ON THE BLOW OFF EXTINCTION OF A DIFFUSION FLAME OVER A THIN SOLID SHEET Effects of elevated gravity on propagating flame over a thin solid fuel sheet By TZUNG-HSIEN LIN Associate Professor Department of Mechanical Engineering, Southern Taiwan University of Technology, Yung Kang, Tainan 710, Taiwan Full-length paper Corresponding Author: Tzung-Hsien Lin Department of Mechanical Engineering Southern Taiwan University of Technology, 1 Nan Tai Street, Yung Kang, Tainan 710, Taiwan Telephone : 886-6-2533131 Ext 3542 FAX : 886-6-2425092 E-mail : thlin@mail.stut.edu.tw ABSTRACT A numerical study was made for the buoyancy effects on the ignition and subsequent flame spread over a thin solid fuel flatly lay on the floor in elevated gravity environments. Ignition was initiated in the middle of the sheet to give two flame fronts propagate in opposite directions. By varying the gravity level, and consequently Damkohler number, seven cases of flame spread over a thin solid fuel at 23.3 % oxygen mass concentration in a range of 1-7 times normal Earth gravity were conducted. The time of ignition delay increase slightly with increasing gravity within the computational range. The rate of flame spread was found decrease with increasing gravity level due to the Damkohler number effects. At gravity = 4 g, the flames were decelerated eventually stagnated. Flame blow off extinction was predicted at gravity = 5 g after few stagnant time. The greater the gravity the weaker the flame structure as well as the rate of flame spread. Because of the short fuel vapor resident time in high gravity environment, the fuel reaction rate reduced cause the flame shrike and temperature drops even to reach extinction. INTRODUCTION Intense theoretical and experimental investigations have recently been conducted on downward flame spread over a solid thin fuel surface. In the experimental studies, Olson et al. [1] and Olson [2] used a drop-tower to investigate the forced, opposed flow and quiescent flame spread in microgravity. The rate of flame spread was measured, and a low velocity-quenching limit was found to exist in low oxygen environments. Quiescent flame spread in microgravity experiments conducted on Space Shuttle facilities were presented by Bhattacharjee et al. [3]. The flame spread rate was determined using a frame-by-frame analysis of the film, and the solid surface temperature was measured. In purely buoyant flow flame spread experiments, Altenkirch et al. [4] investigated the buoyancy effects on downward spreading flames over thermally thin fuel. The parameter variation was determined by performing flame spread experiments in a closed chamber, which was swung on a centrifuge to generate a gravitational acceleration above that of the Earth. The rates of flame spread were obtained as the 5-cm spacing, divided by the elapsed time, was measured using an electrical clock. They found that an increase in the buoyancy level caused the flame spread rate to drop until no propagation was possible, indicating that an increasing gravity level tends to increase induced flow intensity such that it retards downward flame spreading. Lin and Chen [5] developed the foundation of the present study, which is a time-dependent combustion model of the ignition of a downward flame. In this work, attention was focused on both the solid and gas phase response at the moments before and after ignition. The ignition mechanism of a vertical thin solid fuel in a normal gravitational environment, subjected to an external radiant flux as the ignition source, was explored. Although the rate of flame spread was predicted, the flame diminished after a short period because the burn out regime (ash) was retained throughout the computation time. This caused a large amount of heat to stay at the flame tail and thus decreased the flame spread rate. By assuming that the ash was not retained, a moving boundary condition to account for ash removal was applied in this work. This latter procedure has been found successful for the direct simulation of a propagating downward flame. The main purpose of this work is to predict the rate of flame spread and the blow off extinction limit of a thin fuel at various gravity levels using an unsteady combustion model. By varying the Damkohler number through varying the gravity level, a series of parametric studies was performed to examine the effects of buoyancy on both the ignition delay time and the flame spread behavior over a horizontal thin solid fuel. For this time-dependent combustion model the spread rate will be obtained directly from the history of the flame front position, and the extinction phenomena at the blowoff limit will be depicted. A quantitative comparison between the results obtained from the steady model, developed by Duh and Chen [6], and the data measured by Altenkirch et al. [4], will verify the developed time-dependent model. MATHEMATICAL MODEL Figure 1 shows schematic diagram of two flames initiated at the center of a thin solid fuel sheet and propagate outward from the center in a quiescent gravitational environment. Both the left and right flames are opposite mode because the flame spread and the entrained flow directions are in opposite. Initially, the entrained flow along the fuel surface but it turns to flow upward due to heated in the flame zone, as shown in the figure. In this study the gravity levels were varied