Click Here JOURNAL OF GEOPHYSICAL RESEARCH, VOL. 113, D20205, doi:10.1029/2008JD009890, 2008 for Full Article Relationship between ice water content and equivalent radar reflectivity for clouds consisting of nonspherical ice particles Gang Hong,1 Ping Yang,1 Bryan A. Baum,2 and Andrew J. Heymsfield3 Received 30 January 2008; revised 23 July 2008; accepted 7 August 2008; published 21 October 2008. [1] This study investigates the relationship between ice water content (IWC) and equivalent radar reflectivity (Ze) at 94 GHz for clouds consisting of nonspherical ice particles with geometrical shapes of hexagonal solid and hollow columns, plates, 6-branch bullet rosettes, aggregates, and droxtals. The IWC is calculated from a set of 1119 ice particle size distributions (PSDs) measured during several field campaigns, which are discretized to 46 size bins based on particle maximum dimensions ranging from 2 to 10500 mm. The Ze at 94 GHz is calculated from the radar backscattering properties obtained by integrating over the PSD and chosen particle habit distributions. The influence of ice habit on the Ze-IWC relationship is investigated for ice clouds composed of individual ice particle habits and a habit mixture. The Ze-IWC relationship is found to be sensitive to cloud effective particle size and cloud temperature. For an ice cloud with a given IWC, the Ze tends to increase with increasing effective particle size. Similarly, the Ze generally increases with increasing cloud temperature, at least for clouds with IWC over 0.01 g/m3. These features are consistent with the observed relationship between effective particle sizes and cloud temperatures. The present investigation of the effect of temperature on the Ze-IWC relationship indicates that including temperature in the Ze-IWC relationship may not improve the estimates of IWC. However, the dependence of the Ze-IWC relationship on the effective particle size within a given temperature range is more pronounced, and may be potentially useful for inferring the cloud effective particle size from the Ze-IWC relationship. Citation: Hong, G., P. Yang, B. A. Baum, and A. J. Heymsfield (2008), Relationship between ice water content and equivalent radar reflectivity for clouds consisting of nonspherical ice particles, J. Geophys. Res., 113, D20205, doi:10.1029/2008JD009890. 1. Introduction [2] Clouds generally cover between 65-70% of the Earth. Approximately, 30% of these clouds reside at heights corresponding to pressures lower than 400 hPa [e.g., Wylie et al., 2005; Hong et al., 2007]. These high-altitude ice clouds are composed of nonspherical particles. Synoptic cirrus, formed in environments of relatively low updraft velocities, and tend to be composed of pristine habits as droxtals, hexagonal columns and plates, bullet rosettes, and aggregates of these habits. However, in convective situations the habits of ice particles tend to be much more complex. [3] In the past decade, significant efforts have been focused on the calculation of the scattering and absorption properties of these ice particles [e.g., Macke et al., 1998; Mishchenko et al., 2000; Bailey and Hallet, 2004; Heymsfield and Miloshevich, 2003; Yang et al., 2005; Baum et al., 2005a]. Recent improvements offer the capabilities to 1 Department of Atmospheric Sciences, Texas A&M University, College Station, Texas, USA. 2 Space Science and Engineering Center, University of WisconsinMadison, Madison, Wisconsin, USA. 3 National Center for Atmospheric Research, Boulder, Colorado, USA. Copyright 2008 by the American Geophysical Union. 0148-0227/08/2008JD009890$09.00 infer the scattering properties consistently over the electromagnetic spectrum from the ultraviolet (UV) through the far infrared (Far IR). However, relatively little research has focused on the interpretation of millimeter wavelength radar measurements of ice clouds based on the calculated scattering/absorption properties of nonspherical particles. [4] This work is aimed at understanding the effect of ice particle nonsphericity on the relationship between ice water content (IWC) and equivalent radar reflectivity (Ze). In particular, the focus is on measurements offered by CloudSat, a spaceborne radar launched on 28 April 2006, which provides millimeter wavelength measurements at 94 GHz [Stephens et al., 2002]. [5] A number of articles have explored the use of millimeter-wavelength radar reflectivity (Ze) to estimate the IWC of ice clouds [e.g., Liu and Illingworth, 2000; Sassen et al., 2002; Matrosov et al., 2002; Mace et al., 2002; Heymsfield et al., 2005; Shupe et al., 2005; Sato and Okamoto, 2006; Boudala et al., 2006]. The scattering characteristics of nonspherical ice particles at 94 GHz have been done for various ice particle habits [e.g., Aydin and Tang, 1997; Lemke and Quante, 1999; Okamoto, 2002; Battaglia et al., 2001; Sato and Okamoto, 2006]. Recently, Hong [2007a] parameterized the radar backscattering properties at 94 GHz for nonspherical ice particles including solid and hollow hexagonal columns, plates, 6-branched D20205 1 of 9 D20205 HONG ET AL.: ZE-IWC RELATIONSHIPS FOR ICE