Further evidence of solar cycle variability in middle atmospheric ozone and the importance of incorporating solar spectral irradiance in atmospheric modeling Aimee Merkel, Jerald Harder, Thomas Woods, Anne Smith, David Rusch, Mar<n Mlynczak Laboratory for Atmospheric and Space Physics (LASP) University of Colorado Na<onal Center for Atmospheric Research (NCAR ACD ) NASA Langley Research Center, Hampton, VA Jan. 28, 2014 SORCE Science Mee5ng 1 a Lean model 60 0.3 It all started with Haigh et al. Nature 2010 Pressure (hPa) 1 0.3 0.4 0.5 0.6 3 0.3 0.4 0.5 0.6 0.7 0.7 SSI influence study using a 2-­‐D (la5tude-­‐height) radia5ve-­‐chemical-­‐transport model of the atmosphere (IC2-­‐D). LETTERS | 10 0.6 Modeled ozone response (max-­‐min) 0.5 60 0.3 0.3 0.2 1 0.3 0.4 0.5 0 Latitude (°N) 0.7 30 0.3 0.4 0.5 0.6 50 1 –1.4 20 2 0 –2 –4 b 10–6.8 hPa 4 2 0 –2 40 4 60 2 0 –1.2 –1.2 –1.0 –2 –0.8 –0.6 –4 –0.4 –0.2 0.0 0.2 0.4 0.6 0.8 1.0 10–6.8 1.2 1.4 1.6 1.8 4 4 NATURE Vol 0.6 000 | 00 Month 2010 –4 50 0.2 0.4 0.8 20060.61.0 1.2 1.4 1.6 0.0 Approximate altitude (km) 10 –20 40 SORCE model run O3 anomalies (%) 4 0.3 –40 0.8 a 0.68–0.32data hPa b SIM/SOLSTICE Pressure (hPa) Approximate altitude (km) 200-­‐300nm important for mesospheric ozone NRLSSI model run a Lean model Pressure (hPa) 15 Difference in spectral irradiance at >242 nm (mW m–2 nm–1) 30 6 50 Approximate altitude (km) 0.2 O3 anomalies (%) a 0.68–0.32 hP 0.3 O3 anomalies (%) Supplementary Information for further details.) This type of model produces realistic simulations of the upper stratosphere (above about 25 km) but is less reliable at lower altitudes where photochemical time constants are longer and a more accurate representation of transport processes is required. The results below come from four model runs using solar spectra derived from the SIM measurements (with SOLSTICE data for wavelengths less than 200 nm) and those produced by the Lean model, each for both 2004 and 2007. In Fig. 2 we present latitude–height maps of the difference between 2004 and 2007 in December ozone concentrations. The Lean spectral data produce a broad structure of ozone concentrations greater in 2004 than in 2007, with maximum values of around 0.8% near 40 km, whereas the SIM data produce a peak enhancement of over 2% in low latitudes around 35 km, along with significant reductions above 45 km. The predicted temperature differences (Supplementary Difference in spectral irradiance at >242 nm (mW m–2 nm–1) onse of the n the speceen 0.2 mm M) instrut (SORCE) s declining ger decline n our preensated in ible waveear to have atospheric above this ochemical ements of ime period also show, e climate is nsufficient s observed ur findings on temperto current Figure 3 | Tim (solid black lin deseasonalized values reconst dashed lines. T components a Fig. 2. Data we 6.8 hPa (b). Over the p at altitudes 3 increasing co 1.8 40 40 NRLSSI 2000, howev 0.8 Lean model 2.0 stopped decl 2 0 0 SOLSTICE probably also 10 10 0.7 2.0 1.6 0 SIM 0.6 the chemical –2 1.8 30 the present s 30 0.6 1.6 0.5 1.4 –4 factors from –5 –2 30 200 300 400 500 600 700 30 –40 –20 20 2006 40 2005 0 2007seems likely –40 –20 0 20 40 Latitude (°N) Wavelength (nm) ozone below Latitude (°N) Figure 3 | Time series of AURA-MLS v2.2 ozone concentrations. The is data also more Figure 2(solid | Modelled difference in ozone between December 2004 and Figure 1 | Difference in solar spectrum between April 2004 and November b SIM/SOLSTICE data black lines) are percentage anomalies of tropical (22.5 uS–22.5 tral uN) variation Estimates of the percentage difference (2004–2007) in December 2007. 