A nonlinear field theory of deformable dielectrics Zhigang Suo Harvard University

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A nonlinear field theory of deformable dielectrics

Zhigang Suo

Harvard University

Work with

X. Zhao, W. Greene, Wei Hong, J. Zhou

Talk 1 in Session 21-2-2, 10:00 am - 12:00 pm

,

Wednesday, 6 June 2007, McMat 2007, Austin, Texas

Slides are available at http://imechanica.org/node/635

1

Dielectric elastomer actuators

•Electromechanical coupling

•Large deformation, light weight, low cost…

•Soft robots, artificial muscles…

L

A

Dielectric

Elastomer

Compliant

Electrode

Reference State

Pelrine, Kornbluh, Pei, Joseph

High-speed electrically actuated elastomers with strain greater than 100%.

Science 287, 836 (2000).

l a

+

Q

Q

Current State

Φ

2

l

Electromechanical instability

Zhao, X, Hong, W., Suo, Z., 2007. http://imechanica.org/node/1283 .

Φ

Φ

+

Q

Q thick thin

Q

Coexistent states: flat and wrinkled

Plante, Dubowsky,

Int. J. Solids and Structures 43 , 7727 (2006).

3

Trouble with electric force

E i

= − Φ

, i

D i , i

= q

+Q +Q

In a vacuum , force between charges can be measured

Define electric field by E = F/Q

D i

= ε

E i

F

= i qE i

+Q

+Q

In a solid , force between charges is

NOT an operational concept

Historical work

•Toupin (1956)

•Eringen (1963)

•Tiersten (1971)

……

Recent work

•Dorfmann, Ogden (2005)

•Landis, McMeeking (2005)

• Suo, Zhao, Greene (2007)

……

4

Maxwell stress in vacuum (1864?)

E i

= − Φ

, i

D i , i

= q D i

= ε

0

E i

F i

= qE i

=

D j , j

E i

=

(

D j

E i

,

) j

D j

E i , j

D j

E i , j

= ε

0

E j

E j , i

=

ε

0

2

(

E k

E k

)

, i

F i

= ε

0

E j

E i

ε

0

2

E k

E k

δ ij

, j

+

Q

E i , j

= − Φ

, ij

=

E j , i

P

σ =

ε

0

2

E

2

σ ij

= ε

0

E j

E i

ε

0

2

E k

E k

δ ij

Q

5 P

Trouble with Maxwell stress in dielectrics

Maxwell said that he didn’t make progress with dielectrics, but his qualms have not prevented people from using his name anyway…

- - - - - - - - - - - -

+ + + + + + + + +

Maxwell stress

σ

33

= −

ε

2

E

2

- - - - - - - - - - - -

+

-

+ + + + + + + + +

Electrostriction

•In dielectrics, electric force is not an operational concept.

ε varies with deformation in general.

•Why E 2 dependence?

•How about the sign of the Maxwell stress?

In solid, Maxwell stress has NO theoretical basis 6

All troubles are gone if we focus on measurable quantities

Work done by the weight P

δ l

Work done by the battery

Φ δ

Q electrode

δ

Q ground

Φ dielectric

P δ l

A transducer

Suo, Zhao, Greene

JMPS, in press. http://imechanica.org/node/635

A system of elastic conductors and dielectrics is specified by a free-energy function U

( )

δ

U

=

P

δ l

+ Φ δ

Q

P

=

U

∂ l

,

Φ =

U

Q

U

( ) is measurable

7

Intensive quantities

L

Reference State

A l

Current State a

+

Q

Q

Φ

Intensive Quantities

λ = l / L s

=

P / A

~

E

= Φ

/ L

~

D

=

Q / A

( E

= Φ

/ l )

( D

=

Q / a )

P

Work done by the weight P

δ l

=

( ) ( ) ( ) s

δλ

Work done by the battery

Φ δ

Q

=

( ) ( )