CLOUDS bullet rosettes, aggregates, and droxtals, which are the ice crystal models extensively used for ice cloud retrievals based on observations made by infrared and visible satellite sensors [Yang et al., 2005; Baum et al., 2005a, 2005b, 2007; Platnick et al., 2003; King et al., 2003, 2004, 2006]. [6] Sassen et al. [2002] described three approaches for deriving the empirical relationship between Ze the IWC for ice clouds. These Ze-IWC relationships have been intercompared by Sassen et al. [2002], Boudala et al. [2006], and Hong [2007a]. The pronounced differences among the intercomparison results reveal that the sensitivity of Ze-IWC relationship to assumed ice cloud microphysical properties and the methods used to derive the relationship. The Ze-IWC relationship is sensitive to the variability in the particle size distributions (PSD) of ice particles [Schneider and Stephens, 1995; Brown et al., 1995; Aydin and Tang, 1997; Liu and Illingworth, 2000; Sassen et al., 2002]. Heymsfield et al. [2005] note that Ze and IWC depend on the distribution of particle mass versus size. An issue to be reckoned with is to account adequately for small particles at lower radar Ze and large particles at higher Ze. [7] Additional, the relationship between cloud temperature and particle size for ice clouds has been investigated [e.g., Heymsfield and Platt, 1984; Garrett et al., 2003]. There is some evidence that the Ze-IWC relationship is sensitive to cloud temperature [e.g., Sassen et al., 2002; Boudala et al., 2006]. Boudala et al. [2006] developed an IWC retrieval algorithms based on temperature and Ze using ice particle distributions measured in stratiform ice clouds in midlatitude and Arctic regions and assumed irregular ice particle shapes represented by aggregates of plates and dendrites. [8] In this paper we explore the sensitivity of a derived Ze-IWC relationship to assumed ice particle habit. The basis for this analysis is a set of 1119 ice PSDs measured during several field campaigns in tropical and midlatitude regions, which are described in detail by Baum et al. [2005a]. The sensitivity of Ze-IWC relationships to nonspherical ice particle habits is investigated on the basis of a set of six habits (hexagonal solid and hollow columns, plates, 6-branch bullet rosettes, aggregates of columns, and droxtals). These are the same habits as those used for the bulk scattering models from visible through the Far-IR wavelengths in some previous studies [e.g., Platnick et al., 2003; King et al., 2004, 2006; Yang et al., 2005; Baum et al., 2005a, 2005b, 2007]. The effect of cloud environment temperature and ice particle size on the Ze-IWC relationship is also investigated. 2. Data and Methodology [9] Sassen et al. [2002] introduced three approaches to derive the Ze-IWC relationship. In this study, we employ an algorithm to derive Ze from ground-based or airborne microphysical measurements. A set of PSDs used in this study were obtained from in situ measurements in several field campaigns covering tropical to midlatitude regions. The tropical measurements used in this study include two campaigns conducted in Kwajalein, Marshall Islands in 1999 under the auspices of the Tropical Rainfall Measuring Mission (TRMM) [Stith et al., 2002, 2004], and the Cirrus Regional Study of Tropical Anvils and Cirrus Layers D20205 (CRYSTAL) Florida Area Cirrus Experiment (FACE) in 2002. The midlatitude measurements include the First International Satellite Cloud Climatology Project Regional Experiments (henceforth FIRE-1) in Madison, Wisconsin in 1986, Coffeyville, Kansas in 1991 (FIRE-II), and the Atmospheric Radiative Measurement Program (ARM) Intensive Operational Period (IOP) near Lamont, Oklahoma in 2000. Detailed information about the microphysical measurements are provided by Miloshevish and Heymsfield [1997], Heymsfield et al. [2002, 2003, 2004], and Heymsfield and Miloshevich [2003]. A resulting set of 1119 PSDs are summarized by Baum et al. [2005a]. Each PSD is represented in the form of a gamma distribution [e.g., Kosarev and Mazin, 1991; Mitchell, 1991; Heymsfield et al., 2002] as follows: N ð DÞ ¼ N0 Dm e$lD ; ð1Þ where D is the maximum dimension of an ice crystal particle, N(D) is the number density of ice crystal particles with a D, N0 is the intercept, l is the slope, and m is the dispersion. [10] The IWC is derived from IWC ¼ r Z Dmax Dmin " N X i¼1 # fi ð DÞVi ð DÞ N ð DÞdD; ð2Þ N P where r is the ice density with a value of 0.917 g cm$3, i¼1 fi(D) = 1, where i denotes the ice crystal habit in the ice cloud, fi(D) is the ice particle habit fraction for habit i at a D, Vi(D) is the volume of the habit i for a given D, and Dmin and Dmax are the minimum and maximum sizes of D in the given particle size distribution N(D), respectively. [11] The IWC for a cloud composed of either a single habit (i = 1) or a given habit mixture (i > 1) is calculated from equation (2) for each of the 1119 PSDs. Different ice cloud habit distributions have been used for ice cloud retrievals from solar and infrared measurements [e.g., Yang et al., 2005; Baum et al., 2005b; King et al., 