Fiber-optic ultrasound transmitter based on multimode interference in curved adhesive waveguide HUIBO FAN,1,2,3 LIANG CHEN,1 AND XIAOYI BAO1,4 1 Department of Physics, University of Ottawa, Ottawa, Ontario K1N 6N5, Canada College of Physics Science and Technology, Yangzhou University, Yangzhou 225002, China 3 e-mail: hbfan@yzu.edu.cn 4 e-mail: xbao@uottawa.ca 2 Received XX Month XXXX; revised XX Month, XXXX; accepted XX Month XXXX; posted XX Month XXXX (Doc. ID XXXXX); published XX Month XXXX Fiber-optic ultrasound transmitters can be used in structural health monitoring (SHM), material characterization, and biomedical imaging. However, the bandwidth of current fiber-optic ultrasound transmitters is tens of MHz which prevents the ultrasound image on cells with resolution of µm level; for SHM, broadband high sensitivity detection is essential for small defect identification, and they are not available. Here, ultracompact in-fiber ultrasound transmitter is proposed by using the multi-mode interference in the curved UVcured adhesive waveguide, which is fabricated between two fiber endfaces over a sandwiched core-offset spliced fiber segment. The curved adhesive waveguide can improve the contrast of device reflection spectrum from 2.7 dB to 21.7 dB. The ultrasound is generated by optical pulse excitation via photoabsorption and thermal expansion of UV-cured adhesive, and then detected via the multi-mode interference of the same waveguide over hundreds of Hz to 306 MHz broad transverse acoustic waves. This ultra-compact and cost-effective device offers new opportunities to the advanced biomedical and ultrasound-based applications. © 2019 Optical Society of America http://dx.doi.org/10.1364/OL.99.099999 Ultrasound transmitter is widely used in structural health monitoring, nondestructive test (NDT) and biomedical imaging [1-4]. Traditional piezoelectric transducer (PZT) with bulky size and narrow frequency bandwidth is susceptible to electromagnetic interference. Based on photoacoustic effect, laser-ultrasound generation has shown great potential to offer higher frequency in various applications [5,6]. In laserultrasound generation, an optical-absorption material could convert pulsed optical energy into thermal energy with thermal expansion, and then release to produce acoustic wave between two optical excitations [7-9]. Especially, fiber-optic ultrasound transmitters have been further studied based on various photoacoustic materials [6,10-12], such as metal films [13], gold nanocomposite or carbon nanotube mixing with poly-dimethysiloxane (PDMS) [12,14], and epoxy and graphite mixtures [15]. A typical fiber-optic ultrasound generator consists of two reflectors at the fiber end face covered by above mentioned photoacoustic materials, and heated by a pulse laser. The fiber diameter determines the transverse acoustic frequency. For SMF 28 with cladding diameter of 125 µm, it gives tens of megahertz as a transducer [14,16]. An alternative approach is to generate the ultrasound wave from side wall of the optical fibers [17,18]. For instance, fibers with tiny core-offset dislocation could couple light from core mode into cladding modes to enable the ultrasound generation with bandwidth of around 30 MHz via the covered absorption material with thickness of around 200 µm [18]. It is noting that an ideal material for strong photoacoustic generation should have large photoabsorption coefficient and large coefficient of thermal expansion (CTE). Photoacoustic conversion materials such as PDMS and epoxy resin have been widely used for ultrasound generation, while little report on the other polymer materials, such as UV-cured adhesive. Norland Optical Adhesive 61 (NOA 61) with high photoabsorption coefficient and CTE at the room temperature has a potential for ultrasound generation [18,19]. Furthermore, a PZT ultrasound