International Journal of Heat and Fluid Flow 44 (2013) 140–154 Contents lists available at SciVerse ScienceDirect International Journal of Heat and Fluid Flow journal homepage: www.elsevier.com/locate/ijhff Visualization and analysis of the characteristics of transitional underexpanded jets Jingzhou Yu ⇑, Ville Vuorinen, Ossi Kaario, Teemu Sarjovaara, Martti Larmi Department of Energy Technology, Aalto University, Finland a r t i c l e i n f o Article history: Received 1 June 2012 Received in revised form 8 April 2013 Accepted 23 May 2013 Available online 25 June 2013 Keywords: Transitional underexpanded jets Shock waves PLIF LES a b s t r a c t Underexpanded jets can be formed when high-pressure gaseous fuel is injected directly into an engine cylinder. In such conditions, shock waves are formed immediately near the nozzle exit. In the present study, the flow structure and turbulent mixing of pulsed jets issuing from a circular nozzle is investigated using acetone planar laser-induced fluorescence (PLIF). By monitoring axial and various radial cross-sections under different injection pressure conditions, different features of gaseous jets are visualized and interpreted. The temporal development of the axial cross-sections reveals three typical jet flow patterns (subsonic, moderately underexpanded, and highly underexpanded) during the injection. These stages are (1) well described with the observed shock structures and (2) noted to take a considerably long portion of the full injection process. The visualizations from the radial cross sections show how the nozzle inflow conditions may influence the primary and the azimuthal (secondary) instability of the jet which influences the turbulence transition process and the mixing process. The results indicate the importance of inner nozzle flow on the flow behavior. For example, systematic asymmetries in the mean concentration fields are observed. In addition to PLIF data, numerical simulations can be used to support the experimental picture of the jet behavior. We give examples of large-eddy simulations (LESs) in order to further explore the behavior of the underexpanded jets. Results show that LES is able to reproduce the basic physics of underexpanded jets. LES and PLIF compare favorably in terms of the barrel shock structures and the description of the normal shocks. LES also provides detailed flow field information including temperature, Mach number, concentration and scalar dissipation rate (SDR). Ó 2013 Elsevier Inc. All rights reserved. 1. Introduction 1.1. Motivation Reducing air pollution and dependence on fossil fuels is crucial for the sustainable development of the conventional internal combustion engines (ICEs). Natural gas (NG), a fuel abundant in nature, is considered as one of the most promising alternative fuels for ICEs (Korakianitis et al., 2011). Among fossil fuels, NG combustion has the lowest level of greenhouse gas emissions along with negligible amounts of suspended particles and photochemical smog promoters (Baratta et al., 2009). Recently, compressed natural gas (CNG) port-injected spark-ignition (CNG-SI) engines have already reached the commercial production stage (e.g., city buses and taxi cars). However, the power output and the emissions of unburned hydrocarbons are limited by the low volumetric efficiency and a fuel short-circuit from inlet to exhaust. To further improve the performance of CNG engine, many automotive engine ⇑ Corresponding author. Address: Puumiehenkuja 5 A, Espoo, FI-00076 Aalto, Finland. E-mail address: jingzhou.yu@hotmail.com (J. Yu). 0142-727X/$ - see front matter Ó 2013 Elsevier Inc. All rights reserved. http://dx.doi.org/10.1016/j.ijheatfluidflow.2013.05.015 researchers believe that CNG direct-injection compression-ignition (CNG-DICI) engine has a great potential to improve the thermal efficiency and to meet the stringent emission regulation limits in the near future (Kalam and Masjuki, 2011; Li et al., 2011; Yu et al., 2013). A major challenge of CNG-DICI engine is the poor ignition performance of NG due to its low cetane number. This problem could be solved by the dual-fuel (DF) concept (Korakianitis et al., 2011; McTaggart-Cowan et al., 2006). Conceptually, NG would be directly injected into the cylinder as a primary fuel and mixed with air. Subsequently, the fuel–air mixture would be ignited by a small amount of pilot fuel with a high cetane number (e.g. diesel fuel). In order to prevent methane slip and to extend the operation range of the engine with high efficiency, it is necessary for CNG-DICI engine to operate with stratified charge by means of late injection strategy. McTaggart-Cowan et al. (2006) reported that CNG-DICIDF engines not only maintain power output and thermal efficiency levels compared to conventional pure diesel fueled engine, but they also reach lower NOx and particle matter (PM) emissions. In addition, it was stated that the improvement in CNG-DICI-DF engines can be obtained by varying the injection pressure of the CNG fuel and diesel pilot fuel. They further investigated the effects J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 141 Nomenclature D L Ma Pe Po Pinj P1 Reexit Xfuel Xdisk Wdisk r a c diameter of the nozzle axial distance of the jet Mach number in-nozzle pressure upstream fuel-supply pressure of nozzle gas injection pressure back pressure Reynolds number at the nozzle exit gaseous fuel mole-fraction Mach disk height width of the Mach disk radial distance from jet axial shock reflection angle passive scalar concentration of injection pressure on the performance and emissions of a heavyduty dual-fuel engine using a diesel pilot ignition with late-cycle direct-injection CNG from 210 to 300 bar (McTaggart-Cowan et al., 2007). Based on the combustion parameters, such as the profiles of in-cylinder pressure and the rate of heat release, they concluded that the combustion process at all operation conditions is restricted by the rate at which the fuel and oxidizer are mixing. Increasing the injection pressure increases both the mass flux of fuel into combustion chamber and the in-cylinder turbulence, resulting in enhanced mixing, reducing combustion duration and increasing peak combustion intensities. Moreover, they pointed out that the effects of injection pressure may vary substantially with the in-cylinder conditions because of the variation of the injection pressure ratio (injection pressure to in-cylinder pressure). Another main challenge of the CNG-DICI-DF engine is that there is only a very short time for the mixture formation. Thereby, the period of fuel injection can only take 5–10 ms. One of the key questions concerns improving and understanding the mixing efficiency in a CNG engine. In general, when a gaseous fuel is directly injected into the cylinder of an engine, it forms transient turbulent jets that are typically underexpanded jets with strong shock waves near the nozzle exit (Hill and Ouellette, 1999; Ouellette and Hill, 2000). These shock waves can significantly influence the downstream flow field. In the context of DI gas engines, high-resolution imaging of pulsed underexpanded jets has not, to our best knowledge, been previously carried out using the PLIF technique. Thereby, the objective of this work is to gain an in-depth understanding on the characteristics of pulsed turbulent jets in CNG-engines, and to explore the effects of shock waves on the downstream flow structures and the turbulent mixing. This is accomplished by using a planar laserinduced fluorescence (PLIF) technique. Hiller and Hanson (1988), Hiller and Hanson (1990) and Lemoine and Leporcq (1995) have demonstrated the measurement of density and pressure fields of underexpanded flow using the PLIF technique. However, they only focused on the steady flow, and did not give high-resolution flow field images including shock waves phenomena. In the case of high pressure pulsed turbulent jets related to DI gas engine, previous studies have used PLIF technique to study the characteristics of high pressure gas jet in a constant chamber and in optical engines, but they focused more on the macroscopic structures of the jet (e.g., jet penetration), and they did not refer to the shock wave phenomena (Bruneaux, 2002; Bruneaux et al., 2011; Rubas et al., 1998; Salazar and Kaiser, 2009, 2010). In addition to PLIF, we end the paper by showing high-resolution images from gas jet simulations in order to complement the experimentally obtained picture. In particular, we demonstrate the power of large-eddy simulation (LES) t td x, y, z c le qe q Dc Dref Ve v vref jet time injection duration position variables in jet ratio of specific heat dynamic viscosity in-nozzle gas density gas density mixture fraction diffusivity reference diffusivity in-nozzle gas velocity scalar dissipation reference scalar dissipation as a numerical diagnostic tool to give information on e.g. the jet temperature and concentration fields as well as the scalar dissipation rates. 