1 1 2 3 4 5 6 7 8 9 10 11 12 13 14 15 16 17 18 19 20 21 22 23 24 25 26 27 28 29 30 31 Interactions of North African dust with tropical and subtropical Atlantic coupled oceanatmosphere processes Michael J. DeFlorio1, Dillon J. Amaya2, Arthur J. Miller2, Balwinder Singh3, Steven J. Ghan3, Lynn M. Russell2 1 2 = Jet Propulsion Laboratory, California Institute of Technology, Pasadena CA = University of California-San Diego, Scripps Institution of Oceanography, La Jolla CA 3 = Pacific Northwest National Laboratory, Richland WA Corresponding author: Michael J. DeFlorio, Jet Propulsion Laboratory, MS 300-330, 4800 Oak Grove Drive, Pasadena CA 91109 2 32 ABSTRACT 33 34 Recent work has suggested that North African dust variability over the tropical 35 and subtropical North Atlantic can account for a large fraction of decadal changes in 36 SST anomalies. The response of monthly SST anomalies to dust outbreaks on 37 interannual and decadal timescales is characterized by comparing two Community 38 Earth System Model (CESM) simulations with and without interannual variability of 39 dust. These comparisons show an increase in SST variance in the interactive 40 (interannual dust variability allowed) run over the tropical and subtropical North 41 Atlantic, suggesting that fluctuations of North African dust can drive regional changes 42 in SST variability. The leading mode of coupled SST/wind variability in the tropical 43 Atlantic (the Atlantic Meridional Mode (AMM)) is examined. Although the observed 44 SST spatial pattern associated with the AMM appears as an out-of-phase cross- 45 hemispheric dipole pattern, latent heat flux coupling to the surface horizontal wind 46 only occurs in the Northern Hemisphere. In addition, strong cross-equatorial wind flow 47 normally associated with an interhemispheric SST gradient is present in the CESM 48 interactive simulation, but absent in the prescribed simulation. These results indicate 49 that modeled interannual dust variations influence deep tropical WES dynamics. Strong 50 positive anomalies of summertime dust burden over the subtropical North Atlantic are 51 associated with strong negative values of the coupled SST MCA principal components, 52 indicating that interannual variability of North African dust changes the spatial loading 53 of summertime SST associated with the AMM. 54 55 3 56 1. Introduction 57 58 The variability of Atlantic basin sea surface temperature (SST) has substantial 59 impacts on regional and global climate change, and therefore on human life and 60 property. Long term fluctuations in North Atlantic SST can perturb the near-surface 61 atmosphere, altering the associated surface air temperature and shifting storm tracks 62 and precipitation patterns across Europe and the Mediterranean (Buchan et al., 2014; 63 Cattiaux et al., 2011; Sutton and Hodson, 2005; Trigo et al., 2002; Rogers, 1997; 64 Hurrell, 1995). These SST-related changes in regional climate have spawned deadly 65 heat waves (Cassou et al., 2005) and cold winters (Buchan et al., 2014) across Europe. 66 Increases in tropical North Atlantic SST, along with reductions in vertical wind shear, 67 are directly tied to increases in tropical cyclone frequency (e.g. Goldenberg et al., 68 2001) and Sahel rainfall (e.g. Folland et al., 1986), especially on multidecadal 69 timescales (Booth et al., 2012; Mohino et al., 2011; Wang et al., 2012; Zhang and 70 Delworth, 2006; Giannini et al., 2003). Both local and remote economic conditions are 71 greatly affected by the relationship between Atlantic SST variability and these 72 resulting climate patterns. 73 74 Interannual Atlantic SST observations show both natural and remotely forced 75 components. For example, both central and eastern Pacific El Niños have been shown to 76 significantly impact tropical Atlantic SST (Enfield and Mayer, 1997; Amaya and Foltz, 77 2014). On decadal and multidecadal timescales, Atlantic SST has been thought to be 78 mainly impacted by natural variability of both ocean dynamics and near-surface layer 79 atmospheric circulation (Enfield et al., 2001; Kushnir, 1994; Schlesinger and 4 80 Ramankutty, 1994; Cayan, 1992), while external or remote forcing has been shown not 81 to project strongly onto the observed SST anomaly patterns on these timescales (Ting et 82 al., 2009). However, many of the models used to identify physical