Femtosecond Fiber Lasers Based on Dissipative Processes F. W. Wise Department of Applied Physics Cornell University Tuesday, August 2, 2011 Femtosecond fiber lasers… Andy Chong Will Renninger Khanh Kieu Simon Lefrancois Hannah Liu Brandon Bale Edwin Ding Nathan Kutz Tuesday, August 2, 2011 Dissipative solitons… Introduction to nonlinear pulse propagation, short-pulse generation Femtosecond lasers without anomalous dispersion Dissipative solitons Implications for useful devices --------------------------------------------------------------------- Self-similar pulse evolution in a laser Tuesday, August 2, 2011 Disclaimers Lack of mathematical rigor Meaning/use of “soliton” Tuesday, August 2, 2011 Introduction to ultrafast science Tuesday, August 2, 2011 Ultrashort light pulses For λ = 1000 nm, 1 cycle = 3.3 fs Tuesday, August 2, 2011 Why use ultrashort light pulses? “Strobe light” to observe ultrafast processes Tuesday, August 2, 2011 Why use ultrashort light pulses? “Strobe light” to observe ultrafast processes Produce high E field with modest energy/average power nonlinear microscopies Tuesday, August 2, 2011 Why use ultrashort light pulses? “Strobe light” to observe ultrafast processes Produce high E field with modest energy/average power nonlinear microscopies Precision control of (nonlinear) energy deposition material processing (absorbing and transparent) Tuesday, August 2, 2011 Applications of femtosecond lasers Ultrafast phenomena Precision material processing Thin film characterization Terahertz generation and detection Nonlinear microscopy High-field physics Inertial confinement fusion Attosecond science Surgery Tuesday, August 2, 2011 Applications of femtosecond lasers Ultrafast phenomena Tuesday, August 2, 2011 Applications of femtosecond lasers Precision material processing Tuesday, August 2, 2011 Femtosecond lasers Ti:sapphire laser + power + stability + 700 nm < λ < 1000 nm - $120k - >100 W electrical input - water cooling - large size Tuesday, August 2, 2011 Motivations Tuesday, August 2, 2011 Motivations Study a new class of nonlinear waves Reach the performance of solid-state lasers, but with practical benefits of fiber Can we take femtosecond lasers out of labs and into factories, clinics, …? Tuesday, August 2, 2011 Introduction to short-pulse generation Tuesday, August 2, 2011 Laser gain Tuesday, August 2, 2011 Laser oscillator gain Tuesday, August 2, 2011 Laser gain Tuesday, August 2, 2011 Laser gain Tuesday, August 2, 2011 Fiber laser gain Tuesday, August 2, 2011 Fiber laser gain Tuesday, August 2, 2011 Fiber laser gain Advantages waveguide medium not sensitive to alignment perfect beam high efficiency; reduced thermal effects high power (1,000 W cw) telecom infrastructure Tuesday, August 2, 2011 Fiber laser gain Challenge: nonlinear effects ~ intensity x length energy x length/area IL (waveguide) ≈ 10 3 − 10 7 IL (homogeneous) Tuesday, August 2, 2011 Saturable absorber T SA I SA • molecules • semiconductors • nonlinear polarization evolution (NPE) Tuesday, August 2, 2011 Saturable-absorber modelocking gain SA • Shorter pulse experiences less loss • Amplitude modulation directly shapes pulse • Good for picosecond pulses animation by Carsten Krogh Nielsen Tuesday, August 2, 2011 Saturable-absorber modelocking gain SA • Shorter pulse experiences less loss • Amplitude modulation directly shapes pulse • Good for picosecond pulses animation by Carsten Krogh Nielsen Tuesday, August 2, 2011 Terminology “Modelocking” frequency-domain view of short-pulse generation inside lasers Tuesday, August 2, 2011 Shorter pulses: dispersion matters n = n(ω) v(ω) = c/n(ω) animation by Carsten Krogh Nielsen