MANAGEMENT OF FROM COMMERCIAL RADIOACTIVE NUCLEAR VIRGIL 163 E, WASTES POWER JONES PLANTS MANAGEMENT OF RADIOACTIVE WASTES FROM COMMERCIAL NUCLEAR POWER PLANTS Submitted to: Professor Frank Ski H e r n for: Problems in Environmental by: Virgil E. Jones 5-4-79 Law MANAGEMENT OF RADIOACTIVE WASTES FROM COMMERCIAL NUCLEAR POWER PLANTS Nuclear Energy! These two words possess an inherent capacity for stimulating emotional responses. Few p e o p l e , when asked to comment on their feelings regarding the use of nuclear energy for commercial power g e n e r a t i o n , remain noncommittal. Most will align themselves with one of the diametrically opposing views of its virtues or its dangers. During the past three deca-des the development of our advanced nuclear technology has produced a legacy of radioactive waste materials which will retain the potential to affect future generations for thousands of y e a r s . At no time in man's previous history has he possessed a capability to affect the future as he does today. The outcomes of those decisions which are made and the directions taken during the remainder of this century regarding the use of nuclear energy will influence energy policy in the forthcoming centuries. With society having access to such a God-like p o w e r , it is difficult to comprehend the public's general naivety this country's entire nuclear program. concerning E v i d e n t l y , people find themselves overwhelmed by a f o r c e , trapped within an atom which is too small to s e e , but which has such awesome power that it can be used to destroy a city or to light its s t r e e t s , to kill outright or to locate cavities in one's teeth, or to either cause the development of cancers or to destroy them. Until the recent wave of s k e p t i c i s m , the attitude of individuals has been one of trusting 165 2 w i t h o u t question to scientists and engineers w h a t they themselves could not understand. With the emergence of organized groups who question the various aspects of our nuclear p r o g r a m s , public awareness and understanding of nuclear energy has greatly improved. This is especially true with regard to the use of nuclear energy for the production of electricity. As the public has become more know- ledgeable of this issue, its attitudes have shifted. This shift can be seen when reviewing the results of public opinion polls which dealt with issues related" to nuclear power plants. A summary (1) of an analysis of such polls conducted between 1960 and 1976 points out that in 1960 only 6% of those people surveyed had any reservations about the use of nuclear power for generating electricity. Half of those who did oppose its use did so because o f concern about its safety. The remaining opponents gave reasons for their beliefs dealing with either economic r e a s o n s , such as the cost of electricity and the loss of j o b s , or just their satisfaction w i t h the then present system. More recent surveys taken during 1975 and 1976 found an increased percentage of the public (from 19 to 3 5 % , depending on survey) who opposed the use of nuclear p o w e r . When this group was asked to comment on its reasons for o p p o s i t i o n 5 the majority referred to some aspect of the operational of the reactor itself. safety H o w e v e r , national surveys during the same general time frame (1974, 1975) which asked the participant to pick the most serious of a list of known problems associated with nuclear power plants (various safety features as well as the disposal of nuclear w a s t e s ) , approximately 50% picked nuclear w a s t e * 1 t;'Cl 3 disposal as a serious problem. In f a c t , this response occurred twice as often as the next most common response. A similar reaction was obtained in a 1975 survey (2) in which 67% of those questioned felt that the disposal of radioactive wastes was a serious problem. The public is thus shown to recognize the problem of managing radioactive wastes as being a serious one, but evidently the public believes it to be a solvable p r o b l e m , and as such does not think it should stand in the way of the development of commercial nuclear power. Regardless of one's personal convictions on the issue of using nuclear power in commercial generating p l a n t s , it must be realized that from the time the first commercial reactor became operational in 1957, radioactive waste materials from such sources have been accumulating. These wastes must be managed in a manner which will protect the environment from their potentially harmful effects. This paper presents information on the e n v i r o n m e n t a l , t e c h n o l o g i c a l , and legal requirements for the safe management of radioactive waste materials. No attempt will be made to include information dealing directly with those wastes produced by either this country's defense system or any foreign government's. L i k e w i s e , information will be restricted to those radioactive wastes associated with operational systems which are presently in use. }V I 4 j.OJL RADIATION AND ITS BIOLOGICAL EFFECTS To appreciate the problems which are involved with managing radioactive w a s t e s , one must be familiarized with the physical process of r a d i o a c t i v i t y , the materials comprising the w a s t e , and how these factors interact with biological forms. Radiation is an often misunderstood term which conjures up mental images of nuclear w a r , lingering d e a t h , and total destruction. In r e a l i t y , radiation is a physical activity defined (3) as "the process of emitting radiant energy in the form of waves or particles". R a d i a t i o n , t h e r e f o r e , merely dissipates energy from regions of overabundance. Sunlight is the most familiar example of radiant waves or electromagnetic radiation. Without this incoming e n e r g y , life as we know it could not exist on the e a r t h . not all radiation is beneficial. radiant However, Just as too long of an exposure of sensitive skin to full sunlight will cause a " b u r n " , overexposure to other forms of radiation can also produce harmful effects. Radiation given off by radioactive substances consists of alpha and beta particles as well as gamma rays (4). Alpha particles are nothing more than the nuclei of helium atoms (two protons in combination with two n e u t r o n s ) , and as such carry a double positive charge. These particles possess between three and nine MeV — of kinetic e n e r g y , but due to their large size compared to other atomic particles and double charge they are very r e a c t i v e , and thus do riot penetrate deeply into matter before dissipating their energy. A