DSMC Calculation of Supersonic Expansion at a Very Large Pressure Ratio Koji Teshima1 and Masaru Usami2 1 Department of Industrial Arts Education, Kyoto University of Education, Kyoto JAPAN 2 Department of Mechanical Engineering, Mie University, Tsu, Mie JAPAN Abstract. Supersonic expansion of room temperature argon from a sonic orifice at a very large pressure ratio up to 16000 for different stagnation Knudsen numbers, 2x10~3 and 4X10"4 is simulated by the DSMC method. In order to calculate a large flowfield different sized cells and a different time-step scheme were adopted. It was shown that the effects of rarefaction and background gas to the jet size can be evaluated using a rarefaction parameter or a local Knudsen number. The calculation was also made for the expansion to a vacuum for a wide range of the stagnation Knudsen number, 4x10" 4 - 0.1. The terminal parallel temperature dependence to the stagnation Knudsen number agrees well with the sudden freezing model. INTRODUCTION The DSMC calculation of a supersonic expansion at a finite pressure ratio of the stagnation to the expansion chamber pressures, p(/pl9 has shown a good agreement with the experimental observation in the previous paper[l]. However, in the calculation the pressure ratio was limited up to about 100, due mainly to the limitation of the computer memory and the CPU time. In many applications such as manufacturing facilities of electronic devices, molecular beam facilities, and molecular spectroscopy apparatus, the working gas is expanded into a vessel not at vacuum, but still at a finite pressure; at a very large pressure ratio. In such expansion, in addition to the rarefaction effects such as broadening of the shock waves and the merging of the jet boundary with shock wave the background molecules which are accommodated with the vessel wall penetrate into the jet core and they collide with expanding cold molecules, warm up and decelerate them. As a result no distinct jet core cannot be seen in the density field, whereas the jet core, in which the flow is kept supersonic, exists. This supersonic region must become very much narrower than the expected one from the well known relation by Ashkenas and Sherman [2] for the continuum expansion. The jet structure including the length of the supersonic jet core and the distribution of the flow properties are not known well for these large pressure-ratio jets, although estimation of them might be important for the applications. The background gas effect to the jet were studied in relation to molecular beam intensity [3], but these were indirect measurements. Muntz et al.[4] introduced a rarefaction parameter (=d(pcp1)1/2/T0[dyne/cmK], with orifice diameter d and the stagnation temperature T0) which correlated certain of the rarefaction phenomena from shock broadening to the penetration of background gas into the core of the jet. In the previous paper [1] we have shown that the density distribution on axis can be classified by three flow regimes; continuum, transition, and scattering, using the rarefaction parameter for a wide range of the flow condition. A theoretical work of the background gas penetration based on the asymptotic gas kinetic theory for a source flow expansion was made by Brook et al.[5] However, they were limited only on the jet center line. In some applications the radial distribution of the flow properties will be as important as the axial ones. Therefore, the whole flowfield of such rarefied jets needs to be analyzed over a wide range of the pressure ratio and for different stagnation Knudsen numbers. In this study the calculation method has been improved in order to enable the calculation of a very large pressureratio jet; up to 16000 for the stagnation Knudsen numbers Kn=l/50Q and l/2500.The present calculation enables to evaluate the jet structure with not only different stagnation Knudsen numbers but also with a wide range of the pressure ratio. CP585, Rarefied Gas Dynamics: 22nd International Symposium, edited by T. J. Bartel and M. A. Gallis © 2001 American Institute of Physics 0-7354-0025-3/01/$18.00 737 It is well known that in a supersonic expansion non-equilibrium in the translational energy modes; between the translational temperatures in the parallel and perpendicular directions to the expansion, occurs. This phenomena is one of the rarefaction effect of the supersonic expansion. The former (the parallel temperature T//) does not lower enough due to not enough collisions in the parallel direction i.e. freezing of the parallel temperature, while the latter (the perpendicular temperature T 0) continues to decrease with distance. The degree of the parallel temperature freezing has been measured by the molecular beam time-of-flight method [3] and its dependency on the stagnation Knudsen number agreed well with an empirical formula based on a sudden freezing model [6]. In order to confirm the validity of the present calculation method and to demonstrate