A Study A Calculation of Neutron Cross Sections on Real Potential of Optical Model Wint Shwe War Hlaing* Abstract The optical model potential parameters which play an important role in the evaluation of nuclear data for applied purposes are not fully satisfied at low energy neutron scattering. They are fixed according to the target mass and incident energy. In this work the calculated data are compared with those of IAEA data especially for Li-7 and Th-232. Keywords: Neutron Cross-Sections, Optical Model, ABAREX, SCAT2 Introduction Nuclear cross-section data are needed for scientific works as well as for reactor construction. Nuclear cross-section data are provided by experimental work. Nuclear experiments are very expensive, so modal calculations are used to predict cross-sections. Various nuclear codes are developed to calculate nuclear cross-sections. Not all the codes are perfect so we have to find correction factors. Generally, nuclear cross-sections depend on target mass, incident energy and type of incident particle. Nuclear optical model is found to be only successful applicable for energy about 6MeV, and intermediate and heavy nuclides. The improvement for low energy and low mass nuclides is still of great interest for neutron cross sections calculation groups. The theoretical estimation of optical model parameters is still to be modified in low energy, low mass nuclides. The calculated neutron cross sections data were to be compared with those of IAEA data especially for Li-7 and Th-232. In this work the effect of real potential is V r ( r ) V f ( r ), r R1 f ( r ) 1 exp a1 1 where R is the radius and a is the surface diffuseness parameter. Statistical Model for Nuclear Reactions In the study of nuclear reactions the concept of the compound nucleus (the statistical model for nuclear reactions) is not always reliable. The statistical nature of the compound nucleus theory implies that its predictions are at best averages and do not take into account the differences between specific nuclei. Therefore a more detailed model is needed for the description of nuclear reactions. The statistical model assumes that the compound nucleus is formed immediately when the incident neutron reaches the nuclear surface. The cross-section for reaching the surface turns out to be a monotonically decreasing function of the energy, varying as E-1/2 for small energies and reaching the asymptotic value 2R2 for large energies. At the neutron energies involved, between 0.1MeV and several MeV, and for intermediate or 1. Dr., Assistant Lecturer, Department of Geography, Yangon Institute of Education 2. Dr., Assistant Lecturer, Department of Geography, Yangon Institute of Education heavy nuclei, individual resonances cannot be resolved, and the measured cross sections are averages over many levels. Optical Model for Nuclear Reactions The optical model describes the effect of the nucleus on the incident particle by a potential well –V0 (r), but allows for the possibility of compound nucleus formation by adding to the potential a negative imaginary part, -iV1(r). This part produces absorption of the incident particle within the nucleus, and this absorption is supposed to represent the formation of the compound nucleus. On the optical model, compound nucleus formation does not occur immediately or with complete certainty. Even if the incident particle has entered the nucleus, it is removed from its free particle state only with some delay and with a certain probability. The model has also been extended and applied with more complicated potential functions to other nuclear reactions and cross sections. The feature of nuclear scattering cross sections can be explained by a very simple model in which we represent the interaction between the incident nucleons and the nucleus by a one-body potential that depends only on the nuclear radius. This is called the optical model. Methods and Materials Calculation Procedure As the ABAREX runs under DOS, we have to load the Dos. After loading DOS, we have to load the ABAREX