15 January 2001 Optics Communications 187 (2001) 407±414 www.elsevier.com/locate/optcom Formation of higher-order Bessel light beams in biaxial crystals T.A. King a,1, W. Hogervorst b,2, N.S. Kazak c,3, N.A. Khilo d,4, A.A. Ryzhevich c,* a b Laser Photonics, Department of Physics and Astronomy, University of Manchester, M13 9PL Manchester, UK Laser Centre, Department of Physics and Astronomy, Free University, De Boelelaan 1081, 1081 HV Amsterdam, Netherlands c Institute of Physics, NAS of Belarus, 68 F. Skaryna ave., 220072 Minsk, Belarus d Division for optical problems in information technologies, NAS of Belarus, 1-2 Kuprevich str., 220141 Minsk, Belarus Received 5 September 2000; accepted 15 November 2000 Abstract A transformation of the order of a Bessel light beam (BLB) from zeroth to ®rst and from ®rst to second when propagating light through a biaxial crystal has been studied theoretically and experimentally. The possibility of the formation of higher-order BLBs by means of this eect is con®rmed. The transformation of beam order is observed when propagating circularly polarized light along the optical axis of the crystal under conditions of internal conical refraction. It is shown that a proper choice of the crystal length or conicity angle of the incident beam permits complete transformation of a zero-order Bessel input beam into a ®rst-order Bessel beam. Ó 2001 Published by Elsevier Science B.V. PACS: 42.25.Bs; 42.25.Ja; 42.25.Lc Keywords: Bessel light beam; Internal conical refraction; Biaxial crystal 1. Introduction The linear properties of Bessel light beams (BLBs) have been studied in fair detail by now * Corresponding author. Tel.: +375-17-2841751; fax: +37517-2840879. E-mail addresses: terry.king@man.ac.uk (T.A. King), wh@ nat.vu.nl (W. Hogervorst), tol@dragon.bas-net.by (N.S. Kazak, A.A. Ryzhevich), nkhilo@optoinform.bas-net.by (N.A. Khilo). 1 Tel.: +44-1612754181; fax: +44-1612755509. 2 Tel.: +31-20-4447947; fax: +31-20-4447899. 3 Tel.: +375-17-2841751; fax: +375-17-2840879. 4 Tel.: +375-17-2637735. (see, for example, Refs. [1±5]). The main properties of BLBs stem from the conical structure of their spatial spectrum. The result of mutual interference of plane-wave components of BLB is its multi-ring spatial structure. The total number of BLB rings is usually large. The consequence of this is the fact that the divergence of an individual ring inside a beam is much smaller than the divergence of the whole beam. This property is referred to as diffractionless propagation of the BLB and is pronounced in the central zone of the beam at fairly large lengths and at BLB excitation by a collimated Gaussian-type beam. 0030-4018/01/$ - see front matter Ó 2001 Published by Elsevier Science B.V. PII: S 0 0 3 0 - 4 0 1 8 ( 0 0 ) 0 1 1 2 4 - X 408 T.A. King et al. / Optics Communications 187 (2001) 407±414 The ``nondiverging'' optical beams are of interest for alignment and guiding of atoms. For this purpose, both zero-order and higher-order BLBs can be used [6±9]. Besides, higher-order BLBs Laguerre±Gaussian beams are of interest for studying the processes of creation and annihilation of wavefront dislocations [10±13]. The study and application of BLBs call for effective methods of their obtaining. At present, the main method of obtaining zero-order BLBs is based on the use of an axicon [2,14±16]. This method is simple and permits to convert Gaussiantype beams with an eciency close to 100%. To obtain higher-order BLBs, a holographic technique is used now [7,17,18]. Bessel beams of arbitrary order can also be produced by illuminating an axicon with an appropriate Laguerre±Gaussian mode [9]. In this paper the holographic technique is used also to transform a Gaussian beam into a higher order Laguerre±Gaussian beam. The holographic technique is simple and a 40% eciency can be typically obtained. From the physical point of view, in the holographic method a transfer of dislocation of the transmission function from a spatially inhomogeneous hologram to the light ®eld is realized. An alternative physical principle is used in the method of obtaining ®elds with wavefront dislocation based on the use of media with dislocation of optical properties depending on the direction of light propagation. An example of such media is biaxial crystal. They feature dislocation of the polarization of normal modes at light propagation in the vicinity of binormals. Below we show theoretically and experimentally that ®rst-order and higher-order BLBs can be obtained with use of biaxial crystals. formed at internal conical refraction and BLB having a conical structure of the spectrum of spatial frequencies. The presence of such a relationship would permit obtaining higher-order BLBs by passing laser radiation through a homogeneous crystal. It is known that in the vicinity of binormal, the