the effect of the background molecules to the expansion, expansions into a vacuum for different stagnation Knudsen numbers were calculated. The calculated freezing parallel temperature was compared with the existing empirical formula[6]. METHOD OF CALCULATION The position of the Mach disk of a continuum free jet XM can be predicted from the experimental formula presented by Ashkenas and Sherman [2] as xA/d=Q.61(pQ/p1)l/2. That is, since its distance from an orifice is proportional to the square root of a pressure ratio, if a pressure ratio is increased by about 250 times from 60 to 16000, the calculation domain whose length is about 16 times larger and whose volume is about 4000 times larger is required. Of course, since background pressure will become small if stagnation pressure is fixed and a pressure ratio is enlarged, the number of molecules that exist in the calculation domain becomes only about 16 times larger. However, since the calculation time which is required for achievement of a steady state is also proportional to the length of the calculation domain, after all, when a pressure ratio changes 250 times larger, total calculation time is increased by 100 times or more. This is a reason why a jet calculation with a large pressure ratio is difficult. Since a free jet reduces its density quickly at a longer distance from an orifice, for a cell network that subdivides a flowfield, the cell length is made to increase in geometric series not to produce a big difference in the number of molecules of each cell. For example, on x axis, if the length of the cell just behind an orifice is set to a, and a common ratio is set to b, the length of the z-th cell will become abl~l. If the position coordinate of a molecule is set to jc, a cell number n to which the molecule belongs is calculated easily by n=log{x(b-l)/a+l}/log(b)+l (omit under decimal point). Now, when a molecule passes a large cell, it is not efficient calculation that the distance to which a molecule moves per time step dt is too small compared with the cell length. Experientially, the moving distance per step is satisfactory if it is about 1/5 times the cell length. However, since it is difficult to change a time step according to the position coordinates of a cell (it is difficult to synchronize different time steps), a fixed time step is adopted usually over all domain in the conventional program. Since this time step is determined on the basis of the place where density is large, i.e., a small cell, conversely in the cell with large dimension and small density, the time step becomes short beyond necessity. As a result, the amount of the whole calculation increases and the calculation time becomes long. In the present calculation, as shown in Figure 1 (for the case of pQ/pi=16000 and l/Kn=25QQ), the downstream of an orifice is divided into 12 blocks and they are classified into seven classes (Class 1-Class?), where the far block from an orifice has a longer time step. If it takes into consideration that a molecule needs to pass through the boundary of each domain, the value of twice is suitable for the ratio of time step between adjoining blocks. Therefore, a time step increases by a geometric series of the common ratio 2 with the distance of cell from an orifice. That is, after molecules that are in the block near an orifice (Class 1) finish a repetition of 64 movements and intermolecular collisions, molecules in the farthest block (Class?) will perform one long time movement and intermolecular collision. So, calculation time can be shortened as the farthest block is made large and molecules that exist there increase. In regard to molecules that move between blocks, the procedure such as stopping molecules on the boundary of blocks, changing a time step there, and moving them again may be considered. However, this may become a complicated procedure and has a possibility of preventing shortening of calculation time. If a molecule goes through a boundary simply using the time step of the block in which the molecule exists before moving, unbalance of time between "molecular motion" and "intermolecular collision" will arise near the boundary. For example, the half of the molecules that move from a block with a large time step to a block with a small time step has a lack of intermolecular collisions. As will be shown in Figure 3 (left), distortion in the density contour is produced near the boundary of blocks by the above-mentioned simple processing. The straight line which is visible near y/d=3 is the most remarkable distortion. Usually, in the DSMC method, the time step dt for molecules that flow in from outside of a calculation domain is to be multiplied by a random number, and time for molecular motion in the domain is shortened. If this is 738 neglected, the move time of molecules flowing in from a boundary will become larger than collision time, and will make distortion in the flowfield near a boundary. In figure 3 (left), the