2007. The difference (2004–2007) in solar spectral irradiance 0.3 deseasonalized monthly means from August 2004 to November 2007. The 60zonal mean ozone concentration (labels on contour lines in per cent) –1.4 solar signal i (W m22 nm21) derived from SIM data4 (in blue), SOLSTICE data8 (in red) values reconstructed from the 4-component regression model are shown as produced by the model using solar spectra from the Lean model (a) and SIM/ (1979 to 200 and from the Lean model5 (in black). Different scales are used for values at dashed lines. The solar component of the regression is shown in red. Other SOLSTICE data (b). that the decl –1.2 wavelengths less and more than 242 nm (see left and right axes respectively). Mesosphere – out-­‐of-­‐phase –1.2 Stratosphere – in-­‐phase components are shown, along with the solar component, in Supplementary previous and sola Fig. 2. Data were averaged between 0.68 hPa and 0.32 hPa (a) and 10 hPa 1 –1.0 aboratory for Atmospheric and Space Physics, University of Colorado, 1234 Innovation Drive, Boulder, behaviours d also (very 50Fig. 1) are b). different, with the Lean data set showing tempera6.8 hPa –0.8 –0.6 To unders tures 0.3–0.4 K greater in 2004 than in 2007 at the top of the model –0.4 0.2 0.0 –0.2 0.4 Over thethe period from late 1970s to the late 1990s the modelled 1 domain, whereas SIM data setthe produces a peak warming of 1.8tropical K at ozone 0.6 0.8 0.2 0.0 0.4 1.0 0.6 0.8 1.2 at altitudes km decreased by about 9%differences (ref. 13) inare response Thetosharp d the summer polar35–50 stratopause. These temperature 3 1.0 1.4 1.2 1.6 (Fig. 2b) is c increasing of active species. Since about qualitatively similarconcentrations to, but about 50% larger chlorine than, those estimated 1.4 1.8 1.6 40 1.8 with by ref. 2000, 12 withhowever, an idealized a full climate model, possibly the forcing trend inin chlorine has reversed and ozone hasthe dom 2.0 These owing stopped to the broader spectral resolution cooling imposed by andgreenhouse the lack ofgases declining. Stratospheric has losses through pho ozone–temperature feedback in thatto model version.trend reversal by slowing probably also contributed the ozone 10 2.0 1.6 14 nates The the verychemical different scenarios by theittwo spectral setsperiod . Over thedata short ofthe loss reactionsproduced that destroy athese self-healing 1.8 they mightstudy be distinguishable in observational A 30suggestthe present it is not possible statistically torecords. differentiate 1.6 to lower multiple regression has or been carried out of deseasonalized 1.4 factors from analysis each other, from any solar influence. Nevertheless, it leve 30 (SeeinSupplem monthly meanlikely ozonethat datathe from theisMicrowave Sounder (MLS) seems Sun importantLimb in the apparent decrease –40 –20 0 20 40 instrument onbelow the Earth Observing System (EOS) Aura satellite. Four Latitude (°N) ozone 45 km from 2004 to 2007. The change in sign near 45 To kmassess t sured irradia regression indices were used: with a constant, two orthogonal indices is also more consistent the modelled response to the SIM specFigure 2 | Modelled difference in ozone between December 2004 and representing the quasi-biennial oscillation (which dominates ozone 13,15 another set o of the tral variations than to the Lean spectra. Previous analyses December 2007. Estimates of the percentage difference (2004–2007) in SOLSTICE t variability in the tropical stratosphere)13 and a solar index consolar signal in ozone, averaged over approximately 2.5 solar cycles zonal mean ozone concentration (labels on contour lines in per cent) There are dif structed from SIM data integrated over 200–400 nm. Motivated by produced by the model using solar spectra from the Lean model (a) and SIM/ (1979 to 2005 or 2003), have not shown this structure. This suggests fields but the the model results (Fig. 2), we chose two spatial regions, both spanSOLSTICE data (b). the declining phase of solar cycle 23 is behaving differently to stratosphere tropics, one