This article has been accepted for publication in a future issue of this journal, but has not been fully edited. Content may change prior to final publication. Citation information: DOI 10.1109/TMAG.2017.2712860, IEEE Transactions on Magnetics FF-07 1 Improved efficiency of tapered magnetic flux concentrators with double layer architecture J. Valadeiro1,2, D.C. Leitao1,2, S. Cardoso1,2, P.P. Freitas1 1 INESC-MN - Instituto de Engenharia de Sistemas e Computadores –Microsistemas e Nanotecnologias, 1000-029 Lisboa, Portugal 2 Physics Department, Instituto Superior Técnico, Universidade de Lisboa, Lisboa 1049-001 Portugal Being able to increase the sensitivity of magnetoresistive sensors, by orders of magnitude, provides a route towards challenging detection levels and opens the way for new applications. This work describes a novel architecture of magnetic flux concentrators to achieve an improved guiding efficiency, combining materials with different magnetic properties and a vertical tapering. The novelty consists in the concentration of the magnetic flux kept by the entire structure in a reduced cross section area within the vicinity of the spinvalve sensor. Depending on the configuration of the double layer magnetic flux concentrators, average sensitivity gains of ~ 90x and ~ 400x were obtained. This enhanced guiding efficiency also reduced the impact of a misalignment between the device sensing direction and the applied magnetic field, since the device performance is not compromised until a misalignment angle = 45º. This further stabilization may arise from the vertical tapering of the magnetic flux concentrator, being consistent with 2D finite element simulations. Index Terms — magnetoresistive sensors, magnetic flux concentrators, sensitivity gain, vertical tapering I. INTRODUCTION R heads industry have had a major role in the development of soft magnetic materials technology, broadening its applicability from magnetoresistive (MR) sensors shielding to magnetic flux concentrators (MFCs) in recessed read heads [1]. MFCs patterned with an appropriate geometry concentrate the external magnetic field in the sensor region, resulting in a sensitivity improvement and a consequent enhancement of the minimum detection level. The effective gain is defined by the ratio between the magnetic field in the sensor region and its external value, depending on geometrical parameters (e.g. MFCs dimensions) and magnetic properties of the material (e.g. relative magnetic permeability) [2-6]. The integration of MFCs is a reliable alternative for low-field sensing applications when the device footprint is not an issue. Biomedical applications [7] and highly sensitive microscopy tools [8] offer many opportunities for ultra-low magnetic field detection, where detection values in sub-pTesla range are required. The inclusion of MFCs on MR sensing elements increases their sensitivity values in more than one order of magnitude, with a direct enhancement of the minimum detection level. This strategy makes MR sensors competitive for such low field detection applications, not requiring cryogenic operating temperatures as in SQUIDs. Sensitivity gains of MR sensors up to 30 times have been reported for single layer MFCs patterned with funnel shape and a steep profile (90o) at the gap region [6], while a maximum sensitivity enhancement of 100 times was obtained using the same geometry with a 3D tapered profile (45o) [9][10]. In the former process, the thickness difference between the MFC structure (~500 nm) and the spinvalve sensor (~30 nm) limits the amount of magnetic field kept by the sensing element since the majority of the concentrated flux does not reach the sensor. Besides the larger gain, the latter EAD process requires the etching of 0.7 m thick of CoZrNb in the gap region, demanding an accurate end-point control, otherwise it damages the sensing elements and results in a small fabrication yield. None of the presented examples of MFCs address a statistical study about the reliable reproduction of the devices or the dispersion of the reported sensitivity gains. This work proposes a novel MFC architecture with a vertical tapering designed to achieve an improvement of the magnetic flux concentration efficiency in the gap region, to devise extremely sensitive magnetic detection tools. The double layer MFC architecture combines materials with different magnetic properties, with steep and vertical tapered profiles. This strategy