See discussions, stats, and author profiles for this publication at: https://www.researchgate.net/publication/346461477 Large-scale automotive battery cell manufacturing: Analyzing strategic and operational effects on manufacturing costs Article in International Journal of Production Economics · November 2020 DOI: 10.1016/j.ijpe.2020.107982 CITATIONS READS 32 1,543 5 authors, including: Fabian Duffner Lukas Mauler University of Münster University of Münster 8 PUBLICATIONS 250 CITATIONS 5 PUBLICATIONS 81 CITATIONS SEE PROFILE SEE PROFILE Marc Wentker Jens Leker University of Münster University of Münster 8 PUBLICATIONS 240 CITATIONS 142 PUBLICATIONS 2,661 CITATIONS SEE PROFILE SEE PROFILE Some of the authors of this publication are also working on these related projects: Business Chemistry View project Management issues in the chemical industry - Journal of Business Chemistry (JoBC) View project All content following this page was uploaded by Fabian Duffner on 29 November 2020. 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Production Economics 232 (2021) 107982 Contents lists available at ScienceDirect International Journal of Production Economics journal homepage: http://www.elsevier.com/locate/ijpe Large-scale automotive battery cell manufacturing: Analyzing strategic and operational effects on manufacturing costs Fabian Duffner a, b, *, Lukas Mauler a, b, Marc Wentker a, Jens Leker a, c, Martin Winter c, d a Institute of Business Administration at the Department of Chemistry and Pharmacy (IfbM), University of Münster, 48148, Münster, Germany Porsche Consulting GmbH, 74321, Bietigheim-Bissingen, Germany c Helmholtz-Institute Münster (HIMS), 48149, Münster, Germany d MEET Battery Research Center, Institute of Physical Chemistry University of Münster, 48149, Münster, Germany b A R T I C L E I N F O A B S T R A C T Keywords: Battery Automotive Manufacturing Cost Optimization Process-based cost modelling Cost-efficient battery cell manufacturing is a topic of intense discussion in both industry and academia, as battery costs are crucial for the market success of electrical vehicles (EVs). Based on forecasted EV growth rates, battery cell manufacturers are investing billions of dollars in new battery cell plants. Whether these billion-dollar in­ vestments are economically viable depends on the materialization of forecasted EV growth rates and companyspecific competitive market positions. For both, cost-efficient battery cell manufacturing is key for success. To ensure cost-efficient battery cell manufacturing, transparency is necessary regarding overall manufacturing costs, their cost drivers, and the monetary value of potential cost reductions. Driven by these requirements, a cost model for a large-scale battery cell factory is developed. The model relies on the process-based cost modelling technique (PBCM) and includes more than 250 parameters. Based on this cost model, directions are provided, how minimum costs can be achieved reflecting current and future state of technology. Further, it is outlined which process steps and cost elements have the greatest impact on total cost and should thus be focused within future cost reduction activities. 1. Introduction The battery manufacturing industry is forecast to be one of the fastest growing production industries through 2030. Especially driven by the expanded production of electrical vehicles (EVs) with the overall goal of minimizing vehicular CO2 and NO2 emissions, annual global lithium-ion battery capacity demand is expected to increase from 160 GWh cell energy in 2018 to >1000 GWh cell energy in 2030. By 2030, this in­ crease will have triggered investments of more than $100 billion and generate annual revenue of more than $100 billion within battery manufacturing industry (Avicenne Energy, 2019). To transform these investments into sustainable business models, cost efficient battery manufacturing is the key factor as it is the prerequisite to make EVs competitive compared to internal combustion engine vehicles (Pollet et al., 2012; Sierzchula et al., 2014; Wu et al., 2015). The need to produce cost-efficient batteries, the launch of the first mass-market EVs (e.g. Tesla Model 3), and initial investments worth several billion dollars for the first battery-cell factories (e.g. Tesla’s Gigafactory) have made battery-cell cost optimization relevant for both science and industry. Triggered by this, some optimizations have already been achieved, mainly based on new materials and innovative cell chemistries (Liu et al., 2010; Placke et al., 2017; Scrosati and Gar­ che, 2010; Wagner et al., 2013; Winter et al., 2018). Although it has received less attention, battery cell manufacturing has also improved, with notable results in the last two decades. However, due to numerous consecutive process steps, the interaction of these steps and the high number of individual process parameters, it can be assumed that there is potential for further optimization. The realization of this potential will require a deep understanding of the individual production process steps, process parameters, and their impact on cost (Kwade et al., 2018). With regard to costs, cost models with extended capabilities to analyze cost drivers and to simulate a large number of parameters can be the key for success to achieve the necessary transparency (Qian and Ben-arieh, 2008). Driven by this requirement, numerous studies have dealt with the modelling of battery costs (Berg et al., 2015; Nelson et al., 2019; Petri et al., 2015; Schmuch et al., 2018; Vaalma et al., 2018; * Corresponding author. Institute of Business Administration at the Department of Chemistry and Pharmacy (IfbM), University of Münster, 48148, Münster, Germany. E-mail address: duffnerfa@gmail.com (F. Duffner). https://doi.org/10.1016/j.ijpe.2020.107982 Received 30 March 2020; Received in revised form 11 August 2020; Accepted 3 November 2020 Available online 11 November 2020 0925-5273/© 2020 The Authors. Published by Elsevier B.V. This is an open (http://creativecommons.org/licenses/by-nc-nd/4.0/). access article under the CC BY-NC-ND license F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 Fig. 1. Process steps for the manufacture of a lithium-ion pouch battery cell in a large-scale factory. Wentker et al., 2019). However, most of these models focus on material using surcharge rates to forecast processing costs (Duffner et al., 2020b). While such approaches are suitable to forecast rough costs for a new product with less effort, their capabilities to translate new innovations comprehensively into costs are limited (Niazi et al., 2006). Addressing these limitations, within this paper, a model is presented that can translate the academic discussion related to process in­ novations, material & design-innovations, and location alternatives into costs. Therefore, first, cost estimation techniques are reviewed to eval­ uate suitability for the presented requirements. Finding that bottom-up techniques and especially the process-based cost modelling technique fits best, a model for battery manufacturing relying on more than 250 parameters is proposed. Based on this model, cost driver analysis within process steps, cost elements and parameter categories is provided. Further, a current state and a future cost level is introduced by trans­ lating the associated parameter sets from literature into costs. The main innovations of this study are as follows: First, a current and future cost level is presented that is derived by linking an established cost estimation technique (PBCM) with the current battery specific discussion related to process optimization, material & design optimi­ zation and location alternatives. This analytical approach provides the most reliable and up to date basis to evaluate the cost potential of lithium-ion batteries. Second, by presenting the most comprehensive cost driver analysis within lithium-ion battery manufacturing (scenariorelated parameters, process steps and cost elements) guidance is pro­ vided to set focus in future cost optimization activities. Third, due to its extensive parameter foundation, the presented model and the associated model architecture provides an optimal starting point to translate further battery innovations into costs. This is, especially in the highly dynamic battery environment, a valuable capability as it provides the basis for cost-optimal and data-driven decision making. Summarizing, the results of this paper contribute to evaluate the technological po­ tential of lithium-ion batteries and support the materialization of this potential which is relevant for both, science and industry. 2. Background 2.1. Battery design and manufacturing Automotive traction battery systems consist of battery modules and battery cells that are connected and controlled by a battery management system. The cells are a crucial component as they significantly influence the performance and cost of the whole system (Kwasi-Effah and Rabc­ zuk, 2018; Nelson et al., 2019). The major constituents of a lithium-ion battery cell, which is currently the state-of-the-art technology (Aalder­ ing et al., 2019), are the cathode (positive electrode) (Arinicheva et al., 2020; Whittingham, 2004) and the anode (negative electrode) (Andre et al., 2017) as well as the separator and the electrolyte. Lithium tran­ sition metal oxides (LiMO2) with transition metals (M) such as nickel, cobalt, and manganese (NMC) are the most widely used class of positive active materials (Andre et al., 2015; Myung et al., 2017; Schmuch et al., 2018). Carbonaceous materials, in particular synthetic and natural 2 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 Fig. 2. Classification of cost estimation techniques including key advantages, limitations and examples for techniques. graphite, as well as amorphous carbons are mostly used as negative active material (Blomgren, 2017; Schmuch et al., 2018; Scrosati et al., 2015). As electrolyte solvents, a mixture of cyclic and linear organic carbonates with lithium hexafluorophosphate as conductive salt (typi­ cally ~1 mol L− 1) are used (Schmuch et al., 2018; Xu, 2014). The used microporous separator is typically based on polyolefins such as poly­ propylene (Lee et al., 2014). For current collectors, thin sheets of aluminium and copper are used for the cathode and the anode, respec­ tively. Conductive electrode additives are usually carbon-based. With regard to battery cell production, numerous consecutive process steps are required. The manufacturing processes outlined in the following represent large-scale production of