single sheet of newsprint is of sufficient — MeV (million electron volts) is an expression of the quantity of energy possessed, thickness 5 j.OJL to allow only a f e w , if a n y , alpha particles to pass through Beta particles consist of either an emitted electron beta decay) or positron a single charge. it. (negative (positive beta d e c a y ) , and as such carry These particles possess a maximum of only 2.95 MeV of kinetic e n e r g y , but because of their single charge and small size they are less reactive than alpha particles and thus, can penetrate matter to a greater d e p t h . Gamma rays are electromag- netic radiation and possess neither mass nor charge. They are the least reactive of the radioactive decay particles a n d , t h e r e f o r e , the most penetrating. One must now apply this rudimentary knowledge of the forms in which radiant energy may be encountered in assessing its potential effects to biological systems. The first prerequisite in doing this is to realize that life on this planet has and will continue to be bombarded with a continual incidence of background radiation from three principle sources (5). The first of these comes from cosmic s o u r c e s , primarily in the form of cosmic rays and their derivatives. The quantity of radiation obtained from this source is directly proportional to one's location on the earth with regard to altitude and latitude. Since the atmosphere absorbs a high percentage of the cosmic rays which intercept the earth and the earth's magnetic field deflects such r a d i a t i o n , a much lower quantity of radiation reaches the earth's surface near the equator at sea level than at either higher altitudes or latitudes. Naturally occurring radionuclides comprise the second source of background radiation. Radiation from these natural sources has remained relatively stable through t i m e , and as life forms have 6 evolved they have adapted to this normal occurrence of radiation and can cope with its effects. The third source contributing to our present background radiation levels is man m a d e . testing of nuclear devices has Atmospheric released large quantities of radioactive materials into the environment. Although such fallout is distributed w o r l d - w i d e by atmospheric m o v e m e n t s , it tends to concentrate in areas where precipitation intercepted the initial radioactive c l o u d , or along the windward side of high mountain ranges. These man-made contaminants are present in sufficient concentrations in the mountains of Colorado so that the altitude, at which an animal once lived can be established by determining the quantity of fallout materials concentrated in its organs. Other man-made radiation sources include X-ray m a c h i n e s , color T V ' s , nuclear r e a c t o r s , and other common items in our society. level of background radiation is increased by man's As the activities, the assurance that biological systems can continue to overcome its effects is lessened. When an organism is exposed to r a d i a t i o n , those particles and waves which penetrate its being dissipate their energy in one of two w a y s . or excited. Individual atoms of the organism are either ionized Excitation refers to the process whereby an electron is moved from its normal orbit to an orbit at a higher energy l e v e l . In a biological s e n s e , ionization is by far a more important process since it involves the removal of one or more orbital electrons from an atom and thereby changes the charge which the atom normally p o s s e s s e s . An atom in such a "charged" state may either combine with other atoms in unnatural groupings or disassociate itself from those atoms to which it was a t t a c h e d . ,jt 1 y - i /I* If such 7 a rearrangement occurs in an important e n z y m e , m e m b r a n e , genetic s t r u c t u r e , serious consequences can result. or It is well to r e a l i z e , h o w e v e r , that in the vast majority of cases in which a serious cellular abnormality does o c c u r , the abnormality is lethal to only the single cell involved. Few of the total number of abnormalities which may be produced are ever transmitted forwards in t i m e , but there is little comfort in knowing that most of the cells which could have caused one's affliction died before being able to do so. The density of ionization -along the pathway taken by radiation is important in determining what effects may occur to that organism. As discussed e a r l i e r , alpha particles react readily with matter and h e n c e , dissipate their energy over a very short distance. This tends to "bunch" the ionization which they cause within a small a r e a . Gamma r a y s , on the other h a n d , dissipate their energy over a much greater d i s t a n c e , which enables the ionization they cause to be spread over a much greater a r e a . particles produce ion densities which are intermediate the other density patterns. Beta between If cellular damage from ionization is localized within a tissue or organ and enough damage is d o n e , the function of that tissue or organ may be impaired. On the other e x t r e m e , even a single ionization, if occurring in a genetic structure within an egg or sperm c e l l , could conceivably produce a mutated offspring. Exactly how radiation will affect an organism can never be predicted with complete accuracy. A whole body dosage (6) of from 250-450 rad — (0.5 rad the present maximum allowable annual d o s a g e ) is generally considered to be lethal in m a n . Smaller d o s e s , h o w e v e r , can produce latent effects such as bone d i s o r d e r s , c a t a r a c t s , i n f e r t i l i t y , m u t a t i o n s , and a general decrease in life expectancy. Biological dangers associated with radiation exposure are greatly increased if the subject radionuclei gains entry into the body of the o r g a n i s m . For e x a m p l e , an alpha emitting substance w h o s e radiation when external from the body would not penetrate the numerous layers of skin becomes a strong ionizing force when within the body. This is especially true if incorporated in body tissue where it can constantly bathe the surrounding cells with radiation. N e w , rapidly growing cells are known to be much more sensitive to radiation than mature cells. This principle explains w h y radiation can be used to destroy malignancies in humans but also why radiation is a greater risk to fetuses or young children who have a much higher proportion of y o u n g , rapidly growing cells than do a d u l t s . This is the reason that expectant mothers and young children were asked to temporarily move from the immediate area of the Three Mile Island Reactor near H a r r i s b u r g , P e n n s y l v a n i a , when radioactive gases were being emitted from the damaged reactor. Regardless of cell a g e , some cells have been found to be e s p e c i a l l y sensitive to radiation while others are extremely resistant. L y m p h o c y t e s , s p e r m a t o g o n i a , and erythroblasts 2/ — A unit of absorbed dosage for any ionizing radiation. One rad equals 100 ergs absorbed per gram of any substance. 