coal characteristic is assumed to be unchanged. For solvent regeneration in the PCC, some of the steam has to be withdrawn from the inlet of low pressure (LP) steam turbine and sent to the reboiler. As a result, significant power loss PQPCC occurs for the CFPP, which can be calculated by: 2.1. Coal-fired power plant integrated with solvent-based carbon capture plant PQPCC = ηLP ΔhLP mstPCC (4) mstPCC where is the reboiler steam flowrate extracted from the steam turbine; ΔhLP and ηLP are the enthalpy drop and power generation effi­ ciency of the LP turbine, respectively. Consequently, the power output of integrated CFPP-PCC system PCFPP− PCC can be given by: The schematic structure of a 660MWe supercritical CFPP integrated with 30 % monoethanolamine (MEA)-based PCC process is shown in Fig. 2. There are strong interactions between the CFPP and PCC systems because of the interconnections at the flue gas and water-steam systems. The variations of flue gas flowrate during the load ramping of CFPP brings a crucial effect on the operation of PCC, while the change of reboiler steam flowrate for solvent regeneration in the PCC alters the PCFPP− PCC = PCFPP − PQPCC (5) The following model is used to reflect the operating performance of 4 H. Xi et al. Fuel 331 (2023) 125695 circulation flowrate; mstPCC is the reboiler steam flowrate, which can reflect the heat consumption of PCC. The electric power consumption caused by solvent circulation and CO2 compression is directly provided by the regional power grid, which can be calculated by: PCPCC = a × mscf + b × mpro CO2 where a and b are unitary power consumptions for solvent circula­ tion and CO2 compression, respectively. Fig. 3 illustrates the feasible operation region of the integrated CFPPPCC system. The allowable operation range of standalone CFPP is rep­ resented by line E0-A0, which is shifted down to line E-A after the integration with PCC due to the reboiler steam extraction. The feasible operation region of retrofitted CFPP (A-B-C-D-E-A) is thus defined by boiler rated load (BRL) condition (line A-B), 50 % BRL condition (line DE) and the specified minimum and maximum reboiler steam flow con­ ditions (lines A-E and B-C). In addition, the minimum LP steam flowrate requirement (line C-D) should be met for the safe operation of the LP, that the increase of reboiler steam flowrate must be achieved by increasing the BRL. Line 1-5 and line 2-3 respectively represent mini­ mum (40 %) and maximum (95 %) CO2 capture level conditions at designed reboiler temperature (392.2 K). With further consideration of the limitation on minimum solvent circulation flowrate (line 4-5), the feasible operation region of the integrated CFPP-PCC can represented by the area1-2-3-4-5-1. Line 1′ -5′ and line 2′ -3′ denote the 50 % and 90 % CO2 capture level conditions, respectively. The main operating param­ eters of these corner points are listed in Table A1. Given the structure of the surrogate model, corresponding model parameters are then identified based on the operating data generated from a first-principle CFPP-PCC model previously developed in gCCS® platform [33]. The inputs and outputs of the surrogate models are given in Table 1. A total of 2500 steady-state samples covering the feasible region are generated by simulating the first-principle CFPP-PCC model, in which 2000 samples are used for parameter identification through linear regression while the rest are used for validation. Part of the validation results are shown in Fig. 4, which demonstrate that the sur­ rogate model is in good agreement with the first-principle model for most variables within the feasible operating region. Therefore, the sur­ rogate model can be used in the scheduling optimization to improve the Fig. 3. Feasible operation region of the integrated CFPP-PCC system. Table 1 The inputs and outputs of the surrogate models. CFPP-PCC model CFPP PCC Inputs Coal mass flowrate (mcoal ) Feed water flowrate Reboiler steam flowrate (mstPCC ) Main steam valve position Outputs Power output (PCFPP− PCC ) Main steam pressure Flue gas flowrate (mfg ) Flue gas composition (φfg ) Solvent circulation rate (mscf ) Reboiler steam flowrate (mstPCC ) CO2 capture level (CL) Re-boiler temperature (Treb ) CO2 production rate (mpro CO2 ) the PCC process: ( ) ( ) st CL, Treb , mpro CO2 = LPCC mscf , mPCC , mfg , φfg (7) (6) where CL,Treb , mpro CO2 are the CO2 capture level, reboiler temperature and CO2 production rate of the PCC, respectively; mscf is the solvent Fig. 4. Verification results of the surrogate model (red solid line: first-principle model; blue dashed line: surrogate model). (For interpretation of the references to colour in this figure legend, the reader is referred to the web version of this article.) 5 H. Xi et al. Fuel 331 (2023) 125695 Fig. 5. Proposed multi-timescale scheduling framework for the integrated CFPP-PCC. computational efficiency. The data used in model identification and verification can be found in the Supplementary Material. 