sensor or a hydrophone is used to response the acoustic wave, increasing the cost and complexity [18,20]. Laser-induced ultrasound generation and integrated optical probe-sensing measurement with high sensitivity are a potential for ultrasound transmitter. In this Letter, an ultra-compact fiber-based ultrasound transmitter is fabricated, and characterized via a curved UVcured adhesive waveguide as an ultrasound generator. Multimode interference in the same adhesive waveguide between two fiber endfaces over a sandwiched core-offset spliced fiber segment acts as an ultrasound sensor. The curved waveguide greatly increases high-order waveguide modes and enhances multi-mode interference at one passage time of waveguide to increase high frequency response, unlike normal Fabry-Perot interferometers rely on multiple reflection to enhance quality factor at cost of time response. Pulsed pump is used to excite the adhesive waveguide, resulting in the transverse acoustic wave detected by the continuous-wave probe light. Especially, only adhesive is used for the ultrasound generation. Broad bandwidth from hundreds of Hz to 306 MHz is generated and detected thanks to gradually varied thickness of adhesive waveguide along the fiber. amplifier (EDFA) as a broadband source illuminates the device and then reflection spectrum is obtained via an optical circulator to characterize the device. Fig. 1(g) is the fiber device photograph before covering UV-cured adhesive. Fig. 1. (a)-(d) The fabrication process of curved UV-cured adhesive waveguide between two fiber endfaces. (e) Side-view and crosssection diagram of curved adhesive waveguide. (f) A typical photograph of UV-cured adhesive dripping process. (g) & (h) Side-view photographs before and after covering UV-cured adhesive. Fig. 1(a)-1(d) show the fabrication steps of proposed ultrasound transmitter. First, three sections of SMF 28 are core-offset spliced together with the lengths of d1 for region 1 and d2 for region 2. d1 and d2 should be comparable in order to ensure a high contrast and uniform reflection spectrum. Parameter h is the distance between the outer boundary of one SMF and the center of another SMF, as shown in Fig. 1(e). In the top-view, three SMF cores should be aligned in the same axis. After that, a drop of UV-cured adhesive supported by a fiber taper with diameter of about 35 µm is carefully dropped on the top of region 1, as shown in the Fig. 1(c) and 1(f) that is a typical dripping process photograph. Due to the adsorption and surface tension of liquid, adhesive gradually moves to both sides of region 1, finally forming a curved structure with different thicknesses at different locations, as shown in Fig. 1(e) and 1(h) that is a typical sample photograph in the sideview. Then, UV light is used to cure the adhesive for about 20 minutes. Considering adhesive with refractive index of around 1.54 in the 1.55 µm band and mode confinement of circular structure in the optical fiber cross section as shown in Fig. 1(e), a curved adhesive waveguide is formed on the top of region 1. For multi-mode interference and then being reflected at region 2 with cladding modes simultaneously, h is set to less than 20 µm to ensure the curved waveguide has the minimum thickness of < 10-20 µm to generate high ultrasound frequency. After the device fabrication, an Erbium doped fiber Fig. 2. Optical field distributions when the adhesive thickness is 0 µm (a) and 12 µm (b). (c) The energy evolution in the basic mode as light passes through the adhesive waveguide. A defined optimized adhesive thickness (OAT) corresponds to basic mode with most light propagates in the adhesive waveguide. (d) The relationship between OAT and h. To investigate the optical field distribution in the adhesive waveguide between two fiber endfaces, a theoretical analysis is carried via finite element