1.2. High-pressure jets in the DI gas engine Theoretically, when a gas jet is injected through a circular converging nozzle into another gaseous medium, the maximum mass flow occurs when the velocity at the nozzle exit equals the speed of sound. Under such conditions, the inner nozzle exit pressure (Pe) is always higher than the back pressure (P1), the flow is choked and it becomes underexpanded. Assuming a choked flow and an ideal gas that flows isentropically through the nozzle exit, the pressure ratio between upstream fuel-supply pressure of nozzle exit (P0) and the in-nozzle pressure (Pe), can be defined as (Heywood, 1988): Pe ¼ P0 2 cþ1 c c1 ð1Þ For a polytropic gas, the ratio of specific heats (c) is constant (c 1.4). The critical pressure ratio (Pe/P0) is approximately 0.528. For a subsonic jet Pe always equals to P1, so Pe/P1 1.89. Thereby, at high injection pressures the flow can become choked very easily during the injection. At underexpanded conditions, the shock waves can be formed immediately near the nozzle exit. A vast amount of work has been done to investigate the characteristics of the underexpanded free jets in the past years. Most of these studies are related to the aerospace applications, in particular jet aircraft and rocket propulsion systems (Crist et al., 1966; Donaldson and Snedeker, 1971; Ewan and Moodie, 1986; Otobe et al., 2008). According to the previous studies, a free jet usually has three major variations of the flow pattern (subsonic, moderately underexpanded and highly underexpanded), mainly depending on P0/P1. In aerospace applications supersonic jets are usually considered to be steady state jets since the injection periods are very long (typically hours). In contrast, the high-pressure pulsed jets in the engine related field are much more transient since the injection period can be of the order of 1–10 ms. For pulsed jets in the direct-injection (DI) gaseous fuel engine, due to the high compressibility of the gas and the variation of the in-cylinder pressure (or back pressure P1), P0/P1 may also vary significantly during the gas injection. Hence, the jet behavior is more complicated and transient in engine applications than under steady state conditions. Only a few studies have provided detailed information on high pressure pulsed jets in gas engines. Hill and Ouellette (1999) investigated the effects of injection pressure ratio on the penetration in 142 J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 a fixed volume chamber using the Schlieren technique, and they developed an analytical relationship for jet tip penetration based on self-similar characteristics of transient turbulent jets. Rubas et al. (1998) examined the natural gas direct injection and mixing in an optical engine using planar laser-induced fluorescence (PLIF) technique. The injection pressure was 180 bar and cylinder pressure as high as 20 bar was used to match the in-cylinder density during the injection in a firing engine. Recently Salazar and Kaiser (2010) also used PLIF technique to study the mixing process in an optically accessible DI hydrogen engine with high pressure injection (80–116 bar). They found that both the tumble flow and nozzle designs can influence the mixture formation and distribution. Baert et al. (2010) visualized the transient jets using planar laser sheet Mie scattering (PLMS) and measured the jet flow field using particle image velocimetry (PIV). The jet penetration and jet angle were investigated under different injection pressure ratios (15– 40 bar). More recently, the effects of the injection pressure on the mixture formation were also reported by Roy et al. (2011) and Bruneaux et al. (2011) using different optical techniques. Nearly all of the previous studies focused only on the macroscopic characteristics of the jets (e.g., jet penetration and jet cone angle). In contrast, only little attention has been put on detailed investigations on the shock wave patterns and their connections to the mixture formation. Actually, the flow in the near-field region can significantly influence the downstream flow structures and turbulent mixing, in particular for the underexpanded jet, since the jet angle can be increased by the expansion shock waves, but also the jet turbulence can be enhanced by the shock-induced instability. Therefore, the detailed information of the near-field region is crucial for the complete understanding of jet mixing in a DI gas engine. has the ability to capture the characteristics of the high speed turbulent flow (Eckbreth, 1996). The basic principle of PLIF is based on the excitation of tracer molecules within the laser sheet. Consequently, electromagnetic radiation is emitted when the molecule returns back to a lower energy state. Almost all aliphatic hydrocarbons, forming also the major part of combustion fuels, are transparent within the spectral range of interest and therefore do not give any fluorescence signal. Thereby, the tracer used in PLIF usually plays an important role in PLIF measurement system, in particular in the mixing process of non-reacting flows (Schulz and Sick, 2005). Acetone is a well-known and widely used fluorescent tracer. Lozano et al. (1992) confirmed the linearity of acetone fluorescence emission as a function of both incident laser intensity and acetone partial pressure in the constant temperature and pressure nonreacting flow field. A detailed account of the photo-physics of laser exited acetone fluorescence can be found in the reference (Thurber, 1999). Here, we describe results from a 3-year project concentrating on gaining an in-depth understanding on physics of fuel jets in natural gas engines. In particular, the project aimed at using the standard acetone PLIF technique and numerical simulations together as complementary techniques supporting each other. Thereby, the present paper has several objectives. First, we aim at analyzing gaseous fuel jet characteristics in gas engine applications. In particular, this task is to be completed using a measurement system based on the acetone PLIF technique. Second, we aim at providing information on the transient stages and shock development times of the gas jets. Third, the aim is to provide information to jet modelers on the practical matters (e.g. asymmetric features) present in real jets. Fourth, the aim is to demonstrate the usage of LES as a promising diagnostic tool to complement any experimental data on underexpanded jets. 1.3. Laser-based diagnostics for high pressure jets With the development of laser and imaging technology, a number of non-intrusive optical techniques, such as laser Doppler velocimetry (LDV) and particle image velocimetry (PIV), planar laser sheet Mie scattering (PLMS) and phase Doppler particle anemometry (PDPA), have been used to investigate the flow field (Eckbreth, 1996). These optical techniques rely on seeding the flow with small particles (or droplets) and observing the motion of those particles. Thereby, they are very suitable for liquid fuel sprays which naturally contain small droplets in the flow field. With particle seeding, these techniques can be suitable for investigating the low speed gas flows (for example, in-cylinder flow and low pressure gas jets) as the seeding particles can follow the low speed flows very well and represent the true fluid physics. However, the particle-based optical techniques are not efficient for the high speed gas flow, especially for the highly underexpanded jets. First, the particles may not follow such high speed and high frequency containing flow because of the limitation of the response of the seeding particles to the rapid changes of velocities across shock waves. Second, particles cannot be used to observe smallscale structures, since the particle seeding density is limited by secondary scattering, sampling ambiguities, and coherent scattering effects (Miles and Lempert, 1997). In fact, there are two well-known non-intrusive and non-particle seeding flow-field image techniques, the Schlieren technique and the shadowgraphy technique, to visualize the structure of underexpanded jets (Settles, 2001). Based on