AN ABSTACT OF THE THESIS OF Jess Charles Holcomb III for the degree of Master of Science in Soil Science presented on January 20, 2011 Title: Enhanced Efficiency Nitrogen Fertilizers for Nitrogen Management in the Columbia Basin, Oregon Abstract approved: Donald A. Horneck Dan M. Sullivan Ammonia (NH3) volatilization can result in a substantial amount of surface applied nitrogen (N) being lost into the atmosphere, making it an environmental pollutant as well as reducing plant-available N. However, N can also be easily lost from the soil through leaching, and nitrous oxide (NO2). Enhanced efficiency N fertilizers and cultural practices can be used to reduce N pollution and keep N plant-available. The use of these fertilizers and practices has not been examined in the Columbia Basin in Oregon. The objectives of this study were to: (i) examine the effective irrigation rate needed to reduce loss from volatilization from urea, (ii) examine the effectiveness of urease inhibitors in minimizing NH3 loss, measure interactions between inhibitors and irrigation, and measure hydrolysis rates with inhibitors, and (iii) examine if enhanced efficiency N fertilizers could maintain or increase potato yields, whether petiole NO3 accurately reflected plant N with these products, and if they release N according to plant uptake. In the first study, irrigation rates of 0.0 to 22 mm were applied over surface applied urea using a center pivot irrigation system on a wheat field. Ammonia was collected from each plot using the modified passive flux method for 23 days after application (DAA). Cumulative loss of N as NH3 ranged from 3 to 67 kg N acre-1, with the application of 8 mm irrigation reducing loss to 19 kg N ha-1. Peak NH3 loss occurred between 2 and 8 DAA. The reduction of N loss by 90% was obtained through the application of 15 mm irrigation. Increased wheat N concentration was associated with decreased NH3 loss. The second study consisted of recording NH3 loss on a grass seed field from urea, ammonium sulfate, and Agrotain-treated urea. This study also involved recording NH3 loss on a wheat field from urea, Agrotain, and an organo acid complex containing co-polymers (OAC) treated urea at irrigation rates of 0.0, 1.25, and 7.6-mm. Volatilization loss was measured using the modified passive flux method. Urea, Agrotain, and OAC were incubated with soil at three temperatures to measure hydrolysis rates. In the grass seed study Agrotain reduced N loss from NH3 by 71.8% compared to urea, while ammonium sulfate reduced loss by 60.4% compared to urea. In the wheat study, Agrotain lost 5.72 to 6.24% N applied at the 0.00 and 1.25-mm irrigation rate, compared to 53.44% to 60.05% N applied for urea and OAC. With the application of 7.6-mm irrigation, all loss declined with rates of 17.31, 8.11, and 3.17 N applied for urea, OAC, and Agrotain, respectively. Agrotain also decreased urease activity in the wheat field compared to urea and OAC. In incubation, Agrotain delayed complete hydrolysis by 7 days at 26.7oC, 15 days at 16.6oC, and 49 days at 4.4oC compared to urea and OAC. Urea and OAC had similar hydrolysis rates at all temperatures. The use of an effective urease inhibitor, such as Agrotain, can be used to delay hydrolysis and reduce NH3 loss if urea cannot be incorporated. In the final study, enhanced efficiency N fertilizers were applied to Russet Norkota and Russet Burbank potatoes to compare yield and quality with grower standard practices (GSP). Plant N samples were taken from the third year to examine whether petiole nitrate accurately reflected plant N with these products. An incubation of all products for 104 DAA was performed at4.4oC, 16.6oC, and 26.7oC to measure ammonium (NH4) and nitrate (NO3) formation. Similar yields were measured for both years with Russet Norkota. All N treatments were similar, even the 80% GSP, suggesting that N rates were in excess of crop need, thereby reducing sensitivity of N-inhibitor measurements. Reduced yields were measured in two years for Russet Burbank when enhanced efficiency fertilizers were applied compared to 100% GSP. Enhanced efficiency fertilizers maintained yields for one year compared to 100% GSP. Yields with N treatments were usually similar to the 80% GSP, suggesting that N release was not matched with N uptake. In the incubation study, all products except Nutrisphere-N (NSN) were able to delay N release compared to urea. Each product was influenced by temperature, with decreased temperature resulting in a longer delay in conversion of urea to NH4 and conversion of NH4 to NO3 N. Nitamin and N-fusion had only 100% N available at 26.7oC after 104 day. Enhanced efficiency N fertilizers cannot sustain or increase yields on a yearly basis, making their incorporation into Columbia Basin potato production impracticable based on economics. Enhanced efficiency N fertilizers and cultural practices can reduce N loss. However, a reduction in N loss does not always lead to sustained or increased yields. The use of cultural practices can be implemented with minimal expense; however, the fertilizers must present an economical benefit, either as increased yield or a N reduction to be viable in most cropping systems. © Copyright by Jess Charles Holcomb III January 20, 2011 All Rights Reserved Enhanced Efficiency Nitrogen Fertilizers for Nitrogen Management in the Columbia Basin, Oregon by Jess Charles Holcomb III A THESIS submitted to Oregon State University in partial fulfillment of the requirements for the degree of Master of Science Presented January 20, 2011 Commencement June 2011 Master of Science thesis of Jess Charles Holcomb III presented on January 20, 2011. APPROVED: Co-Major Professor, representing Soil Science Co-Major Professor, representing Soil Science Head of the Department of Crop and Soil Science Dean of the Graduate School I understand that my thesis will become part of the permanent collection of Oregon State University libraries. My signature below authorizes release of my thesis to any reader upon request. Jess Charles Holcomb III, Author ACKNOWLEDGEMENTS Sincere appreciation is expressed to my advisors Dr. Don Horneck and Dr. Dan Sullivan. Dr. Horneck helped me with all aspects of my projects, always being there if I had questions, and familiarizing me with the Columbia Basin, the production in it, and all the people. Dr. Sullivan guided me through my time in Corvallis and the continued help and support that I received when I was in Hermiston. I would also like to thank my committee member Dr. George Clough for spending his time to get to know me and my projects, as well as including me in several of his. To my wonderful wife Jesi, for moving with me to Hermiston and making it into our home. She helped me through this entire process, always loving me and supporting me, no matter what path I took. To my family for inspiring me to set the bar for success so high and doing everything to make sure I obtained it. To all my friends along the way who made the journey much more memorable. To the great staff and faculty at the Hermiston Agricultural Research and Extension Center for helping me with all of my projects, my daily activities, and all the great times at HAREC. To Wes and Brenda Wood from Auburn University for helping with the set up of our ammonia devices and answering all the questions that I asked. Thanks to all the growers who lent me their time, resources, crops, and land to conduct my research. Special thanks go to Chet and Art Prior at Eagle Ranch, Kent Madison and Craig at Madison Farms, and Darrin Ditchen at Golden Valley East. I am grateful for the financial support that made these projects possible from Agrotain International and the J.R. Simplot Company. Special thanks to Syngenta for the use of their weather station and IRZ for the use of their soil moisture probes. Finally, to everyone at Oregon State University, who gave me the knowledge to continue down this road and pursue a career in agriculture. CONTRIBUTION OF AUTHORS Dr. Don Horneck assisted with data collection and interpretation for chapters 2, 3, and 4. Dr. Dan Sullivan assisted with data interpretation for chapters 2, 3, and 4. Dr. George Clough along with Dr. Horneck and Dr. Sullivan provided detailed reviews of chapters 2, 3, and 4. TABLE OF CONTENTS Page GENERAL INTRODUCTION………………………………………………………………………………………………. 1 REFERENCES……………………………………………………………………………………………………… 5 EFFECT OF IRRIGATION RATE ON AMMONIA VOLATILIZATION………………………………………… 15 ABSTRACT…………………………………………………………………………………………………………… 12 INTRODUCTION………………………………………………………………………………………………….. 12 MATERIALS AND METHODS………………………………………………………………………………. 14 RESULTS AND DISCUSSION………………………………………………………………………………..… 17 Environmental Conditions………………………………………………………………………. 17 Ammonia Volatilization Loss…………………………………………………………………… 17 Soil and Plant Analyses…………………………………………………………………………… 19 CONCLUSIONS…………………………………………………………………………………………………… 20 ACKNOWLEDGEMENTS……………………………………………………………………………………… 21 REFERENCES………………………………………………………………………………………………………. 21 UREASE INHIBITORS EFFECT ON AMMONIA VOLATILIZATION FROM UREA…….……………… 29 ABSTRACT…………………………………………………………………………………………………………… 30 INTRODUCTION………………………………………………………………………………………………….. 30 MATERIALS AND METHODS………………………………………………………………………………. 33 Grass Seed Study……………………………………………………………………………………. 33 Wheat Study…………………………………………………………………………………………… 34 Incubation Study……………………………………………………………………………………. 35 Statistical Analyses…………………………………………………………………………………. 36 RESULTS AND DISCUSSION………………………………………………………………………………….. 36 Grass Seed Study……………………………………………………………………………………. 37 Wheat Study…………………………………………………………………………………………… 38 Incubation Study……………………………………………………………………………………. 41 CONCLUSIONS…………………………………………………………………………………………………… 41 ACKNOWLEDGEMENTS….……………………………………………………………………………………. 42 REFERENCES………………………………………………………………………………………………………. 42 TABLE OF CONTENTS (Continued) Page EFFECT OF SPECIALTY NITROGEN FERTILIZERS ON RUSSET BURBANK AND RUSSET NORKOTA POTATO YIELD IN THE COLUMBIA BASIN………………………………………………………… 55 ABSTRACT…………………………………………………………………………………………………………… 56 INTRODUCTION…………………………………………………………………………………………………. 56 MATERIALS AND METHODS………………………………………………………………………………. 60 Potato Field Study………………………………………………………………………………… 60 Incubation Study……………………………………………………………………………………. 61 Statistical Analyses…………………………………………………………………………………. 62 RESULTS AND DISCUSSION………………………………………………………………………………..… 62 Russet Norkota……………………………………………………………………………………… 62 Russet Burbank………………………………………………………………………………………. 64 Incubation Study……………………………………………………………………………………. 67 CONCLUSIONS…………………………………………………………………………………………………… 71 REFERENCES……………………………………………………………………………………………………… 71 GENERAL CONCLUSIONS…………………………………………………………………………………………………. 97 BIBLIOGRAPHY……………………………………………………………………………………………………………….. 100 APPENDICES…………………………………………………………………………………………………………………… 110 LIST OF FIGURES Figure 2.1 2.2 2.3 3.1 3.2 3.3 3.4 3.5 3.6 3.7 4.1 4.2 Page (a) Air temperature and soil temperature at 2.54-cm; and (b) wind speed measured every 15 minutes during the study period from 9 March to 2 April 2010……………………………………………………………………………………………………………………. 25 Cumulative loss of NH3 during the period of 9 March to 2 April 2010 following application of 112 kg urea-N ha-1 to winter wheat as affected by rate of irrigation……………..……………………………………………………………………………………………… 26 Cumulative loss of NH3 during the period of 9 March to 2 April 2010 following application of 112 kg urea-N ha-1 to winter wheat as affected by rate of irrigation application.……………………………............................................................... 27 Infrared photo of wheat field displaying layout of irrigation study. Irrigation rates are randomly selected within each block.…………………………………………………… 47 (a) Air temperature and soil temperature at 2.54-cm, soil temperature data before 4 DAA was lost; and (b) wind speed measured at the grass seed fields……. 48 Cumulative loss of NH3 during the period of 28 September to 13 October 2009 following application of 112 kg N/ha to Kentucky bluegrass as affected by N source. ……………………………………………………………………………………………………………….. 49 (a) Air temperature and soil temperature at 2.54-cm; and (b) wind speed measure at the wheat field. ……………………………………………………………………………… 50 Cumulative loss of NH3 during the period of 9 March to 2 April 2010 following application of 112 kg N ha-1 to winter wheat as affected by N and irrigation rate treatments. ………………………………………………………………………………………………………… 51 Cumulative loss of NH3 within irrigation rates for the period of 9 March to 2 April 2010 following application of 112 kg N ha-1 to winter wheat for urea, Agrotain, and OAC. …………………………………………………………………………………………….. 52 Net NH4-N from fertilizer, as affected by N treatment at incubation temperature (a) 4.4oC, (b) 16.6oC, and (c) 26.7oC……………………………………………………………………… 53 Available NH4 at 4.4oC from (a) urease and nitrification inhibitors, (b) polymer coated urea, and (c) slow release N in incubation as affected by N treatment.…. 77 Available NH4 at 15.6oC from (a) urease and nitrification inhibitors, (b) polymer coated urea, and (c) slow release N in incubation as affected by N treatment……. 78 LIST OF FIGURES (Continued) Figure 4.3 4.4 Page Available NH4 at 26.7oC from (a) urease and nitrification inhibitors, (b) polymer coated urea, and (c) slow release N in incubation as affected by N treatment……. 79 Soil pH at (a) 4.4oC, (b) 15.6oC, and (c) 26.7oC in incubation as affected by N treatment……………………………………………………………………………………………………………. 80 LIST OF TABLES Table 2.1 Page Soil urease activity from 0-2.54 cm soil depth, wheat dry matter, wheat N concentration, and wheat N uptake sampled 23 DAA.…………............................... 28 Wheat response and soil urease activity (0-2.5 cm) as affected by N treatment and irrigation rate ………………………………………………………………………………………………. 54 4.1 Modes of action for enhanced efficiency nitrogen fertilizers………………………………. 81 4.2 Nitrogen treatments for Russet Norkota and Russet Burbank for 2007, listing N source, N rates (kg ha-1), and application timing…………………………………………………. 82 Nitrogen treatments for Russet Norkota and Russet Burbank for 2008, listing N source, N rates (kg ha-1), and application timing…………………………………………………. 83 Nitrogen treatments for Russet Burbank for 2009, listing N source, N rates (kg ha-1), and application timing………………………………………….……………………………………. 84 Mean monthly air temperature, soil temperature, and total precipitation for years 2007-2009………..………………………………………………………………………………………. 85 Yield, potato class, specific gravity, and internal damage for Russet Norkota in 2007 as affected by N treatment………………………………………………………………………. 86 Petiole nitrate levels for Russet Norkota in 2007 as affected by N treatment and sampling date (DAP)……………………………………………………………………………………………. 87 Yield, potato class, and specific gravity for Russet Norkota in 2008 as affected by N treatment…………..……………………………………………………………………………………………. 88 Petiole nitrate levels for Russet Norkota in 2008 as affected by N treatment and sampling date (DAP)……………………………………………………………………………………………. 89 Yield, potato class, specific gravity, and internal damage for Russet Burbank in 2007 as affected by N treatment………………………………………………………………………. 90 Petiole nitrate levels for Russet Burbank in 2007 as affected by N treatment and sampling date (DAP)……………………………………………………………………………………………. 91 Yield, potato class, specific gravity, and internal damage for Russet Burbank in 2008 as affected by N treatment………………………………………………………………………. 92 Petiole nitrate levels for Russet Burbank in 2008 as affected by N treatment and sampling date (DAP)……………………………………………………………………………………………. 93 3.1 4.3 4.4 4.5 4.6 4.7 4.8 4.9 4.10 4.11 4.12 4.13 LIST OF TABLES (Continued) Table 4.14 4.15 4.16 Page Yield, potato class, specific gravity, and internal damage for Russet Burbank in 2009 as affected by N treatment………………………………………………………………………. 94 Petiole nitrate levels for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP)……………………………………………………………………………………………. 95 Potato plant N concentration (%) for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP)……………………………………………………………………. 96 LIST OF APPENDIX FIGURES Figures 6.1 Page Absorbance from ammonium as affected by using ammonium standards in deionized water and in 0.013835 M oxalic acid……………………………………………………… 111 Absorbance from ammonia samplers tested (a) with 1 drop (4 drops NH4OH/1 L de-ionized water (DI)) and (b) 3 drops (4 drops NH4OH/1 L DI) as affected by the frequency of shaking with DI water…………………………………………………………………… 112 Concentration from ammonia samplers tested with 1 drop, 2 drops, and 2 mL of NH3 cleaner and 1 drop (4 drops NH4OH/1 L de-ionized water (DI)) as affected by the extraction with de-ionized water or KCl solution……………………………………… 113 Absorbance of NH4-free water compared to NH4-free water shaken in a burned tube, tube was burned at 450oC for 16 hours……………………………………………………… 114 Absorbance from ammonium standards as affected from the standards being ammonium or nitrate decomposed in Devarda’s alloy to ammonium………………… 115 Absorbance from ammonium standards from nitrate decomposition in Devarda’s alloy as affected by the length of time decomposition was allowed in Devarda’s alloy…………………………………………………………………………………………………… 116 Absorbance from ammonium as affected by using ammonium standards in deionized water and in 2 M KCl solution…………………………………………………................. 117 Cumulative loss of NH3 during the period of 29 July to 24 August 2009 following application of 112 kg N/ha to wheat stubble as affect by N source of urea and Agrotain coated urea…………………………………………………………………………................... 118 6.9 Average diurnal nitrogen loss as ammonia across treatments on wheat stubble… 119 6.10 Cumulative loss of NH3 during the period of 23 October to 9 November 2009 following application of 112 kg N/ha to unburned grass seed field as affect by N source of urea and Agrotain coated urea………………………………………....................... 120 Percent of plots burned after the application of 112 kg N/ha to unburned grass seed field as affect by N source of urea and Agrotain coated urea……................... 121 Soil moisture at varying depths for irrigation rates (a) 0.0-mm, (b) 3.8-mm, and (c) 11.4-mm…………………………………………………………………………………………................. 122 Available (a) NO3 and (b) total N (NH4 + NO3) at 4.4oC in incubation as affected by N treatment……………………………………………………………………………………………………. 123 6.2 6.3 6.4. 6.5 6.6 6.7 6.8 6.11 6.12 6.13 LIST OF APPENDIX FIGURES (Continued) Figures 6.14 6.15 6.16 Page Available (a) NO3 and (b) total N (NH4 + NO3) at 15.6oC in incubation as affected by N treatment…………………………………………………………………………………………………… 124 Available (a) NO3 and (b) total N (NH4 + NO3) at 26.7oC in incubation as affected by N treatment……………………………………………………………………………………………………. 125 Size of fertilizer prills based on product………………………………………………………………. 126 LIST OF APPENDIX TABLES Table 6.1 Page Linear regression for absorbance from N standards with concentrations ranging from 0 to 15 ppm NH4-N as affected by time of color determination…………………. 127 Ammonium levels measured after nitrate decomposition as affected by the initial rate of nitrate added to Devarda’s alloy…………………………………………………… 128 6.3 Average 12-hour weather data for diurnal wheat stubble data…………………………… 129 6.4 Average ppm nitrogen (N) as ammonia for the sampling period before (Aug 6), during (Aug 7), and after (Aug 10) a smoke event……………………………………………… 130 Cumulative loss of NH3 from plots during 1 hour on 20 November 2009 resulting from the application of waste water to an alfalfa field through irrigation…………… 131 Soil N present as NH4 and NO3 at varying soil depth after the application of 112 kg N as urea/ ha as affected by irrigation rate…………………………………………………….. 132 Soil pH at varying soil depths after the application of 112 kg N ha-1 as urea as affected by irrigation rate…………………………………………………………………………………… 133 Accountable N at varying soil depth after the application of 112 kg N ha-1 as urea as affected by irrigation rate; accountable N = wheat N uptake + soil N corresponding to soil depth………………………………………………………………………………… 134 Soil pH at varying soil depths after the application of 112 kg N/ha as affected by irrigation rate and N source……………………………………………………………………………. 135 Soil N present as NH4 and NO3 at varying soil depth after the application of 112 kg N/ha as affected by irrigation rate and N-source………………………………………… 136 Accountable N at varying soil depth after the application of 112 kg N/ha as affected by irrigation rate and N-Source; accountable N = wheat N uptake + soil N corresponding to soil depth…………………………………………………………………………… 137 Urease activity 104 days after application of N fertilizer as affected by N-source and incubation temperature……………………………………………………………………………….. 138 Potato vine tonnage for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP)……………………………………………………………………………………………. 139 Potato tonnage for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP)…………………………………………………………………………………………… 140 6.2 6.5 6.6 6.7 6.8 6.9 6.10 6.11 6.12 6.13 6.14 LIST OF APPENDIX TABLES (Continued) Table 6.15 Page Potato plant N uptake for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP)…………………………………………………………………………………….. 141 Potato N concentration (%) for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP)……………………………………………………………………. 142 Potato N uptake for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP)…………………………………………………………………………………………… 143 Linear regression for NH3 loss from 2 DAA to 8 DAA following application of 112 kg urea-N/ha to Winter Wheat as affected by rate of irrigation application………… 144 Linear regression for NH3 loss from 2 DAA to 8 DAA following application of 112 kg urea-N/ha to Winter Wheat as affected by N treatment and rate of irrigation application. ………………………………………………………………………………………………………… 145 6.20 Soil urease activity in incubation as affected by N treatment and temperature….. 146 6.21 Available NH4 at 4.4oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05………………… 147 Available NO3 at 4.4oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05…………………. 148 Total N (NH4 + NO3) at 4.4oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05………………….. 149 Available NH4 at 15.6oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05………………… 150 Available NO3 at 15.6oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05…………………. 151 Total N (NH4 + NO3) at 15.6oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05…………………. 