section of wave vectors surface represents two coaxial coni (Fig. 1). The geometrical parameters of the coni are such that the wave vectors kp of two normal modes propagating at a small angle with binormal are equal kp q kx e1 ky e2 k ÿ bkx ÿ pbq ÿ q2 =2ke3 ; 1 where q kx2 ky2 1=2 , 1=2 ÿ1 b arctgc2 eÿ1 3 ÿ e2 ÿ1 =2v2 is the parameter of crystal an eÿ1 2 ÿ e1 isotropy, k x=v, v is the phase velocity of waves in the direction of binormals, e1;2;3 are the principal values of the permittivity tensor. Indices p 1 enumerate the slow and the fast modes, and e1 , e2 , e3 are the unit vectors of the Cartesian coordinate system with the z-axis parallel to the binormal (Fig. 1). The polarization of normal waves in the vicinity of the binormal is linear, and depending on an azimuth angle u arctg ky =kx [20]. As the azimuth angle is changed by the value of u, the polarization vectors of the normal waves cp p 1 rotate by angle u=2 (Fig. 2). These polarization vectors can be expressed in the form 2. Theoretical model It is known that when the light wave propagates in the vicinity of binormals, the eect of internal conical refraction shows up (see, for example, Ref. [19]) that is the incident ®eld forms a cone of directions of the energy ¯ow inside a crystal. On the basis of this, a theoretical model may be proposed, in which there is a relationship between the ®elds Fig. 1. Cross-section of the wave vector surface in the vicinity of the binormal by the crystallographic plane XZ. a is anisotropy parameter and indices p 1 enumerate a slow and a fast mode. T.A. King et al. / Optics Communications 187 (2001) 407±414 409 Fig. 2. Azimuth dependence of the polarization of the fast and slow eigenmodes in the vicinity of the biaxial crystal binormal. c1 u sin u=2e1 cos u=2e2 ; cÿ1 u cos u=2e1 ÿ sin u=2e2 2 or in an alternative form in terms of vectors of the rightpand left circular polarization e e1 ie2 = 2: ÿi c1 u p e exp iu=2 ÿ eÿ exp ÿiu=2; 2 1 cÿ1 u p e exp iu=2 eÿ exp ÿiu=2: 2 3 Normally, the eect of internal conical refraction is considered for the case of linear polarization of the incident light (see, for example, Refs. [21,22]). It should be noted that due to the azimuth dependence of the polarization direction of normal waves inside the crystal the transmitted radiation has, accordingly, the azimuthally inhomogeneous intensity distribution. Therefore, in order to solve the problem of formation of azimuthally homogeneous beams, it is necessary to use circularly polarized input radiation. Speci®cally, we shall assume that the incident ®eld has, for example, right-hand circular polarization with an amplitude at the input face of the crystal equal to a0 q; u a0 e fin q; u: 4 To ®nd the refracted waves, we represent the incident ®eld polarization vector in the form of a linear superposition of eigenvectors (2) as follows: X ap ucp u 5 e p p with eigenvalues a1 u p i exp ÿiu=2= 2 and aÿ1 u exp ÿiu=2= 2. Then the Fourier spectrum of the ®eld (4) just before the crystal can be given in the form X 6 A0 q; u a0 Fin q; uap ucp u; p where Fin q; u Z Z fin q; u exp iqq cos u ÿ u1 q dq du1 7 is the Fourier spectrum of the function fin q; u. In a particular case of the azimuth-independent input ®eld, Z 8 Fin q 2p fin qJ0 qqq dq; where J0 qq is the zero-order Bessel function. When passing over the crystal boundary, each Fourier component (6) experiences re¯ection depending on the quantity q. This dependence can be neglected for paraxial beams. For such beams the Fourier components of the ®eld inside the crystal, near its boundary, are described by expression (6). Consequently, the ®eld in the crystal is Z Z a0 X F q; u1 ; zap u1 cp u1 a q; u; z 2p2 p exp iqq cos u ÿ u1 ÿ ipbqzq dq du1 ; 9 where 410 T.A. King et al. / Optics Communications 187 (2001) 407±414 F q; u1 ; z Fin q; u1 exp ÿiq2 z=2k; q 2 q x ÿ bz y 2 : Let the input ®eld be azimuthally symmetric. Then, substituting the polarization vectors from Eq. (3) into Eq. (9), integrating with respect to u1 and summing over p, we obtain Z a0 a q; u; z F q; z 2p J0 qqe cos bqz ÿ J1 qq exp ÿiueÿ sin bqzq dq: 10 Now let us assume that the input ®eld is lefthand circularly polarized. In this case, in expan u sion (5) the p eigenvalues are equal to a1p ÿi exp iu=2= 2 and aÿ1 u exp iu=2= 2. A calculation similar to the previous one gives Z a0 F q; z a q; u; z 2p J0 qqeÿ cos bqz ÿ J1 qq exp iue sin bqzq dq: 11 As follows from Eqs. (10) and (11), the circularly polarized wave excites in the biaxial crystal the superposition of two waves with orthogonal polarizations one of which contains wavefront dislocation. Let us consider the particular case of incidence of a zero-order BLB on the crystal. Then fin q J0 qin q. Neglecting the in¯uence of the ®nite transverse extension of the Bessel beam on its Fourier spectrum we obtain Fin q 2pd q ÿ qin = qin , where d x is the delta function. Integrating Eqs. (10) and (11) we ®nd the ®eld amplitudes at the output face of a crystal of thickness L: the de®nition of F q; u; z after Eq. (9), which is immaterial for calculating the intensity pattern, is omitted. Thus, the output ®eld is the superposition of the zero-order and the ®rst-order BLBs with orthogonal polarizations. The amplitude ratio of these beams depends on the distance covered in the crystal by the simple harmonic law. When the condition bqin L 2n 1p=2; where n 0; 1; . . . is ful®lled, the term in Eqs. (12) and (13) proportional to the Bessel function J0 qin q becomes zero. Consequently, complete conversion of the circularly polarized zero-order Bessel beam into the ®rst-order Bessel beam with orthogonal polarization will take place. Estimation of the oscillation period L0 p=2bqin at b 0:016 (KTP crystal), qin 2pcin =k, k 0:63 lm, cin 0:02 gives L0 0:5 mm. It is important to note that the process of increasing the Bessel function order can be continued. To do this, it is necessary to extract from output ®eld Eqs. (12) and (13) the ®rst-order Bessel beam and realize its repeated passage through the crystal. In the general case of incidence on the crystal of a Bessel beam of order m with the phase factor exp imu, integrating Eq. (7), we ®nd m Fin q; u 2p i exp imud q ÿ qin =qin : for the right-hand polarized incident beam, and a q; u; L a0 J0 qin q cos bqin Leÿ 15 Substitution of Eq. (15) into Eq. (9) leads to formulas generalizing Eqs. (12) and (13): a q; u; L a q; u; L a0 J0 qin q cos bqin Le ÿ J1 qin q exp ÿ iu sin bqin Leÿ 12 14 a0 Jm qin q cos bqin Le 2p Jmÿ1 qin q expi m ÿ 1u sin bqin Leÿ ; 16 a q; u; L a0 Jm qin q cos bqin Leÿ 2p ÿ Jm1 qin q expi m 1u sin bqin Le : 17 ÿ J1 qin q exp iu sin bqin Le 13 for the left-hand polarized one. In Eqs. (12) and (13) the phase factor exp ÿq2in z=2k inferred from Formulas (12), (13), (16), (17) describing the eect of BLB order transformation hold for paraxial BLBs within the applicability limits of the original relation (1). In the case of a KTP crystal, BLBs T.A. King et al. / Optics Communications 187 (2001) 407±414 with a cone angle not exceeding 10° can be adequately described by formulas (16) and (17). Thus, theoretical analysis indicates the possibility of formation in biaxial crystals of light beams with screw dislocations and, in particular, of higher-order BLBs. 3. Experimental results and discussion The eect of transformation of the order of a BLB was tested experimentally. The experimental setup shown in Fig. 3. A collimated, circularly polarized Gaussian beam of a He±Ne laser had a waist size of 2.5 mm and was transformed into a zero-order BLB using an axicon with an internal angle of 2:2° and refractive index of 1.5. Consequently, the cone angle cin qin =k0 of the zeroorder BLB was about cin 1:1°. This Bessel beam had illuminated a 12 mm thick KTP crystal oriented perpendicularly to the binormal and located at a distance of 16 cm from the axicon. The radius of the BLB formed by the axicon, within the limits of the crystal position, was about 1.5 mm. In the output ®eld, the right and left circularly polarized components were separated and investigated independently. The intensity distribution in their cross-section was measured and compared to squared zero- and ®rst-order Bessel functions in accordance with Eq. (12). Fig. 4(a) and (b) show the images of the central part of the beams crosssections beyond the polarizer±analyzer. Fig. 5(a) and (b) give the corresponding intensity distributions in comparison with the squared Bessel functions J02 ck0 q and J12 ck0 q. It is clear that 411 good quantitative agreement between theoretical and experimental data is obtained. In addition to these radial distributions of intensity, an important attribute of ®rst-order BLBs is their wavefront dislocation. To display this, an interference of the BLB with plane and spherical reference waves has been studied. The numerically calculated interference pictures are shown in Fig. 6. It is visible that in the case of interference with a plane reference wave, a characteristic indication of dislocation is the bifurcation of the maximum at the center of the BLB and in case of interference with a spherical wave ± a spiral structure (see, also Ref. [23]). The above properties have been observed in experimental interference patterns. Images of these patterns are given in Fig. 7(a) and (b) for plane and spherical reference waves respectively. Note that the direction of spiralling as well as the orientation of the bifurcated maximum reverse when we change the sign of input beam circular polarization. After crystal 6 the output ®rst- and zero-order Bessel beams by virtue of the small cone angle and relatively small longitudinal dimensions of the crystal, exist practically