Tuesday, August 2, 2011 Shorter pulses: dispersion matters n = n(ω) v(ω) = c/n(ω) animation by Carsten Krogh Nielsen Tuesday, August 2, 2011 Shorter pulses: dispersion matters Tuesday, August 2, 2011 • LDS (1 ps, glass) ~ 10 m • LDS (100 fs, glass) ~ 10 cm • LDS (10 fs, glass) ~ 1 mm Shorter pulses: dispersion matters Tuesday, August 2, 2011 • LDS (1 ps, glass) ~ 10 m • LDS (100 fs, glass) ~ 10 cm • LDS (10 fs, glass) ~ 1 mm Dispersive phase accumulation t φ t normal group-velocity dispersion Tuesday, August 2, 2011 Dispersive phase accumulation t t φ t anomalous group-velocity dispersion Tuesday, August 2, 2011 Dispersion control Anomalous dispersion from • Fiber material or waveguide structure • Prism pairs • Grating pairs • Chirped mirrors normal dispersion pulse duration chirp Tuesday, August 2, 2011 anomalous position Nonlinear phase accumulation n = n0 + n2 I Tuesday, August 2, 2011 Nonlinear phase accumulation n = n0 + n2 I Re χ(3) € Tuesday, August 2, 2011 P = χ(1) E + χ(2) EE + χ(3) EEE + ... Nonlinear phase accumulation I n (t) = n0 + n2 I(t) t Tuesday, August 2, 2011 Nonlinear phase accumulation I n (t) = n0 + n2 I(t) t n t Tuesday, August 2, 2011 Nonlinear phase accumulation I n (t) = n0 + n2 I(t) t n t φ φNL φ(t) ~ n(t) phase varies across pulse t ω ω ~ - dφ/dt Tuesday, August 2, 2011 t Nonlinear Schrodinger Equation E (z, t) = A(z, t) e i( kz −ωt ) ∂A(z, t) β (2) ∂2 A(z, t) 2 +i = in | A(z, t) | A(z, t) € 2 2 ∂z 2 ∂t dispersion nonlinear refraction • Tuesday, August 2, 2011 Launched pulse generally decays Soliton formation ∂A(z, t) β (2) ∂2 A(z, t) 2 +i = in | A(z, t) | A(z, t) 2 2 ∂z 2 ∂t dispersion Δφ Δφ nonlinearity t (anomalous) dispersion cancels nonlinearity for A(t) = A0 sech(t / τ p )exp(iz / z sol ) Tuesday, August 2, 2011 t Soliton laser gain saturable absorber anomalous dispersion β2 < 0 self-focusing nonlinearity n2 > 0 Tuesday, August 2, 2011 Theoretical modeling of short-pulse lasers Nonlinear Schrodinger Equation GVD Kerr Nonlinearity E (z, t) = A(z, t) e i( kz −ωt ) € Tuesday, August 2, 2011 Theoretical modeling of short-pulse lasers Net Gain Tuesday, August 2, 2011 Cubic SA Term Spectral Filter Theoretical modeling of modelocked lasers Cubic Ginzburg-Landau Equation (CGLE) • Assumes homogeneous medium • Static solutions • Some coefficients depend on solutions Tuesday, August 2, 2011 Numerical modeling Vector model accounts for both polarizations 2 ∂ A x iβ 2 ∂ 2 A x 2 iγ * 2 − 2iΔβz 2 + = iγ A x + A y A x + A x A y e 2 ∂z 2 ∂t 3 3 2 ∂ 2 iβ 2 A y 2 iγ * 2 2iΔβz 2 + = iγ A y + A x A y + A y A x e 2 ∂z 2 ∂t 3 3 ∂ Ay Δβ = 2π Tuesday, August 2, 2011 LB Static pulse solutions NLSE CGLE • Stability? Tuesday, August 2, 2011 Static pulse solutions NLSE CGLE • Stability? Tuesday, August 2, 2011 Static pulse solutions NLSE CGLE • Stability? Tuesday, August 2, 2011 Static pulse solutions NLSE CGLE • Stability? Tuesday, August 2, 2011 Numerical modeling Solve with appropriate terms in each segment of oscillator Periodic boundary condition Launch noise, look for pulsed solutions Tuesday, August 2, 2011 Making a pulse Starting dynamics • saturable absorber allows pulse to build up from noise Steady state • pulse feels average (anomalous) cavity dispersion • phase modulations determine steady-state pulse Examples • soliton fiber lasers • femtosecond Ti:sapphire lasers Tuesday, August 2, 2011 Soliton lasers Quantitative differences between solid-state and fiber Tuesday, August 2, 2011 Femtosecond lasers Soliton-like pulse-shaping + passive modelocking - limited energy € - Eτ ∝ β2 n2 → requires anomalous dispersion materials have normal dispersion for λ < 1.3 µm Tuesday, August 2, 2011 Femtosecond lasers