a lithium-ion pouch cell, as pre­ sented in Kwade et al. (2018). This production can be divided into three value-adding superordinate main processes: electrode production, cell production, and cell conditioning. Other processes are also necessary to support the execution of these three value-adding processes (e.g. inter-process material handling). Fig. 1 shows the individual process steps. In electrode production, anodes and cathodes are produced. Anode and cathode production are spatially separated, but basically the same process steps are followed. For the sake of simplification, the process steps for cathode production only are described here. First, the cathode components, namely the active material, typically NMC622 in state-ofthe-art (Schmuch et al., 2018), polymer binder (e.g. PVdF), solvent (e. g. NMP), and conductive additives (e.g. carbon), are batch-wise mixed in a planetary mixer for several hours to produce a cathode slurry. The target of this process step is to achieve the desired homogeneity and viscosity of the slurry ensuring the electrode’s subsequent electro­ chemical performance and adhesion to the current collector foil (Dreger et al., 2015). In current cathode chemistries, this adhesion is provided by PVdF binders whose processing relies on the toxic and teratogen solvent NMP. For anode production, NMP has already been replaced by water which could also be implemented in cathode processing. This reduces the drying effort due to a lower boiling point (water 100 ◦ C vs. NMP 203 ◦ C), eliminates the complex and costly solvent recovery process, decreases associated material cost (water < $0,02 L− 1 vs. NMP $1-3 L− 1) and results in more sustainable manufacturing (lower CO2 emissions, less toxic materials) (Bresser et al., 2018a). The Mixing process is fol­ lowed by the four continuous and interconnected process steps Coating, Drying, Calendering and Slitting, which can be summarized as roll-to-roll processes. These four adjacent processes should be linked and hence share the roll-to-roll working speed as an essential process parameter. State-of-the-art electrode processing has already reached working speeds of 25–50 m min− 1 (Kwade et al., 2018). Within the Coating process step, thin metal carrier foils (e.g. aluminum) are coated on both sides with the active material slurry and directly dried to solidify the slurry by evaporating the solvent. As the working width of the coater (up to 1500 mm) exceeds the width of common single electrodes, the Fig. 3. Battery-cell-specific process-based cost modelling (PBCM) framework. 3 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 (Ciez and Whitacre, 2017). To enable electrode production, cell production and cell condition­ ing additional supporting processes are necessary: ensuring a clean at­ mosphere required for cell production through the use of a dry room, recycling the NMP solvent used for cathode production, ensuring proper material handling through all process steps, and managing the receipt of purchased materials and the shipping of finished cells (Nelson et al., 2012). Table 1 Product characteristics of battery cells considered for Base and Optimistic Scenario. Cell Design Specifications Base Energy 193 Energy density 265 Format Pouch Chemistry NMC622 ||G Number of two-sided electrodes Cathode 30 Anode 30 Coating Thickness Cathode 65 Anode 74 Width of electrodes* Cathode 93 Anode 95 Length of electrodes* Cathode 294 Anode 296 * based on ISO cell format Pouch VIFB-/99/300 Optimistic Unit 211 296 Wh cell− 1 Wh kg− 1 NMC811 ||G 20 20 pieces cell− pieces cell− 100 120 μm μm 1 2.2. Cost estimation and battery cost modeling 1 Cost estimation involves the forecasting of costs of activities that have not yet been carried out at the time the estimation is conducted (H’midaa et al., 2006; Shehab and Abdalla, 2002). Over the last decades, a variety of different cost-estimation techniques have been developed that researchers categorize using various criteria (Cavalieri et al., 2004; Hueber et al., 2016; Niazi et al., 2006; Qian and Ben-Arieh, 2008b; Shehab and Abdalla, 2001, 2002; Zhang et al., 1996). Referencing the approach published by Hueber et al. (2016), the techniques can be categorized as intuitive, analogical, parametric or bottom-up. Intuitive techniques rely on the estimator’s knowledge and experi­ ence. Within these techniques, rough, somehow subjective and arbitrary results can be generated without greater effort but they are neither comprehensible nor repeatable for a third person (Niazi et al., 2006). Analogical techniques link historical cost data to a new product using regression models or neural network approaches. These techniques rely on the assumption that similar products have similar costs (Curran et al., 2004). Parametric cost estimation techniques use product-specific cost functions to predict costs. The cost functions can consist of several pa­ rameters or variables, like part weight or part size (International Society of Parametric Analysts, 2018). Within the bottom-up techniques a product is first broken down into its individual components. The com­ ponents are then broken down into resources and processes required to produce them, with costs assigned to each (Ben-Arieh and Qian, 2003). Fig. 2 presents the categories and summarizes the key advantages and limitations per category. Further research on intuitive techniques can be found in Ficko et al. (2005), Rush and Roy (2001), Sakti et al. (2017), Shehab and Abdalla (2002), on analogous techniques in Cavalieri et al. (2004), Hagen et al. (2015), Verlinden et al. (2008), Wang (2007), on parametric techniques in Duverlie and Castelain (1999), Nelson et al. (2019), Patry et al. (2015) and on bottom-up techniques in Ciez and Whitacre (2017), Cooper and Kaplan (1988), Ficko et al. (2005), Field et al. (2007), Schulze et al. (2012). Relying on these techniques and driven by the relevance of battery costs, various battery cost models have been developed within the last years. Most of these models focus on the calculation of material costs (Berg et al., 2015; Petri et al., 2015; Schmuch et al., 2018; Wentker et al., 2019). A detailed description and analysis of these models can be found in the review article published by Duffner et al. (2020). However, to date, across this literature, no battery cost study is available that neither deals with the state-of-the-art nor with further optimized future pa­ rameters, that have already been reported within literature, compre­ hensively. This paper will address this gap by translating current and future parameters characteristics into costs. Therefore, a more comprehensive lithium-ion battery manufacturing cost model, which relies on more than 250 calculation parameters, is presented. mm mm mm mm electrodes are cut to the desired width after Calendering by roll knives. In the Coating and Calendering processes the targeted electrode thick­ ness is manufactured, which strongly effects cell properties. Current cathode thicknesses of high-energy cells range from 65 to 80 μm (Schmuch et al., 2018). Increasing electrode thickness results in higher energy densities but has a decreasing effect on rate capability and therefore power density, which also applies vice versa (Zheng et al., 2012). Further, electrode thickness has an impact on cost, as thicker electrodes result in a higher share of active material in the cell and hence, lower material cost for non-active components can be achieved (Patry et al., 2015). Finally, within the last process step of electrode production, the electrodes are dried under vacuum to further reduce moisture before they are transferred to a dry room (Kaiser et al., 2014; Nelson et al., 2019). To produce battery cells in a z-folded format, which is a state-of-theart electrode stacking order for lithium-ion pouch cells produced in large scale, the anodes and cathodes are first cut into single sheets. Second, the separator is fed as an endless folded band, and the anodes and cathodes are alternately inserted into the interstitial space. This is a highly automated process which is currently conducted at an operating speed of 60 sheets min− 1 (Mooy, 2019). Third, within Contacting, in­ ternal contacts between the anode, cathode, and separator assembly are created by welding. Subsequently, the assembly is inserted into the housing (e.g. pouch). After insertion, the cell is filled with electrolyte (e. g. LiPF6) and closed (Kwade et al., 2018; Tagawa and Brodd, 2009). Cell conditioning begins during the Formation and Final sealing process step. During Formation, the cell is charged for the first time, followed by discharge and further charging cycles at different charging rates. This procedure currently takes several days (Wood et al., 2015). The Formation process is crucial for cell performance and safety, as it builds up the solid electrolyte interphase (Winter 2009), which protects the graphite-anode from adverse ongoing reactions with the electrolyte (Arora, 1998). During the Formation procedure, gas is generated within the cell. Applied external pressure causes the cell to expel the gas, and the cell is finally sealed. Lastly, an Aging procedure is conducted that takes up to several weeks and consists of storing the cells under controlled conditions and performing several quality measurements to detect non-standard properties such as short circuits. (Michaelis et al., 2016; Tagawa and Brodd, 2009; Verma et al., 2010). Only cells that fulfill quality requirements in Final Control can be sold according to their original purpose. If a cell does not fulfill these requirements it is stated as end-of-line scrap. The later a process step takes place in the value chain the more sensitive it is to scrap cost as more and more value has already been added in previous process steps (Kwade et al., 2018). Hence, low end-of-line scrap rates are crucial for a competitive cell production. Typically, 95% of finished cells fulfill quality requirements 3. Cost model To develop the cost model presented within this study, PBCM is used, which is a bottom-up technique that calculates manufacturing costs analytically based on technical and operational parameters. Its reliance on technical parameters makes the technique powerful, especially for predicting costs for unexplored technologies, as technical data is usually more easily available then historical cost data. Further, it generates transparency in regard to which parameters contribute the most to the 4 International Journal of Production Economics 232 (2021) 107982 F. Duffner et al. manufacturing processes and to answer