at altitude 10–6.8 hPa, where the model predicts 2 Jan. 28, 2014 SORCE Science Mee5ng ning thethat previous solar2004–2007, cycles or possibly the solarhPa, cyclewhere exhibits tosphere. Th the largest difference and onethat at 0.68–0.32 the different itsvalues. ascending and descending Fig. 1) are also very different, with the Lean data set showing temperaresponse but model behaviours shows largestduring negative Figure 3 shows the rawphases. data and To understand the different spatial structures, and itmagnitudes, tures 0.3–0.4 K greater in 2004 than in 2007 at the top of the model the of impact o the fits reconstructed from the four regression components; also the ozone responses we consider photochemical domain, whereas the SIM data set produces a peak warming of 1.8 Kshows at the radiative (in modelled red) the derived solar component, which is statisticallyprocesses. The atsharp in ozone above 45 km with thelevels SIM spectra the summer polar stratopause. These temperature differences are significant .95%decrease at the upper levels and .99% at the lower The respon 0.6 3 0.7 0.7 3 Decreased ozone at solar max. Approximate altitude (km) MLS ozone regression b O3 anomalies (%) 5 Pressure (hPa) 2 242 ed as numDecember ce between IM. This is cal models, nd area, as e SIM data a factor of e radiation, r empirical aviolet than rent in the m, are indeance Com. The data hPa 2005 2007 Merkel et al. 2011 GEOPHYSICAL RESEARCH LETTERS, VOL. 38, L13802, doi:10.1029/2011GL047561, 2011 Simulate Irradiance SORCE Difference (%) NRLSSI Difference Changes in W(%) ACCM WACCM 10-2 Active 2004 Quiet 2007 Active 2004 Quiet 2007 Active 2002/2003 Quiet 2008/2009 Difference (%) o N-15 S Avg. 15o– 25S 25N spectral irradiance variability 10 on middle atmospheric ozone Pressure (hPa) -1 10 TIMED/SABER Day Aimee W. Merkel,1 Jerald W. Harder,1 Daniel R. Marsh,2 Anne K. Smith,2 O3 emission measurements 1 1 Juan M. Fontenla,1 and Thomas N. 10Woods from the 9.6μm channel – 80 0 Received Version 24 March 12011; 18 May 2011; published 2 July 2011. 2 .07 revised 15 May 2011; accepted 10 60 SABER 02/03-08/09 04-07 Model w/NRLSSI Model w/SORCE 40 20 Approximate Altitude (km) 3-­‐D fully coupled chemistry, radia5on and The impact ofmsolar dynamics global odel. Compare Simula<ons with SABER SABER Difference (%) Observa<ons Pressure (hPa) Approximate Altitude (km) [ 1 ] This study presents the impact of solar spectral 2009]. The SIM irradiance measurements have an accuracy 3 irradiance (SSI) variability on middle 10atmospheric of -50better0 than -50 0 ozone 50 50 2% -10 -8 -6 Based -4 -2 0 on 2 4 the -60 [Harder -40 -20 0 et 20 al., 40 602010]. over the declining phase of solar cycle 23. differentNRLSSI comparison independent SIM long‐ Δ O3 (%) a) Two Latitude d) channels, b) Latitude of thec)two Latitude model types of spectral forcing are applied to the Whole term uncertainty in the 200–300 nm region is ∼0.5–0.1%, 80 10-2 Atmosphere Community Climate Model (WACCM) to from 310–400 nm it is ∼0.2–0.05%, and in the 400–1600 nm SABER O3 average vmr between periods SABER ozone: 2-­‐yitr isrunning annual mean trends simulate the ozone response of quiet and range better than 0.05%.zonal Currently there is no direct 10-1 60 25°S – 2 5°N high solar activity. One scenario uses the solar proxy validation through independent irradiance observations that 0 a 0.2 .08 r e c o n s t r u c t i o n s m o d e l f r o m t h e 10N v ato l 0R e smeb a r c h have a physically et al., Day based degradation correction [Harder Night Night 40 60-­‐66km Laboratory (NRLSSI), and the other is based on SSI 2009, auxiliary material]. We present a modeling study on 1 10 observations from the Solar Radiation and Climate the impact of SORCE SSI variability on middle atmospheric Experiment (SORCE). The SORCE observations show 3– ozone. 