above the normal gravity. The ignition and subsequent flame spread behaviors in elevated gravitational field were examined. The mathematical model of the physical problem described proceed include unsteady gas-phase and solid-phase governing equations which coupled each other. The governing equations are described as follows: Governing Equations The gas phase model consist of two-dimensional, time-dependent continuity, complete elliptic Navier-Stokes, energy and species equations. The combustion is described by a one-step overall chemical reaction with finite rate global kinetics. The solid phase is modeled by an unsteady energy and mass conservation equations, which coupled with the gas phase through the energy feed back term from the gas phase. The solid pyrolysis is described by first-order Arrhenius expression. The nondimensional governing equations for the gas phase are summarized in Table 1. The dimensionless solid-phase governing equations can be expressed as follows for mass conservation: ms s E A s s exp( s ) . t Ts (1) and for energy conservation: Ts 2 Ts T s s m L ( 1 C )( T 1 ) qex s s t x 2 y Pr Gr w (2) . Boundary and Initial Conditions I. Boundary conditions in dimensionless form are, for gas phase: At x=xmin and x=xmax: u 0, v 0, T 1, YF 0, YO YO . , P P . (3) At y=0: u 0, T Ts , mw w v w mw mw YFw mw YOw Y F Pr Le Gr y Y O Pr Le Gr y w w . (4) At y=ymax: u v T YF YO 0 , P P . x x x x x (5) and for the solid phase: At x=xmin: s 1, Ts 1 . (6) At x=xmax: s 1, Ts 1 . II. Initial conditions in dimensionless form are, for the gas phase: (7) At t0: u 0, v 0, T 1, YF 0, YO YO , P P (9) and for the solid phase: At t0: s 1, Ts 1 . (10) Computational Grid The strong coupling between pressure and velocity in the full unsteady Navier-Stokes equations in gas phase are solved using the SIMPLE algorithm [7](Patankar, 1980). The detail computational procedure can be referred to Ref [5](Lin and Chen 1999). A non-uniform grid of exponential distribution in the gas phase was used with the grid points being concentrated near the gas-solid interface, where ignition is likely, to capture the significant change in the temperatures and flow field. A grid test has been conducted to ensure that the solutions are independent of grid size. The grid numbers of the entire computational domain were 238 for x, 153 for y direction, the corresponding nondimensional dimensional computational computational domain area was was 445.36363.21, 61.2450.16 cm2. and The nondimensional time step for computation was 13 corresponding 0.0712 s of the physical time. RESULTS AND DISCUSSION The ignition delay time as a function of gravity level was shown in Figure 2. The ignition delay time was defined as the time elapse from the external radiation applied to the instance of local maximum fuel reaction rate exceeds 110-4 g/cm3/s. The choice of this ignition criterion is because of we defined this value of contour in fuel reaction rate distribution as a visible flame boundary. As shown in the Figure2, the ignition delay time increase slightly with increasing in gravity level. This is because of higher buoyancy force enhance the convection to carry more amount of fuel vapor downstream. Therefore, it is need more time to accumulate enough fuel vapors to form a flammable mixture. The same trend of increase was found in the work of Nakamura (2000)[8] for gravity near normal gravity. Figure 3 shows the time histories of both right and left flames propagate in different gravities. The gravity varies from normal earth up to five times of normal gravity with increment of one. In this unsteady flame model the rate of flame spread can obtain from the slope of the loci of flames propagate. As shown in the figure, the rate of flame spread in 1g environment is about 0.29 cm/s but it decrease with the increasing in gravity due to the Damkohler number effects (Fernandz-Pello and Hirano 1983)[9]. Comparing to the downward flame spread (Altenkirch et al 1980[4], Duh and Chen 1991[6], Lin 2001[10]), the rate of flame spread in this horizontal direction is faster then that in downward. This result coincides with the experimental observations in the work of Hirano et al. (1974)[11]. Also, the rate of flame spread in horizontal direction obtained from this present unsteady flame model is near that obtained from the steady flame model (Chen and Chan 1992)[12], which using the integration of mass blowing rate from the solid surface to calculate the rate of flame spread. The case of 4-g in Figure 3 shows that the rate of flame spread was decelerated and eventually reaches zero after 4 s; the flame fronts almost no further advance, in other words, flame was stagnated. This is because of that, in this buoyancy level, the gas residence time becomes too small for the completion of the exothermic chemical reaction to maintain the flame spread process at a constant rate, the blow off extinction may occurs somewhere. Consequently, as expected, the blow off extinction occurs in the case of gravity = 5 g when the flames propagate little distance at 4.77 s after the external radiation applied. The blow off extinction process will be illustrated later. The flames shape, flow velocities vector distributions and temperature contours after 2 s of ignition occurs at various gravities are shown in the Figure 4 and Figure 5, respectively. As shown in the figures, the flame structure in 