various research questions, including those focused on the evaluation of alternative processes, ma­ terials and concepts or the evaluation of process improvements (Ciez and Whitacre, 2017; Farooq et al., 2018; Fuchs et al., 2006; Johnson and Kirchain, 2009a, 2009b; Nadeau et al., 2010; Sakti et al., 2015). The PBCM framework was introduced by Field et al. (2007). As total cost and it enables the monetary quantification of potential parameter improvements. These properties make the method highly suitable for industries based on unexplored technologies that are facing high cost pressure and therefore, anticipate numerous parameter opti­ mizations (Field et al., 2007; Fuchs et al., 2006; Nadeau et al., 2010). Based on its mentioned strengths, PBCM has been used for multiple Table 2 Cost categories, related parameters, parameter descriptions and sources of parameter specifications. Cost category Parameter description Source PVSalable Required number of annual salable units Derived from Michaelis et al. (2018) PCEnergy Energy content per unit Wentker et al., 2019a r Annual discount rate Ciez and Whitacre (2017) DPY Operating days per year Nelson et al. (2019); Schnell et al. (2020) CTotal Total unit cost Calculated (see Supplementary information) Gross number of units produced in process step j Calculated (see Supplementary information) j Cost for process step j Calculated (see Supplementary information) j Variable cost for process step j Calculated (see Supplementary information) Unit cost for cost element e ∈{Material, Labor, Energy} Calculated (see Supplementary information) ACe Annual cost for cost element e ∈{Material, Labor, Energy} Calculated (see Supplementary information) Mj,Material Net mass of the material required BatPaC, 2018, Wentker et al., 2019a x Machine-specific scrap losses for process step j Nelson et al. (2019), Ciez and Whitacre (2017) Scrapj,Mat. Material type-specific scrap losses for process step j Nelson et al. (2019), Ciez and Whitacre (2017) UMaterial Unit cost of materials Nelson et al. (2019), Wentker et al., 2019a NLaborers Number of laborers required per machine Nelson et al. (2019), 2012; Sakti et al. (2015); Schünemann (2015); expert discussions NOS Number of shifts per day Ciez and Whitacre (2017) OHS Operating hours per shift Ciez and Whitacre (2017) UB Unpaid breaks hours per shift Fuchs et al. (2006) PB Paid breaks hours per shift Derived from Fuchs et al. (2006); Sakti et al. (2015) APOT Annual paid operating time Calculated (see Supplementary information) ULabor Unit cost of labor Eurostat (2019) • Energy SREnergy Surcharge rate for energy Ciez and Whitacre (2017); Sakti et al. (2015) Fixed cost j CFixed Fixed cost for process step j Calculated (see Supplementary information) Unit cost for cost element e ∈{Machine, Building, Maintenance, Overhead} Calculated (see Supplementary information) ACe Annual cost for cost element e ∈{Machine, Building, Maintenance, Overhead} Calculated (see Supplementary information) CT Cycle time UD Unplanned downtime Derived from Kaiser et al. (2014); Knoche (2017); Kwade et al. (2018); Mao et al. (2018); Nelson et al. (2019), 2012; Sakti et al. (2015); Schünemann (2015); Tagawa and Brodd (2009); Wood et al. (2015); Yoshio et al. (2009) Sakti et al. (2015) LMachine Useable lifetime of machines Nelson et al. (2019); Schnell et al. (2020) Unit cost of machines Nelson et al. (2019), 2012; Sakti et al. (2015); Schünemann (2015); expert discussions RjMachine Annual allocated machine costs for process step j Calculated (see Supplementary information) NMachine Number of machines required for process step j Calculated (see Supplementary information) Annual required machine time for process step j Calculated (see Supplementary information) availMTj Annual available operating time of a machine Calculated (see Supplementary information) FPMachine UBuilding Overarching j PVEffective CProcess Variable cost CVariable Cje j • Material • Labor j Ce j • Machine UMachine j reqMT • Building j Footprint per machine Nelson et al. (2019), 2012; Sakti et al. (2015); Schünemann (2015); constructive design LBuilding Useable lifetime of buildings PwC (2020) Unit cost of buildings Turner and Townsend (2018); ECC, 2019 RjMachine Annual allocated building costs for process step j Calculated (see Supplementary information) • Mainten. SRMainten. Surcharge rate for maintenance Ciez and Whitacre (2017); Sakti et al. (2015) • Overhead SROverhead Surcharge rate for overhead Ciez and Whitacre (2017); Sakti et al. (2015) 5 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 shown in Fig. 3, it consists of three interconnected sub-models: the process model, operations model, and financial model. The process model transforms product characteristics (e.g. size, shape, and material) into technical parameters (e.g. cycle time, machine capacity, downtime, and rejection rate) based on engineering, scientific, and technological principles. The operations model derives the overall resource re­ quirements (e.g. equipment, footprint, labor, and energy) based on operating conditions (e.g. working days/year, shifts/day and hours/­ shift) and technical parameters. The financial model adds factor prices to resources, which results in the manufacturing costs for a specific amount of a specific product (Field et al., 2007; Nadeau et al., 2010). Since battery manufacturing comprises of a large number of indi­ vidual and complex process steps, all of which mutually influence each other, not all of the engineering, scientific, and technological principles involved have been studied in a holistic way in efforts to translate product characteristics into technical parameters. To address the infor­ mation gap for technical parameters, we rely on empirical data. To map the battery-specific approach in the PBCM framework, we enlarged the framework by adding an additional input parameter category, namely technical observations, as shown in Fig. 3. The model parameters related to the categories Technical Observa­ tions, Operating Conditions, and Factor Prices are listed in Table 2. For reasons of clarity, these parameters have been classified according to their cost category (e.g. variable, fixed) and their associated cost element (e.g. material, labor). 4. Scenario-based analysis The target of the scenario-based analysis is to identify the current battery cost level by initializing the process-based cost model with stateof-the-art large-scale parameter specifications and to forecast a future cost level by translating most relevant innovations reported in academic discussion into costs. Therefore, two scenarios are defined, a Base Sce­ nario representing the state-of-the-art in large-scale battery manufacturing and a future-oriented Optimized Scenario. For the Base Scenario, the battery literature is surveyed regarding characteristics that represent both, the state-of-the-art production technology and materials and designs that are currently in use for large-scale production. Further, a typical high-cost country for battery manufacturing is assumed as plant location. For the Optimized Scenario, a categorized approach is taken that classifies reported innovations from literature into processrelated, material & design-related and location-related simulation pa­ rameters. For process-related simulation parameters, based on the resulting cell cost calculation in the Base Scenario, a literature review for the most cost-driving process steps is conducted and related process innovations are identified. For material & design-related simulation parameters, based on the resulting cell cost calculation in the Base Scenario, a literature review for the most cost-driving component is conducted and reported material and design innovations are identified. For location-related simulation parameters, a typical low-cost country for battery manufacturing is assumed as plant location, respective country-specific characteristics are taken from literature and integrated in the parameter set. Finally, in order to ensure inter-scenario consis­ tency of the underlying parameters taken from various sources, both parameter sets have been discussed with industry experts. In the following, each simulation parameter is described, including its effect on the cell cost calculation, its value in both scenarios and potential chal­ lenges in implementing respective improvements. 3.1. Model architecture The presented model architecture operationalizes the PBCM tech­ nique for the manufacture of battery cells. Similar architecture de­ scriptions have been introduced for other technologies (see e.g., Johnson and Kirchain, 2009a). The model architecture used for the presented cost model is adapted, as it must ideally meet the specific requirements of battery-cell cost modelling. In the following, the most important variable definitions and calculation rules are introduced. The complete model architecture can be found in Appendix A. The total unit cost CTotal is calculated by summing up the cost of all process steps of battery cell manufacturing (see Fig. 1). The cost for j j process step j, CProcess , can be divided into variable CVariable and fixed j j CFixed . The variable cost CVariable includes the cost elements for Material j j j j CMaterial , Labor CLabor , and Energy CEnergy whereas the fixed cost CFixed j j includes the cost elements for Machine CMachine , Building CBuilding , j j Maintenance CMaintenance , and Overhead COverhead . The mathematical re­ lations are shown in equations (1)–(4), where n is the total number of considered process steps and j is the number of the specific process step. n ∑ CTotal = 4.1. Process-related simulation parameters [1] Increased roll-to-roll working speed (1) j CProcess The speed at which the so-called roll-to-roll processes (Coating & Drying, Calendering, and Slitting) are performed depends on material properties, process competencies and machine capabilities. An increase in working speed decreases the time needed to produce the electrodes required for one battery cell. This effect is represented in the cost model with a reduced cycle time for these process steps (CTj=Coating&Drying , CTj=Calendering , CTj=Slitting ). Where the cycle time is in general calculated process step specific, for the process steps Coating & Drying, Calen­ dering and Slitting the identical parameters are used. Namely, working width of machine, working speed, cathodes/anodes per cell, width of cathode/anode, length of cathode/anode are used. A reduced cycle time reduces the number of machines needed to produce a target volume of a product (NM). While a higher