9 (precursor to red blood cells) of mammals are extremely sensitive to radiation (7). Dosages as low as 5 rad can produce adverse effects in these c e l l s , whereas the single celled organism, Paramecium, can survive dosages of over 300,000 rad (8). Biolo- gists do not know why such discrepancies exist. Probably the most frightening aspect of radiation exposure is the risk of unknown latent effects, A summary of data (9) pertaining to low dosage exposure of humans to radiation exemplifies such latent effects by presenting data showing that children of mothers who received from three to five pelvic x-rays during pregnancy were twice as likely to develop leukemia by age ten as were children of non-x-rayed mothers. Likewise, exposure of a fetus to only 80 mr (.08 rad) in the first trimester doubled the risk of cancer for that child. Associated directly with the nuclear power industry was the reported increase in infant mortality near three boiling water reactors. This increase was felt to be linked with the radioactive waste gases being released into the atmosphere during normal operations of these plants. Other evidence presented suggests a relationship between exposure to low doses of radiation and premature births, an increased incidence of respiratory diseases, and congenital birth defects. In addition to the well-known radiation hazard associated with nuclear waste materials is the extreme toxicity of the transuramic elements (those elements with an atomic number greater than uraniurn—-usually man-made). These heavy m e t a l s , of which the most notorious is plutonium, are more dangerous from a standpoint of toxicity than of radiation. M 1 HH /O Plutonium, as an example, 10 can enter the body via the food w e e a t , the air we b r e a t h e , or by skin absorption. Its dangers were emphasized by T . B. Taylor (10) as follows: On a scale of lethal doses it is at least 20,000 times m o r e toxic than cobra venom or potassium cyanide and 1,000 times more toxic than any modern nerve gas. An individual can safely absorb no more than one tenmillionth of a gram in his l i f e t i m e , and inhaled as dust in a quantity no larger than a p i n h e a d , it is deadly. Within a few days it will cause death from lesions in lung tissue and lesser dosages result in cancer over a longer period of time. Biological responses to radiation a r e , t h e r e f o r e , dependent on 1) the type of radiation emitted (i.e., a l p h a , b e t a , or gamma r a y ) , 2) the type of exposure (i.e., external or internal), 3) the length of e x p o s u r e , 4) the half-life of radionuclides, and 5) the biological effects due to causes other than radiation ( i . e . , toxicity of transuramic elements). WASTES ASSOCIATED WITH NUCLEAR POWER PLANTS Nuclear power plants are similar to conventional thermal plants except that rather than using a fossil fuel they utilize fissionable e l e m e n t s , usually uranium 235 (11) in a controlled chain reaction as a heat source. This chain reaction is continued by the absorption of neutrons by the nuclei of a fissionable element. The resulting "heavy" nuclei are not stable and release the extra energy by either disintegrating into parts plus addi- tional neutrons (fission), or by the less frequent release of gamma rays. As the fission products collide with surrounding m a t t e r , their kinetic energy is transformed into heat. This is the heat that is extracted from the reactor core in the form of hot water. 13 In the ordinary combustion of a fuel s o u r c e , various compounds are produced which can be collectively called waste materials. N u c l e a r chain reactions proceed one step further. Not only do they produce waste compounds; they also create new elements and isotopes of both the common and new elements. of these products are not stable and undergo spontaneous Many radio- active d e c a y , with the rate of decay being unique to each. The rate at which this decay occurs determines the length of time that the substance remains radioactive and h e n c e , the time span over which we must consider its m a n a g e m e n t . Radioactive decay is not a linear function with respect to time. A given period of time is required for one-half of the total number of radionuclei to d e c a y . The same length of time is then required for one-half of the remaining nuclei to d e c a y , and so forth until all have decayed to a stable s t a t e . Half-life is the term used to refer to the time necessary for one-half of the radioactivity of a substance to decay. Typical half-lives associated with nuclear waste materials range from seconds to thousands of y e a r s . Sixteen common radionuclides found in waste materials produced by nuclear power plants are presented as Appendix A with their approximate half-lives. Three basic categories of radioactive waste materials are produced by commercial tions. nuclear power plants during normal opera- These consist of 1) structural m a t e r i a l s , disposable e q u i p m e n t , potentially contaminated protective c l o t h i n g , paper p r o d u c t s , e t c . , 2) radioactive g a s e s , and 3) spent fuel j.OJL assemblies. 12 As the n u c l e a r chain reaction takes place within the core of the r e a c t o r , t h e structural material of the reactor itself and its shielding is bombarded with radiation. Over a reactor's lifespan this b o m b a r d m e n t produces an induced radioactivity in these structural m a t e r i a l s . Pieces of disposable equipment ranging from tools, the p r o t e c t i v e clothing worn by plant p e r s o n n e l , and paper products such as the filters used in the cooling may be c o n t a m i n a t e d . not compromise the systems All of these materials must be managed to environment. Radioactive g a s e s such as T r i t i u m , Iodine, K r y p t o n , and Xenon (12) are e m i t t e d into the atmosphere from nuclear power p l a n t s , with the q u a n t i t y being dependent upon the type of reactor involved. O f the 72 (13) commercial nuclear power plants operating in this c o u n t r y , practically all are light water reactors (LWR). transfer T h i s means that ordinary water is used to heat