=

( ) ~

E

δ

~

D

δ

U

=

Free energy per unit volume W

P

δ l

+ Φ δ

Q

δ

W

= s

δλ +

~

E

δ ~

D

⎩ s

~

E

=

=

W

W

/

/

∂ λ

~

D

8

Ideal dielectric elastomer

Decouple elastic and dielectric energy

W

( )

=

W

0

( )

+

W

1

( )

Linear dielectric liquid W

1

( )

=

D 2

2

ε

D

=

Q a

=

Q

λ

1

λ

2

A

= λ

~

D

Arruda-Boyce elastomer:

W

0

= µ

⎢⎣

1

2

(

I

3

)

+

1

20 N

(

I

2

9

I

µ

: small-strain shear modulus

N: number of rigid units between neighboring crosslinks

= λ

2

1

+ λ

2

2

+ λ

2

3

)

+

11

1050 N

2

(

I

3

27

)

+

...

⎥⎦

9

Hysteresis and coexistent states

l

+

Q

Q

~

E

= Φ

/ L

~

D

=

Q / A

( E

= Φ

/ l )

( D

=

Q / a )

Φ

10

Zhao, X, Hong, W., Suo, Z., 2007. http://imechanica.org/node/1283 .

Equilibrium & Stability

Free energy of the system

G

=

L

1

L

2

L

3

W

(

λ

1

,

λ

2

,

~

D

)

P

1

λ

1

L

1

P

2

λ

2

L

2

− Φ

Q

Elastomer weights battery

δ

G

L

1

L

2

L

3

+

1

2

∂ 2

W

∂ λ

2

1

=

⎜⎜

⎛ ∂

W

∂ λ

1

δλ

2

1

+

1

2

− s

1

⎟⎟

δλ

1

+

⎜⎜

⎛ ∂

W

∂ λ

2

∂ 2

W

∂ λ

2

2

δλ

2

2

+

1

2

− s

2

⎟⎟

δλ

2

2

W

~

D

2

δ ~

D

2

+

⎛ ∂

W

~

D

~

E

δ

~

D

+

∂ 2

W

∂ λ

1

∂ λ

2

δλ

1

δλ

2

+

∂ λ

2

1

W

~

D

δλ

1

δ

~

D

+

∂ λ

2

2

W

~

D

δλ

2

δ

~

D

Equilibrium state s

1

=

W

∂ λ

1 s

2

=

W

∂ λ

2

~

E

=

W

~

D det

( )

=

0

,

11

Pre-stresses enhance actuation

Experiment : Pelrine, Kornbluh, Pei, Joseph

Science 287, 836 (2000).

Theory : Zhao, Suo http://imechanica.org/node/1456

12

Inhomogeneous field

A field of weights F iK

=

∂ x i

X

K

∫ s iK

∂ ξ i

X

K dV

= ∫

⎜⎜

~ b i

∂ 2

∂ t x i

2

⎟⎟

ξ i dV

+ ∫ t

~ i

ξ i dA

A field of batteries

~

E

K

= −

∂ Φ

X

K

⎜⎜

∂ η

X

K

⎟⎟

~

D

K dV

= ∫ η q dV

+ ∫ η ω dA

Material laws

δ

W

= s iK

δ

F iK

+

~

D

K

δ ~

E

K s iK

=

W

F iK

~

E

K

•Linear PDEs

•Nonlinear material laws

=

W

F

~

D

( )

K

,

δ

Q

Φ

Suo, Zhao, Greene

JMPS, in press. http://imechanica.org/node/635 P δ l

13

Finite element method

Thick State

Transition

Thin State

Thin State

Transition

Thick State

14

Zhou, Hong, Zhao, Zhang, Suo http://imechanica.org/node/1447

Summary

• A nonlinear field theory. No Maxwell stress. No electric body force. No polarization vector.

• Electromechanical instability.

• Hysteresis and coexistent states.

• Finite element method.

These slides are available at http://imechanica.org/node/635 .

iMechanica get together . Wednesday, 5.45pm-9:00pm, Room 2.120. Beer, snacks…

15

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