20 2 5 times more variability in ultraviolet 10 (UV) radiation than [3] Up to the present time, most climate and solar cycle predicted by the proxy model. The NRLSSI forcing had related modeling studies have relied on solar input spectra 2 to 4 mb 3 10 long‐term of -10 solar minimal impact on ozone, however, the UV that -50are scaled 0 50 by -60 -40 -20 0proxies 20 40 60 -50 higher 0 50 -8 -6activity -4 -2 0 such 2 4 as 38-­‐44km the F10.7 radio flux [Marsh et al., 2007; Randel and Wu, variability from SORCE induced a 4% reduction in ozone e) f) g) Latitude h) Δ O3 (%) Latitude Latitude concentration above 40 km at solar active conditions. The 1999] or an equivalent Mg II core‐to‐wing [Soukharev model result is supported by 8 years (2002–2010) of and Hood, 2006]. A more dependable solar model emDescending phase of SC23 based on combined 3 ploys solarMirradiance reconstructions ozone observations from the Sounding of the JAtmosphere an. 28, 2014 SORCE Science ee5ng usin g B roa dba nd Emiss ion Rad iometr y (SABER) sunspot and facular proxy indicators (predominately the instrument. The SABER ozone variations have greater photometric sunspot index and the Mg II index) such as the similarity with the SORCE SSI model simulations. The Naval Research Laboratory SSI model (NRLSSI) [Lean, SSI Solar Forcing and Earth Atmospheric Response Understandably, this discovery revitalized the irradiance and atmospheric modeling communi5es. Lots of recent modeling ac5vity! Author Reference Model/Topic Haigh et al. Nature, 2010 IC2D model/SC Ozone Cahalan et al. GRL, 2010 GISS ModelE/Trop. Temp. Merkel et al. GRL, 2011 WACCM/SC ozone & TIMED SABER Ineson et al. Nature Geosci., 2011 HadGEM3/NAO Oberländer et al. GRL, 2012 EMAC-­‐FUB/Strat. temp Radia5ve response Swartz et al. ACP, 2012 GEOS CCM/ Strat. Ozone & temp Circula5on -­‐ NAO Wang et al. PNAS, 2013 WACCM/MLS & grnd based hydroxyl Shapiro et al. JGR, 2013 SOCOL/SC response Wen et al. JGR, 2013 GISS ModelE/Temp. response Ineson et al. (in prepara5on) HadGEM3/NAO/CMIP5 study, Maunder Minimum response Jan. 28, 2014 SORCE Science Mee5ng Modeling studies focusing on SSI implica5ons: Photochemistry “Top down” vs “Bojom up” 4 (a) Compiled Modeling Results (b) Fig. 10. Differences for January between 2004 and 2007 averaged over the tropics from 25◦ S to NRLSSI (solidKlines) and the SORCE/SIM andGSORCE/SOLSTICE data (dashed lin In the Ermolli using et al. the 2013 ACP data paper, atja M ajhes (GEOMAR, ermany) compiled −1 Kelvin per day (K day ) and (b) the temperature in Kelvin (K). For details please see text. the results of these modeling studies. Ozone response (max-­‐min) to SORCE and NRLSSI 1 GEOSCCM NRLSSI GEOSCCM SORCE IC2D NRLSSI IC2D SORCE SOCOL NRLSSI SOCOL SIM SOCOL SOLSTICE WACCM NRLSSI WACCM SORCE WACCM* NRLSSI MMM NRLSSI MMM SORCE 60 GEOS CCM 55 IC2D 50 SOCOL WACCM 45 MMM 40 35 10 Height (km) Pressure (hPa) 0.1 30 25 20 100 −10 −8 −6 −4 −2 0 2 4 6 8 10 Percent zone ariability due into solar Fig. 11. As Fig. 10 butofor the vozone response percent. Jan. 28, 2014 SORCE Science Mee5ng the tropospheric AO and NAO already respond to lower UV Even though the solar the 11 yr solar cycle is b should note here again t ergy source of the clim activity in the past few solar cycles) and its poss evolution has attracted th public (e.g. Lockwood e Jones et al., 2012; Rozan 4.3 Discussion of CCM We described the impact represent the lower and cle estimated variations, depicted in CCM simula provide the standard dat past and future (e.g. SPA 2012). The atmospheric 5 dard data set is compared estimate to understand n Ques5ons and Debate Now there is sugges5ve evidence of this surprising SC signal in mesospheric ozone measurements that you can only get if more UV variability is incorporated into atmospheric models. Lots of ques5ons