the index-of-refraction effects, the general profile of shock waves can be observed with these two optical techniques. However, the main limitation of these two techniques is that the obtained two-dimensional images are integrated across the whole flow field, which means that the inner flow structure cannot be observed. As a non-intrusive non-particle seeding laser-sheet based optical technique, PLIF 2. Experimental setup 2.1. Experimental setup and conditions The experimental setup is shown in Fig. 1. It consists of three major parts: the gas supply and the tracer seeding system, the gas injection system and the optical measurement system, as shown in Fig. 1a. For safety reasons, the injected gas is nitrogen instead of natural gas. This approximation is considered to be adequate since the two gases have very similar properties in the present conditions. A flow capacitor is connected to the injector to weaken the fluctuations of injection pressure during the injection. The volume of the capacitor is approximately 1 l. The injection pressure can be flexibly controlled and adjusted by a pressure regulator near the high-pressure nitrogen bottle. A photograph of the experimental setup and the gas injector is shown in Fig. 1b. The solenoid valve gas injector has a single nozzle hole with diameter D = 1.4 mm. The typical needle fully opening time is about 0.4 ms. As mentioned earlier, the jet behavior is mainly dependent on the ratio P0/P1. However, it is very difficult to directly control P0/ P1 in high pressure pulsating gas jets for two reasons (1) the needle lift-off time is relatively long (0.4 ms) and (2) the pressure losses inside the nozzle are significant (50%). Hence, in the present experimental study we focus on controlling the jets using Pinj/ P1 rather than P0/P1, since P0 has a close relationship with the initial injection pressure Pinj which can be flexibly adjusted by a gas regulator. During the experiment, Pinj is adjusted from 5 bar up to 40 bar while the chamber pressure (P1) remains constant as ambient pressure (1 bar). Thereby, Pinj/P1 corresponds from 4 to 40 and it can cover almost the whole range of a high pressure DI gas engine. In addition, the injection duration is fixed to td = 4.0 ms for the all the experimental cases. This time is comparable to J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 143 Fig. 1. Experimental setup for the pulsed jets measurement using PLIF technique. (a) Schematic diagram of experimental setup. (b) Photograph of the experimental setup and the gas injector tip (D = 1.4 mm). typical injection durations in practical applications. During the injection time the transient stages of the jets were captured and all the jets were noted to reach eventually steady flow conditions. 2.2. Tracer seeding As mentioned previously, acetone is a widely used as a tracer for the PLIF measurement. Since acetone is liquid phase at room conditions, it should be vaporized and homogeneously mixed with the carrier gas before injection. A normal way for acetone seeding is that the carrier gas is introduced at the bottom of the acetone vessel through small holes, and the acetone vapor is formed as the bubbles are rising through the liquid acetone. However, the major disadvantage of this approach is that the acetone seeding rate cannot be flexibly controlled. Since acetone has high volatility and high vapor pressure, it can be evaporated rapidly into these bubbles. Cody and Lester (2011) examined the evaporation of a dual-stage acetone bubbling system, comprising two seeding vessels. It was found that essentially all evaporation takes place in the first seeder for the lower flow rate, and only under high carrier gas flow rate conditions the first seeder is insufficient to bring acetone to saturation pressure and some of the evaporation takes place in the second seeder. In this study, the acetone vapor can be kept at saturation in the carrier gas nitrogen, which avoids the uncontrolled acetone seeding rate. Since the gas flow rate is very low due to the very short jet duration (4 ms) and very long time interval between injections (10–15 s), the acetone vapor could be efficiently saturated under such conditions, although there is only one seeder in the present experimental step-up. Actually, the saturated acetone vapor in the carrier gas nitrogen has been also confirmed, because very little condensed acetone can be observed in the flow capacitor after the experiment. It is worth to note that the concentration of fully saturated acetone vapor in the carrier gas nitrogen can be significantly varied with the pressure of carrier gas. For example, under room temperature (25 °C), the concentration of acetone saturation vapor is appropriately 30% (by volume) if the carrier gas pressure is room pressure (1 bar). However, the acetone saturation concentration is rapidly decreased (only 0.75% by volume) if the carrier gas pressure is 40 bar. It means that the acetone concentration in the high pressure mixture is quite small, although the acetone vapor is saturated. Nevertheless, based on Dalton’s law, the mass flow rate of acetone should be almost the same under the saturated condition. Hence, the laser energy absorption could be little different under different inlet conditions. Table 1 shows the estimation of the acetone saturation concentration based on Dalton’s law. 2.3. Imaging and data reduction The fluorescence is excited by the 266 nm output of a frequency-quadrupled Quanta-Ray Lab-170-10 model Nd:YAG laser. The laser pulse duration is 8–10 ns and the maximum laser energy is approximately 90 mJ/pulse. Before entering the spray chamber, J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 Table 1 Acetone saturation concentration (by volume) under different conditions. Mixture pressure (bar) Mixture temperature (K) Acetone saturation concentration (by% volume) 1 5 10 20 30 40 295 295 295 295 295 295 30 6 3.3 1.5 1 0.75 the laser beam is expanded into a light sheet using a group of optical lens. The fluorescence signal is detected and recorded by an intensified CCD camera. A Nikon 94 mm f/4.1 lens is associated with the CCD camera. Spurious reflections of the incident laser light are filtered out by an UV filter (300–450 nm) prior to imaging, and the image intensifier gate (8 ns) is used to minimize the scattered light. For the axial flow structure visualization, the laser sheet goes through the jet center line from jet tip to the nozzle tip (Fig. 1) and the nominal resolution is 43 lm/pixel. For the radial cross-sectional visualization, the laser sheet is perpendicular to the jet axis and the nominal resolution is 25 lm/pixel. The camera is always perpendicular to the laser sheet in both cases. It is worth to mention that an unintensified CCDs can capture finer flow structures (i.e. higher gradients) in mixing zone than the intensified CCD, which is better suitable for quantitative scalar measurement (Gordon et al., 2009). However, unintensified CCDs have in general the major disadvantage that they rely on a (slow) mechanical shutter to block unwanted light, and therefore the shortest exposure times are several orders of magnitude longer than for ICCDs, which routinely are gated for less than 100 ns (Salazar and Halter, 2009). In the present experimental setup, although there is no combustion flame in the jet chamber, the laser sheet lighting the inner wall of the chamber may lead to significant spurious scattered light for the PLIF images resulting from the big gate of CCD. Therefore, it is better to use ICCD in the current PLIF detection system. For the data reduction, the raw instantaneous PLIF images were processed to correct for background scattered light. An average background image which was obtained from 100 instantaneous background images was used for background subtraction. Every instantaneous background image was collected without gas injection but with the same intensification, aperture and laser sheet emission. Then, the corrected images were filtered with a 5 5 Gaussian filter to reduce noise at a minimal cost to image resolution. Finally, these post-processing images which were shown in the present study were individually normalized by their maximum intensity. 