working speed of the roll-to-roll process steps increases the machine capabilities required, the cost-increasing effects must also be considered. In particular, this means higher unit investments and larger machine footprints for all roll-to-roll processes. Within this increase, additional capabilities are crucial for process step j = Coating&Drying, as a higher number of electrodes must be dried in a certain time. This is technically achieved by increasing the length of the dryer that is part of the Coating & Drying machine unit. Accordingly, a linear cost function for machine unit investments and the machine footprint of the dryer unit must be assumed. A parameter value of 25 m j=1 j CProcess j = CVariable + j CFixed (2) j j j j CVariable = CMaterial + CLabor + CEnergy (3) j j j j j CFixed = CMachine + CBuilding + CMaintenance + COverhead (4) 3.2. Input parameters The presented cost model consists of more than 250 parameter characteristics from the Product Characteristics, Technical Observa­ tions, Operating Conditions, and Factor Prices categories. The origin of the data for the specific parameters used in the model is described in the following. Product Characteristics were mainly defined using the CellEst bat­ tery cost model by Wentker et al., 2019. It proposes the selected cell dimensions, the pouch cell format and different cell chemistries, reflecting a battery cell for a vehicle that is purely electric. For some parameters that are not considered in CellEst (e.g. process-related ma­ terial cost like NMP), data from BatPac has been included in the analysis. Table 1 lists the product characteristics used for this study. 6 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 min− 1 is characterized as state-of-the-art and therefore applied in the Base Scenario (Kwade et al., 2018). Regarding future developments, it is reported that a coating speed of up to 100 m min− 1 is feasible and is therefore set for the Optimized Scenario (Schmitt, 2015). To materialize this higher coating speed, the bead pressure and low-flow limit (maximum speed at a given film thickness, or the minimum film thick­ ness at a given speed, at which the coating bead remains stable) and its associated parameters must be controlled especially to avoid film break-ups and to ensure film uniformity as basis to not deteriorate scrap rate and/or cell performance (especially unfavorable current distribu­ tions in operating cell and reduced power density due to increased cell volume) (Carvalho and Kheshgi, 2000; Romero et al., 2004; Schmitt et al., 2014). Within the Formation procedure, the cell is charged and discharged several times using specific charging rates to build up the solid elec­ trolyte interphase (Winter 2009). Both, the number of charge and discharge cycles required and the rate at which they can be executed (C-rate), defines the duration of the formation procedure within process step j = Formation&Final Sealing. Optimizing these parameters results in a cycle time reduction for this process step (CTj=Formation&Final Sealing ). For the Base Scenario, reported as state-of-the-art, we assume a typical formation procedure with 3.5 charge/discharge cycles and C-rates ranging from 0.05 to 0.5 C resulting in a formation time of 75 h (Wood et al., 2015). In the Optimized Scenario, a reduced formation protocol is followed with 1.5 charge/discharge cycles and a C-rate of 0.5 C that totals in 11 h (Mao et al., 2018). As the graphite anodes are thermo­ dynamically unstable against the electrolyte, an optimal solid electro­ lyte interphase layer is the basis to protect the graphite-anode from adverse ongoing reactions with the electrolyte (Arora, 1998) which would have negative effects on cell capacity due to continuous elec­ trolyte decomposition, and graphite exfoliation (Mao et al., 2018; Winter 2009). Thus, when further reducing charging cycles and/or increasing C-rates, the product specific fulfillment of the solid electro­ lyte interface requirements must be considered. To reduce formation time while fulfilling these requirements at the same time, optimized charging protocols (Mao et al., 2018) as well as optimized electrode surfaces and electrolyte compositions (Winter 2009) can be key to success. [2] Usage of alternative solvent As described in section 2.1, water is currently used as solvent to produce active anode material slurry and teratogen and toxic NMP (Nmethyl-2-pyrrolidone) is used to produce active cathode material slurry. With regard to future, it is reported that water can also be used as solvent to produce the active cathode material slurry (Bresser et al., 2018a; Du et al., 2017; Ibing et al., 2019; Wood et al., 2015). Using water instead of NMP results in three beneficial main effects: (1) The solvent recovery process can be completely omitted as it is only necessary due to the js=Solvent revovery properties of the NMP (ACSupporting = 0). (2) The dryer length of the Coating & Drying unit can be reduced as the evaporation rate of water is twice as high as that of NMP (Wood et al., 2015). This reduction leads to reduced machine unit investments j=Coating & Drying j=Coating & Drying (UMachine ) [5] Decreased end-of-line scrap rate and a decreased Battery manufacturing is very cost sensitive to the scrap produced due to the high number of process steps and the high share of material costs. The end-of-line scrap rate (xj=Aging&Final Control ) indicates the per­ centage of rejected parts identified during process step j = Aging&Final Control. The rate depends on the process quality of the in­ dividual upstream process steps as well as the ability to detect defective parts at an early stage and exclude them from further production pro­ cess. In general, if scrap can be reduced, a lower number of cells must be produced to reach a certain target quantity of salable products. Typi­ cally, 5% of finished cells do not fulfill quality requirements, hence this rate is applied for the state-of-the-art Base Scenario. For the Optimized Scenario we assume the lower bound of 1% as end-of-line scrap (Ciez and Whitacre, 2017). There are in general two strategies to further reduce the end-of-line scrap rate: (1) Increase process quality within the process steps along the whole value chain for which an in-depth un­ derstanding of the process steps, its process parameters as well as its interaction is of utmost relevance (Kwade et al., 2018), (2) The early detection of scrap components, as the later a process step takes place in the value chain the more value is lost when identifying a defect. To materialize strategy (1), data-driven approaches (Turetskyy et al., 2020), and for materialization of strategy (2), advanced quality man­ agement concepts (Schnell and Reinhart, 2016) are currently discussed as promising approaches. ). (3) The material unit cost for NMP machine footprint (FPMachine (Uz=NMP ) can be replaced by the lower cost of water(Uz=Water Material Material ). Hence, a state-of-the-art NMP-process is assumed for the Base Scenario and an aqueous cathode coating process for the Optimized Scenario, respec­ tively. However, a prerequisite for the substitution of NMP is the ability to control the negative effects of using water: (1) Risk of metal disso­ lution in water which can result in capacity losses if ions cannot be intercalated back to the cathode active material, (2) Risk of reduced cycle life due to higher slurry surface tension and lower adhesion strengths between slurry and current collector, (3) Risk of reaction be­ tween the cathode alkaline water solution and the processing machines and the collector foils (Bresser et al., 2018a; Du et al., 2017; Ibing et al., 2019; Wood et al., 2015). [3] Increased stacking speed Within the state-of-the-art z-folding procedure, the stacking speed is defined as the speed at which the electrodes (anodes and cathodes) are positioned in the zigzag fold separator during process step j = Stacking. The speed reached depends on the process competencies and the capa­ bilities of the stacking machine. An increase in stacking speed reduces the cycle time of the process step Stacking (CTj=Stacking ). For the Base Scenario, a state-of-the-art parameter value of 60 electrode sheets picked and placed min− 1 is applied (Mooy, 2019). In recent literature, higher stacking speeds of or even exceeding 180 sheets min− 1 can be observed (Sakti et al., 2015; Schnell et al., 2020; Schünemann, 2015). Therefore, this value is set for the Optimized Scenario. The main chal­ lenge to materialize higher stacking speeds is the increase of machine capabilities to accelerate the highly automated pick-and-place operation while keeping sheet positioning and orientation accuracy. This accuracy is crucial for cell performance (especially capacity and safety), as it determines the area coverage of anode and cathode sheets and prevents the physical contact of the electrode as basis to avoid short circuits (Mooy, 2019). 4.2. Material and design-related simulation parameters [6] Increased electrode thickness Electrode thickness within battery cells can vary depending on the target product specifications of the battery cell. Using thick electrodes requires a fewer number of electrodes to achieve the target cell energy (Ibing et al., 2019; Patry et al., 2015; Singh et al., 2016). Reducing the number of electrodes has three cost-effective impacts: (1) a reduced cycle time of the roll-to-roll processes (CTj=rtr ), the cutting process (CTj=Cutting ), and the stacking process (CTj=Stacking ), (2) a reduced mass of Cathode foil Anode foil non-active electrode materials required (MMaterial ; MMaterial ), (3) an increase in the dryer length of the Coating & Drying machine unit, since a [4] Accelerated formation procedure 7 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 Table 3 Names of simulation parameter, parameter categories, parameter characteristics, and initial sources. Number and name of simulation parameter Parameter category Unit [1] Increased roll-to-roll working speed [2] Usage of alternative solvent Process-related Working speed in m min− Process-related [3] Increased stacking speed Process-related [4] Accelerated formation procedure Process-related [5] Decreased end-of-line scrap rate [6] Increased electrode thickness Process-related Material & designrelated [7] Material change from NMC622 to NMC811 [8] Decreased unit cost for labor [9] Decreased unit cost for building space [10] Increased number of operating days [11] Increased depreciation period for machines [12] Increased depreciation period for buildings Material & designrelated