and debate. Solar ques5ons: -­‐ Integrity of the SORCE dataset (Degrada5on correc5ons?) -­‐ Why do previous measurements at these wavelengths disagree with SORCE? -­‐ Can we use a solar spectrum scaled by a variability proxy (TSI, MgII, Lyman α, F10.7) as a standard to characterize the sun in atmospheric models? -­‐ Do all wavelengths vary the same way as TSI? -­‐ How good do the solar measurements need to be? Gaps in 5meseries? -­‐ Does this variability only pertain to SC23-­‐24 or has it been there all along? Atmospheric ques5ons: -­‐ Integrity of the ozone measurements. Why haven’t we seen this signal before? -­‐ Why is the mesospheric signal out of phase with solar cycle and different than stratospheric ozone? -­‐ Is this a special solar cycle? Is it in previous measurements? -­‐ What does this mean for the modeling community? Is a SSI proxy good enough for atmospheric modeling studies? Are we missing important SC variability? Jan. 28, 2014 SORCE Science Mee5ng 6 Interes5ng Conundrum The modelers -­‐ want the solar physicist to give them something to put in their models. Most models have been upgraded to included SSI on a daily cadence. The solar physicist -­‐ want the modelers to tell them how good they need to measure the Sun. • Good enough is different depending on the model, atmospheric region studied, type of model (photochemistry, radia5ve). Work in progress: We are having a workshop next month with the NCAR folks to discuss this very thing. Jan. 28, 2014 SORCE Science Mee5ng 7 Understanding Mesospheric Ozone Variability Top of the atmosphere ozone~ 1% of total column – Dominated by photochemistry. – Photochemical life5me is hours. – Strong diurnal component. Local 5me is important for solar cycle analysis. – More UV causes more loss of ozone at solar maximum. Loss due to photolysis and cataly5c cycles with OH and H. Mesospheric ozone influenced by the solar radia5on in the 200-­‐300nm band. (produc5on and loss) Herzberg Con5nuum Hartley bands Herzberg Con5nuum (200-­‐242nm) J2 rate: O2 Photolysis O3 produc5on Hartley Bands (200-­‐300nm)– J3 rate -­‐ O3 Photolysis O3 loss Jan. 28, 2014 SORCE Science Mee5ng 8 TIMED/SABER Ozone – 12 years of ozone data We can now look at the ascending phase of solar cycle 24. Did the mesosphere respond? • Data now spans from 2002 – 2013 (12 years of data) • Recently updated to Version 2 – Reprocess all results • 9.6μm channel – O3 emission measurements • Version-­‐2 data validated by A. Smith (NCAR) 2012. Known systema5c bias compared to other ozone measurements. Bias is constant over 5me, so does not influence differences. Jan. 28, 2014 SORCE Science Mee5ng 9 SABER Ozone Time Series – Yearly average Mesosphere – Out-­‐of-­‐phase 9.6 day +/-25deg Meso. yearly average .2-.08mb Equatorial average 5me series O3 VMR 0.87 0.86 ~4% 0.85 0.84 0.83 0.82 2002 2004 2006 2008 2010 2012 2014 Stratopause – Licle varia5on +/-25deg Stratpause yearly average 1-2mb 1 mb 48 km O3 VMR 5.6 5.5 5.4 5.3 5.2 2002 2004 2006 2008 2010 2012 Stratosphere – in-­‐phase 2014 9.6 day +/-25deg Strat. yearly average 2-4mb 10.0 9.8 O3 VMR SABER O3 Average vmr 0.2 to 0.08 mb 60-­‐66km 0.88 2 to 4 mb 38-­‐44km 9.6 9.4 9.2 9.0 2002 ~5% 2004 2006 Jan. 28, 2014 SORCE Science Mee5ng 2008 2010 2012 2014 10 SABER Ozone Time Series Mesosphere – Oyearly ut of average phase .2-.08mb 9.6 day +/-25deg Meso. 0.2 to 0.08 mb 60-­‐66km 0.88 0.10 0.84 0.08 0.83 0.82 2002 0.06 2004 2006 2008 2010 2012 2014 0.04 0.02 0.00 2002 Stratosphere in phase 9.6 day +/-25deg Strat.