2.4. Measurement uncertainty In general, turning PLIF signal intensity into local mixture fraction is a delicate task, in particular for getting the quantitative mixing information, since there are quite many measurement uncertainties in the PLIF measurement system. First, laser absorption along the laser sheet propagation in acetone seeded jet could be an important measurement uncertainty. Gordon et al. (2009) pointed out that the acetone seeding density (or concentration) would significantly affect the laser energy absorption as high as 25% over 1 cm beam path. In order to reduce the laser energy absorption, the acetone seeding densities below 10% was recommended in their study. In the present experiment, the acetone seeding densities is much less than 10% under the mixture pres- sure, as shown in Table 1. Hence, the laser absorption can be relatively low. In addition, according to the results of signal to noise ratios, Gordon et al. (2009) recommended that an intensified relay optics (IRO) intensifier is necessary under such conditions. The second important measurement uncertainty would be from the fluctuation of the shot-to-shot laser energy. A frequency-quadrupled Quanta-Ray Lab-170-10 model Nd:YAG laser is used in the present experiment. The laser output energy (at 266 nm) is set to approximately 90 mJ/shot. Under such conditions, the root mean square (RMS) stability of the laser energy output is about 3.5% for every 50 laser pulses. The laser energy per shot is monitored by an advanced laser energy monitor. In our previous study, the RMS stability was about 2.7% for every 50 laser shots when the laser output energy (at 266 nm) was about 65 mJ/shot (Yu et al., 2012). Although there are shot-to-shot laser energy fluctuations, theoretically the time-averaged of the laser energy should not change too much if there are enough snapshots. As mentioned earlier, previous studies have proven that the intensity of the fluorescence signal is proportional to the acetone concentration (Lozano et al., 1992; Schulz and Sick, 2005; Thurber, 1999). In other words, the total sum of fluorescence intensity (TSFI) should be linearly related to the total gas quantity under the same laser energy. Fig. 2 shows the normalized TSFI with injection time under Pinj/P1 = 10. Results confirm the linear relationship between PLIF signal intensity and the injection gas quantity in the present experiment. The TSFI is based on time-averaged PLIF images with injection time. Every time-averaged image is obtained from 100 snapshots. As can be seen that TSFI linearly increases with the injection time (or injection quantity) after the solenoid valve is fully open when t > 0.2 ms. This is due to that the mass flow rate is almost the same during such a small period time (0.2 ms < t < 0.7 ms) when the flow starts to be choked under Pinj/P1 = 10. Thus, the total injection quantity of the gas is only linearly increased with time. The definition of the injection time t is after the start of injection (ASOI). On the other hand, the mixture density, temperature and pressure fields of the underexpanded jets can vary widely in space and time in the jet core region resulting from the strong shock waves. This causes a very challenging environment to get quantitative mixing information of the underexpanded jet, since the acetonePLIF signal is pressure-dependent and temperature dependent (Narayanaswamy et al., 2010). For example, in the jet core region of the underexpanded jet, the temperature and pressure can be much lower than the ambient conditions. The pressure and temperature dependence of the acetone LIF signal for a 266 nm excitation was determined at low temperature and low pressure Normalized TSFI 144 1.3 1.2 1.1 1.0 0.1 0.2 0.3 0.4 0.5 0.6 0.7 Injection time t (ms) Fig. 2. Normalized total sum of the fluorescence intensity (TSFI) with injection time, Pinj/P1 = 10. J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 145 Fig. 3. Time evolution of the pulsed jet, left column shows instantaneous images and right column is the corresponding time-average images based on 100 instantaneous images, (a) subsonic jet, (b) moderately underexpanded jet, and (c) highly underexpanded jet. (Pinj/P1 = 10 and td = 4.0 ms). conditions by Bryant et al. (2000). The results showed that a 5% variation of the relative acetone LIF signal intensity was observed as the gas pressure increased from 0.1 to 1 bar and 6% as the gas temperature was increased from 240 to 295 K. Therefore, considering these findings, we estimate the effect from the temperaturedependence and pressure-dependence to be relatively small in the current study. 3. Results and discussion 3.1. Evolution of flow structures of the pulsed jet The time evolution of PLIF images of gas jets under Pinj/P1 = 10 is shown in Fig. 3. The left column shows instantaneous images, and the right column is the corresponding time-averaged images. Each time-averaged image is obtained from 100 snapshots. Clearly, the high-pressure pulsed jets cover three typical flow patterns (subsonic, moderately underexpanded and highly underexpanded) at different injection times. Before going any further, it is worth to clarify that since the fluorescence signal is from the excited acetone molecules which are already homogeneously mixed with the gas flow, the fluorescence intensity is proportional to the density of the jet. Moreover, due to the fact there is no fuel–air mixing in the jet potential core region, the color bar only represents density distribution, which has been normalized by its maximum intensity in every case. In the beginning of the jet, the jet is characterized as subsonic, as shown in Fig. 3a. In the subsonic jet (Pe/P1 = 1 and 1 < P0/ P1 < 1.89), a potential core region is quite evident and the length of the potential core is usually very short, only several nozzle diameters. It is surrounded by the turbulent shear layer mixing region which is induced by the Kelvin–Helmholtz instability. Due to the spreading of this mixing region, the potential core no longer exists when its two edges meet each other. Theoretically, there is no viscous turbulent mixing and no mean velocity gradients in the potential core region in the subsonic jet. It is very interesting to notice, however, that the gas density field in the jet potential core region seems to be disturbed when the flow is issuing from the gas injector, as shown in Fig. 3a. Probably the main reason is that the flow in the duct has been disturbed resulting from the solenoid valve of the gas injector. These instability sources can be further amplified during the flow issuing out of the nozzle, which can significantly affect the jet potential core. 146 J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 Fig. 4. Schematic of the near-field of a highly underexpanded jet (a is the shock reflection angle). Over time, once the upstream pressure is built-up enough (Pe/ P1 P 1.1 and (P0/P1 P 2.08), the jet flow is choked and becomes underexpanded. When this choked flow is issuing into the ambient, it expands immediately downstream of the nozzle to equilibrate with ambient conditions. However, the flow may be expanded too far causing the internal pressure to drop lower than the ambient pressure. As a result, the jet flow is compressed or squeezed inward by the surroundings to increase the flow pressure. The oblique shock waves and the ‘shock cell’ structure are formed in this process, as shown in Fig. 3b. In general, the jet with the ‘‘shock cell’’ structure is named moderately underexpanded jet (Donaldson and Snedeker, 1971). Due to the friction and viscosity existing in the actual gas flow, the difference between the internal and external pressure is reduced each time when the flow passes through one of these compression and expansion processes. As a result, the dimension of the shock diamonds is decreased gradually until the jet becomes subsonic. Although the profile of ‘shock cell’ is perfectly clear and smooth in the time-averaged images, it is quite irregular in the instantaneous PLIF images. Probably the reason is that ‘shock cell’ structures are very sensitive, and they can be easily disturbed by the turbulent instabilities in the actual high speed compressible flow. If the upstream fuel-supply pressure P0 is further increased (Pe/ P1 P 2 and P0/P1 P 3.85)), the moderately underexpanded jet will change its characteristics and become the highly underexpanded. Under such conditions, a barrel-shaped shock pattern is formed closed to the nozzle exit, as shown in Fig. 3c. The barrel shock structure is an axisymmetric curved shock produced by the merging of Prandtl–Meyer expansion waves. However, after the supersonic flow passes through the Mach disk, the gas jet becomes chaotic along with the shock cell disappearing. One reason is that the high energy loss causes the jet axial momentum flux to drop sharply (Man et al., 1998). Another reason would be that the Richtmyer–Meshkov (RM) instability may lead to the formation of the turbulent mixing zone after the Mach disk. This will be further discussed in Section 3.5. 