phenomenon that is similar with this arises near a block boundary. In the present calculation, in order to prevent this, the following procedure is considered (See Fig.2). Numbers given under the arrow express the length of collision time. (a) When moving to the block-B with a large time step from the block-A with a small time step. (a-1) The molecules that pass through the boundary by the first step dt of the block-A continue their movement at the second step of the block-A after entering into the block-B. However, intermolecular collisions are not calculated between both steps. After movement of the second step, the calculation of intermolecular collisions in the block-B follows it. (a-2) For the molecules that pass through the boundary at the second step of the block-A, the calculation of intermolecular collisions in the block-B follows the molecular motion as usual. (b) When moving to the block-A with a small time step from the block-B with a large time step. (b-1) The molecules that pass through the boundary earlier than the half of the time step 2dt of the block-B stop their movement at one half of the time step. From this state, the calculation of intermolecular collisions in the blockA continues. (b-2) The molecules that could not cross a boundary within the half of the time step of the block-B finish their movement in the time step 2dt of the block-B. After that, the intermolecular collisions and the molecular motions in the first step of the block-A are paused once, respectively. And the calculation starts again from the subsequent intermolecular collisions. In above (a-1), the collision time (the average of the collision time between pre-movement and post-movement) is l.5dt on contrary to the move time of molecules through the boundary being dt+dt. However, in (a-2), since the collision time is l.5dt on contrary to the move time being dt, if both of (a) are averaged, the unbalance between the move time and the collision time is cancelled. Moreover, in (b-1), the collision time is l.5dt on contrary to the move time of molecules through the boundary being dt. However, in (b-2), since the collision time is l.5dt on contrary to the move time being 2dt, if both of (b) are averaged again, the unbalance between the move time and the collision time is also cancelled. The fundamental idea on the above procedure is such that molecules that flow into a new block act as if they exist in the block for a long time. /'/, '' / ./ClassS Class4 Downstream boundary Class6 Block A Block B Time step = dt Time step = 2dt dt+dt T o ) ^ 2 Po/Pl=16000 Class? dt <a-2). (2dt) Classl \xxO-ciass4 Class2 ClassS Collision time Figurel. Downstream computational domain divided into 12 blocks. 20 25 Figure!. Molecular motion between different blocks. Axial distance (x/d) Axial distance (x/d) Figure 3. Comparison of density contours with (right) and without (left) considering the time-step difference between different blocks. 739 Figure 3 (right) is the result obtained by the above-mentioned procedure. Although calculation conditions are the same as that of the left, the distortion near the boundary is canceled completely. And it agrees well with the result of conventional calculation obtained using constant time step in all domains. Thus, using the procedure mentioned above, it is possible to simulate the jet flowfield efficiently with variable time steps without complicated processing. Figure 3 (right) is the result obtained by the above-mentioned procedure. Although calculation conditions are the The calculation speed about 8 times faster than that by the conventional program has been obtained (in the case of same as that of the left, the distortion near the boundary is canceled completely. And it agrees well with the result of pQ/pl=l60QQ and l/Kn=25QQ). As large-sized data (a big array), the array which memorizes a name of block in which conventional calculation obtained using constant time step in all domains. Thus, using the procedure mentioned each above, molecule to arrays usedwith by general calculation program. processing. Its size is the it is exists possibleistorequired simulatein theaddition jet flowfield efficiently variable DSMC time steps without complicated sameThe as the number of molecules. However, since it is memorizable with one byte integer, it does not become calculation speed about 8 times faster than that by the conventional program has been obtained (in the case so of big a burden. p0/p1=16000 and 1/Kn=2500). As large-sized data (a big array), the array which memorizes a name of block in which Now, although exists the above procedure has tobeen devised the calculation time balance between each molecule is required in addition arrays used bymaintaining general DSMC program. Its size"molecular is the movement" "intermolecular collisions", paying attention to with a motion of integer, each molecule, same as and the number of molecules. However,ifsince it is memorizable one byte it does