152 Available NH4 at 26.7oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05………………… 153 Available NO3 at 26.7oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05………………… 154 6.16 6.17 6.18 6.19 6.22 6.23 6.24 6.25 6.26 6.27 6.28 LIST OF APPENDIX TABLES (Continued) Table Page Total N (NH4 + NO3) at 26.7oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05………………… 155 6.30 Soil pH at 4.4oCin incubation as affected by N treatment…………………………………… 156 6.31 Soil pH at 15.6oCin incubation as affected by N treatment………………………………… 157 6.32 Soil pH at 26.7oC in incubation as affected by N treatment………………………………… 158 6.29 DEDICATION To Jesi, my perfect and wonderful wife, my best friend! ENHANCED EFFICIENCY NITROGEN FERTILIZERS FOR NITROGEN MANAGEMENT IN THE COLUMBIA BASIN, OREGON GENERAL INTRODUCTION Jess Charles Holcomb III 2 Nitrogen (N) and potassium are typically the most abundant minerals found in crops and are the most limiting nutrients for crop production (Olson and Kurtz, 1982; Hopkins et al., 2008). One reason for the lack of N in agricultural systems is due to soils not having a mechanism for long-term storage of large amounts of plant-available N, preventing a N build up (Olson and Kurtz, 1982; Meisinger et al., 2008). The lack of long-term storage results in N being added during production to obtain maximum yield. Symbiosis with N-fixing organisms would negate the need for additional N (Havelka et al., 1982; Meisinger et al., 2008). Nitrogen added to meet plant demand is subject fixation in the soil along with loss through nitrate (NO3) leaching, ammonia (NH3) volatilization, and nitrous oxide (N2O) emissions, with the total loss ranging from 10 to 60% of N applied (Nommik and Vahtras, 1982; Goulding, 2000). Leaching of NO3 typically represents the majority N loss, followed by volatilization, while the loss of N as N2O is usually negligible except in anaerobic soils (Zebarth and Rosen, 2007). As a result of N loss, an average crop’s N uptake efficiency ranges from 40 to 75% (Allison, 1955; Elkashif et al., 1983). Low N uptake efficiency results in the need to over apply N to obtain maximum crop yield (Waddell et al., 1999). Nitrate leaching is a prominent concern in well-drained sandy soil, such as are found in production areas in the Columbia Basin in Oregon and Washington (Peralta and Stockle, 2001; Alva et al., 2002). Sandy soils along with irrigation and increased N fertilization can result in a large NO3 loss (Jones and Wagner, 1995; Ryker and Jones 1995; Zvomuya et al., 2003; Zebarth and Rosen, 2007). Unlike ammonium which is strongly sorbed to soil, NO3 is weakly held by soil making it more susceptible to leaching (Mulla and Strock, 2008). Excessive irrigation of sandy soils allows NO3 to leach out of the root zone at a faster rate (Shock et al., 2007). Leaching of NO3 can be large if a field is not cropped immediately after harvest, as mineralized N from residue adds to soil N. (Asfary et al., 1983; Goulding, 2000; Peralta and Stockle, 2001; Honisch et al., 2002). In random surveys in the Columbia Basin, 30 to 33% of all groundwater sources were above the EPA standard of 10 ppm NO3-N (Alva et al., 2002). Surface water containing leached NO3 can also be a pollutant, leading to increased vegetative productivity in lakes and estuaries causing eutrophication (Keeney, 1982). Loss of N from ammonia volatilization usually ranges from 15 to 40% of N applied, with loss measured up to 83% N applied (Lightner et al., 1990; Grant et al., 1996; Sommer and Ersboll, 1996; Ledgard et al., 1999; Martha Jr. et al., 2004; Vaio et al., 2008; Kissel et al., 2009). 3 Urea is especially vulnerable to ammonia volatilization because it must hydrolyze before plant use according to the following reaction by Kissel et al. (1988): urea + 2H2O + H+ urease 2NH4+ + HCO3further reacting as: HCO3- + H+ CO2(g) + H2O and NH4+NH3 + H+ The consumption of H+ during urea hydrolysis results in a pH increase (Zaman et al., 2008). Increased pH results in more NH3 which increases potential volatilization loss (Kissel et al., 1988). Ammonia loss not only represents an agronomic loss of N, but also an environmental pollutant. Agriculture is responsible for an estimated 90% of anthropogenic ammonia emissions (Boyer et al., 2002), with 12% resulting from fertilizer application and the remainder from animal production (Ferm, 1998). Most atmospheric NH3 is deposited locally at its origin (Boyer et al., 2002). The remaining NH3 can be transported long distances as secondary aerosol particles (Schjoerring et al., 1992; Boyer et al., 2002). Secondary aerosols are created by the reaction of NH3 with NOx and SOx which results in light scattering atmospheric haze (Ferm, 1998; Sharma et al., 2007). Ammonium is the limiting factor for haze formation in the Columbia River Gorge between Oregon and Washington (Pitchford et al., 2008). In the winter of 2003-2004, a 19-week study set in the Columbia River Gorge reported total inorganic N deposition for the study ranging from 1.09 kg ha-1 to 1.71 kg ha-1 (Fenn et al., 2007). The origins of the N was attributed to livestock operations and fertilizer applications in the Columbia Basin. This is a direct concern for the Columbia Basin as an NH3 source. Increased N deposition levels favor nitrophillic organisms and suppress organisms adapted to low N environments, altering native ecosystems (Fenn et al., 2003; Geiser and Neitlich, 2007). This has been observed in the Columbia River Gorge as fewer N-sensitive lichen are now present and there is intrusion by two non-native nitrophillic lichen species (Gieser and Neitlich, 2007). Loss of N from N2O is not agronomically important in aerobic soils as emissions from most crops rarely exceed 2% N applied; however, loss over 10% has been reported (Delgado and Mosier, 1996; Ruser et al., 2001; Shoji et al., 2001; Venterea et al., 2005). Agriculture is estimated to produce over 75% of anthropogenic N2O (Isermann, 1994). The atmospheric life of N2O is about 120 years and has a global warming potential 320 times greater than CO2 (IPCC, 1995). Nitrous oxide is an intermediate product formed during denitrification (Mosier, 1998; Zebarth and Rosen, 2007). The addition of N to saturated soils increases N2O production (Ruser 4 et al., 2001). Although the Columbia Basin is intensively managed with large quantities of N being applied in several production areas, the formation of N2O may be minimal as most soils are sandy and well drained, limiting saturation and anaerobic conditions. The development of enhanced efficiency fertilizers (EEF’s) can limit N loss to the environment and/or increase nutrient availability compared to conventional fertilizers (OlsonRutz et al., 2009). Enhanced efficiency fertilizers accomplish this through inhibition of a N conversion pathway, slow release, or controlled release. Urease inhibitors slow the hydrolysis of urea allowing soil to buffer a pH increase, therefore reducing loss from volatilization and allowing time for incorporation, such as Agrotain (Jones et al., 2007). An inhibitor preventing nitrification, like Dicyandiamide (DCD), slows the conversion of NH4 to NO3; NH4 is less susceptible to leaching (Vos, 1994). Inhibitors also can be mixed together to get the benefit of both such as Super-U. Slow-release N is made available through microbial breakdown of a fertilizer like Nitamin (Vaio et al., 2008; Olson-Rutz et al., 2009). Controlled-release fertilizers are coated with a soluble membrane that acts as a diffusion barrier which releases N based on soil temperature or water content, such as Environmentally Smart Nitrogen (ESN) (Hanafi et al., 2002; Taysom et al., 2007; Wilson et al., 2009). Enhanced efficiency fertilizer products have been recorded to reduce N loss into the environment (Carmona et al., 1990; Zhengping et al., 1991; Vos, 1994; Delgado and Mosier, 1996; Grant et al., 1996; Waddell et al., 2000; Shoji et al., 2001; Zvomuya et al., 2003; Sanz-Cobena et al., 2008; Vaio et al., 2008; Zaman et al., 2008; Zaman et al., 2009). Nitrogen release rates from EEF’s depending on environmental conditions and plant N demand have resulted in cases of sustained or increased yields as well as yield reduction (Lorenz et al., 1972; Lorenz et al., 1974; Cox and Addiscott, 1976; Liegel and Walsh, 1976; Elkashif et al., 1983; Vos, 1994; Shoji et al., 2001; Zvomuya and Rosen, 2001; Zvomuya et al., 2003; Pack et al., 2006; Taysom et al., 2007). The variability of N release often not coinciding with plant demand and the premium for EEF’s often makes them unusable compared to a standard N form (Pasda et al., 2001; Hopkins et al., 2008). Nitrogen loss reductions also can be obtained through cultural practices. By mechanically incorporating urea into the soil, N loss associated with NH3 volatilization can be reduced (Malhi et al., 2003). Volatilization loss can be reduced from surface-applied urea through incorporation by irrigation or precipitation (Harper et al., 1983; Bouwmeester et al., 1985; Black et al., 1987; Mugusha and Pluth, 1995). However, an effective irrigation rate 5 needed for reduction have not been fully researched. Splitting applications of N can increase N use efficiency; less N is available for leaching and it is more likely to remain in the root zone (Singh and Sekhon, 1976; Elkashif et al., 1983; Lauer, 1985; Lauer, 1986; Westermann et al., 1988; Vos, 1999). The reduction of N2O can be accomplished by reducing anaerobic soil conditions brought on by excessive irrigation and soil compaction (Ruser et al., 1998). The EEF N products and cultural practices are currently being used in the Columbia Basin but not enough is known about methods or effectiveness in order to maximize yield and reduce loss. The objective of this study was to: (i) examine the required irrigation rate needed to minimize NH3 volatilization; (ii) examine the effectiveness of specialty N fertilizers to minimize NH3 volatilization; (iii) examine whether specialty N fertilizers could maintain or increase potato yields in the Columbia Basin; and (iv) examine the formation rate of NH4 from EEF N products. REFERENCES Allison, F.E. 1955. The enigma of soil nitrogen balance sheets. Adv. Agron. 7:213-250. Alva, A.K., T. Hodges, R.A. Boydston, and H.P. Collins. 2002. Effects of irrigation and tillage practices on yield of potato under high production conditions in the Pacific Northwest. Commun. Soil Sci. Plant Anal. 33:1451-1460. Asfary, A.F., A. Wild, and P.M. Harris. 1983. Growth, mineral nutrition and water use by potato crops. J. 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Potato J. 65:337-386. Wilson, M.L., C.J. Rosen, and J.F. Moncrief. 2009. Potato response to a polymer-coated urea on an irrigated, coarse-textured soil. Agron. J. 101:897-905. Zaman, M., M.L. Nguyen, J.D. Blennerhassett, and B.F. Quin. 2008. Reducing NH3, N2O, and NO3-N losses from a pasture soil with urease or nitrification inhibitors and elemental Samended nitrogenous fertilizers. Biol. Fertil. Soils 44:693-705. Zaman, M., S. Saggar, J.D. Blennerhassett, and J. Singh. 2009. Effect of urease and nitrification inhibitors on N transformation, gaseous emissions of ammonia and nitrous oxide, pasture yield and N uptake in grazed pasture system. Soil Biol. Biochem. 41:1270-1280. Zebarth, B.J. and C.J. Rosen. 2007. Research perspective on nitrogen BMP development for potato. Amer. J. Potato Res. 84:3-18 Zhengping, W., O.V. Clemmput, P. Demeyer, and L. Baert. 1991. Effect of urease inhibitors on urea hydrolysis and ammonia volatilization. Biol. Fertil. Soils 11:43-47. Zvomuya, F., and C.J. Rosen. 2001. Evaluation of polyolefin-coated urea for potato production on a sandy soil. HortScience 36:1057-1060. Zvomuya, F., C.J. Rosen, M.P. Russelle, and S.C. Gupta. 2003. Nitrate leaching and nitrogen recovery following application of polyolefin-coated urea to potato. J. Environ. Qual. 62:480-489. 11 EFFECT OF IRRIGATION RATE ON AMMONIA VOLATILIZATION Jess C. Holcomb III, Donald A. Horneck, Dan M. Sullivan, and George H. Clough Soil Science Society of America Journal 5585 Guilford Road Madison, WI 53711 In Review 12 ABSTRACT Sprinkler irrigation can limit loss from ammonia (NH3) volatilization when urea is surface applied. This study was conducted to find the effective irrigation rate needed to limit loss from volatilization with urea. A gradient of six irrigation rates (0.0, 1.25, 3.8, 7.6, 11.4, and 21.6-mm) was used to find effective irrigation depth for urea. Ammonia was collected by the modified passive flux method for 23 days after application (DAA). Cumulative NH3 loss ranged from 3.1 to 67.3 kg Nitrogen (N)/ha, with 7.6 mm reducing loss to 19.4 kg N/ha. During peak ammonia loss from 2-8 DAA, the application of 11.4 mm irrigation was able to reduce loss to 0.5% of N applied/day. To reduce total loss from NH3 by 90%, 14.6 mm of irrigation needed to be applied. Decreased NH3 loss associated with higher irrigation rate led to increased wheat N concentrations. The application of 14.6 mm of irrigation can successfully incorporate urea and reduce loss from NH3 volatilization. INTRODUCTION Urea is an important source of N because of its high N content (46%), low cost, ease in handling and its compatibility with other fertilizer materials (Harre and Bridges, 1988; Kissel et al., 2009). In the presence of the enzyme urease with water, urea hydrolyzes according to the reaction (Kissel et al., 1988): urea + 2H2O +H+ urease 2NH4+ + HCO3further reacting as: HCO3- + H+ CO2(g) + H2O. Both reactions consume H+ and raise soil pH around reaction site. This increases the ratio of ammonia to ammonium which promotes volatilization loss (Fenn and Hossner, 1985). Reported ammonia volatilization losses from urea range from 15-40% of N applied (Lightner et al., 1990; Sommer and Ersboll, 1996; Vaio et al., 2008; Kissel et al., 2009). Agricultural activity is estimated to be responsible for 90% of anthropogenic NH3 emissions (Boyer et al., 2002), with the majority coming from livestock production and 12% from N fertilizer application (Ferm, 1998). Ammonia volatilization represents an agronomic N loss as well as an environmental pollutant. In the atmosphere the reaction of NH3 with NOX and SOX 13 creates particulate matter 2.5 μm aerosols that scatter light resulting in haze (Asman et al., 1998; Ferm, 1998; Sharma et al., 2007). In the Columbia River Gorge in Oregon and Washington, the deposition of inorganic N from 133 days in 2003-2004 ranged from 0.61 kg/ha to 0.81 kg/ha with N sources originating from livestock operations and fertilizer applications in the Columbia Basin (Fenn et al., 2007). Increased N deposition favors species that tolerate or thrive in a high N environment while suppressing those adapted to low N (Fenn et al., 2003; Geiser and Neitlich, 2007). Urea needs to be incorporated to a depth of 5 cm or more in soil to minimize ammonia volatilization (Fenn and Miyamoto, 1981) with mechanical or irrigation incorporation being suitable to minimize loss. Research on effective irrigation depth has varied from 5-75 mm to minimize volatilization (Harper et al., 1983; Bouwmeester et al., 1985; Black et al., 1987; Mugusha and Pluth, 1995). Vaio et al. (2008) reported loss occurring after 52 mm of rainfall on a tall fescue pasture. Kissel et al. (2004) found rainfall had no effect on ammonia loss with rain between 0 and 40 mm in a Loblolly pine plantation. These studies used either predetermined irrigation rates and timing or recorded that volatilization ceased or continued after precipitation events. No study compared a gradient of irrigation rates to determine irrigation depth required to minimize volatilization loss. This has left effective irrigation requirements not established. Typically, measurements of NH3 loss have been conducted in a laboratory by placing soil and N fertilizer in a container and forcing air through an acid trap (Ernst and Massey, 1960; Stumpe et al., 1984; Ferguson and Kissel, 1986; Whitehead and Raistick, 1990; Zhengping et al., 1991; Sommer and Ersboll, 1996). It is difficult to relate laboratory conditions to field losses as many parameters are controlled, however laboratory studies do provide valuable insight into parameters affecting ammonia loss. Using polyvinyl chloride (pvc) inserted into the soil and temporarily capping the system and recording NH3 loss by acid traps allowed field measurement of ammonia loss (Keller and Mengel, 1986; Lightner et al.,1990). Using the same system but suspending the cap to allow air movement allowed NH3 loss to be measured on a daily basis and totaled for a study period (Oberle and Bundy, 1987; Grant et al., 1996; Martha Jr. et al., 2004). Cabrera et al. (2001) constructed a chamber that automatically opened its lid when finished testing; when the lid was closed, a pump simulated the current wind conditions outside the chamber by forcing the air through an acid trap. These laboratory and field techniques prove useful in measuring NH3, but they may not express NH3 loss under natural conditions as 14 enclosures alter air movement, precipitation, soil temperature, air temperature and/or solar radiation inside the chambers (Martha Jr. et al., 2004). Leuning et al. (1985) constructed an ammonia flux sampler that was placed at the center of a plot and trapped ammonia at five heights with a sampler “shuttle” that pivoted into the wind at each height. Schjoerring et al. (1992) used a four-mast system where the masts were placed on the edge of the plot and measured NH3 flux at four heights with inexpensive glass sampler tubes that allow frequent sampling. The advantage of these systems was not altering the treatment area and measuring field scale NH3 volatilization loss. Both are expensive for startup and sample analysis (Wood et al., 2000). Wood et al. (2000) reduced the cost by combining the systems of using a single mast with glass samplers that rotated into the wind at the center of a plot. This method has been used successfully to measure NH3 loss in field conditions (Wood et al., 2000; Sullivan et al., 2003; Vaio et al., 2008; Holcomb III and Horneck 2009). The objective of this study was to measure the effect of irrigation rate on NH3 volatilization from urea, account for the loss of N from NH3 loss, and determine the effective irrigation rate needed to incorporate urea to minimize NH3 loss. MATERIALS AND METHODS This study was conducted in a center-pivot irrigated 50-ha wheat field in Umatilla County near Echo, OR. The soil was classified as an Adkins fine sandy loam (coarse-loamy, mixed, superactive, mesic Xeric Haplocalcids). The surface soil (0-30 cm) had an average pH of 6.5 (1:1 soil/deionized water). The field was watered 2 days before our study with 25.4-mm irrigation to incorporate prior N application, raise the soil to field capacity, and even out surface soil moisture. The field was split into 18 wedges of 20o; each wedge contained a circular (30-m diameter) plot with urea surface-applied at 112 kg N/ha and with each plot separated by at least 100 m to avoid contamination of NH3 between treatments. The pivot was programmed to irrigate wedges with 0.0, 1.25, 3.8, 7.6, 11.4, and 21.6-mm corresponding to treatments, with the treatments arranged in a randomized complete block design. A rain gauge was placed in each treatment wedge in order to record irrigation rate. As this was the first irrigation of the 15 season, irrigation rates fluctuated due to inconsistent pressure in the irrigation lines and rates reported are averages (Standard errors for irrigation rates are 0.00, 0.15, 0.19, 0.66, 0.59, and 3.29 for 0.0, 1.25, 3.8, 7.6, 11.4, and 21.6-mm irrigation, respectively). Immediately after irrigation, measurement of ammonia volatilization loss was initiated using the modified passive flux method (Wood et al, 2000; Vaio et al., 2008). This consists of a rotating mast placed at the center of each circular plot. A tripod which did not interfere with the rotation of the mast was placed on the mast in order to stabilize it during high wind events. Each mast was equipped with a passive-flux sampler at five heights (0.45, 0.75, 1.50, 2.25, and 3.00 m; Leuning et al., 1985). Each passive flux sampler consisted of a glass tube (0.7-cm i.d. by 20 cm long) with the inside surface coated with 3% w/v oxalic acid in acetone to trap the NH3 in the air flowing through the tube and an attached nozzle with a 1 mm hole to restrict incoming air flow. Four identical background masts were placed in the field to measure ambient NH3, three on the outside and one in the center. Background masts were place over 100-m from treatments to protect against contamination. Most background NH3 levels were near zero during the study. Ammonia flux samplers were replaced at 2, 3, 4, 5, 6, 7, 8, 10, 13 15, 17, and 24 days after application (DAA) of fertilizer. Flux samplers were extracted by adding 2-mL deionized water and shaken for 10-minutes. Extracts were analyzed colormetrically for NH4 (Sims et al., 1995). Horizontal NH3 flux (Fx, μg N m-2 s-1) for each flux sampler was calculated by Fx = (C*V)/(πr2KΔt) [1] where C is the concentration of NH4-N (μg N/ml) in deionized water used to extract sorbed NH4N, V is the volume of deionized water used for extraction (2mL), r is the radius of the hole in the disc on the nozzle (0.0005 m), K is a correction factor (0.77), and Δt is the time at which the sampler was exposed (s) (Schjoerring et al., 1992; Wood et al., 2000; Vaio et al., 2008). Net horizontal flux for each sampler (Fx,p) was determined by subtracting horizontal flux from the corresponding sampler height on the background mast (Fx,b). Net vertical flux (Fy, ug N m-2 s-1) from each plot was estimated by integrating each horizontal flux with vertical distance for each sampler accounted for: Fy=(1/R)Σ(Fx,p-Fx,b)Δh [2] where R is the radius of the plot (15-m), and Δh (m) is the vertical distance corresponding to each sampler. 16 An Adcon Telemetry (Klosterneuburg, Austria) weather station was placed at the study area to measure air temperature, soil surface temperature, humidity, rainfall, wind speed, and wind direction. Sentek Enviroscan (Stepney, Australia) moisture probes were placed at the 0.0, 3.8 and 11.4 mm irrigation rates in block 1 to measure soil moisture at 10.1, 20.3, 30.4, 50.8, and 91.4 cm depths. Soil samples were taken at 23 days after application (DAA) from depths of 0-2.5, 0-15.2, and 0-30.4 cm. Soil samples were extracted with 2 M KCl (1:10 soil/KCl) and extracts were analyzed colormetrically for NH4-N and NO3-N (Sims et al., 1995). The pH for each soil treatment was analyzed using a 1:1 soil/water solution. Urease activity was determined for the 0-2.5 cm depth only according to Torello and Wehner (1983). This consisted of 2, 2-g soil samples from each treatment which were incubated for 5 hours in a phosphate buffer - urea solution; one sample was inhibited by AgSO4 during the incubation. After incubation, both soils received KCl and the uninhibited soil received AgSO4. Soils were then shaken for 1 hour. Solutions were filtered through a Whatman No. 1 filter paper and the extract was analyzed colorimetrically for ammonium (Sims et al., 1995). Net urease activity was calculated by subtracting the inhibited sample from the uninhibited sample and expressed as μg NH4-N g-1 h-1. Wheat samples were randomly sampled from each treatment (0.126 m2) at 23 DAA. Above-ground dry matter was measured and total N was analyzed using the total N combustion method (Gavlak et al., 2003) with an Elementar Vario Max CN analyzer (Hanau, Germany). Ammonia loss from volatilization, soil ammonium and nitrate, soil pH, urease activity, wheat dry matter, and wheat N concentration and uptake were subjected to an analysis of variance and analyzed for linear and quadratic relationships with irrigation rate. Irrigation loss rates between 2-8 DAA were analyzed with a linear regression (Statistix 9, 2008; SAS 9.1.2, 2004) and all means were separated with a LSD at a 0.05 probability level. Ammonia loss was plotted vs irrigation rate, and fit to an exponential model (SigmaPlot, 2002). 