3.2. Barrel shock structure and the Mach disk Barrel shock structure plays an important role in downstream flow structure and turbulent mixing. Fig. 4 illustrates the schematic of the barrel shock system in the highly underexpanded jet. Due to the strong expansion and compression waves, the highly underexpanded jet usually has three flow directions near the nozzle exit: outward expansion flow (yellow1 arrows), inward compression flow (green arrows) and parallel flow (blue arrows). The 1 For interpretation of color in Fig. 4, the reader is referred to the web version of this article. expansion waves (parallel flow) are capable of accelerating the flow velocity and decaying the density distribution until to the Mach disk in the jet axial direction. In addition, it is worth to clarify that in a gas jet injection system several pressure levels can be defined, as shown in Fig. 4. Similar as previous study (Donaldson and Snedeker, 1971), three pressure levels P0, Pe and P1 are defined in present study, where Pe depends on P0 and P1 based on Eq. (1). In a real fuel supply system we further define the injection pressure Pinj which is the pressure level provided by the regulator. It is important to note that Pinj is not equal to P0 because of pressure losses inside the nozzle. Fig. 5 shows the evolution of barrel shock structure with time at Pinj/P1 = 17. As can be seen, the first barrel shock structure with weak Mach disk is discerned at t = 0.5 ms. At the same time, the first shock cell is split by the supersonic parallel flow. The barrel shock grows slowly with time due to the increase of P0 while the shock cells disappear almost completely after t = 1.0 ms. After t = 2.5 ms, the barrel shock is fully developed, and the Mach disk height Xdisk stays nearly stable. Table 2 summarizes the evolutions of Xdisk/D, Wdisk/D and the shock reflection angle a under Pinj/P1 = 17. As can be seen, the values of Xdisk and Wdisk are increased simultaneously with the jet time, while the value of a is obviously decreased. This is mainly attributed to the increase of P0/P1. For the pulsed jet, P0 always increases from a low starting to a high later value owing to the high compressibility of the gas and the opening delay of the solenoid valve. P0 can also be considered as the effective injection pressure, which is one of important boundary parameters for gas jet simulation. Hence, it is desirable to obtain experimental information of P0. However, a transducer that is mounted prior to the nozzle hole is intrusive and may interfere with the nozzle flow, and then affect the downstream flow field. Nonetheless, it is possible to effectively estimate P0/P1 based on the information of barrel shock structures. Previous studies show that the Mach disk is one of the most factors specifying highly underexpanded jets, and the Mach disk location is insensitive to the ratio of specific heat, condensation, solid boundary geometry at the nozzle exit, and the absolute pressure level, but it is strongly dependent on the pressure ratio between P0 and P1 (Crist et al., 1966; Maté et al., 2001; White and Milton, 2008). Empirical Eq. (2) provides the relation between P0 and Xdisk (Maté et al., 2001). sffiffiffiffiffiffiffi X disk P0 ¼ 0:67 D P1 ð2Þ Based on Eq. (2), P0/P1 was calculated for different injection pressures, as shown in Fig. 6. Apparently, it can be seen that P0/P1 is much lower than Pinj/P1. Due to the high compressibility of gas flow, P0/P1 is built-up gradually during the injection regardless of the injection pressure levels. The peak value of P0/P1 increases with the increase of Pinj/P1. It can also be seen that the lowest the pressure P0/P1 is about 4 for all the cases, which is very close to the theoretical critical value 3.85 when the jet character changes from moderately under expanded to highly underexpanded conditions (Donaldson and Snedeker, 1971). On the other hand, the Reynolds number is an important parameter to predict whether the flow is laminar or turbulent. For the pulsed jet, the nozzle exit Reynolds number Reexit is always changing because of the variation of the upstream fuel-supply pressure. To calculate Reexit of underexpanded jet, the isentropic and inviscid adiabatic flow in the nozzle was assumed. Reynolds number at nozzle exit can be calculated as: Reexit ¼ qe V e D=le ð3Þ where D, qe, Ve and le are the nozzle exit diameter (m), the gas density (kg/m3), the velocity (m/s) and the dynamic viscosity (Pa s) at the nozzle exit, respectively. The details of Reexit calculation at underexpanded conditions can be found in some references 147 J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 (Anderson, 2003; Wilkes et al., 2005). Fig. 7 shows the effects of Pinj/ P1 on Reexit of fully developed highly underexpanded jets (at t = 3.5 ms). As can be seen that the effects of the injection pressure on the Reexit is remarkable. The order of Reexit is as high as 105. High Reynolds number would be very helpful to enhance the gaseous fuel–air turbulent mixing and mixture formation in the engine cylinder. In other words, higher injection pressure is beneficial to the jet turbulent mixing in CNG-DICI engine. Table 2 Summary of results for highly underexpanded jets (Pinj/P1 = 17). t (ms) Xdisk/D Wdisk/D a (°) 0.5 1.0 1.5 2.0 2.5 3.0 1.36 1.51 1.66 1.71 1.76 1.78 0.29 0.49 0.61 0.69 0.8 0.84 42.4 37.1 35.5 34.5 31.1 28.4 3.3. Visualization of the radial cross-sections For jets issuing from an axisymmetric nozzle, the perturbations can be either axial (longitudinal) or azimuthal (Inman et al., 2008). As a primary instability, Kelvin–Helmholtz waves, the axial perturbations, play an important role in initiating the transition process of the turbulent jets. In general, the primary instability is evident as a train of Kelvin–Helmholtz vortex rings at the sides of the jet in the near-field region. As these vortex rings convect downstream, they develop a secondary instability which manifest itself as azimuthal oscillations on each ring (Nichols et al., 2007). Zaman (1996) pointed out that both the azimuthal and streamwise vortices, which are respectively corresponding to the secondary and primary instability, are of equal importance to jet mixing process, and they are not independent of each other. However, most of the previous studies were focused on steady state flows. Fig. 8 shows the evolution of the time-averaged radial crosssections of the highly underexpanded pulsed jet under different conditions. Fig. 8 gives the cross-sectional visualization of a fully developed highly underexpanded jet at different locations under Pinj/P1 = 20. Obviously, the vortex ring is non-pertabative at the location of L/D = 1, while the star-shaped patterns are clearly discerned at the locations of L/D = 2 and 3 due to the development of the secondary instability. These star-shaped patterns are blurred and become smooth when the jet becomes fully turbulent, for example, at the locations of L/D = 4, 8 and 14. Interestingly, the cross-sectional concentration filed of the jet exhibits rather asymmetric in the far-field region, even though the gas injector used in this study has a round and straight single-hole nozzle. Probably one main reason is that the drilled nozzle hole is not perfect round which can considerably influence on the downstream flow structure. This reasoning would also explain why the realistic jet usually differs from their numerical counter parts. Fig. 9 shows radial cross-sections of the highly underexpanded pulsed jet with injection time at a fixed location (L/D = 3) under Pinj/P1 = 40. It is notable that the star-shaped pattern can be formed rapidly under higher injection pressure ratio. In particular, the star-shaped pattern becomes quite clear after the barrel shock structure is large enough (e.g. t 6 2.0 ms), since the gradual increasing of P0/P1 results in the stronger primary instability and azimuthal oscillations during the injection. Theoretically, the azimuthal oscillation is one of the typical characteristics of the high speed gas flow. Nonetheless, it should be pointed out that although each timeaveraged image is obtained from 100 instantaneous images, the star-shaped pattern is still clearly visualized. It means that the source of instability in every single jet is located in the same positions, regardless of the injection pressure ratio. One main reason would be that surface roughness of the drilled nozzle hole exceeds the boundary layer thickness (106 m), which contributes to the initial perturbations at the same positions and then further similarly affects the primary and the secondary instability during the injection process (e.g., the dashed elliptical region in Figs. 8 and 9). Apparently, a careful design and manufacturing of the inner surface structure of the nozzle hole is important for the gas jet performance. 