a w a y from the core of the reactor. The majority of these L W R 1 s are o f the pressurized water type (14) and as such employ a highly p r e s s u r i z e d water system (primary loop) to transfer heat from the c o r e to a secondary water system (secondary from which steam TS generated for use in the turbines. loop) With this type of system the w a t e r in the secondary loop never enters the core of the r e a c t o r . This is unlike the boiling water reactor which has only one water loop in which as the steam is condensed into water it is r e c y c l e d into the core and heated into steam again. Pressure t y p e reactors release a much smaller total amount of radioactive g a s e s into the atmosphere (15) than does the boiling water type. The t w o loop system prevents the w a t e r which is 13 transformed into steam from ever entering the reactor core where radioactive gases and other substances leached from the fuel assemblies are a c c u m u l a t e d . Attempts at removing dissolved gases from the w a t e r in either or both systems are not completely successful and some gases do escape into the a t m o s p h e r e . emissions under normal operations do not exceed limits under federal These established regulations. NUCLEAR WASTE MANAGEMENT Nuclear power plants are designed to have a usable lifespan of from 30 to 40 y e a r s . This being the c a s e , no utility company has as y e t been forced to decommission an entire reactor c o m p l e x . H o w e v e r , a number of the original power plants have either reached or exceeded the halfway point of their expected and will soon have to be decommissioned. lifespans Changes in the regula- tions governing the level of allowable emissions or which reactor designs are acceptable could hasten obsolescence if changes to present equipment cannot be economically m a d e . There is also the possibility that a nuclear power plant can be damaged to such an extent that repair or salvage is impossible. The recent accident involving the Three Mile Island Reactor may well force its permanent closure. If this is the c a s e , Consolidated Edison will be forced to decommission the plant at a time when there are few alternatives for handling radioactive w a s t e s , no experience at d e c o m m i s s i o n i n g , and little or no tested methodology to follow. Regardless of the method used, which presently would j.OJL 14 include only mothballing or e n t o m b m e n t , the task will undoubt- edly be a multi-million dollar venture. The methods presently employed to manage nonstructural materials other than fuel elements consist of either shallow surface burial or on-site s t o r a g e , as is the case of some gases and liquids. Containment lasts until radioactive decay progresses to the point that the materials can be diluted and released into the environment. A g a i n , it is assumed that these diluted quanti- ties of radiation are harmless. By far the most serious waste management problem presently associated with nuclear power plants involves the spent fuel assemblies. These highly radioactive units have to date been stored on site in holding pools after removal from the reactor core. The one exception to this practice involved a limited quan- tity of assemblies which were shipped to a reprocessing plant for recovery of the remaining fissionable m a t e r i a l s , but at present no commercial reprocessing plants are operating within this country. The one plant which was in operation reprocessed 640 metric tons of spent fuel during a six year period (16). This plant was closed in 1972 to allow design modifications to be made and has not been reopened. With the recently published report by the Ford Foundation which recommended that reprocessing and plutonium recycling should be deferred (17), followed shortly by an announcement by President Carter that the United States would refrain from all commercial reprocessing as a means of reducing the risk of nuclear p r o l i f e r a t i o n , it seems unlikely that any commercial reprocessing will be available within the foreseeable future. 15 With n e i t h e r commercial r e p r o c e s s i n g nor a p e r m a n e n t disposal m e t h o d c u r r e n t l y a v a i l a b l e , those utility companies o p e r a t i n g n u c l e a r power plants are faced with the problem of w h a t to do with t h e i r rapidly increasing q u a n t i t y of spent a p p r o x i m a t e l y 1700 M e t r i c Tons o f Uranium (MTU) per y e a r fuel, (18). P r e s e n t options range from m a x i m i z i n g the SDace c u r r e n t l y avail- able to total c u r t a i l m e n t of p l a n t o p e r a t i o n s . latter S i n c e the choice will be c o n s i d e r e d by u t i l i t i e s only as a last r e s o r t , emphasis m u s t be placed on how t e m p o r a r y storage facilities will be u s e d . On J a n u a r y 1 , 1 9 7 7 , 17 n u c l e a r plants did not have enough reserve s t o r a g e a v a i l a b l e to a c c o m m o d a t e a full of the reactor core (19). discharge The n e c e s s i t y of such a d i s c h a r g e w o u l d occur in the event t h a t m a j o r m a i n t e n a n c e or a full safety tion o f the core w a s r e q u i r e d . The m a j o r i t y of these inspec- plants, h o w e v e r , already had taken steps w h i c h w o u l d allow them to regain a full core d i s c h a r g e capacity. By this same date (January 1 , 1 9 7 7 ) , the N u c l e a r Commission Regulatory (NRC) had been notified by utilities operating 36 reactors that they w e r e p l a n n i n g to increase s t o r a g e c a p a c i t y by c o m p a c t i n g their p r e s e n t stores (20). has been q u e s t i o n e d by the National The safety of compacting Resources D e f e n s e Council regarding 1) the risk of u n i n t e n t i o n a l c r i t i c a l i t y , 2) the n e c e s s i t y of using boron panels as neutron a b s o r b e r s and t h e r e b y decreasing the flow rate of c o o l a n t , and 3) the p o s s i b i l i t y of exceeding capacity of p r e s e n t cooling (21) the systems, The NRC had also received numerous requests for licenses p e r m i t the c o n s t r u c t i o n of additional o n - s i t e s t o r a g e j.OJL to facilities. 