3. Multi-timescale hierarchical scheduling of the integrated CFPP-PCC system 2.2. Renewable power generations To maximize the decarbonization and flexibility of carbon capture technology and achieve an optimal coordinated operation of the inte­ grated CFPP-PCC system, a multi-timescale hierarchical scheduling scheme is set up as shown in Fig. 5. The scheduling hierarchy is composed by three layers with different timescales. The upper layer of the hierarchy implements a day-ahead stochastic scheduling, which minimizes the overall operating costs of the CFPP-PCC within the next 24 h by providing the hourly optimal operating instructions according to the forecasts of renewable generations and power demands. The middle layer of the hierarchy carries out a rolling horizon intraday scheduling to modify the corresponding day-ahead scheduling results for the next 4 h at a 15-minute interval. Because the intraday short-term predictions of renewable generation and load demand are much more accurate than the day-ahead prediction, the operating economics of the CFPP-PCC can get improved in this layer. In addition, a novel index reflecting the power adjustment contribution of the PCC is introduced in this layer to promote the flexible operation of PCC in a small timescale, which is useful to upgrade the power ramping performance of the CFPP. The lower layer of the hierarchy offers a closed-loop dynamic scheduling to bridge the gap between the optimality of the scheduling and the feasi­ bility of the underlying control. Finally, the intraday scheduling results are further refined in a minute-scale and issued to the real time control. RESs of wind turbines and solar PV are considered in the regional power system. The power output of wind turbine can be calculated by [34]: ⎧ 0, v < vci ; v⩾vco ⎪ ⎪ ⎪ ⎪ ⎨ (v)3 − (vci )3 , vci ⩽v⩽vr PWT = Prate (8) WT × ⎪ (vr )3 − (vci )3 ⎪ ⎪ ⎪ ⎩ Prate WT , vr < v < vco where PWT and Prate WT are the real power output and rated capacity of wind turbine;v,vr , vci and vco are wind speed at the height of the turbine hub, rated wind speed, cut-in and cut-out wind speeds, respectively. The power output of PV panel can be calculated by [35]: PPV = ηPV Prate PV GT [1 + αp (TC − TSTC )] GSTC (9) where PPV and Prate PV are the real power output and the rated capacity of PV array, respectively; ηPV is the power attenuation coefficient; GT and TC are the insolation and temperature at the surface of PV array; GSTC and TSTC are the insolation and temperature of standard test condition; αp is the power-temperature coefficient. 3.1. Day-ahead stochastic scheduling The upper layer of the hierarchy carries out a day-ahead economy6 H. Xi et al. Fuel 331 (2023) 125695 ( s = αCO2 CCO 2 24 ∑ 1 ,s mLCO (t) − σ 2 t=1 24 ∑ ) 1 ,s PLCFPP− PCC (t) (13) t=1 1 ,s where mLCO (t) is the carbon emission of integrated CFPP-PCC system; 2 αCO2 is unitary trading price of CO2 and σ denotes the carbon quota allocation [38] of CFPP. The supply–demand imbalance penalty is calculated by: s Cimb = αcut 24 ∑ PLcut1 ,s (t) + 24 ∑ t=1 1 ,s αbuy PLbuy (t) (14) t=1 1 ,s where PLbuy (t) and PLcut1 ,s (t) are respectively the amount of purchased electricity from external grid and the curtailment of renewable power at time t under scenario s; whereas αcut and αbuy are the curtailment penalty coefficient and electricity price, respectively. The following constraints should also be satisfied under each sce­ nario in the day-ahead scheduling. First is the power balance constraints of the regional power system given by: Fig. 6. Power output responses corresponding to step changes of coal mass flowrate and reboiler steam flowrate. 1 ,s PLCFPP− oriented scheduling, in which hourly operating instructions of the CFPPPCC within the next day are optimized according to the forecast of RES generations and load demands. Given that the scheduling interval is one hour, which is much longer than the closed-loop dynamic response time of the process, the steady-state model of the CFPP-PCC developed in Section 2 is applied in this layer to represent the interactions among coal, heat, power, and carbon. Besides, scenario-based anti-uncertainty approach is used in the scheduling to alleviate the impact of unavoidable day-ahead forecasting error. Many possible scenarios of renewable generations and load demands are generated to reflect the forecast un­ certainties using hyper-Latin sampling [36]. Then the simultaneous backward scenario reduction scheme [37] is used to select several representative scenarios from the initial scenario set to ease the computational burden. The following objective function is considered in the day-ahead scheduling to minimize the daily operating costs of the integrated sys­ tem JL1 under all representative scenarios: S ∑ minJL1 = min d L1 dL1 + ] 24 ∑ ( ) L1 ,s 1 ,s αcoal mLcoal (t) + βopex CFPP PCFPP (t) (10) (11) t=1 where αcoal is the unitary price of coal and βopex CFPP is the unitary maintenance cost of CFPP. The operation costs of PCC can be calculated by: s CPCC = 24 ∑ ( pro,L1 ,s βopex (t) PCC mCO2 ) (16) L1 ,s Treb (t) = 392.2K (17) The middle layer of the hierarchy implements intraday scheduling of the CFPP-PCC in a rolling horizon optimization manner [39]. For every 15 min, the intraday scheduling refines the day-ahead scheduling results of the next four hours into 15-min resolution according to the intraday short-term forecast of load demands and RES generation. The objective of this layer is to alleviate the impact of day-ahead prediction error and provide more dispatchable power in small timescale to ease the inte­ gration of intermittent renewable power. Considering that the time interval of intraday scheduling is short­ ened to 15 min, it is necessary to consider the dynamic response of power output to improve the load ramping performance of the CFPP. Fig. 6 shows the responses of power output corresponding to step changes of coal mass flowrate and reboiler steam flowrate. It can be observed that the power output is mostly influenced by the coal mass flowrate, but it takes more than 8 min to reach a new steady state because of the inertia and time delay lumped in the