REFERENCES AND NOTES CHAPTER 1 1. 2. 3. 4. 5. 6. 7. Sheth JP, Xu J, Wilkes GL (2002) Polymer 44, p743. Sheth JP, Wilkes GL, Semi-Crystalline Segmented Poly(ether-block-amide) Copolymers: An Overview of their Solid-state Structure Property Relationships and Uniaxial Deformation Behavior, Ed. Fakirov S, to be published in the Handbook of Condensation Thermoplastic Elastomers, Wiley-VCH Publications. Sheth JP, Aneja A, Wilkes GL, Yilgor E, Atilla GE, Yilgor E, Beyer FL (2004) Polymer 45, p6919. Sheth JP, Aneja A, Wilkes GL (2004) Polymer 45, p5979. Sheth JP, Fornof A, Yilgor I, Long TE, Wilkes GL, Probing the hard segment phase connectivity and percolation in model segmented polyurethaneurea copolymers (submitted). Unal S, Yilgor I, Yilgor E, Sheth JP, Wilkes GL, Long TE, A new generation of highly branched polymers: hyperbranched, segmented poly(urethaneurea) elastomers, Macromolecules 37, p7081. Sheth JP, Klinedinst DB, Yilgor E, Yilgor I, Wilkes GL, Segmented copolymers with hard segments based on only a single diisocyanate molecule (submitted). CHAPTER 2 1. 2. 3. 4. 5. 6. 7. 8. 9. 10. 11. 12. 13. 14. 15. Schollenberger CS (1955) U S Patent 2,871,218 Schollenberger CS, Scott H, Moore GR (1962) Rubber Chem Tech 35, p742. Cooper SL, Tobolsky AV (1966) Textile Res J 36(9), p800. Helfand E, ZR Wasserman in Developments in Block Copolymers – I (1982) Ed. Goodman I, Applied Science Publishers, New York, NY, p99. Park C, Yoon J, Thomas EL (2003) Polymer 44, p6725. Hamley IW (1998) The Physics of Block Copolymers, Oxford Science Publications, New York. Meier DJ (1996) J Poly Sci: Part B Poly Phy 34, p1817. Leibler L (1980) Macromolecules 13, p1602. Benoit H, Hadziioannou G (1988) Macromolecules 21, p1449. Zielinski JM, Spontak RJ (1992) Macromolecules 25, p653. Olmsted PD, Milner ST (1994) Macromolecules 27, p1964. Matsen MW, Schick M (1994) Macromolecules 27, p7157. Semenov AN, Likhtman AE (1998) Macromolecules 31, p9058. Olmsted PD, Milner ST (1998) Macromolecules 31, p4011. Bates FS, Frederickson GH (1990) Ann Rev Phy Chem 41, p525. 165 16. 17. 18. 19. 20. 21. 22. 23. 24. 25. 26. 27. 28. 29. 30. 31. 32. 33. 34. 35. 36. 37. 38. 39. 40. 41. 42. 43. 44. 45. 46. 47. Richards RW (1985) Adv Poly Sci 71, p1. Sakurai S (1996) Current Trends Poly Sci 1, p119. Kawai H, Hashimoto T (1979) Contemporary Topics Poly Sci 3, p245. Richards RW (1985) Adv Poly Sci 71, p1. Vonk CG, Balta-Calleja FJ (1989) X-ray Scattering of Synthetic Polymers, Poly Sci Library v8, Elsevier Science Publishers, Amsterdam, The Netherlands. Cebe P, Hsiao BS, Lohse DJ (Eds.) (2000) ACS Symposium Series, American Chemical Society v739. Goh MC (1995) Adv Chem Phy 91, p1. Khandpur AK, Forster S, Bates FS, Hawley IW, Ryan AJ, Bras W, Almdal K, Mortensen K (1995) Macromolecules 28, p8796. Lodge TP, Muthukumar M (1996) J Chem Phy 100, p13275. Flory PJ (1952) Principles of Polymer Chemistry, Cornell University