1-g gravity is strongest because the flame length and flame temperature are greatest. While the flame structure in 4-g gravity is weakest because the flame length and temperature are weakest. The weaker of the flame is due to the shorter of the gas residence time caused by the greater of the buoyant flow. This can be confirmed from the 4-g plot of Figure 4 in which the buoyant flow velocity vectors are the biggest compare to the other cases. The maximum buoyant flow velocity in 4-g case within the region show in the plot is about 236 cm/s compare to the that in 1-g case of 137 cm/s. Figure 4 also shows the flame in normal gravity propagate farthest within 2 s indicates that the rate of flame spread is fastest. The blow off extinction process in 5-g case is illustrated in Figure 6 and Figure 7. Figure 6 shows enlarge view for the sequence of gas-phase fuel reaction rate during the blow off extinction process while Figure 7 shows enlarge view for the sequence of gas-phase temperature. At gravity = 5g the buoyancy flow is strong enough such that the fuel vapor resident time in the flame is too short for exothermic chemical reaction completion. Consequently, the vigorous chemical reaction was reduced and the left and right straight flames shrinks into one flat flame after some stagnated times as shown in Figure 6 at 4.70 s. Meanwhile, the amount of heat release from the chemical reaction reduced cause the flame temperature drops as shown in Figure 7 at 4.70 s. Finally, the flat flame shrinks and the temperature drops continuously to become a point flame and disappear eventually, as shown at 5.06 s and 5.34 s in Figure 6 and Figure 7, respectively. CONCLUSIONS A numerical study was made for the buoyancy effects on the ignition and subsequent flame spread over a thin solid fuel flatly lay on the floor in elevated gravity environments. In this present time-dependent model we can readily simulate the flame propagation behavior over a thin fuel surface. By varying the gravity level, and consequently Da, we conducted seven cases of flame spread over a thin solid fuel at 23.3 % oxygen mass concentration in a range of 1-7 times normal Earth gravity. The computational results shown that the time of ignition delay increase slightly with increase gravity within the computational range. The time histories of flame front positions was plotted for various gravity, then the rate of flame spread was the slope of the flame propagation loci. The rate of flame spread was found decrease with increasing gravity level due to the Damkohler number effects. At gravity = 4 g, the flames were decelerated eventually stagnated. Flame blow off extinction was predicted at gravity = 5 g at 4.77 s after ignition occurs. The temperature and flame length in normal gravity were greatest indicated that it was the strongest flame. In the case of 4 g, the induced buoyant flow velocity reaches a value of 236 cm/s compare the 137 cm/s in normal gravity, but the temperature and flame size were lowest indicated that it was the weakest flame. The flame in normal gravity propagate farthest within 2 s indicates that the rate of flame spread is fastest. In case of 4-g gravity, the rate of flame spread decelerates to become stagnated at the final stage of propagates. The blow off extinction may occur some where for time greater than 6 s. At gravity = 5 g, the left and right straight flames shrinks into one flat flame after some stagnated times at 4.70 s. Meanwhile, the amount of heat release from the chemical reaction reduced cause the flame temperature drops. The flat flame shrinks and the temperature drops continuously to become a point flame and disappear eventually. ACKNOWLEDGMENTS The author would like to thank the National Science Council of the Taiwan for financially supporting this research under Contract No. NSC 90-2212-E-218-006. REFERENCES 1. S. L. Olson, P. V. Ferkul and J. S. T’ien, Twenty-Second Symposium (international) on Combustion, pp. 1213-1222, The Combustion Institute, Pittsburgh, 1988. 2. S. L. Olson, Combust. Sci. Technol., vol. 76, pp. 233-249, 1991. 3. S. Bhattacharjee, R. A. Altenkirch, and K. Sacksteder, Combust. Sci. Technol., vol. 91, pp. 225-242, 1993. 4. K. A. Altenkirch, R. Eichhorn, and P. C. Shang, Combust. Flame, vol. 37, pp. 71-83, 1980. 5. T. H. Lin, and C. H. Chen, Numerical Analysis of Ignition and Transition to Downward Flame Spread Over a Thermally-Thin Solid Fuel, I. J. Trans. Phenomena, vol. 1, pp. 255-275, 1999. 6. F. C. Duh, and C. H. Chen, A theory for Downward Flame Spread over a Thermally Thin Fuel, Combust. Sci. Technol., vol. 77, pp. 291-305, 1991. 7. S. V. Patankar, Numerical Heat Transfer and Fluid Flow, McGraw-Hill, New York, USA, 1980. 8. Nakamura, Y., Yamashita, H., and Takeno, T., Combust. Flame 120:34 (2000). 9. A. C. Fernandez-Pello and T. Hirano, Controlling Mechanisms of Flame Spread, Combust. Sci. Technol., vol. 32, pp. 1-31, 1983. 10. Lin, T. H., Num. Heat Transfer A 40:841 (2001). 11. Hirano, T., Noreikis, S. E., and Waterman, T. E., Combust. Flame 22353 (1974). 12. Chen, C. H., and Chan, S. C. Combust. Sci. Technol., 107:59 (1995). Table 1 Gas Phase Governing Equations u v S t x y x x y y Equation Continuity 1 x-Momentum u y-Momentum v Energy T Fuel YF Oxidizer YO S 0 p Su x Gr Gr p Sv y F F q Pr Gr F Pr Gr Le F f Pr Gr Le where Su 1 u v 2 v 3 x Gr x y Gr x 3 x Gr y Sv 1 v u 2 u 3 y Gr y x Gr y 3 y Gr x