Location-related Location-related Location-related Location-related Location-related Base Optimized Source 25 100 Type of solvent NMP Water Electrode sheets picked and placed min− 1 Number of charge/discharge cycles c-rate Scrap rate in % Coating thickness Cathode in μm Coating thickness Anode in μm Type of material 60 180 3.5 1.5 0.05–0.5 5 65 0.5 1 100 Base: Kwade et al. (2018) Optimized: Schmitt (2015) Base: Ciez and Whitacre (2017); Nelson et al. (2019), 2012; Sakti et al. (2015) Optimized: Bresser et al. (2018a); Du et al. (2017); Wood et al. (2015) Base: Mooy (2019) Optimized: Schnell et al. (2020); Schünemann (2015) Base: Wood et al. (2015) Optimized: Mao et al. (2018) 78 120 NMC 622 38 2345 NMC 811 10 1292 300 360 6 8 25 50 1 Unit costs for labor in $ h− 1 Unit costs for buildings in $ m− 2 Operating days year− 1 Useful life of machines in years Useful life of buildings in years Base & Optimized: Ciez and Whitacre (2017) Base: Schmuch et al. (2018) Optimized: Zheng et al. (2012) Base & Optimized: Derived from CellEst, Wentker et al., 2019a Base: Schmuch et al. (2018) Optimized: Wentker et al. (2019) Base & Optimized: Eurostat (2019) Base & Optimized: Turner and Townsend (2018); ECC, 2019 Base: Nelson et al. (2019); Optimized: Schnell et al. (2020) Base: Nelson et al. (2019) Optimized: Schnell et al. (2020) Base & Optimized: PwC, 2020 Fig. 4. Cost reduction per simulation parameter (single simulation-parameter approach) in $ kWh− 1 @ 35 GWh annual factory capacity; [n] number of single simulation parameters; Categorical affiliation: Process-related, Material & design-related, Location-related. higher quantity of material must be dried per electrode (anode and cathode) in the same time period. This increase leads to higher machine j=Coating& Drying unit investments (UMachine j=Coating&Drying (FPMachine ). Scenario a more cost-effective thicker electrode of 100 μm (Zheng et al., 2012) is assumed. Producing electrodes with a thickness of 100 μm and above is technical feasible. However, as mentioned, the optimum thickness of the electrodes depends on the target product specifications of the battery cell. Thin electrodes are advantageous for products that are sensitive to durability and power. Thick electrodes are used for ) and increased machine footprints For the Base Scenario, a common electrode thickness of 65 μm (Schmuch et al., 2018) is applied, whereas for the Optimized 8 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 still are under consideration) as a large-scale battery factory location. For the Base Scenario, we choose Germany as plant location. This is firstly due to the fact that several battery manufacturers (e.g. SAFT, Northvolt) have decided to localize here (Michaelis et al., 2018) and secondly it shows comparatively high labor cost levels ($38 h− 1, Euro­ stat, 2019). For the Optimized Scenario, we choose Hungary as plant location, as there are already plants in operation or under construction (e.g. Samsung SDI, SK Innovation) (Michaelis et al., 2018) and labor costs are low within European comparison ($10 h− 1, Eurostat, 2019). [9] Decreased unit costs for building space Unit costs for building space (UBuilding ) depend on the location and building requirements. Building requirements are fixed by the product being produced and thus do not vary for a battery cell plant. Location dependency, on the other hand, is variable and thus relevant for the study, since different locations are considered for a battery cell factory. To remain consistent with the labor cost scenarios introduced above, building cost levels of Germany ($2345 m− 2) and Hungary ($1292 m− 2) are considered for the Base Scenario and the Optimized Scenario, respectively (ECC, 2019; Turner and Townsend, 2018).1 Fig. 5. Cost reduction per category (categorized simulation-parameter approach) in $ kWh− 1 @ 35 GWh annual factory capacity. products that are more sensitive to energy density and costs. Conse­ quently, increasing electrode thickness without changing cell di­ mensions (as in the here presented model) results in altered battery characteristics such as increased energy density and decreased power density. As the present study is focused on costs, simultaneous variations in cell specifications are accepted (see Table 1). [10] Increased number of operating days A plant’s operating days per year (DPY) mainly depend on the fac­ tory’s production strategy. While some shut down days per year are necessary for maintenance or due to public holiday, especially factories using highly automated and cost-intensive manufacturing equipment are encouraged to maximize the number of operating days, as this results in an increased annual available operating time of machines (availMT). Therefore, the number of machines required to produce a target volume (NM) decreases. A parameter value of 300 days year− 1 has been set in the Base Scenario to limit fixed assets to a reasonable extent (Nelson et al., 2019). For the Optimized Scenario a value of 360 days year− 1 was taken into account that has been used in recent literature (Schnell et al., 2020). [7] Material change from NMC622 to NMC811 Since cathode active materials represent the most cost-driving cell components (cell cost share > 30% in the Base Scenario) and they currently represent a bottleneck for cell performance (Schmuch et al., 2018), significant research effort has been spent on their development. An improvement in their inherent characteristics, such as specific ca­ pacity or crystallographic density, results in a higher energy content per unit PCEnergy , thereby reducing material input quantities required to produce a certain amount of energy output and hence reducing cell cost (Schmuch et al., 2018). While NMC622 is considered a state-of-the-art cathode active material (Schmuch et al., 2018) and is therefore applied in the Base Scenario, one strategy to enhance energy content is to increase the nickel share. Hence, the use of NMC811 with a higher nickel content is assumed for the Optimized Scenario (Wentker et al., 2019). The resulting product characteristics for both scenarios such as cell energy, energy density and number of electrodes per cell are pre­ sented in Table 1. However, when enhancing the nickel share, the cobalt and manganese shares are reduced simultaneously. As the nickel and the cobalt provide structure stability within the cathode active material, which is primarily responsible for cell properties like thermal stability or cycle life, strategies must be developed to address these challenges to avoid limitations in cell performance (Andre et al., 2015). Promising approaches were already reported in literature related for example to structural design (core–shell structure, concentration gradient, etc.) and intrinsic structure optimization (Wang et al., 2020). [11] Increased depreciation period for machines The time span in which a machine is depreciated is represented by its useful life, LMachine , which depends on its technical durability and the length of time it can economically produce products with the required performance. In general, depreciation periods are longer in low cost countries (e.g. Hungary) compared to high cost countries (e.g. Germany) (PwC, 2020). Battery related literature report periods range from 6 to 8 years. Therefore, we used 6 years (Nelson et al., 2019) for the Base Scenario and 8 years (Schnell et al., 2020) for the Optimized Scenario. [12] Increased depreciation period for buildings 1 To survey the location-specific factor cost of building, we use a two-stage approach as no data are directly available. Turner and Townsend (2018) pub­ lished absolute construction costs for some European countries, and ECC (2019) published percentage values of construction costs for all EU-28 countries. Hence, we defined the United Kingdom as the baseline since, among EU countries, Turner and Townsend published the most comprehensive data for this country, including the differentiation of costs in the United Kingdom ac­ cording to region, industry affiliation, and type of building. Since cell produc­ tion involves many consecutive and complex production steps (Kwade et al., 2018), which are partly performed under increased environmental re­ quirements (Ahmed et al., 2017; Nelson et al., 2015; Yoshio et al., 2009), we use values from the industrial high-tech factory/laboratory category to calcu­ late an average cost based on the region-specific values in the United Kingdom. Using this baseline value from Turner and Townsend and the percentage values from EEC, we calculate the construction cost per square meter for each Ger­ many and Hungary. 4.3. Location-related simulation parameters [8] Decreased unit costs for labor The unit costs for labor (ULabor ) depend on the location, the required competence level of workers, and the industry. The required level of competence and industry are fixed by the product and are thus not variable. Location dependency, on the other hand, is variable and thus relevant for this study, since different locations are considered for a battery cell factory. In Europe, several countries have been chosen (or 9 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 Fig. 6. Cost walk from the Base Scenario to the Optimized Scenario based on cost elements (overall simulation-parameter approach) in $ kWh− factory capacity. The time span in which a building is depreciated is represented in its useful life, LBuilding , which depends on its durability and production re­ quirements regarding the shop floor layout and environment. Produc­ tion requirements can change over time, even if the same type of product is manufactured. Again, to remain consistent with the building cost scenarios, Germany as a high cost country is chosen for the Base Sce­ nario (depreciation period of 25 years for buildings, PwC, 2020) and Hungary as a low cost country is chosen for the Optimized Scenario (depreciation period of 50 years for buildings, PwC, 2020). To enable an overarching discussion of cost effects and to derive a total cost level, beside the evaluation of the single simulation parameters and the evaluation of the described scenarios, an evaluation based on parameter categories (Process-related, material & design related, and location-related simulation parameters) is conducted. Table 3 lists the simulation parameters, the associated characteris­ tics, their sources and the associated parameter category. 