envisages the concentration of the magnetic flux kept by the entire MFC structure (large thickness at the entrance) in a reduced cross-sectional area in the sensor region (thinner MFC structure at the pole). Average sensitivity gains of ~90x and ~400x were obtained depending on the double layer MFCs spatial configuration. Still, an accurate control of the sensor operation point is required to take advantage of such sensitivity enhancement. The use of MFCs as a strategy to reduce the misalignment impact between the external field and the device sensing direction was also addressed. II. EXPERIMENTAL METHOD The MFCs structure consists of: (i) a 100 nm layer of Ni80Fe20 defined by ion milling etch at 45o angle, leading to a tapered profile near the sensor; and (ii) a 500 nm layer of Co93Zr3Nb4 defined by lift-off with a steep profile. The latter is recessed d = 50 or 100 m relative to the Ni80Fe20 pole below. Fig. 1(a) shows a schematic representation of the 0018-9464 (c) 2016 IEEE. Personal use is permitted, but republication/redistribution requires IEEE permission. See http://www.ieee.org/publications_standards/publications/rights/index.html for more information. This article has been accepted for publication in a future issue of this journal, but has not been fully edited. Content may change prior to final publication. Citation information: DOI 10.1109/TMAG.2017.2712860, IEEE Transactions on Magnetics FF-07 2 (a) (b) (d) 1.0 Easy axis M/Msat 0.5 (c) Hard axis 0.0 Msat = 725 kA/m -0.5 Hk = 1.5 mT r = 803 NiFe 100 nm/ CoZrNb 500 nm -1.0 -9 (e) -6 -3 0 3 0.H (mT) 6 9 (f) Fig. 1. (a) Schematic view of the device: top view and cross section, showing the double layer MFCs composition and vertical tapering (NiFe [100 nm] defined with an angle of 45o in the pole region; recessed CoZrNb layer [500 nm] with a steep profile). A 5 m nominal gap was left between the MFCs poles, were the SV sensor is placed. (b) Simulation of the magnetic flux distribution in the CoZrNb – NiFe transition, showing the field kept by the CoZrNb layer drives into the NiFe layer (cross section). (c) Simulation of the magnetic flux distribution in the MFCs gap region, between the NiFe pole and the SV element (cross section). (d) VSM characterization (M(H)) of the double layer materials (bulk) used as MFCs: [buffer/ NiFe (100 nm)/ CoZrNb (500 nm)]. (e)-(f) SEM images of the fabricated devices showing the funnel shape of the patterned MFCs (left) and its vertical profile in the outer width edge (right). device cross section, highlighting the vertical architecture of the MFCs. This configuration allows a MFC thickness reduction in the pole region and increases the flux concentration efficiency in the sensor area since the field kept by the thick Co93Zr3Nb4 is driven into the thin Ni80Fe20 layer, as seen in the simulation of the magnetic flux distribution (fig. 1(b)-(c)). An unpatterned (continuous thin film) sample of the used soft magnetic double layer was characterized by a vibrating sample magnetometer (VSM). A relative permeability r = 803 was obtained together with an intrinsic anisotropy μ0Hk = 1.5 mT, setting the linear M(H) region (H = 2Hk) where the MFCs gain is well controlled (Fig. 1(d)). The NiFe and CoZrNb were deposited under an applied field of 5 and 10 mT respectively, without post annealing. The MFCs were patterned with a funnel shape and a nominal gap distance of 5 m. The NiFe layer has a pole width of 40 m and an outer width (length) ranging from 500-2000 m (2652420 m). The spinvalve (SV) sensors in the gap were deposited by ion beam with the following stack: Ta 2.0/ Ni80Fe20 3.0/ Co80Fe20 2.2/ Cu 2.1/ Co80Fe20 2.5/ Ir24Mn76 6.5/ Ta 10.0 (thickness in nanometer and alloy compositions in at.%). The sensors were defined by optical lithography and ion-beam milling, being patterned in single elements with an active area of 40 x 2 m2. The metallic contacts were done by lift-off of 300 nm-thick AlSiCu films protected by 15 nm thick TiWN layer. The sensors were then passivated with 50 nm of sputtered Al2O3 which also protected them during the ion milling etch required for the MFC first layer definition. After the double layer MFC fabrication, vias for the metallic contacts through the oxide were opened by ion milling etching. Fig. 1(e)-(f) show scanning electron microscope (SEM) images of the fabricated devices, being visible the integration of the SV sensor with the double layer MFCs and its vertical profile. The device transfer curve [MR(H)] was measured using a dc two-point probe method within a field range of ±14 mT and ±200 mT. The Helmholtz coils allowed an accurate MR(H) characterization with a precision down to 3 T/mA. III. RESULTS AND DISCUSSION The MR(H) curves obtained for a SV sensor prior and upon the integration of the double layer MFCs (MR = 8.4 % and Rmin = 520 ) are shown in Fig. 2(a). In the absence of MFCs, the SV sensor exhibits a linear and hysteresis free transfer curve with a sensitivity S = 1.7 %/mT. A. Improved device sensitivity The integration of the double layer MFCs (outer width = 1500 m, d = 50 m) increases the transfer curve transition slope, 0018-9464 (c) 2016 IEEE. Personal use is permitted, but republication/redistribution requires IEEE permission. See http://www.ieee.org/publications_standards/publications/rights/index.html for more information. This article has been accepted for publication in a future issue of this journal, but has not been fully edited. Content may change prior to final publication. Citation information: DOI 10.1109/TMAG.2017.2712860, IEEE Transactions on Magnetics FF-07 0.H (mT) -75 -50 -25 0 8 S = 1.7 %/mT 6 2 Sensitivity gain = 104 x 4 MR (%) 6 4 25 50 75 Hexch = 33 mT SV with double layer MFCs 0 MR (%) -10 -5 0 300 150 SV sensor 2 Hexch = 12 mT (a) 0 -15 8 400x Gain S = 175 %/mT SV sensor 4 450 MR = 8.4 % Rmin = 520 5 10 15 Sensitivity (%/mT) 6 SV sensor with double layer MFCs MR = 8.4 % d = 50 m d = 100 m S = 170 %/mT Gain = 100 x S = 730 %/mT Gain = 430 x 0 800 600 400 200 0 6 4 2 0 2 MFC dimension outer = 1500 m width (b) 0 -0.4 -0.2 90x 8 MR (%) MR (%) 8 3 0.0 0.2 0.4 Fig. 2.(a) Effect of the double layer MFC inclusion in the magnetotransport curve of a single SV sensor. Inset: Influence of the MFCs inclusion in the exchange field of the SV sensor. (b) Detailed view of the obtained curves upon the inclusion of double layer MFCs with different NiFe - CoZrNb separations (d = 50, 100 m). Characterization within [-0.3, 0.3] mT range with 0.01 mT steps. yielding a sensitivity enhancement of 104x (S = 175 %/mT). The observed coercivity of the final device remained unchanged upon the MFCs inclusion (20.Hc ~ 0.3 mT). The coercivity is more notorious upon the MFCs integration as a consequence of the higher measurement precision (0.01 mT steps), while for the isolated SV sensor a coarser characterization was performed (0.2 mT steps). However, M(H) for continuous thin films of NiFe – CoZrNb (unpatterned, fig. 1(d)) indicates a small remanent magnetization at the hard axis. Assuming a similar behavior for the patterned structure, such remanence was previously seen to lead to a field in gap which polarizes the SV sensor [11]. Such effect translates into a shift of both MR curve branches masking the expected reduction in the coercivity of the final device. Despite the coercivity, a correct selection of the curve branch allows the device to operate with a large sensitivity. To evaluate the MFCs effect on the SV element exchange bias field (Hex), a MR(H) characterization in a wider field NiFe - CoZrNb distance: d = 50 m d = 100 m 500 1000 1500 MFCs outer width (m) 2000 Fig. 3 Summary of the device features – MR, sensitivity and sensitivity gain – obtained upon the inclusion of the double layer MFCs with different dimensions (outer width and length). A comparison of the results depending on the NiFe - CoZrNb distance d is also presented. An average sensitivity gain ~ 90x (~ 400x) is obtained for d = 50 m (d = 100 m). range was performed [inset Fig. 2(a)]. A 0.Hex reduction from 33 mT to 12 mT (factor ~ 3x) was observed upon double layer MFCs inclusion. The maximum gain of the MFCs occurs within the linear transition range of the material H=2Hk, with an abrupt reduction for external applied fields larger than Hk [12]. The presence of magnetostatic coupling between the pinned layer and the MFCs is not taken into account, but is well known to affect the calculated gain [13]. The influence of NiFe - CoZrNb separation (d = 50, 100 m) in the device transfer curve is presented in Fig. 2(b), where a finer characterization of the obtained curves within the [-0.3, 0.3] mT range (0.01 mT step) is shown. Both presented curves have a square shape, exhibiting a coercivity 0.Hc < 0.1 mT. Taking the sensitivity as the average value of the two transition branches in the transfer curve, a sensitivity enhancement of 430x (100x) is obtained upon the integration of MFCs with d = 100 (50) m. With the configuration