Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
Irradiations at LANSCE May 2 – 19 2005
• Flight path 4FP15R was used, the same one used for NASA in 2001-3.
• The accelerator was not running well.
• Much of the time, it was running with a lower rep. rate of 40 Hz rather
than 100 Hz.
• Result:
Additional corrections required to account for the different rates
of production during an irradiation.
Longer irradiation times were required to get the desired yields.
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
•
All NASA irradiations had 5 cms of polyethylene upstream.
•
In 2005, there were 15 cms of polyethylene upstream
15R Flux
1.00E+07
5 cm Poly
5 cm
10 cm Poly
15 cm Poly
20 cm Poly
n/sr/MeV/To
1.00E+06
1.00E+05
15 cm
1.00E+04
1.0E+00
1.0E+01
1.0E+02
1.0E+03
Energy (MeV)
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
5 cm poly
15 cm poly
• 2005: Comparison of measured spectrum with MCNPX
calculation.
• The increase in fluence at lowest energies is an artifact but we still
need to understand what it is.
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
Ion chamber
• Irradiation set-up at LANSCE in beam line 4FP15R
• Looking upstream.
• The transmission ion chamber is behind the lead shield
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
• Targets irradiated: 5 x 5 cm targets of SiO2 and Si.
• I made three separate irradiations to measure the cross sections for
following reactions:
• 1) O(n,x)14C and Si(n,x)14C; 100 Hz only.
• 2) O(n,x)10Be and Si(n,x)10Be; Mixed 40 and 100 Hz.
• 3) O(n,x)Ne and Si(n,x)Ne; Mixed 40 and 100 Hz.
• Three runs were needed to keep the target stack thickness such that the
neutron beam transmission was >90% at almost all but the lowest
energies.
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
• Monitor foils of Al, Ni, Cu and Au were included in the target stacks.
• Cross sections for reactions producing relatively short-lived
radionuclides were measured.
• These can be used to:
1) Check that the corrections made for the different run
conditions were reasonable.
2) Explore how the different neutron energy spectra affect the
values measured for the energy integrated cross sections
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
• Many energy integrated cross sections measured in 2005 were measured
from 1998-2003 using the softer neutron energy spectrum.
• Average cross sections for reactions producing the relatively short lived
radionuclides are published in J. Sisterson and J. Ullmann, Nucl. Instr.
Meth. B 234 (2005) 419.
• These reactions have different thresholds, some are as low as 0.0 MeV
• Comparing these values to those that we measured in 2005 may be valuable
and give us insight into how the hardness of the neutron spectrum affects
the average cross section.
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
• In addition to these measurements of energy integrated cross sections,
cross sections at unique neutron energies ranging from ~70 - ~150
MeV were measured at iThemab LABS, South Africa.
• Cross sections for reactions in Cu producing relatively short lived
radionuclides are published in J.M. Sisterson et al. Nucl. Instr. Meth.
B 240 (2005) 617.
• A paper reporting similar cross section measurements for reactions in
Ti, Fe and Ni has been submitted (Nov. 2005) to Nucl. Instr. Meth.
• For all the reported reactions, the cross section values at unique
neutron energies are consistent with the average cross sections.
• Thus, average cross sections are very useful as a guide to the values
the cross section can assume as a function of energy.
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
Examples of some results: Do these graphs make sense?
Calculations were made where the shape of the energy spectra with 2 and 6
in of poly used were similar to those calculated using MCNPX:
(1) The reaction has a low threshold energy and initially the cross section is
high then falls to a smaller constant value, for example Ni(n,x)58Co.
Result: the cross section calculated for 6 in of poly tended to be lower than
that for 2 in of poly.
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
Examples of some results: Do these graphs make sense?
Calculations were made where the shape of the energy spectra with 2 and 6
in of poly used were similar to those calculated using MCNPX:
(2) The reaction has a high threshold and the cross section is zero at low
energies and then is like a step function, for example. Ni(n,x)52Mn.
Result: the cross section calculated using 6 in of poly was higher than that
calculated with 2 in of poly.
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
Future Plans
The budget for LANSCE was cut for fiscal 2006
This means:
1) Reduced number of days available for experimenters.
2) The accelerator will run at 40 Hz only
As a result:
1) We must think carefully what we want to do next.
2) We must be efficient in our use of time.
3) Perhaps we should concentrate on measuring cross sections for which
NO energy integrated cross sections have been measured.
December 2005
CRONUS Annual Meeting
Francis H. Burr Proton Therapy Center
Massachusetts General Hospital
Which targets should I irradiate next?
Kuni’s ideal list is below.
What other targets should be added to this list?
Irradiated with
2 in poly
6 in poly
Si


SiO2


Si3N4
x
CaCO3

MgO
Mg
KNO3
K2CO3
Fe

FeS
x
Ni

Ba
x
December 2005
CRONUS Annual Meeting