Press, Ithaca, NY. Camberlin Y, Pascault JP (1984) J Poly Sci: Poly Phy Ed 22, p1835. Pascault JP, Camberlin Y (1986) Poly Comm 27, p230. Legge NR, Holden G, Schroeder HE (Eds.) (1987) Thermoplastic Elastomers: A Comprehensive Review, Hanser Publishers, New York, 1st ed. Meckel W, Goyert W, Wieder W in Thermoplastic Elastomers: A Comprehensive Review (1987) Eds. Legge NR, Holden G, Schroeder HE, Hanser Publishers, New York, NY, 1st ed., p13. Hepburn C (1992) Polyurethane Elastomers, Elsevier Applied Science Publishers, New York, NY, 2nd ed. Abouzahr S Wilkes GL in Processing, Structure and Properties of Block Copolymers (1985) Ed. Folkes MJ, Elsevier Applied Science Publishers, New York, 2nd ed., p165. Schollenberger CS in Handbook of Elastomers (2001) Eds. Bhowmick AK, Stephens HL, Marcel Dekker Inc., New York, NY, p387. Peebles Jr LH (1974) Macromolecules 7, p872. Peebles Jr LH (1976) Macromolecules 9, p58. Abouzahr S, Wilkes GL (1984) J Appl Polym Sci 29, p2695. Van Krevelen DW (1972) Properties of Polymers, Elsevier Publishers, New York. Noshay A, McGrath JE (1977) Block Copolymers: Overview and Critical Survey, Academic Press, New York, NY. Allport DC, Jones WH (Eds.) (1973) Block Copolymers, Applied Science Publishers, London, UK. Schneider NS, Sung CSP (1977) Polym Engg Sci 17, p73. Lilaonitkul A, Cooper SL (1979) Advances in Urethane Science and Technology 7, p163. Takahara A, Tashita J, Kajiyama T, Takyanagi, MacKnight WJ (1985) Polymer 26, p987. Schollenberger CS, Dinbergs K (1979) Adv Urethane Sci Tech 7, p1. Wilkes GL, Bagrodia S, Humphries W, Wildnauer R (1975) J Poly Sci: Poly Lett Ed 13, p321. Wilkes GL, Wildnauer R (1975) J Appl Phy 46, p4148. Wilkes GL, Emerson JA (1975) J Appl Phy 47, p4261. Lagasse RR (1977) J Appl Poly Sci 21, p2489. Hesketh TR, Van Bogart JWC, Cooper SL (1980) Poly Engg Sci 20, p190. 166 48. 49. 50. 51. 52. 53. 54. 55. 56. 57. 58. 59. 60. 61. 62. 63. 64. 65. 66. 67. 68. 69. 70. 71. 72. 73. 74. 75. Yokoyama T (1978) Adv Urethane Sci Tech 6, p1. Sung CSP, Schneider PC (1975) Macromolecules 8, p68. Schroeder LR, Cooper SL (1976) J Appl Phy 47, p4310. Coleman MC, Schrovanek DJ, Howe SE, Painter PC (1985) Macromolecules 18, p299. MacKnight WJ, Yang M (1973) J Poly Sci: Poly Symp 42, p817. Senich GA, MacKnight WJ (1980) Macromolecules 13, p106. Stadler R, Freitas LDL (1986) Poly Bull 15, p173. McKiernan RL, Heintz AM, Hsu SL, Atkins EDT, Penelle J, Gido SP (2002) Macromolecules 35, p6970. Rosen SL (1993) Fundamental Principles of Polymeric Materials, Wiley-Interscience, New York, NY, 2nd ed. Yilgor E, Yilgor I (2001) Polymer 42, p7953. Ryan AJ, Stanford JL, Still RH (1988) Polym Comm 29, p196. Grulke EA in Polymer Handbook (1999) Eds. Bandrup J, Immergut EH, Grulke ED, Willey-Interscience, New York 4th ed., pVII-701. Yilgor E, Burgaz E, Yurtsever E, Yilgor I (2000) Polymer 41, p849. Sung CSP, Schneider NS (1978) J Mat Sci 13, p1689. Harrell Jr