APPLIED PHYSICS LETTERS 90, 011502 共2007兲 Thomson scattering diagnostics of the plasma generated in a hollow anode with a ferroelectric plasma source D. Yarmolich, V. Vekselman, J. Z. Gleizer, Y. Hadas, J. Felsteiner, and Ya. E. Krasika兲 Physics Department, Technion, 32000 Haifa, Israel 共Received 31 October 2006; accepted 27 November 2006; published online 2 January 2007兲 Thomson scattering of a laser beam was applied to study the plasma parameters inside a hollow anode having a ferroelectric plasma source incorporated in it. This method allowed avoiding difficulties related to spectroscopical measurements in the case of unknown electron energy distribution. It was found that the electron density and energy of the ferroelectric plasma are ⬃1015 cm−3 and 艋5 eV, respectively, and the density of the hollow anode bulk plasma is ⬃6 ⫻ 1013 cm−3. Applying an accelerating pulse for electron extraction from the bulk plasma leads to an increase in the electron density and energy of the ferroelectric plasma up to 6 ⫻ 1016 cm−3 and 艋20 eV, respectively. © 2007 American Institute of Physics. 关DOI: 10.1063/1.2426886兴 Ferroelectric plasma source1 共FPS兲 has been used for different applications, namely, as an electron source for generation of high-current electron beams,2,3 triggering of gaseous switches,4 microwave generation,5 ion acceleration,6 microthruster7 propulsion, and for heavy ion beam charge neutralization.8 Also, recent experiments9–11 have shown that using FPS one can ignite and sustain a hollow-anode 共HA兲 discharge with current amplitude of 艋1.5 kA and pulse duration of ⬃20 s at pressure of 艋5 ⫻ 10−5 Torr. This FPSassisted HA plasma source served as a cathode in a diode generating electron beam with amplitude of ⬃1 kA and electron energy of ⬃200 keV. A common important feature for all these applications is the FPS surface plasma which is generated at the ferroelectric surface under the application of a driving pulse. However, the parameters of this plasma require additional research. Indeed, the analysis of spectroscopic data10 concerning plasma parameters required a preassumption of the electron energy distribution 共EED兲 which is difficult to measure in non-Maxwellian plasma.11 The use of Thomson scattering allows one to avoid the above drawback of the spectroscopic measurements and to determine the plasma EED and density by analyzing the scattered light spectrum and intensity.12,13 A pulsed neodymium-doped yttrium aluminium garnet laser permits application of this method for a plasma with density down to ne ⬇ 5 ⫻ 1013 cm−3. Here let us note that in the case of ne 艋 1017 cm−3 the light scattering due to collective plasma effects is negligibly small.13 Thus one can describe light scattering in such plasma as Thomson light scattering by free electrons. Here the electrons may have an arbitrary EED which results in spectral broadening of the scattered photons due to the Compton or inverse Compton effects. For a single scattering the dependence of the photon frequency shift ⌬ on the electron momentum p is14 ⌬ = − c关p · 共n̂ − n̂⬘兲兴 + ប2共1 − n̂ · n̂⬘兲 mc2关1 + 共ប/mc2兲共1 + n̂ · n̂⬘兲 − p · n̂/mc兴 , ity, and ប is the incident photon energy. Thus, analysis of the spectrally resolved scattered light allows one to obtain the EED. In the case of an absolute scattered light intensity calibration, one obtains also the plasma electron density. The experimental setup used in the present research was similar to the one described in Ref. 11. Namely, a HA with incorporated seven identical FPSs was used. The application of a driving pulse 共⬃2 kV, ⬃200 ns兲 caused plasma formation at each FPS front surface. Electron and ion flows emitted from the plasma initiated the HA bulk plasma discharge by means of an additional pulse generator 共艋7 kV, 20 s兲. During the HA discharge, the FPS plasma was selfconsistently formed at the front surfaces of the FPSs. An accelerating pulse 共⬃200 kV, ⬃300 ns兲 applied with a time delay d ⬵ 15 s with respect to the beginning of the FPS driving pulse caused extraction of electrons from the HA plasma through the HA output grid. To make available an optical access to the plasma, longitudinal slots were prepared in the HA electrode. The laser beam 共SureLite laser, = 5320 Å, 0.2 J, and 8 ns兲 was collimated and focused at a distance of either d ⬵ 3 mm or d ⬵ 5 mm from the central FPS front surface 共see Fig. 1兲. After passing the HA, the laser beam was absorbed by a graphite damper placed at the bottom of the vacuum chamber. Also, black velvet sheets placed at the HA wall were used as “viewing dampers”15 in order to decrease the parasitic laser beam scattering inside the HA and vacuum chambers. The laser beam focus 共⬃1 mm in diameter兲 was im- 共1兲 where m is the electron mass, n̂ and n̂⬘ are the incident and scattered photon directions, respectively, c is the light veloca兲 Electronic mail: fnkrasik@physis.technion.ac.il FIG. 1. Experimental setup 共only the central FPS is shown兲. 0003-6951/2007/90共1兲/011502/3/$23.00 90, 011502-1 © 2007 American Institute of Physics Downloaded 23 Feb 2008 to 132.68.75.124. Redistribution subject to AIP license or copyright; see http://apl.aip.org/apl/copyright.jsp 011502-2 Yarmolich et al. FIG. 2. Framing spectral images of the scattered laser beam: 共a兲 driving pulse only, 共b兲 the HA discharge prior to applying the accelerating pulse, and 共c兲 during the accelerating pulse. aged at a 250 mm imaging Chromex spectrometer 共600 groove/ mm grating兲 input slit using an achromatic lens. The spectrometer resolution was 1.3 Å / pixel. The spectrometer optical axis was perpendicular to the laser beam propagation direction and to the FPS surface normal. The laser beam polarization was perpendicular to the FPS surface 共see Fig. 1兲. Hence, the scattered light had the same polarization as the laser beam. At the same time, the parasitic light was randomly polarized. Thus, a polarizer which transmits only perpendicular polarized light was placed in the front of the spectrometer slit in order to increase the signal to noise ratio. The image of the spectral line profile at the output of the spectrometer was recorded using a 4Quik05A camera with frame duration of 20 ns. Already the first experiments without HA discharge when only the FPSs were ignited showed that at d = 15 s and d = 3 mm there was laser beam scattering by microparticles, whose generation accompanied the ferroelectric surface discharge.16 In Ref. 16 it was shown that the mean microparticle size and velocity are ⬃5 m and ⬃6 ⫻ 103 cm/ s, respectively. For this case, which further will be referred as case 共a兲, an example of the spectral image of the laser beam scattering is shown in Fig. 2共a兲. In order to obtain the image of the laser beam, a spectrometer entrance slit width of 0.3 mm was used. Typical spectral framing images of the scattered light obtained during the HA discharge prior to and during the accelerating pulse are shown in Fig. 2共b兲 关case 共b兲兴 and in Fig. 2共c兲 关case 共c兲兴, respectively. Also, with the same experimental setup, the mean backgrounds 共the 4Quik05A camera self-background and the Appl. Phys. Lett. 90, 011502 共2007兲 background of the plasma light emission without the laser during and without the accelerating pulse and the laser background, i.e., without the FPS and HA discharge兲 with statistical averaging over ten shots were obtained. All the spatially resolved spectral images were transformed to spectral curves by vertical summing of the camera pixel intensities. These spectral curves are shown in Fig. 3 after the subtraction of the corresponding backgrounds. In case 共a兲 the spectral line is not broadened or shifted because at d = 15 s and d = 3 mm, ne 艋 1010 cm−3.2 Thus the obtained spectrum is related to the laser light scattering by the microparticles.16 In cases 共b兲 and 共c兲, the spectra of the scattered light showed significantly different features: the peak intensity is increased and wings appear in the spectra. These wings are related to the Compton shifted photons which were scattered by the plasma electrons. The absolute calibration of the Thomson experimental setup was carried out using the laser beam Rayleigh scattering by nitrogen gas whose pressure was changed in the range of 0.1– 5.5 Torr. The increase in the Rayleigh scattered light intensity SR with the increase in the nitrogen pressure by 1 Torr was used to determine the electron density ne. The ratio of the measured light intensity obtained in the Thomson scattering ST and the Rayleigh scattering SR at the N2 gas density of 3.5⫻ 1016 cm−3 is13 ST n e T = = 3.7 ⫻ 10−13ne , SR 3.5 ⫻ 1016R 共2兲 where T = 6.65⫻ 10−25cm2 共Ref. 13兲 and R = 5.1 ⫻ 10−27 cm2 for = 5320 Å 共Ref. 17兲 are the Thomson and Rayleigh cross sections, respectively. Let us note that the increase in the intensity in case 共b兲 as compared with case 共a兲 could be due to the increase in the amount of microparticles. In order to avoid this uncertainty and to obtain the EED, the averaged case 共b兲 spectrum was normalized to the averaged case 共a兲 spectrum. Namely, the intensities of case 共a兲 spectrum were multiplied by the ratio of the areas of case 共b兲 and case 共a兲 spectra. Thus, the difference between the wings of case 共b兲 spectrum and the normalized case 共a兲 spectrum is due to the Compton shifted photons. This Compton spectrum was transformed to the EED using Eq. 