processes of coal pulverizing, combustion, and heat and mass transfer, etc. In contrast, reboiler steam flowrate has a much quicker influence on power output, and the response time is found to be less than 1 min. The results indicate that flexible regulation of the reboiler steam can effectively improve the power ramping performance of CFPP, and thus provide more dis­ patchable power in short timescale. To promote the participation of PCC in power plant load ramping, a novel index γL2 reflecting the power adjustment contribution of PCC is proposed in the intraday scheduling: in which dL1 is the decision variables of the day-ahead scheduling 1 including the power output of the integrated CFPP-PCC PLCFPP− PCC and the CO2 capture levelCLL1 ; CsCFPP and CsPCC stand for the operating costs of CFPP and PCC, respectively; CsCO2 is the CO2 trading cost and Csimb rep­ resents the penalties on the imbalance between supply and demand. The index s denotes the s-th scenario considered in the optimization, whereas π s is the occurrence probability of scenario s. The operating costs of CFPP are composed by the fuel and mainte­ nance costs: s CCFPP = 50\% ⩽CLL1 ,s (t)⩽90% 3.2. Intraday scheduling ( L1 PCC ; CL (15) is the load demands at time t under scenario s. where To ensure an efficient operation of the PCC, the following constraints on CO2 capture level and reboiler temperature are also considered in the optimization in addition to the feasible operating region of CFPP-PCC given in Fig. 3. s s s πs CCFPP + CCO + CPCC 2 ) [ 1 , dL1 = PLCFPP− L1 ,s L1 ,s 1 ,s PC,L PCC (t) − Pcut (t) = Pload (t) 1 ,s (t) PLload s=1 s Cimb L1 ,s L1 ,s L1 ,s PCC (t) + PPV (t) + PWT (t) + Pbuy (t) − (12) t=1 γ L2 = where βopex PCC is the unitary maintenance costs of PCC. The CO2 trading costs are presented by: 2 2 ΔPQ,L ΔPQ,L PCC PCC = L2 L2 2 ΔPCFPP− PCC ΔPCFPP + ΔPQ,L PCC 2 ΔPLCFPP− = 7 2 (PLCFPP 2 = PLCFPP− − PL 1 ( PCC L2 CFPP− LPCC ) L1 1 PCFPP ) + − (PPCC − PPCC ) 2 2 = ΔPLCFPP + ΔPQ,L PCC PCC − (18) (19) H. Xi et al. Fuel 331 (2023) 125695 Like the day-head scheduling, the following power balance con­ straints also need to be satisfied at intraday scheduling stage: 2 where ΔPLCFPP− PCC is the adjustment of intraday power load instruc­ tion of CFPP-PCC based on the corresponding day-ahead instruction, L2 2 and ΔPQ,L PCC and ΔPCFPP denote the power adjustment contributions of PCC reboiler steam and coal mass flowrate, respectively. A large value of γ represents a great contribution of PCC to the power ramping in a short timescale. The following objective function is then used in the intraday scheduling: ( ) ] [ 2 L2 ,t0 L2 L2 ,t0 minJLt02 = min θ1 Cimb − θ2 Cpac , dL2 = PLCFPP− PCC ; CL dL2 2 PLCFPP− ⎪ ⎪ ⎪ ⎪ ⎪ ⎩ L2 ,t0 Cpac = t∑ 0 +NP (20) where dL2 is the decision variables of the intraday scheduling 2 including the power output of the integrated CFPP-PCC PLCFPP− PCC and the L2 ,t0 L2 CO2 capture levelCL ; Cimb is the intraday supply–demand imbalance penalty within the future horizon starting from t0 + 1 to t0 + Np (Np = 16 in this study, since the next four hours with the time interval of 15 min is 2 ,t0 reflects the power adjustment considered at each sampling time t0); CLpac contributions of the PCC within the next four hours; θ1 and θ2 are cor­ responding weighting coefficients. Considering that division between variables is contained inγL2 (t), the objective function (20) cannot be directly solved by conventional linear solver. It is thus rewritten into the following form to improve the computational efficiency: ( ) ] [ 2 L2 ,t0 L2 L2 ,t0 minJLt02 = min θ1 Cimb , dL2 = PLCFPP− + θ2 Cpac PCC ; CL (23) − ΔCLmax ⩽CLL2 (t + 1) − CLL2 (t)⩽ΔCLmax (24) 50% − ε⩽CLL2 ⩽90% + ε (25) L2 Treb (t) = 392.2K (26) where ε is the relaxation value. When ε is set to 0, the capture level issued from day-ahead scheduling must be strictly followed in the intraday stage. Because the main variables within the CFPP-PCC can approach the steady-state within 15 min, the steady-state model developed in Section 2 can still be used in the intraday scheduling, and the feasible operating region given in Fig. 3 has to be considered as additional constraints. At each sampling time, by minimizing the objective function (21) subject to the above constraints, the best instruction sequence for the power output and CO2 capture level within the given horizon Np can be determined. However, only the current instructions are issued to the lower layer of the hierarchy. The optimization will repeat at next sam­ pling period using the latest forecast data of RES generations and power demands. dL2 (21) ⎪ t∑ t∑ 0 +NP 0 +NP ⎪ ⎪ L2 ,t0 2 2 ⎪ ⎪ ΔPLCFPP (t) + λ2 ΔPQ,L ⎩ Cpac = λ1 PCC (t) t=t0 +1 L2 L2 max − ΔPmax CFPP ⩽PCFPP (t + 1) − PCFPP (t)⩽ΔPCFPP where and ΔCLmax are respectively the maximum ramping power and CO2 capture level for the CFPP and PCC within the sched­ uling interval. The CO2 capture level constraints given in the day-ahead scheduling is relaxed as follows in the intraday scheduling to better unlock the power adjustment role of PCC; whereas the same reboiler temperature constraint is still required to be met. γL2 (t) ⎧ t∑ t∑ 0 +NP 0 +NP ⎪ L2 ,t0 ⎪ 2 ⎪ Cimb = αcut PLcut2 (t) + αtbuy PLbuy (t) ⎪ ⎪ ⎨ t=t0 +1 t=t0 +1 (22) ΔPmax CFPP t=t0 +1 dL2 L2 L2 2 PC,L PCC (t) − Pcut (t) = Pload (t) The rate constraints of CFPP-PCC need to be added in intraday stage due to a short scheduling time interval: dL2 ⎧ t∑ t∑ 0 +NP 0 +NP ⎪ L2 ,t0 ⎪ 2 ⎪ PLcut2 (t) + αtbuy PLbuy (t) ⎪ Cimb = αcut ⎪ ⎨ t=t0 +1 t=t0 +1 L2 L2 L2 PCC (t) + PPV (t) + PWT (t) + Pbuy (t) − 3.3. Control-perceptive dynamic scheduling t=t0 +1 where λ1 and λ2 (λ1 > λ2) are the weighting coefficients to promote the participation of PCC in power load regulation. In the lower layer of the hierarchy, the time interval of scheduling is further shortened to 5 min or smaller, so that the CFPP-PCC can provide Fig. 7. Open-loop responses of PCC corresponding to the step changes of solvent circulation flowrate and reboiler steam flowrate. 