Solitons - limited energy => limited impact of fiber oscillators Tuesday, August 2, 2011 Femtosecond lasers Anomalous dispersion is required with • normal linear dispersion • self-focusing nonlinearity (n2 > 0) “All femtosecond lasers include anomalous dispersion.” Tuesday, August 2, 2011 Can we make a femtosecond laser without soliton formation? Tuesday, August 2, 2011 Can we make a femtosecond laser without anomalous dispersion? Tuesday, August 2, 2011 Pulse shaping at normal dispersion t Tuesday, August 2, 2011 I(t) ~ I(ω) in chirped pulse Spectral filter acts as saturable absorber Gain dispersion provides a filter t All-Normal-Dispersion Laser Output Spectral filter SMF ~3 m Tuesday, August 2, 2011 Saturable Absorber Gain fiber ~20 cm SMF ~1 m ANDi Laser Output Spectral filter SMF ~3 m Tuesday, August 2, 2011 Saturable Absorber Gain fiber ~20 cm SMF ~1 m Simulation: temporal evolution Tuesday, August 2, 2011 Highly-chirped pulse throughout cavity Weak temporal breathing Simulation: temporal evolution Tuesday, August 2, 2011 Highly-chirped pulse throughout cavity Weak temporal breathing Filter dominates pulse-shaping Output SMF ~3 m Saturable Absorber Gain fiber ~20 cm Intensity Wavelength Tuesday, August 2, 2011 Wavelength SMF ~1 m Intensity Wavelength Spectral filter Intensity Intensity Simulation: spectral evolution Wavelength Analytic theory Why should a partial differential equation work? • • No dispersion map Weak temporal breathing CGLE fails • • • • • stability of solutions multiple solutions with identical energy spectral shapes existence of maximum pulse energy “area theorem” qualitatively wrong Tuesday, August 2, 2011 Ginzburg-Landau Equations (NLSE) Tuesday, August 2, 2011 Ginzburg-Landau Equations (NLSE) (CGLE) Tuesday, August 2, 2011 Ginzburg-Landau Equations (NLSE) (CGLE) (CQGLE) Tuesday, August 2, 2011 Ginzburg-Landau Equations (NLSE) (CGLE) (CQGLE) Quintic SA Term Tuesday, August 2, 2011 Ginzburg-Landau Equations (NLSE) (CGLE) (CQGLE) Quintic SA Term T I Tuesday, August 2, 2011 Known pulse solutions NLSE CGLE CQGLE Tuesday, August 2, 2011 Known pulse solution CQGLE Tuesday, August 2, 2011 Theoretical pulses Tuesday, August 2, 2011 Theoretical pulses δ>0 B=1 δ<0 Tuesday, August 2, 2011 Theoretical pulses δ>0 B=1 δ<0 theoretically unstable Tuesday, August 2, 2011 Dissipative solitons CQGLE Static solutions balance dispersion nonlinear phase gain, loss saturable absorption spectral filtering Solutions not realized previously in a physical system Tuesday, August 2, 2011 Dissipative solitons CQGLE Tuesday, August 2, 2011 Dissipative solitons CQGLE Tuesday, August 2, 2011 Dissipative solitons CQGLE Tuesday, August 2, 2011 Dissipative solitons Tuesday, August 2, 2011 Dissipative solitons Much theory, little experiment Tuesday, August 2, 2011 Dissipative solitons Much theory, little experiment N. Akhmediev and A. Ankiewicz Dissipative Solitons (Springer, Berlin Heidelberg, 2005) Ultanir et al., Phys. Rev. Lett. 90, 253903 (2003) Bakonyi et al., J. Opt. Soc. Am. B 19, 487 (2002) Tuesday, August 2, 2011 Experiments output QWP collimator birefringent plate isolator QWP collimator PBS HWP SMF SMF WDM Yb-doped fiber 980nm pump Fixed parameters fiber nonlinearity (γ) fiber dispersion (D) Tuesday, August 2, 2011 Variable parameters birefringent plate varies Ω waveplates vary α, δ pump power varies B Experimental setup ANDi laser Tuesday, August 2, 2011 Comparison to analytic theory Theory Tuesday, August 2, 2011 Comparison to analytic theory Theory Tuesday, August 2, 2011 Comparison to analytic theory Theory Experiment Renninger et al., Phys Rev A 2008 Tuesday, August 2, 2011 Comparison to analytic theory