beam propagation method. Considering that the launch light, propagating in the region 1, is primarily absorbed by the silica cladding of region 1 and transmits into the region 2, two-dimensional analysis with the uniform adhesive thickness is used for the simplicity. The diameters and refractive indexes of single-mode fiber are set as 8 µm and 1.4521 for fiber core and 125 µm and 1.4469 for fiber cladding [18]. d1 = d2 = 120 µm and h is set to 6 µm as an example. In order to enhance the pumping efficiency for ultrasound generation, the basic mode in SMF should deliver power to adhesive waveguide with rare light diffusion and power loss. Fig. 2(a) demonstrates the optical field distribution (left) and the basic mode propagation (right) as launch light passes through fiber device without covering adhesive, showing that much light propagates into the fiber cladding of region 1. In Fig. 2(b) with adhesive thickness of 12 µm, the basic mode with most power propagates in the adhesive waveguide with little light diffusion. Fig. 2(c) shows the energy evolution in the basic mode as the adhesive thickness varies from 0 to 24 µm. For the cases of adhesive thickness less than 12 µm, periodic optical oscillation is created in the region 1 due to the interference between modes in the adhesive waveguide and air. As the adhesive thickness increases gradually to 12 µm, less light propagates into the air, resulting in the reduced interference. Furthermore, much light in the single-mode fiber would diffuse into air and silica cladding in the region 1 with thin adhesive, resulting in the pump intensity decrease in adhesive waveguide. As the adhesive thickness is larger than 12 µm, much power transfers into the high-order waveguide modes, corresponding to the basic mode power drop in the adhesive waveguide. Therefore, an optimized adhesive thickness (OAT) is defined, corresponding to the basic mode with most power propagating in the adhesive waveguide for more efficient ultrasound generation. For h = 6 µm, the OAT is 12 µm, which would be varied as h is changed gradually, as shown in Fig. 2(d). Furthermore, thicker waveguide would induce lower transverse ultrasound frequency. Many highorder modes interference in the adhesive waveguide with large thickness could enhance the ultrasound response with high frequency. Therefore, ultrasound generation and detection should consider an optimal waveguide thickness. Fig. 3. (a) The reflectivity of fiber device before and after covering adhesive with h = 11.8 µm. (b) Contrast comparison before and after covering adhesive with 8 samples. In experiment, the reflectivity of fiber device before and after covering adhesive are first characterized with h = 11.8 µm, as shown in Fig. 3(a). Before covering adhesive, the device contrast is 2.7 dB with the maximal reflectivity of -15.1 dB, while 21.7 dB and -27.8 dB after covering adhesive, corresponding to the increased contrast by 19 dB to enhance the dynamic range for ultrasound sensing. The reduced reflectivity, due to the optical absorption of adhesive, could be offset by increasing the input probe power. The curved structure has the varied thickness ranging from maximum of 66 µm to minimum of 11.3 µm. We tested 8 devices under the same fabrication condition, the spectrum contrast comparison as shown in Fig. 3(b), revealing the increased contrasts for most samples after covering adhesive. As the original contrast gradually increases, it’s harder to obtain higher contrast due to the irregularly curved structure and large optical absorption of adhesive. In addition, all samples’ contrasts are larger than 8 dB. In the following experiment of ultrasound generation and detection, the pump wavelength is set at the valley of reflection spectrum to achieve the resonant optical absorption by the adhesive waveguide, while the probe wavelength at