16 Utilities can also ship spent fuel assemblies from plants with little storage to newer plants which still have an excess of storage space available. This p r o c e s s , called " s h a r i n g " , h o w e v e r , tends to cause all storage facilities to become full at the same time and in the long run may be a more difficult problem to overcome than even periodic closures. A sizable amount of off-site storage could be supplied by using the storage facilities at the nonoperatina General Electric and Exxon reprocessing plants at M o r r i s , I l l i n o i s , and Oak Ridge, T e n n e s s e e , respectively. It has been estimated (22) that the additional 4500 MTU of storage capacity that these facilities would provide would allow a full core reserve for all reactors through 1986. A l s o , if the Energy Research and Development Administration's (ERDA) estimate of 1985 as the date when full scale operation of a national depository is m e t , the problem of on-site storage capacity will be alleviated. h o w e v e r , is probably optimistic This estimate, (23). It is inevitable that any comprehensive waste management plan will require the shipment of spent fuel assemblies from on-site storage facilities to other repositories or disposal sites. T h e s e shipments will have to travel by conventional rail and highway systems. The risks associated with such transportation schemes can be reduced (24) by 1) decreasing the number of shipments (rail shipments can be l a r g e r , hence less frequent), 2) decreasing the distance s h i p p e d , 3) the use of stronger shipping v e s s e l s , 4) the reduced speed of transportation v e h i c l e s , and 5) routing around high density population centers. Of the five pro- posed risk abatement p r o c e d u r e s , the t h i r d , development of stronger 17 shipping v e s s e l s , has received considerable attention. Sandia Laboratories have conducted extensive testing (25, 26) on the ability of specially designed shipping containers to retain their integrity in accident situations. These tests have shown these containers to be able to survive probable accident situations with ease. Upon solving all other management p r o b l e m s , one question remains: How does one assure long term isolation of up to thousands of years for these waste materials? General consensus within the scientific community holds that isolation would best be accomplished by disposing of these materials in s t a b l e , deep geologic f o r m a t i o n s . Of the many such strata that e x i s t , bedded salt formations are looked upon with favor by a majority of scientists (27). The advantages of using salt beds as disposal sites were presented in a 1970 National Academy of Sciences Committee Report as quoted in the environmental impact statement for the now defunct waste repository at L y o n s , Kansas (28). The listed advantages were: 1. A highly radioactive source separated from the environment by a thickness of good-quality bedded salt in an area of tectonic stability is effectively isolated from that environment for at least 1,000 years and probably for significantly longer. 2. Bedded salt has a high compressive strength but flows plastically at relatively low temperatures and pressures. This will relieve stress concentrations produced by the mining operation or by the heat generated by the radioactive w a s t e . j.OJL 3. Fractures that might develop in bedded salt are "self-healing". This is indicated in part by the absence of solution cavities in the rock salt that has been studied. 4. The natural plasticity of the salt at the temperature imposed by the highly radioactive waste will effectively seal the remnants of the containers in cells of crystalline salt. Should m a n , for a now unforeseen r e a s o n , have to remove the buried radioactive w a s t e , it could be accomplished with specialized mining e q u i p m e n t , albeit with considerable difficulty and e f f o r t . 5. Bedded salt permits the dissipation of larger quantities of heat than is possible in other types of rock. 6. Rock salt is approximately equal to concrete for gamma-ray shielding. Experimental radiation exposure has caused very little detectable radiolytic change in rock s a l t . 7. The loss of our salt resources would be negligible. There is a great abundance of bedded salt in the United States (particularly in Kansas) that is of satisfactory quality and in suitable geological environments that can be used for the burial of specified radioactive wastes produced by the nuclear plants that are anticipated in the United States over the next two or three decades. 8. The burial of the radioactive wastes under consideration in deep-bedded salt greatly reduces chances for release by accidental or malicious acts in both the near and distant future. U n f o r t u n a t e l y , until a full scale test of a salt bed disposal system is completed, numerous questions will unanswered. remain To d a t e , such a test has been repeatedly delayed. In the late 1960's, a salt mine in Central Kansas was extensively tested to determine its suitability as a waste depository. Only after the Atomic Energy Commission had announced that the L y o n s , K a n s a s , site had been selected was it discovered that an unknown a r\r*) 19 number of abandoned gas wells penetrated the proposed This i n f o r m a t i o n , coupled with mounting political caused the AEC to abandon this s i t e . formation. opposition, A later try at establishing a depository in Michigan also was cancelled due to political opposition. P r e s e n t efforts are being directed towards surveying potential sites in numerous states and the Waste Isolation Plant (WIPP) near C a r l s b a d , Mew M e x i c o . Pilot WIPP is foreseen as a permanent disposal site for transuramic wastes from the defense program and as a research and development installation studying the effects of radioactive wastes on a salt formation. It has been suggested that WIPP could also function as a test site for the disposal of up to 1,000 spent fuel assemblies tive plans call for mining out chambers into which vessels will be p l a c e d . (29). Tenta- containment The chambers will then be back filled with loose s a l t . Some limited testing of salt's suitability as a repository medium has shown bedded salt to not be as anhydrous as previously thought (30). It is now known that when heat is a p p l i e d , such as would be generated by radioactive d e c a y , moisture trapped within the crystalline structure tends to migrate to the heat source. Any sizable accumulation of moisture would form a brine pocket surrounding the containment vessel and would represent a potential corrosion p r o b l e m . Test drilling at the WIPP site has also located previously unsuspected aas and water reservoirs at some locations in that salt formation. To what extent such factors decrease the suitability of salt as a depository medium is y e t unknown. 