1 @ 35 GWh annual parameter approach). Thereby, a cost walk at the cost-element level is presented from the total costs of the Base Scenario to the total costs of the Optimized Scenario. The total costs are $106 kWh− 1 in the Base Scenario and $64 kWh− 1 in the Optimized Scenario. This corresponds to a cost reduction of 40%. The cost walk shows that the presented simulation parameters reduce, in particular, the cost elements Material, Machine and Labor. The improvement in the cost element Material mainly results from Increased electrode thickness and Material change from NMC622 to NMC811 that both induce an increased energy content per cell, thereby reducing material input quantities required to produce a certain amount of energy output. For cost elements Machine and Labor, this reduction is regarding that, on the one hand, in the Optimized Scenario, fewer factor quantities (less machinery and less working hours per unit of output) are necessary to produce the target volume, and, on the other hand, the factor price for labor is lower. Looking at the cost reductions by cost element at the single-parameter level reveals that all simulation pa­ rameters have a cross-cost-element effect. Nevertheless, the level of the effect of each parameter differs. The simulation parameters for Increased electrode thickness and Material change from NMC622 to NMC811 affect each of the eight cost elements. On the other hand, the simulation pa­ rameters Decreased unit cost for labor, Decreased unit cost for building space, and Increased depreciation period for buildings each affect only two of the eight cost elements. When looking at the superordinate catego­ rization level, it is striking that all simulation parameters from the process-related and material & design-related categories have a strong cross-cost element, as they affect at least six of the eight cost elements considered. On the other hand, the simulation parameters of the location-related categories influence only two or three of the eight cost elements considered. Although all parameter characteristics within the Optimized Sce­ nario are derived from literature, there is an uncertainty to which extend the assumed parameter optimizations can be achieved within future large-scale manufacturing. To evaluate this uncertainty a sensitivity analysis is conducted and can be found in Appendix C. Transforming these overall cost results into vehicle-level figures and linking them to revenues and profits illustrates the importance of costefficient battery production. Multiplying the average energy content of a battery for a mid-range vehicle, 60 kWh (Schmuch et al., 2018), with the cost per kWh from the Base Scenario and the cost per kWh from the Optimized Scenario results in a cost difference of approximately $2500 per vehicle, thereby in the case of full materialization, significantly impacting the economic success of EVs. Fig. 7 shows the percentage distribution of the total costs among the cost elements for the two overall scenarios (overall simulationparameter approach). In both the Base Scenario and the Optimized Scenario, the cost elements that drive costs the most are Material and Machine. The sharp increase of the Material cost share in the Optimized 5. Results and discussion The following section presents and discusses the results of the study, which are based on the presented model architecture (see Section 3.1), the presented input parameters (see Section 3.2), the presented simu­ lation parameters (see Section 4) and a targeted annual production ca­ pacity of 35 GWh. Fig. 4 shows the cost reduction per simulation parameter (single simulation-parameter approach) in $ kWh− 1. The highest values result from the two material and design-related optimizations Increased elec­ trode thickness at $12.9 kWh− 1 and Material change from NMC622 to NMC811 at $8.9 kWh− 1. This is followed by the process-related opti­ mization Accelerated formation procedure at $6.9 kWh− 1 and the location-related optimization Decreased unit cost for labor at $6.3 kWh− 1. The value of each of the remaining simulation parameters is < $5 kWh− 1. Fig. 5 shows the results based on the categorized simulationparameter approach. The results reveal that the highest cost re­ ductions, at $20.3 kWh− 1 result from the process-related category. This is followed by the material & design-related and location-related cate­ gories, with cost reductions of $19.4 kWh− 1 and $14.9 kWh− 1, respec­ tively. The result that process-related innovations have the highest impact on cell cost indicates that cost-optimal cell production depends in particular on company-and factory-specific process competence. Compared to this process competence, the often-discussed locationdriven parameters (Brodd and Helou, 2013; Duffner et al., 2020a), which are represented by the location-related category, are of minor importance. Especially in the context of labor, this is because batteries are manufactured using highly automated and thus less labor-intensive processes. Fig. 6 shows the results of the overall scenarios (overall simulation10 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 Fig. 7. Percentage of costs per cost element for the Base Scenario and Optimized Scenario @ 35 GWh annual factory capacity. Fig. 8. Cost share between process steps in % for the Base Scenario and Optimized Scenario @ 35 GWh annual factory capacity. Scenario results from the disproportionately low decrease of material cost compared to other cost elements. This is due to the fact that only three out of twelve examined simulation parameters have an impact on material costs. In contrast, Machine cost decreases overproportionately since it is optimized by nine simulation parameters. In addition, it is striking that the proportion of the cost element Labor is 2% in the Optimized Scenario, compared to 8% in the Base Scenario. This effect is mainly driven by the simulation parameter Decreased unit cost for labor as it has a high absolute value and mainly affects the cost element Labor, whereas the other simulation parameters with a high value, as 11 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 described, have a much stronger cross-cost-element effect. The high ratio of the cost elements Material (77% in the Optimized Scenario) and Material-Scrap (6% in the Optimized Scenario) to total costs show that large-scale battery-cell production is highly sensitive to net material input quantities, scrap rates and costs of purchased mate­ rials. From a materials-related point of view, measures to optimize cell chemistry that focus on using fewer and more cost-effective materials are appropriate to reduce both Material and Material-Scrap costs. From a process-related point of view, the focus has to be set on Scrap as its cost impact is amplified by the large number of interlinked and complex process steps in cell production. Thus, measures to produce a smaller number of process-step-specific defective parts and measures to identify defective produced parts as soon as possible so that no additional costs arise from subsequent process steps are suitable to reduce MaterialScrap costs. In addition to the cost elements Material and Material-Scrap, the cost element Machine should be the focus of future cost-reduction activities, as this cost element accounts for the second largest share in the Opti­ mized Scenario at 8%. Both operational and strategic measures can contribute to reducing costs from this cost element. From an operational point of view, measures that contribute to the production of specific quantities of acceptable parts with fewer machines are suitable. These include measures to reduce cycle time, increase the annual operating time (e.g. by reducing unplanned downtime), or to reduce the scrap rate. From a strategic point of view, cost reductions can be achieved by extending the useful life of machines. This would be conceivable if a cell manufacturer, after a period of producing state-of-the-art cells (regarding quality and performance), decides not to scrap deprecated machines but continue producing battery cells with lower performance and quality requirements. Fig. 8 shows the process steps that drive costs the most in the Base Scenario and the Optimized Scenario. To increase comparability with the focus on operative process step execution, Material and MaterialScrap have been excluded for evaluation. This approach was chosen because material costs, as described above, make up a high proportion of the cost of battery cells and are for calculation purposes allocated to a specific process step. This allocation is correct from a calculation point of view but not ideal for comparability of the process steps, since the process steps in which cost-intensive materials are used would exhibit disproportionately high costs, even though the added material costs are not directly related to execution of the cell making process. In the Base Scenario, the three most cost-driving process steps are Formation & Final Sealing (25%), Stacking (22%) and Coating & Drying (12%). Due to their cost-driving properties, these process steps have been focused within past research. The reported optimization has been considered within the Optimized Scenario, which reduces their share significantly. Formation loses its cost dominance to Mixing as a result of the Accelerated formation procedure and plays only a subordinate role in the Optimized Scenario. Mixing process costs get most relevant as they are only decreased by one optimization of the process-related category (Decreased End-of-line Scrap). The process steps Stacking and Coating & Drying however, remain cost drivers in the Optimized Scenario despite the optimized parameter assumptions of a tripled stacking speed from 60 to 180 sheets min− 1 (simulation parameter: Increased stacking speed), a quadrupled roll-to-roll speed from 25 to 100 m min− 1 (simulation parameter: Increased roll-to-roll speed) and a reduction of the cathode dryer length by replacing water with NMP (simulation parameter: Usage of alternative solvent). It should also be noted that in the Optimized Scenario, the cost-driving process steps Mixing, Coating & Drying and Stacking are supplemented by the process step Aging & Final Control. As this step is no roll-to-roll process and no specific parameter optimization has been simulated, its cost share is increasing compared to the Base Scenario. Interestingly, in the Base Scenario, process costs are almost evenly shared between the three superordinate main processes Electrode Production (32%), Cell Production (37%), and Cell Conditioning (31%). In the Optimized Scenario, the dominance of the Mixing process and the reduction in Formation & Final Sealing lead to a cost shift from Cell Conditioning (20%) to