– yearly average 2-4mb 10.0 2004 2006 2008 Year 2010 2012 2014 2 to 4 mb 38-­‐44km 9.8 Courtesy of Jerry Harder O3 VMR Fractional Irradiance Change O3 VMR Irradiance Variability 0.87 0.86 Ac5ve Area Network -­‐PSPT 0.85 240-­‐260nm SSI Proxy basedSIM on the Active Network Area, SIM 240-260nm 9.6 9.4 9.2 9.0 2002 2004 Jan. 28, 2014 SORCE Science Mee5ng 2006 2008 2010 2012 2014 11 20 4-­‐component regression, deseasonalized 5me series at each pressure level. Solar, Annual, 2-­‐QBO Solar Coefficient Mesosphere out-­‐of-­‐phase Mesosphere ozone–variation, 0.08 mb 66 km Percent ozone variation due to solar -10 Residual ozone variation regression fit solar component Polynomial fit 10 -5 0 5 10 70 0 -10 -20 2002 2004 2006 2008 Year 2010 2012 2014 Stratosphere in-­‐phase Stratosphere ozone–variation, 5.5 mb 36 km 15 Residual ozone variation regression fit solar component Polynomial fit 10 60 50 1.0 approximate altitude (km) 0.1 Pressure levels (mb) Residual ozone variation in percent Residual ozone variation in percent SABER Regression Analysis 40 5 0 -5 10.0 30 -10 -15 2002 -1.5 2004 2006 2008 Year 2010 2012 2014 Jan. 28, 2014 SORCE Science Mee5ng -1.0 -0.5 0.0 0.5 Solar coefficient 1.0 1.5 12 Ozone measurements in previous solar cycles JOURNAL OF GEOPHYSICAL RESEARCH, VOL. 111, D20314, doi:10.1029/2006JD007107, 2006 Ques5on: Why have we not seen this mesospheric ozone behavior in Figure 7. Same format as Figure 5 but as calculated from the UARS HALOE zonal mean time series Full (1992 –2003). previous solar cycles? Article Click Here for for each of the three satellite data sets were averaged over the 25!S to 25!N latitude band and the averaged time series were then analyzed using the same multiple regression model (1). Results are plotted in Figure 8 as vertical profiles of the solar minimum to maximum regression coefficient with 95% confidence error bars for each data set. It is seen that the basic features of the SBUV(/2) tropical ozone Reason response (Figure 8a) are also present in the SAGE II response (Figure 8b) and in the HALOE response (Figure 8c). In the lower stratosphere, a statistically significant positive response is obtained with a percent amplitude that increases with decreasing altitude (with the exception of the lowest level for the SAGE II data, which may be less reliable). In the middle stratosphere, the 2-s error bars Solar cycle variation of stratospheric ozone: Multiple regression analysis of long-term satellite data sets and comparisons with models Regression analysis results B. E. Soukharev1 and L. L. Hood1 Remsberg et al., 2SOLAR 008 CYCLE IN OZONE AND TEMP REMSBERG: Historical ozone data comprised of occulta5on [ ] Previous multiple of the solar cycle stratospheric data or regression only analyses measure up variation to 5of0km. ozone are improved by (1) analyzing three independent satellite ozone data sets with D22304 Received 22 January 2006; revised 28 June 2006; accepted 24 July 2006; published 31 October 2006. SAGE SBUV HALOE 1 1991-­‐2005 lengths extending up to 25 years and (2) comparing column ozone measurements with ozone profile data during the 1992–2003 period when no major volcanic eruptions occurred. Results show that the vertical structure of the tropical ozone solar cycle response has been consistently characterized by statistically significant positive responses in the upper and lower stratosphere and by statistically insignificant responses in the middle stratosphere (!28–38 km altitude). This vertical structure differs from that predicted by most models. The similar vertical structure in the tropics obtained for separate time intervals (with minimum response invariably near 10 hPa) is difficult to explain by random interference from the QBO and volcanic eruptions in the statistical analysis. The observed increase in tropical total column ozone approaching the cycle 23 maximum during the late 1990s occurred primarily in the lower stratosphere below the 30 hPa level. A mainly dynamical origin for the solar cycle total ozone variation at low latitudes is therefore likely. The amplitude of the solar cycle ozone variation in the