20 A growing number of scientists feel that not. enough informa- tion is available on the effects of radioactive wastes on bedded salt to allow accurate predictions of what the consequences of long periods of storage will be. These doubts were expressed in a GAO report (31) which pointed out that the present NRC requirements of from five to ten years for the retrievabi1ity of wastes deposited in test facilities may not be of sufficient length. Other concerns w e r e raised by a team of U. S. Geological Survey scientists (32) about selecting repository s i t e s . included: These 1. the unknown effects that heat will have on the subject strata and water and gases in the strata; 2. the little knowledge about ground water movement through cracks in granite or basalt; and 3. the fact that no one can guarantee future stability. These scientists also suggested five areas in which information was critically needed. These research included: 1. the effects of small amounts of water on s a l t , how this affects its s t r e n g t h , and how to guarantee retrievability from such formations; 2. the necessity for conducting research with other strata such as s h a l e , crystalline r o c k , and zeolitic tuffs; 3. the ways to determine ground water movements at repository sites; 4. the need to improve methods of determining geologic s t a b i l i t y ; and 5. what the short and long term effects of the repository will be on the geologic environment around it. Not all scientists feel that deposition in bedded salt formations is the best or only solution to our nuclear waste problem. j.OJL These scientists have suggested alternative methods such as the use of other bedded f o r m a t i o n s , including g r a n i t e , b a s a l t , s h a l e , etc. Disposal in s p a c e , on the Antarctic ice sheet (33), and in deep sea sediments (34) has also been proposed. Other promising techniques for handling wastes include the use of lasers (35) to separate usable components and actual radioactive materials from the general w a s t e m a s s , thereby reducing the quantity that would have to be managed and the use of linear accelerators to transmute radioactive wastes into stable forms. TERRORIST ACTIVITIES The Irish Republican A r m y , P . L . O . , 15th of September Movement, and the Red Brigade are but a few of the well o r g a n i z e d , well financed terrorist groups operating on a worldwide scale today. There is little doubt that any of these groups or numerous other revolutionary organizations would not rejoice at the opportunity of acquiring a nuclear threat capacity. The possibility of terrorist activities being directed towards the commercial nuclear industry at either the plant or waste management level is one of the most serious dangers associated with nuclear power today. It is almost inconceivable that a serious attempt at nuclear blackmail will riot occur in the near future. The unfortunate aspect of this forecast is that with the present world s i t u a t i o n , the United States is a prime target for attack. R e v o l u t i o n a r i e s , for e x a m p l e , would probably more easily gain the freedom of cohorts jailed in another country having close ties to the United States 22 by threatening New York City or W a s h i n g t o n , D. C. , than cities w i t h i n the other country. Terrorist a c t i v i t i e s , if and when they o c c u r , will probably be directed towards 1) procurring an atomic b o m b , 2) procurring plutonium or other highly toxic radioactive s u b s t a n c e , 3) gaining control of a nuclear facility, or 4) the destruction of said facility. The ultimate of these terrorist activities is undoubtedly the acquisition of a nuclear bomb by gift or direct t h e f t , or by diverting the fissionable materials necessary for building a crude bomb. Only such diversions as might presently occur from the commercial nuclear power industry are within the scope of this p a p e r . The present ban on reprocessing spent fuel has greatly reduced the potential of terrorist groups acquiring the fissionable materials (highly enriched u r a n i u m , uranium 233 or plutonium) necessary for an atomic bomb. These substances are not present in sufficiently high concentrations in the fuel assemblies (either new or spent) of light water reactors so that the fuel itself could be used directly in a b o m b . Expensive reprocessing would be required, which is probably beyond the scope of an unassisted terrorist group. These fuel a s s e m b l i e s , if s t o l e n , would also be difficult to smuggle in or out of a country due to their size. It is logical to assume that terrorists would rather obtain a product such as plutonium which is already refined. A quantity the size of a baseball of this element or of either isotope of uranium (3G) would provide the critical mass necessary for an atomic bomb with a yield of from five to six tons of high e x p l o s i v e s , plus the threat of radiation and contamination. j.OJL 23 The only commercial reactors in use today which are in variance with the above stated facts are several high temperature gas cooled reactors that require a highly enriched uranium fuel (37), H o w e v e r , even this fuel could not be used in a bomb directly because the enriched uranium is dispersed in graphite and as s u c h , would present the same problems of logistics and extraction as fuel from L W R ' s . The logical point at which to attack this system would be at the fuel fabrication plant before the highly enriched uranium is dispersed in the graphite base. If a terrorist group obtained a fissionable mass of plutonium they would not be restricted to using it in a bomb. The mere threat of dispersing such a toxic substance would be sufficient to blackmail most governments. In the event that the threat was carried o u t , or if the plutonium was dispersed as a tactical act, large areas would be made uninhabitable and possibly millions of people would be killed by its direct or latent effects. The third action that a terrorist group might employ would be to secure a nuclear facility. Since most nuclear plants in this country are in populous a r e a s , the demands of a group holding and threatening to destroy such a plant and thereby releasing c o n t a m i n a n t s , would probably be granted. A fourth alternative t h a t a group or even a determined individual could accomplish as a tactical movement would be the unannounced destruction of a nuclear plant or support facility. This could be done by either armed ground a t t a c k , s a b o t a g e , or an aerial attack such as crashing an airplane loaded with explosives into the target. It seems probable that the transportation of commercial nuclear w a s t e s does not present a choice target for terrorist acts due to /"V** 1H / M 