NILES EAL603-2013 Dr. Salah Hassab Elnaby Lecture 9 Electro Optic and Photorefractive effects Electro Optic effect The electro optic effect is the change in refractive index of a material induced by the presence of a static (or low-frequency) electric field. 1- Pockels effect. In some materials, the change in refractive index depends linearly on the strength of the applied electric field Since the linear electro optic effect can be described by a second-order nonlinear susceptibility, it follows that a linear electro optic effect can occur only for materials that are noncentrosymmetric. The relation between the electric field strength and the electric displacement vector Let us define Then we get For uniaxial crystal NILES EAL603-2013 Dr. Salah Hassab Elnaby The change in the refractive index depend on the direction of polarization of the light and the direction of the applied static (or low frequency) this should be calculated from : For example for KDP and ADP this coefficients are NILES EAL603-2013 Dr. Salah Hassab Elnaby Longitudinal electro_optic modulation For KDP for example if the applied field is in the Z-direction then the indicatrix ellipsoid becomes To find the new principle coordinate system we define Substituting we get NILES EAL603-2013 ( ( So we get Dr. Salah Hassab Elnaby ) ) This means that the XY section of the ellipsoid before the applied voltage was a circle. Now applying a voltage V in the Z direction will produce a field EZ= V/L where L is the length of the crystal. A wave incident in the Z-direction polarized in the X=direction shall have two components in the x and y directions. The phase difference between the is nx-nycL= Note that in this case the modulation angle doesn’t depend on the length of the crystal. As a home work study the case of transverse electro_optic modulation NILES EAL603-2013 Dr. Salah Hassab Elnaby Photo refractive effect The photorefractive effect often leads to a very strong nonlinear response. This response usually cannot be described in terms of a χ(3) (or an n2) nonlinear susceptibility, because the nonlinear polarization does not depend on the applied field strength in the same manner as the other mechanisms listed. The propagation of an optical wave in insulating or semi-insulating electrooptical crystals induces a charge transfer. The new distribution of charges induces in turn an electric field which produces a variation of the refraction index. The main characteristics of this effect are the following: (1) Sensibility to energy (and not to the electric field), (2) Nonlocal effect (charge distributions and the electric field are not located at the same position), (3) Inertia (charges need a certain time to move), (4) Memory and reversibility (in the dark the space charge, and therefore the index variation, is persistent but an uniform light redistributes uniformly all charges — this yields applications to holography). NILES EAL603-2013 Dr. Salah Hassab Elnaby Photorefractive materials exhibit photoconductive and electro-optic behavior, and have the ability to detect and store spatial distributions of optical intensity in the form of spatial patterns of altered refractive index. Photoinduced charges create a space-charge distribution that produces an internal electric field, which, in turn, alters the refractive index by means of the electro-optic effect. Ordinary photoconductive materials are often good insulators in the dark. Upon illumination, photons are absorbed, free charge carriers (electron-hole pairs) are generated, and the conductivity of the material increases. When the light is removed, the process of charge photogeneration ceases, and the conductivity returns to its dark value as the excess electrons and holes recombine. In photorefractive materials the refractive index can be modified by illumination with light. The photorefractive effect can show very high light sensitivity in appropriate material thus permitting the observation of such effects at very low light power(< μW). There are many different effects which can lead to photorefraction as for example photochemical effects, photoinduced reorientation of molecules, Kerr effect at high intensity, or photoinduced thermal effects. We will restrict the NILES EAL603-2013 Dr. Salah Hassab Elnaby definition of the photorefractive effect to the light induced refractive index change due to charge transport in electro-optic materials. This definition has become common in literature. Photorefraction gives rise to many interesting effects as for example light induced wave-guiding, phase conjugation , beam amplification , and four wave mixing. NILES EAL603-2013 Dr. Salah Hassab Elnaby Conventional Model The so-called conventional model was elaborated by Kukhtarev et al. [7,8,9] considering only photo-excitation and recombination of one species of charge carriers between a single donor level and the corresponding conduction band. This single-level band scheme, along with the involved physical mechanisms, is depicted in Fig. 1.3. Note that while this simplified model describes satisfactorily the processes in a large number of materials showing the photorefractive effect, there exist several crystals where details of the charge transport mechanism are better described by considering additional defect levels [10, 11]. Another important limitation is that the photon energies of the light illumination must be smaller than the band-gap energy. The involved processes can