the peak for the maximal reflection signal, as shown in Fig. 3(a). As the adhesive waveguide expands and shrinks because of pulse pumping, the shift of reflection spectrum could be detected by the probe light. Fig. 4 shows the experimental setup for the ultrasound generation and detection based on curved adhesive waveguide device. By using a polarization controller and an electro-optic modulator, a pulse laser is realized with a repetition rate of 100 kHz and duration time of 600 ns, and then amplified via an EDFA. The reason of this duration time which is larger than those values in many references is that optical absorption coefficient of UV-cured adhesive is lower than those of optical absorption materials such as graphite or carbon nanotube, resulting in the completely thermal expansion with long time in UV-cured adhesive [14,18]. 10% pump goes to oscilloscope to monitor the peak power. The remaining pump laser and probe laser are sent to the curved adhesive waveguide via a coupler and a circulator. A filter is used to exclude the pump light; only the probe light is detected by oscilloscope. The time delay between the pump pulse by PD 2 and PD 1 is 54 ns, which has been calibrated in advance in the following data. A variable optical attenuator is used to avoid the optical power saturation of PD 1. As pump light and probe light transmit to the curved adhesive waveguide device, pulsed energy is quickly absorbed by adhesive and then converted into the thermal energy due to high photoabsorption coefficient of adhesive, subsequently expanding via large thermal expansion and shrinking when the pulse disappears, followed by the acoustic wave generation. Due to the core-offset silica splicing structure, only the transverse expanding and shrinking direction is favoured for the adhesive waveguide, resulting in dominated transverse acoustic wave with certain direction. Therefore, several parameters of curved adhesive waveguide could be changed and then detected by probe light, such as the structure, optical path and effective refractive index, as shown in Fig. 5. Fig. 4. The experimental setup for ultrasound generation and detection. PC: polarization controller; EOM: electro-optic modulator; AFG: arbitrary function generator; EDFA: Erbium doped fiber amplifier. VOA: variable optical attenuator; PD: photodetector. Fig. 5(a) shows the time-domain traces of pump light with calibrated peak power of 321 mW at wavelength of 1560.83 nm and the probe light with input power of 2.5 mW at wavelength of 1555.85 nm. It clearly shows that at the time of around 150 ns after the disappearance of pump power, an ultra-short pulsed vibration is excited, corresponding to the transverse acoustic wave generated from the contraction of curved adhesive waveguide. Fig. 5(b) is the magnified plot of probe light time-domain traces with calibrated pulsed peak power of 113 mW and 321 mW, respectively. Higher pump power gives larger vibration amplitude of adhesive waveguide. Note trace with higher pump power has large delay time relative to that with lower pump power due to the aging of adhesive waveguide when the pump power is gradually increased to observe the variation of time-domain traces. Therefore, the broad ultrasound is created and detected based on curved adhesive waveguide. In summary, we have demonstrated an ultra-compact fiberbased curved adhesive waveguide device for ultrasound generation and detection. Owing to the curved structure with varied thickness and multi-mode interference effect, ultrasound with broad band, ranging from hundreds of Hz to 306 MHz, is realized and detected. This novel ultrasound transmitter offers new opportunities to the advanced biomedical and NDT applications. Funding. This research has been primarily supported by the Natural Sciences and Engineering Research Council (NSERC) of Canada (STPGP 