tropical upper stratosphere derived here is somewhat reduced in comparison to earlier results. Additional data are needed to determine whether this upper stratospheric response is or is not larger than8.model estimates. Figure 12. Profiles of the 11-year and the SC-like, Figure Solar cycle ozone regression coefficients (expressed as percent change from solar minimum The solar signal is “washed out” due to the mixing of source and loss mechanisms in a photochemical dominate region of the atmosphere. (sunrise and sunset) to maximum) for (a) the SBUV(/2) data set, (b) the SAGE II data set, and (c) the HALOE data set. The maximum minus minimum responses (in percent) for the Citation: Soukharev, B. E., and L. L. Hood (2006), Solar cycle variation of stratospheric ozone: Multiple regression analysis of longregression coefficients were obtained by applying equation (1) to 3-month time series averaged over the tropical to subtropical ozone from HALOE. The solid curve termto satellite data sets 25!S 25!N latitude band.and comparisons with models, J. Geophys. Res., 111, D20314, doi:10.1029/2006JD007107. is the model result for 5!N from Brasseur [1993]. 9 of 18 formation in the stratosphere [Heath and Schlesinger, 1986; Viereck and Puga, 1999]. 3.3. Solar Cycle (or SC-Like) Responses of HALOE [2] The observed solar cycle variation of stratospheric Ozone and11-year Temperature of the ozone re[3] Observational estimates ozone is a key constraint on climate models that include sponse as a function of altitude and latitude have been 40] In order to obtain estimates of the actual response of [ solar variability as a forcing mechanism and that account for reported by a number of analysts based mainly on Solar atmospheric ozone and temperature to a proxy for the direct the existence of the stratosphere [Haigh, 1994, Jan. 1996; 28, Backscattered 2014 SORCE Ultraviolet Science M ee5ng (SBUV) forcing data fromand the Stratospheric UV flux, their sets of responses from Shindell et al., 1999; Rind, 2002]. It is also important to Aerosol and Gas Experiment (SAGE) I and II data using Figures 9a and 11a have been adjusted by the amount that determine and understand the solar cycle variation of ozone multiple regression methods they were not exactly [Chandra, 1991; Hoodinetphase al., from Figures 9b and 11b. so that anthropogenic trends, including possible evidence 1993; Chandra and McPeters, Those1994; adjustments were made McCormack andby multiplying the responses for an ozone ‘‘recovery,’’ can be more accurately evaluated Hood, 1996; Wang et al., 1996]. by the cos analyses [2p p/11],ofwhere p is the deviation of Forfactor, example, 1. Introduction are model/HALOE ozone responses wit in part, to not accou in the present HAL McCormack et al., [42] Lee and Smit SBUV data for a s SAGE II are simila Figure 9a, at leas latitudes; their resu though, especially results from SAGE [2006]). Lee and Sm the SC response, b phases of the QBO with the QBO in responses in the s hemispheres, but t QBO indexes that th for the present HAL QBO and its asso accounted for to fir those terms in the H were able to simulat 20 to 30 hPa, but response at about 5 lations reported by M positive ozone respo period of 1979 to 2 1950 to 2003. It is spheric ozone respon 13 to solar cycl related [43] The SC-like, for ozone (in perc summarized in Tab and for three distinc Solar Mesosphere Explorer – 1982 -­‐ 1989 • UV ozone channel (Rusch et al. 1984) Solar irradiance measurements. (Rojman et al. 1982) • SME covers parts of solar cycle 21-­‐22 -­‐ Good ozone measurements between 1982-­‐1986 • Day5me (3pm) limb profiles of ozone with good global coverage. • SME ozone measurements are analyzed consistent with SABER analysis. (Woods and Rojman 1997) Jan. 28, 2014 SORCE Science Mee5ng 14 Solar Irradiance variability 2 decades