in the same region in which the zero-order initial beam would exist if the crystal was removed from the system. This region approximately corresponds to the ®gure formed by rotating the shaded rhomb (if the refraction in the crystal is ignored) and has ®nite dimensions (see Fig. 3). The maximum distance from axicon 5, on which the ®rst-order output BLB still exists, zmax Rd =cin where Rd is the radius of the diaphragm opening limiting the Gaussian beam illuminating the axicon. The intensity distributions Fig. 3. Optical system for transformation of the order of the Bessel beam: 1 ± 20 telescope; 2 ± polarizer; 3 and 7 ± quarter-wave plates, 4 ± diaphragm, 5 ± axicon; 6 ± KTP crystal; 8 ± polarizer±analyzer; 9 ± microscope; 10 ± recording system; 11 ± additional axicon. 412 T.A. King et al. / Optics Communications 187 (2001) 407±414 Fig. 5. Experimental intensity distribution (curve 1) of the output ®eld with polarization (a) equal to the input one and (b) orthogonal to it as compared to design-theoretical zero- and ®rst-order Bessel beam intensity distributions (curve 2). Fig. 4. Images of the ®eld beyond the polarizer±analyzer for radiation with circular polarization (a) coinciding with the input one (zero-order BLB) and (b) orthogonal to it (®rst-order BLB). and interference patterns given by us correspond to one of the cross-section of this region. However, in all the cross-sections of the above region, after the polarizer±analyzer 8 the intensity distribution is analogous to that given in the ®gure. At distance from axicon 5 larger then zmax ®rst-order BLB is transformed into a ring ®eld which preserves, nevertheless, the azimuthal phase modulation inherent in the ®rst-order BLB. Using an additional axicon 11, this ring ®eld can be transformed into a ®rst-order BLB again. We also checked the theoretical result of Section 2, indicating the possibility of stepwise increase of the order of Bessel function under repeated passage of light through a crystal. For this purpose we used an experimental set-up with two crystals in series. In the ®rst stage a zero-order BLB, incident on the KTP crystal, is transformed into a ®rst-order BLB. Next, the ®rst-order beam polarization is converted from left-circular to right-circular polarization and the beam is directed T.A. King et al. / Optics Communications 187 (2001) 407±414 413 Fig. 7. Images generated by interference of a ®rst-order Bessel beam (a) with a reference plane wave and (b) with a reference spherical wave. Fig. 6. Distribution of interference maxima, calculated for the case of interference of the ®eld exp iu with (a) a plane wave and (b) a spherical wave. towards the second biaxial crystal a-HIO3 (iodic acid) along the direction of its optical axis. According to Eq. (16) the output ®eld then involves a superposition of ®rst- and second-order BLBs. Fig. 8 shows the radial intensity distribution of the output ®eld component with polarization orthogonal to the input polarization. It is seen that this distribution is reasonably well approximated by the squared second-order Bessel function. When incident on the crystal is Gaussian beam instead of Bessel one, it can be transformed into a Laguerre±Gaussian mode LG01 where radial index is 0 and azimuthal index is 1. Then we generated a ®rst-order BLB by illuminating an axicon with this mode with total eciency of about 60%. It can be concluded that the eect of transformation of Bessel beams when propagating along the biaxial crystal binormal as expressed by Eqs. (12) and (16) is con®rmed experimentally. 414 T.A. King et al. / Optics Communications 187 (2001) 407±414 biaxial crystals permits to transform several light beams simultaneously. Acknowledgements Financial support from INTAS (INTAS-BELARUS 97-0533) is gratefully acknowledged. References Fig. 8. Experimental intensity distribution (curve 1) of the output ®eld behind the second crystal with polarization orthogonal to the input ®eld polarization as compared to designtheoretical second-order Bessel beam intensity distribution (curve 2). 4. Conclusions In this work an optical eect of transformation of transversal structure of light ®eld propagating along a binormal of biaxial crystal is investigated theoretically and experimentally. It is shown that circularly polarized input beam excites two circularly polarized beams in the crystal. The beam polarized orthogonally to the input beam has a screw wavefront dislocation if the input beam had no dislocation. When the input beam contains a dislocation of order m, the above mentioned beam has a dislocation of m 1 or m ÿ 1 order. The physical essence of such wavefront transformation is a transfer of singularity of optical properties of biaxial crystal in the vicinity of its binormal to the light ®eld wavefront. 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