506628, RGPIN-2015-06071), as well as the Canada Research Chairs (CRC) Program (950231352). Acknowledgment. We thank Dr. Liang Zhang for helpful discussion. REFERENCES Fig. 5. (a) The time-domain traces of pulsed pump light and probe light, corresponding to the ultrasound generation. (b) The magnified plot of probe light time-domain traces with different pulsed peak power. (c) Frequency spectrum via fast Fourier transform of Fig. 5(b). (d) The detailed diagram of curved adhesive waveguide device. Frequency spectrum, ranging from hundreds of Hz to 306 MHz, is obtained from the probe time-domain trace via fast Fourier transform, as shown in Fig. 5(c). The generated broad ultrasound bandwidth is attributed to the gradually varied thickness of curved adhesive waveguide, as shown in the detailed diagram of Fig. 5(d). In the region of part 1, adhesive thickness gradually changes from maximum of 66 µm to minimum of 11.3 µm. The transverse acoustic frequency is inversely proportional to adhesive thickness. The region of part 2 with minimum thickness of 11.3 µm and length of 25 µm corresponds to the highest transverse ultrasound frequency of around 306 MHz. Due to the curved adhesive waveguide with core-offset splicing structure, high-order waveguide modes interference is created at one passage time in the adhesive waveguide and reflection at the fiber segment of region 2, as shown in Fig. 5(d), subsequently enhancing the high frequency response due to short relaxation time. In addition, the mode number that could exist in the asymmetric waveguide is higher than those in the fiber taper or multi-mode fiber. In our previous reference of ultrasound sensing based on core-offset splicing fiber device, it is demonstrated that different resonant modes have different ultrasound frequency response [21]. 1. D. G. Aggelis, N. M. Barkoula, T. E. Matikas, and A. S. Paipetis, Compos. Sci. Technol. 72, 1127 (2012). 2. X. Zhao, R. L. Royer, S. E. Owens, and J. L. Rose, Smart Mater. Struct. 20, 105002 (2011). 3. R. J. Colchester, E. Z. Zhang, C. A. Mosse, P. C. Beard, I. Papakonstantinou, and A. E. Desjardins, Biomed. Opt. Express 6, 1502 (2015). 4. P. A. Fomitchov, A. K. Kromine, and S. Krishnaswamy, Appl. Opt. 41, 4451 (2002). 5. L. V. Wang, and S. Hu, Science 335, 1458 (2012). 6. C. Hu, Z. Yu, and A. Wang, Opt. Express 24, 20287 (2016). 7. S. J. Davies, C. Edwards, G. S. Taylor, and S. B. Palmer, J. Phys. D: Appl. Phys. 26, 329 (1993). 8. M. Oksanen, and J. Wu, Ultrason. 32, 43 (1994). 9. T. Sanderson, C. Ume, and J. Jarzynski, Ultrason. 33, 415 (1995). 10. B. Lee, Opt. Fiber Technol. 9, 57 (2003). 11. O. Volodarsky, Y. Hazan, and A. Rosenthal, Opt. Express 26, 22405 (2018). 12. X. Zou, N. Wu, Y. Tian, and X. Wang, Opt. Express 22, 18119 (2014). 13. E. Biagi, M. Brenci, S. Fontani, L. Masotti, and M. Pieraccini, Opt. Rev. 4, 481 (1997). 14. J. A. Guggenheim, J. Li, T. J. Allen, R. J. Colchester, S. Noimark, O. Ogunlade, I. P. Parkin, I. Papakonstantinou, A. E. Desjardins, E. Z. Zhang, and P. C. Beard, Nature Photon. 11, 714 (2017). 15. E. Biagi, F. Margheri, and D. Menichelli, IEEE Trans. Ultrason. Ferroelectr. Freq. Control 48, 1669 (2001). 16. R. K. Poduval, S. Noimark, R. J. Colchester, T. J. Macdonald, I. P. Parkin, A. E. Desjardins, and I. Papakonstantinou, Appl. Phys. Lett. 110, 223701 (2017). 17. V. Kochergin, K. Flanagan, Z. Shi, M. Pedrick, B. Baldwin, T. Plaisted, B. Yellampalle, E. Kochergin, and L. Vicari, Proc. SPIE 7292, 72923D (2009). 18. X. Dong, S. Gao, J. Tian, and Y. Yao, Photon. Res. 5, 287 (2017). 19. S.-H. Nam, J.-W. Kang, and J.-J. Kim, Appl. Phys. Lett. 87, 233504 (2005). 20. R. R. Kumar, E. Hahamovich, S. Tsesses, Y. Hazan, A. Grinberg, and A. Rosenthal, IEEE Photon. J. 11, 1 (2019). 21. H. Fan, L. Zhang, S. Gao, L. Chen, and X. Bao, Opt. Lett. 44, 3606 (2019). References 1. 2. 3. 4. 5. 6. 7. 8. 9. 10. 