LL (1969) Macromolecules 2, p607. Samuels SL, Wilkes GL (1973) J Poly Sci: Symp 43, p149. Ibid. (1971) J Poly Sci: Poly Lett 9, p761. Aneja A, Wilkes GL (2003) Polymer 44, p2221. Wilkes GL, Wildnauer R (1975) J Appl Phy 46, p4182. Herrington R, Hock K (Eds.) (1990) Flexible Polyurethane Foams, The Dow Chemical Company, 2nd ed. Woods G (1982) Flexible Polyurethane Foams: Chemistry and Technology, Applied Science Publishers, Essex, England. Wilkes GL, Abouzahr S, Radovich D (1983) J Cellular Plast 19, p248. Armistead JP, Wilkes GL (1988) J Appl Poly Sci 35, p601. Rossmy GR, Lollmeier HJ, Lidy W, Schator H, Wiemann M (1977) J Cellular Plast 13, p26. Ibid. (1981) J Cellular Plast 13, p319. Bailey Jr FE, Critchfield FE (1981) J Cellular Plast 17, p333. Elwell MJ, Ryan AJ, Grünbauer HJM, Van Lieshout HC (1996) Polymer 37, p1353. Ibid. (1996) Macromolecules 29, p2960. CHAPTER 3 1. 2. 3. 4. 5. 6. Legge NR, Holden G, Schroeder HE (Eds.) (1987) Thermoplastic elastomers: A comprehensive review, Hanser Publishers, New York, 1st ed., Chapters 8 and 9. Cella RJ (1973) J Poly Sci, Poly Symp 42, p727. Seymour RW, Overton JR, Corley LS (1975) Macromolecules 8, p331. Wegner G, Fuji T, Meyer W, Lieser G (1978) Angew Makromol Chem 74, p293. Zhu LL, Wegner G (1981) Makromol Chem 182, p3625. Deleens G, Foy P, Marechal E (1977) Eur Poly J 13, p337. 167 7. 8. 9. 10. 11. 12. 13. 14. 15. 16. 17. 18. 19. 20. 21. 22. 23. 24. 25. 26. 27. 28. 29. 30. 31. 32. 33. 34. 35. 36. 37. 38. 39. 40. 41. 42. 43. 44. 45. Deleens G (1981) ANTEC, p419. Yu YC, Jo WH (1994) J Appl Poly Sci 54, p585. Yu YC, Jo WH (1995) J Appl Poly Sci 56, p895. Yu YC, Jo WH, Lee MS (1997) J Appl Poly Sci 64, p2155. Bouma K, Wester GA, Gaymans RJ (2001) J Appl Poly Sci 80, p1173. Boulares A, Tessier M, Maréchal E (2000) Polymer 41, p3561. Deleens G, Foy P (1975) French Patent 2,382,060. Deleens G, Guerin B, Poulain C (1976) French Patent 2,359,879. Deleens G, Guerin B, Poulain C (1976) French Patent 2,378,058. Deleens G, Ferlampin J, Gonnet M (1977) French Patent 2,401,947. Faruque HS, Lacabanne C (1986) Polymer 27, p527. Xie M, Chamberlin Y (1986) Makromol Chem 187, p383. Alberola N (1988) J Appl Poly Sci 36, p787. Bornschegl E, Goldbach G, Meyer K (1985) Prog Colloid Poly Sci 71, p. 119. Hatfield GR, Guo Y, Killinger WE, Andrejak A, Roubicek PM (1993) Macromolecules 26, p6350. Warner S (1990) J Elast Plast 22, p166. Niesten MCE, Gaymans RJ (2001) J Appl Poly Sci 81, p1372. Niesten MCEJ, Gaymans RJ (2001) Polymer 42, p6199. McLean RS, Sauer BB (1999) J Polym Sci 37, p859. Sauer BB, McLean RS, Brill DJ, Londono DJ (2001) Poly Mat Sci Eng 85, p268. Sauer BB, McLean RS, Brill DJ, Londono DJ (2002) J Poly Sci B: Poly Phys 40, p1727. Ward IM (Ed.) (1977) Structure and properties of oriented polymers, Chapman & Hall, New York, p 44. The 1H NMR experiments were conducted by J. Lizotte of Prof. T. E. Long’s group in the department of chemistry