3.4. Variation of the jet field Due to the strong compression and expansion shock waves, the density variations can be revealed by the fluorescence signal Fig. 5. Evolution of time-averaged PLIF images of highly underexpanded jet in the near-field region (Pinj/P1 = 17 and td = 4.0 ms). 148 J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 region (e.g. L/D = 14), although it is not purely axisymmetric. It indicates that the underexpanded jet has become turbulent and subsonic in the far-field region. 25 20 3.5. Shock wave and turbulent mixing 15 10 5 0 1 2 3 4 5 Injection time t (ms) Fig. 6. Calculated P0/P1 based on the Mach disk distance (Xdisk) under different injection conditions (td = 4.0 ms). 7x105 Reexit 6x105 5x105 4x105 3x105 2x105 10 20 30 40 Fig. 7. Calculated Reynolds number at the nozzle exit (Reexit) at t = 3.5 ms. intensity. Fig. 10a shows the normalized fluorescence intensity of fully-developed underexpanded jets for different injection pressures. The y-coordinate, the fluorescence signal intensity, is nondimensionalized by the peak intensity value of each jet. As a result of the expansion waves close to the nozzle exit, the fluorescence intensity smoothly and rapidly decreases from the nozzle exit until to the Mach disk or the first shock cell, and then rises suddenly resulting from the compression waves. In the case of moderately underexpanded (Pinj/P1 = 7), the oscillation of fluorescence intensity represents the consequence of the repeating expansion and compression oblique shock structure in the jet. At the location of L/D = 10, the jet becomes subsonic and fully turbulent. The decay of the oscillation amplitude is due to the viscous dissipation and the growth of the surrounding mixing layer. Under highly underexpanded conditions (Pinj/P1 = 20 50), when the flow passes through the Mach disk, the fluorescence intensity keeps nearly constant in the downstream field. On the other hand, despite the fact that the variations of the temperature and pressure distribution can cause non-linear relation between fluorescence signal intensity and tracer density, it is somewhat surprising to note that the profiles of the centerline fluorescence intensity coincide with each other very well near the nozzle tip regardless of the injection pressure levels. Fig. 10b presents to the normalized radial fluorescence intensity at different locations under Pinj/P1 = 20. In the jet potential core region (e.g. L/D = 2 and 7), the density variation is high due to the compression and expansion shock waves, while the general trend of the density profiles exhibits almost self-similarity in the far-field In general, for the subsonic flow the shear-induced turbulence plays an important role in the turbulent mixing, while for the underexpanded jet, in particular the highly underexpanded jet, the flow structure and turbulent mixing are not only dependent on the shear-induced turbulence, but also strongly affected by shock-induced turbulence. The shock-induced instability is often called the Richtmyer–Meshkov instability, which arises as a shock wave interacts with an interface separating two fluids with different density. When two different fluids are impulsively accelerated into each other by a shock wave, small perturbations at the interface grow first linearly and then evolve into non-linear structures formed of ‘‘bubbles’’ and ‘‘spikes’’. Afterwards, it may lead to the formation of a turbulent mixing zone (Bai, 2012), which can cause the shock cells disappearing after Mach disk. Usually, both the intersection point (red points) and the shock triple point (green points) shown in Fig. 4 are considered as two main sources of instabilities (Inman et al., 2008). Fig. 11 shows the effects of shock waves on the flow structure and turbulent mixing in highly underexpanded jet under different conditions. Clearly, under higher pressure ratio (e.g. Pinj/P1 P 20), the turbulence takes place immediately after the Mach disk due to the strong Richtmyer–Meshkov instability, and then leads to the turbulent mixing zone. On the other hand, the growth of barrel shock leads to the increase in the jet cone angle in the near-field region, which is very important for improvement of the fuel–air mixing efficiency and mixture spatial distribution. According to the results and discussions in the above sections, the characteristics of the main structures in underexpanded jets can be captured quite well by means of acetone-PLIF technology. However, it is very challenging to quantitatively measure the local mixture fraction in the underexpanded jet due to the wide variation of temperature and pressure in space and time. In order to gain an in-depth understanding in the underexpanded jets which is beyond the capability of the current optical technology, LES is used to further explore the underexpanded jet in the next section. The aim of the next section is to demonstrate the use LES as a diagnostic tool to support PLIF and other experimental techniques in supersonic flow research. 3.6. Large-eddy simulation of underexpanded gas jets 3.6.1. Brief introduction to the present large-eddy simulation Using LES, turbulent flow may be simulated by solving the Navier–Stokes equations with high spatial and temporal resolution (Garnier et al., 2009). Thereby, LES may offer a complete transient 3D visualization of the flow field. In supersonic flows LES potentially resolves the shock structures, acoustic waves, thermodynamic fields and mixing. In fact, LES of supersonic flows is a relatively new research topic which has achieved more attention only recently. During the past 3 years several groups in the field of aeroacoustics have adopted LES as a computational diagnostic tool to support different experimental techniques (Dauptain et al., 2010; Gieseking et al., 2011; Kawai and Lele, 2010; Munday et al., 2011; Vuorinen et al., 2013). The recent studies have mostly focused on moderately underexpanded jets exhibiting oblique shocks in various nozzle geometries (Dauptain et al., 2010; Kawai and Lele, 2010; Munday et al., 2011) or overexpanded conditions (Gieseking et al., 2011). Very recently, highly underexpanded jets were studied using LES in a setup emulating the present experimental conditions (Vuorinen et al., 2013). 149 X fuel J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 Pinj P∞ = 20 X fuel Fig. 8. Visualization of the cross-section of the pulsed jet (time-averaged) at different locations. (Pinj/P1 = 20, t = 3.5 ms, and td = 4.0 ms). Pinj P∞ = 40 (a) 1.0 Normalized fluorescence intensity Normalized fluorescence intensity Fig. 9. The evolution of the cross-section of the pulsed jet (time-averaged) at the fixed location L/D = 3 (Pinj/P1 = 40, and td = 4.0 ms). 0.8 0.6 0.4 0.2 0.0 0 2 4 6 L/D 8 10 12 (b) 1.2 Nozzle 0.8 0.4 0.0 -4 -2 0 2 4 r/D Fig. 10. Variation of normalized fluorescence intensity for different injection pressures, (a) normalized centerline fluorescence intensity, and (b) normalized radial fluorescence intensity at different location. Every profile is based on the time-averaged PLIF image at t = 3.5 ms and td = 4.0 ms. 150 J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 In the present LES we discretize the detailed information concerning the numerical methods and setup of the present LES can be found in the recent study focusing on the computational modeling of highly underexpanded gas jets (Vuorinen et al., 2013). Here, we briefly summarize some of the most important numerical details. In the present LES, a gas jet is formed by modeling a smooth and converging nozzle. The upstream pressure of the nozzle is simulated by taking into account a very large pressure reservoir which forces the jet through the nozzle into the ambient conditions. The Navier–Stokes equations are solved using an explicit, density based Runge–Kutta method with fourth order temporal accuracy. The grid resolution is D/70 in the radial and D/35 in the axial direction offering a good spatial resolution comparable to previous studies in similar flows (Dauptain et al., 2010; Munday et al., 2011; Vuorinen et al., 2013). LES of