11. 12. 13. 14. 15. 16. 17. 18. 19. 20. 21. D. G. Aggelis, N. M. Barkoula, T. E. Matikas, and A. S. Paipetis, "Acoustic structural health monitoring of composite materials : Damage identification and evaluation in cross ply laminates using acoustic emission and ultrasonics," Compos. Sci. Technol. 72, 1127-1133 (2012). X. Zhao, R. L. Royer, S. E. Owens, and J. L. Rose, "Ultrasonic Lamb wave tomography in structural health monitoring," Smart Mater. Struct. 20, 105002 (2011). R. J. Colchester, E. Z. Zhang, C. A. Mosse, P. C. Beard, I. Papakonstantinou, and A. E. Desjardins, "Broadband miniature optical ultrasound probe for high resolution vascular tissue imaging," Biomed. Opt. Express 6, 1502-1511 (2015). P. A. Fomitchov, A. K. Kromine, and S. Krishnaswamy, "Photoacoustic probes for nondestructive testing and biomedical applications," Appl. Opt. 41, 4451-4459 (2002). L. V. Wang, and S. Hu, "Photoacoustic Tomography: In Vivo Imaging from Organelles to Organs," Science 335, 1458 (2012). C. Hu, Z. Yu, and A. Wang, "An all fiber-optic multi-parameter structure health monitoring system," Opt. Express 24, 20287-20296 (2016). S. J. Davies, C. Edwards, G. S. Taylor, and S. B. Palmer, "Laser-generated ultrasound: its properties, mechanisms and multifarious applications," J. Phys. D: Appl. Phys. 26, 329-348 (1993). M. Oksanen, and J. Wu, "Prediction of the temporal shape of an ultrasonic pulse in a photoacoustic sensing application," Ultrason. 32, 43-46 (1994). T. Sanderson, C. Ume, and J. Jarzynski, "Hyperbolic heat equations in laser generated ultrasound models," Ultrason. 33, 415-421 (1995). B. Lee, "Review of the present status of optical fiber sensors," Opt. Fiber Technol. 9, 57-79 (2003). O. Volodarsky, Y. Hazan, and A. Rosenthal, "Ultrasound detection via low-noise pulse interferometry using a free-space Fabry-Pérot," Opt. Express 26, 22405-22418 (2018). X. Zou, N. Wu, Y. Tian, and X. Wang, "Broadband miniature fiber optic ultrasound generator," Opt. Express 22, 18119-18127 (2014). E. Biagi, M. Brenci, S. Fontani, L. Masotti, and M. Pieraccini, "Photoacoustic Generation: Optical Fiber Ultrasonic Sources for Non-Destructive Evaluation and Clinical Diagnosis," Opt. Rev. 4, 481-483 (1997). W J. A. Guggenheim, J. Li, T. J. Allen, R. J. Colchester, S. Noimark, O. Ogunlade, I. P. Parkin, I. Papakonstantinou, A. E. Desjardins, E. Z. Zhang, and P. C. Beard, "Ultrasensitive plano-concave optical microresonators for ultrasound sensing," Nature Photon. 11, 714-719 (2017). E. Biagi, F. Margheri, and D. Menichelli, "Efficient laser-ultrasound generation by using heavily absorbing films as targets," IEEE Trans. Ultrason. Ferroelectr. Freq. Control 48, 1669-1680 (2001). R. K. Poduval, S. Noimark, R. J. Colchester, T. J. Macdonald, I. P. Parkin, A. E. Desjardins, and I. Papakonstantinou, "Optical fiber ultrasound transmitter with electrospun carbon nanotube-polymer composite," Appl. Phys. Lett. 110, 223701 (2017). V. Kochergin, K. Flanagan, Z. Shi, M. Pedrick, B. Baldwin, T. Plaisted, B. Yellampelle, E. Kochergin, and L. Vicari, "All-fiber optic ultrasonic structural health monitoring system," Proc. SPIE 7292, 72923D (2009). X. Dong, S. Gao, J. Tian, and Y. Yao, "Multipoint fiber-optic laser-ultrasound generation along a fiber based on the core-offset splicing of fibers," Photon. Res. 5, 287-292 (2017). S.-H. Nam, J.-W. Kang, and J.-J. Kim, "Temperature-insensitive flexible polymer wavelength filter fabricated on polymer substrates," Appl. Phys. Lett. 87, 233504 (2005). R. R. Kumar, E. Hahamovich, S. Tsesses, Y. Hazan, A. Grinberg, and A. Rosenthal, "Enhanced Sensitivity of Silicon-Photonics-Based Ultrasound Detection via BCB Coating," IEEE Photon. J. 11, 1-11 (2019). H. Fan, L. Zhang, S. Gao, L. Chen, and X. Bao, "Ultrasound sensing based on in-fiber dual-cavity Fabry-Perot interferometer," Opt. Lett. 44, 36063609 (2019).