apart LISIRD site Courtesy of Jerry Harder Jan. 28, 2014 SORCE Science Mee5ng 15 SME Ozone Time Series SME yearly average vmr SME yearly ean 5me series SME m yearly average 70 0.5 2.0 1.0 0.2 2.0 50 0.77 1982 0.5 0.2 45 -50 0 latitude 0.79 0.78 1983 1984 1985 1986 1987 50 SME irradiance variability 240-260nm 0.07 Delta Irradiance (W/m^2) 0.5 1.0 55 0.2 to 0.08 mb 60-­‐66km 0.80 O3 VMR 60 1.0 approximate altitude (km) 65 0.5 0.2 Pressure level (mb) 10-1 100 0.81 0.2 0.2 0.06 0.05 0.04 0.03 0.02 0.01 0.00 1982 Jan. 28, 2014 SORCE Science Mee5ng 1983 1984 1985 Year 1986 1987 1988 16 Solar Coefficient Mesosphere 60 km 0.2 mb 60km Mesosphere ozone–variation, Percent ozone variation due to solar -5 0 5 4 70 2 0 Residual ozone variation regression fit solar component Polynomial fit -4 1982 1983 1984 Year 1985 1986 1987 Stratopause– 48 km 1 mb 48km Mesosphere ozone variation, 4 60 55 2 approximate altitude (km) 65 0.1 -2 Pressure levels (mb) Residual ozone variation in percent Residual ozone variation in percent SME Regression 50 1.0 0 -2 Residual ozone variation regression fit solar component Polynomial fit -4 1982 1983 1984 Year 1985 1986 45 -1.5 -1.0 1987 Jan. 28, 2014 SORCE Science Mee5ng -0.5 0.0 Solar coefficient 0.5 1.0 17 SME compared to SABER Regression – solar component 0.10 Day Solar Variation 0.08 SME UV - SC 21 SORCE - SC 23-34 SABER 0.04 SME UV 0.1 0.00 -0.02 -8 -6 -4 -2 0 2 Years from solar minimum 4 6 Ozone yearly 5me series 1980 1982 1984 1986 1988 1990 Pressure levels (mb) 0.02 70 60 50 1.0 1.04 approximate altitude (km) 0.06 Normalized ozone variability Fractional Irradiance Change Irradiance Variability 240-­‐260nm 40 1.03 10.0 30 1.02 -15 1.01 1.00 2002 -10 -5 0 5 10 Percent Solar variation 15 SME UV - SC 21 SABER 9.6 - SC 23-34 2004 2006 2008 2010 2012 2014 Jan. 28, 2014 SORCE Science Mee5ng 18 Summary • Sugges5ve evidence that UV variability in the 240-­‐260nm range and mesospheric ozone from SC 21 are consistent with SC 23-­‐24. Has it been there all along? Further evidence that this signal is real. • Mul5ple modeling studies show that increased UV variability as observed by SORCE (both SIM and SOLSTICE) helps to resolve differences between modeled ozone and observa5ons in the mesosphere. • The UV variability is probably somewhere in between NRLSSI and SORCE, however it is apparent that the atmosphere is sensi5ve to this difference. When compiling SSI proxy model please consider that this type of variability in the UV majers in the mesospheric photochemistry. • Need to approach the issue from both direc5ons. Atmospheric modelers and solar physicists/modelers need to work together to constrain this variability . The atmospheric modelers can perform case studies to fine tune the response to different solar variability but this can’t be used to validate the solar, can only be used as a guideline. Wavelength dependent. • Importance of the con5nua5on of mesospheric ozone measurements in the future. Jan. 28, 2014 SORCE Science Mee5ng 19 Thank You! Jan. 28, 2014 SORCE Science Mee5ng 20 9.6 day +/-25deg Meso. yearly average .3-.08mb 1.08 O3 VMR 1.06 Version 1.07 Version 2 1.04 1.02 1.00 2002 2004 2006 2008 2010 Jan. 28, 2014 SORCE Science Mee5ng 2012 21 Analyze SABER as if Occulta5on Experiment Day Night Par5al Day-­‐Night Annual Mean Difference 25S-­‐25N -­‐ When SABER is analyzed with only measurements taken at “occulta5on” local 5mes: Solar signal is washed out and response is more similar to night results Jan. 28, 2014 SORCE Science Mee5ng 22 Analyze WACCM at Occulta5on local 5mes Modeled ozone results Day Night Par5al Day-­‐Night When WACCM is analyzed with only measurements taken at “occulta5on” local 5mes: Solar signal is washed out and response is more similar to night results. Confirms results from SABER. Jan. 28, 2014 SORCE Science Mee5ng 23