mechanisms 83 associated with the observed Atlantic SST variability did not include external forcings 84 such as atmospheric aerosols, which a plethora of studies have identified as important 85 modulators of atmospheric circulation and mixed layer ocean characteristics (Allen et 86 al., 2012; Evan et al., 2009; Zhu et al., 2007). Indeed, studies that have sought to 87 explain Atlantic SST variability using climate models with a greater number of relevant 88 physical processes (e.g. interactive aerosol variability with meteorology and 89 microphysics) have suggested that aerosols can explain up to 76% of simulated decadal 90 and multidecadal Atlantic SST variability (e.g. Booth et al., 2012). 91 One region within the Atlantic basin where aerosols are omnipresent is over the 92 tropical and subtropical North Atlantic basin, where large quantities of mineral dust are 93 advected from the North African continent year-round (e.g., Prospero et al., 1970). 94 Because of its effectiveness as both a scatterer and absorber of solar radiation, dust has 95 been shown to impact both sea surface temperature and cloud fraction due to direct and 96 semi-direct radiative effects (DeFlorio et al., 2014; Doherty and Evan, 2014; Evan et al., 97 2009). Booth et al. (2012) showed that aerosol-cloud microphysical interactions, which 98 were omitted from previous modeling studies, dominated the spatial pattern of aerosol 99 forcing on North Atlantic SST variability during the 20th century. The Community Earth System Model (CESM), which is included in the Coupled 100 101 Model Intercomparison Project Phase 5 (CMIP5), contains state-of-the-art 102 parameterizations for aerosols which allow species such as dust to interact with 5 103 modeled meteorology and cloud microphysics. This is one of the models used in studies 104 such as Booth et al. (2012). Aerosol-cloud microphysics interactions were absent in 105 CMIP3 models, and in many of the model studies used previously to analyze Atlantic 106 basin SST variability on decadal timescales. The inclusion of these interactions, along 107 with better aerosol parameterizations relevant to aerosol-radiation interactions, provides 108 a unique opportunity for utilization of CESM (and other CMIP5 models that include 109 these aerosol processes) to investigate the relationship between North African dust 110 outbreaks and tropical Atlantic SST. 111 In addition to the Atlantic Multidecadal Oscillation (AMO) (Schlesinger and 112 Ramankutty, 1994), the Atlantic Meridional Mode (AMM) is a tropical Atlantic cross- 113 hemispheric variation of SST that varies on interannual and decadal timescales (though 114 the AMM can intermittently destruct on monthly timescales), and is the dominant 115 source of coupled ocean-atmosphere variability in this region (Vimont and Kossin, 116 2007; Chiang and Vimont, 2004). In particular, the AMM can play a large role in 117 modulating the seasonal march of the Intertropical Convergence Zone (ITCZ), 118 significantly impacting Northeastern Brazil rainfall and the associated agricultural 119 communities that rely on it (Foltz et al., 2012; Xie and Carton, 2004). Additionally, the 120 AMM has been shown to impact tropical cyclone development (Vimont and Kossin, 121 2007). 122 It has been suggested that dust-forced variability of SST in the tropics is of 123 comparable magnitude to the observed variability (Evan et al., 2012). Therefore, it is 124 important to discern whether interannual- and decadal-scale dust outbreaks can 125 modulate AMM activity, as shown in an idealized modeling framework in Evan et al. 6 126 (2011). In this study, we seek to clarify the role of North African dust outbreaks in 127 exciting the AMM on these timescales by comparing two CESM simulations: one with 128 interactive aerosols which are free to interact with modeled meteorology and vary on 129 interannual and decadal timescales, and one with a prescribed seasonal cycle of aerosol 130 concentration and no interannual and decadal variability. 