supersonic flows aims at simultaneous capturing of shock waves and turbulence. These objectives are particularly challenging as resolving the discontinuous shock waves requires robust numerics (typically reduction of the spatial accuracy to first order) with high level of dissipation whereas turbulence should be treated with non-dissipative discretization schemes (at least second order spatial accuracy) (Grinstein et al., 2007). In the present LES we discretize the convection terms using a second order accurate scale-selective filtering procedure that was recently developed, tested and validated for LES by Vuorinen et al. (2012). The third order diffusive error of the scale-selective discretization (SSD) scheme acts as a stand-alone turbulence model similar to implicit LES (ILES) and thereby we do not apply an explicit turbulent viscosity (Grinstein et al., 2007). A detailed spectral analysis of the SSD scheme has been given by Vuorinen et al. (2012). In fact, it should be noted that in LES of supersonic jets the ILES approach seems to be the most com- monly used approach as it has been noted to favorably capture the turbulence transition process (Kawai and Lele, 2009). Also the shock capturing needs to be accounted for with a separate model and in the present LES the shock waves are treated with the bulk-viscosity method by Cook and Cabot (2005) which only influences the dilational part of the viscous stress tensor. This approach has become one of the state-of-the-art methods in LES of supersonic flows as the dilational part of the stress tensor is typically assumed to be small in comparison to the symmetric part of the stress tensor (Cook and Cabot, 2005; Dauptain et al., 2010; Kawai and Lele, 2009). To summarize, the present LES has been tailored to involve minimal numerical dissipation while still capturing the supersonic features involving high gradients. Next, we further discuss the present PLIF measurements in the light of present LES. The capability of LES at two different nozzle pressure ratios (P0/P1) is investigated using a simulation model detailed earlier by Vuorinen et al. (2013) who used the model in highly underexpanded conditions. Here, we carry out two simulations: one at moderately underexpanded conditions (P0/P1 = 3) and one at highly underexpanded conditions (P0/P1 = 5.5). 3.6.2. Comparison of PLIF and LES near the nozzle exit It should be noted that Pinj in experiments and P0 in the present LES are not equal due to pressure losses in the injector. Thereby, P0 in experiments is not known whereas in LES it can be controlled by the boundary condition in the pressure reservoir. One way to compare PLIF and LES with each other is to use the empirical Eq. (2). For a PLIF case with injection pressure Pinj/P1 = 15 the Mach disk height is noted to be about 2.39 mm for which Eq. (2) gives P0/ P1 = 6.5. The PLIF image is captured under a quasi-steady jet (t = 9 ms, td = 10 ms) with constant Pinj/P1 = 15. Under such Pinj P∞ = 5 Pinj P∞ = 10 Pinj P∞ = 10 Pinj P∞ = 20 Pinj P∞ = 20 Pinj P∞ = 30 Pinj P∞ = 30 Pinj P∞ = 40 Pinj P∞ = 40 X fuel Pinj P∞ = 5 Fig. 11. Effects of injection pressure on the jet structures and turbulent mixing process in highly underexpanded jets at t = 3.5 ms. td = 4.0 ms. 151 J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 conditions, the underexpanded jet is fully developed and the upstream pressure of the gas supply P0 can be considered as steady state. Thereby, in order to compare LES and PLIF we need to compare the experimental case Pinj/P1 = 15 and LES case P0/P1 = 6.5 with one another. Fig. 12 shows the comparison between timeaveraged LES (upper half) and time-averaged PLIF (lower half) in the near nozzle region. It is noted that the basic aspects of the underexpanded jet are well reproduced by LES including (1) the location of the Mach disk and (2) the angle and shape of shock reflection. However, a meaningful quantitative comparison is not possible as there are several differences between the two results. For example, in reality the inner nozzle boundary layers are very thin and thereby they are left unmodeled in LES. Thus, the inflow condition in LES is laminar whereas in PLIF it is likely to be transitional which results in obvious differences already at the inlet. However, as shown previously, a very good agreement between LES and PLIF may be observed for the number of shock cells and general flow topology (Vuorinen et al., 2013). 3.6.3. Effects of injection pressure ratio on the underexpanded jet Fig. 13 shows the temperature field of the fully developed underexpanded jets. The left side shows a jet under moderately underexpanded at nozzle pressure ratio P0/P1 = 3 and the right side shows a highly underexpanded jet at P0/P1 = 5.5. As was mentioned previously, the temperature varies widely in the underexpanded jet in time and space due to the strong expansion of the supersonic flow. This phenomenon can be clearly captured in the temperature field in Fig. 13a. With the increase of P0/P1 from 3 to 5.5, the variation of the temperature field is obviously increased, as shown in Fig. 13b. The minimum temperature is of the order 160 K, which is observed in the intersection point of the oblique shocks at P0/P1 = 3, and the temperature fluctuations have almost disappeared after 10D. At P0/P1 = 5.5, the minimum temperature decreases rapidly to 100 K, and visible temperature fluctuations exist even as far as 20D. The position of the minimum temperature is pointed by the white arrow in Fig. 13a and b, respectively. The Mach number (Ma) is a very important parameter of the supersonic jet flow field. However, it is not possible to measure Ma in the flow field using PLIF technology. Furthermore, such complicated velocity flow field cannot be accurately measured even by PIV either (Miles and Lempert, 1997). Based on LES, Ma can be efficiently captured. Fig. 14a and b display the velocity field (indicated by Ma) of the underexpanded jet under different inlet conditions. Due to the intensive expansion and compression shock waves, the velocity varies strongly between supersonic and subsonic values in the near field of the jet. The maximum Ma is approximately 2 when P0/P1 = 3, while Ma is increased to 3 under P0/P1 = 5.5. The position of the maximum Ma is pointed by the white arrows in Fig. 14a and b, respectively. Additionally, it is noted how the stagnation conditions are approximately met inside the shock cells as expected. Fig. 14c and d demonstrate the concentration (qc) normalized with the inlet value in the underexpanded jets at P0/P1 = 3 and 5.5, respectively. Here, c is a passive scalar that is used to visualize and study mixing similar to acetone concentration in PLIF (Vuorinen et al., 2013). In addition to temperature and Mach number fields, the passive scalar field reveals additional details concerning the mixing. For example, the fine resolution LES captures vortex instabilities resembling the classical Kelvin–Helmholtz waves in the shear layers of the jets. There are clear differences in the formation of the vortex structures. For example, the moderately underexpanded jet exhibits a symmetric vortex pattern whereas an antisymmetric, helical vortex structure forms for the highly underexpanded jet (Vuorinen et al., 2013). It is important to (1) note the ability of LES to capture the presence of these structures and (2) note that the structures were not seen as clearly for PLIF. These Fig. 12. Comparison between time-averaged LES (upper half) and time-averaged PLIF (lower half) of the underexpanded jet. examples provide evidence on the ability of LES to capture fine scale details of moderately and highly underexpanded jets thereby supporting the experimentally obtained picture. We note that, despite the obvious similarities, the LES and PLIF results differ to some extent. In LES, the transition to turbulence begins visibly after the Mach disk in the form of the shear layer instability. In contrast, in PLIF some flow exists already outside the barrel shock which can be explained by the flow being turbulent/transitional in the experiments already at the nozzle exit. In LES the nozzle exit condition is laminar which explains the differences. The observed asymmetries in the experiments (see e.g. Fig. 11) also imply that the scalar fields may be even asymmetric in practice. A possible explanation to this anomaly could be the inner nozzle surface roughness. In other words, the boundary conditions are crucial for LES of underexpanded jets to obtain results close to the experiments. 