at Virginia Polytechnic Institute & State University. Private Communication from Atofina via Sauer BB. Boublil H, Okroafor E, Belhoucine M, Rault J (1989) Poly Eng Sci 29, p679. McCrum NG, Read BE, Williams G (1967) Anelastic and dielectric effects in polymeric solids, Dover Publications Inc, New York, 1st ed., p561. Wunderlich B (1980) Macromolecular physics, Academic Press, New York, v3, p52. Cojazzi G, Ficher A, Garbuglio C, Malta V, Zannetti R (1973) Makromol Chem 168, p. 289. Norholt MG, Tabor BJ, van Aartsen JJ (1972) J Poly Sci Poly Phy Ed 10, p191. Andrews EH (1964) Proc R Soc Lon A277, p562. Oth JFM, Flory PJ (1958) J Am Chem Soc 80, p1297. Desgrand JV (1832) UK Patent 6334. Mertens A (1841) UK Patent 9186. Baare F, Garelly JG (1859) US Patent 24,691. Sheperd TL (1935) US Patent 423,997. Lilaonitkul A, West JC, Cooper SL (1976) J Macromol Sci Phys B12, p589. Samuels SL, Wilkes GL (1971) Poly Lett 9, p761. Mody PC, Wilkes GL (1981) J Appl Poly Sci 26, p2853. Alexander LE (1969) X-ray diffraction methods in polymer science, Wiley/Interscience, New York. 168 46. Tyagi D, McGrath JE, Wilkes GL (1986) Poly Eng Sci 26, p1371. CHAPTER 4 1. 2. 3. 4. 5. 6. 7. 8. 9. 10. 11. 12. 13. 14. 15. 16. 17. 18. 19. 20. 21. 22. 23. 24. 25. 26. 27. 28. 29. 30. 31. 32. Yilgor I, McGrath JE (1988) Adv Poly Sci 89, p1. Noshay A, McGrath JE (1977) Block copolymers: Overview and critical survey, Academic Press, New York. Mark JE (2000) ACS Symposium Series, American Chemical Society 729, p1. Summers JD, Elsbernd CS, Sormani PM, Brandt PJA, Arnold CA, Yilgor I, Riffle JS, Kilic S, McGrath JE (1988) ACS Symposium Series, American Chemical Society 360, p181. Yilgor I, McGrath JE (1984) Poly Bull 12, p 499. Mark JE (1979) Acc Chem Res 12, p49. Dvornic PR, Jovanovic JD, Govedarica MN (1993) J Appl Poly Sci 49, p1497. Vaughn Jr HA (1969) J Poly Sci B: Poly Phy 7, p569. Van Aert HAM, Neliessen L, Lemstra PJ, Brunelle DJ (2000) Polymer 42, p1781. Noshay A, Matzner M, Merriam CNJ (1971) J Poly Sci 9, p3147. Tyagi D, Hedrick JL, Webster DC, McGrath JE, Wilkes GL (1988) Polymer 29, p833. Saam JC, Fearon FWG (1971) Ind Eng Chem: Prod Res Dev 10, p10. David G, Robin JJ, Lacroix-Desmazes P (2002) Poly Preprints 43, p1095. Morton M, Kesten Y, Fetters L J (1974) Poly Preprints 15, p175. Smith SD, McGrath JE (1986) Poly Preprints 27, p31. Risch BG, Rodrigues DE, Lyon K, McGrath JE, Wilkes GL (1996) Polymer 37, p1229. Yilgor I, Lee B, Steckle Jr. WP, Riffle JS, Tyagi D, Wilkes GL, McGrath JE (1983) Poly Preprints 24, p35. Otsuki T, Kakimoto M, Imai Y (1991) J Poly Sci A: Poly Chem 29, p611. Yilgor I, Yilgor E, Johnson BC, Eberle J, Wilkes GL, McGrath JE (1983) Poly Preprints 24, p78. McGrath JE, Dunson DL, Mecham SJ, Hedrick JL (1999) Adv Poly Sci 140, p61. Ward Jr RS, Nyilas E in Organometallic Polymers (1978) (Eds.) Carraher Jr CE, Sheats JE, Pittman Jr CU, Academic Press, New York, p219. Leir