131 132 2. Model description and data used 133 134 Two model simulations are compared in this study. Both are CESM 1.0.3 150- 135 year pre-industrial control simulations run at a horizontal resolution of 2.5 longitude 136 (lon) x 1.9 latitude (lat). The only difference in the configuration of the two 137 simulations is that one contains fully interactive dust concentration (free to vary 138 interannual and decadally), while the other prescribes the seasonal cycle of dust 139 concentration using the climatology of the interactive run, such that there is no 140 interannual or decadal variability of dust in the model. For more information regarding 141 these specific simulations, see DeFlorio et al., 2016, DeFlorio et al., 2014, Hurrell et al., 142 2013, Liu et al., 2012, and Zender et al., 2003. 143 For model evaluation, we use monthly mean skin temperature (TS), 10-meter 144 horizontal winds, and the net surface latent heat flux from the National Centers for 145 Environmental Prediction-National Center for Atmospheric Research (NCEP-NCAR) 146 Reanalysis (Kalnay et al., 1996) from January 1948 to December 2014. The skin 147 temperature was chosen to be consistent with model outputs and because it has the 7 148 added benefit over low-level surface air temperature in that it is exactly the SST over 149 ocean grid points. 150 All fields have been linearly detrended at each grid point and we apply a 3- 151 month running mean to the data used in all figures except Figures 8 and 9. We also 152 linearly regress out the influence of the El Niño Southern Oscillation (ENSO), since we 153 are not interested in the influence of tropical Pacific SST on tropical Atlantic SST 154 variability. We follow Chiang and Vimont (2004) and define ENSO using the cold 155 tongue index (CTI) over the domain 6S to 6N, 180W to 90W. Monthly anomalies in 156 observations are relative to the climatology 1980-2010; the model anomalies are 157 computed from a long-term monthly mean climatology which includes all months. 158 159 3. Dust and tropical Atlantic TS interannual variability 160 161 The time evolution of dust burden over West Africa (central Mauritania; 10W, 162 20N) for both the interactive and prescribed CESM simulations is shown in Figure 1. 163 There is clearly interannual and lower frequency variability in the interactive 164 simulation, while we have allowed no interannual or lower frequency variability in the 165 prescribed simulation. 166 Dust burden peaks in magnitude during boreal summer between 5N and 20N 167 over the North Atlantic in CESM (see Figure 6 of DeFlorio et al. (2014)). The 168 variability of July TS monthly anomalies in observations and both CESM simulations is 169 shown in Figure 2. Standard deviation levels in observations and the interactive CESM 170 simulation are substantially higher over the climatologically high dust burden regions 8 171 than in the prescribed CESM simulation. This suggests that interannual-decadal 172 variability of North African dust can drive changes in tropical Atlantic TS. A 173 probability density function (PDF) of TS anomalies during the top 5% “dustiest” 174 months in the interactive CESM simulation reveals that 64% of these high-dust months 175 are concurrent with negative TS anomalies over the tropical North Atlantic downstream 176 of North Africa (40W to 20W, 10N to 20N). This, coupled with the negatively 177 skewed PDF towards cooler TS anomalies, reinforces the notion that increased 178 dustiness can cool TS through radiative effects (Figure 3). 179 The leading and second modes of tropical Atlantic TS variability and their 180 associated temporal evolution are shown in Figures 4 and 5. The leading mode of 181 variability is the Atlantic Niño (Xie and Carton, 2004). We are most interested in the 182 second mode of variability (Figure 5), which displays a spatial structure and interannual 183 to decadal variation over time that is reminiscent of the AMM. Consistent with other 184 CMIP5 models summarized in Flato et al. (2013), the AMM is too weak in magnitude 185 in both interactive and prescribed CESM (middle, bottom panels), especially in the 186 northern hemisphere, though the spatial structure agrees reasonably well with 187 observations (top panel). 188 189 4. Representation of the Atlantic Meridional Mode in CESM 190 191 Though the cross-equatorial dipole pattern associated with the AMM can be 192 seen as the second EOF mode of tropical Atlantic TS anomalies (Figure 5), an 193 alternative approach is to define the AMM as the leading mode of coupled variability 9 194 between horizontal surface winds and TS anomalies (Chiang and Vimont, 2004). This 195 definition encompasses the cross-equatorial wind flow associated with shifts in the 196 position of the ITCZ that are thought to externally force the TS anomalies associated 197 with the AMM pattern through WES feedback processes (e.g., Nobre and Shukla, 1996; 198 Xie et al., 1993a,b). 