8 H. Xi et al. Fuel 331 (2023) 125695 Fig. 8. Schematic diagrams of the conventional and proposed control structures of PCC. (a) solvent circulation flowrate to control CO2 capture level, reboiler steam flowrate to control reboiler temperature, (b) reboiler steam flowrate to control CO2 production rate, solvent circulation flowrate to control reboiler temperature. more flexible support for the grid to handle the real time fluctuations on both the RES and power load. Within such a small time period, the dy­ namic transition for most concerned variables cannot be finished. Therefore, the steady-state model-based scheduling approach is chal­ lenging to provide optimal and feasible instructions in practice. To this end, a control-perceptive dynamic scheduling is proposed in this layer, in which closed-loop dynamic model of the CFPP-PCC is applied to bridge the gap between the optimality of the scheduling and the feasibility of control. The closed-loop dynamic model of the CFPPPCC can be described in the following form based on the first princi­ ple model developed in [32]: dx/dt = f (x, u) y = h(x, u) u = g(r − y) s.t. umin ⩽u⩽umax − Δumax ⩽Δu⩽Δumax closed-loop system model (27) can fully consider the performance of the controller and estimate the dynamic variations of manipulated and controlled variables according to the scheduling instructions. Considering that the first-principle dynamic model (27) is compli­ cated and time-consuming for the minute-scale dynamic optimization, the following discrete state-space model is identified and applied in the control-perceptive scheduling to improve the computational efficiency: { z(t + 1) = Az(t) + Br(t) [y(t); u(t)] = Cz(t) + Dr(t) ] [ L3 ,r pro,L3 ,r L3 ,r (t); Treb (t) r(t) = PCFPP− PCC (t); mCO2 [ L3 ] L3 L3 3 y(t) = PCFPP− PCC (t); mpro,L CO2 (t); Treb (t); CL (t) [ ] L3 3 3 u(t) = mLcoal (t); mst,L PCC (t); mscf (t) (27) (28) where A, B, C, D are the parameters of state-space model; z(t) is the state variables of the state-space model at time t, which do not have specific physical meaning but is used to reflect the dynamic relationship pro,L3 ,r 3 ,r between input and output; PLCFPP− (t) are the scheduling PCC (t) and mCO2 where × denotes the internal state variables of integrated CFPP-PCC, such as the steam temperature in the heat exchangers and the CO2 loading in the solvent; u stands for manipulated variables, such as coal mass flowrate, solvent circulation flowrate and reboiler steam flowrate; y denotes the controlled variables, such as power output, CO2 produc­ tion rate and reboiler temperature; umin, umax and Δumax are magnitude and rate limitations of u; f and h denote the first-principle functions of CFPP-PCC; g stands for the feedback controller function which calculates u based on the deviation between y and the scheduling instruction r. The L3 ,r (t) is the instructions of power output and CO2 production rate; Treb reboiler temperature. The selection of scheduling instructions of the PCC process in this layer is dependent on the control system development, which will be introduced in the next section. Based on the dynamic model (28), the objective function of controlperceptive scheduling is given by: 9 H. Xi et al. Fuel 331 (2023) 125695 [ 3 ,r L3 ,t0 L3 ,t0 L3 ,t0 minJL3 = min(θ3 Cimb + θ4 Cpac + θ5 Ctra ), dL3 = PLCFPP− dL3 ⎧ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎨ dL3 L3 ,t0 Cimb = αcut t∑ 0 +Ns t=t0 +1 L3 ,t0 Cpac = λ3 t∑ 0 +Ns t∑ 0 +Ns PLcut3 (t) + PCC (t) ] 3 αtbuy PLbuy (t) t=t0 +1 3 ,r ΔPLCFPP (t) + λ4 t=t0 +1 ⎪ t∑ 0 +Ns ( ⎪ ⎪ L3 ,r L3 ,t0 ⎪ ⎪ PCFPP− ⎪ Ctra = ω1 ⎪ ⎪ t=t0 +1 ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎪ ⎩ pro,L3 ,r PCC ; mCO2 t∑ 0 +Ns 3 ,r ΔPQ,L PCC (t) (29) t=t0 +1 3 − PLCFPP− )2 PCC (t) + ω2 t∑ 0 +Ns ( )2 3 ,r 3 mpro,L (t) − mpro,L CO2 (t) CO2 t=t0 +1 +ω3 t∑ 0 +Ns ( L3 ,r L3 Treb (t) − Treb (t) )2 t=t0 +1 50% − ε⩽CLL3 ⩽90% + ε (31) On the other hand, Fig. 7 also shows that the CO2 production rate can be quickly influenced by the reboiler steam flowrate. This motivates us to select the CO2 production rate as controlled variable and regulate it through the reboiler steam flowrate. The CO2 production rate can also serve as an indicator to evaluate the performance of CO2 capture. Moreover, under such a design, the CO2 production rate instruction is­ sued by the scheduling can lead to a rapid response of reboiler steam flowrate, which is helpful to exploit the flexibility of PCC in a small timescale to upgrade the power ramping performance of the CFPP. For these reasons, a novel control structure as visualized in Fig. 8(b) is developed in the proposed scheduling scheme. The CO2 production rate and reboiler temperature are selected as controlled variables, and the reboiler steam flowrate and solvent circulation rate are selected as the corresponding manipulated variables to adjust them. To improve the response ability of the PCC to flue gas and ensure an efficient operation of absorber, flue gas feedforward is added in the proposed control structure to speed up the adjustment of solvent circulation flowrate. L3 ,r Treb (t) = 392.2K (32) 4. Results 3 ,t0 3 ,t0 Like the intraday