where d = 100 m, a sharper transition between the saturation states occurs (within 0.01 mT), yielding sensitivity gains of ~ hundreds of times. However, besides these gain values, the device is always in a saturation state at remanence with both MFCs configurations, implying a fine control of its operation point to place it in one of the transition branches. Fig. 3 summarizes the main sensor features (MR, sensitivity and sensitivity gain) upon the inclusion of MFCs 0018-9464 (c) 2016 IEEE. Personal use is permitted, but republication/redistribution requires IEEE permission. See http://www.ieee.org/publications_standards/publications/rights/index.html for more information. This article has been accepted for publication in a future issue of this journal, but has not been fully edited. Content may change prior to final publication. Citation information: DOI 10.1109/TMAG.2017.2712860, IEEE Transactions on Magnetics FF-07 Fig. 4 (a) Schematic view of the performed experiment, where is defined between the device sensing direction and the applied external field. (b) Normalized sensitivity dependence of the characterized devices with the angle . Angular stability results obtained for: single SV sensor, SV sensor with double layer MFCs, and SV sensor with single layer MFCs. Comparison of the experimental results with the trend obtained from 2D finite element method simulation, taking into account the NiFe – CoZrNb unpatterned r and the MFCs funnel shape (no vertical tapering considered). with different dimensions. While MFCs with a NiFe - CoZrNb separation d = 50 m allowed an average sensitivity gain ~ 90x, this increased to ~ 400x when a pole separation of 100 m was used. A considerable dispersion of the sensitivity gain is observed for both configurations. This dispersion suggests the need of local magnetic control of the MFCs elements, particularly in the pole region. The possible presence of defects in the MFCs poles and the small remanence in gap affect the structure magnetic domains and consequently the obtained gain value. An overall trend of the obtained sensitivity gains with the MFCs dimensions (outer width and length) was not observed for the studied geometries. B. Improved resilience to misalignment As a consequence of its field guidance capability, the MFCs were also evaluated as a strategy to minimize the impact of misalignment between the device sensing direction and the signal-of-interest direction. In this work, the angular dependency of the device transfer curve (and sensitivity) with the direction of the external magnetic field was addressed. The angle () of the external field, measured relative to the SV sensing axis (Fig. 4(a)), was consecutively changed in the [0, 90]º range with an increment = 15º. This experiment was performed for devices with three different specifications: (i) single SV sensor; (ii) SV sensor with double layer MFCs; and (iii) SV sensor with single layer MFCs, defined with the same shape but without vertical tapering (500 nm-thick CoZrNb, step profile in the gap region as described elsewhere [3][6]). Fig. 4(b) shows the dependence of the devices normalized 4 sensitivity with the angle . The sensitivity of a SV sensor reduces to 80% of its initial value already for = 15º. This angle increases to = 45o upon the inclusion of the double layer MFCs, denoting advantageous angular stability in the device performance. For the same conditions, single layer MFCs only operate within an angular range up to = 30o. The developed MFCs increase the angular operation range rendering the device insensitive to misalignments relative to the applied field without compromising its performance. Fig. 4(b) also displays the field amplification gain dependence obtained through 2D finite element method (FEM) simulations. The MFCs geometry was the same used in the fabrication process (funnel shape, pole width = 40 m, outer width = 1000 m, length = 675 m) but without accounting with the vertical tapered profile. A single material was considered taking the bulk r = 803 of the NiFe/ CoZrNb double layer. To further approximate the simulated model to the fabricated device, a stripe of magnetic element was placed in the MFCs gap (SV total dimensions 50 x 2 m2, r = 480). The MFCs and the magnetic element are placed in a squared air box (r = 1, length = 5000 m), being subjected to a constant magnetic field 0.H = 10 mT. The field gain is obtained from the ratio between the magnetic flux calculated in the