199 We investigate this inquiry by using Maximum Covariance Analysis (MCA) 200 (Bretherton et al., 1992) on tropical Atlantic horizontal surface wind and temperature 201 anomalies to calculate the AMM in observations (Figure 6, top row). The MCA 202 technique is analogous to Empirical Orthogonal Function (EOF) analysis, but instead 203 requires a singular value decomposition of the cross-covariance matrix of horizontal 204 surface wind and TS anomalies. The resulting left and right singular vectors are then 205 projected onto the original data fields to obtain spatial structure and temporal evolution 206 of TS and winds. 207 The TS and wind spatial structures in the northern hemisphere are reasonably 208 simulated in the leading CESM MCA modes, but the out-of-phase cross-hemispheric 209 TS gradient is not captured. In observations and both CESM simulations, the second 210 mode of coupled variability (not shown) is distinctly reminiscent of the Atlantic Niño 211 (Zebiak, 1993). The correlation coefficients (i.e. the coupling strength) between the 212 leading TS and wind principal components (PCs) for NCEP, CESM interactive, and 213 CESM prescribed are 0.70, 0.49, and 0.48, respectively. 214 The erroneous spatial structure of the southern hemisphere coupled TS and 215 wind field MCA in CESM may be related to the well-known tropical Atlantic SST 216 biases in CMIP5 models discussed in Toniazzo and Woolnough (2013). This bias is 10 217 present in our CESM simulations as well (not shown) and could potentially affect the 218 representation of the Wind-Evaporation-SST (WES) feedback in this region, which is 219 thought to be an important element of sustaining the AMM in reality. This lack of 220 realism is emphasized by the much weaker correlation coefficient between the leading 221 TS and wind PCs in CESM interactive (0.49) and CESM prescribed (0.48) compared to 222 observations (0.70). Such a low coupling strength for the CESM simulations implies 223 that the leading mode of TS and surface winds may not be the most useful technique to 224 characterize model AMM variability. Therefore, we explore auxiliary methods to 225 capture model TS and wind coupled variability in the following sections. 226 227 5. Coupled variability of horizontal winds and latent heat flux 228 229 An important coupled ocean-atmosphere heat budget term which links SST and 230 horizontal surface winds is latent heat flux (Cayan, 1992). Indeed, it has been shown 231 that the WES feedback in the tropics manifests itself through latent heat flux anomalies 232 forced by the horizontal surface winds (e.g. Xie et al., 1993a,b). 233 MCA analysis of the leading mode of surface wind and latent heat flux 234 anomalies is shown in Figure 7. The convention for the latent heat flux is such that a 235 negative anomaly corresponds to the atmosphere losing heat to the ocean. The 236 correlation coefficients between the leading latent heat flux and wind principal 237 components for NCEP, CESM interactive, and CESM prescribed are 0.71, 0.84, and 238 0.80, respectively. 11 239 It is clear from the observed leading spatial pattern (Figure 7, top left) that latent 240 heat flux and wind coupling is much stronger in the northern hemisphere than in the 241 southern hemisphere. Strong southwesterly wind anomalies override a basin-scale swath 242 of negative latent heat flux anomalies from 15N-30N. This is consistent with a 243 weakening of the climatological trade winds, which leads to a reduction in evaporation 244 at the surface and flux of latent heat energy from the atmosphere into the ocean 245 (negative latent heat flux anomalies). Therefore, the negative latent heat flux anomalies 246 seen in Figure 7 are consistent with a warm phase AMM (Figure 6, top panel). 