notunnaturalness become so bigwill a burden. remain in the calculation processing in the case of moving of molecules from a block with large time step to a block Now, the Since above aprocedure devised maintaining time through balance abetween "molecular with small timealthough step in (b). molecule has stopsbeen its movement for dt whenthe passing boundary, small time andhere. "intermolecular collisions", if payingofattention a motion molecule,On unnaturalness will for delaymovement" is generated If a calculation is an analysis a steadytoflow, thereofis each no problem. the other hand, remain inofthe processing in the case of moving a blockHowever, with largesince time step to a block the analysis ancalculation unsteady phenomenon, a simulation will of bemolecules distorted from delicately. the time scale of with small time step in (b). Sincethan a molecule stops movement for dt when passing a boundary, small time the unsteady phenomenon is larger time step dt its generally, it hardly becomes thethrough problem. delay is generated here. If a calculation is an analysis of a steady flow, there is no problem. On the other hand, for The Knudsen number is defined by a mean free path at stagnation divided by an orifice diameter d. As boundary the analysis of an unsteady phenomenon, a simulation will be distorted delicately. However, since the time scale of conditions applied to molecules that flow in from an upstream boundary, the Maxwell distribution with some flow the unsteady phenomenon is larger than time step dt generally, it hardly becomes the problem. velocityThe perpendicular to theis boundary assumed. On at thestagnation other hand, on by a downstream boundary, the Maxwell Knudsen number defined byisa mean free path divided an orifice diameter d. As boundary distribution at background pressurethat without velocity is assumed. Thethe diffuse reflection is assumed on aflow wall of conditions applied to molecules flow flow in from an upstream boundary, Maxwell distribution with some an orifice. The collision between molecules performed by the null-collision method using VHS molecular model velocity perpendicular to the boundary is is assumed. On the other hand, on a downstream boundary, the Maxwell for argon. For pjpi=16000, the size of a flowfield (axially symmetric field) is 0.75d x 0.75J for an upstream of an distribution at background pressure without flow velocity is assumed. The diffuse reflection is assumed on a wall of orifice, and 247d 54d forbetween a downstream orifice. by The of molecules is about millionsmodel and the an orifice. The xcollision moleculesofisan performed thenumber null-collision method using VHS16 molecular number of cellsFor is about 140,000. for argon. the size of a flowfield (axially symmetric field) is 0.75d x 0.75d for an upstream of an p0/p1=16000, orifice, and 247d x 54d for a downstream of an orifice. The number of molecules is about 16 millions and the number of cells is about 140,000. RESULTS AND DISCUSSION RESULTS AND DISCUSSION The Mach number profile of a jet at pressure ratio of 16000 for l/Kn=25QQ and 500 are shown in Figure 4. The Mach number reaches about 20 for l/Kn=25QO and begins to decrease gradually at a distance much shorter than Xy/d The Mach number profile of a jet at pressure ratio of 16000 for 1/Kn=2500 and 500 are shown in Figure 4. The and eventually thereaches flow becomes No distinct shock or jet core exists. The supersonic expansion region Mach number about 20subsonic. for 1/Kn=2500 and begins to decrease gradually at a distance much shorter than xM/d has been and narrowed due to the rarefaction effects by the broaden and merged shock waves with the jet boundary and to eventually the flow becomes subsonic. No distinct shock or jet core exists. The supersonic expansion region has the background gasdue effect byrarefaction penetration of the molecules into the jet core and/or collisionsand of towith been narrowed to the effects by background the broaden and merged shock waves with the jet boundary expanding molecules. l/Kn=5QO the attainable number becomesinto lower andcore the supersonic regionofbecomes the background gasFor effect by penetration of the Mach background molecules the jet and/or collisions with narrower. expanding molecules. For 1/Kn=500 the attainable Mach number becomes lower and the supersonic region becomes narrower. 1/Kn=250G, pressure ratio=16000 1/Kn=500, pressure ratio=16000 20 15 10 5 0 Figure 4. Mach number distribution a jetat/?^ at p07/p for 1/^=2500 1/Kn=2500 (left) 1=16000 for Figure 4. Mach number distribution ofofa jet =16000 (left)and and500 500(right). (right). 