program. Under ABAREX program we open INPUT.DAT and make some changes to input data file. C:\> ABAREX > EDIT INPUT The file is saved and closed. The calculation is done when we type this command. C:\> ABAREX >DEL OUTPUT C:\> ABAREX >DEL PUNCH C:\> ABAREX > ABAREX To see and edit output results, we open ABAREX and rename it. C:\> ABAREX >EDIT OUTPUT Results and Discussions The calculated data and respective graphs are shown in the following tables and figures. Table 1. Comparison of Calculation data and IAEA Data for Li-7 Total Cross Sections (b) E(MeV) SCAT2 Vr = 46 MeV JENDL EXFOR 1 1.5571 1.2094 1.3200 1.5779 2 1.3728 1.1483 1.3938 1.7424 3 1.3875 1.1764 1.8628 2.0074 Total Cross Sections (b) E(MeV) SCAT2 Vr = 46 MeV JENDL EXFOR 4 1.4546 1.2434 2.1298 2.3836 5 1.5084 1.3148 2.0989 2.4544 6 1.5304 1.3683 2.0292 2.1725 7 1.5276 1.3980 1.9356 1.9662 8 1.5114 1.4081 1.8514 1.8078 9 1.4896 1.4056 1.7752 1.7786 10 1.4666 1.3965 1.6987 1.6628 11 1.4444 1.3846 1.6277 1.5808 12 1.4233 1.3723 1.5608 1.5813 13 1.4033 1.3608 1.4937 1.4968 14 1.3837 1.3504 1.4313 1.4391 15 1.3639 1.3410 1.3100 1.4533 16 1.3437 1.3324 1.3328 1.3562 17 1.3226 1.3240 1.2854 1.2684 18 1.3008 1.3154 1.2381 1.1828 19 1.2782 1.3064 1.1977 1.1718 20 1.2550 1.2976 1.1706 1.1858 Comparison of Cross-sections Data for Li-7 Total Cross-section (b) 3.00 2.50 SCAT2 2.00 Vr = 46 MeV 1.50 JENDL EXFOR 1.00 0.50 0.00 0 5 10 15 20 25 Neutron Incident Energy (MeV) Figure 1. Comparison of Calculation data and IAEA Data for Li-7 The comparison of total cross-sections for Li-7 using real potential 46 MeV with those of SCAT2 data, JENDL data and EXFOR data is given in Table 1 and the respective graph is shown in Figure 1. It can be seen that ABAREX data agree with SCAT2 data, and EXFOR data agree with JENDL data. Table 2. Comparison of Calculated Data and IAEA Data for Th-232 Total Cross Sections (b) E(MeV) SCAT2 Vr = 46 MeV JENDL EXFOR 1 7.8896 8.6491 6.9350 7.3790 2 6.8074 6.8441 7.0400 7.2210 3 6.9426 6.7317 7.7100 7.9620 4 7.2415 7.1399 7.8800 8.0210 5 7.3122 7.4845 7.5100 7.6910 6 7.1488 7.6346 6.9800 7.1490 7 6.7833 7.6056 6.4900 6.5900 8 6.3204 7.4540 6.0800 6.3500 9 5.8968 7.2212 5.7600 6.1550 10 5.5879 6.9347 5.6200 5.9480 11 5.4103 6.6367 5.6150 5.9360 12 5.3363 6.3787 5.6300 5.8680 13 5.3300 6.1880 5.6800 5.8150 14 5.3727 6.0227 5.7400 5.9330 15 5.4584 5.8236 5.8250 6.0120 16 5.5817 5.6618 5.9900 6.0380 17 5.7325 5.5833 6.1500 6.1090 18 5.8936 5.5833 6.2700 6.2600 19 6.0437 5.6497 6.3500 6.2640 20 6.1645 5.7617 6.4100 6.4370 Comparison of Cross-sections Data for Th-232 Total Cross-section (b) 10.00 9.00 8.00 7.00 6.00 SCAT2 5.00 4.00 JENDL Vr = 46 MeV EXFOR 3.00 2.00 1.00 0.00 0 5 10 15 20 25 Neutron Incident Energy (MeV) Figure 2. Comparison of Calculated Data and IAEA Data for Th-232 The comparison of total cross-sections for Th-232 using real potential 46 MeV with those of SCAT2 data, JENDL data and EXFOR data is given in Table 2 and the respective graph is shown in Figure 2. It can be seen that calculated cross sections show some difference from other below 14 MeV. Table 3. Best Fixed Real Potential for Total Cross-sections of Li-7 Total Cross Sections (b) E(MeV) Vr = 54MeV Vr = 46 MeV JENDL EXFOR 1 1.5213 1.2094 1.3200 1.5779 2 1.1354 1.1483 1.3938 1.7424 3 1.0994 1.1764 1.8628 2.0074 4 1.1507 1.2434 2.1298 2.3836 5 1.2049 1.3148 2.0989 2.4544 6 1.2387 1.3683 2.0292 2.1725 7 1.2549 1.3980 1.9356 1.9662 8 1.2606 1.4081 1.8514 1.8078 9 1.2616 1.4056 1.7752 1.7786 10 1.2614 1.3965 1.6987 1.6628 11 1.2621 1.3846 1.6277 1.5808 12 1.2645 1.3723 1.5608 1.5813 13 1.2689 1.3608 1.4937 1.4968 14 1.2747 1.3504 1.4313 1.4391 15 1.2809 1.3410 1.3100 1.4533 16 1.2866 1.3324 1.3328 1.3562 17 1.2910 1.3240 1.2854 1.2684 18 1.2936 1.3154 1.2381 1.1828 19 1.2942 1.3064 1.1977 1.1718 20 1.2927 1.2976 1.1706 1.1858 Best Fixed Real Potential for Total Cross-sections of Li-7 Total Cross-section (b) 3.00 2.50 Vr = 54MeV 2.00 Vr = 46 MeV 1.50 JENDL EXFOR 1.00 0.50 0.00 0 5 10 15 20 25 Neutron Incident Energy (MeV) Figure 3. Best Fixed Real Potential for