1 2 3 4 Radon mitigation system approach to avoid interferences at the measurements room of a radioactive laboratory Luis Alfonso Fernández-Serantes, Alberto Otero-Pazos, Alfonso Calleja-Garcı́a, Marı́a Isabel Fernández-Ibañez, Andrés José Piñon-Pazos, José Luis Calvo-Rolle 7 University of A Coruña, Departamento de Ingenierı́a Industrial, Avda. 19 de febrero s/n, 15495, Ferrol, A Coruña, España 8 Tel.: +34 981 337400 ext. 3117 Fax.: +34 981 337401 5 6 9 Abstract 15 Radon gas is the second reason of lung cancer, causing thousands of deaths. It can be a problem for people or animals at houses, workplaces, schools or any building. Due to this fact, its mitigation has become very important to avoid health problems, among others. Also, radon interferes at radioactive measurements. This study describes how a radon mitigation system was carried out to reduce interferences in the different works of a radioactivity laboratory. A large set of radon concentration samples is obtained from measurements at the laboratory. Several mitigation methods were taken into account and the implemented solution is explained in detail. With it, very good results have been obtained by reducing the radon concentration by 76 %. 16 Keywords: Radon, mitigation, positive ventilation, sump system, sealing, radon reduction 17 1. Introduction 10 11 12 13 14 18 19 20 21 22 23 24 25 26 27 28 29 30 31 32 33 Radon is a gas that is produced by the natural radioactive decay of U 238 , which is a very active chemical element capable of associating with many others and move with them [1]. Uranium exist in almost all rocks and soils of the planet in small proportions (ppm) [2]. Galicia Autonomy (Spain) is a prone area to radon gas, due to the fact that granites, one type of rock and soil that have great concentration of uranium, are very common [3]. Radon, which is an inert radioactive gas that is naturally occurring; is odorless, colorless and tasteless [4]. It is easily released from the soil into the air, where it disintegrates forming various products of short duration which are known as radon progeny [5]. As these are decay, radioactive and alpha particles are emitted and they adhere to aerosols, dust and other airborne particles [6]. When people breathe, radon progeny is deposited on epithelial cells lining the airways where alpha particles can damage DNA and, therefore, cause lung cancer [7] and thousands of deaths all over the world each year [8]. According to the United States Environmental Protection Agency (EPA), radon gas is the second cause of lung cancer, after smoking, causing 21 thousand of deaths per year in the United States [9]. Due its accumulation, radon can be a problem at houses, workplaces, schools or any building where people or animals are. It came from the soil basement where buildings are placed. Thus, it gets into them through cracks in the floors, constructions joints, gaps in suspended floors, cavities inside walls or water supply. Normally, radon gas is not produced by common building materials [8]. Email address: luis.alfonso.fernandez.serantes@udc.es (Luis Alfonso Fernández-Serantes) 1 / Radiation measurements 00 (2016) 1–10 34 35 36 37 38 39 40 41 42 43 44 45 46 47 48 49 50 2 Usually, outdoors radon concentrations are very low. On average, it varies between 5 and 15Bq/m3 [6]. Conversely, indoor concentrations are higher and reach maximums in places like: mines, caves, treatment water plants and so on [6]. Spanish legislation says that radon average concentration at work places should be less than 600Bq/m3 (300Bq/m3 if workplace with high permanence of workers). Over this value (> 600Bq/m3 ), a mitigation control system with periodical tests should be implemented to keep radon concentration levels low [10]. With the aim of reducing radon gas concentration at working places there are several mitigation solutions depending on the case. The main generic solutions are: • Sealing: trying to seal all obvious cracks, gaps and holes in floors or walls to prevent radon from entering the building. However, in most cases reduction is not effective [11, 12]. • Positive ventilation: installing small fans to blow filtered fresh air into the building. The fundamental principle is to increase the pressure inside the building in relation with outside pressure, so radon gas cannot flow inside it[11, 12, 13]. • Sump systems: the purpose is to exhaust the air from inside the building when the concentration reaches a set point value. Usually, the extraction is forced to improve the performance and to reduce the response time [14, 12]. • Underfloor ventilation: installing vents at the foundations to provide natural or force ventilation underfloor to suck or blow radon [12, 13]. 