740 In Figure 5 the density distributions on axis at different pressure ratios for l/Kn=25QQ are shown. The expected In Figure 5 the density onby axis at different for with 1/Kn=2500 are shown. The expected locations XM of the Mach diskdistributions are indicated lateral lines. pressure It can be ratios seen that increasing the pressure ratio the locations of the Mach disk are indicated by lateral lines. It can be seen that with increasing the pressure ratiowith the x density begins M to increase upstream of XM and the supersonic region has been relatively narrowed in comparison begins to increase of xtheory. and the supersonic region has been relatively narrowed in comparison with thedensity expected region from theupstream continuum This is more clearly seen from the temperature distribution shown in M the expected from the continuumbetween theory. the Thisparallel is moreand clearly seen from the distribution in Figure 6, whereregion an average temperature perpendicular onestemperature is shown, and from theshown velocity Figure 6, where an average between the parallel and perpendicular ones isinto shown, and from the velocity distribution on axis, shown intemperature Fig.7. In these figures flow properties for expansion vacuum are also shown. distribution shown into in Fig.7. In these figures flowway properties forbackground expansion into vacuum are The also average shown. They follows on the axis, expansion vacuum in almost same until the effects appear. They follows thetoexpansion into vacuum in almost samethe way until begins the background temperature begins increase upstream the location where density to increase.effects appear. The average temperature begins to increase upstream the location where the density begins to increase. EH 0.1 EH I 0.01 £ >1 3rd 0.1 M CD 0.001 a -P i 0.0001 0.01 Q 1e-05 10 100 10 Axial distance (x/d) Axial distance (x/d) Figure 5. 5. Density profile ononaxis. Figure Density profile axis.l/Kn=250Q. 1/Kn=2500. Figure l/Kn=25QO. Figure6.6.Average Averagetemperature temperature profile profile on on axis. axis. 1/Kn=2500. = In In thethecase 16000, when caseofofl/Kn=25QQ 1/Kn=2500and andP(/PI whenthe theorifice orificediameter diameter d=l mm the the pressure pressure in in the the expansion expansion p0/p1=16000, d=1 mm chamber will be 1 Pa. At this background pressure the effect to the supersonic jet is still severe; the attainable Mach chamber will be 1 Pa. At this background pressure the effect to the supersonic jet is still severe; the attainable Mach number will be less than 20. In case of l/Kn=5QQ the background pressure will be 0.2 Pa with the same orifice, number will be less than 20. In case of 1/Kn=500 the background pressure will be 0.2 Pa with the same orifice, the the attainable Mach number becomes This rarefaction and background gas effect can be evaluated using using attainable Mach number becomesabout abouthalf half(11). (11). This rarefaction and background gas effect can be evaluated 05 a local Knudsen number rarefaction a local Knudsen numberdefined definedbybyKn^Knfa^pj) theinverse inverseof ofwhich which isis essentially essentially the the same same as as the the rarefaction KnL=Kn(p0/p' 1,)0.5,the parameter . Here, we assume the supersonic expansion distance as a distance x , where the velocity 10% 09 falls 10% parameter ξ. Here, we assume the supersonic expansion distance as a distance x0.9, where the velocity falls from the value obtained for the expansion into a vacuum. The relative supersonic expansion distance on axis to the from the value obtained for the expansion into a vacuum. The relative supersonic expansion distance on axis to the expected location of the Mach disk X is plotted as a function of l/Kn and in Figure 8. It can be seen that the L L and ξ in Figure seen that the expected location of the Mach disk MxM is plotted as a function of 1/Kn rarefaction and background gas effects on the jet core length can be evaluated by Kn or for wide ranges of the rarefaction and background gas effects on the jet core length can be evaluated by KnLL or ξ for wide ranges of the stagnation Knudsen number stagnation Knudsen numberand andthe thepressure pressureratio. ratio. 1.8 1.6 1.4 1.2 1 0.8 0.6 0.4 0.2 0 Axial distance (x/d) Figure8.8.Rarefaction Rarefaction effect effect to tojet jet core core length. length. Figure Pressureratio ratioranges ranges from from 15 15 to to 16000. Pressure 16000. Figure Axial velocity profile.l/Kn=2500. 1/Kn=2500. Figure 7. 7. Axial velocity profile. 741 The density field of the supersonic jet is often approximated by the following equation (Boyntons's formula) [7], (x,0) = cos2 cos7( 12 J, where =tan1(y/x), / = 2/( -1) , and m= {[( +!)/( -l)]1/2-l}/2 for the gas with the specific heat ratio .In Figure 9 radial density distributions at different axial distances for the jet of p(/p1=l6QOQ and l/Kn=25QO are compared with above equation. It can be seen that the Boyntons's formula is a good approximation for the off-axis density distribution in a certain region, which depends on the flow condition. 