17 RESULTS AND DISCUSSION Environmental Conditions Total precipitation at the study site was 9.6 mm with precipitation of 1.6, 0.6, 4.4, 1.2, and 1.8-mm on 3, 12, 19, 20, and 24 DAA respectively. Relative humidity fluctuated from 22 to 97% with an average of 65%. Air temperature varied between -4.9oC and 19.7oC with an average of 6.9oC. Soil temperature at 2.54 cm varied from 0.5oC to 17.9oC with an average of 7.8oC (Figure 2.1). Wind speeds varied from 0 to 12.2 m/s with an average of 2.4 m/s. Average weather was calculated from measurements taken every 15 minutes. Ammonia Volatilization Loss Ammonia loss was measured for each treatment starting 2 DAA (Figure 2.2). Nitrogen loss followed a linear trend between 2 DAA and 8 DAA when approximately 70% of treatment total loss occurred. The 0.0 mm irrigation rate lost 7.41% of N applied per day which was not different than the 6.63% N applied per day lost by the 1.25 mm irrigation rate. The 3.8 mm irrigation rate lost 4.71% of N applied per day which differed from all other treatments (p =0.05). The 7.6 mm irrigation rate also differed from all treatments with a loss of 1.89% of N applied per day. The 11.4 mm and 21.6 mm irrigation rate were not different from each other with losses of 0.59% and 0.15% of N applied per day, respectively. Ammonia loss starting at 8 DAA decreased and was not linear. The linear NH3 loss up to 8 DAA showed there was adequate soil moisture to hydrolyze the urea, irrespective of irrigation rate. No irrigation rate was able to totally prevent NH3 volatilization; however, irrigation was effective in minimizing the amount of daily NH3 loss and therefore total NH3 lost. The lowest cumulative loss of ammonia was associated with the highest irrigation rates of 11.4 and 21.6 mm (Figure 2.2) with 5.5% and 2. 8% of N applied respectively. These were lower than the 0.0 to 3.8 mm rates of irrigation (p = 0.05). The 7.6 mm irrigation rate lost 17.31% of N applied which was different from the 0.0 and 1.25 mm irrigation rates but not the 3.8, 11.4, or 21.6 rates (p = 0.05). The 0.00 mm irrigation rate lost the greatest amount of N as ammonia, 60.06% of N applied, but this was not different from the 1.25 and 3.8 mm irrigation 18 rates with 53.44% and 38.73% respectively (p = 0.05). The substantial ammonia loss with low irrigation reflects the failure of irrigation to move urea away from the granular site and into the soil, increasing ammoniacal-N in soil solution and surrounding pH (Burch and Fox, 1989). Ammonia loss from volatilization has been reported from 43-83% of N applied when urea was broadcasted on moist soil (Carmona et al., 1990; Grant et al., 1996; Kissel et al., 2009). The most NH3 was lost from treatments with low irrigation rates despite a low average soil temperature (7.8oC). Near-freezing temperatures have been shown to allow ammonia volatilization (Steenhuis et al., 1979), and can lead to large losses as NH3 can volatilize over a longer period of time (Sommer and Olesen, 1991). Vaio et al. (2008) attributed loss over a longer period for 68% of total NH3 loss (19%) from urea on tall fescue in the first month of a trial when the average temperature was 10oC. Lightner et al. (1990) found similar losses of 30-40% on orchard grass even though temperatures ranged from from 5 to 25oC. Plotting irrigation rate by total N loss as NH3 (Figure 2.3) yields the following equation (R2 = 0.9193): N Loss as NH3 (% N of applied) = 62.655e^ (-0.1559* irrigation rate (mm)) [3] Figure 2.3 demonstrates that when water is applied there is an immediate reduction in volatilization with increasing irrigation rate. Using the model to solve for 80% reduction in loss results in a need for 10.3 mm of irrigation, a 90% reduction in loss needs 14.8 mm of irrigation, and a 95% reduction needs 19.2 mm irrigation. This illustrates that as irrigation increases, volatilization decreases but with a diminishing return particularly at irrigation rates above 14.8 mm. Black et al. (1987) found an irrigation rate of 16 mm was enough to reduce NH3 loss to 2% which is similar to our 14.8 mm. Similar to this study, the irrigation was applied soon after application to a ryegrass and white clover pasture. Irrigations of 12-mm and 10-mm in another study were also found to reduce loss by over 50% (Marshall and Debell, 1980; Mundy, 1995). Black et al. (1987) found that irrigation was not effective after 48 hours as hydrolysis had already occurred. When Kissel et al. (2004) applied 24-mm rain immediately after application, they found less than 1% loss, compared to 5% when irrigation was applied at day 7 and losses of 49% and 58% when precipitation occurred on day 16 and 30, respectively. Holcomb and Horneck (2009) found similar results with losses of over 15% of N applied after 9-mm precipitation 5 days after application on two Kentucky bluegrass fields. This demonstrates that 19 irrigation or rainfall is most efficient at reducing loss when applied prior to urea hydrolysis; otherwise, ammonia volatilization loss still can be significant. Soil and Plant Analyses There was no difference in urease activity across treatments (p>0.05) and no trend with irrigation rate (p>0.05) (Table 2.1). Urease activity at the study site, 7.13 to 10.51 μg NH4-N g-1 h-1, were comparable to the lower values reported from nine Kansas soils, 9 to 71 μg NH4-N g-1 h-1 (Sullivan and Havlin, 1992) and lower than one soil in Washington, 63.9 μg NH4-N g-1 h-1 (Proctor et al., 2010). A visual increase in wheat vigor/growth was observed in plots receiving N compared to area of the field that received no additional N. The 0.00 mm irrigation had less wheat dry matter than the 3.8 mm rate (p<0.05). No differences in dry matter were measured between the remaining treatments (Table 2.1). There was no relationship between dry-matter and irrigation rate (p>0.05), most likely a result of collecting samples 23 DAA and slight differences in stand. The wheat matured from Feekes 5 to Feekes 7 by 23 DAA. At Feekes 7, the amount of N in the soil, even from the treatments that lost large amounts, the plant was not stressed for N. Average N in 0-30.4 cm soil profile across treatments was 135 kg ha-1. Dry matter or grain protein samples were not taken later in the season where supply effects may have been more observable. A difference in plant N concentration was measured, irrigation rates of 11.4 and 21.6 mm had higher N concentrations than the 0.0 mm (p<0.05) (Table 2.1). There is also a linear trend relating increased N concentration with increased irrigation rate (y=39.642+0.4134x; p < 0.05). Wheat N uptake differences were minimal with only the 3.8 mm irrigation having more N uptake than the 0.0 mm irrigation. Similar to the dry matter, there is no trend between irrigation and N uptake (p >0.05). A linear trend existed between N uptake and wheat dry matter (p<0.05) and there was no trend between wheat N concentration and N uptake (p>0.05). This suggests that wheat N uptake is dependent on wheat dry-matter, not wheat N concentration. There were no differences in pH at any depth between treatments at (data not shown), likely a result of pH samples taken 23 days after the application of urea. There may have been differences in pH at the surface between treatments if samples had been taken earlier in the 20 experiment. Eighteen days following a urea application, Ferguson et al. (1984) measured soil pH at or below original pH after an increase over 2 pH units the first 5 days after application. There was a difference across all treatments between the 1 inch and 6 and 12 inch (p<0.05). This is most likely from fertilizer applications that have been shown to decrease the surface pH of the soil due to acidification (Olson and Kurtz, 1982). Despite an average soil pH of 6.5 at 0-30 cm (pH 6 in upper 2.5 cm), large losses of ammonia occurred at this site. Fenn and Hossner (1985) have shown that buffering capacity can be more important than initial soil pH because pH increases markedly in response to alkaline inputs when soil buffering capacity is low. A poorly buffered soil, such as the sandy loam at this site, has the ability to rapidly increase pH temporarily resulting from a urea application (Hargrove, 1988). Whitehead and Raistick (1990) found an increase in pH from 5.5 and 6.1 to 7.5 and 7.9 resulting in ammonia losses of 22% and 36%. Similarly, Mundy (1995) found a pH increase over 2.5 pH units from 6.1 to over 8.5 after a urea application on moist soils. A temporary increase in pH could explain the large losses from the field as well as the uniform pH measured 23 days after application. CONCLUSIONS The use of a gradient of irrigation rates established an effective irrigation rate to minimize volatilization. Ammonia volatilization loss from urea ranged from 3 to 67 kg N ha-1 depending on irrigation rate; irrigation reduced loss by 7 to 64 kg N ha-1 based on rate. Increased irrigation rate decreased ammonia loss from volatilization. The decrease in volatilization resulted in an increase in wheat N concentration. A reduction of 90% in NH3 loss can be achieved by the application of 15 mm of irrigation, a savings of 61 kg N ha-1. Total NH3 loss from volatilization can be reduced by the addition of 8 mm irrigation and the addition of 11 mm irrigation can reduce the rate of ammonia loss during 2 – 8 DAA when loss from volatilization is greatest. Further irrigation will result in minor decreases in ammonia volatilization. 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Soils 11:43-47. 25 20 Air Temperature 2.54-cm Soil Temperature a) Temperature (oC) 15 10 5 0 -5 0 4 8 12 16 Days after application 20 24 14 b) Wind Speed Wind Speed (m/s) 12 10 8 6 4 2 0 0 4 8 12 16 Days after application 20 24 Figure 2.1. (a) Air temperature and soil temperature at 2.54-cm; and (b) wind speed measured every 15 minutes during the study period from 9 March to 2 April 2010. 26 70 A NH3-N loss (% N Applied) 60 A 50 0.0 mm Irrigation 40 AB 30 1.25 mm Irrigation 3.8 mm Irrigation 7.6 mm Irrigation 11.4 mm Irrigation 20 BC 21.6 mm Irrigation 10 C C 0 25 20 15 10 5 0 Days after Application Figure 2.2. Cumulative loss of NH3 during the period of 9 March to 2 April 2010 following application of 112 kg urea-N ha-1 to winter wheat as affected by rate of irrigation. Irrigation rates represent averages of irrigation applied as rates varied across plots. 27 NH3-N loss (% of N applied) 80 70 60 50 40 30 20 10 0 0 5 10 15 20 Irrigation Rate (mm) 25 30 Figure 2.3. Cumulative loss of NH3 during the period of 9 March to 2 April 2010 following application of 112 kg urea-N ha-1 to winter wheat as affected by rate of irrigation application. 28 Table 2.1. Soil urease activity from 0-2.54 cm soil depth, wheat dry matter, wheat N concentration, and wheat N uptake sampled 23 DAA. Irrigation Rate mm 0.0 1.25 3.8 7.6 11.4 21.6 LSD (0.05) Linear Quadratic Urease Activity μg NH4-N/(g h) 10.51 A † 10.01 A 9.37 A 7.13 A 8.66 A 7.70 A 1.81 NS NS Wheat Dry Matter kg/ha 3403.3 B † 4398.0 AB 4478.3 A 3986.1 AB 3807.4 AB 3636.4 AB 474.2 NS NS Wheat N g N/kg wheat 36.63 B † 41.00 AB 43.40 AB 43.73 AB 45.83 A 46.13 A 4.04 * NS Wheat N Uptake kg N/ ha 124.7 B † 179.2 AB 193.6 A 174.7 AB 172.9 AB 169.3 AB 24.75 NS NS †Within a column, values followed by the same letter are not significantly different according to LSD at P = 0.05. NS signifies no significant relationship with irrigation rate in a linear or quadratic relationship at p=0.05. * signifies a significant relationship with irrigation rate in a linear or quadratic relationship at p = 0.05. 29 UREASE INHIBITORS EFFECT ON AMMONIA VOLATILIZATION FROM UREA Jess C. Holcomb III, Donald A. Horneck, Dan M. Sullivan, and George H. Clough Soil Science Society of America Journal 5585 Guilford Road Madison, WI 53711 Publishing Date TBA 30 ABSTRACT When urea cannot be incorporated, urease inhibitors may be used to limit N loss from NH3 volatilization. The objectives of this study were to: (i) examine the effectiveness of urease inhibitors in minimizing NH3 loss on grass seed and wheat; (ii) measure interaction between urease inhibitors and differing irrigation rates; and (iii) measure urea hydrolysis with inhibitors. Volatilization loss was measured from urea, ammonium sulfate, and urea coated with the urease inhibitors using the modified passive flux method under differing irrigation rates. Urease inhibitors used were stabilized N-(n-butyl) thiophosphoric triamide (Agrotain) and an organoacid complex containing malic acid and copolymers (OAC). In the grass seed study Agrotain coated urea and ammonium sulfate reduced loss by 71.8% and 60.4% respectively compared to urea. In the wheat study, urea and OAC lost 53.44% to 60.05% of N applied at the 0.00 and 1.25 mm irrigation rate while Agrotain lost 5.72% to 6.24% of N applied. The addition of 7.6 mm irrigation reduced volatilization loss across N treatments to 17.31%, 8.11%, and 3.17% N applied for urea, OAC and Agrotain, respectively. In the wheat study, urease activity was inhibited 23 days after application of fertilizer in all Agrotain plots. In the incubation study, Agrotain delayed complete hydrolysis by 7 days at 26.7oC, 15 days at 16.6oC and 49 days at 4.4oC compared to OAC and urea, which hydrolyzed at the same rate. Agrotain is an effective way to inhibit urea hydrolysis and reduce N loss from NH3 volatilization when immediate incorporation is not possible or feasible. INTRODUCTION Urea is a widely accepted N fertilization source as it has a high N content (46%), and is low cost, easy to handle, and compatible with other fertilizer materials (Harre and Bridges, 1988; Kissel et al., 2009). Unlike other forms of N fertilizer, urea must be hydrolyzed before plant use. Hydrolysis of urea follows the reaction according to Kissel et al. (1988): urea + 2H2O +H+ urease 2NH4+ + HCO3further reacting as HCO3- + H+ CO2(g) + H2O and NH4+NH3 + H+ 31 The consumption of H+ in both reactions raises pH around the granular site (Zaman et al., 2008). Increased pH results in higher ammonia concentration which increases loss (Kissel et al., 1988). Ammonia loss associated with urea has been reported as high as 83% of N applied, but more typical loss has ranged from 15% to 40% of N applied (Lightner et al., 1990; Grant et al., 1996; Sommer and Ersboll, 1996; Ledgard, 1999; Martha Jr. et al., 2004; Vaio et al., 2008; Kissel et al 2009). Agriculture is responsible for an estimated 90% of anthropogenic ammonia emissions (Boyer et al., 2002). With 12% resulting from fertilizer application and the remainder from animal production (Ferm, 1998). Ammonia volatilization not only represents a loss in plant available N, but also an environmental pollutant. Up to 75% of NH3 that is volatilized is redeposited locally; however 25% can be transported long distances (Boyer et al., 2002), usually as secondary aerosol particles (Schjoerring et al., 1992). An aerosol is created by the reaction of NH3 with NOx and SOx which scatters light causing atmospheric haze (Ferm, 1998; Sharma et al., 2007). Cumulative inorganic N deposition in the Columbia River Gorge ranged from 1.09 kg ha-1 to 1.71 kg ha-1 in 19 weeks in the winter of 2003-2004(Fenn et al., 2007). Nitrogen is speculated to be originating in the Columbia Basin of Oregon and Washington from livestock operations and fertilizer applications. Nitrogen deposition favors nitrophilic organisms and suppresses organisms that are adapted to low N environments, altering native ecosystems far from the emission sites (Fenn et al., 2003; Geiser and Neitlich, 2007). This is evident in the Columbia River Gorge which has fewer lichen species that favor low N and two species of nitrophilic lichen which probably are not native to the Pacific Northwest (Gieser and Neitlich, 2007). Measuring NH3 loss has typically been conducted in a laboratory by placing soil and N fertilizer in a container and forcing air through an acid trap (Ernst and Massey, 1960; Stumpe et al., 1984; Ferguson and Kissel, 1986; Whitehead and Raistrick, 1990; Zhengping et al., 1991; Sommer and Ersboll, 1996). Since parameters are controlled in laboratory conditions, losses are hard to relate to the field. However, laboratory trials do provide valuable insight into ammonia loss parameters. The use of polyvinyl chloride (pvc) pipe inserted into the soil, temporarily capping the system and recording NH3 loss with acid traps enables relative loss analysis in the field (Keller and Mengel, 1986; Lightner et al., 1990). Allowing air movement by suspending the cap on this system allows daily collection of NH3 loss and can be totaled for a study period (Oberle and Bundy, 1987; Grant et al., 1996; Martha Jr. et al., 2004). These laboratory and field 32 techniques have limitations as they alter the environment by affecting air and soil temperature, precipitation, wind, and solar radiation and put into question the calculated loss compared to what which may actually occur in the field (Martha Jr. et al., 2004). Leuning et al.’s (1985) ammonia flux sampler allowed NH3 sampling at multiple heights with shuttles collecting ammonia loss without altering the environment. Schjoerring et al. (1992) used a similar method with four poles positioned at the edge of a circular plot with inexpensive glass samplers, but this required a large number of analyses. Wood et al. (2000) combined the two methods with one mast in the center with glass tube samplers which are inexpensive and simple to set up. This method has been used several times to measure NH3 loss in field conditions (Wood et al., 2000; Sullivan et al., 2003; Vaio et al., 2008; Holcomb III et al., In Review). To limit loss associated with NH3 volatilization, urea needs to be incorporated at least 5cm into the soil (Fenn and Miyamota, 1981). Urea can be incorporated to this depth mechanically or with 14.8 mm irrigation (Holcomb III et al., In Review). Urease inhibitors may be used to delay hydrolysis if urea cannot be incorporated after application. Agrotain International, LCC (St. Louis, MO) markets a urease inhibitor, Agrotain, with stabilized N-(n-butyl) thiophosphoric triamide (NBPT) that can be applied to both urea and urea ammonium nitrate (UAN or Solution 32) and has been reported to reduce NH3 loss (Carmona et al., 1990; Zhengping et al., 1991; Grant et al., 1996; Sanz-Cobena et al., 2008; Zaman et al., 2008; Zaman et al., 2009). NBPT forms a tridentate ligand with urease (Manunza et al., 1999), which slows the hydrolysis of urea. By slowing hydrolysis, H+ is not rapidly consumed which allows soil to buffer pH without much change (Christianson et al., 1993; Blossfeld et al., 2009; Zaman et al., 2009). This results in a more moderate pH and a lower concentration of NH4 in soil solution which reduces chances for volatilization (Zaman et al., 2008). Although there has been research on the use of Agrotain and other urease inhibitors, studies on a field scale are limited. The objectives of this study were to: (i) determine the effectiveness of different urease inhibitors for lowering ammonia volatilization without irrigation; (ii) determine the effect of irrigation rate on urease inhibitors; and (iii) account for urea hydrolysis with urease inhibitors. 33 MATERIALS AND METHODS Grass Seed Study The grass seed study consisted of two center-pivot irrigated 50-ha burned Kentucky bluegrass fields in Umatilla County near Echo, OR. The first field had a soil classified as a Quincy loamy sand (Mixed, mesic Xeric Torripsamments) with a pH of 6.5 and the second field consisted of two soils, one classified as an Adkins fine Sandy loam (coarse-loamy, mixed, superactive, mesic Xeric Haplocalcids) and one a Quincy loamy sand with a field pH of 5.9. Treatments were arranged in a randomized complete block design with three replications. Treatments included urea, ammonium sulfate and urea coated with Agrotain (5.21 L Agrotain/Mg urea). Each N treatment consisted of a circular (30 m diameter) plot with N fertilizer surface applied at 112 kg N ha-1. Each plot was separated by at least 100 m to avoid contamination of NH3 between treatments. Fields were pre-watered with 25.4 mm irrigation to incorporate prior N applications and raise soil to field capacity. Loss from ammonia volatilization was measured immediately after application using the modified passive flux method (Wood et al., 2000; Vaio et al., 2008), which consisted of a rotating mast placed at the center of each plot. A tripod which did not interfere with rotation of the mast was placed on the mast in order to add stabilization during high winds. Each mast was equipped with a passive flux sampler at five heights (0.45, 0.75, 1.50, 2.25, and 3.00 m; Leuning et al., 1985). Each passive flux sampler consisted of a glass tube (0.7 cm i.d. by 20 cm long) with the inside surface coated with 3% w/v oxalic acid in acetone to trap the NH3 in the air flowing through the tube. A nozzle with a 1 mm hole to restrict air flow was attached to the flux sampler. Identical background masts were placed around the field to measure ambient NH3. Background masts were placed over 100 m from treatments to protect against contamination. Most background NH3 levels were near zero. Flux samplers were replaced 1, 2, 3, 4, 5, 6, 8, 10, 12, and 15 days after fertilizer application (DAA). Samplers were extracted by adding 2 ml deionized water and shaken for 10 minutes with extracts analyzed colorimetrically for NH4 (Sims et al., 1995). Horizontal NH3 flux (Fx, μg N m-2 s-1) for each flux sampler was calculated by [1]: Fx = (CV)/(πr2KΔt) [1] 34 where C is the concentration of NH4-N (μg N/mL) in deionized water used to extract sorbed NH4N, V is the volume of deionized water used for extraction (2 mL), r is the radius of the hole in the disc on the nozzle (0.0005 m), K is a correction factor (0.77), and Δt is the time during which the sampler was exposed (s) (Schjoerring et al., 1992; Wood et al., 2000; Vaio et al., 2008). Net horizontal flux for each sampler (Fx,p) was determined by subtracting horizontal flux from the corresponding sampler height on the background mast (Fx,b). Net vertical flux (Fy, ug N m-2 s-1) from each plot was estimated by integrating each horizontal flux with vertical distance for each sampler accounted for [2]: Fy=(1/R)Σ(Fx,p-Fx,b)Δh [2] where R is the radius of the plot (15 m), and Δh (m) is the vertical distance corresponding to each sampler. An Adcon Telemetry (Klosterneuburg, Austria) weather station was placed at the study area to measure air temperature, soil surface temperature, humidity, rainfall, wind speed, and wind direction with measurements taken every 15 minutes. Wheat Study The wheat study was conducted in a center pivot irrigated 50 ha wheat field in Umatilla County near Echo, OR. The soil was classified as an Adkins fine sandy loam with an average pH of 6.5 (0-30 cm). The field was arranged in a split-plot design with 20o irrigation wedges of approximately 2.8 ha. Three N treatments, urea, urea coated with Agrotain (5.21 L Agrotain/ton urea), and urea coated with an Organo-Acid Complex containing malic acid and copolymers (OAC) were surface applied to circulare (30 m diameter) plots at 112 kg N ha-1 (Figure 3.1). Wedges received 0.0, 1.25, and 7.6 mm of overhead irrigation following treatment application. A rain gauge was placed within each treatment wedge to record the amount of irrigation applied. Loss from ammonia volatilization was measured using the same method as the grass seed study, except flux samplers were replaced 2, 3, 4, 5, 6, 7, 8, 10, 13 15, 17, and 24 DAA. Along with the weather station in the field, Sentek Enviroscan (Stepney Australia) moisture probes were placed in the 0.0, 3.8 and 11.4 mm irrigation rate plots (not replicated) in block 1 to measure soil moisture at the 10.1, 20.3, 30.4, 50.8, and 91.4 cm depths. 