CM, Hoffman JJ, Tushaus LA, Wiederholt GT, Mazurek MH, Sherman AA (1995) US Patent 5,512,650. Seth J, Bany SW, Kinning DJ (1999) US Patent 5,866,222. Yilgor I, Wilkes GL, McGrath JE (1982) Poly Preprints 23, p286. Tyagi D, Yilgor I, Wilkes GL, McGrath JE (1983) Poly Preprints 24, p39. Yilgor E, Yilgor I (1998) Poly Preprints 39, p465. Yilgor E, Unal S, Makal U, Yilgor I (2001) Poly Preprints 42, p120. Chun YC, Kim KS, Shin JS, Kim KH (1992) Poly Intnl 27, p177. Yilgor I, Yilgor E, Eberle J, Steckle Jr WP, Johnson B C, Tyagi D, Wilkes G L, McGrath JE (1983) Poly Preprints 24, p170. Tyagi D, Yilgor I, Wilkes GL, McGrath JE (1983) Poly Preprints 24, p39. Ibid (1984) Polymer 25, p1807. Ho T, Wynne KJ, Nissan RA (1993) Macromolecules 26, p7029. 169 33. Shibayama M, Suetsugu M, Sakurai S, Yamamota T, Nomura S (1991) Macromolecules 24, p6254. 34. Cho G, Natansohn A, Ho T, Wynne KJ (1996) Macromolecules 29, p2563. 35. Kajiyama M, Kakimoto M, Imai Y (1990) Macromolecules 23, p1244. 36. Stanciu A, Airinei A, Timpu D, Ioanid A, Ioan C, Bulacovschi V (1999) Eur Poly J 35, p1959. 37. The SAXS experiments were conducted by the author on the instrument in the laboratory of Dr. Frederick L. Beyer at the Army Research Laboratories in Aberdeen, Marlyland. 38. Glinka CJ, Barker JG, Hammouda B, Krueger S, Moyer JJ, Orts WJ (1998) J Appl Cryst 31, p430. 39. Russell TP, Lin JS; Spooner S, Wignall GD (1988) J Appl Cryst 21, p629. 40. Clarson SJ, Dodgson K, Semlyen JA (1985) Polymer 26, p930. 41. Yilgor E, Yilgor I (2001) Polymer 42, p7953. 42. Wilkes GL, Wildnauer R (1975) J Appl Phy 46, p4148. 43. Treloar LRG (1975) The Physics of Rubbry Elasticity, Clarendon Press, New York, 3rd ed. 44. Yilgor I, Riffle JS, Wilkes GL, McGrath JE (1982) Poly Bulletin 8, p535. 45. Yeh F, Hsiao BS, Sauer BB, Michel S, Siesler HW (2003) Macromolecules 36, p1940. 46. Tyagi D, McGrath JE, Wilkes GL (1986) Poly Eng Sci 26, p1371. 47. Balta-Calleja FJ, Vonk CG (1989) Polymer Science Library 8: X-ray Scattering of Synthetic Polymers, Elsevier Science Publishing, New York. 48. Vonk CG (1973) J Appl Cryst 6, p81. 49. Vonk CG (1975) J Appl Cryst 8, p340. 50. Sha’aban AK, McCartney S, Patel N, Yilgor I, Riffle JS, Dwight DW, McGrath JE (1983) Poly Preprints 24, p130. 51. Chen X, Gardella Jr JA, Ho T, Wynne KJ (1995) Macromolecules 28, p1635. CHAPTER 5 1. 2. 3. 4. 5. 6. 7. 8. 9. 10. 11. 12. Mark JE (2000) ACS Symposium Series, American Chemical Society 729, p1. Yilgor I, McGrath JE (1988) Adv Polym Sci 89, p1. Zang YH, Carreau PJ (1991) J Appl Poly Sci 42, p1965. Kinning DJ (2001) J Adh Sci 75, p1. Hergenrother RW, Yu XH, Cooper SL (1994) Biomaterials 15, p635 Ho T, Wynne KJ, Nissan RA (1993) Macromolecules 26, p7029. Chun YC, Kim KS, Shin JS, Kim KH (1992) Poly International, 27, p177. Yang CZ, Li C, Cooper SL (1991) J Poly Sci B: Poly Phy 29, p75. Shibayama M, Inoue M, Yamamoto T, Nomura S (1990) Polymer 31, p749. Kajiyama M, Kakimoto M, Imai Y (1990) Macromolecules 23, p1244. Tyagi D, Yilgor I, Wilkes GL, McGrath JE (1984) Polymer 25, p1807. Sheth JP, Aneja A, Wilkes GL, Yilgor E, Atilla GE, Yilgor I, Beyer FL (2004) Polymer 45, p6919. 