Electrode Production (44%). The process cost share of Cell Production remains at the same magnitude (36%). Taking all the results into account, for cost reduction in optimized large-scale battery cell factories, the focus should be on the process steps Mixing, Coating & Drying, Stacking, Formation & Final sealing and Aging & Final Control. For this purpose, in the following, process-step-specific measures for cost reduction are described that complement the previ­ ously described cost-reduction measures. • Mixing: Measures to reduce the quantity of material to be mixed per salable cell, such as reducing the solvent quantity; measures to reduce mixing time, such as optimizing process specification; and measures to optimize batch capacity. In addition, from a cost perspective, promising approaches are taken in science and industry to switch from batch-wise mixing to continuous mixing (Bühler Group, 2017; Dreger et al., 2015). • Coating & Drying: Measures to further increase working speed; measures to increase working width; measures to reduce solvent quantity up to complete elimination (dry coating); measures to reduce the number of electrodes, such as increasing the coating thickness. • Stacking: Measures to increase the pick and place speed of the electrodes; measures to reduce positioning time during cell ex­ change; measures to reduce the number of electrodes, such as increasing the layer thickness. • Formation & Final Sealing: Optimized cycle programs to reduce cycle time. Therefore, measures to reduce number of cycles or to increase the charging rate per cycle are appropriate. • Aging & Final Control: Measures to reduce aging duration due to improved quality forecast methods. Fig. 9 compares the results of the Base Scenario and the Optimized Scenario with the reported cell costs across battery-related literature. Therefore, a comprehensive literature review of reported cell cost esti­ mations has been conducted.2 Firstly, as cathode chemistry strongly influences cell cost, values for NMC have been taken into account wherever possible to allow for a more precise comparison with the re­ sults of the present study. Secondly, as not all publications report cost based on cell level (e.g. on pack level), corrective factors have been calculated (derived from Nelson et al., 2019) and applied to the origi­ nally reported cost values. The underlying data, associated sources and corrective factors are included in Appendix D. The plot of the reported values over the years of publication shows a continuously decreasing cost trend that is characterizing for technologies that are undergoing mass industrialization. Reported cost estimations range from far above $200 kWh− 1 in 2015 (Sakti et al., 2015) to below $100 kWh− 1 in 2018 (Schmuch et al., 2018). Furthermore, a tendency to a lower spread be­ tween values can be noticed throughout the years which might result from increasingly existent and accessible empirical evidence in industry. The comparison of the derived value of our state-of-the-art oriented Base Scenario ($106 kWh− 1, horizontal dotted line) with literature values shows that it is in line with recently reported values albeit it lies on the 2 To survey battery cost literature, 14 publications between 2014 and 2019 have been reviewed. Wherever possible, reported values regarding NMC have been taken into account to allow for a more precise comparison with the pre­ sent study. If multiple values have been reported (e.g. due to different sce­ narios) an average of those values has been calculated. As values have not always been reported based on cell level, these have been normalized by corrective factors derived from Nelson et al. (2019): Reported pack cost have been multiplied by 0.75 and reported cell material cost have been multiplied by 1.31 to derive a cell-based cost value. 12 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 Fig. 9. Comparison of costs for NMC based battery cells reported in literature over time. lower end of the range. In contrast, the value of the Optimized Scenario ($64 kWh− 1, horizontal solid line) is significantly lower than historically published cost estimations. The comparison with the most recent liter­ ature shows that costs of both, the Base Scenario and the Optimized Scenario, are significantly lower than those reported for example by Ciez and Whitacre (2017). The main reason for this is that Ciez and Whitacre used manufacturing parameters based on a much smaller factory size (0.87 GWh annual production capacity). Although simulation for larger factory sizes is conducted, cost decrease is limited as the manufacturing parameters are not adapted. Compared with Nelson et al. (2019), the values are in a similar range, with costs for the Base Scenario above the BatPaC range and costs for the Optimized Scenario below the BatPaC range. In summary, we introduce with the Optimized Scenario a lower cost level for the manufacturing of battery to literature and give di­ rections which technical parameters reported in literature must there­ fore be industrialized in large-scale. model that can be used as basis for data-driven decision making within location decisions, make or buy decisions and to evaluate process and material alternatives. (3) We introduce and prove the feasibility of a new and lower cost level which, if materialized, will have a positive effect on the EV penetration rate. Accordingly, it should be considered in future research studies and product planning of automotive original equipment manufacturers cost optimizations. The presented model has several limitations that need to be addressed by future research. First, it is limited to lithium-ion battery technology, which is currently the most beneficial battery technology for automotive applications (Betz et al., 2019; Bresser et al., 2018b; Placke et al., 2017; Schmuch et al., 2018). However, there are other technologies such as lithium metal, solid-state, sodium-ion, lithium|| sulfur, or metal||air batteries with promising advantages for some characteristics such as costs or safety (Eftekhari and Kim, 2018; Tan et al., 2017; Zhang et al., 2017) and also for other applications than automotive. These new technologies are still in the development stage, and it will take years until they are produced in large scale, but the presented approach can be adapted to them. Second, the selection of simulation parameters is focused on the process-related, material & design-related and location-related parameters that drive cost most. This cross-category approach gives a comprehensive indication of current and future cost levels within battery manufacturing but makes no claim to completeness within each single category. As described in Section 5, for example, there are also future process improvement possibilities for the process steps Mixing and Aging & Final Control, which are not considered in the Optimized-Scenario. Third, although the used pa­ rameters are derived from literature, are validated by industry experts, and are translated into costs by using an established cost estimation technique, the calculated costs are not yet validated by empirical data of a battery cell manufacturer what offers together with the other mentioned limitations new perspectives for future research. 6. Conclusion This study at hand successfully applies the process-based costmodelling technique to the manufacture of battery cells. Accordingly, the study contributes to the research fields of both process-based cost modelling and battery technology. The PBCM research field is complemented by the application of the technique to a complex technology whose manufacturing process con­ sists of a variety of individual, complex, and interdependent process steps and whose engineering, scientific, and technological principles have not been fully researched. Therefore, we enlarge the PBCM framework introduced by Field et al. (2007). In the field of battery research, we make several contributions (1) We give directions how further cost reductions within large-scale manufacturing can be achieved (Optimized Scenario) and which cost drivers within process steps, cost elements and parameter categories should be focused for future cost reduction activities. (2) We introduce a 13 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 Declaration of competing interest related to this manuscript. The authors of this article states that there are no conflicts of interest Appendix Appendix A. Detailed cost model Overall The following describes the calculation of the variables, which have an overarching character as they are used as basis for the calculation of various j cost elements. The first variable of this type is the annual gross number of units PVEffective that must be produced within process step j to reach the required number of annual salable units, PVSalable . Therefore, the logic must consider that a process step must compensate for the scrap losses of the subsequent process steps. This means that process steps located early in the process chain must produce more units than later steps. For the last process j step within the presented process chain, the gross number of units required, PVEffective , is calculated as shown in equation (5). For the other process steps, the gross numbers of units required are calculated as shown in equation (6), wherexj is the machine-specific scrap losses for process step j. PVSalable j ) PVEffective =( 1 − xj j+1 PVEffective j ) PVEffective =( 1 − xj (j = n) (5) (j < n) (6) A second key variable is the number of required machines, Nj , at process step j. This is calculated by the process-step-specific annual operating time required to produce the target volume, reqMT j , and the annual available operating time of the machine, availMT j , at process step j. The result is rounded to the next highest whole number, as it is assumed in the present study that machines may be underutilized as they are not used to produce other products. j NMachine = reqMT j availMT j (7) The annual time required to produce the target volume, reqMTj , at process step j is calculated as the product of the associated cycle timeCT j , which j is the time interval after one unit is produced, and the associated gross number of cell equivalents required, PVEffective . (8) j reqMT j = CT j x PVEffective The annual available operating time of a machine, availMT , at process step j is calculated according to equation (9), where DPY is the operating days per year, NOS is the number of shifts per day, OHS is the operating hours per shift, UB is the unpaid breaks hours per shift, PB is the