scheduling, CLimb and CLpac are considered in the objective function to reduce the supply–demand imbalance penalty in 5minute timescale and promote the PCC to participate in power adjust­ ment. Besides,CLtra3 ,t0 , the dynamic tracking offset between scheduling instructions and controlled variables within the future horizon starting from t0 + 1 to t0 + Ns is also included to reflect the feasibility of the scheduling results; ω1, ω2 and ω3 are corresponding weighting co­ efficients. The control-perceptive scheduling aims to optimize the operating performance of the CFPP-PCC within the next one hour at the time resolution of 5 min, thus Ns is set as 12 in this layer. In addition to the feasible region given in Fig. 3, the following con­ straints are also imposed on the scheduling optimization to ensure power balance and safe operation of the PCC process: 3 ,r PLCFPP− L3 L3 L3 PCC (t) + PPV (t) + PWT (t) + Pbuy (t) − L3 L3 3 PC,L PCC (t) − Pcut (t) = Pload (t) (30) Rolling horizon optimization strategy will also be applied in this layer using the latest forecast data of RES generations and power demands. This section verifies the effectiveness of the proposed scheduling scheme through simulation study of a 660MWe super-critical CFPP in­ tegrated with 30 % MEA-based PCC in an integrated energy mix. Besides 3.4. Underlying control Since the lower layer scheduling is designed with control perceptive, the dynamic performance of underlying PCC control system will affect the scheduling results. Therefore, the open-loop dynamic responses of CO2 capture level, reboiler temperature and CO2 production rate are investigated with +5 % step changes of reboiler steam flowrate and solvent circulation flowrate respectively, which are shown in Fig. 7. It can be found that reboiler steam flowrate has a very slow influence on the CO2 capture level, and the transient time to a new steady state is more than 2.5 h. Meanwhile, solvent circulation flowrate also shows a slow effect on reboiler temperature. The reason for these two features can be explained by the large time constant caused by solvent holdup in packing and buffer tank. Given that solvent circulation flowrate shows an instantaneous effect on CO2 capture level, conventional control structure of PCC [16,26], as shown in Fig. 8(a), manipulates the solvent circulation flowrate to achieve fast adjustment of CO2 capture level, whilst maintaining the reboiler temperature by changing the reboiler steam flowrate. However, such a control structure requires continuous adjustment of reboiler steam flowrate to compensate for the slow in­ fluence induced by the solvent circulation rate, which is easy to cause long-term fluctuations in power generation from the perspective of the integrated CFPP-PCC system. Fig. 9. Uncertain predictions and representative scenarios of renewable power and load demands (light grey line: uncertain predictions; colored line: repre­ sentative scenarios considered in the day-ahead scheduling). 10 H. Xi et al. Fuel 331 (2023) 125695 Table 2 Economic parameters for the scheduling of integrated CFPP-PCC system. Parameters Units Values Coal costs Maintenance costs of CFPP Renewable power curtailments penalty CO2 trade costs carbon quota allocation Electricity purchasing prices $/ton $/MWh $/MWh $/ton tCO2/MWh $/MWh 140 [40] 5.73 [12] 80 25 [41] 0.3 83.7 [42] Table 3 Weight coefficients in scheduling. Parameters Values Parameters Values θ1 θ2 θ3 θ4 θ5 10 2 10 2 2 5 λ1 λ2 λ3 λ4 4 0.05 10 0 20 1 ω2 ω1 ω3 Fig. 10. Day-ahead scheduling results of the CFPP-PCC system. generated and sent to the PCC absorber. As a result, more steam is withdrawn from the turbine for solvent regeneration to maintain the given day-ahead CO2 capture level. Such an action reduces the power generation in turn, making the PCC a stumbling block for the flexible operation of the CFPP. Therefore, as observed in the bottom right figure of Fig. 11, the power adjustment contribution of the PCC is negative most of the time. This feature is more prominent in case of large dayahead prediction error, because more power adjustments are required to be made by the CFPP. The proposed intraday scheduling scheme also modifies the dayahead scheduling instructions, trying to reduce the RES curtailment and electricity purchase in this layer. However, since the power adjustment contribution of the PCC is considered in the objective function of intraday scheduling, the PCC is actively changing the reboiler steam to support the power ramping of the CFPP. The bottom left figure of Fig. 11 illustrates that around 25 % of the power adjustment task in the intraday scheduling is contributed by the PCC throughout the day. In case of small day-ahead prediction error, PCC can complete most of the power adjustment task, which will reduce the load varying operation difficulties of the upstream CFPP. Moreover, by imposing the relevant constraint in the scheduling, the CO2 capture level is fluctuating within a given range around the day-ahead scheduling instructions. The scheduling results of the bottom layer hierarchy and real-time dynamic operating performance of the CFPP-PCC for both conven­ tional and proposed approaches are presented in Figs. 12 and 13. The key operating performance indices are listed in Table 4. As shown in Fig. 13, different scheduling instructions are generated by the two scheduling schemes, which lead to remarkable differences in the realtime operating performance. Without considering the dynamic oper­ ating practice of the CFPP-PCC system, the scheduling instructions is­ sued by the conventional