247 The leading spatial patterns of latent heat flux and winds in CESM interactive 248 and prescribed (Figure 7, middle left and bottom left, respectively) are very realistic and 249 similar to each other in the northern hemisphere. However, the interactive simulation 250 contains a cross-equatorial wind pattern and the classic C-shaped turn of the winds that 251 we normally associate with interhemispheric SST gradients and the AMM. This is 252 comparable to the observed leading latent heat flux and wind MCA, which displays a 253 similar, albeit weaker, cross-equatorial flow and C-shape turn of the winds (top row, 254 Figure 7). On the other hand, the prescribed simulation does not have this cross- 255 equatorial flow (bottom row, Figure 7). This suggests that interannual variability of dust 256 can modulate the magnitude of latent heat flux and wind coupling near region of the 257 AMM. Understanding why the interactive simulation produces a much stronger cross- 258 equatorial flow is beyond the scope of this study and should be the focus of future 259 modeling efforts. 260 12 261 262 6. Can summertime North African dust storms excite the AMM on interannual timescales? 263 264 Though we have shown that interannual variations in North African dust can 265 project onto subtropical North Atlantic TS variability, it remains unclear whether dust 266 can influence the spatial structure and magnitude of the coupled Atlantic Meridional 267 Mode, which has been suggested in idealized modeling studies by Evan et al. (2011) 268 and others. Climatological dust burden is highest during June and July over the 269 subtropical North Atlantic (DeFlorio et al., 2014 and others). Therefore, we repeat the 270 MCA calculation shown in Figure 6, but limit the analysis to only July months. We also 271 limit our MCA analysis to north of the equator in an effort to isolate the TS-wind 272 coupled variability most strongly associated with North African dust variations and to 273 limit the influence of the equatorial and South Atlantic regions on the leading modes. 274 The “July months only” MCA analysis for TS and horizontal winds reveals that 275 interannual variability of dust has a significant impact on the TS spatial loading in the 276 tropical North Atlantic (Figure 8). The correlation coefficients between the leading TS 277 and wind principal components (PCs) for NCEP, CESM interactive, and CESM 278 prescribed are 0.61, 0.66, and 0.81, respectively. The magnitude of this spatial pattern is 279 higher in the CESM simulation with interannually varying dust by a factor of two 280 compared to CESM prescribed (Figure 8, middle and bottom row). Indeed, the TS 281 principal components from the TS/wind MCA analysis are negatively correlated with 282 subtropical North Atlantic dust burden in CESM interactive during both June and July 283 (Figure 9). 13 284 However, the observed horizontal wind pattern is poorly simulated in both the 285 CESM interactive and prescribed simulations during July (Figure 8, wind vectors). In 286 particular, strong equatorial horizontal divergence normally associated with the Atlantic 287 Niño appears in both CESM leading modes, but is absent in observations. The 288 meridional component of the horizontal winds over the subtropics is also too weak in 289 the CESM simulations. This is a physical shortcoming of the coupled SST and wind 290 fields in CESM which may explain why the AMM is too weakly represented in CESM 291 (Figures 5-6). 292 In spite of this, the stark difference in the magnitude of TS MCA spatial loading 293 patterns between CESM interactive, which closely matches observations, and CESM 294 prescribed, which is roughly two times weaker than observations, provides evidence 295 that interannual variability of North African dust not only projects strongly onto 296 tropical-subtropical North Atlantic TS variability, but onto the TS spatial structure of 297 the coupled Atlantic Meridional Mode. 298 299 7. Summary and discussion 300 301 We use observations and two coupled climate model simulations (with and 302 without interannual variability of dust concentration) to examine the interaction 303 between North African dust fluctuations and interannual variability of tropical Atlantic 304 SST and coupled SST/wind processes. 305 Our CESM interactive aerosol simulation provides clear evidence that increased 306 dustiness over the tropical North Atlantic decreases co-located SST and increases year- 14 307 to-year SST variance, especially during boreal summer. The probability distribution of 308 SST is negatively skewed on the dustiest months over the subtropical North Atlantic; 309 indeed, 64% of the dustiest months are concurrent with negative surface temperature 310 anomalies in this region. 