20 40 radial distance (y/d) Figure 9. Radial density distribution at different axial locations. and l/Kn=25QQ. In order to compare the calculation with the experimental observation using the laser-induced fluorescence (LIF) method [8] the calculated results were used to produce a pseudo-LIF intensity distribution. In Figure 10 the pseudoLIF intensity is compared with the LIF visualization. Although the comparison is only relative, because the sensitivity of the film in not linear, the pseudo-LIF intensity distribution gives a similar image as observed by the LIF method. PQ/P=8000 20 60 x/d 80 100 120 J__| 10 20 30 40 50 60 70 80 90 100 110 x/d Figure 10. The pseudo-LIF intensity compared with the corresponding LIF photograph. In a rarefied jet it is well known that the parallel translational temperature does not lowered from a certain value, which depends on the stagnation condition p^d or the stagnation Knudsen number Kn, due to not enough collisions during the expansion. The terminal speed ratio S// ^ defined by this terminal parallel temperature (S// =u /(2kT// ^ 742 /m)°'5, with u ^is the isentropic terminal velocity, k the Boltzmann constant and m the atomic mass) is given as S// L =l.QlKnQA [6] using a sudden freezing model. In order to confirm the validity of the present calculation method and to demonstrate the effect of the background molecules to the expansion, calculation was made for the expansion into vacuum; without interaction with background molecules for a wide range of the stagnation Knudesn number, 4x10"40.1. The calculated parallel and perpendicular temperatures are shown in Figure 11. Both temperature can be assumed to be equilibrium at the orifice for Knudsen numbers smaller than 0.01. The parallel temperature tends to freeze and the attainable parallel temperature (the terminal parallel temperature, T// ) decreases with decreasing Kn, whereas the perpendicular temperature continues to decrease in an almost similar manner for different Kn smaller than 0.01. For expansions with the stagnation Knudsen number larger than 0.01 the temperature non-equilibrium already occurs in the upstream region of the orifice. By using the definition of the speed ratio and by assuming that the flow velocity has reached to its terminal value, the terminal parallel temperature can be written as T// L /T0=2.18Kn°-8 from the above equation. In Figure.12 the terminal parallel temperatures are plotted against l/Kn and are compared with the equation reduced from the sudden freezing model. The calculated values agree well with the existing relation and then the present DSMC calculation method proves to be a good simulation of the supersonic jets in a wide flow conditions. 100 10 10000 Axial distance (x/d) Figure 12. Terminal parallel temperature as a function of inverse of Knudsen number; comparison with the sudden freezing model. Figure 11. Parallel and perpendicular temperature on axis for expansion into vacuum. CONCLUSIONS We have applied the DSMC method to simulation of the supersonic free jet issuing from a thin circular orifice and have obtained the following conclusions. 1. By adopting the different time-step scheme a large flow field could be treated and a jet of a very large pressure ratio, up to 16000, could be simulated. 2. The rarefaction and background gas effects to the jet size can be evaluated quantitatively by the local Knudsen number defined by Kn^Knfa^pjf'5 or the rarefaction parameter introduced by Muntz[4]. 3. The empirical equation (Boyntons's formula[7]) for the radial density distribution is a good approximation for the off-axis density in a limited region, which depends on the flow condition. 4. Computation of the expansion into vacuum for a wide range of the stagnation Knudsen number showed that the dependence of the frozen parallel temperature to the stagnation Knudsen number agrees well with the sudden freezing model [6]. 5. Above conclusions give the validity of the present DSMC calculation method to simulate the supersonic jets in wide ranges of the pressure ratio and the stagnation Knudsen number. 743 REFERENCES 1. Teshima, K. , and Usami, M., An Experimental Study and DSMC Simulation of Rarefied Supersonic Jets, Rarefied Gas Dynamics, ed. by C. Shen, Beijin University Press, pp.567-572, 1997. 2. Ashkenas, H. and Sherman, F.S., The Structure and Utilization of Supersonic Free Jets in Low Density Wind Tunnel, Rarefied Gas Dynamics, Fourth Symposium, Vol.11, Academic Press, New York, 1966, pp.84-95. 3. Anderson J.B. , Molecular Beams from Nozzle Sources, in Molecular Beams and Low Density Gas Dynamics, Wegener, P.P ed., Dekker, N.Y. 1974. 4. Muntz, E.P., et al., Some Characteristics of Exhaust Plume Rarefaction, AIAA J. 8, 1984, pp.1651-1658. 5. Brook, LJ.W., Hamel, B.B., and Muntz, E.P., Theoretical and Experimental Study of Background Gas Penetration into Underexpanded Free Jets, Phys. Fluids, Vol.18, 1975, pp.517-528. 6. Anderson, J.B. and Fenn, J.B., Phys. Fluids, 8, 1965, p.780. 7. Boynton, F.P. AIAA J. 5, 1967, p. 1703. 8. Teshima, K. and Nakatsuji, H., Visualization of Rarefied Gas Flows by a Laser Induced Fluorescence Method, Rarefied Gas Dynamics, ed. by Oguchi, H., University of Tokyo, 1984, pp.447-454. 744