58 The proposed solutions explained on the present work are based on positive ventilation to mitigate radon concentration. The main aim is to avoid interferences with the working place equipment in a radioactivity laboratory. This work is focused on the analysis of different steps that have been carried out at the mentioned case. For each step, a change have been introduce and several measurement have been done. Finally, a comparative is made taken all cases into account. This paper begins with a description of the case of study, where the focused installation is described as well as all the different components used to decrease radon concentration. It follows with the carried out process that analyses the approach, step by step. Then, the results are shown and finally the conclusions are exposed. 59 2. Case of study 51 52 53 54 55 56 57 63 The Environmental Radioactive Laboratory carries out different works related to radioactive measurements and the analysis of the obtained data. These tasks are made at a specific room (measurement room), where all the different equipment is and where a radioactivity interference was found. The case of study is described in detail in the following subsections. 64 2.1. Environmental Radioactive Laboratory 60 61 62 65 66 67 68 69 70 71 72 73 74 75 76 The proposal has been implemented at the “Laboratorio de Radiactividad Ambiental” (LRA) of the University of A Coruña, located in Ferrol (Galicia Autonomy) at the Faculty of Engineering. The laboratory carries out different researches about the radiological characterization of soils on the north coast of Galicia or an specific agreement with the Nuclear Safety Council, on a program of Environmental Radiation Monitoring, for example. The measurements of characterization of soils are done in a small room, which is presented after, where a concentration of radon gas has been detected. This laboratory measurement room was chosen because it is a small room, closed and with few ventilation, an appropriated place where radon gas concentrations can be high. Due to the fact that the presence of this gas could affect the measurements carried out in this laboratory, different mitigation methods were studied. The studied method were proposed and, finally, some of them were implemented with the consequently reduction of the radon gas. The radon level was measure in the laboratory measurement room, showing an enough important activity that could affect and disturb the measurements. 2 / Radiation measurements 00 (2016) 1–10 77 78 79 80 81 3 2.2. Laboratory measurement room The LRA measurement room is a small room of 20.60m2 where all radioactive measurements are done and where the used equipment is placed. The room is located inside the LRA, second floor of the building. It is west-oriented and its dimensions are, approximately, 3.20 meters high, 5.80 meters long and 3.55 meters wide. Figure 1 shows what the room looks like. Figure 1. Measurement room 86 The building structure and the floor are made of reinforce concrete with the walls made of coated bricks and painted. Due to the fact that the equipment is very heavy, it was necessary to install steel sheets on the floor with the aim of distribute the weight uniformly. To get inside this room, there is a door that connects with the chemistry laboratory and the office. Also, there is a window situated on the west wall where the different mitigation systems are installed. 87 3. Radon mitigation solution approach 82 83 84 85 88 89 90 91 92 93 94 95 96 97 With the aim of reducing radon gas concentration and avoiding perturbations in the equipment, several mitigation methods have been taken into account. The implemented solution had to consider building limitations and restrictions. On the other hand, due to the fact that the measurement room is independent of the office, the applied solution does not disturb the work environment. The measurement room is on the second floor. Owing to this fact, some methods are impossible to carry out, such as underfloor ventilation. Also, sealing cannot be implement due to the age of the building and because there are different entrances to the room. Thus, for the same reason, sump systems could not be installed. In any case, radon gas would have entered the measurement room through the cracks. Instead, the positive ventilation could be a good solution because of its viability and low cost implementation. Finally, due to the reasons described above, this is the chosen solution to mitigate radon. 