311 Though the Atlantic Meridional Mode is weaker in both CESM simulations than 312 in observations, analyses confined to boreal summer and the northern hemisphere 313 (when/where dust loading is high over the subtropical North Atlantic) reveal that 314 interannual variability of North African dust projects strongly onto the SST spatial 315 structure in the Northern Hemisphere associated with the AMM. This builds on 316 previous idealized modeling studies (e.g. Evan et al. (2011)) which also found that 317 interannual variability of dust could excite the AMM. 318 Latent heat flux and surface wind coupling is only an important forcing term for 319 the observed AMM in the northern hemisphere (Figure 7). There is no clear signal in 320 the southern hemisphere of this coupling, which could be due to the fact that the 321 southern hemisphere lobe of the AMM is thought to be independent of the northern 322 hemisphere lobe and can act on different timescales (e.g., Mehta and Delworth, 1995; 323 Enfield et al., 1999). Therefore, the southern hemisphere coupled interactions between 324 latent heat flux and surface wind could be found in a higher order MCA mode not 325 presented in this study. 326 It is also shown that modeled interannual variability of North African dust can 327 modulate the magnitude of latent heat flux and surface wind coupling over the tropical 328 Atlantic. Indeed, this coupling is much weaker throughout the tropical Atlantic in the 329 prescribed CESM simulation with no interannual variability of dust concentration, 15 330 especially in the equatorial and southern hemisphere regions (Figure 7). Although it 331 remains unclear whether this enhanced latent heat flux and wind coupling alone can 332 substantially influence the SST spatial structure and magnitude of the AMM in CESM 333 as defined by the SST/wind coupling, the interactive CESM simulation’s ability to 334 reproduce a strong cross-equatorial flow that is typically associated with 335 interhemispheric SST gradients is an indication that interannual dust variations 336 influence deep tropical WES dynamics. 337 The AMM and other coupled ocean-atmosphere processes in this region are of 338 vital socioeconomic interest because of their well-documented impacts on surrounding 339 precipitation and tropical cyclogenesis. Consequently, we feel it is critical that future 340 modeling efforts build on the results shown here and focus on understanding and 341 ultimately reducing the strong CMIP5 bias in tropical Atlantic SSTs such that a more 342 realistic representation of coupled ocean atmosphere processes in this region may be 343 obtained. Such efforts could allow for a better representation of the AMM in climate 344 models, and can help better constrain the role of dust forcing in exciting and/or 345 sustaining the AMM. 346 347 8. Acknowledgments 348 349 This research was partly carried out at the Jet Propulsion Laboratory, California 350 Institute of Technology, under a contract with the National Aeronautics and Space 351 Administration. Funding for this study was provided by NSF AGS-1048995 and OCE- 352 1419306 and NOAA NA14OAR4310276. 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Res., 112, D16208. 21 FIGURE CAPTION LIST 560 561 562 563 Figure 1: Dust burden (kg/m2) over central Mauritania (West Africa) in CESM 564 interactive aerosol (top) and prescribed aerosol (bottom) simulations for 50 (left) and 10 565 (right) year subsets of the 150-year simulation. 566 567 Figure 2: Standard deviation of detrended July tropical Atlantic TS monthly anomalies 568 in NCEP/NCAR (top), interactive CESM (middle), and prescribed CESM (bottom). 569 570 Figure 3: Probability density function of monthly TS anomalies in interactive CESM 571 over the tropical-subtropical North Atlantic (40W to 20W, 10N to 20N), on the top 572 5% dustiest months. 64% of the dustiest months are concurrent with negative surface 573 temperature anomalies in this region. 