24 the materials involved. At best only a localized area would be c o n t a m i n a t e d , and since routing in transporting these wastes will be designed to go through low density a r e a s , only a limited threat is involved. This would also apply to repositories or disposal sites which did not contain any refined or highly concentrated waste m a t e r i a l s . By their very n a t u r e , these facilities will be isolated from major population centers. To entirely dissolve the threat of attack on the commercial nuclear industry is probably impossible. Increased security at key sites (nuclear power p l a n t s , fuel fabricating p l a n t s , etc.) w o u l d be a d e t e r r e n t , but it is doubtful that a sufficiently armed and dedicated group could be repelled. Present security levels have been e n h a n c e d , but as recently as early 1977 a government report (38) chided the NRC for not acting decisively or effectively in the security a r e a . The then present security systems at some nuclear plants would not have reportedly met the threat of even minimum sabotage attempts. A majority of the blame was placed on the N R C 1 s failure to establish minimum requirements for security s y s t e m s . LEGAL ISSUES Little legal precedence has been established regarding the m a n a g e m e n t of nuclear w a s t e m a t e r i a l s . placed the authority for locating 5 Congressional action has constructing, and operating nuclear waste repositories for high level wastes (including fuel assemblies) with DOE subject to NRC regulation. Low level repositories are not currently being managed under a single 1 8 G spent 25 management scheme but one operated by D O E , private c o n c e r n s , and states with NRC approval. The recent DOE Task Force Report on Nuclear Waste Management (39) recommended that all 22 low level waste repositories (18 o p e r a t i o n a l , 4 closed) be placed under DOE ownership and m a n a g e m e n t . to accomplish Legislative procedures were suggested this. Other legislative action that has been proposed is to grant the states the right to veto any proposed nuclear waste repository that is sited within their borders (40). This proposed grant has been suggested as a means of overcoming political opposition and for gaining public support. Senator H a r t , Chairman of the Nuclear Regulations S u b c o m m i t t e e , has suggested a compromise measure whereby the state would receive a qualified right to v o t e , but one which could be overruled by the President for reasons of national interest. Any nuclear w a s t e disposal site will be licensed and operated by federal agencies and as s u c h , leaves no question as to w h e t h e r major federal action is involved. T h i s , coupled with the fact that nuclear waste management undoubtedly has the potential of affecting the human e n v i r o n m e n t , assures by the reasoning in MRDC v. A d m i n i s t r a t o r , ERDA (451 F. S u p p . 1245) that a detailed environmental statement subject to the provisions of the National Environmental Policy Act of 1969 is required. m f -r% 26 APPENDIX A HALF-LIVES OF TYPICAL RADIOACTIVE WASTE COMPONENTS Radionuclide Half-life (years) — Americium-241 460 Americium-242 150 Cesi um-135 Cesium-137 (41) 2 x 106 30 Curium-242 • Curium-243 32 Curium-244 18 Iodine-129 1.6 x 1 0 7 Neptuni um-237 2.1 x 1 0 6 Plutoni um-239 2.4 x 1 0 4 PIutoni um-241 Radon~226 Strontium-90 13 1600 28 Technetium-99 2.0 x 1 0 5 Thori um-230 7.6 x 1 0 4 Tritium 13 — The half-life is the time necessary for half of the radionuclei to d e c a y . 27 FOOTNOTES R a n k i n , W . L. and S . M . N e a l e y , "Attitudes of the Public About Nuclear Wastes," Nuclear N e w s , Vol. 2 1 , No. 8 , PD. 1121 1 5 , 1978. 2 "Second Harris Poll Finds Public Still Favors Nuclear," Nuclear N e w s , Vol. 2 0 , N o . 1, pp. 3 1 - 3 5 , 1977. ^Webster's Seventh New Collegiate D i c t i o n a r y , G . & C. Merriam C o m p a n y , S p r i n g f i e l d , M a s s a c h u s e t t s , 1 9 6 7 , p. 705. ^Choppin, G . R . , Nuclei and Radioactivity, W . A. B e n j a m i n , I n c . , New York and A m s t e r d a m , 1 9 6 4 , pp. 20-28. 5 P i z z a r e l l o , D. J . and R. L. W i t c o f s k i , Basic Radiation B i o 1 o g y , Lea and F e b i g e r , P h i l a d e l p h i a , 1967, p. 22. 6 C a s a r e t t , A . P . , Radiation B i o l o g y , P r e n t i c e - H a l l , Inc., Englewood C l i f f s , N . J . , 1 9 6 8 , p. 220.~ \ o u t i t , J . F. , Irradiation of Mice and M e n , The University of Chicago P r e s s , Chicago and L o n d o n , 1962, p p . 6 - 7 . 8 C a s a r e t t , p. 2 2 0 . Q S t e r n g l a s s , E. J . , "The Health Effects from Radiation," Vital Speeches of the D a y , Vol. 3 7 , N o . 2 2 , pp. 6 9 9 - 7 0 3 , 1971. ^ T a y l o r , T. B . , with D. C o l l i g a n , "Nuclear Terrorism: Threat of the Future?" Science D i g e s t , Vol. 7 6 , pp. 14-15, A u g u s t , 1974. A ]1 T h e Science and Public Policy Program (including Doi E . K a s h , Director, e t . a l . ) , Energy Alternatives: A Comparative A n a l y s i s , University of O k l a h o m a , N o r m a n , O k l a h o m a , 1975, C h a p . " 6 , "The Nuclear Energy--Fission Resource System," p . 3. 12 1 b i d . , p . 33. 13 " A t o m i c Power's Future," T i m e , April 9 , 1 9 7 9 , p. 20. 14 1 9 7 7 - 1 9 8 6 LWR Spent F u e l Disposition C a p a b i l i t i e s , Energy Research and Development A d m i n i s t r a t i o n , U. S. Government Printing O f f i c e , W a s h i n g t o n , D. C. , 1977, p. 14. ^ S c i e n c e and Public Policy P r o g r a m , p. 33. 1 C o m p t r o l l e r General of the United States, "Nuclear Energy' Dilemma: Disposing of Hazardous Wastes Safely," Report to the C o n g r e s s , General Accounting O f f i c e , U . S. Government Printing O f f i c e , W a s h i n g t o n , D . C . , September 9 , 1977, p . 4 . 28 1? M e t z , W . D . , "Ford-MITRE Study: Nuclear Power Y e s , Plutonium No," S c i e n c e , Vol, 196, N o . 4 2 8 5 , p . 4 1 , 1977. 18 Comptroller General of the United S t a t e s , "Nuclear Energy's Dilemma," p . 52. 19 1 9 7 7 - 1 9 8 6 LWR Spent Fuel Disposition C a p a b i l i t i e s , p. 4 , 20 Comptroller General of the United S t a t e s , "Nuclear Energy's Dilemma," p . ix. 2 1 Ibid., p p . 15-16. 977-1986 LWR Spent Fuel Disposition C a p a b i l i t i e s , p . 5. Report of Task Force for Review of Muc1 ear Waste Management , U. S . D e p a r t m e n t of E n e r g y , Directorate of Energy R e s e a r c h , U. S , Government Printing O f f i c e , W a s h i n g t o n , D. C . , 1978, p. 15. ^ A s s i s t a n t Secretary for the E n v i r o n m e n t , "Everything You've Always Wanted to Know About Shipping High-Level Nuclear Wastes," U. S . Department of E n e r g y , Division of Environmental Control T e c h n o l o g y , 1978. 