approach cannot be well tracked by the underlying control system. The variations of power output set-points are poorly tracked by the control system within the scheduling interval. Apparent steady-state offsets appear in cases of large set-point changes. The supply–demand imbalance caused by the tracking error is up to 103.36MWh under the conventional scheduling approach throughout the day, which equals to an additional cost of $2.8 k based on the eco­ nomic parameters considered. By contrast, using the control-perceptive scheduling approach, the load instructions issued by the proposed scheduling scheme can be well tracked by the underlying control system. Moreover, the use of power adjustment contribution index and control system matched with this idea further upgrades the power ramping capability of the CFPP. The supply–demand imbalance is reduced by 36.7 % compared with the conventional approach, which means that more RES power can be accommodated in the power grid. the CFPP, 165 MWe wind power generation and 100 MWe PV power generation are also included in the energy mix for power supply. Real weather and load demands data derived from [12] are used in the simulation. Fig. 9 shows the uncertain forecasts of wind power outputs, PV power outputs and power demands for the next 24 h and the corre­ sponding representative scenarios selected through the simultaneous backward scenario reduction [37]. Economic parameters and weight coefficient in scheduling are listed in Tables 2 and 3, respectively. Large θ1 and θ3 are applied in the scheduling because the prior target of CFPP is to eliminate the demand–supply imbalance. We also set λ1 > λ2, λ3 > λ4 to improve the initiative of PCC in power adjustment, and set a larger ω1 in the controlperceptive scheduling layer to ensure the feasibility of the scheduling instructions. The conventional PCC scheduling approach [22] is also applied in the same day-ahead scheduling layer and compared with the proposed approach. However, in the middle and lower layers of the scheduling, only the CFPP changes the load according to the latest forecasts of RES generations and power demands, and the PCC only follows the flue gas variation of CFPP, maintaining the CO2 capture level according to the instructions optimized in the day-ahead scheduling. Besides, steadystate model is used in all three scheduling layers, and the dynamic operating practice is not considered in the scheduling. The scheduling results and real time operation performance of the CFPP-PCC system under the two scheduling approaches are shown in Figs. 10-13. Fig. 10 shows the day-ahead scheduling results of the CFPP-PCC. It can be observed that, during valley load periods, higher CO2 capture level instructions are dispatched to the PCC, which enables the CFPP to further lower the power output to accommodate more renewable power. While during the peak load periods, the CO2 capture level is reduced so that more steam can be used in the turbine for power generation. Even so, 25.83MWh of electric power still needs to be purchased during 10:00–12:00 because of the high load demands and insufficient renew­ able power. In general, the economic operation of integrated system within the next 24 h can be achieved through flexible change of CO2 capture level in an hourly-based timescale. Based on the day-ahead scheduling, the intraday scheduling results of the proposed and conventional scheduling schemes are compared in Fig. 11. Both scheduling schemes refine the power output instructions of CFPP to 15-minute timescale according to the latest forecast informa­ tion. For the conventional scheduling approach, the flexibility of PCC in small timescale is not activated as it tightly follows the day-ahead cap­ ture level instructions. Most of the time, the power adjustment task of CFPP is undertaken only through the variation of coal mass flowrate. When CFPP needs to increase power output, more flue gas flowrate is 11 H. Xi et al. Fuel 331 (2023) 125695 Fig. 11. Intraday scheduling results of the CFPP-PCC system: (a) proposed scheduling scheme, (b) conventional scheduling scheme. Fig. 12. Control-perceptive scheduling results of the (a) proposed scheme, and (b) conventional scheme. The proposed scheduling scheme fully exploits the flexibility support function of the PCC process in multiple timescales, which significantly improves the load ramping performance of the CFPP. This improvement allows the fluctuations of CO2 capture level during the operation. However, it is worth noting that a little higher daily average CO2 capture level is achieved in the case study under the proposed scheduling scheme compared with the conventional scheme. This finding indicates the importance of refining the scheduling instructions of CO2 capture level according to the latest forecasts of RES generations and load de­ mands, because the accommodated RES power allows the PCC to withdraw more steam from the CFPP to increase the CO2 capture level. The case study illustrates that better load following and economic per­ formance of the CFPP-PCC can be achieved under the proposed sched­ uling scheme. 12 H. Xi et al. Fuel 331 (2023) 125695 Fig. 13. Real-time dynamic operation performance of the CFPP-PCC under two scheduling schemes: (a) power output, (b) CO2 production rate, and (c) CO2 cap­ ture level. 