35 Soil samples were taken from each treatment at depths of 0-2.5, 0-15.2, and 0-30.4 cm at 23 DAA. Soil samples were extracted with 2 M KCl (1:10 soil/KCl) and extract analyzed colormetrically for NH4-N and NO3-N (Sims et al., 1995). The pH for each soil sample was analyzed in a 1:1 soil/water slurry (McLean, 1982). Urease activity was analyzed for the 0-2.5 cm depth soil samples according to Torello and Wehner (1983). Two 2-g soil samples from each treatment were incubated for 5-hours in a phosphate buffer and urea solution, with one sample inhibited by AgSO4 during the incubation. After incubation KCl was added to both soils and AgSO4 was added to the uninhibited control soil, then shaken for 1 hour. Solutions were filtered through a Whatman No. 1 filter paper and analyzed colorimetrically for NH4-N (Sims et al., 1995). Net urease activity was calculated by subtracting the treatment value from the uninhibited control value and expressed as μg NH4-N g-1 h-1. Wheat plants were randomly sampled from within each treatment (0.126 m2) at 23 DAA. Above ground dry matter was measured and total N was analyzed using the total N combustion method (Gavlak et al., 2003) with an Elementar Vario Max CN analyzer (Hanau, Germany). Incubation Study Soil (Adkins coarse-loamy, mixed, superactive, mesic Xeric Haplocalcids, pH = 7.0) at field capacity was collected from a winter wheat field at the Hermiston Agricultural Research and Extension Center in Hermiston, OR to a depth of 30 cm. Soil was homogenized and subsamples of 0.65 kg of soil (roughly 0.5 kg dry soil) were placed into gallon Ziploc™ Freezer bags. Urea, Agrotain, OAC and a control were incubated at 4.4OC, 15.6 OC and 26.7OC. Each treatment contained about 1.05 g N kg-1 soil (variation due to adding whole prills), applied to the soil in Ziploc™ bags and thoroughly mixed. A drinking straw, to insure aerobic conditions, was inserted into each bag which was then zipped shut around the straw. At 1, 3, 6, 13, 20, 28, 34, 48, 63, 76, and 104 DAA of N, bags were thoroughly remixed, then subsamples were collected (5 g soil for N analysis and 10 g soil for water content and pH). Gravimetric soil moisture was determined by drying at 60OC. Soil pH was measured in a 1:1 dry soil/water slurry (McLean, 1982). Soil N was analyzed by adding 50 mL 2 M KCl solution to the 5 g wet soil sample and shaking for 1 hour on an oscillating shaker. The solution was passed through Whatman No. 1 36 filter paper (Keeney and Nelson, 1982) and extracts were analyzed colorimetrically for NH4-N (Sims et al., 1995). Statistical Analyses Ammonia loss and soil and plant response data were analyzed via analysis of variance (SAS Institute Inc., 2004; Statistix 9, 2008). Daily loss rates for the grass seed and wheat trial were analyzed via linear regression (Statistix 9, 2008) and means separated by LSD at a 0.05 probability level. RESULTS AND DISCUSSION Field studies were conducted on acid soils. The wheat field had a pH of 6.5 and the grass seed fields had 6.5 and 5.9 pH. Despite low soil pH, loss of NH3 in all fields exceeded 15% of N applied with the larger loss on the wheat field. Soil pH has been shown to be less important than soil buffering capacity, as low buffered soils can have large pH swings (Fenn and Hossner, 1985). Temporary pH increases from urea hydrolysis helps explain field NH3 loss. Increased pH results in a higher ammonia concentration which increases loss. A temporary pH increase explains why no pH differences were measured across treatments in the wheat study after 23 DAA. Sandy soils have low pH buffering capacity allowing a rapid temporary pH increase resulting from urea hydrolysis (Hargrove, 1988). A pH increase from 5.5 and 6.1 to 7.5 and 7.9 was found by Whitehead and Raistrick (1990) with 22-36% NH3 loss. A similar increase of 2.5 pH units after a urea application on moist soils from 6.1 to 8.5 was found by Mundy (1995). Ammonia loss was measured despite low air and soil temperatures at all three locations. The wheat study had an average soil temperature of 7.8oC while the grass seed study was 10.1oC. Sommer and Olesen (1991) found that NH3 loss can occurs at near freezing temperatures from volatilization occurring over a longer period of time than at warmer temperatures. Steenhuis et al. (1979) measured loss occurring at near freezing temperatures. Loss of 19% urea applied was measured by Vaio et al. (2008) with an average air temperature of 10oC. 37 Grass Seed Study Precipitation totaled 18.6 mm with rainfall of 0.4, 9.0, 4.4, and 4.8 mm on 4, 5, 6, and 15 DAA, respectively. Relative humidity fluctuated between 7% to 95% averaging 54%. Air temperature varied between -5.2oC and 24.4oC averaging of 7.8oC (Figure 3.2). Soil temperature at 2.54 cm varied from 0.9oC to 21.5oC averaging of 10.1oC. Wind speeds varied from 0 to 8.33 m/s averaging of 1.7 m s-1. Since ammonia loss was not significantly different between fields (data not shown), the results are averaged across both fields. Ammonia loss began immediately after application, and cumulative loss increased until 10 DAA (Figure 3.3). After 10 DAA loss from treatments virtually ceased. Percent of N applied lost averaged 15.4, 6.1, and 4.3% for urea, ammonium sulfate, and Agrotain, respectively. Final cumulative N loss was similar for ammonium sulfate and Agrotain (p<0.05). Ammonium sulfate represented a 60.4% reduction in N loss compared to urea and Agrotain represented a 71.8% reduction. Although cumulative loss between Agrotain and ammonium sulfate did not differ, average daily loss from 1 to 15 DAA was different (p=0.08). Agrotain loss was 0.356 kg N ha-1day-1 (r2 = 0.973), while loss from ammonium sulfate was 0.444 kg N ha-1day-1 (r2=0.903). Unlike urea, ammonium sulfate does not hydrolyze so pH does not increase temporarily. Without the pH increase from hydrolysis, NH4 would be the dominant form thus decreasing loss (Fenn and Hossner, 1985). Zhengping et al. (1991) found a loss of 18.8% with urea and less than 3% using the active ingredient for Agrotain NBPT, a reduction of 84%. In that incubation study, however, the N was mixed into the soil, so N loss may have been greater had it been left on the soil surface. Ammonia loss increased after precipitation on Days 4, 5, and 6. All N sources increased loss on 4 DAA after the first precipitation event (Figure 3.3). Prior to precipitation on 4 DAA, prills were still visible for all N treatments. This suggested that there was not enough soil moisture or relative humidity to completely dissolve the prills. Relative humidity for the first four days averaged 18% with average air temperature of 12oC. The lack of water inhibited the diffusion of urea to urease for hydrolysis (Ferguson and Kissel, 1986). Nitrogen fertilizers did not completely dissolve even though the field was irrigated with 2.54 cm two days prior to N application. The surface had dried enough to hinder urea dissolution and subsequent hydrolysis. Soil moisture, humidity, and temperature were adequate at application to allow 38 some prill dissolution and hydrolysis as NH3 loss did occur prior to precipitation on 4 DAA. This agrees with Stumpe et al. (1984) who reported that decreasing initial soil water content decreased volatilization, as a result of delayed dilution and urea hydrolysis. Precipitation of 0.4 mm, on 4 DAA provided adequate water for hydrolysis but was inefficient for moving urea into the soil resulting in increased NH3 loss, as also observed by Craig and Wollum II (1982). The 9 mm of precipitation 5 DAA should have slowed future volatilization as incorporation should decrease NH3 loss. However, partial urea hydrolysis had already occurred prior to this event. Because of its charge, NH4+ moves slower than urea through soil, so even with precipitation, hydrolysis products remained close to the surface enabling further ammonia loss (Wagenet et al., 1977). Zaman et al. (2009) found complete urea hydrolysis delayed by 1-2 weeks with Agrotain. This helps explain the reduction in NH3 loss with Agrotain. Agrotain treated urea was not hydrolyzed and it moved into the soil with the precipitation on 4, 5, and 6 DAA. With urea incorporated, NH3 loss was minimal. Wheat Study Precipitation totaled 9.6 mm with rainfall of 1.6, 0.6, 4.4, 1.2, and 1.8 mm on 3, 12, 19, 20, and 24 DAA, respectively. Relative humidity fluctuated between 22% to 97% averaging 65%. Air temperature varied between -4.9oC and 19.7oC averaging of 6.9oC. Soil temperature at 2.54 cm ranged from 0.5oC to 17.9oC averaging 7.8oC (Figure 3.4). Wind speeds varied from 0 to 12.2 m/s averaging 2.4 m/s. Similar to the grass seed study, loss started soon after application with little loss after 10 DAA. Unlike the grass seed study, prills melted prior to the first sampling date at 2 DAA. Precipitation of 1.6 mm on 3 DAA did not affect daily loss rates as they remained linear from 2-8 DAA. Daily loss rates from 2-8 DAA with 0.00 mm irrigation for urea and OAC did not differ from each other at 8.30 and 8.36 kg N ha-1day-1, respectively while Agrotain’s daily loss rate at 0.54 kg N ha-1day-1 was lower than urea and OAC. With 1.25 mm irrigation, daily N loss from 2-8 DAA was again similar for urea and OAC at 7.43 and 8.05 kg N ha-1day-1, respectively and Agrotain’s daily loss of 0.35 kg N ha-1day-1 was less than urea and OAC. Daily N loss rates from 2-8 DAA with 7.6 mm irrigation was highest with urea (2.11 kg N ha-1day-1), intermediate with OAC (1.05 kg N ha-1day-1), and lowest with Agrotain (0.34 kg N ha-1day-1). 39 When comparing daily N loss from 2-8 DAA across irrigation rates, urea and OAC with 0.0 mm and 1.25 mm irrigation had the highest and similar rate of daily N loss. Agrotain did not differ across irrigation rates and had the lowest daily N loss from 2-8 DAA. OAC with 7.6 mm irrigation had higher daily N loss than Agrotain treatments but lower than urea with 7.6 mm irrigation. Urea with 7.6 mm irrigation had lower daily N loss from 2-8 DAA than urea and OAC with 0.0 mm and 1.25 mm irrigation. Agrotain reduced daily N loss from 2-8 DAA regardless of irrigation rate. OAC reduced daily N loss rate only with 7.6 mm irrigation, with rates similar to urea at 0.0 and 1.25 mm irrigation. Nitrogen loss as NH3 from N treatments across irrigation rates and sampling dates followed a similar trend, with the majority of loss occurring before 10 DAA (Figure 3.5). Final cumulative NH3-N loss from N treatments across irrigation rates was greatest for urea and OAC at 0.00 and 1.25 mm irrigation. All other treatments had lower final loss and did not differ from each other but N treatment and irrigation interacted significantly (p<0.05). At 0.0 mm irrigation, Agrotain’s final N loss was 5.72% of N applied, significantly less than 59.1% and 60.1% for OAC and urea, respectively (Figure 3.6). There was no difference between urea and OAC. Agrotain at 1.25 mm irrigation had a final cumulative N loss of 6.2% compared to 53.4% and 55.4% for urea and OAC, respectively, a reduction of 88.3% compared to urea. However, at 7.6 mm irrigation, Agrotain’s and OAC’s final cumulative loss did not differ at 3.17% versus 8.11%, respectively. Both Agrotain and OAC had a lower N loss than urea at 17.31% of N applied. Agrotain reduced final loss by 81.6% and OAC by 53.1% compared to urea. When N is at the soil surface (0.00 mm irrigation) or near the surface (1.25 mm irrigation) Agrotain reduces N loss from NH3 more effectively than OAC. Agrotain also had less loss than OAC at 7.6 mm irrigation but it was not significant. The difference in volatilization loss between Agrotain and urea with 0.00 mm irrigation was similar to the findings of Carmona et al. (1990) who reported a reduction of 82.6-95% using the active ingredient of Agrotain (NBPT) compared to urea with loss of 2.329.4% and 54%, respectively. However, this was conducted under laboratory conditions. Grant et al. (1996) measured a reductions in volatilization loss of 85.2% and 93.9% when using the active ingredient of Agrotain (NBPT) compared to urea (12.32% and 2.32% versus 83% and 38%, respectively) in Canadian prairies. There was no irrigation effect on soil urease activity at 0-2.5 cm soil depth (Table 3.1). Urease activity differed significantly between products, ranging from 4.85 μg NH4-N g-1 h-1 for 40 Agrotain to 9.20 μg NH4-N g-1 h-1 for urea and 11.85 μg NH4-N g-1 h-1 for OAC. Why OAC increased urease activity compared to urea is not known. Urease activity reduction with Agrotain is a result of the urease inhibiting characteristic of its active ingredient, NBPT. Urease activity ranged from 0.90 to -2.59 μg NH4-N g-1 h-1, which are comparable to the lower values reported for Kansas soils 9-71 μg NH4-N g-1 h-1 (Sullivan and Havlin,1992) and a lower than a Washington soil 63.9 μg NH4-N g-1 h-1 (Proctor et al., 2010). There was a visible increase in wheat stand/vigor and color in fertilized plots compared to the remainder of the field which received no additional N. Neither N treatments nor irrigation rate affected wheat dry matter (Table 3.1). This is likely the result of the whole field being fertilized one week prior to our treatment applications, collecting samples only 23 DAA, and observable differences in the stand density. Wheat growth progressed from Feekes 5 at application to Feekes 7 at 23 DAA. Wheat at Feekes 7 would not have been stressed for N, even treatments where 60% of N was lost, since average soil N at 23 DAA from the 0-30.4 cm depth was 118.8 kg N/ha across the field. Wheat protein at harvest may have differed but this was not measured as part of our objectives. Wheat N concentration was not affected by N treatment or irrigation but the interaction between N treatment and irrigation rate was significant at (Table 3.1). Increased irrigation rates led to increased wheat N concentration when urea and Agrotain were applied. This is likely a result of urea losing upward of 60% N through volatilization at low irrigation rates, however OAC would be expected to have a similar concentration as it lost a similar amount of N. Although Agrotain lost less N through volatilization, Agrotain may still have been inhibiting urease which would keep some of the N from being plant available. This may explain the lack of N concentration increase in the plant. There was no difference between N treatment, irrigation rate, or an interaction between N treatment and irrigation rate for wheat N uptake (Table 3.1). Soil pH was not affected by N treatment or irrigation rate (data not shown). The lack in pH difference is a result of sample collection date (23 DAA). After 18 days following a urea application Ferguson et al. (1984) measured soil pH at or below original pH after an increase over 2 pH units the first 5 days after application. Agrotain would be expected to resist this initial pH increase as Agrotain extends the hydrolysis period therefore allowing the soil to buffer the H+ consumption. Zaman et al. (2009) measured slow hydrolysis of Agrotain, limiting consumption of H+ and increased pH. 41 OAC had a larger fraction of pellets greater than 4 mm (data not shown) which may lead to a larger loss of NH3 from the presence of a higher concentration of urea in a smaller area. Incubation Study At 4.4oC, urea and OAC were completely hydrolyzed at 13 DAA (Figure 3.7). Agrotain delayed complete hydrolysis until 63 DAA. At 16.6oC urea and OAC were completely hydrolyzed at 6 DAA while Agrotain was not completely hydrolyzed until 28 DAA. At 26.7oC OAC was completely hydrolyzed by 6 DAA, while urea and Agrotain were completely hydrolyzed at 13 and 20 DAA, respectively. At all three temperatures urea and OAC followed similar rates of hydrolysis suggesting that OAC has no urease inhibition properties. Although OAC is not an effective urease inhibitor it reduced NH3 loss at 7.6 mm irrigation compared to urea. It is not known why OAC decreased loss after incorporation with irrigation. Agrotain delayed complete hydrolysis at each temperature compared to urea and OAC. NBPT is a known urease inhibitor (Manunza et al., 1999). There was an effect of temperature on hydrolysis and an interaction between temperature and N treatment (p<0.05). Increased incubation temperature for all products led to increased hydrolysis rates (P<0.05), therefore increased rate of NH4 formation. Although urea and OAC were both completely hydrolyzed by 13 DAA at all temperatures, there were differences with hydrolysis prior to 13 DAA. Agrotain at lower temperatures led to a longer delay in hydrolysis compared to higher temperatures. This may warrant examining lowering rates of Agrotain when used at low temperatures to meet desired hydrolysis delays. CONCLUSIONS Agrotain reduced ammonia volatilization loss. Agrotain reduced N loss by 71.8% in the grass seed study compared to urea, 4.3% versus 15.3% of N applied respectively. Ammonium sulfate reduced loss to 6.07% of N applied in the grass seed study. In the wheat study, ammonia loss from urea, OAC, and Agrotain ranged from 17.3-60.0%, 8.1-59.0%, and 3.1-6.2% depending on irrigation rate, respectively. Agrotain reduced loss regardless of irrigation rate unlike urea and OAC which relied on irrigation application to decrease volatilization. Agrotain reduced urease activity in the irrigation study. During incubation, Agrotain delayed complete hydrolysis 42 by 49 days at 4.4oC, 15 days at 16.6oC, and 7 days at 26.7oC compared to urea. Urea and OAC hydrolyzed at similar rates at all incubation temperatures. Agrotain is an effective urease inhibitor and can reduce ammonia volatilization loss if urea cannot be incorporated. ACKNOWLEDGEMENTS Agrotain International and the J.R. Simplot Company provided financial support for this project. 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Effect of urease inhibitors on urea hydrolysis and ammonia volatilization. Biol. Fertil. Soils 11:43-47. 47 Figure 3.1. Infrared photo of wheat field displaying layout of irrigation study. Irrigation rates are randomly selected within each block. Within an irrigation rate, N treatment plots are the bright red circles with a diameter of 30 meters (The “T” in Block 3 with arrows is pointing to N treatments in the 0.00 mm irrigation rate). The “B” in Block 3 is the approximate location of a background mast, background masts in Blocks 1 and 2 are beyond the scope of the image. 48 25 Air Temperature 2.5 cm Soil Temperatue a) Temperature (oC) 20 15 10 5 0 -5 0 2 4 6 8 10 12 14 16 Days after application 9 Wind Speed b) 8 Wind Speed (m/s) 7 6 5 4 3 2 1 0 0 2 4 6 8 10 12 14 16 Days after application Figure 3.2. (a) Air temperature and soil temperature at 2.54-cm, soil temperature data before 4 DAA was lost; and (b) wind speed measured at the grass seed fields. Data were measured every 15 minutes during the study period from 28 September to 13 October 2009. 49 18 Urea 16 Ammonium Sulfate Agrotain NH3-N loss (% of N applied) 14 12 10 8 6 4 2 0 16 14 12 10 8 6 4 2 0 Days after application Figure 3.3. Cumulative loss of NH3 during the period of 28 September to 13 October 2009 following application of 112 kg N/ha to Kentucky bluegrass as affected by N source. Bars represent standard error. 50 20 Air Temperature 2.54-cm Soil Temperature a) Temperature (oC) 15 10 5 0 -5 0 4 8 12 16 20 24 Days after application 14 b) Wind Speed 12 Wind Speed (m/s) 10 8 6 4 2 0 0 4 8 12 16 20 24 Days after application Figure 3.4. (a) Air temperature and soil temperature at 2.54-cm; and (b) wind speed measure at the wheat field. Data were measured every 15 minutes during the study period from 9 March to 2 April 2010. 51 70 Urea + 0.0 mm Irrigation A A A A N Loss as NH3 (% of N applied) 60 Urea + 1.25 mm Irrigation Urea + 7.6 mm Irrigation 50 Agrotain + 0.0 mm Irrigation 40 Agrotain + 1.25 mm Irrigation 30 Agrotain + 7.6 mm Irrigation 20 B 10 B B B B 0 0 5 10 15 20 Days after application OAC + 0.0 mm Irrigation OAC + 1.25 mm Irrigation OAC + 7.6 mm Irrigation 25 Figure 3.5. Cumulative loss of NH3 during the period of 9 March to 2 April 2010 following application of 112 kg N ha-1 to winter wheat as affected by N and irrigation rate treatments. Treatments followed by the same letter are not significantly different according to LSD at P = 0.05. 52 0.00 mm Irrigation 70 A A N Loss as NH3 (% of N Applied) 60 1.25 mm Irrigation 70 60 A A 50 40 40 40 30 30 30 20 20 20 10 10 0 B 0 0 5 10 15 20 25 Days After Application Urea Urea+ 7.6 mm Irrigation NBPT + 7.6 mm Agrotain Irrigation OAC OAC+ 7.6 mm Irrigation 60 50 B 7.60 mm Irrigation 70 50 A 10 B B 0 0 5 10 15 20 25 Days After Application 0 5 10 15 20 25 Days After Application Figure 3.6. Cumulative loss of NH3 within irrigation rates for the period of 9 March to 2 April 2010 following application of 112 kg N ha-1 to winter wheat for urea, Agrotain, and OAC. Treatments followed by the same letter are not significantly different according to LSD at P = 0.05. 53 160 Urea Net NH4-N Produced (% of N applied) 140 Agrotain OAC a) 120 100 80 60 40 20 0 0 10 20 Agrotain OAC 30 40 50 60 70 160 Urea b) Net NH4-N Produced (% of N applied) 140 120 100 80 60 40 20 0 0 10 20 30 40 50 60 70 Net NH4-N Produced (% of N applied) 160 Urea 140 Agrotain OAC c) 120 100 80 60 40 20 0 0 10 20 30 40 Days after application 50 60 70 Figure 3.7. Net NH4-N from fertilizer, as affected by N treatment at incubation temperature (a) 4.4oC, (b) 16.6oC, and (c) 26.7oC. Bars represent standard error. 54 Table 3.1. Wheat response and soil urease activity (0-2.5 cm) as affected by N treatment and irrigation rate. Wheat and soil samples were taken at 23 DAA. N Treatment Irrigation Rate Urease Activity -1 -1 Wheat Dry Matter kg / ha mm µg NH4-N g h Urea 0.00 10.51 3403.3 Agrotain 0.00 5.29 OAC 0.00 Urea Wheat N Concentration Wheat N Uptake g N / kg wheat kg N / ha 124.7 4499.0 36.63 C† 42.33 B 191.9 10.57 4253.0 42.30 B 179.9 1.25 10.01 4398.0 41.00 BC 179.2 Agrotain 1.25 4.70 3773.7 40.16 BC 151.1 OAC 1.25 12.02 3566.5 42.26 B 151.5 Urea 7.6 7.13 3986.1 43.73 AB 174.7 Agrotain 7.6 4.48 3820.4 47.33 A 183.2 OAC Irrigation 7.6 12.94 NS 4309.9 NS 41.33 BC NS 177.7 NS N Treatment * NS NS NS Interaction NS NS * NS †Within a column, values followed by the same letter are not significantly different according to LSD at P=0.05. * signifies a significant relationship at p = 0.05. NS signifies no significant relationship at p=0.05. 