13. Li C, Yu X, Spechard TA, Cooper SL (1988) J Poly Sci B: Poly Phy 26, p315. 170 14. Yilgor E, Burgaz E, Yurtsever E, Yilgor I (2000) Polymer 41, p849. 15. Rochery M, Vroman I, Lam TH (2003) J Macromol Sci A40, p321. 16. Wang LF, Ji Q, Glass TE, Ward TC, McGrath JE, Muggli M, Burns G, Sorathia U (2000) Polymer 41, p5083. 17. Gunatillake PA, Meijs GF, McCarthy SJ, Adhikari R (2000) J Appl Poly Sci 76, p2026. 18. Stanciu A, Airinei A, Timpu D, Ioanid A, Ioan C, Bulacovschi V (1999) E Poly J 35, p1959. 19. Fan Q, Fang J, Chen Q, Yu X (1999) J Appl Pol Sci 74, p2552. 20. Shibayama M, Inoue M, Yamamoto T, Nomura S (1991) Macromolecules 24, p6254. 21. Clarson SJ, Dodgson K, Semlyen JA (1985) Polymer 26, p930. 22. Johari GP, Hallbrucker A, Mayer E (1988) J Poly Sci B: Poly Phy 26, 1923. CHAPTER 6 1. 2. 3. 4. 5. 6. 7. 8. 9. 10. 11. 12. 13. 14. 15. 16. 17. 18. 19. 20. Wilkes GL, Abouzahr S, Radovich D (1983) J Cellular Plast 19, p248. Armistead JP, Wilkes GL, Turner RB (1988) J Appl Poly Sci 35, p601. Elwell MJ, Ryan AJ, Grünbauer HJM, Van Lieshout HC (1996) Polymer 37, p1353. Ibid (1996) Macromolecules 29, p2960. Aneja A, Wilkes GL (2004) Polymer 45, p927. Aneja A, Wilkes GL, Yurtsever E, Yilgor I (2003) Polymer 44, p757. Aneja A, Wilkes GL, Yilgor I, Yilgor E, Yurtsever E (2003) J Macromol Sci B: Phy 42, p1125. O’Rourke MJE, Ding D-K, Thomas EL, Perec V (2001) Macromolecules 34, p6658. Wilkes GL, Wildnauer R (1975) J Appl Phy 46, p4148. Camberlin Y, Pascault JP (1984) J Poly Sci: Poly Phy Ed 22, p1835. Sung CSP, Schneider NS (1975) Macromolecules 8, p68. Pimentel GC, McClellan AL (1960) The Hydrogen Bond, Reinhold Publications, New York, NY. These copolymers with HS branching were synthesized with the help of Ann R. Fornof, a graduate student in the research group of Prof. T. E. Long, and under the guidance of Dr. Iskender Yilgor of Koc University in Turkey. Armistead JP, Wilkes GL, Turner RB (1988) J Appl Poly Sci 35, p601. Moreland JC, Wilkes GL, Turner RB, Rightor EG (1994) J Appl Poly Sci 52, p1459. Dounis DV, Wilkes GL (1997) Polymer 38, p2819. Kaushiva, BD, Wilkes GL (2000) Polymer 41, p6987. Aneja A, Wilkes GL (2003) Polymer 44, p7221. See Chapter 8 for details. Sauer BB, Mclean RS, Gaymans RJ, Niesten MCJE (2004) J Poly Sci B: Poly Phy 42, p1783. 171 CHAPTER 7 1. 2. 3. 4. 5. 6. 7. 8. 9. 10. 11. 12. 13. 14. 15. 16. 17. 18. 19. 20. 21. 22. 23. 