25 Ibid. 26 "Wrecking Trains for Science," Science D i g e s t , Vol. 8 0 , N o . 1 7 , 1976. 27 Hol l i n g s w o r t h , R. E . , "Environmental Statement--Radioactive Waste R e p o s i t o r y — L y o n s , Kansas," United States Atomic Energy Commission, U. S. Government Printing O f f i c e , W a s h i n g t o n , D. C . , 1 9 7 1 , p. 9. 28 I b i d . , p p . 10-11. 29 Report of Task Force for Review of Nuclear Waste Management , p. 16. 30 C a r t e r , L. J . , "Nuclear Wastes: The Science of Geologic Disposal Seen as Weak," S c i e n c e , Vol, 2 0 0 , pp. 1135-1137. 31 Comptroller General of the United S t a t e s , "Nuclear Energy's Dilemma," p. 37, ^ B r e d e h o e f t , J . D . , et, a l . , "Geoloaic Disposal of Highlevel Radioactive Uastes--Earth Science Perspective," U. S , Geologic Survey C i r c u l a r , N o . 7 7 9 , pp. 1 - 1 5 . 33 Z e l l e r , E, J , , et, a l . , "Putting Radioactive Wastes on Ice," Bulletin of the Atomic S c i e n t i s t s , Vol. 2 9 , N o . 1 , p p . 4 - 9 , 5 0 - 5 2 . i a ? 29 G r i m w o o d , P . D . , and G. A. M . W e b b , "Assessment of the Radiological Protection Aspects of Disposal of High Level Waste on the Ocean Floor," Her Majesty's Stationery O f f i c e , 49 High Hoi b o r n , London WC1V 6 H B , U. K. 35 " L a s e r s Reduce Nuclear Waste," C h e m i s t r y , Vol. 5 0 , N o . 4 , p p . 2 4 - 2 5 , 1977. oc W i l l r i c h , M . , "Terrorists Keep Out!" Bulletin of the Atomic S c i e n t i s t s , Vol. 31, N o . 5 , p. 13. 37 Science and Public Policy P r o g r a m , p. 2 1 . 38 Comptroller General of the United S t a t e s , "Security at Nuclear Powerplants--At B e s t , Inadequate," Report to the C o n g r e s s , April 7 , 1977, p. 17. ~ ^ R e p o r t of Task Force for Review of Nuclear Waste Management , p. "19. C a r t e r , L. J . , "Congressional Committees Ponder Whether to Give States a Right of Veto Over Radioactive Waste Repositories," S c i e n c e , Vol. 2 0 0 , p p . 1136-1137, 1978. ^ F i s h e r , A . , "What Are We Going to Do About Nuclear Waste?" Popular S c i e n c e , Vol. 2 1 3 , No. 6 , p. 9 8 , 1978. 30 BIBLIOGRAPHY A s s i s t a n t Secretary for the E n v i r o n m e n t , "Everything You've Always Wanted to Know About Shipping High-Level Nuclear Wastes," U. S. Department of E n e r g y , Division of Environmental Control T e c h n o l o g y , 1978. "Atomic Power's Future," T i m e , April 9 , 1979, p* 20. B r e d e h o e f t , J . D . , et. a l . , "Geologic Disposal of High-level Radioactive Wastes—Earth Science Perspective," U. S . Geologic Survey Circular, N o . 779. C a r t e r , L. J . , "Congressional Committees Ponder Whether to Give States a Riaht of' Veto Over Radioactive Waste Repositories," S c i e n c e , Vol. 2 0 0 , pp. 1136-1137. "Nuclear Wastes: The Science of Geologic Disposal Seen as Weak," S c i e n c e , Vol. 2 0 0 , pp. 1135-1137. s C a s a r e t t , A . P . , Radiation Biology, P r e n t i c e - H a l l , Inc., Englewood C l i f f s , N . J , , 1968. C h o p p i n , G . R . , Nuclei and R a d i o a c t i v i t y , W . A . B e n j a m i n , Inc., New York and A m s t e r d a m , 1964. Comptroller General of the United S t a t e s , "Nuclear Energy's Dilemma: Disposing of Hazardous Wastes Safely," Report to the C o n g r e s s , General Accounting O f f i c e , U. S . Government Printing O f f i c e , W a s h i n g t o n , D. C . , September 9 , 1977. Comptroller General of the United S t a t e s , "Security at Nuclear Powerplants--At B e s t , Inadeauate," Report to the C o n g r e s s , April 7 , 1977. ' F i s h e r , A . , "What Are We Goinq to Do About Nuclear Waste?" Popular S c i e n c e , Vol. 2 1 3 , N o . 6 , pp. 9 0 - 9 7 , 146, 1978. G r i m w o o d , P. D . , and G. A. M. W e b b , "Assessment of the Radiological Protection Aspects of Disposal of High Level Waste on the Ocean Floor," Her Majesty's Stationery O f f i c e , 49 High Hoi b o r n , London WC1V 6 H 3 , U. K. Hoi 1 ingsworth, R, E . , "Environmental Statement—Radioactive Waste R e p o s i t o r y — L y o n s , Kansas," United States Atomic Energy C o m m i s s i o n , U. S, Government Printing O f f i c e , W a s h i n g t o n , D. C. , 1971. "Lasers Reduce Nuclear Waste," C h e m i s t r y , Vol. 5 0 , N o . 4 , pp. 24-25. fK * 31 L o u t i t , J . F . , Irradiation of Mice and M e n , The University of Chicago P r e s s , Chicago and L o n d o n , 1962. 1977-1986 LWR Spent Fuel Disposition C a p a b i l i t i e s , Energy Research and Development A d m i n i s t r a t i o n , U,~ S. Government Printing O f f i c e , W a s h i n g t o n , D. C . , 1977. M e t z , W . D . , "Ford-MITRE Study: Nuclear Power Y e s , Plutonium No," S c i e n c e , V o l . 196, N o . 4 2 8 5 , p . 4 1 , 1977. P i z z a r e l l o , D. J . and R. L. W i t c o f s k i , Basic Radiation B i o l o g y , Lea and F e b i g e r , P h i l a d e l p h i a , P e n n s y l v a n i a , 1967. R a n k i n , W . L. and S . M . N e a l e y , "Attitudes of the Public About Nuclear Wastes," Nuclear N e w s , Vol. 2 1 , N o . 8 , pp. 112-117, 1978. Report of Task Force for Review of Nuclear Waste M a n a g e m e n t , U. S. Department of Energy", Directorate of Energy Research, U. S . Government Printing O f f i c e , W a s h i n g t o n , D. C . , 1978. The Science and Public Policy Program (including Don E. K a s h , D i r e c t o r , e t . a l . ) , Energy Alternatives: A Comparative A n a l y s i s , University of O k l a h o m a , N o r m a n , OkTancSma, 1 9 7 5 , Chap. 6 , "The Nuclear Eneray--Fission Resource System," pp. 1-74. "Second Harris Poll Finds Public Still Favors Nuclear," N e w s , Vol. 2 0 , N o . 1, pp. 31-35. Nuclear S t e r n g l a s s , E . J . , "The Health Effects from Radiation," Vital Speeches of the D a y , Vol. 3 7 , N o . 2 2 , pp. 6 9 9 - 7 0 3 , 1971. T a y l o r , T . B . , with D , C o l l i g a n , "Nuclear Terrorism: A T h r e a t of the Future?" Science D i g e s t , Vol. 76, pp. 1 2 - 1 7 , A u g u s t , 1974. Webster's Seventh New Collegiate Pi c t i o n a r v , G . S C . Company, S p r i n g f i e l d , M a s s a c h u s e t t s , 1967. Merriam Will r i c h , M . , "Terrorists Keep Out!" Bulletin of the Atomic S c i e n t i s t s , V o l . 3 1 , N o . 5 , pp. 12-16. "Wrecking Trains for Science," Science D i g e s t , Vol. 8 0 , N o . 1 7 , 1976. Z e l l e r , E. J . , et. a l . , "Putting Radioactive Wastes on Ice," Bulletin of the Atomic S c i e n t i s t s , Vol. 2 9 , M o . 1, pp. 4 - 9 , 50-52.