55 EFFECT OF SPECIALTY NITROGEN FERTILIZERS ON RUSSET BURBANK AND RUSSET NORKOTA POTATO YIELD IN THE COLUMBIA BASIN Jess Charles Holcomb III, Donald A. Horneck, Dan M. Sullivan, and George H. Clough Styled according to Soil Science Society of America Journal 5585 Guilford Road Madison, WI 53711 56 ABSTRACT Enhanced efficiency nitrogen (N) fertilizers may limit N loss into the environment, however they must also maintain or increase yield in order to be viable. This study was conducted to: (i) examine whether these fertilizers could maintain or increase yield in Russet Burbank and Norkota potatoes; (ii) whether petiole NO3 accurately reflects plant N concentration with these products; and (iii) whether they released N in accordance to plant demand. A three year field study was conducted at the Hermiston Agricultural Research and Extension Center to compare yields with grower standard practice (GSP). An incubation study was conducted with fertilizers at 4.4oC, 15.6oC, and 26.7oC for 104 days, measuring rate of NH4 and NO3 formation. No yield difference was measured between GSP and N treatments with Russet Norkota. Russet Burbank yields were lower than GSP for two years and similar for one year. Yields for N treatments were similar to 80% GSP suggesting that N availability is limited with these products. Petiole NO3 cannot be used with some N treatments, as some inhibit NO3 formation and therefore NO3 uptake. All N products were affected by temperature in the incubation study. Increased temperature led to increased NH4 and NO3 availability. No difference was measured between Nutrisphere-N and urea for the formation of NH4 and NO3. Nitamin and N-fusion only had 100% available N at 26.7oC after 104 days. Enhanced efficiency N fertilizers cannot sustain or increase yields on a yearly basis on Russet Burbank and are not economically viable as a result. INTRODUCTION In the western United States, irrigated potatoes (Solanum tuberosum) is a crop of major economic importance, with production dominating several heavily productive areas (Taysom et al., 2007). These are typically on sandy soils that are N limiting, so N must be added as potatoes contain more N and K than any other nutrient (Errebhi et al., 1998; Westermann, 2005). Applications of at least 340 kg N/ha are typical and usually represent one of the more expensive parts of production (Lauer, 1985; Ojala et al., 1990). Nitrogen is often over-applied to ensure against N deficiency and yield loss (Kleinkopf et al., 1981; Waddell et al., 1999). Typical N use efficiency (NUE) ranges from 28% to 56% of N applied depending on environmental conditions 57 (Westermann et al., 1988; Joern and Vitosh, 1995; Errebhi et al., 1998). Low NUE results from potatoes having a shallow rooting depth with up to 90% of their roots in the surface 23-38 cm of soil (Asfary et al., 1983; Yamaguchi and Tanaka, 1990; Joern and Vitosh, 1995). The large irrigation demand of potatoes combined with sandy soils results in NO3-N being leached below the rooting zone (Singh and Sekhon, 1976; Prunty and Greenland, 1997; Shock et al., 2007). As a result, the typical practice in the region is to add a small amount of N at preplant and then split applications of N through fertigation based on petiole NO3-N concentration (Meyer and Marcum, 1998; Zomuya and Rosen, 2001; Taysom et al., 2007). Split applications increase nitrogen use efficiency (NUE) as less NO3 is available for leaching at any given moment and N remains in the root zone for longer periods of time (Singh and Sekhon, 1976; Elkashif et al., 1983; Lauer, 1985; Lauer, 1986; Westermann et al., 1988; Vos, 1999). This practice, however, can be labor intensive and costly (Taysom et al. 2007). Nitrogen management is critical for potatoes as deficient N can reduce canopy growth, resulting in premature senescence, reduced yields, and less US #1’s (Taysom et al., 2007; Zebarth and Rosen, 2007). Excessive N can delay tuber initiation and slow bulking in favor of vegetative growth, reduce yield, and decrease tuber specific gravities (Lauer, 1985; Westermann et al., 1985; Ojala et al., 1990; Biemond and Vos, 1992; Errebhi et al., 1998; Taysom et al., 2007). Fluctuating N from low to high in-season can result in irregular growth leading to misshapen tubers and internal damage (Taysom et al., 2007). Defects are important since processors pay premiums for potatoes with good symmetry, free of defects and abnormalities, and higher specific gravities (Zomuya and Rosen, 2001; Shock et al., 2007). Loss of N affects environmental quality as well as agronomics. Loss of N into the environment results from NO3 leaching, NH3 volatilization, and loss of N2O. Leaching represents the majority of loss, followed by volatilization, and N2O loss is negligible (Zebarth and Rosen, 2007). Leaching of NO3 is the biggest concern in potato production as NO3 is easily lost on well drained sandy soils (Jones and Wagner, 1995; Ryker and Jones, 1995). Loss from NO3 also is important after harvest because potatoes leave large amounts of N in residue that is readily mineralized which can leach, especially if the field is not followed by a crop (Goulding, 2000; Peralta and Stockle, 2001; Honisch et al., 2002). Random surveys in the Columbia Basin show that 30 to 33% of wells tested had NO3 levels above EPA standard of 10 ppm (Alva et al., 2002). 58 Ammonia volatilization loss can range from 15 to 40% N applied depending on field conditions (Lightner et al., 1990; Grant et al., 1996; Sommer and Ersboll, 1996; Ledgard et al., 1999; Martha Jr. et al., 2004; Vaio et al., 2008; Kissel et al., 2009). Although volatilization loss can be large, most N applications on potatoes in the Columbia Basin are applied by fertigation which should limit volatilization loss. Irrigation should move N into the soil where volatilization risk is minimized, however this has not been verified. Nitrous oxide production is an intermediate product formed in the denitrification process and increases with N applications and saturated soils leading to anaerobic environments (Mosier, 1998; Zebarth and Rosen, 2007).The loss of N2O from soils is not agronomically important on aerated soils. Loss on most crops is typically low, with maximums of 2% with most below 1% N applied, however this work was not done on potatoes (Delgado and Mosier, 1996; Shoji et al., 2001). Research on potatoes has demonstrated loss ranging from 2.77% up to 4.8% N applied as N2O during the growing season (Ruser et al., 2001). This research was conduct on a silt loam soil which unlike sands are aerated thus N2O loss may be less. Although loss is small, agriculture is estimated to account for over 75% of anthropogenic N2O (Isermann, 1994; Ruser et al., 2001). Enhanced Efficiency Fertilizer’s (EEF’s) are fertilizers that reduce loss to the environment and/or increase nutrient availability compared to conventional fertilizers (Olson-Rutz et al., 2009). Typically EEF’s either inhibit an N conversion pathway or gradually release N. For example, the use of an inhibitor on the urease enzyme slows hydrolysis while reducing volatilization loss. Another example, inhibiting nitrification leaves N as NH4 which is less susceptible to leaching (Vos, 1994). The gradual release of N from slow release fertilizer is from microbial breakdown releasing N (Olson-Rutz et al., 2009). Controlled release fertilizers (CRF’s) have an active soluble coated membrane that acts as a diffusion barrier and releases N based on water content or soil temperature (Hanafi et al., 2002; Taysom et al., 2007; Wilson et al., 2009). Because of the ability to release N over time or keep N in a form less susceptible to loss, N applications could be placed upfront without split applications or petiole testing. These products carry a 10% to 30% premium over conventional forms of N which often makes them impracticable based on economics (Pasda et al., 2001; Hopkins et al., 2008). Enhanced Efficiency Fertilizers have been shown to reduce some environmental consequences of N applications. Fluxes of N2O were reduced by 81%, 35%, and 35% by using dicyandiamide (DCD), polyolefin-coated urea (POCU), or a CRF, respectively on barley (Delgado 59 and Mosier, 1996; Shoji et al., 2001). Dicyandiamide also kept N as NH4 by inhibiting the conversion to NO3 and reducing leaching (Vos, 1994). Leaching of NO3 was reduced by 58% with sulfur coated urea and 40% with polymer coated urea compared to urea alone (Waddell et al., 2000; Zvomuya et al., 2003). The use of the urease inhibitor N-(n-butyl) thiophosphoric triamide (NBPT) and Nitamin have reduced NH3 loss from 45-95% with NBPT and 26-68% with Nitamin compared to urea (Carmona et al, 1990; Zhengping et al., 1991; Grant et al., 1996; Sanz-Cobena et al., 2008; Vaio et al., 2008; Zaman et al., 2008; Zaman et al., 2009). Although EEF’s have been reported to reduce loss to the environment, the ability to sustain or increase yields has been mixed. Early work with sulfur coated urea and urea formaldehyde resulted in lower marketable and total yield compared to NH4NO3 and (NH4)2SO4, as a result of N not meeting plant uptake demand (Lorenz et al., 1972; Lorenz et al., 1974; Cox and Addiscott, 1976; Liegel and Walsh, 1976; Elkashif et al., 1983). Pack et al. (2006) found low N removal efficiencies as some CRF pellets were unopened, had broken polymer shells, or released N too fast or slow. Recent work with polymer coated urea (PCU), including ESN, and POCU have sustained or increased marketable and total yield over urea (Zvomuya and Rosen, 2001; Zvomuya et al., 2003; Taysom et al., 2007). Yields alsohave been maintained by several different CRF’s and DCD (Vos, 1994; Shoji et al., 2001; Pack et al., 2006). Measuring potato N sufficiency levels through petiole NO3 may not be valid with some products as they either inhibit nitrification or the released N does not allow nitrification to occur before plant uptake. Pasda et al. (2001) found DCD treated potatoes took up more NH4 than NO3. Vos (1994) measured lower NO3 and higher NH4 in the petioles with DCD compared to calcium-ammonium-nitrate with no yield reduction. Deficient petiole NO3 were measured in mid to late season when PCU was incorporated at preplant with no yield decrease compared to urea (Wilson et al., 2009). The Pacific Northwest’s Columbia Basin is an intensely irrigated and managed system that produces the highest yielding potatoes in the country: 78 Mg/ha compared to 38 Mg/ha national average (Alva et al., 2002). Research on the effectiveness of new EEF’s is limited in this region, so it is not known if these products can sustain or increase the already high yields, or if they provide an advantage over the current N practices in the area. The objectives of this study were to: (i) measure the ability of EEF’s to meet potato N need to sustain or increase yield and quality; (ii) determine if petiole nitrate is an effective testing tool for plant N when using EEF’s; 60 and (iii) identify the N release rates of EEF’s and determine if they meet demand for the potato crop. MATERIALS AND METHODS Potato Field Study This study was conducted at the Hermiston Agricultural Research and Extension Center in Hermiston, Oregon (Lat 45o 49’ 10”, Long 119o 17’ 00”, Elev. 607 ft) from 2007 to 2009. The soil was an Adkins fine sandy loam (coarse-loamy, mixed, superactive, mesic Xeric Haplocalcids). Seven different enhanced efficiency nitrogen fertilizers were used in the study, each had a different mode of action to maximize plant uptake of N (Table 4.1). Treatments varied across years to alter application rates and timing to find a method that could sustain or increase yields (Table 4.2, Table 4.3, and Table 4.4). The study was set up in a randomized complete block design with five replicates per treatment. Each plot was 7.62 m in length and consisted of 4 rows of potatoes, row spacing of 0.86 m with seed pieces planted every 0.22 m. Cut seed pieces were bulk planted on 4/12/2007, 4/15/2008, and 4/20/2009. Pesticides were applied as needed to control pests, diseases, and weeds according to standard commercial practices in the area. Irrigation was applied through a center pivot irrigation system. Petiole samples were collected on 56, 90, 101, 112, 128 days after planting (DAP) in 2007; 76, 83 DAP in 2008; and 49, 59, 95, 115 DAP in 2009. Ten petioles were taken from the first fully expanded leaf (Porter and Sisson, 1993a), dried at 60oC and analyzed for extractable nitrate (Gavlak et al., 2003) using a Thermo Orion nitrate ion selective electrode (Waltham, MA USA). Plants and tubers were collected on 60, 64, 78, 95, 113 DAP in 2009. Samples were taken from 0.91 m of row, dried at 60oC, and ground on a Wiley Mill. Total N concentration was analyzed using the combustion method (Gavlak et al., 2003b) with an Elementar Vario Max CN analyzer (Hanau, Germany). All potatoes were mechanically lifted and hand harvested at 169 DAP in 2007, 160 DAP in 2008, and 154 DAP in 2009. Samples of 6.66 m were taken to compare yield from the center two rows. Yield and grade were determined (culls, <113 g, US #2’s, 113-340 g, and > 340 g). 61 Samples were measured for specific gravity (SG) using the weight in air and weight in water method (Hutchinson et al., 2003). Ten potatoes from the 113-340 g group were inspected for internal defects. Incubation Study Soil at field capacity was collected from a winter wheat field at the Hermiston Agricultural Research and Extension Center in Hermiston, OR (soil was an Adkins coarse-loamy, mixed, superactive, mesic Xeric Haplocalcids, with pH 6.99) to a depth of 0.30 m. Soil was homogenized and subsamples of 0.65 kg of soil (roughly 0.5 kg dry soil) were placed into gallon Ziplock™ Freezer Bags. Seven treatments and a control were used for each temperature regime with treatments consisting of urea, Agrotain, super-u, environmentally smart nitrogen (ESN), Nutrisphere-N (NSN), Nitamin, and Nitamin N-Fusion. Each treatment had 1.05 g N kg-1 soil applied. Nitrogen was applied to the soil in the Ziploc™ bags and thoroughly mixed. A drinking straw was inserted into each bag which was then sealed around the straw. The straw insured aerobic conditions. Samples were placed in incubators at 4.4OC, 15.6 OC, and 26.7OC. At 1, 3, 6, 13, 20, 28, 34, 48, 63, 76, and 104 DAA of N, bags were thoroughly remixed and sub sampled. Sub samples consisted of 5 g soil for N analysis and 10 g soil for water content and pH. Soil moisture was determined by drying at 60OC, measuring gravimetric soil content. Soil pH was measured using a 1:1 soil/water solution on the dry soil (McLean, 1982). Soil N was analyzed by adding 50 ml 2 M KCl solution to the 5 g wet soil sample and shaken for 1hour on an oscillating shaker. The solution was passed through a Whatman No. 1 filter paper (Keeney and Nelson, 1982) and extracts were analyzed colorimetrically for ammonium (Sims et al., 1995). At 104 days after N was applied urease activity was measured for all treatments according to Torello and Wehner (1982). Two 2-g soil samples from each treatment were incubated for 5-hours in a phosphate buffer-urea solution, with one sample inhibited by AgSO4 during the incubation. After incubation, both soils received KCl and the uninhibited soil received AgSO4. Soils were then shaken for 1 hour. Solutions were filtered through a Whatman No. 1 filter paper and extract analyzed colorimetrically for ammonium (Sims et al., 1995). Net urease 62 activity was calculated by subtracting the inhibited sample from the uninhibited sample and expressed as μg NH4-N g-1 h-1. Statistical Analyses All data were subjected to an analysis of variance (Statistix 9, 2008; SAS Institute Inc., 2009) and means were separated using a LSD at 0.1 probability level for all potato data and a 0.05 probability level for the incubation data. RESULTS AND DISCUSSION Average air and soil temperature for months of production were similar between the three years with average temperature increasing from lows below 10oC in March to mid to high 20oC in July and August (Table 4.5). Average monthly air and soil temperatures varied little between years, with typical monthly temperatures within 1-2oC from year to year. Precipitation for months of production varied from year to year, with total precipitation being the least in 2008 with 25.4 mm less precipitation than the high in 2009. However, the difference in precipitation should not alter the outcome of the trial as irrigation was the primary supply of water for the crop based on ET measurements. Yields were greatest in 2007 (p<0.05). Yields in 2008 were lower than 2007 but higher than in 2009, which had the lowest yields. This could be due to environmental factors; however, weather data for all three years suggest that conditions were similar. There was no interaction between year and treatments. Russet Norkota In 2007 there were no differences between GSP and N treatments for US #1’s, total marketable yield, and total yield (Table 4.6). Applying 80% GSP yielded similarly to the 100% GSP, suggesting that this variety will maintain yields at lower N inputs. Differences were measured between treatments in size classes of 113-340 g and >340 g; however, these differences were offset by lower values of smaller tubers. No differences were measured for 63 internal damages between GSP and any N treatment. There were also no differences in SG between any N treatment. Petioles taken 56 DAP measured GSP with lower petiole nitrate than all except 80% ESN at planting, 80% ESN at emergence, and 80% N-guard at emergence (Table 4.7). Sampling on 90 DAP 100% GSP had more nitrate than 100% N-guard at planting, 80% Nguard at planting, 80% ESN at emergence, and 80% GP-30 at emergence while 101 DAP there were no differences between treatments. Petioles taken 112 DAP, 100% GSP had higher petiole nitrate concentration than all other treatments. Petiole nitrate did not seem to affect Norkota yield as all treatments yielded similarly despite varying nitrate levels. In 2008, there were no differences between GSP and treatments within size class, US #1’s, total marketable yield, and total yield (Table 4.8). The 80% GSP produced similar yields as the 100% GSP, illustrating that Norkota N rates (340 kg ha-1) could be reduced and produce similar yields. No differences were measured for internal defects. The 80% SU at emergence plus had a lower SG and 80% NSN at emergence had a higher SG than the 100% GSP. However, the 80% NSN at emergence’s SG was the same as the 80% GSP. Specific gravities does not have an impact on Russet Norkota marketing, as it is a fresh market product. Petiole sampling 76 DAP resulted in no differences in NO3 concentrations between treatments. At 83 DAP, 80% and 100% ESN at planting, 80% and 100% NSN at emergence, and 80% N-guard at emergence had higher petiole NO3 than 100% GSP and all treatments had higher petioles than 80% GSP (Table 4.9). With only two petiole samples during this year, interpreting these data is difficult; however, differences in petiole NO3 concentration did not result in difference in yield. The use of EEF’s did not affect yields from Russet Norkota. This cultivar showed little to no response to the use of N products and it maintained yields at lower GSP N rates. Differences in petiole nitrate levels did not affect total yield. This cultivar may not require the full GSP N rate which may be the reason that no differences were measured between N treatments. Although N treatments yielded similarly to the GSP, these products come at a premium price so their use in this cropping system does not appear to be economically viable. The use of Russet Norkota was dropped from the 2009 research as a result of no differences between GSP and N treatments. 