be described by the following set of equations where the photoexcited charges are assumed to be electrons. The symbols in the above equations are: NILES EAL603-2013 Dr. Salah Hassab Elnaby Equation (1) is the rate equation for the concentration of the ionized donors. The first term describes the photoionization process (seI) and the thermal excitation of electrons from the donor level. The second term takes into account the recombination of the electrons (e) into traps, in our case ionized donors. The second equation (2) is the continuity equation for the electron density. The additional term with respect to Eq. (1) describes the divergence of the electron current density. Eq. (3) describes the different contributions to the electron current density. The first term gives the drift current in the total electric field E = Esc+E0, where E0 is the applied field. The second term describes the diffusion process of the electrons generated by the electron concentration gradient. Thus, this term only gives a contribution for inhomogeneous illumination. The last term gives the photo galvanic current, if present. The last equation (4) is the Poisson equation for the electric field. It describes the spatially modulated part of the electric field generated by the nonuniform distribution of the charge carriers in the crystal. NILES EAL603-2013 Dr. Salah Hassab Elnaby Applications of the Photorefractive Effect An image I(x, y) may be stored in a photorefractive crystal in the form of a refractive-index distribution n(x, y). The image can be read by using the crystal as a spatial-phase modulator to encode the information on a uniform optical plane wave acting as a probe. Phase modulation may be converted into intensity modulation by placing the cell in an interferometer, for xample. Because of their capability to record images, photorefractive materials are attractive for use in real-time holography. An object wave is holographically recorded by mixing it with a reference wave. The intensity of the sum of two such waves forms a sinusoidal interference pattern, which is recorded in the photorefractive crystal in the form of a refractive-index variation. The crystal then serves as a volume phase hologram. To reconstruct the stored object wave, the crystal is illuminated with the reference wave. Acting as a volume diffraction grating, the crystal reflects the reference wave and reproduces the object wave. Since the recording process is relatively fast, the processes of recording and reconstruction can be carried out simultaneously. The object and reference waves travel together in the medium and exchange energy via reflection from the created grating. This process is called two-wave mixing. Waves 1 and 2 interfere and form a volume grating. Wave 1 reflects from the grating and adds to wave 2; wave 2 reflects from the grating and adds to wave 1. Thus the two waves are coupled together by the grating they create in the medium. Consequently, the transmission of wave 1 through the medium is controlled by the presence of wave 2, and vice versa. For example, wave 1 may be amplified at the expense of wave 2. Home Work 1- A GaAs crystal with refractive index n = 3.6 and electro-optic coefficient r = 1.6 pm/V is used as an electro-optic phase modulator operating at = 1.3 pm in the longitudinal configuration. The crystal is 3 cm long and has a 1-cm2 cross-sectional area. Determine the half-wave voltage V the transit time of light through the crystal, and the electric capacitance of the device (the dielectric constant of GaAs is o = 13.5). The voltage is applied using a source with 50 resistance. Which factor limits the NILES EAL603-2013 Dr. Salah Hassab Elnaby speed of the device, the transit time of the light through the crystal or the response time of the electric circuit? 2- In a KDP crystal an electric field is applied along the optic axis of this uniaxial crystal, it changes into a biaxial crystal. The new principal axes are the original axes rotated by 45o about the optic axis. Assume a longitudinal modulator configuration .(d/L = 1) in which the wave travels along the optic axis. The two normal modes have refractive indices given in the lecture. Calculate the half wave voltage. 3- Cascaded Phase Modulators. (a) A KDP crystal (r41 = 8 pm/V, r63 = 11 pm/V; no = 1.507, ne = 1.467 at o = 633 nm) is used as a longitudinal phase modulator. The ray is incident in the z direction and polarization as in the preveous problem. Determine the half-wave voltage V at o = 633 nm. (b) An electro - optic phase modulator consists of 9 KDP crystals separated by electrodes that are biased as shown below. How should the plates be oriented relative to each other so that the total phase modulation is maximized? Calculate V for the composite modulator. 4- Double Refraction in an Electra-Optic Crystal. (a) An unpolarized He-Ne laser beam (o = 633 nm) is transmitted through a l-cm-thick LiNbO3 plate (ne = 2.17, no = 2.29, r33 = 30.9 pm/V, r13 = 8.6 pm/V). The beam is orthogonal to the plate and the optic axis lies in the plane of incidence of the light at 45o with the beam. The beam is double refracted. Determine NILES EAL603-2013 Dr. Salah Hassab Elnaby the lateral displacement and the retardation between the ordinary and extraordinary beams. (b) If an electric field E = 30 V/m is applied in a direction parallel to the optic axis, what is the effect on the transmitted beams? What are possible applications of this device?