Total Cross-sections of Li-7 The comparison of total cross-sections for Li-7 using real potential value of 46 MeV and 54 MeV, JENDL data and EXFOR data is given in Table 3 and the respective graph is shown in Figure 3. It can be seen that increasing the real potential makes the data more agree with EXFOR and JENDL data. Table 4. Best Fixed Real Potential for Total Cross-sections of Th-232 Total Cross Sections (b) E(MeV) Vr = 45 MeV Vr = 46 MeV JENDL EXFOR 1 8.3845 8.6491 6.9350 7.3790 2 6.8296 6.8441 7.0400 7.2210 3 6.8877 6.7317 7.7100 7.9620 4 7.3272 7.1399 7.8800 8.0210 5 7.6222 7.4845 7.5100 7.6910 6 7.6772 7.6346 6.9800 7.1490 7 7.5439 7.6056 6.4900 6.5900 8 7.3021 7.4540 6.0800 6.3500 9 7.0211 7.2212 5.7600 6.1550 10 6.7253 6.9347 5.6200 5.9480 11 6.4405 6.6367 5.6150 5.9360 12 6.2044 6.3787 5.6300 5.8680 13 6.0456 6.1880 5.6800 5.8150 14 5.9522 6.0227 5.7400 5.9330 Total Cross Sections (b) E(MeV) Vr = 45 MeV Vr = 46 MeV JENDL EXFOR 15 5.8497 5.8236 5.8250 6.0120 16 5.7167 5.6618 5.9900 6.0380 17 5.6350 5.5833 6.1500 6.1090 18 5.6342 5.5833 6.2700 6.2600 19 5.7042 5.6497 6.3500 6.2640 20 5.8257 5.7617 6.4100 6.4370 Best Fixed Real Potential for Total Cross-sections of Th-232 10.00 9.00 Total Cross-section (b) 8.00 7.00 6.00 Vr = 45 MeV 5.00 Vr = 46 MeV 4.00 JENDL EXFOR 3.00 2.00 1.00 0.00 0 5 10 15 20 25 Neutron Incident Energy (MeV) Figure 4. Best Fixed Real Potential for Total Cross-sections of Th-232 The comparison of total cross-sections for Th-232 using real potential value of 45 MeV and 46 MeV, JENDL data and EXFOR data is given in Table 4 and the respective graph is shown in Figure 4. It shows that Vr = 45 MeV much agree with EXFOR and JENDL than default value Vr = 46 MeV for Th-232. Conclusion Generally, from the results, the optical model fitting procedure for light nuclides and for heavy nuclides need more factors other than real potential, and for intermediate nuclides need less factors. And then, when it is compare with IAEA data, the calculated results are a bit difference for light nuclides and intermediate nuclides. So, they also need more effective parameters in the low energy range (below 5MeV). But, for heavy nuclides, the results are agreed with IAEA data. It is found that the calculated real potential is applicable for neutron energy range (1MeV to 20MeV) So in conclusion it can be said that calculation of cross-sections on the real potential of optical model well agree with those obtained given in JENDL and EXFOR especially for above 5MeV of neutron energy by using IAEA nuclear codes. The results are valid for various targets. The codes are also applicable for light nuclides, intermediate nuclides and heavy nuclides. Thus, the codes are the efficient tools for the determination of nuclear cross- section and other useful nuclear information. Acknowledgements I would like to express my profound thanks to Dr Lwin Lwin Soe and Dr Pyay Thein, Pro-Rectors of Yangon Institute of Education, for their constructive suggestions for the manuscript. I would also like to extend my gratitude and deep appreciation to Professor Dr Khin Mu Soe, Head of the Department of Physics, Yangon Institute of Education, and Dr Khin Tint, Associated Professor, Department of Physics, Yangon Institute of Education, for their kind permission and encouragement to carry out this research work. Special thanks should also go to Dr Win Sin, Lecturer, Department of Physics, Yangon University, for his kind help in writing my research paper. References Enge H A 1975 “ Introduction to Nuclear Physics ” (London ׃Addison-Wesley). Ganesan S 1991 “ABAREX, Optical-Statistical Model ” (OECD NEA Data Bank ׃PSR 248/ABAREX). ICTP 1984 “ Nuclear Theory for Applications _1982 ” (Vienna ׃IAEA). Jackson D F 1970 “ Nuclear Reactions ” (London ׃Methuen). Kaplan I 1962 “ Nuclear Physics ” (New York ׃Addison-Wesley). Morrison P & Feld B T 1953 “ Experimental Nuclear Physics ” (London ׃Chapman & Hall). Sedre E 1953 “ Experimental Nuclear Physics ” (New York ׃John Wiley). 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