13 H. Xi et al. Fuel 331 (2023) 125695 CFPP power regulation. As a result, the power adjustment contribution rate of PCC is zero for most of the day, which indicates that all power output modifications caused by the day-ahead forecast error are handled by the CFPP independently. By contrast, with smaller λ2 and λ4 in the scheduling, Cases 2 and 3 give higher power adjustment contribution rates to the PCC, which effectively promote the PCC to flexibly change the CO2 production rate to upgrade the power ramping ability of CFPP. As can be observed from Fig. 15, Cases 2 and 3 achieve superior power load tracking performance compared with Case 1 and reduce the dy­ namic tracking offset to 70.10MWh and 65.43MWh, respectively as shown in Table 5. Besides, due to the zero mean normal distribution of the forecast error [43], the adjustment of reboiler steam also presents the similar trend for power output modification. Therefore, although the instantaneous CO2 capture level is fluctuating over the scheduling pe­ riods, the daily average CO2 capture level is changed little. Table 4 Key operating performance indices of proposed and conventional scheduling schemes. Real operation results Conventional scheme Proposed scheme Purchased power (MWh) Curtailed power (MWh) Average capture level CO2 emission (ton) Coal consumption (ton) Total costs (k$) 76.90 52.29 0.814 1773.4 5150.7 793.0 58.57 32.69 0.818 1767.2 5154.2 790.2 5. Discussion The case study results have demonstrated the advantages of pro­ posed scheduling scheme for the economic and flexible operation of integrated CFPP-PCC system. The following discussions are carried out in this section to elaborate the benefits of the innovations proposed in this study. 5.2. The effect of control-perceptive scheduling To demonstrate the underlying control performance in the bottom layer scheduling, scheduling results based on steady-state and close-loop dynamic models are compared in Fig. 16. Because the control-perceptive scheduling knows that the power ramping speed of CFPP is not that fast during the scheduling interval due to the slow impact of coal mass flowrate, the variations of power output instruction are smaller compared with that issued by the steady-state scheduling. In contrast, stronger variations of CO2 production rate instructions are issued by the control-perceptive scheduling, since it can be rapidly regulated by the reboiler steam flowrate, thus facilitates the use of carbon capture for CFPP power ramping. Nevertheless, the steady-state scheduling [12,23,24] ignores the dynamic operating practice of the plant and assumes that the load changes can be finished instantaneously. Consequently, infeasible in­ structions are issued, which cannot be followed by the control system within the scheduling interval. Moreover, the fast impact of reboiler steam flowrate on the power output cannot be fully exploited although the power adjustment contribution rate of PCC has been considered in the scheduling. As shown in Fig. 16, the scheduling result issued by the control-perceptive scheduling can be more closely followed by the un­ derlying control. The supply–demand imbalance caused by dynamic tracking offset is reduced by 12.07 MWh compared with the steady-state scheduling. 5.1. The effect of power adjustment contribution rate index of PCC The power adjustment contribution rate index of PCC is considered in the intraday and control-perceptive scheduling layers to encourage the use of PCC in CFPP load ramping. To demonstrate its effectiveness, case studies of the proposed scheduling scheme under three different index weighting coefficients are compared in Table 5. Small values of λ2 and λ4 represent strong preferences of using PCC in power ramping in the intraday and control-perceptive scheduling layers, respectively. The PCC power adjustment contribution rates under three cases are shown in Fig. 14. Case 1 applies the biggest values of λ2 and λ4 in the scheduling, which imposes severe penalty for the participation of PCC in Table 5 Key operating performance indices of the scheduling under different power adjustment contribution rates of PCC. Cases Value of λ Tracking offset of power output Average CO2 capture level Case 1 λ2 = 10; λ4 = 10 λ2 = 10; λ4 = 0 λ2 = 0.05; λ4 =0 88.37 MWh 81.6 % 70.10 MWh 65.43 MWh 81.8 % 81.8 % Case 2 Case 3 Fig. 14. The PCC power adjustment contribution rates in intraday and control-perceptive layer scheduling under three cases. 14 H. Xi et al. Fuel 331 (2023) 125695 Fig. 15. Participation of PCC on (a) power output ramping performance and (b) set-points of CO2 production rate in three cases. 5.3. The superiority of proposed control structure in the scheduling scheme acceptable performance in the capture-level following. The goal to enhance the power ramping performance cannot be focused in the scheduling, which overshadows the flexibility of the PCC unit. Fig. 17 also illustrates that although CO2 capture level is not directly controlled in the proposed PCC control system, it shows a highly synchronous variational trend with the conventional control. Therefore, such a PCC control system can better serve in the proposed scheduling scheme for power adjustment to support the short-term RES accommodation. All the scheduling schemes compared in Sections 4 and 5 are sum­ marized in Table 6, which quantitatively illustrate the superiority of the proposed scheduling scheme. The real-time operation performance of the CFPP-PCC under the two control strategies visualized in Fig. 8 is compared in Fig. 17. The pro­ posed PCC control system uses reboiler steam flowrate to control the CO2 production rate. The CO2 production rate instruction issued by the scheduling can cause a rapid and smooth regulation of reboiler steam flowrate, which is a benefit for the power adjustment of