3 / Radiation measurements 00 (2016) 1–10 4 Figure 2. Measurement room with one fan 98 99 100 101 102 103 104 105 106 107 108 109 110 111 112 113 For measuring radon concentrations the AlphaGuard PQ 2000PRO was used. This equipment measured the concentration of radon gas every ten minutes every day of the year. With the obtained values, the equipment do the avarage as in equation 1. n 1 X Average = · xi (1) n i=1 It also calculates the uncertainty as the standard deviation using the equation 2. sP n 2 i=1 (xi − x) Uncertainty = (n − 1) (2) 3.1. Positive ventilation solution Positive ventilation consists of installing fans to blow fresh and filtered fresh air into the measurement room, by pressurizing to prevent radon from entering and diluting it [11, 12]. To implement the selected solution, two fans and an air conditioning system were installed. Different steps were followed to carried out this option. The fans were installed with the aim of pressurizing and diluting radon gas. A second fan has been necessary installed due to the fact that only one unit was not enough. Also, an air conditioning system was installed to reduce air humidity, keep the temperature around the value of 20 Celsius degrees and to weatherize the measurement room. Moreover, this system blows filtered air into the measurement room, contributing to radon mitigation and its stability throughout the year. Air conditioning was necessary to avoid variations at measurement conditions and because electronic device performance is better at a constant temperature and low humidity. These systems also benefits the installation because they reduce condensation. 4 / Radiation measurements 00 (2016) 1–10 5 Figure 3. Measurement room with two fans 114 115 116 117 They were installed at the unique window of the room, so the works done for their installation were minimal. Figure 1 shows the measurement room where all the systems have been installed. The components used to decrease radon concentration are the following: • Fans: The used fans are the model HV-230 from S&P. These fans characteristics are: 118 – Rotating speed of 1250 revolutions per second. 119 – Extraction caudal at high speed of 600m3 /h and at low speed of 450m3 /h. 120 – Impulsion caudal of 330m3 /h. 121 122 123 The power that the fans consume is 34 watts each, and the absorbed current is 0.15 amperes. • Air conditioning: The used air conditioning is the model PCA-RP50xB7KA from Mitsubishi Electric. The are conditioning characteristics are: 124 – For cold, 5 kW and 4300 kCal/h. 125 – For hot, 5.5 kW and 4730 kCal/h. 126 – Sound level, for low speed, around 32/40 dB. 127 128 129 130 131 132 133 134 3.2. Steps followed until the final solution is reached In this subsection, the steps carried out to get the desired results are explained: a) The first step was the installation of one fan, to pressurize the measurement room, see figure 2. Radon concentration was measured some time later, once its level had achieved a steady state, but the level did not decrease enough with this action. b) Due to this fact, as it is shown on figure 3, a second fan was installed to increase the pressure inside the measurement room. After several measurements, it was noticed that the introduced air was enough to reduce radon concentrations, thus avoiding interferences in the measurements. 5 / Radiation measurements 00 (2016) 1–10 6 Figure 4. Measurement room with all systems 135 136 137 138 139 140 141 c) Once the fan systems were implemented, air conditioning was installed, see figure 4. Furthermore, it blows air inside the measurement room and weathered it at constants condition during all time. The air conditioning helps to have stable measurements and, thus, reducing the uncertainty. This fact is because of the temperature control of the room and, also, because of the reduction in humidity. d) In the end, all systems -fans and air conditioning- were working together with the aim to decrease radon concentration and to have repeatable conditions for the measurements. Also, different analysis were done periodically to keep control of radon levels in order to know how it varies along the year. 143 In this case, fans work in impulsion mode and the air conditioning works keeping the temperature around the value of 20◦ C and controlling air humidity. 