24. Kim YH, Webster OW (1988) Poly Preprints 29, p310. Kim YH (1998) J Poly Sci A: Poly Chem 36, p1685. Voit B (2000) J Poly Sci, A: Poly Chem 38: 2505-2525. Jikei M, and Kakimoto M (2001) Prog Poly Sci 26: 1233-1285. Froehling P (2004) J Poly Sci A: Poly Chem 42, p3110. Flory PJ (1952) J Am Chem Soc 74, p2718. Spindler R, Fréchet JMS (1993) Macromolecules 26, p4809. Kumar A, Ramakrishnan S (1993) J Chem Soc Chem Comm, p1453. Ibid. (1996) J Poly Sci A: Poly Chem 34, p839. Kumar A, Meijer EW (1998) Chem Comm, p1629. Yan D, Gao C (2003) Macromolecules 36, p613. Unal S, Yilgor I, Yilgor E, Sheth JP, Wilkes GL, Long TE (2004) Macromolecules 37, p7081. Zang YH, Carreau PJ (1991) J Appl Poly Sci 42, p1965. Thomas Mourey of Eastman Kodak Company in Rochester, NY conducted the SEC measurements. The solution viscosity of the copolymers was measured by utilizing the cone-and-plate rheometer in Dr. Charles E. Frazier’s laboratory at Virginia Tech. Faucher JA, Koleske JV (1968) Polymer 9, p44. Tong JD, Jerome R (2000) Macromolecules 33, p1479. Johari GP, Hallbrucker A, Mayer E (1988) J Poly Sci B: Poly Phy 26, p1923. Schollenberger CS, Dinbergs K (1979) Adv Urethane Sci Tech 7, p1. Ryan AJ, Macosko CW, Bras W (1992) Macromolecules 25, p6255. Fredrickson GH, Milner ST (1991) Phy Rev Lett 67, p835. Fredrickson GH, Milner ST, Leibler L (1992) Macromolecules 25, p6341. O'Sickey MJ, Lawrey BD, Wilkes GL (2003) J Appl Poly Sci 89, p3520. Tadokoro H (1979) Structure of Crystalline Polymers, Wiley Interscience, New York. CHAPTER 8 1. 2. 3. 4. 5. 6. 7. 8. 9. Hepburn C (1992) Polyurethane elastomers, Elsevier Applied Science, New York, NY. Noshay A, McGrath JE (1977) Block copolymers: Overview and critical survey, Academic Press, New York, NY. Tyagi D, McGrath JE, Wilkes G L (1986) Poly Eng Sci 26, p1371. Harrell, Jr LL (1969) Macromolecules 2, p607. Samuels SL, Wilkes GL (1973) J Poly Sci Symp 43, p149. Aneja A, Wilkes GL (2003) Polymer 44, p7221. Sauer BB, Mclean RS, Gaymans RJ, Niesten MCJE (2004) J Poly Sci B: Poly Phy 42, p1783. Barikani M, Hepburn C (1987) Cell Poly 6, p41. Differential scanning calorimetry of PTMO-pPDI-U indicated two convoluted endothermic peaks centered at 43 and 50°C that correspond to the melting transition of 172 10. 11. 12. 13. 14. 15. 16. the pPDI based HS phase. The melting point of pure pPDI is 97°C. In addition, the 2D WAXS of PTMO-pPDI-U indicated a sharp azimuthally independent reflection at 4.1Å. We conducted tensile tests of the sample PTMO-pPDI-Ur before and after compression molding. Both samples exhibited comparable Young’s modulus, tensile strength, and elongation at break thereby indicating that degradation or chemical cross-linking upon remolding was limited, if any at all. Pan N (1996) Sci Eng Composite Mat 5, p63. Mark JE (Ed.) (1996) Physical properties of polymers handbook, American Institute of Physics, New York. Lotz B, Kovacs AJ (1969) Poly Preprints 10, p820. Xu JT, Ryan AJ, Mai SM, Yuan JJ, Cheng YY (2004) J Macromol Sci B: Phy 43, p685. Balsamo V, Urdaneta N, Perez L, Carrizales P, Abetz V, Muller AJ (2004) Polymer 40, p1033. Zhu L, Mimnaugh BR, Ge Q, Quirk RP, Cheng SZD, Thomas EL, Lotz, B, Hsiao BS, Yeh F, Liu L (2001) Polymer 42, p9121. 173