CFPP. There­ fore, the proposed control structure shows better power tracking per­ formance as can be observed in Fig. 17. On the other hand, the conventional PCC control system [16,26] uses the solvent circulation rate to control the CO2 capture level and the reboiler steam flowrate to stabilize the reboiler temperature. The issued CO2 capture level in­ struction can cause a long-term variation of reboiler steam flowrate due to the slow dynamics of the PCC. Such a feature causes the control dif­ ficulty for the CFPP, because the coal mass flowrate has to be continually altered to compensate the influence of reboiler steam on the power output. Therefore, poorer power ramping performance is observed with the conventional PCC control system, which results in 11.16MWh higher power tracking offset compared with the proposed control structure. In addition, because the CO2 capture level is difficult to be controlled within the 5-min scheduling interval, great concern on the CO2 capture level has to be given in the control-perceptive scheduling to attain an 6. Conclusion This paper proposes a complete and practical scheduling scheme for the operation of integrated coal-fired power plant-carbon capture sys­ tem, in which three hierarchical scheduling layers with different time­ scales are incorporated to fully exploit the decarbonization and flexibility of carbon capture technology. The upper layer of the sched­ uling hierarchy utilizes the flexibility of carbon capture on the hourly scale to optimize the economic performance of the integrated plant in the next 24 h; while the middle and lower layers exploit the flexibility of carbon capture on minute timescale to unlock superior power ramping capability of the power plant. Moreover, a control-perceptive scheduling 15 H. Xi et al. Fuel 331 (2023) 125695 Fig. 16. Real-time operation results under dynamic scheduling and steady-state scheduling: (a) power output, (b) CO2 production rate. 16 H. Xi et al. Fuel 331 (2023) 125695 Fig. 17. Real-time operation results under different PCC control structure: (a) power output, (b) CO2 capture level. Table 6 The summary of comparison results. Proposed Conventional Case 2 in Section 5.1 Case 3 in Section 5.1 Steady-state scheduling in Section 5.2 Conventional control in Section 5.3 PCC power adjustment contribution rate Dynamic scheduling Control structure Tracking offset of power output (MWh) Average capture level (%) High Not applied Medium Low High ✓ × ✓ ✓ × Proposed Conventional Proposed Proposed Proposed 65.43 103.36 70.10 88.37 77.50 81.8 81.4 81.8 81.6 81.7 High ✓ Conventional 76.59 82.0 is developed for the lower layer to make the scheduling instructions more feasible for the operating practice; and a novel PCC control system is also presented to better support the power adjustment of CFPP in the proposed scheduling framework. The case study results show that better power ramping and economic performance can be achieved for the in­ tegrated CFPP-PCC system under the proposed scheduling framework. On the premise of maintaining a satisfactory CO2 capture performance, 36.7 % of the supply–demand mismatch caused by power tracking offset can also be eliminated, with 19.6 MWh of renewable power accommo­ dated over the 24 h. This paper points to the new scheduling approach for the economic and flexible low carbon operation of the power plant- carbon capture system in multiple timescale, which is beneficial for the deployment of PCC technology in the context of increasing renewable energy penetration. CRediT authorship contribution statement Han Xi: Conceptualization, Methodology, Investigation, Software, Writing – original draft. Mingjuan Zhu: Methodology, Validation, Software. Kwang Y. Lee: Writing – review & editing. Xiao Wu: Conceptualization, Methodology, Validation, Writing – review & edit­ ing, Funding acquisition. 17 H. Xi et al. Fuel 331 (2023) 125695 Declaration of Competing Interest [7] Bernhardsen IM, Knuutila HK. 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Computational Optimization and Applications 2003;24(2–3):187–206. The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper. Data availability Data will be made available on request. Acknowledgements The authors would like to acknowledge the National Natural Science Foundation of China (NSFC) under Grant 51976030, Natural Science Foundation of Jiangsu Province for Outstanding Young Scholars under Grant BK20190063, National Key R&D Program of China under Grant 2021YFE0112800, and EU H2020 Marie Skłodowska-Curie Research and Innovation Staff Exchange Scheme under Grant 101007963 for funding research into this work. Appendix A Table A1 Main operating parameters of the feasible operation region of CFPP-PCC. Points coal mass flowrate (kg/s) reboiler steam flowrate (kg/s) power output (MW) flue gas flowrate (kg/s) solvent flowrate (kg/s) CO2 capture level (%) A0 E0 A B C D E 1 2 3 4 5 1′ 2′ 3′ 4′ 75.3 34.2 75.3 75.3 41.9 34.2 34.2 75.3 75.3 34.2 34.2 45.6 75.3 75.3 34.2 34.2 0.0 0.0 40.0 180.0 180.0 124.8 40.0 62.4 164.0 120.8 49.5 50.1 79.0 165.2 117.0 56.4 660.0 300.0 641.3 575.6 279.4 238.6 280.3 631.6 583.6 240.8 274.5 374.9 623.0 582.7 242.5 272.3 556.1 399.9 556.1 556.1 426.6 396.9 396.9 556.1 556.1 396.9 396.9 441.1 556.1 556.2 396.9 396.9 / / / / / / / 250.3 632.7 452.4 200.0 200.0 313.3 588.9 423.7 225.7 / / / / / / / 40.0 95.0 95.0 44.3 40.0 50.0 90.0 90.0 50.0 Appendix B. Supplementary data Supplementary data to this article can be found online at https://doi. org/10.1016/j.fuel.2022.125695. 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