共1兲 and the Rayleigh calibration 关see Fig. 4共a兲兴. Here it was assumed that the electrons possessing velocities parallel to the laser beam or to the observation directions give a major contribution to the Compton wavelength shift. One can see that during the HA discharge, ne ⬃ 2 ⫻ 1015 cm−3 and a major part of the plasma electrons has energy 艋5 eV. The same analysis of the EED during the accelerating pulse for case 共c兲 is shown in Fig. 4共b兲. In this case ne increases up to ⬃5 ⫻ 1016 cm−3 and the major part of plasma electrons increases its energy up to 20 eV. It is reasonable to assume that during the first 150 ns of the accelerating pulse, the amount of microparticles remains FIG. 3. Spectrum of the scattered laser beam: 共a兲 driving pulse only, 共b兲 HA discharge prior to applying the accelerating pulse, and 共c兲 during the accelerating pulse. Downloaded 23 Feb 2008 to 132.68.75.124. Redistribution subject to AIP license or copyright; see http://apl.aip.org/apl/copyright.jsp 011502-3 Appl. Phys. Lett. 90, 011502 共2007兲 Yarmolich et al. FIG. 4. HA plasma electron energy distribution: 共a兲 prior to applying the accelerating pulse and 共b兲 during the accelerating pulse. the same for cases 共b兲 and 共c兲. Thus the increase in the spectrum area for case 共c兲 could be explained by the increase in ne by ⬃8 ⫻ 1016 cm−3 which agrees satisfactorily with the previous analysis. The same Thomson scattering experiments were carried out at d = 15 mm where the plasma density is significantly lower.10 To increase the system sensitivity, the width of the spectrometer slit was increased up to 2 mm and the 4Quik05A camera magnification was set to maximum. Also, a 150 groove/ mm spectrometer grating was installed. The changes in the spectrometer setup resulted in spectral resolution of 5.2 Å / pixel and instrumental linewidth of 90 Å full width at half maximum that did not allow us to observe the Compton broadening of the scattered light spectrum. The image was obtained as a result of summing up of 20 shots in order to increase the resulting intensity. It was found that microparticles already appear also at this distance when d 艌 5 s. With the increase in d the amount of microparticles increases significantly. Thus one can conclude that a small amount of microparticles acquires velocities up to 3 ⫻ 105 cm/ s. Analyzing only the horizontal lines of the images without the microparticle spots, it was found that the intensity of the scattered light in cases 共b兲 and 共c兲 exceeded the intensity in case 共a兲. The latter allows one to estimate the HA bulk plasma density as ⬃6 ⫻ 1013 cm−3. During the ac- celeration pulse, the statistical error in the density measurements did not permit us to confirm the density changes. To summarize, it was shown that the application of Thomson scattering diagnostics with pulsed laser, imaging spectrometer, and intensified framing camera allows one to improve significantly the time and space resolutions, to avoid difficulties related to spectroscopic data analysis in the case of non-Maxwellian EED 共Ref. 11兲 and to obtain in a single shot ne 艌 4 ⫻ 013 cm−3 and EED for ne 艌 1014 cm−3. It was found that the ferroelectric surface plasma during the HA operation is characterized by ne ⬃ 1015 cm−3 and electron energy 艋5 eV prior to applying the accelerating pulse. During the accelerating pulse, the FPS surface plasma density increases up to ⬃共3 – 6兲 ⫻ 1016 10−3 and the electron energy increases up to ⬃20 eV. The obtained increase in ne and in the electron energy of the FPS plasma could be related to the increase in the HA plasma potential10 during the accelerating pulse. The latter leads to an increase in the energy of the HA bulk plasma ions whose bombardment causes formation of the surface plasma. 1 G. Rosenman, D. Shur, Ya. E. Krasik, and A. Dunaevsky, J. Appl. Phys. 88, 6109 共2000兲. 2 J. Ivers, D. Flechter, C. Golkowski, G. Liu, J. Nation, and L. Schachter, IEEE Trans. Plasma Sci. 27, 707 共1999兲. 3 A. Dunaevsky, Ya. E. Krasik, J. Felsteiner, and A. Sternlieb, J. Appl. Phys. 90, 3689 共2001兲. 4 H. Gundel, H. Riege, J. Handerek, and K. Zioutas, Appl. Phys. Lett. 54, 2071 共1989兲. 5 M. Einat, E. Jerby, and G. Rosenman, Appl. Phys. Lett. 79, 4097 共2001兲. 6 S. D. Kovaleski, IEEE Trans. Plasma Sci. 33, 876 共2005兲. 7 M. A. Kemp and S. D. 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