paid break hours per shift, and UDj is the process-specific unplanned downtime hours per shift− 1. ) ( (9) availMT j = DPY x NOS x OHS − UB − PB − UDj j The costs presented in this study are on a kWh cell energy basis. Therefore, the annual cost for each cost element, ACjElement, must be divided by the number of annual salable units (number of cells), PVSalable , an the energy content per unit (kWh cell − 1) PCEnergy, as shown in equation (10). Element is used to differentiate between the cost elements Material, Labor, Energy, Machine, Building, Maintenance, and Overhead. j CElement = j ACElement PVSalable x PCEnergy (10) Machines and buildings are capital goods used over a specific period. In the present model, this is considered by distributing the investment in capital goods such as machines and buildings over their life cycles. In addition, opportunity costs are considered by means of a capital recovery factor. These costs arise because capital is tied up in machines and buildings and thus cannot be used to generate alternative revenue. The annual allocated costs Rje for process step j are calculated as shown in equation (11), where Uje is the unit cost for a machine or building, e is used to differentiate between machine and building, r is the annual discount rate, and Lje is the useable lifetime in years. j Rje = Uej r(1 + r)Le (11) j Le (1 + r) − 1 Material j The calculation of annual material costs, ACMaterial , for process step j considers that several material types z may be used within process step j. Therefore, annual material costs, j ACMaterial , are calculated as the sum of the corresponding annual material-type-specific material costs, ACzj, Material , as shown in equation (12), where z is a specific material type and d is the total number of material types used within process step j. j ACMaterial = d ∑ (12) ACj,z Material z=1 14 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 The annual material costs for a material type z within a process step j, ACzj,Material , are calculated using equation (13), where Mzj,Material is the net mass z of material type z required, within process step j, to produce one unit; UMaterial is the unit cost of material type z (usually currency weight− 1); j is the process-step-specific annual gross Scrapzj,Material is the percentage of specific losses of additional material type z within process step j; and PVEffective number of units required. z ACj,Material z z = Mj,Material x UMaterial x total 1 j x PVEffective 1 − Scrapzj,Material (13) To ensure a holistic calculation and enable computation of the cost elements for Energy CjEnergy and Overhead CjOverhead , total annual material costs, were calculated in the present cost model as shown in equation (13). For evaluation, we focused on the part of the annual material costs ACzj,Material total , that are potentially influenced by production, which, in principle, is the part induced by scrap losses. Annual material-scrap costs, ACzj,Material scrap , are calculated as shown in equation (14). This approach ensures the focus of the evaluation remains on the costs relevant to manufacturing. Otherwise, the results would be overshadowed by the part of material costs that is not potentially influenced by production, as this is dominant within battery cells. z ACj,Material (14) j z z = Mj,Material x UMaterial x Scrapzj,Material x PVEffective scrap Labor j As shown in equation (15), the labor costs for process step j are calculated as the product of the number of machines required for that step, NMachine , the number of laborers required per machine, operating time, APOT j . j NLaboreres per Machine , the unit cost of labor, j ULabor (usually in currency per unit time), and the annual paid (15) j j j j j ACLabor = NMachine x NLaboreres = Supporting) per Machine x ULabor x APOT ; (j ∕ Labor costs for process step j = Supporting are calculated differently, since this process step cannot be described on a machine basis. Nevertheless, the same calculation logic is used, referring to reference bases (e.g., annual GWh plant capacity) instead of machines. As process step j = Supporting consists of various sub-processes with different characteristics, the reference bases were built to be specific to each sub-process step. For each reference base and sub-process step, the necessary number of laborers was determined. The following reference bases were used: annual factory capacity for the sub-process - Inter-process material handling, Control lab, and Receiving and shipping including scrap recycle; annual amount of NMP solvent used for the sub-process step -Solvent recovery; and footprint required for the processes to be carried out under dry room conditions (cell production) for the subprocess step -Dry room management. Based on this, the labor costs of process step j = Supporting comprise the sum of the labor costs of the subjs processes, as shown in equation (16), where NRBs is the number of reference bases required; NjsLaboreres per RB is the number of laborers required per reference base; UjLabor is the unit cost of labor (usually in currency unit time− 1); APOTjs is the annual paid operating time; js is a specific sub-process of process step j = Supporting, and ns is the total number of sub-processes of process step j = Supporting. j ACLabor = ns ∑ (16) js js js js NRBs x NLaboreres per RB x ULabor x APOT ; (j = Supporting) js Machine j As shown in equation (17), the annual machine costs ACMachine for process step j ∕ = Supporting are calculated as the product of the annualized equivalent of the machine investment of produced units, j PVEffective . j RMachine j and the number of machines NMachine required to produce the process-step-specific gross target number (17) j j ACMachine = NMachine x RjMachine ; (j ∕ = Supporting) As described in the section on the labor cost element, process step j = Supporting cannot be described on a machine basis. Therefore, the cost element for this process step, ACj=Supporting , is calculated using the described reference bases, where NjsRBs is the number of reference bases required; Machine RjsRB Machine is the annualized equivalent of the machine investment per reference base; js is a specific sub-process of process step j = Supporting; and ns is the total number of sub-processes of process step j = Supporting. The following equation describes the calculation: j=Supporting ACMachine = ns ∑ js NRBs x RjsRB (18) Machine ; (j = Supporting) js Building j As shown in equation (19), the annual building costs for process step j ∕ = Supporting, ACBuilding , are calculated as the product of the annualized equivalent of building investment, RBuilding ($ m− 2), the number of machines required to produce the process-step-specific gross target number of cell j equivalents, j NMachine , j and the footprint per machine, FPMachine (m2 machine− 1). (19) j j ACBuilding = RjBuilding x NMachine x FPjMachine ; (j ∕ = Supporting) As shown in equation (20), the building costs for process step j = Supporting, CjBuilding are again calculated using the reference bases, where NjsRBs is the number of reference bases required;FPjsRB is the footprint per corresponding reference base; js is a specific sub-process of process step j = Supporting; 15 F. Duffner et al. International Journal of Production Economics 232 (2021) 107982 and ns is the total number of sub-processes of process step j = Supporting. j=Supporting = CBuilding d ∑ (20) js RjBuilding x NRBs x FPjsRB ; (j = Supporting) z=1 Energy, maintenance, and overhead j j j As shown in equations (21)–(23), the annual costs for Energy ACEnergy , Maintenance ACMaintenance , and Overhead ACOverhead for process step j are j calculated based on the percentage of surcharge rates SR. The surcharge rates are applied to known cost elements (e.g., Machine ACMachine ). Both the surcharge rates SR and associated application bases are specific for the production of battery cells. ) ( j j j x SREnergy ACEnergy = ACLabor + ACMaterial (21) j j ACMaintenance = ACMachine x SRMaintenance (22) ) ( j j j j ACOverhead x SROverhead = ACMachine + ACBuilding + ACMaintenance (23) Appendix B. Overlapping phenomena between simulation parameters Fig. 10. Pairwise combination of simulation parameters and resulting effect on cell cost. Appendix C. Sensitivity analysis3 3 For each simulation-parameter the improvement between Base Scenario and Optimized Scenario has been calculated. To account for uncertainty regarding the extend of achievement has been varied. (1) Only 80% or (2) 120% of improvement can be materialized. The resulting impacts on cell costs are displayed in the tornado plot. [2] Usage of Alternative solvent & [7] Material change from NMC622 to NMC811 have been excluded from the analysis as the parameter value can either be yes or no in both cases 16 International Journal of Production Economics 232 (2021) 107982 F. Duffner et al. Fig. 11. Tornado plot showing the sensitivity of simulation-parameters. Appendix D. Reported cell cost estimations in literature Table 4 Source, year of publication and reported battery cost Source Year Cathode material Cost Base Reported cost [$ kWh− 1] Average value [$ kWh− 1] Corrective Factor [-] Resulting cell cost [$ kWh− 1] Gallagher et al. Patry et al. Sakti et al. Berg et al. Nelson et al. Wood et al. Schünemann 2014 2015 2015 2015 2015 2015 2015 NMC NMC NMC NMC NMC NMC NMC Pack Cell Pack Cell Pack Pack Cell 234 251 341 224 188 437 203 0.75 – 0.75 – 0.75 0.75 – 175 251 256 224 141 327 203 Petri 2015 NMC 122 1.31 159 Ciez and Whitacre Ahmed et al. Berckmans et al. Schmuch et al. 2017 NMC Cell mat. Cell 178; 289 306; 231; 231; 239; 247 545; 325; 265; 230 224 188 503; 370 189; 173; 163; 156; 189; 188; 188; 187; 292; 267; 245 122 244; 182; 174 200 – 200 2017 2017 2018 NMC NMC NMC 811 148; 155; 139; 146 432; 300; 293 79; 68 147 342 73 0.75 0.75 1.31 110 256 96 Wentker et al. 2019 NMC 811 Pack Pack Cell mat. Pack 142 0.75 106 Nelson et al. 2019 NMC 811 Cell 179; 167; 154; 143; 163; 152; 139; 129; 134; 125; 113; 103 127; 109; 106; 103; 132; 105; 101 112 – 112 Funding sources This work was partly funded and supported by the Bundesministerium für Bildung und Forschung (BMBF) and the Ministerium für Wirtschaft, Innovation, Digitalisierung und Energie des Landes Nordrhein-Westfalen within the project BenchBatt [03XP0047A]. References Arinicheva, Y., Wolff, M., Lobe, S., Dellen, C., Fattakhova-Rohlfing, D., Guillon, O., Böhm, D., Zoller, F., Schmuch, R., Li, J., Winter, M., Adamczyk, E., Pralong, V., 2020. Ceramics for electrochemical storage. 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