Theory Experiment Renninger et al., Phys Rev A 2008 Tuesday, August 2, 2011 Comparison to numerical simulations Experiment Numerical simulation Chong et al., JOSA B 2008 Tuesday, August 2, 2011 How do dissipative solitons form? Tuesday, August 2, 2011 Amplitude balance Dispersion broadens pulse Spectral filtering shortens the pulse filter Tuesday, August 2, 2011 Phase balance dispersive phase φ(z+Δz) φ(z) Δφ t t • Normal dispersion balances self-focusing nonlinearity Tuesday, August 2, 2011 Overall balance NLSE conservative soliton anomalous GVD amplitude (sech) phase Tuesday, August 2, 2011 Overall balance spectral filter dissipative soliton saturable absorber nonlinear phase amplitude (chirped pulse) NLSE conservative soliton normal GVD anomalous GVD (sech) phase Tuesday, August 2, 2011 Comparison to simulations Tuesday, August 2, 2011 High-performance femtosecond lasers Tuesday, August 2, 2011 High pulse energies pulse evolution maximum pulse energy in ordinary fiber soliton 0.1 nJ ΦNL ~ 0 dispersion-managed soliton 1 nJ ΦNL < π/2 solid-state lasers (Ti:sapphire) 10 nJ dissipative soliton 40 nJ so far Tuesday, August 2, 2011 ΦNL ~ 20π Dissipative soliton laser with double-clad fiber output filter DC Yb-doped fiber pump Tuesday, August 2, 2011 Average power > 1 W • • • Tuesday, August 2, 2011 80 fs / 30 nJ / 2 W after dechirping 200 kW peak power performance comparable to Ti:sapphire Kieu et al., Opt Lett 2009 2-photon fluorescence imaging (with C. Schaffer) • • YFP labels pyramidal neurons Texas Red labels vasculature • 0-200 µm: dendrites, surface vessels • 400-600 µm: cell bodies, capillaries • 700-900 µm: cell bodies, axons Tuesday, August 2, 2011 Toward all-fiber instruments Tuesday, August 2, 2011 All-fiber dissipative soliton lasers • 130 fs / 3 nJ / 150 mW Kieu et al., Opt Express 2008 Zhao et al. , unpublished Tuesday, August 2, 2011 All-fiber laser Tuesday, August 2, 2011 Self-similar evolution in gain fiber: amplifier similaritons Tuesday, August 2, 2011 Self-similar pulse propagation Monotonic chirp avoids wave-breaking (Anderson et al., JOSA B 1993) Wave-breaking-free solutions of NLSE with normal dispersion asymptotic solutions exist a(t,z) = a0 (z) 1− (t / τ (z)) 2 exp(ib(z)t 2 ) parabolic intensity profile, linear chirp € Tuesday, August 2, 2011 Self-similar pulse evolution passive fiber Anderson et al. (1993) (theory) amplifier fiber Fermann, Kruglov et al. (2000) (expt, theory) z z I(t,z) I(t,z) Tuesday, August 2, 2011 t Pulse evolves self-similarly -- “similariton” t Amplifier similaritons n2 > 0 normal dispersion gain asymptotic solution Fermann, Kruglov et al, Phys. Rev. Lett. 2000 Tuesday, August 2, 2011 Amplifier similaritons n2 > 0 normal dispersion gain nonlinear attractor Fermann, Kruglov et al, Phys. Rev. Lett. 2000 Tuesday, August 2, 2011 Amplifier similariton laser Can we stabilize an amplifier similariton in an oscillator? amplifier ? Tuesday, August 2, 2011 Amplifier similariton laser Can we stabilize an amplifier similariton in an oscillator? amplifier ? Answer in 2002: No. Spectral breathing will be uncontrollable. Tuesday, August 2, 2011 Amplifier similariton laser Hypothesis: a spectral filter alone can stabilize an amplifier similariton fiber laser. amplifier narrow spectral filter Tuesday, August 2, 2011 Simulations gain fiber Tuesday, August 2, 2011 sat abs filter Simulations evolution narrow filter (2 nm) stabilizes an amplifier similariton with feedback Tuesday, August 2, 2011 output pulse Simulations filter gain fiber pulse evolves to parabolic self-similar solution in the amplifier Tuesday, August 2, 2011 Experimental setup all-normal-dispersion Yb fiber laser with NPE