144 4. Results 142 145 146 147 In this section, the radon concentration measurements for the different cases mentioned above are shown. At first, the radon concentration was measured on different days to quantify its level. Table 1 shows the average concentration for the period from 25th of April to 23th of November of the previous year, without any mitigation solution. Radon-222 activity Average Uncertainty Maximum concentration Number of measurements Concentration (Bq/m3 ) 79 37 158 212 Table 1. Concentration before applying any solution 148 149 150 151 Then, from the 30th of November of the previous year to the 25th of January of the next year, one fan was installed and measurements were carried out. The next period of measuring was from the 25th of January to the 01 st of December. During this period, a second fan was installed and several measurements were taken with both fans working. Table 2 shows concentration during these times. The analysis of the concentration while the mitigation 6 / Radiation measurements 00 (2016) 1–10 152 153 7 solutions were implemented, from 30th of November of the previous year to the 01 st of December, revealed how it decrease to the values shown in table 2. Radon-222 activity Average Uncertainty Maximum concentration Number of measurements One fan (Bq/m3 ) 29 18 64 56 Two fans (Bq/m3 ) 19 10 53 278 One/Two fans (Bq/m3 ) 21 13 64 334 Table 2. Concentration after fans installation 154 155 156 157 After the installation of the two fans, an air conditioning system was installing, thus achieving the results shown in table 3. The period when this system (both fans and air conditioning) is on goes from the 01 st of December to nowadays. At that moment, the value of radon concentration is very low. Finally, table 4 shows the concentration reduction summary by using the different components of the mitigation solution. Radon-222 activity Average Uncertainty Maximum concentration Number of measurements Concentration (Bq/m3 ) 19 9 40 1174 Table 3. Concentration after air conditioning installation Radon-222 activity Average Uncertainty Average Uncertainty Average Uncertainty Average Uncertainty Average Uncertainty Mitigation solution One fan One fan Two fans Two fans Two fans Two fans One or two fans One or two fans Two fans and air conditioning Two fans and air conditioning Compared with Any method Any method One fan One fan Any method Any method Any method Any method Any method Any method Reduction % 62.8 50.3 35.6 43.7 76.0 72.0 73.8 65.8 76.0 75.7 Table 4. Concentration reduction after mitigation systems installation 158 159 160 161 The figure 5 is a picture of the measurement room with all the systems applied. It is possible to see the two fans and the air conditioning system. Also, the figure 6 shows a summary of the reduction of the radon gas with the different systems, showing how it get reduced when the methods are implemented. 7 / Radiation measurements 00 (2016) 1–10 Figure 5. Picture of the measurement room with all systems 8 8 / Radiation measurements 00 (2016) 1–10 9 Figure 6. Evolution of radon gas measurement with the different systems 162 5. Conclusion 170 With the radon mitigation solution approach explained in this document, very good results have been obtained. As it is shown in the results section, after the installation of the different removing systems, the radon concentration decreased in a very significant way. It was reduced up to the value of 76 %. In this way, the implemented solution avoids the interferences at the laboratory measurements. Positive ventilation achieved good results by pressurizing the measurement room and avoiding radon entrance. For this purpose, two fans were installed with the aim of reducing the radon concentration to a low value. Also, air conditioning contributes slightly to radon mitigation and allows a very good repeatable condition performance for the measurements. 171 6. Acknowledgments 163 164 165 166 167 168 169 175 This research has been funded by the University of A Coruña, and by the Spanish Ministry of Education, Culture and Sport (grant for Collaboration in University Departments). We would like to express our utmost gratitude to the Nuclear Security Council of Spain, without whose collaboration this research would not have been possible. 176 7. References 177 References 172 173 174 178 179 180 181 [1] P. Sahu, D. P. Mishra, D. C. Panigrahi, V. Jha, R. L. Patnaik, Radon emanation from low-grade uranium ore, Journal of Environmental Radioactivity 126 (0) (2013) 104 – 114. doi:http://dx.doi.org/10.1016/j.jenvrad.2013.07.014. [2] J. Llerena, D. Cortina, I. Durn, R. 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