64 Russet Burbank In 2007, there were no differences between treatments within the class size unders, culls, and >340 g along with US #1’s (Table 4.10). There was a difference in US #2’s, where 100% GSP out yielded more than all other treatments except 100% ESN at emergence. The 80% GSP had more than all except 100% ESN at emergence, 100% N-guard at emergence and 100% ESN at planting. The 80% GP-30 100 UAN was the only treatment that had a higher yield of 113-340 g range potatoes than the GSP. The 100% GSP had higher total marketable yield than all except 80% GSP and the 80% GSP had higher total marketable yield than all except 80% N-guard at emergence and 80% GP-30 100 UAN. The 100% GSP had greater total yield than all treatments except 80% GSP, with 80% GSP out-yielding all except 100% GP-30 100 UAN. There was no treatment difference in internal defects and in SG with all treatments above the penalty threshold of 1.076 (Pavek and Knowles, 2009). AT 56 DAP 100% GP-30 100 UAN and 80% GP-30 100 UAN had higher petiole nitrate concentration than both GSP rates (Table 4.11). All other treatments were similar to the GSP treatments. Petiole nitrates did not differ at 90 DAP. At 101 DAP 100% GSP had higher nitrate concentration than all except 100% ESN at emergence, with most treatments having similar nitrate levels to 80% GSP. At 112 DAP 100% GSP petioles were higher in nitrate than all treatments except 100% ESN at emergence and 100% N-guard at planting with 80% GSP having similar nitrate levels as 80% ESN at emergence, 100% N-guard at emergence, 80% N-guard at emergence, 100% ESN at planting and 80% GP-30 100 UAN. The last sample at 128 DAP measured no differences between treatments. The petiole data show that most N treatments are not maintaining nitrate levels similar to 100% GSP but closer to 80% GSP. This suggests that they are not releasing N according to plant needs and not meeting peak demand. This lack of release resulted in lower yields in N treatments with yields comparable to the 80% GSP. In 2008, there were differences within potato class sizes except the >340 g (Table 4.12). However, differences in class sizes were similar between GSP and N treatments with most not differing from the 100% GSP. With US #1’s, 80% ESN at emergence plus 20% urea and 80% NSN at emergence plus 20% later yielded similarly as the 100% GSP and all other treatments had lower yields. All treatments except 100% SU at emergence were similar to the 80% GSP. The 80% SU at emergence was the only treatment that had similar yields as 100% GSP for total 65 marketable yield and total yield, with all other treatments having lower yields. All treatments had similar total marketable yield as 80% GSP except 100% ESN at emergence which had lower. All treatments had similar total yield as the 80% GSP. Similarities in yield between N treatments and 80% GSP suggest that their entire N is not available to the crop, as most continue to have lower yields than the 100% GSP. There was no difference in treatments for internal defects or SG, with most treatments above the penalty threshold of 1.076 (Pavek and Knowles, 2009). On 76 DAP, petiole nitrate concentrations were similar between 100% GSP and all treatments 80% GP-30 90 UAN at emergence. The 100% ESN at planting, 100% ESN at emergence, 80% ESN at emergence plus 20% urea, 100% NSN at emergence, 80% NSN at emergence plus 20% later, 80% NSN at emergence, 100% GP-30 90 UAN at emergence, and 80% SU at emergence with 70 urea had similar nitrate levels as 80% GSP (Table 4.13). On 83 DAP, both GSP’s had similar petiole nitrate concentrations and were lower than all other treatments. Only 100% ESN at planting, 80% ESN at planting, and 100% GP-30 90 UAN at emergence had similar nitrate as 100% GSP and 100% ESN at planting, 80% ESN at planting, 100% GP-30 90 UAN at emergence, and 80% GP-30 90 UAN at Emergence nitrate as 80% GSP. As these were the only petioles from this year, very little can be suggested as these were taken early in the season and we do not know if nitrate levels varied later in the season. In 2009 there were two 100% GSP: 100% GSP at emergence and 100% GSP at planting. There were differences within potato size classes for US 2’s and 113-340g however differences between GSP and N treatments were minimal (Table 4.14). There was no difference between treatments for >340 g, US 1’s, total marketable yield, and total yield. There were no differences in specific gravity between treatments and GSP and no differences in internal damages. Although no differences were measured in specific gravities, several treatments did have values below the threshold of 1.076 which would result in a penalty at a processing plant (Pavek and Knowles, 2009). These data shows that yields were maintained with all N treatments. However, the 100% GSP yielded the same as 80% GSP suggesting that N levels were not as limiting as in previous years. Although there were petiole nitrate differences between treatments, there was no difference in petiole nitrate between GSP’s and N treatments at the 49 DAP (Table 4.15). At 59 DAP several treatments had higher and lower nitrate levels than the GSP. On 95 DAP ESN 180 Emerg, SU 330 Plant, and SU 260 Emerg had lower nitrate than both 100% GSP’s. The 80% GSP had higher nitrate than SU 104 Emerg, 70 NF + 55 UAN, 88 NF + 152 UAN, 70 NF + 190 UAN, 66 and 88 NF + 242 UAN. On 115 DAP ESN 180 Emerg, SU 104 Emerg, 88 NF + 37 UAN, 70 NF 100 UAN, 88 NF 152 UAN, 70 NF + 190 UAN, and 88 NF + 242 UAN had lower nitrate than 100% GSP at emergence. The 100% GSP at emergence was only higher than 70 NF 100 UAN and 88 NF + 242 UAN and lower than ESN 330 Emerg, ESN 290 Emerg, ESN 250 Emerg, ESN 210 Emerg, ESN 260 Emerg, and SU 260 Emerg. The 100% GSP at planting was lower than ESN 330 Plant, ESN 330 Emerg, ESN 290 Emerg, ESN 250 Emerg, ESN 210 Emerg, ESN 260 Emerg, SU 330 Plant, SU 260 Emerg, and 70 NF + 55 UAN. It does not appear that petiole nitrate reflected N in the plant as differences between treatments did not result in yield differences. Plant dry matter samples taken during 2009 were not affected by treatments when sampled 64, 78, 95, and 113 DAP (data not shown). Only dry matter samples collected 60 DAP had differences between treatments; however, N treatments did not differ from GSP. There were no differences in potato dry matter at any point during the study. This is partly due to inaccurate collection of potatoes at early sampling dates. Potato vine N uptake for sampling periods only measured differences in three out of the five sampling periods, with minimal difference between GSP and N treatments (data not shown). Tuber N uptake could not be accurately accounted for as a result of inaccurate collection of potatoes during the sampling periods. At 60 DAP plant N concentration was similar with all treatments, but petiole NO3 varied between products and GSP(Table 4.15 and Table 4.16). On 95 DAP there were differences for both plant N concentration and petiole nitrate. There was no difference in N concentration between GSP and the treatments except 70 NF + 55 UAN was lower than the GSP. Petiole data for SU 104 Emerg, 70 NF + 55 UAN, 88 NF + 37 UAN, 70 NF 100 UAN, 88 NF 152 UAN, 70 NF + 190 UAN, and 88 NF + 242 UAN were all below the GSP. This difference in petiole nitrate may prompt a grower to apply more N even though the N concentrations in the plants are similar. Sampling 113 DAP there were differences between GSP and treatments for N concentration. The 88 NF + 37 UAN, 70 NF 100 UAN, 88 NF 152 UAN, 70 NF + 190 UAN, and 88 NF + 242 UAN had less N concentration than all GSP and several treatments had less than one GSP. These treatments had similar nitrate as GSP when examining petiole nitrate. Comparing these differences, petiole nitrate does not accurately reflect the N content in the plant with some N treatments. This is likely a result of some N products keeping N in NH4 form or slowly releasing N and not allowing nitrate to form before plant uptake. Vos (1994) found that the use of DCD, 67 which is in Super-U, posed problems with nitrate interpretation as DCD inhibits nitrate formation. When inhibiting nitrate and supplying NH4 instead, nitrate sampling does not reflect the N concentration in the plant as N in the plant is NH4. Whole plant samples and plant N only were measured in 2009 when yields were similar across treatments, so differences between plant matter and plant N did not result in different yields. Data from previous years when treatment yields were lower than GSP would have given valuable information on how these processes affect potato yield. In both 2007 and 2009, 80% GSP yielded similarly to 100% GSP, while 2008 100% GSP out-yielded 80% GSP. However, in 2008 and 2009 the 80% produced similar yields to most N treatments and only in 2009 did N treatments produce similar yields to the 100% GSP. Nitrogen treatments yielded similar to 80% GSP for two years which suggests that N availability may be a problem with some of these products. There have been measured increases and maintained yields with the use of ESN and DCD (Vos, 1994; Taysom et al., 2007; Wilson et al., 2009); however, these were performed in regions outside the Columbia Basin. The intensively managed, high yielding potato production in the Columbia Basin could be a reason these N products are decreasing or maintaining yields. Current split N application practices supply available N to the potato plant when it is needed. Maintaining yields with these N treatments is economically unviable as they come with a premium, so a yield increase or a cost saving attribute must be observed in order to make these practical for potato production in the Columbia Basin. Incubation Study All products at 4.4oC slowed the release of N compared to urea except NSN (Figure 4.1). NSN followed the same hydrolysis rate as urea through 100 DAA as well as the same NO3 formation. Urea and NSN had all N available by 13 DAA, either as NH4 or NO3. Agrotain and Super U followed similar rates of NH4 formation with most N being present as NH4 by 63 DAA. These products were able to slow urea hydrolysis, as both contain the urease inhibitor NBPT. Both products had similar NO3 conversion rates. It would be expected that Super-U have lower NO3 levels as it has the nitrification inhibitor DCD in its composition. Agrotain and Super-U had all N available by 63 DAA. ESN and Nitamin had similar rates of NH4 formation although 68 different modes of action were used. ESN supplied 46% of its N by 20 DAA and then slowly released the rest. ESN was the only product that showed large increases in NO3 formation, exhibiting that it only regulates N release, it is not an inhibitor. ESN had all N available by the end of the study on 104 DAA. Nitamin released about 48% of its N as NH4 by 13 DAA similar to ESN, however its NO3 formation was lower throughout the study and only had NO3 formation after 63 DAA. Nitamin also had only 60% of its total N available by the end of the study on 104 DAA. N-fusion released its N slowly with NH4 levels at 16% and NO3 levels at 8% by 104 DAA. Final N available after 104 DAA was only 25%. At 40oF the use of Nitamin and N-fusion would not be wise as the N released would not be able to meet plant need. The use of Agrotain, Super-U, and ESN all released N slowly over time and had all N available at 104 DAA. Urea and NSN behaved the same showing that NSN has no inhibiting capability. At 15.6oC all products slowed release of N compared to urea except NSN (Figure 4.2). NSN and urea had all their N as NH4 at 6 and 13 DAA respectively. The only difference was at 6 DAA when urea was 100% hydrolyzed and NSN was only 80%. Other than this all NH4 rates for the two were similar throughout the study. At 20 DAA both NH4 levels began to decline as a result of NO3 formation and NO3 formation for both products was similar for the trial. Urea and NSN had similar N available for the entire study with all N available by 13 DAA. Agrotain and Super-U both hydrolyzed at the same rate with 100% of their N available as NH4 by 28 DAA. After 28 DAA Agrotain had more NO3 conversion and subsequent NH4 decline than Super-U as a result of Super-U containing DCD. Both products had similar total N available throughout the study, however the difference between the two was in the form of N, with Agrotain having more N converting to NO3 than Super-U. ESN had 50% of its N as NH4 by 13 DAA and then after 20 DAA available NH4 declined with time. Available N continued to increase as NH4 was converted to NO3 and by 104 DAA over 60% of total N in the form of NO3. Available N for ESN was 100% by 48 DAA. This exhibits that N from ESN is slowly released from the polymer and can be readily hydrolyzed and then nitrified. Nitamin had the formation of 62% NH4 by 6 DAA, then NH4 declined with an increase in NO3 formation. Total N available was 73% at 104 DAA, with the majority of N available in the first 20 DAA. Formation of NH4 for N-fusion was 24% by 20 DAA and then slowly increased to 29% at 104 DAA. Formation of NO3 was low and increased after 20 DAA and remained around 15% from 50 to 104 DAA. By 104 DAA, 42% of total N was available. This product seems to release N extremely slow and not meet N demands of the plant. Nitamin 69 would have a similar response on plant demand, as less than 80% of its N is available. Agrotain, Super-U and ESN slowly release N and would have all N available by 48 DAA. Urea and NSN have no slow release capabilities. At 26.7oC, all products delayed available N compared to urea except NSN (Figure 4.3). NSN and urea both had 100% hydrolysis by day 13 and both had NH4 decline after 20 DAA. Both also had similar NO3 formation throughout the study except on the 104 DAA sampling period when urea had less. NSN and urea also had all N available from 6 DAA onward. Agrotain and Super-U followed similar hydrolysis rates with 100% N available as NH4 by 20 DAA. After this time levels of NH4 declined as NO3 was formed. However, Super-U had less NO3 formation than Agrotain as a result of DCD, as DCD is a nitrification inhibitor slowing conversion of NH4 to NO3 (Vos, 1994). Both products had 100% N available from 20 DAA onward. ESN had 32% N available as NH4 at 13 DAA and then NH4 remained steady as NO3 conversion increased. By 48 DAA, ESN had all N available, close to 67% as NO3. Nitamin had 56% N available as NH4 by 6 DAA then NH4 levels decreased as NO3 formed. By 104 DAA NO3 levels were 60% with total available N about 100%. N –fusion had 23% N available as NH4 by 13 DAA, then slowly increased to 38% by 104 DAA. Nitrate formation began at 20 DAA with final NO3 representing 60%. Total N available from N-fusion after 104 DAA reached 100%. N-fusion and Nitamin exhibited slow release with 100% N available after 104 DAA, which could stress the plant for N early in the season. Agrotain, Super-U, and ESN all release N over time making it plant available. Urea and NSN had no slow release capabilities. At all temperatures NSN and urea performed similarly with no gradual release of N. Agrotain and Super-U delayed the formation of NH4 as a result of NBPT. NBPT is a known urease inhibitor therefore slowing the hydrolysis of urea (Manunza et al., 1999). After complete hydrolysis, NO3 formation increased; however, Super-U was able to limit NO3 formation as it contained DCD. ESN had initial N available as NH4 which was then converted to NO3, with NO3 levels increasing and NH4 levels staying consistent or declining. ESN was able to slowly release urea and get N to the plant. Nitamin had an initial increase of N as NH4, since 30% of its N is urea with the rest in a urea polymer form that slowly makes N available (Vaio et al., 2008). This increase only reached 100% N available at 26.7oC showing that this product releases N too slowly for plant demand at cooler temperatures. N-fusion was slow in releasing N, and slow in formation in both NH4 and NO3. This product works too slowly to meet plant demands, 70 especially since potatoes can take up to 80% of N 20-60 days after emergence (Munoz et al., 2005). Pack et al. (2006) found similar issues with controlled-release fertilizers as N release was either too fast or too slow for plant demand. The lack of N availability from these products at certain temperatures could be the reason for lower yields than the GSP in 2007 and 2008 and comparable yields to the 80% GSP in 2007, 2008, and 2009. It is believed that the rapid hydrolysis of urea, NSN, Agrotain, and Super-U along with the high rates of N in this experiment may have reduced nitrification bacteria populations as a result of increased NH3 levels. Ammonia could be smelled from certain bags during the experiment. This problem may have resulted in a delay in NO3 formation. ESN had highest NO3 levels at all temperatures and is believed to not have affected nitrifying populations as it never reached high NH4 levels like urea, NSN, Agrotain, and Super-U. No differences were measured in urease activity between treatments (Table 6.20). This may be due to sampling at 104 DAA; earlier sampling may have measured differences as Agrotain and Super-U have a known urease inhibitor NBPT in their formulation. By 104 DAA, the NBPT already would have decomposed. There was an effect of temperature on available N (p<0.05) and an interaction between temperature and N treatment (p<0.05). This was measured for NH4 formation, NO3 formation, and total available N for each treatment. Increased incubation temperature led to increased hydrolysis rates and increased NH4 formation. This led to increased NO3 formation and an increase in total available N. ESN is specifically designed to release N based on soil temperature with its micro-thin polymer coating (Taysom et al., 2007; Wilson et al., 2009). Consequently, soil temperature greatly affects N release. The effect of temperature on release rate from these N products will affect N available to the plant, and will vary according to N treatment. This may make it difficult to incorporate these products into a cropping system as N release is dependent on environmental conditions, and environmental conditions are unpredictable. The GSP also accounts for unpredictability as N is available when the plant demands it. At all three temperatures, soil pH increased with all treatments (Figure 4.4). However, all products increased soil pH faster than the control, likely a result from hydrolysis. At 4.4oC, Agrotain and Super-U delayed peak pH until 13 DAA; at 15.6oC, Agrotain, Super-U, and ESN delayed peak pH until 3 DAA. Agrotain, Super-U, ESN, and N-fusion all delayed peak pH until 6 DAA at 26.7oC. The delay in peak pH is due to slowing of urea hydrolysis. After increasing, the 71 pH declined for the rest of the study for treatments. Some variation between pH exists between products after the peak; however, they follow no pattern between sampling dates. CONCLUSIONS Specialty N fertilizers maintained yield for Russet Norkota potatoes; however, a reduction of GSP N also sustained yields. Although yield was maintained, the use of specialty N fertilizers with Russet Norkota is still prohibitive due to the premium involved. Specialty N fertilizers do not appear to produce a competitive yield at this time with grower standard practice for Russet Burbank. Yields were below GSP for two out of three years of production, with the third year only maintaining yields. 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Nitrate leaching and nitrogen recovery following application of polyolefin-coated urea to potato. J. Environ. Qual. 62:480-489. 77 Urea Agrotain Super-u NSN a) Available NH4 (% N applied) 100 80 60 40 20 0 0 20 Urea 40 60 80 100 ESN b) Available NH4 (% N applied) 100 80 60 40 20 0 0 20 Urea Nitamin 40 60 80 100 N-fusion c) Available NH4 (% N applied) 100 80 60 40 20 0 0 20 40 60 80 100 Figure 4.1. Available NH4 at 4.4oC from (a) urease and nitrification inhibitors, (b) polymer coated urea, and (c) slow release N in incubation as affected by N treatment. Values are the average of the replications. 78 Urea Available NH4 (% N applied) 120 Agrotain Super-u NSN a) 100 80 60 40 20 0 0 Available NH4 (% N applied) 120 20 Urea 40 60 80 100 ESN b) 100 80 60 40 20 0 0 Urea 120 Available NH4 (% N applied) 20 Nitamin 40 60 80 100 N-fusion c) 100 80 60 40 20 0 0 20 40 60 80 100 Figure 4.2. Available NH4 at 15.6oC from (a) urease and nitrification inhibitors, (b) polymer coated urea, and (c) slow release N in incubation as affected by N treatment. Values are the average of the replications. 79 Urea Agrotain Super-u NSN Available NH4 (% N applied) 120 100 a) 80 60 40 20 0 0 Urea 120 Available NH4 (% N applied) 20 40 60 80 100 ESN 100 b) 80 60 40 20 0 0 20 Urea Nitamin 40 60 80 100 N-fusion Available NH4 (% N applied) 120 c) 100 80 60 40 20 0 0 20 40 60 80 100 Figure 4.3. Available NH4 at 26.7oC from (a) urease and nitrification inhibitors, (b) polymer coated urea, and (c) slow release N in incubation as affected by N treatment. Values are the average of the replications. 80 Control 8.4 Urea Agrotain Super-U NSN ESN Nitamin N-Fusion a) 8.2 pH 8 7.8 7.6 7.4 7.2 7 0 20 40 60 80 100 8.5 b) 8 pH 7.5 7 6.5 6 5.5 0 20 40 60 80 100 8.5 c) 8 pH 7.5 7 6.5 6 5.5 5 0 20 40 60 Days after application 80 100 Figure 4.4. Soil pH at (a) 4.4oC, (b) 15.6oC, and (c) 26.7oC in incubation as affected by N treatment. Values are the average of the replications. 81 Table 4.1. Modes of action for enhanced efficiency nitrogen fertilizers. Product Agrotain Super-U Nutrisphere-N (NSN) Environmentally Smart N (ESN) Nitamin N-Fusion Mode of Action Urease Inhibitor Urease and Nitrification Inhibitor Urease Inhibitor Polymer Coated Urea Slow Release N (Microbial Breakdown of urea polymers) Slow Release N (Microbial Breakdown of urea polymers) Table 4.2. Nitrogen treatments for Russet Norkota and Russet Burbank for 2007, listing N source, N rates (kg ha-1), and application timing. Unless noted, N rates represent N treatment product. All plots received 22 kg N/ha preplant. N Source Russet Norkota 100% ESN at planting 80% ESN at planting 100% N-guard at planting 80% N-guard at planting 80 % ESN at emergence 80% N-guard at emergence 100% GP-30 80% GP-30 100% GSP N at Planting 80% GP-30 100 UAN 100% GSP 80% GSP Other N 392 313 392 313 392 392 112 UAN 112 UAN 80% GSP Russet Burbank 100% ESN at emergence 80% ESN at emergence 100% N-guard at emergence 80% N-guard at emergence 100 % ESN at planting 100% N-guard at planting 100% GP-30 100 UAN N at Emergence 112 Urea 70x4 50x4 269 Urea 89 Urea 201 Urea 392 313 392 313 313 313 112 140x2 112 112 Urea 112x2 269 Urea 89 Urea 201 Urea Notes All at Emergence All at Emergence All at Emergence All at Emergence All at Planting All at Planting Applied for 4 weeks starting at Emergence Applied for 4 weeks starting at Emergence Other 240 kg N-urea split 5 times in growing season Other 180 kg N-urea split 5 times in growing season All at Planting All at Planting All at Planting All at Planting All at Emergence All at Emergence Applied for 2 weeks starting at Emergence Applied for 2 weeks starting at Emergence Other 240 kg N-urea split 5 times in growing season Other 180 kg N-urea split 5 times in growing season 82 Table 4.3. Nitrogen treatments for Russet Norkota and Russet Burbank for 2008, listing N source, N rates (kg ha-1), and application timing. Unless noted, N rates represent N treatment product. All plots received 22 kg N/ha preplant. N Source Russet Norkota 100% ESN at planting 80 % ESN at planting 80% ESN at emergence 100% NSN at emergence 80% NSN at emergence 80% N-guard at emergence 100% GP-30 90 UAN 80% GP-30 90 UAN 100% N standard 80% N standard 100 % SU at emergence 80% SU at emergence 70 urea 80% SU at emergence Russet Burbank 100 % ESN at planting 100% ESN at emergence 80% ESN at emergence plus 100% NSN at emergence 80% NSN at emergence plus 20% later 80% NSN at emergence 100% GP-30 90 uan at 80% GP 30 90 uan at 100% N standard 80% N standard 100 % SU at emergence 80% SU at emergence plus 80% SU at emergence Planting Emergence 336 269 Other 67 Urea 269 336 269 269 100 UAN 100 UAN 100 Urea 89 Urea 336 269 269 392 313 67 67x4 38x4 212 Urea 156 Urea 67 78 Urea 313 392 313 313 100 UAN 100 UAN 100 Urea 89 Urea 392 313 313 78 67x4 39x4 269 Urea 201 Urea 78 Notes All at Planting All at Planting All at Emergence All at Emergence Other Applied June 26 All at Emergence Other Applied for 4 weeks starting after Emergence Other Applied for 4 weeks starting after Emergence Other 212 kg N-urea split 5 times during growing season Other 156 kg N-urea split 4 times during growing season All at Emergence Other Applied June 19 All at Emergence All at Planting All at Planting All at Emergence All at Emergence Other Applied June 26 All at Emergence Other Applied for 4 weeks starting at emergence Other Applied for 4 weeks starting at emergence Other 269 kg N-urea split 7 times during growing season Other 201 kg N-urea split 6 times during growing season All at Emergence Other Applied on June 1 All at Emergence 83 Table 4.4. Nitrogen treatments for Russet Burbank for 2009, listing N source, N rates (kg ha-1), and application timing. Unless noted, N rates represent N treatment product. All plots received 22 kg N/ha preplant. Nitrogen Source ESN 330 Plant ESN 330 Emerg ESN 290 Emerg ESN 250 Emerg ESN 210 Emerg ESN 260 Emerg ESN 180 Emerg GSP 350 Emerg GSP 280 Emerg GSP 350 Plant SU 330 Plant SU 260 Emerg SU 104 Emerg 70 NF +55 UAN 88 NF + 37 UAN 70 NF 100 UAN 88 NF 152 UAN 70 NF +190 UAN 88 NF + 242 UAN Planting 369 Emergence 0 369 325 280 235 291 244 100 Urea 100 Urea 118 Urea 369 Other 44 Urea 89 Urea 134 Urea 89 Urea 246 Urea 190 Urea 251 Urea Notes All at Planting All at Emergence All at Emergence All at Emergence All at Emergence All at Emergence All at Emergence Other 246 kg N-urea split 5 times during growing season Other 190 kg N-urea split 4 times during growing season Other 251 kg N-urea split 5 times during growing season 291 123 Agrotain, 127 Urea 118 78 NF, 61 UAN 98 NF, 41 UAN 100 NF 151 UAN 229 UAN 78 NF, 112 UAN 98 NF, 271 UAN 78 NF, 212 UAN 98 NF, 271 UAN Other, urea split 2 times, Agrotain split 3 times (5 separate applications) Other 151 kg N-UAN split 3 times during growing season Other 229 kg N-UAN split 5 times during growing season Other all at tuberization Other all at tuberization Other 4 equal applications starting at emergence Other 4 equal applications starting at emergence 84 Table 4.5. Mean monthly air temperature, soil temperature, and total precipitation for years 2007-2009. o o ----------Air Temp C----------- --------Soil Temp C------------ -------Precipitation mm-------- 2007 2008 2009 2007 2008 2009 2007 2008 2009 March 9.17 6.58 5.86 8.83 8.00 7.07 12.19 16.26 25.40 April 11.51 9.38 10.82 14.03 11.42 12.13 11.94 2.79 12.95 May 16.47 16.26 16.47 18.05 17.78 17.26 10.16 10.16 26.67 June 19.58 18.83 20.56 20.92 20.73 23.43 24.13 12.95 3.05 July 25.63 23.99 25.24 24.61 24.59 27.17 0.51 0.00 1.27 August 22.19 22.22 23.61 23.18 23.27 26.32 1.27 5.33 2.03 September 17.68 17.39 18.85 20.62 20.62 23.28 6.35 0.76 2.29 Average (total) 17.48 16.40 17.35 18.61 18.07 19.52 (66.55) (48.26) (73.66) 85 Table 4.6. Yield, potato class, specific gravity, and internal damage for Russet Norkota in 2007 as affected by N treatment. Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment 100% ESN at planting 80% ESN at planting 100% N-guard at planting 80% N-guard at planting 80 % ESN at emergence 80% N-guard at emergence 100% GP-30 80% GP-30 100% N standard 80% N standard Significance LSD (0.1) <113 g Culls 2’s 113-340 g > 340 g US No 1 Total Total Mrktbl yield ---------------------------------------------------Mg/ha-----------------------------------------7.6 0.0 B 0.9 65.7 ABC 27.6 BCD 93.5 94.6 102.4 8.3 0.0 B 1.3 65.5 ABC 20.8 D 86.3 87.7 96.4 6.9 0.9 A 1.1 51.1 E 39.2 A 90.3 91.7 99.5 7.6 0.0 B 1.3 54.9 DE 33.8 AB 88.8 90.3 98.2 7.6 0.0 B 1.3 67.7 AB 20.8 D 88.5 90.1 98.0 7.2 0.0 B 1.3 60.3 CD 30.3 BC 90.6 91.9 99.3 7.8 0.2 B 7.6 57.8 D 33.0 AB 91.0 98.6 106.9 9.4 0.0 B 1.6 50.7 E 39.5 A 90.3 91.9 101.5 7.8 0.0 B 1.3 61.4 BCD 35.0 AB 96.4 97.7 106.1 7.8 1.1 A 1.8 69.3 A 22.2 CD 91.5 93.5 102.6 NS * NS * * NS NS NS 2.0 0.4 4.9 6.5 8.5 8.3 8.1 7.6 Specific Gravity 1.0679 1.0691 1.0703 1.0712 1.0684 1.0705 1.0689 1.0684 1.0673 1.0676 NS 2.0 Total Internals % 12.5 7.5 10 2.5 7.5 0 20 15 7.5 10 NS 0.4 *Significance at the 0.1 probability level 86 87 Table 4.7. Petiole nitrate levels for Russet Norkota in 2007 as affected by N treatment and sampling date (DAP). Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment 100% ESN at planting 80% ESN at planting 100% N-guard at planting 80% N-guard at planting 80 % ESN at emergence 80% N-guard at emergence 100% GP-30 80% GP 30 100% N standard 80% N standard Significance LSD (0.1) Sample Dates 56 90 101 112 ---------------------------g NO3-N/kg-------------------25.6 CD 16.1 AB 17.1 18.1 BC 23.2 E 16.6 AB 8.5 19.4 B 26.5 BC 12.2 B 9.5 14.2 BC 28.1 AB 12.4 B 10.8 12.8 C 23.5 E 12.3 B 8.3 14.3 BC 24.7 CDE 15.3 AB 11.4 15.3 BC 28.9 A 20.4 A 14.7 17.8 BC 27.8 AB 14.0 B 12.2 18.9 BC 24.5 DE 20.9 A 15.3 27.2 A 24.3 DE 11.1 B 13.2 16.1 BC * * NS * 1.9 5.6 6.9 6.6 *Significance at the 0.1 probability level Table 4.8. Yield, potato class, and specific gravity for Russet Norkota in 2008 as affected by N treatment. Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment 100% ESN at planting 80 % ESN at planting 80% ESN at emergence 100% NSN at emergence 80% NSN at emergence 80% N-guard at emergence 100% GP-30 90 UAN at emergence 80% GP-30 90 UAN at emergence 100% N standard 80% N standard 100 % SU at emergence 80% SU at emergence with 70 urea 80% SU at emergence Significance LSD <113 g Culls 2’s 113-340 g > 340 g US No 1 Total Total Mrktbl yield -----------------------------------------Mg/ha--------------------------------------------------4.7 0.0 4.7 59.0 13.0 72.0 76.7 81.8 5.2 0.2 3.4 60.1 8.1 68.1 71.5 77.1 6.3 0.2 3.1 58.5 13.0 71.5 74.6 81.1 5.6 0.0 4.9 56.5 17.0 73.3 77.3 83.8 5.6 0.0 4.5 59.4 16.6 76.0 80.3 85.9 4.7 0.4 6.5 59.9 13.2 72.9 79.4 84.7 6.5 0.0 4.0 62.5 9.4 72.0 76.0 82.5 5.4 0.0 4.5 61.6 9.2 70.8 75.5 80.9 5.4 0.2 4.9 62.5 13.5 75.8 80.9 86.8 4.0 0.0 3.6 60.1 13.2 73.3 76.9 81.1 5.2 0.0 4.3 62.3 10.5 72.9 76.9 82.0 7.2 0.9 4.9 51.3 11.4 62.5 67.5 75.5 4.0 0.0 3.1 58.3 10.5 68.8 72.0 76.0 NS NS NS NS NS NS NS NS 1.6 0.7 2.0 7.4 7.8 8.7 8.7 8.7 Specific Gravity 1.0712 AB 1.0698 ABCD 1.0676 DE 1.0688 CD 1.0718 A 1.0706 ABC 1.0694 BCD 1.0702 ABC 1.0694 BCD 1.0714 AB 1.0698 ABCD 1.0656 E 1.0698 ABCD * 0.002 *Significance at the 0.1 probability level 88 89 Table 4.9. Petiole nitrate levels for Russet Norkota in 2008 as affected by N treatment and sampling date (DAP). Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment Sample Dates 76 83 -----g NO3-N/kg----100% ESN at planting 26.0 25.3 AB 80 % ESN at planting 24.6 26.4 A 80% ESN at emergence 23.8 23.1 BC 100% NSN at emergence 25.0 26.7 A 80% NSN at emergence plus 20% later 24.7 25.1 AB 80% N-guard at emergence 22.2 24.9 AB 100% GP-30 90 UAN at emergence 23.8 24.4 ABC 80% GP-30 90 UAN at emergence 23.0 23.4 BC 100% N standard 24.8 22.3 C 80% N standard 21.7 18.2 100 % SU at emergence 27.6 24.5 ABC 80% SU at emergence with 70 urea 27.1 23.5 BC 80% SU at emergence 25.8 24.2 ABC Significance NS * LSD (0.1) 3.3 2.3 *Significance at the 0.1 probability level D Table 4.10. Yield, potato class, specific gravity, and internal damage for Russet Burbank in 2007 as affected by N treatment. Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment 100% ESN at emergence 80% ESN at emergence 100% N-guard at emergence 80% N-guard at emergence 100 % ESN at planting 100% N-guard at planting 100% GP-30 100 UAN 80% GP-30 100 UAN 100% N standard 80% N standard Significance LSD (0.1) <113 g Culls 2’s 113-340 g > 340 g US Total Total No 1 Mrktbl yield ---------------------------------------------------Mg/ha------------------------------------------------11.2 2.5 29.6 ABC 36.5 D 16.6 53.1 82.9 C 96.8 C 10.5 0.7 23.1 CDE 43.3 BCD 15.7 59.0 82.0 C 93.5 C 11.4 1.1 24.4 BCD 39.5 BCD 20.6 60.1 84.7 C 97.5 C 6.9 0.2 13.7 E 47.3 B 31.2 78.7 92.6 BC 100.0 C 10.1 0.7 25.6 BCD 37.9 CD 24.0 61.9 87.7 C 98.6 C 7.6 0.2 17.3 DE 40.8 BCD 28.7 69.5 87.0 C 94.8 C 8.1 1.1 19.5 CDE 46.2 BC 30.5 76.7 96.2 BC 105.6 BC 10.5 0.7 15.5 DE 57.8 A 18.2 76.2 91.7 BC 103.1 C 8.3 0.7 38.1 A 39.0 BCD 34.1 73.3 111.4 A 120.6 A 10.1 0.9 34.5 AB 41.0 BCD 30.0 71.1 105.6 AB 116.8 AB NS NS * * NS NS * * 3.4 1.8 10.3 8.7 13.7 16.8 14.1 13.0 Specific Gravity 1.0768 1.0817 1.0801 1.0835 1.0805 1.0868 1.081 1.0832 1.0774 1.0793 NS 0.0063 Total Internals % 20 8 4 4 2 8 8 4 10 12 NS 12 *Significance at the 0.1 probability level 90 91 Table 4.11. Petiole nitrate levels for Russet Burbank in 2007 as affected by N treatment and sampling date (DAP). Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment Sample Dates 56 90 101 112 128 --------------------------------g NO3-N/kg------------------------------100% ESN at emergence 80% ESN at emergence 22.1 22.0 C C 26.8 23.3 24.9 22.6 AB BCDE 23.4 20.8 AB BC 14.7 10.9 100% N-guard at emergence 80% N-guard at emergence 23.0 22.1 C C 21.6 17.7 22.8 16.8 BCD F 13.8 16.6 D CD 11.2 12.0 100 % ESN at planting 22.4 C 26.3 24.2 BC 21.0 BC 13.0 100% N-guard at planting 100% GP-30 100 uan at planting 23.4 25.1 BC AB 22.9 21.1 23.1 20.1 BCD DEF 25.4 21.5 AB B 13.4 12.8 80% GP 30 100 uan at planting 100% N standard 26.2 22.9 A C 23.6 25.1 19.5 27.7 EF A 20.8 27.4 BC A 12.3 15.9 80% N standard Significance 21.9 * C 22.0 NS 21.4 * CDE 16.6 * CD 14.2 NS LSD 0.1 1.8 5.3 3.2 *Significance at the 0.1 probability level 4.6 4.6 Table 4.12. Yield, potato class, specific gravity, and internal damage for Russet Burbank in 2008 as affected by N treatment. Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment 100 % ESN at planting 100% ESN at emergence 80% ESN at emergence plus 20% urea 100% NSN at emergence 80% NSN at emergence plus 20% later 80% NSN at emergence 100% GP-30 90 uan at emergence 80% GP 30 90 uan at emergence 100% N standard 80% N standard 100 % SU at emergence 80% SU at emergence and 80% SU at emergence Significance LSD (0.1) Total Total Mrktbl yield ------------------------------------------------------Mg/ha-----------------------------------------------7.8 1.1 12.3 C 39.5 BCDE 18.8 58.3 BCDE 70.4 DE 79.6 CD 9.4 0.2 11.4 C 40.1 BCD 15.0 55.1 DEF 66.6 E 76.2 D 7.8 0.4 12.1 C 44.2 AB 22.4 66.6 AB 78.7 BCD 87.2 BC 1.074 1.072 1.092 Total Internals % 32 42 32 8.3 6.5 0.0 0.4 14.3 BC 15.0 BC 35.0 CDE 41.5 ABC 24.7 24.2 59.6 BCDE 65.7 ABC 73.8 CDE 80.7 BC 82.3 CD 87.9 BC 1.071 1.077 28 28 5.6 7.8 1.3 0.2 13.2 C 17.0 ABC 48.6 A 39.9 BCD 14.1 16.8 62.8CD 56.7 CDEF 76.0 CDE 73.5 CDE 82.9 CD 81.8 CD 1.08 1.082 26 26 8.1 0.2 15.5 BC 34.3 CDE 22.6 57.2 CDE 72.6 CDE 81.1 CD 1.078 36 7.4 6.7 0.2 1.1 16.4 ABC 14.6 ABC 46.2 AB 40.8 BCD 27.8 20.4 74.2 A 61.2 BCDE 90.6 A 77.6 BCD 1.088 1.087 48 42 7.6 7.6 6.7 NS 3.1 1.3 0.9 0.2 NS 1.1 22.2 A 19.5 AB 22.9 A * 6.1 32.1 E 34.1 DE 39.9 BCDE * 7.4 15.7 19.1 24.2 NS 9.2 47.7 F 53.1 EF 63.9 BCD * 9.0 69.9 DE 72.4 CDE 86.8 AB * 15.2 98.2 A 85.4 BCD 79.1 CD 80.9 CD 93.9 AB * 9.6 1.091 1.082 1.079 NS 0.0161 40 26 38 NS 19 <113 g Culls 2’s 113-340 g > 340 g US No 1 Specific Gravity *Significance at the 0.1 probability level 92 93 Table 4.13. Petiole nitrate levels for Russet Burbank in 2008 as affected by N treatment and sampling date (DAP). Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment 100 % ESN at planting 100% ESN at emergence 80% ESN at emergence plus 20% urea 100% NSN at emergence 80% NSN at emergence plus 20% later 80% NSN at emergence 100% GP-30 90 uan at emergence, 80% GP 30 90 uan at emergence planting 100% N standard 80% N standard 100 % SU at emergence 80% SU at emergence and 80% SU at emergence Significance LSD (0.1) *Significance at the 0.1 probability level Sample Date 76 83 ------------g NO3-N/kg---------22.6 ABC 19.7 CD 23.0 ABC 19.3 CDE 22.7 ABC 25.4 AB 23.6 AB 22.9 ABC 19.6 C 25.5 A 19.8 C 22.5 ABC 24.1 AB 21.4 ABCD 13.9 D 15.1 E 23.3 ABC 23.2 ABC 21.0 BC 17.4 DE 25.0 A 21.0 BCD 24.5 AB 21.4 ABCD 25.1 A 25.3 AB * * 3.7 4.4 Table 4.14. Yield, potato class, specific gravity, and internal damage for Russet Burbank in 2009 as affected by N treatment. Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment ESN 330 Plant ESN 330 Emerg ESN 290 Emerg ESN 250 Emerg ESN 210 Emerg ESN 260 Emerg ESN 180 Emerg GSP 350 Emerg GSP 280 Emerg GSP 350 Plant SU 330 Plant SU 260 Emerg SU 104 Emerg 70 NF +55 UAN 88 NF + 37 UAN 70 NF 100 UAN 88 NF 152 UAN 70 NF +190 UAN 88 NF + 242 UAN Significance LSD (0.1) <113 g Culls 2’s 113-340 g > 340 g US No 1's Total Mrkble Total Yield --------------------------------------------------------Mg/ha------------------------------------------------------------------7.8 0.4 9.2 A 44.2 EFG 16.1 60.3 69.7 78.2 5.8 0.4 6.9 ABCDE 46.4 DEFG 15.5 61.9 69.0 75.5 5.8 0.0 8.7 AB 40.6 G 21.1 61.9 70.6 76.7 5.6 0.0 4.7 DEF 41.2 G 15.9 57.4 62.1 68.1 7.2 0.2 5.2 CDEF 43.3 FG 15.5 59.0 64.1 72.0 7.4 0.0 4.0 EF 49.8 BCDE 10.8 60.8 65.0 72.6 6.9 0.7 4.3 EF 41.7 G 15.7 57.4 61.9 69.7 6.7 0.0 8.5 ABC 43.0 FG 17.5 60.8 69.3 76.2 7.4 0.4 3.8 EF 49.5 BCDE 13.5 63.2 67.0 75.1 6.9 4.0 5.6 BCDEF 44.8 EFG 13.7 58.7 64.3 75.5 7.2 0.4 5.8 ABCDEF 44.4 EFG 16.4 61.0 67.0 74.9 5.6 0.2 3.8 EF 45.5 DEFG 12.1 57.6 61.6 67.7 7.8 0.4 8.1 ABCD 52.9 ABC 12.1 65.2 73.3 81.8 9.0 0.2 4.9 DEF 55.6 AB 11.0 66.6 71.5 80.9 7.4 0.0 6.7 ABCDEF 51.6 ABCD 13.2 64.8 71.7 79.4 8.3 0.4 3.4 F 48.6 CDEF 6.3 54.9 58.5 67.5 8.1 0.2 4.7 DEF 49.5 BCDE 14.1 63.9 68.8 77.3 8.3 0.2 4.7 DEF 48.9 CDEF 11.7 60.8 65.5 74.0 6.7 0.0 4.0 EF 57.2 A 14.1 71.3 75.3 82.3 NS NS * * NS NS NS NS 1.8 2.0 3.4 6.1 6.5 9.0 9.0 8.7 Specific Gravity 1.0753 1.0775 1.0759 1.0741 1.0772 1.0793 1.0785 1.0648 1.0794 1.0769 1.0698 1.0776 1.0769 1.0790 1.0516 1.0760 1.0755 1.0838 1.0823 NS 0.0144 AB AB AB AB AB A AB BC A AB AB AB AB AB C AB AB A A Total Internals % 14 6 8 8 6 6 4 8 8 10 8 14 4 12 4 26 4 10 4 NS 10.8 *Significance at the 0.1 probability level 94 95 Table 4.15. Petiole nitrate levels for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP). Values followed by the same letter are not significantly different at the 0.1 probability level. Treatments Sample Dates 49 59 95 115 ------------------------------------------g NO3-N/kg--------------------------------------ESN 330 Plant 18.9 ABC 20.0 AB 7.1 CDE 12.8 ABCD ESN 330 Emerg 19.1 AB 18.5 ABCD 15.1 A 15.4 AB ESN 290 Emerg 19.5 A 18.1 ABCD 12.9 AB 15.2 ABC ESN 250 Emerg 18.8 ABC 19.5 ABC 13.6 AB 16.6 A ESN 210 Emerg 19.0 AB 19.9 AB 14.8 AB 13.7 ABC ESN 260 Emerg 16.7 CDEFG 15.4 CDEF 14.0 AB 13.6 ABC ESN 180 Emerg 18.1 ABCD 19.4 ABC 7.9 CD 11.2 CDEF GSP 350 Emerg 17.5 ABCDEF 14.5 12.2 AB 14.3 ABC GSP 280 Emerg 17.7 ABCDE 16.0 BCDE 10.9 BC 8.8 DEFG GSP 350 Plant 17.1 BCDEF 11.6 13.7 AB 7.6 FGH SU 330 Plant 19.2 AB 20.6 A 7.7 CD 12.7 ABCD SU 260 Emerg 17.9 ABCD 19.7 ABC 7.5 CD 15.4 AB SU 104 Emerg 16.8 CDEFG 8.7 HI 4.1 DEFG 7.6 DEF 12.2 BCDE DEFG EFGH FGH 70 NF +55 UAN 15.6 EFG 11.8 EFGH 5.8 88 NF + 37 UAN 16.4 DEFG 11.4 FGH 7.1 CDE 8.3 EFG 70 NF 100 UAN 17.2 BCDEF 16.6 ABCD 3.4 EFG 3.9 H 88 NF 152 UAN 16.3 16.8 ABCD 5.3 DEFG 5.6 GH DEFG 70 NF +190 UAN 14.8 G 6.3 I 1.6 G 5.0 GH 88 NF + 242 UAN 15.5 FG 10.2 GHI 3.1 FG 3.9 H Significance * * * * LSD (0.1) 2.1 4.4 3.9 4.1 *Significance at the 0.1 probability level 96 Table 4.16. Potato plant N concentration (%) for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP). Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment Sample Dates 59 64 78 95 115 -------------------------------------------------%--------------------------------------------ESN 330 Plant 2.85 4.38 3.93 ABCD 3.44 AB 2.52 ESN 330 Emerg 2.80 3.85 4.10 ABC 3.28 AB 3.13 A ESN 290 Emerg 3.39 4.26 3.91 ABCD 3.41 AB 2.99 ABCD ESN 250 Emerg 3.74 4.29 4.29 A 3.19 ABC 3.05 AB ESN 210 Emerg 3.71 4.37 3.90 ABCDE 3.29 AB 2.80 BCDEF ESN 260 Emerg 3.38 4.18 3.69 CDEFG 3.13 ABC 2.62 EFGH ESN 180 Emerg 3.10 4.20 4.02 ABC 3.08 BC 2.53 FGHI GSP 350 Emerg 2.98 4.27 4.06 ABC 3.36 AB 3.04 ABC GSP 280 Emerg 2.95 4.48 3.82 BCDEF 3.18 ABC 2.72 GSP 350 Plant 2.59 4.45 3.87 ABCDE 3.12 ABC 2.79 BCDEFG SU 330 Plant 3.11 4.42 4.26 AB 3.49 A 2.76 CDEFGH SU 260 Emerg 2.51 4.01 3.86 ABCDE 3.40 AB 2.50 SU 104 Emerg 2.81 4.77 3.83 BCDEF 3.11 ABC 2.87 ABCDE 70 NF +55 UAN 3.10 3.29 3.50 DEFGH 3.33 AB 2.64 EFGH 88 NF + 37 UAN 2.91 4.02 3.44 EFGH 2.86 C 2.29 IJ 70 NF 100 UAN 2.39 4.57 3.40 FGH 2.38 2.11 JK 88 NF 152 UAN 2.99 4.24 3.36 GH 2.40 D 1.93 K 70 NF +190 UAN 2.66 4.33 3.20 H 2.39 D 1.87 K 88 NF + 242 UAN 3.01 4.13 3.22 H 2.30 D 1.99 K Significance NS NS * * * LSD (0.1) 0.85 0.45 0.37 0.28 0.73 *Significance at the 0.1 probability level D GHI DEFGH HI 97 GENERAL CONCLUSIONS Jess Charles Holcomb III 98 The use of enhanced efficiency nitrogen (N) fertilizers and cultivation practices were able to reduce loss of N into the environment. Agrotain-treated urea reduced NH3 loss by 71.8% over urea in grass seed. Across irrigation rates of 0.0 and 1.25-mm, N loss was 5.7 to 6.2% of N applied for Agrotain compared to urea and OAC with loss of 53.4 to 60.0% of N applied. Only at 7.6 mm of irrigation did loss decline for urea and OAC with 17.3 and 8.1%, respectively. Agrotain at 7.6 mm irrigation lost 3.17% of N applied. Agrotain also was inhibiting urease after 23 days after application compared to urea and OAC. Organo acid complex did not reduce NH3 loss unless it was incorporated into the soil. Although the use of Agrotain reduced N loss, enhanced efficiency fertilizers are not the sole options. The use of ammonium sulfate reduced NH3 loss by 60.4% of N applied compared to urea. Irrigation also reduced loss and incorporated urea; an application of 14.6 mm reduced NH3 loss by 90% compared to no irrigation. The reduction in N loss measured in the NH3 volatilization studies did not translate to increased yield in potato trials. Enhanced efficiency N products maintained yield in only one year of the study, with reduced yield for two years with Russet Burbank. Products typically produced yields similar to the 80% N treatments, suggesting N was not being released according to plant uptake. These products were able to maintain yields for two years with Russet Norkota. However, all treatments in the Russet Norkota study maintained yields; even the 80% N treatments suggested that N was not limiting. These products also make nitrate petiole sampling obsolete, as nitrate does not accurately reflect plant N levels. Since these products do not consistently maintain yield and are more expensive, they cannot be incorporated into production systems in the Columbia Basin at this time. The use of cultural practices, such as split applications of N, continue to produce maximum yields as well as reduce N loss compared to applying N all at once. Further work with these products needs to be done in order to link the reduction in environmental N loss to increased yields or lower N rates. Yield data from the nonirrigated and irrigated NH3 loss studies may have provided valuable insight into whether a reduction in N loss did result in greater yield. The N release rates from enhanced efficiency products exhibited how they reduce N loss and how it may be affecting yield. All products tested, excluding NSN and OAC, were able to delay N release compared to urea. Delay was affected by temperature, with lower temperatures leading to a longer delay period. The delay in N release protects it from loss, as less N is susceptible. It also allows more time for incorporation, further reducing loss. However, 99 delayed N can stress the plant, as adequate N is not available. Nitrogen release from these products must meet N uptake demands for the crop in order to be successful. This may be a problem since all products increased delay with cooler temperatures, so environmental conditions will affect available N on a yearly basis. Growers have multiple tools to use to reduce N loss into the environment. When applying N, applying irrigation or a non-urea N source can be used reduce N volatilization. If these are not available, the use of a urease inhibitor such as Agrotain may be used to reduce loss. However, the reduction obtained with the use of products needs to result in an increased yield or a reduction in N rate to make them viable. This may be heavily dependent on the crop and cropping system used, as evident with the lack in yield increase in the potato study. Further work needs to be done to determine into which cropping systems these products can be successfully incorporated. 100 BIBLIOGRAPHY Allison, F.E. 1955. 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Nitrate leaching and nitrogen recovery following application of polyolefin-coated urea to potato. J. Environ. Qual. 62:480-489. 110 APPENDICES 111 2 Oxalic Acid 1.8 A A Water 1.6 Absorbance 1.4 1.2 1 0.8 0.6 0.4 0.2 0 0 3 6 9 12 15 Concentration (ppm NH4-N) Figure 6.1. Absorbance from ammonium as affected by using ammonium standards in deionized water and in 0.013835 M oxalic acid. Trend lines followed by same letter are not significantly different according to p=0.05. Absorbance Absorbance 112 0.2 0.18 0.16 0.14 0.12 0.1 0.08 0.06 0.04 0.02 0 0.2 0.18 0.16 0.14 0.12 0.1 0.08 0.06 0.04 0.02 0 a) A A A A A A A A A A A A A A b) A A A A A A Figure 6.2. Absorbance from ammonia samplers tested (a) with 1 drop (4 drops NH4OH/1 L deionized water (DI)) and (b) 3 drops (4 drops NH4OH/1 L DI) as affected by the frequency of shaking with DI water. A shake represents water moving from one side of the tube to the other, continuous shaking represents rapid movement of water from ones side of tube to the other. Columns followed by same letter are not significantly different according to LSD p=0.05. 113 3.5 KCl 3 A A Water A A Concentration (ppm NH4-N) 2.5 2 B 1.5 C B C 1 0.5 0 11 Drop 3 Cleaner Drop NH NH3 Cleaner 4 Drops Drop NH 3 Cleaner NH3 Cleaner 2 mL NH3 NH3 Cleaner Cleaner 11 Drop 4OH Drop NH NH4OH Figure 6.3. Concentration from ammonia samplers tested with 1 drop, 2 drops, and 2 mL of NH3 cleaner and 1 drop (4 drops NH4OH/1 L deionized water (DI)) as affected by the extraction with deionized water or KCl solution. Columns followed by same letter are not significantly different according to LSD p=0.05. 114 0.09 0.08 0.07 Abosrbance 0.06 0.05 0.04 0.03 0.02 0.01 0 NH NH4 Free Water Water in in Burned Burned Tube Tube 4-Free NH4-Free Water NH4 Free Water Figure 6.4. Absorbance of NH4-free water compared to NH4-free water shaken in a burned tube, tube was burned at 450oC for 16 hours. 115 2.5 Ammonium Nitrate A 2 Absorbance B 1.5 1 0.5 0 0 2 4 6 8 10 12 14 16 Concentration (ppm NH4-N) Figure 6.5. Absorbance from ammonium standards as affected from the standards being ammonium or nitrate decomposed in Devarda’s alloy to ammonium. Trend lines followed by same letter are not significantly different according to p=0.05. 116 2 1.8 A A 1.6 A A 1 Hour 2 Hour 3 Hour 4 Hour 5 Hour 24 Hour 1.4 B Absorbance 1.2 C 1 0.8 0.6 0.4 0.2 0 0 2 4 6 8 10 Concentration (ppm NH4-N) 12 14 16 Figure 6.6. Absorbance from ammonium standards from nitrate decomposition in Devarda’s alloy as affected by the length of time decomposition was allowed in Devarda’s alloy. Trend lines followed by same letter are not significantly different according to p=0.05. 117 2.5 KCl Water A A 2 Absorbance 1.5 1 0.5 0 0 3 6 9 12 15 Concentration (ppm NH4-N) Figure 6.7. Absorbance from ammonium as affected by using ammonium standards in deionized water and in 2 M KCl solution. Trend lines followed by same letter are not significantly different according to p=0.05. Urea Background Agrotain Background Urea Background Agrotain 120 N loss as NH3 (% N applied) 100 80 60 40 20 0 0 5 10 15 20 25 30 Days after application Figure 6.8. Cumulative loss of NH3 during the period of 29 July to 24 August 2009 following application of 112 kg N/ha to wheat stubble as affected by N source of urea and Agrotain coated urea. Background represents NH3 flux between treatment plots. 118 119 7 6 Nitrogen Loss (kg/ha/12 hrs) 5 4 3 2 1 Aug 3; PM Aug 3; AM Aug 2; PM Aug 2; AM Aug 1; PM Aug 1; AM Jul 31; PM Jul 31; AM Jul 30; PM 0 Figure 6.9. Average diurnal nitrogen loss as ammonia across treatments on wheat stubble after application of 112 kg N/ha. 120 100 Urea 90 Agrotain 80 N loss as NH3 (% of N applied) 70 60 50 40 30 20 10 0 0 4 8 Days after application 12 16 Figure 6.10. Cumulative loss of NH3 during the period of 23 October to 9 November 2009 following application of 112 kg N/ha to unburned grass seed field as affected by N source of urea vs. Agrotain-coated urea. Bars represent standard error. 121 30 A Grass Burn (% of plot burned) 25 20 15 10 5 B 0 Urea Agrotain Figure 6.11. Percent of plots burned after the application of 112 kg N/ha to unburned grass seed field as affect by N source of urea and Agrotain-coated urea. Columns followed by same letter are not significantly different according to LSD p=0.05. 122 10.1 cm Soil moisture (mm water/100mm soil) 0.25 20.3 cm 30.4 cm 50.8 cm 91.4 cm a) 0.2 0.15 0.1 0.05 0 24 20 16 12 8 4 0 Days After Application 0.25 Soil moisture (mm water/100mm soil) b) 0.2 0.15 0.1 0.05 0 24 20 16 12 8 4 0 Days After Application Soil moisture (mm water/100mm soil) 0.25 c) 0.2 0.15 0.1 0.05 0 0 4 8 Days After12 Application 16 20 24 Figure 6.12. Soil moisture at varying depths for irrigation rates (a) 0.0 mm, (b) 3.8 mm, and (c) 11.4 mm. Moisture probe at irrigation rate 0.0 mm (a) was removed 17 DAA. 123 Urea Agrotain Super-u NSN ESN Nitamin N-fusion 60 Available NO3 (% N applied) a) 50 40 30 20 10 0 0 20 40 60 80 100 160 b) Available N (% N applied) 140 120 100 80 60 40 20 0 0 20 40 60 Days after application 80 100 Figure 6.13. Available (a) NO3 and (b) total N (NH4 + NO3) at 4.4oC in incubation as affected by N treatment. 