grating filters provide narrow bandwidths (<4 nm) Tuesday, August 2, 2011 Experimental results theory Tuesday, August 2, 2011 output 2 output 1 output 2: approximates pulse at end of gain output 1: beam splitter output Features of amplifier similariton narrowband filter allows pulse to reach self-similar solution contrast with dissipative solitons large (10-20x) spectral breathing smooth, broad spectra local nonlinear attractor in cavity suppress fluctuations? Ilday et al., Nat Photon 2010 Renninger et al., Phys Rev A 2010 Harvey et al., Opt Express 2010 Tuesday, August 2, 2011 amplifier High energy and short pulses 40 fs / 10 nJ output 250 kW peak power Much broader bandwidths can be generated Nie, Dantus, Wise Opt Express 2011 Tuesday, August 2, 2011 Summary and outlook (Temporal) dissipative solitons new nonlinear waves chirping and filtering Tuesday, August 2, 2011 Regimes of propagation soliton anomalous GVD phase modulations Tuesday, August 2, 2011 ANDi normal GVD dissipative processes Summary and outlook (Temporal) dissipative solitons new nonlinear waves chirping and filtering Major performance advantages 10-100x energy of prior fs fiber lasers Competitive with solid-state lasers Tuesday, August 2, 2011 Summary and outlook (Temporal) dissipative solitons new nonlinear waves chirping and filtering Major performance advantages 10-100x energy of prior fs fiber lasers Competitive with solid-state lasers What is the maximum pulse energy? What is the minimum pulse duration? Tuesday, August 2, 2011 Summary and outlook (Temporal) dissipative solitons new nonlinear waves chirping and filtering Major performance advantages 10-100x energy of prior fs fiber lasers Competitive with solid-state lasers What is the maximum pulse energy? What is the minimum pulse duration? Self-similar evolution in gain segment Strong spectral breathing Benefits of local attractor? Tuesday, August 2, 2011 Summary and outlook (Temporal) dissipative solitons new nonlinear waves chirping and filtering Major performance advantages 10-100x energy of prior fs fiber lasers Competitive with solid-state lasers What is the maximum pulse energy? What is the minimum pulse duration? Self-similar evolution in gain segment Strong spectral breathing Benefits of local attractor? Simple, inexpensive construction Tuesday, August 2, 2011 Acknowledgements Tuesday, August 2, 2011 Tuesday, August 2, 2011 Laser gain Tuesday, August 2, 2011 Laser gain Tuesday, August 2, 2011 Modes of a cavity Tuesday, August 2, 2011 Modes of a cavity Tuesday, August 2, 2011 Modes of a cavity Tuesday, August 2, 2011 Modes with random phases Intensity Time Tuesday, August 2, 2011 Modes with phases locked to same value Intensity Time Tuesday, August 2, 2011 Modelocked Intensity Time Tuesday, August 2, 2011 Analytic approach to pulse evolution Variational principle yields coupled equations for parameters of solution in homogeneous segments Fixed-point analysis yields stable node Filter creates strong evolution about fixed point Bale, Kutz et al., Opt Lett 2008 Tuesday, August 2, 2011 Scaling to large mode area PCF with 40-micron core Theory: stable to 300 nJ Experiment: limited by pump • 100 nJ / 115 fs • 1 MW peak power • 8 W average power Lefrancois et al., Opt Lett 2010 (also Lecaplain et al., Baumgartl et al.) Tuesday, August 2, 2011 What about stability? δ>0 B=1 δ<0 theoretically unstable Tuesday, August 2, 2011 What about stability? δ>0 B=1 δ<0 experimentally stable Tuesday, August 2, 2011 What about stability? δ>0 B=1 δ<0 stabilized by gain saturation? Tuesday, August 2, 2011 Reduced pulse structure • Output after filter chirped 1.4 ps Tuesday, August 2, 2011 dechirped 75 fs