MFC pole – SV middle point and the fixed field applied outside the MFCs. For misalignments < 45º, the simulated curve approaches the experimental results of the device with single layer MFCs. This behavior suggests that for a low misalignment range [0, 45]º the further stabilization obtained upon the double layer MFCs arises from its vertical tapering and consequent enhanced guiding efficiency, exhibiting a deviation from the simulated curve which only accounts for the in-plane funnel shape geometry. Consequently, the close matching of the simulated curve with the experimental data for single layer MFCs (sharp profile in the pole) supports the vertical tapering influence in the sensitivity stabilization. However, for > 45º the simulated curve tends to the experimental results of double layer MFCs, suggesting that for larger misalignments the MFCs in-plane geometry and the materials magnetic properties (r) are the main contribution factors for the observed trend. Therefore the vertical tapering of the proposed double layer MFCs architecture provides an enhanced sensitivity stabilization, resulting in a wider angular operating range without sensitivity loss. IV. CONCLUSION This paper addresses the enhanced guiding efficiency of MFCs obtained through a double layer architecture with a vertical tapering. The presented strategy allows a vertical concentration of the flux together with an in-plane magnetic flux concentration. Sensitivity gains surpassing the values for single layer concentrators were achieved, being obtained an average gain ~ 400x for a NiFe – CoZrNb distance of 100 m. The impact of a misalignment between the device sensing direction and the external magnetic field was minimized for a larger angular range upon the inclusion of the developed MFCs. The device performance is not compromised within a 0018-9464 (c) 2016 IEEE. Personal use is permitted, but republication/redistribution requires IEEE permission. See http://www.ieee.org/publications_standards/publications/rights/index.html for more information. This article has been accepted for publication in a future issue of this journal, but has not been fully edited. Content may change prior to final publication. Citation information: DOI 10.1109/TMAG.2017.2712860, IEEE Transactions on Magnetics FF-07 5 misalignment range [0, 45]º. This further stabilization arises from the MFCs vertical tapering. ACKNOWLEDGMENT Work partially supported by FCT-project EXCL/CTMNAN/0441/2012 and EU-FP7-ICT project nº 600730 (Magnetrodes). J. Valadeiro acknowledges FCT for scholarship grant PD/BD/113956/2015 within the Doctoral Programme AIM-Advanced Integrated Microsystems and support through POPH. D C Leitao acknowledges financial support through FSE/POPH. INESC-MN acknowledges FCT funding through the Associated Laboratory IN. REFERENCES [1] [2] [3] [4] [5] [6] [7] [8] [9] [10] [11] [12] [13] G. A. Prinz. J. Magn. Magn. Mater. vol. 20, issues 1-3, pages 57-68, 1999. R. Chaves, P.P. Freitas, B. Ocker, W. Maass. Appl. Phys. Lett. 91, 102504, 2007. J. Valadeiro, J. Amaral, D.C. Leitao, R. Ferreira, S. Cardoso and P.P. Freitas. IEEE Trans. Magn., vol. 51, no. 1. 2015 Hu, J., Pan, M., Tian, W., Chen, D., & Luo, F. (2012). Applied Physics Letters, 101(23), 234101. Liou, S. H., Yin, X., Russek, S. E., Heindl, et al.. (2011). IEEE Transactions on Magnetics, 47(10), 3740-3743. A.V. Silva, D.C. Leitao, J. Valadeiro, J. Amaral, P.P. Freitas and S. Cardoso. Eur. Phys. J. Appl. Phys., (2015) 72: 10601 M. Pannetier-Lecoeur, C. Fermon, G. Le Goff, J. Simola, E. Kerr. Science 2004, 304, 1648–1650. Y Kim and I Savukov, Scientific Reports 6, 24773 (2016) Z. Marinho, S. Cardoso, R. Chaves, R. Ferreira, L. Melo and P.P. Freitas. J. Appl. Phys., 109, 07E521 (2011) J. Valadeiro, S. Cardoso, R. Macedo, A. Guedes, J. Gaspar and P.P. Freitas. Micromachines, 7(5):88, 2016 I.G. Trindade, D.C. Leitao, Y. Pogorelov, J.B. Sousa, R. Chaves, S. Cardoso and P.P. Freitas. Applied Physics Letters 94, 073501 (2009) P.M. Drljača, F. Vincent, P.A. Besse and R. S. Popović. Sensors and Actuators A: Physical, vol. 97–98, pages 10-14, 2002 I.G. Trindade, J. Oliveira, R. Fermento, J. Sousa, S. Cardoso, P.P. Freitas, A. Raghunathan and J. Snyder. IEEE Trans. Magn., vol. 45, no. 1, pp. 168-171, 2009. 0018-9464 (c) 2016 IEEE. Personal use is permitted, but republication/redistribution requires IEEE permission. See http://www.ieee.org/publications_standards/publications/rights/index.html for more information.