124 Urea Agrotain Super-u NSN ESN Nitamin N-fusion 70 Available NO3 (% N applied) a) 60 50 40 30 20 10 0 0 20 40 60 80 100 160 b) Available N (% N applied) 140 120 100 80 60 40 20 0 0 20 40 60 Days after application 80 100 Figure 6.14. Available (a) NO3 and (b) total N (NH4 + NO3) at 15.6oC in incubation as affected by N treatment. 125 Urea Agrotain Super-u NSN ESN Nitamin N-fusion Available NO3 (% N applied) 100 a) 90 80 70 60 50 40 30 20 10 0 0 20 40 60 80 100 b) 140 Available N (% N applied) 120 100 80 60 40 20 0 0 20 40Days after application 60 80 100 Figure 6.15. Available (a) NO3 and (b) total N (NH4 + NO3) at 26.7oC in incubation as affected by N treatment. 126 90 80 70 Urea % Fertilizer 60 NSN 50 40 30 20 10 0 >4 2.38 - 4 2 - 2.38 Size (mm) 0.841 - 2 0.595 - 0.841 Figure 6.16. Size of fertilizer prills based on product. Agrotain is coated urea, so it would have the same percentages as urea. 127 Table 6.1. Linear regression for absorbance from N standards with concentrations ranging from 0 to 15 ppm NH4-N as affected by time of color determination. R 2 Time Intercept Slope Hours Absorbance Absorbance/ppm NH4-N 0 0.05403 B† 0.10942 B† 0.9989 0.5 0.07128 A 0.11808 A 0.9987 1 0.0716 A 0.11802 A 0.9987 2 0.07055 A 0.1178 A 0.9987 3 0.07144 A 0.11736 A 0.9986 † Within a column, values followed by the same letter are not significantly different according to LSD at P = 0.05. 128 Table 6.2. Ammonium levels measured after nitrate decomposition as affected by the initial rate of nitrate added to Devarda’s alloy. Added NO3-N to Devarda’s Alloy ppm NO3-N 25 100 200 400 800 1000 Average Measured NH4-N ppm NH4-N 27.13 23.14 25.83 25.48 18.57 15.36 22.58 129 Table 6.3. Average 12-hour weather data for diurnal wheat stubble data. No precipitation occurred. Date 2009 7/30; PM 7/31; AM 7/31; PM 8/1; AM 8/1; PM 8/2; AM 8/2; PM 8/3; AM 8/3; PM Air Temp O C 33.8 24.2 35.3 25.1 37.7 27.8 34.9 27.2 32.9 2 Inch Soil Temp O C 31.9 27.1 32.4 27.3 33.1 28.7 33.7 28.9 33.0 Wind Speed m/s 2.3 1.2 2.1 1.4 1.7 1.5 1.6 2.6 3.6 Rel. Hum. % 21.8 45.6 21.3 40.3 20.1 39.4 18.1 36.5 18.8 130 Table 6.4. Average ppm nitrogen (N) as ammonia for the sampling period before (Aug 6), during (Aug 7), and after (Aug 10) a smoke event. Samplers refer to height of ammonia collection. Height of samplers m 3.00 2.25 1.50 0.75 0.50 Total Before Aug 6 ppm N 2.68 1.13 1.79 2.64 5.24 13.49 SMOKE Aug 7 ppm N 1.94 2.20 2.96 6.45 10.97 24.51 After Aug 10 ppm N 0.92 1.05 0.96 1.47 2.43 6.85 131 Table 6.5. Cumulative loss of NH3 from plots during 1 hour on 20 November 2009 resulting from the application of waste water to an alfalfa field through irrigation. Plot N loss as NH3 kg N/ha 1 0.034 2 0.031 3 0.070 132 Table 6.6. Soil N present as NH4 and NO3 at varying soil depth after the application of 112 kg N as urea/ha as affected by irrigation rate. Irrigation Rate Soil Depth -------0-2.5 cm----- -----0-15.2 cm ----- -----0-30.4 cm ------- mm NH4 NH4 NH4 0 33.7 10.9 B 34.9 27.4 97.4 26.5 1.25 42.0 13.3 B 33.0 17.3 157.7 20.0 3.8 24.7 17.1 AB 46.4 24.7 107.3 20.5 7.6 18.8 19.8 AB 11.0 38.0 102.3 30.8 11.4 15.6 25.7 A 18.5 28.5 65.0 31.1 21.6 9.6 22.9 A 14.2 45.5 24.2 43.3 Significance NS * NS NS NS NS NO3 NO3 NO3 ------------------------------------kg N/ha---------------------------------------- † Within a column, values followed by the same letter are not significantly different according to LSD at P = 0.05. 133 Table 6.7. Soil pH at varying soil depths after the application of 112 kg N ha-1 as urea as affected by irrigation rate. Irrigation Rate mm 0.0 0.1 0.25 0.5 0.75 1.0 Significance Soil Depth 0-2.5 cm 0-15.2 cm 0-30.4 cm --------------------pH-----------------5.85 6.32 6.51 5.85 6.36 6.20 5.88 6.13 6.29 6.04 6.07 6.51 5.72 6.24 6.50 5.88 6.25 6.27 NS NS NS 134 Table 6.8. Accountable N at varying soil depth after the application of 112 kg N ha-1 as urea as affected by irrigation rate; accountable N = wheat N uptake + soil N corresponding to soil depth. Irrigation Rate Soil Depth 0-2.5 cm 0-15.2 cm 0-30.4 cm mm ------------------------------------kg N/ha----------------------------------- 0 169.5 187.2 248.7 1.25 234.5 229.6 357.0 3.8 235.5 264.8 321.5 7.6 213.4 223.8 307.9 11.4 214.4 220.0 269.2 21.6 201.9 229.1 236.9 Significance NS NS NS 135 Table 6.9. Soil pH at varying soil depths after the application of 112 kg N/ha as affected by irrigation rate and N source. N Source Urea Agrotain OAC Urea Agrotain OAC Urea Agrotain OAC N Source Irrigation Rate Treatment*N Source Irrigation Rate mm 0.00 0.00 0.00 1.25 1.25 1.25 7.6 7.6 7.6 Soil Depth 0-2.5 0-15.2 0-30.4 cm cm cm ---------------------pH-----------------5.85 6.32 6.51 6.42 6.30 6.87 6.09 6.33 6.39 5.85 6.36 6.20 6.04 6.08 6.41 5.94 6.12 6.40 6.04 6.07 6.51 5.92 6.19 6.55 6.08 5.98 6.61 NS NS NS NS NS NS NS NS NS 136 Table 6.10. Soil N present as NH4 and NO3 at varying soil depth after the application of 112 kg N/ha as affected by irrigation rate and N-source. N-Source Irrigation Rate Soil Depth mm -0-2.5 cmNH4 NO3 Urea 0.00 ------------------------kg N/ha----------------------33.7 10.9 34.9 27.4 97.4 26.5 Agrotain 0.00 53.7 13.6 93.1 24.8 60.4 23.7 OAC Urea 0.00 1.25 22.2 42.0 17.3 13.3 43.9 33.0 18.8 17.3 89.9 157.7 12.7 20.0 Agrotain OAC 1.25 1.25 45.7 26.8 14.6 20.8 53.4 40.9 15.4 7.2 124.7 92.6 16.2 9.7 Urea 7.6 18.8 19.8 11.0 38.0 102.3 30.8 Agrotain OAC Irrigation N-Source 7.6 7.6 20.8 9.5 * * 25.3 28.3 * * 46.4 40.0 * * 22.5 29.0 NS NS 52.9 88.9 * NS 39.3 22.7 NS NS NS NS NS NS NS NS Irrigation*N Source -0-15.2 cmNH4 NO3 -0-30.4 cmNH4 NO3 137 Table 6.11. Accountable N at varying soil depth after the application of 112 kg N/ha as affected by irrigation rate and N Source; accountable N = wheat N uptake + soil N corresponding to soil depth. N-Source Irrigation Rate Soil Depth 0-2.5 cm 0-15.2 cm 0-30.4 cm mm ---------------kg N/ha----------------- Urea 0 113.8 131.5 193.1 Agrotain 0 161.9 212.6 178.8 OAC 0 105.9 129.1 169.1 Urea 1.25 147.9 143.0 270.4 Agrotain 1.25 158.4 167.0 239.0 OAC 1.25 93.4 93.9 148.1 Urea 7.6 102.6 113.0 197.1 Agrotain 7.6 108.4 131.2 154.5 OAC 7.6 113.9 145.1 187.7 Irrigation NS NS NS N-Source NS NS NS Irrigation*N Source NS NS NS 138 Table 6.12. Urease activity 104 days after application of N fertilizer as affected by N source and incubation temperature. N-Source o Temperature ( C) 4.4 15.6 26.7 --------μg NH4-N/(g h)-------Control 0.72 1.83 1.32 Urea 0.29 0.85 1.75 Agrotain 1.16 0.56 0.12 Super-U 0.31 0.43 1.75 NSN 0.74 1.85 0.41 ESN 0 1.71 0.27 Nitamin 0.21 0.48 0.99 N-fusion 0.48 0.54 1.28 Treatment NS NS NS Temp NS NS NS Temp*Treat NS NS NS 139 Table 6.13. Potato vine mass for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP). Treatment Sample Date 60 64 78 95 113 ------------------------------Mg/ha------------------------------ESN 330 Plant 5.51 4.39 4.77 4.48 1.79 ESN 330 Emerg 7.69 3.74 4.95 4.73 2.35 ESN 290 Emerg 5.96 4.55 4.42 4.93 3.21 ESN 250 Emerg 6.14 3.74 5.63 6.05 3.12 ESN 210 Emerg 7.17 3.59 4.73 5.38 3.09 ESN 260 Emerg 6.61 4.06 4.19 5.56 2.31 ESN 180 Emerg 7.31 4.60 5.45 5.47 2.44 GSP 350 Emerg 5.25 4.26 4.84 6.48 2.73 GSP 280 Emerg 7.26 4.42 5.22 5.60 2.91 GSP 350 Plant 4.69 2.87 5.65 4.51 2.26 SU 330 Plant 6.19 3.92 4.69 6.23 2.49 SU 260 Emerg 4.55 4.42 4.75 5.02 2.47 SU 104 Emerg 6.75 3.12 5.02 5.58 2.20 70 NF +55 UAN 4.01 4.21 4.80 6.37 2.62 88 NF + 37 UAN 5.96 5.18 4.55 5.25 1.37 70 NF 100 UAN 4.57 4.55 4.30 4.35 1.97 88 NF 152 UAN 6.86 4.93 4.71 4.10 2.58 70 NF +190 UAN 6.14 4.15 5.25 4.37 1.88 88 NF + 242 UAN 8.63 4.55 4.55 3.83 1.59 Significance NS NS NS NS NS 140 Table 6.14. Potato mass for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP). Treatment ESN 330 Plant ESN 330 Emerg ESN 290 Emerg ESN 250 Emerg ESN 210 Emerg ESN 260 Emerg ESN 180 Emerg GSP 350 Emerg GSP 280 Emerg GSP 350 Plant SU 330 Plant SU 260 Emerg SU 104 Emerg 70 NF +55 UAN 88 NF + 37 UAN 70 NF 100 UAN 88 NF 152 UAN 70 NF +190 UAN 88 NF + 242 UAN Significance Sample Date 78 95 113 -------------Mg/ha-----------0.16 1.84 3.56 1.23 3.43 3.90 0.45 2.00 5.25 1.14 2.51 5.42 1.39 1.79 4.39 1.48 8.32 4.91 1.05 2.60 5.69 0.94 1.97 4.35 1.35 1.43 4.24 0.63 2.08 4.53 0.47 3.07 4.75 1.10 1.86 5.74 0.99 2.73 4.77 0.54 3.03 4.98 1.05 3.27 4.69 1.23 1.93 5.96 1.48 3.03 7.26 1.39 3.41 4.51 1.01 2.62 4.84 NS NS NS 141 Table 6.15. Potato plant N uptake for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP). Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment ESN 330 Plant ESN 330 Emerg ESN 290 Emerg ESN 250 Emerg ESN 210 Emerg ESN 260 Emerg ESN 180 Emerg GSP 350 Emerg GSP 280 Emerg GSP 350 Plant SU 330 Plant SU 260 Emerg SU 104 Emerg 70 NF +55 UAN 88 NF + 37 UAN 70 NF 100 UAN 88 NF 152 UAN 70 NF +190 UAN 88 NF + 242 UAN Significance Sample Date 60 64 78 95 113 ------------------------lbs N/acre--------------------------------308.7 384.0 373.7 304.1 BCD 91.9 CDE 428.2 286.5 406.4 312.2 ABC 147.7 ABC 410.2 382.9 354.2 343.4 AB 192.7 A 471.2 322.4 486.2 392.0 AB 193.9 A 544.7 309.8 380.6 353.2 AB 177.3 AB 464.5 337.2 307.3 350.1 AB 125.9 BCD 466.9 232.2 437.4 350.6 AB 123.5 BCDE 309.8 360.2 391.6 432.4 A 170.1 AB 419.6 396.1 402.6 365.6 AB 160.7 AB 235.2 257.6 437.8 286.2 BCD 129.1 BCD 373.5 328.0 405.1 431.3 A 139.4 ABC 221.3 340.3 372.1 339.3 AB 121.2 BCDE 379.7 297.0 383.6 349.7 AB 123.2 BCDE 250.4 270.8 339.2 434.8 A 144.8 ABC 365.6 398.6 321.2 299.2 BCD 64.3 E 209.2 417.9 287.4 208.6 CD 86.9 CDE 455.3 406.2 316.8 195.7 CD 97.2 CDE 345.0 322.6 337.2 211.2 CD 73.0 DE 552.4 380.9 301.7 180.2 D 63.2 E NS NS NS * * *Significance at the 0.1 probability level 142 Table 6.16. Potato N concentration (%) for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP). Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment ESN 330 Plant ESN 330 Emerg ESN 290 Emerg ESN 250 Emerg ESN 210 Emerg ESN 260 Emerg ESN 180 Emerg GSP 350 Emerg GSP 280 Emerg GSP 350 Plant SU 330 Plant SU 260 Emerg SU 104 Emerg 70 NF +55 UAN 88 NF + 37 UAN 70 NF 100 UAN 88 NF 152 UAN 70 NF +190 UAN 88 NF + 242 UAN Treatment Sample Date 78 95 113 -------------------% N------------------1.5785 1.532 1.524 1.528 1.602 1.552 1.6415 1.504 1.424 1.74 1.53 1.484 1.87 1.56 1.424 1.6265 1.524 1.38 1.572 1.566 1.436 1.674 1.618 1.594 1.508 1.542 1.5 1.566 1.594 1.402 1.676 1.542 1.552 1.752 1.58 1.428 1.564 1.588 1.48 1.516 1.6167 1.456 1.484 1.416 1.454 1.666 1.51 1.35 1.6 1.466 1.346 1.51 1.422 1.32 1.48 1.434 1.456 NS NS NS *Significance at the 0.1 probability level 143 Table 6.17. Potato N uptake for Russet Burbank in 2009 as affected by N treatment and sampling date (DAP). Values followed by the same letter are not significantly different at the 0.1 probability level. Treatment ESN 330 Plant ESN 330 Emerg ESN 290 Emerg ESN 250 Emerg ESN 210 Emerg ESN 260 Emerg ESN 180 Emerg GSP 350 Emerg GSP 280 Emerg GSP 350 Plant SU 330 Plant SU 260 Emerg SU 104 Emerg 70 NF +55 UAN 88 NF + 37 UAN 70 NF 100 UAN 88 NF 152 UAN 70 NF +190 UAN 88 NF + 242 UAN Treatment Sample Date 78 95 113 -------------Mg/ha------------5.8 55.6 114.8 38.1 111.9 118.1 15.7 59.9 156.7 40.1 74.9 165.2 51.3 54.7 124.9 49.5 244.1 135.2 34.3 76.7 163.0 31.6 59.9 137.9 41.9 44.2 125.8 21.1 64.3 130.7 15.5 91.9 145.7 36.5 58.1 157.8 32.1 88.3 138.1 17.5 70.4 144.1 25.3 93.9 140.1 41.5 60.3 159.6 48.6 88.1 185.4 41.5 92.4 113.2 28.7 74.0 139.7 NS NS NS *Significance at the 0.1 probability level 144 Table 6.18. Linear regression for NH3 loss from 2 DAA to 8 DAA following application of 112 kg urea-N/ha to Winter Wheat as affected by rate of irrigation application. Irrigation Rate Slope R2 -1 mm % N applied day 0.0 7.41 A† 0.6305 1.25 6.64 A 0.7673 3.8 4.71 B 0.9542 7.6 1.89 C 0.7068 11.4 0.59 D 0.3613 21.6 0.15 D 0.0334 † Within a column, values followed by the same letter are not significantly different according to LSD at P = 0.05. 145 Table 6.19. Linear regression for NH3 loss from 2 DAA to 8 DAA following application of 112 kg urea-N/ha to Winter Wheat as affected by N treatment and rate of irrigation application. N Irrigation Treatment rate mm Daily N loss as NH3 Significant Difference R2 % N applied kg N ha-1day-1 Within Across -1 day Irrigation Irrigation Urea 0.00 7.41 8.30 A† a‡ 0.6305 Agrotain 0.00 0.49 0.54 B d 0.4903 OAC 0.00 7.46 8.36 A a 0.8334 Urea 1.25 6.64 7.43 A a 0.7673 Agrotain 1.25 0.32 0.35 B d 0.6568 OAC 1.25 7.20 8.05 A a 0.8073 Urea 7.60 1.89 2.11 A b 0.7068 Agrotain 7.60 0.18 0.35 C d 0.1269 OAC 7.60 0.94 1.05 B c 0.8755 † Within a column and irrigation rate, daily loss values followed by the same letter are not significantly different according to LSD at P = 0.05. ‡Within a column, daily loss values followed by the same letter are not significantly different according to LSD at P=0.05. 146 Table 6.20. Soil urease activity in incubation as affected by N treatment and temperature. N-Source Control Urea Agrotain Super-U NSN ESN Nitamin N-Fusion Control Urea Agrotain Super-U NSN ESN Nitamin N-Fusion Control Urea Agrotain Super-U NSN ESN Nitamin N-Fusion N-Source Temperature Interaction Temperature (oC) 4.4 4.4 4.4 4.4 4.4 4.4 4.4 4.4 15.6 15.6 15.6 15.6 15.6 15.6 15.6 15.6 26.7 26.7 26.7 26.7 26.7 26.7 26.7 26.7 Urease Activity 3.60 1.45 5.80 1.55 3.70 0.00 1.05 2.40 9.15 4.25 2.80 2.15 9.25 8.55 2.40 2.70 6.60 8.75 0.60 8.75 2.05 1.35 4.95 8.40 NS NS NS Table 6.21. Available NH4 at 4.4oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 34 48 63 76 104 91.0 A 91.0 A 94.8 A 78.7 A 89.8 A NH4 Urea 15.0 A 37.2 A 64.3 A Agrotain 4.0 C 5.8 C 10.3 Super-U 3.0 CD 4.9 C 8.3 NSN 13.9 A 33.7 A 60.4 B ESN 2.4 7.1 C 20.2 Nitamin 6.8 B N-Fusion 0.0 Standard Error 0.5 D E 95.6 A E E D 95.6 A 96.3 A 18.9 D 25.1 C 33.9 C 41.7 C 59.0 B 84.4 A 81.1 A 93.4 A 15.6 D 19.8 C 26.4 30.5 48.6 C 72.7 B 74.8 A 84.6 A 98.5 A 101.0 A 101.4 A 95.8 A 93.0 A 91.8 A 81.1 A 92.0 A 36.5 C 46.6 B 51.5 B 52.8 B 55.8 B 54.2 C 48.6 B 48.6 B D D 20.5 B 40.0 C 48.8 B 51.4 B 54.2 B 55.8 B 54.6 BC 52.2 C 43.9 B 38.3 C 0.0 2.4 3.5 5.5 8.5 9.8 11.5 14.6 16.7 C 16.5 5.0 4.6 1.8 D 1.7 F 3.1 E 2.7 D 2.7 E 2.5 E 2.9 D 5.2 D D 147 Table 6.22. Available NO3 at 4.4oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 34 48 63 76 104 40.6 AB 3.6 B 18.1 AB 27.9 B 17.2 B NO3 Urea 0.0 A 0.0 B Agrotain 0.0 A 0.6 AB 0.0 B 0.1 B 0.0 A 2.3 B 10.0 C 14.0 A 16.0 ABC 28.6 B 21.8 B Super-U 0.0 A 3.5 A 0.0 B 0.0 B 0.0 A 2.9 B 8.5 C 2.7 B 27.8 A 25.2 B 16.4 B NSN 0.0 A 0.2 B 2.0 A 7.5 A 9.0 A 14.2 A 51.2 A 9.4 AB 20.9 A 25.7 B 16.9 B ESN 0.3 A 0.4 B 1.7 A 3.0 AB 1.7 A 2.6 B 21.3 BC 7.9 AB 11.0 ABC 41.2 A 46.6 A 0.4 AB 2.8 AB 7.0 A 8.9 AB Nitamin 0.0 A 0.0 B 0.0 B 0.0 B 0.0 A 0.5 B 0.5 C 0.0 B 0.9 BC 14.2 C 21.2 B N-Fusion 0.0 A 0.0 B 0.0 B 0.0 B 0.0 A 0.0 B 1.1 C 0.0 B 0.0 C 0.0 8.6 C Standard Error 0.1 1.4 0.7 2.7 5.3 4.6 11.8 4.7 8.0 2.6 D 2.8 148 Table 6.23. Total N (NH4 + NO3) at 4.4oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 34 48 63 76 104 93.3 A 112.9 A 106.6 A 107.1 AB Total N (NH4 + NO3) Urea 15.0 A 36.9 A 64.5 A 96.9 A 101.3 A 105.2 A 131.7 A Agrotain 4.0 C 6.3 C 9.5 D 18.5 C 22.7 C 35.3 C 51.7 BC 72.7 B 100.4 A 109.7 A 115.2 A Super-U 3.0 CD 8.4 C 7.8 D 14.9 C 17.4 CD 28.8 C 39.0 CD 51.0 D 100.6 A 100.0 AB 101.1 BC NSN 13.9 A 33.9 A 62.0 A 105.3 A 107.2 A 115.7 A 147.1 A 102.5 A 112.8 A 106.8 A 109.0 AB ESN 2.7 7.4 C 21.6 C 39.3 B 46.7 B 53.2 B 74.1 B 63.8 BC 65.2 B 89.9 B 95.3 C D Nitamin 6.8 B N-Fusion 0.0 Standard Error 0.5 E 20.3 B 38.7 B 46.5 B 47.4 B 53.8 B 55.5 BC 52.3 CD 52.3 B 58.1 C 59.5 D 0.0 1.1 1.2 D 1.2 5.6 D 10.8 8.0 13.0 C 12.4 25.2 E 6.2 8.0 6.4 13.2 10.0 5.5 2.4 D 1.7 E D D 5.8 E D 4.9 149 Table 6.24. Available NH4 at 15.6oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 34 48 63 76 104 97.2 A 61.2 C 56.5 B 52.3 B 45.4 B NH4 Urea 26.1 A 86.90 A Agrotain 4.8 D 11.1 CD 16.9 C 38.0 D 79.3 B 107.3 A 104.6 A 81.4 B 60.9 B 54.4 B 46.1 B Super-U 3.7 D 8.3 CD 14.0 C 34.1 D 75.7 B 108.1 A 103.9 A 99.5 A 83.4 A 72.4 A 71.4 A NSN 22.8 B 77.1 A 77.0 AB 104.0 A 106.7 A 104.3 A 97.8 A 62.7 C 56.2 B 52.9 B 45.2 B ESN 3.9 18.5 C 35.2 C 50.7 C 55.0 C 45.7 B 48.0 B 49.6 D 49.4 C 48.0 C 39.4 C Nitamin 13.5 C 54.2 B 62.3 B 59.7 B 57.3 C 41.5 B 39.7 C 39.1 E 42.1 D 42.6 D 43.8 B N-Fusion 0.0 6.3 12.2 C 19.5 22.9 C 20.3 22.2 F 25.6 E 27.3 E 29.4 Standard Error 1.0 11.2 2.4 24.0 D 3.6 3.1 3.7 D E 5.1 D 96.7 A 103.8 A E 106.9 A 104.2 A D 2.4 2.6 1.4 D 1.2 150 Table 6.25. Available NO3 at 15.6oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 34 48 63 76 104 39.3 C 39.9 AB 60.1 A 45.1 C NO3 Urea 0.0 A 0.0 C 5.1 B 0.1 A 2.0 B 5.6 BC 6.7 BC Agrotain 0.0 A 0.0 C 1.0 B 0.0 A 9.3 B 19.6 A 42.3 A 32.0 C 41.1 A 54.2 AB 51.5 BC Super-U 0.0 A 0.0 C 0.0 B 3.3 A 12.1 AB 12.9 ABC 7.6 BC 5.1 28.5 C 54.1 AB 29.4 NSN 0.2 A 11.5 A 36.2 A 1.3 A 10.6 AB 6.2 BC 16.3 BC 61.3 A 40.5 A 49.2 BC 53.9 B ESN 0.0 A 3.4 B 1.6 B 1.4 A 26.4 A 24.9 A 31.2 AB 50.4 B 46.2 A 42.3 C 62.5 A Nitamin 0.0 A 0.2 C 0.0 B 0.0 A 9.4 AB 16.9 AB 13.6 BC 36.3 C 30.1 BC 32.1 D 29.4 D N-Fusion 0.0 A 0.0 C 0.0 B 0.0 A 0.0 B 3.3 C 1.7 C 13.4 15.3 13.9 E 13.5 E Standard Error 0.1 1.0 10.1 1.9 7.9 5.5 11.9 3.7 E D 4.6 D 4.2 D 3.7 151 Table 6.26. Total N (NH4 + NO3) at 15.6oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 34 48 63 76 104 100.6 C 96.56 B 112.5 B 90.6 B Total N (NH4 + NO3) Urea 26.1 A 86.6 A Agrotain 4.8 D 10.9 CD 17.9 D Super-U 3.7 D 8.0 12.8 D NSN 23.0 B 88.6 A 113.3 A ESN 3.9 21.9 C 36.4 C D D 101.8 A 103.0 A 106.2 AB 109.1 B 101.7 BC 36.9 C 87.2 BC 127.0 A 146.9 A 113.4 B 102.0 B 108.7 B 97.6 A 36.6 C 86.4 BC 121.0 AB 110.2 B 102.9 C 111.9 A 126.5 A 100.8 A 104.9 A 116.4 A 110.6 B 114.2 B 124.0 A 96.7 B 95.3 C 99.1 A 52.1 B 81.5 BC 70.6 C 79.3 CD 100.0 C 95.6 B 97.2 C 101.9 A Nitamin 13.5 C 54.3 B 61.0 B 58.3 B 66.7 C 58.4 C 53.4 D 75.4 D 72.2 C 74.8 D 73.2 C N-Fusion 0.0 6.0 10.9 18.1 20.0 25.2 20.4 E 35.6 E 40.9 41.3 E 42.9 Standard Error 1.0 E 5.2 D 6.4 D 3.2 D 11.6 D 7.6 D 13.4 3.5 3.0 D 4.3 D 3.2 152 Table 6.27. Available NH4 at 26.7oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 34 48 63 76 104 86.2 AB 69.6 B 56.9 B 44.8 CD 40.8 CD 41.1 BC 37.1 CD NH4 Urea 21.4 A 34.3 B 89.3 B 99.7 A 109.7 A Agrotain 4.0 D 5.3 D 12.4 E 74.9 B 105.8 A 73.0 B 62.5 B 55.4 B 44.5 CD 39.6 Super-U 2.9 DE 5.4 D 11.5 E 73.5 B 109.9 A 98.5 A 87.4 A 71.9 A 70.8 A 66.3 A 65.7 A NSN 18.4 B 48.0 A 98.2 A 103.6 A 104.1 A 92.4 A 72.1 B 59.0 B 51.5 B 45.5 BC 43.7 B ESN 1.4 4.2 22.9 32.2 34.5 B 35.0 C 36.0 C 36.0 40.1 36.4 34.4 53.5 C 39.0 B 38.0 C 39.9 C 43.0 C 46.5 BC 45.9 B 23.9 21.2 C 25.6 C 27.0 C 32.2 35.3 33.9 4.9 6.3 6.4 1.8 EF Nitamin 9.0 C N-Fusion 0.0 Standard Error 0.8 F D D 27.6 C 56.3 C 0.0 6.24 1.1 E 2.0 F 4.4 D D D D 2.4 DE E 2.3 D DE D 40.1 BC E 38.7 CD 2.2 153 Table 6.28. Available NO3 at 26.7oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 34 48 63 76 104 36.6 AB 58.1 AB 60.3 A 63.0 A 49.7 NO3 Urea 0.0 A 8.4 A 12.8 A 0.2 C 2.3 A 22.0 AB D Agrotain 0.0 A 0.0 C 0.0 B 3.5 BC 0.2 A 35.3 A 41.7 AB 43.6 BC 47.5 AB 50.4 AB 80.4 AB Super-U 0.0 A 0.0 C 0.0 B 0.0 C 0.0 A 4.4 B 23.7 B 34.4 C 29.4 BCD 41.5 B 71.3 ABC NSN 0.1 A 2.1 B 0.0 B 1.4 BC 2.5 A 11.5 B 34.2 AB 45.8 BC 36.0 BC 49.9 AB 75.4 ABC ESN 0.0 A 0.0 C 0.0 B 16.5 A 3.1 A 39.2 A 52.9 A 67.1 A 64.3 A 63.6 A 86.9 A Nitamin 0.0 A 0.0 C 0.0 B 4.8 B 8.1 A 22.5 AB 24.6 B 32.8 C 25.7 CD 34.3 B 59.8 CD N-Fusion 0.0 A 0.0 C 0.0 B 0.0 C 4.3 A 21.0 AB 24.3 B 34.2 C 16.7 38.2 B 66.5 BCD Standard Error 0.1 0.4 1.0 1.9 4.9 9.8 11.3 7.4 8.4 9.3 9.4 D 154 Table 6.29. Total N (NH4 + NO3) at 26.7oC in incubation as affected by N treatment. Values followed by the same letter are not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 34 48 63 76 104 Total N (NH4 + NO3) Urea 21.4 A Agrotain 4.01 D 5.2 D 11.0 D Super-U 2.9 DE 5.2 D 10.2 DE NSN 18.6 B 50.1 A 97.3 A ESN 1.4 4.0 21.9 C 42.7 B EF Nitamin 9.0 C N-Fusion 0.0 Standard Error 0.8 F D 102.1 A 99.3 A 108.8 A 105.9 A 106.2 A 115.0 A 105.2 A 103.8 A 90.8 C 77.8 B 102.6 A 108.4 A 104.2 A 99.1 A 92.1 A 90.1 ABC 117.6 AB 71.5 B 106.5 A 101.7 A 111.1 A 106.3 A 100.3 A 107.8 A 137.1 A 104.4 A 104.9 A 102.4 A 106.4 A 104.9 A 87.6 AB 95.5 AB 119.2 AB 48.8 C 35.9 BC 74.3 B 88.9 AB 103.2 A 104.4 A 100.1 AB 121.3 AB 27.4 C 54.9 B 58.4 C 43.8 B 60.6 BC 64.5 BC 75.8 B 72.3 B 80.3 BC 99.9 BC 0.0 4.9 21.9 23.8 C 46.6 C 51.4 C 66.5 B 52.1 C 72.2 C 105.2 BC 8.1 12.2 11.6 8.8 8.9 10.0 10.7 1.2 E 2.7 E 4.9 D 155 Table 6.30. Soil pH at 4.4oCin incubation as affected by N treatment. Values followed by a like letter at not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 F 7.70 C 8.30 A 28 34 48 63 76 104 7.94 A 7.81 C 7.61 7.59 C 7.45 C 7.69 7.72 CD 7.51 7.41 CD 7.88 B 7.59 C 7.56 B pH Control 7.01 Urea 7.79 AB 8.15 A 7.92 BC 7.72 C 7.68 Agrotain 7.30 D 7.61 CD 7.80 D 8.06 AB 8.21 B Super-U 7.28 DE 7.58 7.67 NSN 7.84 A ESN 7.19 Nitamin N-Fusion Standard Error F 7.09 E 8.24 A D 7.67 E 8.15 B 7.34 E 7.86 B D 7.98 A DE E 8.12 AB 8.20 B 8.18 B 7.97 AB 7.86 B 7.47 E 7.36 7.89 BC 7.75 C 7.72 7.67 E 7.33 E 7.70 7.74 C 7.44 E 7.39 CD 7.74 BC 7.94 B 8.12 A 8.13 C 8.02 D 7.66 D 7.91 B 8.06 A 7.71 B 7.59 B 7.70 BC 8.03 A 8.10 A 8.11 AB 8.09 C 8.06 D 7.73 C 7.99 A 8.07 A 7.79 A 7.72 A 7.60 C 7.78 B 7.85 CD 8.05 B 8.19 B 8.11 C 7.84 B 7.98 A 8.06 A 7.57 CD 7.29 0.04 0.07 0.03 0.03 0.02 0.01 0.01 0.02 0.05 0.03 0.02 D 7.91 A D 8.01 A E D 7.28 D D E 156 Table 6.31. Soil pH at 15.6oCin incubation as affected by N treatment. Values followed by a like letter at not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 8.18 A 34 48 8.03 A 7.70 63 76 104 7.34 AB 7.38 A pH Control 6.95 Urea 7.95 A 7.89 BC Agrotain 7.37 C Super-U NSN D 7.22 D 7.36 D 7.57 D 8.32 A 7.53 C 7.57 D 7.70 7.82 C 7.89 B 8.11 A 7.29 C 7.88 BC 7.89 B 8.12 A 7.93 A 7.91 BC 7.50 C 7.61 ESN 7.30 C 7.94 AB 8.03 A 7.96 C 8.05 C 7.93 C Nitamin 7.92 A 8.03 A 7.95 AB 7.92 C 7.96 N-Fusion Standard Error 7.59 B 7.96 AB 7.95 AB 8.05 B 0.04 0.05 0.03 0.02 E 8.03 C 8.07 C D D 7.72 D 7.56 E 7.39 E 7.88 A 8.07 A 7.49 A 6.70 C 7.62 D 7.45 DE 7.75 BCD 8.04 A 7.55 A 6.49 C 7.64 D 7.47 D 7.72 CD 7.88 BC 7.44 AB 7.36 A 7.42 DE 7.84 AB 8.00 AB 7.51 A 6.56 C 7.69 C 7.67 D 7.39 E 6.87 C 5.68 8.01 B 7.80 B 7.42 E 7.53 E 7.07 BC 7.02 B 8.16 B 8.06 B 7.87 B 7.81 ABC 7.82 CD 7.34 AB 7.25 A 0.02 0.02 0.03 0.05 0.06 0.18 0.10 7.62 F D 7.50 F D 157 Table 6.32. Soil pH at 26.7oC in incubation as affected by N treatment. Values followed by a like letter at not significantly different at p=0.05. Treatment Days After Application 1 3 6 13 20 28 34 48 63 76 104 pH Control 7.00 Urea 7.97 A Agrotain 7.26 D 7.62 C 7.85 BC Super-U 7.21 DE 7.55 C 7.77 CD NSN 7.98 A 8.14 A 7.74 ESN 7.12 7.61 C 7.80 CD Nitamin 7.77 B 8.10 A 8.05 A 7.92 A N-Fusion Standard Error 7.61 C 7.80 B 7.91 B 8.00 A 0.04 0.06 0.04 0.09 0.12 F 7.11 D 8.16 A E 7.25 E 7.54 B 8.27 A 8.10 A 7.99 A 7.65 AB 7.51 A 7.29 A 6.93 A 7.82 CD 7.84 A 7.90 BC 7.90 AB 7.81 AB 7.33 ABC 6.45 B 6.15 B 5.73 CD 7.91 A 7.78 CD 7.82 BC 7.75 AB 7.06 C 6.54 B 5.94 B 5.54 7.93 A 7.81 BCD 7.65 CD 7.56 B 7.81 A 7.15 A 6.84 A 6.78 A 7.87 A 7.95 BC 7.91 AB 7.77 AB 7.50 ABC 7.28 A 6.22 B 5.87 C 7.34 C 7.58 7.13 E 6.83 6.26 6.13 B 5.76 B 5.34 8.05 AB 7.55 D 7.24 C 7.37 ABC 7.18 A 6.99 A 6.50 B 7.85 BC 7.60 CD 7.28 C 7.21 BC 7.59 A 6.83 A 6.36 B 0.11 0.12 0.23 0.21 0.22 0.09 D D D D DE E 158