3.6.4. Scalar dissipation rate of underexpanded jets Scalar dissipation rate (SDR) is typically used to estimate high concentration gradients and estimate the local mixing activity of the flow field. It is particularly important in combustion applications because it is fundamentally related to the structure of turbulent non-premixed flames and appears directly or indirectly in most turbulent combustion models (Frank and Kaiser, 2007; Gordon et al., 2009; Wang and Barlow, 2007). The scalar dissipation is defined as v (Pope, 2000) v ¼ 2Dc " @c ax 2 @c þ @y 2 2 # @c þ az ð4Þ where Dc is the mixture fraction diffusivity; c is the passive scalar concentration; x, y, z are the position variables of the jet. It is noted from Eq. (4) that the definition of scalar dissipation is 3d and thereby it can be directly evaluated from the instantaneous LES data as further discussed below. Previous experimental studies on subsonic jets have indicated that SDR exhibits narrow string-like structures where the mixing rate is high (Gordon et al., 2009; Karpetis and Barlow, 2005; Wang et al., 2007a; Wang et al., 2007b). In addition, the previous studies have also indicated that compared to intensified CCDs, unintensified CCDs offer better quantitative scalar measurements because of the lower level of noise (Frank and Kaiser, 2010; Frank and Kaiser, 2007; Kaiser and Frank, 2009). However, the PLIF image captured from intensified CCD can be heavily obscured by the intensifier noise. Therefore, the current experimental PLIF data 152 J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 Fig. 13. Temperature field of LES instantaneous snapshots of quasi-steady underexpanded jets under different inlet conditions. (a) P0/P1 = 3 and (b) P0/P1 = 5.5. Fig. 14. LES of instantaneous snapshots of quasi-steady underexpanded jets under different inlet conditions. Left (a and b) P0/P1 = 3, and right (c and d) P0/P1 = 5.5. may not be suitable for SDR analysis. Here, we use the 3d LES data for visualizing how the dissipation rate structures based on the resolved quantities appear in LES of supersonic jets. Fig. 15a and b shows SDR (log10(v/vref)) of underexpanded jets under P0/P1 = 3 and 5.5 at jet time t = 0.5 ms. Here, v is made nondimensional using the integral scales to define a reference quantity vref = 2Dref(cmax/D)2, where cmax = 1, and Dref is the reference diffusivity in the far-field. Clearly, in the near-field of the jet, the turbulence transition process results in the onset of intense mixing and high-level of SDR. In contrast, in the far field, the SDR decreases as the turbulence has further evolved and mixed the flow. Fig. 15c and d are the corresponding areas of the dashed yellow box in Fig. 15a and b, respectively. The left and right sides of the dashed yellow box are 6D and 13D away from the nozzle exit, respectively. It is noted that the differences between the two underexpanded jets are relatively small. The SDR exhibits narrow, string-like structures which mostly highlight the edges between high and low concentration regions. According to the definition of SDR, high values of SDR indicate that mixing is still incomplete as high gradients exist. As seen from Fig. 15, it should be noted that SDR varies over roughly 2–3 orders of magnitude. Higher SDR values are seen in the lower pressure ratio case implying stronger concentration gradients which have high potential for further mixing. On the other hand, the higher pressure ratio case exhibits reduced SDR compared to the lower pressure ratio case indicating reduced concentration gradients due to mixing that has already taken place. In general low SDR would imply good mixing as the gradients have dissipated away. Hence, these results point to the direction where a higher P0/P1 would imply a better mixing. It is a highly interesting question how to really use this kind of detailed data for mixture quality analysis. For example, future studies could involve tailoring the objectives for good mixture quality in DI CNG engines based on LES data such as that presented in Fig. 15. Last, it is noted that any LES may only offer an approximation of SDR based on the resolved scalar fields. For example, as the scalar gradients are eventually determined by the Batchelor scales, the quantitative value of SDR is likely to depend to some extent on the grid resolution in any practical LES. Similar problems occur also in experiments as capturing the smallest flow scales depends on the pixel size in addition to background noise and other measurement errors. One of the advantages of the present LES is that the simulations are carried out on a relatively fine grid where the scale-selective implicit filtering acts as a stand-alone turbulence model similar to ILES (Grinstein et al., 2007). Using the ILES approach has been common in previous literature for supersonic flows (Kawai and Lele, 2009; Munday et al., 2011). Thereby, we note that the results of Fig. 15 are not influenced by an explicit subgrid scale turbulence model. Instead, as previously explained, the turbulence is modeled by the higher order dissipative terms of the truncation error of the SSD scheme (Vuorinen et al., 2012). We note the similarity between the relatively clear string-like structures of SDR for supersonic jets as has been previously noted for reacting flows in the literature (Frank and Kaiser, 2010; Kaiser and Frank, 2011). In addition, to our best knowledge, such SDR structures of supersonic jets have not been previously reported in the literature. 4. Conclusions This work has been motivated by our attempt to develop CNG direct-injection compression-ignition (CNG-DICI) dual-fuel engines with high efficiency and low emissions. In general, shock waves can be formed immediately when the gaseous fuel with high pressure ratio is injected into the cylinder. It is highly important to gain an in-depth understanding of the jet mixing to develop such kind of CNG engine. For this purpose, the experimental study of high-pressure pulsed jets based on planar laser-induced fluorescence (PLIF) was carried out in a constant-volume vessel under different injection pressure ratios. In order to better understand the characteristics of underexpanded jets, LES was further used in the present study. The main findings of this work are summarized as follows. First, the standard acetone PLIF visualization could be used to capture J. Yu et al. / International Journal of Heat and Fluid Flow 44 (2013) 140–154 153 Fig. 15. The effect of inlet conditions on the scalar dissipation rate of underexpanded jets at t = 0.5 ms. (a) P0/P1 = 3.0, (b) P0/P1 = 5.5, and (c) and (d) are the enlarge area of the yellow box in (a) and (b), respectively. (For interpretation of the references to color in this figure legend, the reader is referred to the web version of this article.) the average concentration fields in jets which can already reveal very useful information on the transient and average features of the jets. Second, the results revealed that pulsed jet in DI CNG type applications at high pressure ratios contain three typical flow patterns: subsonic, moderately underexpanded and highly underexpanded in the jet core region. Importantly, all these stages are long-lasting in comparison to the duration of injection and thereby the present jets are also highly transient. Third, the results indicate that realistic gas jets in DI CNG type engines may involve asymmetric features. The visualizations of the radial cross-section identify that the azimuthal instability which is the development of the primary instability exists in the highly underexpanded jet. Surprisingly, the star shaped pattern can still be clearly discerned in the time-averaged images, although the gas injector is circular. The main reason would be the surface roughness of the drilled hole which exceeds the boundary layer thickness (106 m), which contributes to the initial perturbations at the same positions and then further similarly affects the primary and azimuthal instability in the realistic gas jet. Hence, the careful design and manufacturing of the nozzle would be important for the physical characteristics of the jets. Considering this together with the transient nature of the jets poses a significant challenge to modelers since the observations point to the direction where also the flow inside the injector needs to be modeled. Fourth, we demonstrated the capability of LES to capture flow features of transient underexpanded jets which are out of the reach of any experimental configuration. 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