574 575 Figure 4: Leading EOF and associated PC of tropical Atlantic TS monthly anomalies in 576 NCEP/NCAR (top), interactive CESM (middle), and prescribed CESM (bottom). The 577 percentage variance of the total signal explained by each mode is indicated in 578 parentheses. Note the different x-axes for the observed and model PCs. 579 580 Figure 5: as in Figure 4, but for second EOF. Note the different x-axes for the observed 581 and model PCs. 582 583 Figure 6: Leading maximum covariance analysis (MCA) heterogeneous mode and 584 associated temporal evolution of coupled TS (K) and wind (m/s) variability in NCEP 22 585 (top row), CESM interactive (middle row), and CESM prescribed (bottom row). The 586 percentage covariance of the total signal explained by each mode is indicated in 587 parentheses. Note the different x-axes for the observed and model PCs. 588 589 Figure 7: Leading maximum covariance analysis (MCA) heterogeneous mode and 590 associated temporal evolution of coupled latent heat flux (W/m2) and wind (m/s) 591 variability in NCEP (top row), CESM interactive (middle row), and CESM prescribed 592 (bottom row). The percentage covariance of the total signal explained by each mode is 593 indicated in parentheses. Note the different x-axes for the observed and model PCs. 594 595 Figure 8: Leading “July months only” maximum covariance analysis (MCA) 596 heterogeneous mode and associated temporal evolution of coupled TS (K) and wind 597 (m/s) variability in NCEP (top row), CESM interactive (middle row), and CESM 598 prescribed (bottom row). The percentage covariance of the total signal explained by 599 each mode is indicated in parentheses. Note the different x-axes for the observed and 600 model PCs. 601 602 Figure 9: Scatterplots of vertically integrated subtropical North Atlantic dust burden 603 anomalies (40W to 20W, 10N to 20N) and MCA surface temperature (left column) 604 and horizontal wind (right column) principal components during June (top row) and 605 July (bottom row). 23 606 607 Figure 1: Dust burden (kg/m2) over central Mauritania (West Africa) in CESM 608 interactive aerosol (top) and prescribed aerosol (bottom) simulations for 50 (left) and 10 609 (right) year subsets of the 150-year simulation. 610 611 24 612 613 Figure 2: Standard deviation of detrended July tropical Atlantic TS monthly anomalies 614 in NCEP/NCAR (top), interactive CESM (middle), and prescribed CESM (bottom). 25 615 616 617 Figure 3: Probability density function of monthly TS anomalies in interactive CESM 618 over the tropical-subtropical North Atlantic (40W to 20W, 10N to 20N), on the top 619 5% dustiest months. 64% of the dustiest months are concurrent with negative surface 620 temperature anomalies in this region. 621 622 26 623 624 Figure 4: Leading EOF and associated PC of tropical Atlantic TS monthly anomalies in 625 NCEP/NCAR (top), interactive CESM (middle), and prescribed CESM (bottom). The 626 percentage variance of the total signal explained by each mode is indicated in 627 parentheses. Note the different x-axes for the observed and model PCs. 628 27 629 630 Figure 5: as in Figure 4, but for second EOF. Note the different x-axes for the observed 631 and model PCs. 632 633 634 635 28 636 637 638 Figure 6: Leading maximum covariance analysis (MCA) heterogeneous mode and 639 associated temporal evolution of coupled TS (K) and wind (m/s) variability in NCEP 640 (top row), CESM interactive (middle row), and CESM prescribed (bottom row). The 641 percentage covariance of the total signal explained by each mode is indicated in 642 parentheses. Note the different x-axes for the observed and model PCs. 29 Figure 7: Leading maximum covariance analysis (MCA) heterogeneous mode and associated temporal evolution of coupled latent heat flux (W/m2) and wind (m/s) variability in NCEP (top row), CESM interactive (middle row), and CESM prescribed (bottom row). The percentage covariance of the total signal explained by each mode is indicated in parentheses. Note the different x-axes for the observed and model PCs. 30 Figure 8: Leading “July months only” maximum covariance analysis (MCA) heterogeneous mode and associated temporal evolution of coupled TS (K) and wind (m/s) variability in NCEP (top row), CESM interactive (middle row), and CESM prescribed (bottom row). The percentage covariance of the total signal explained by each mode is indicated in parentheses. Note the different x-axes for the observed and model PCs. 31 Figure 9: Scatterplots of vertically integrated subtropical North Atlantic dust burden anomalies (40W to 20W, 10N to 20N) and MCA surface temperature (left column) and horizontal wind (right column) principal components during June (top row) and July (bottom row).