2004, 2006; Hong, 2007a, 2007b]. The habit distribution derived by Baum et al. [2005a] for MODIS Collection 5 cloud retrieval [King et al., 2006] is used in this study. The habit distribution consists of 100% droxtals when D < 60 mm, 15% bullet rosettes, 50% solid columns, and 35% plates when 60 mm < D < 1000 mm, 45% hollow columns, 45% solid columns, and 10% aggregates when 1000 mm < D < 2500 mm, and 97% bullet rosettes and 3% aggregates when D > 2500 mm. [12] We assume that the Ze-IWC relationship has a form of IWC = aZbe , where IWC is in units of g m$3 and Ze is in units of mm6 m$3 (dBZ in terms of 10log Ze). The radar equivalent reflectivity factor Ze at horizontal (vertical) copolarization in units of mm6 m$3 is defined as [e.g., Atlas et al., 1995; Donovan et al., 2004; Sato and Okamoto, 2006; Hong, 2007a] l4 Ze ¼ 0:93p5 Z Dmax Dmin " N X i¼1 # fi ð DÞsi ð DÞ N ð DÞdD; ð3Þ where l is the wavelength at 94 GHz, si is the backscattering cross section for the ith ice crystal habit at a D. The nonspherical ice particles in general have been assumed 2 of 9 HONG ET AL.: ZE-IWC RELATIONSHIPS FOR ICE CLOUDS D20205 D20205 Figure 1. The relationship between ice water content (IWC) and equivalent radar backscattering reflectivity (Ze) at 94 GHz for clouds consisting of individual habits: (a) solid columns, (b) hollow columns, (c) plates, (d) 3D bullet rosettes, (e) aggregates, and (f) droxtals. to be randomly orientated so that Shh = Sw and Shv = Svh. The backscattering cross section s for each of the habits is computed from the DDA model [Hong, 2007a] at 46 discrete values of D in a range of 2 – 10500 mm. [13] The particle effective size De is calculated for each of the 1119 PSDs, and is given by [e.g., Foot, 1988; King et al., 2004; Yang et al., 2005; Baum et al., 2005b]: !N R Dmax P " fi ð DÞVi ð DÞ N ð DÞdD 3 Dmin i¼1 !N " ; De ¼ 2 R Dmax P f ð D ÞA ð D Þ N ð D ÞdD i i Dmin ð4Þ i¼1 where Ai(D) is the averaged projected area of the habit i for a given D. 3. Results [14] Figure 1 shows the Ze-IWC relationship for clouds composed of six individual habits: hexagonal solid and hollow columns, plates, 3D bullet rosettes, aggregates, and droxtals. The differences in the Ze-IWC relationships for different habits show some sensitivity to the choice of habit for deriving the relationship. [15] On the basis of the mass-volume-size relationship assumed for each of the 6 individual habits [Yang et al., 2005; Hong, 2007a, 2007b], a value of IWC can be calculated for each of the PSDs (i.e., equation (2)). These IWC values can be compared to those derived using the Ze-IWC relationships for the various habits shown in Figure 1, with results shown in Figure 2. The correlation coefficients of the IWC values are lower for hollow and solid columns and 3D bullet rosettes than for plates, droxtals, and aggregates. The correlation coefficient for aggregates is the highest of the various individual habits. This is in agreement with the representation of aggregates for irregular ice particles by Boudala et al. [2002]. [16] Under natural conditions, ice clouds consist of a variety of habits, with the smallest particles having aspect ratios of near unity (like droxtals) and larger particles with various shapes. It may be unrealistic to apply the Ze-IWC relationships shown in Figure 1 to naturally occurring ice clouds. To gain some sense of the variability caused by the assumption of habit, however, we can develop a Ze-IWC relationship from the entire set of PSDs based on this set of six individual habits (i.e., 6 % 1119 pairs of IWC and Ze) to build the Ze-IWC relationship. The resulting Ze-IWC relationship is shown in Figure 3 along with those previously shown in Figure 1. It is clear that the Ze-IWC relationships for ice clouds composed of individual habits have distinct differences. The relationship is very similar for ice clouds composed of solid columns, hollow columns, and 3D bullet rosettes. With a given value of Ze, the inferred IWC can vary by a factor of 1.5 – 2.0. In particular, the variability in IWC increases when Ze has negative values of dBZ. When the Ze values are above 0 dBZ, the Ze-IWC relationship more closely approximates the individual relationships for aggregates, droxtals, and plates. However, when the Ze values are less than 0 dBZ, the Ze-IWC relationship more closely approximates the individual relationships for 3D bullet rosettes, solid columns, and hollow columns. 3 of 9 D20205 HONG ET AL.: ZE-IWC RELATIONSHIPS FOR ICE CLOUDS D20205 Figure 2. Comparisons between the ice water contents (IWC) inferred from the Ze-IWC relationships and the IWC derived from the microphysical measurements for a set of 1119 ice particle size distributions (PSDs) for clouds consisting of individual habits: (a) solid columns, (b) hollow columns, (c) plates, (d) 3D bullet rosettes, (e) aggregates, and (f) droxtals. [17] In addition to the assumption of habit, ambiguities in the Ze-IWC relationship arise from the characterization of the particle size distribution. The PSD is often characterized by the effective diameter and also the median mass diameter (Dm). The dependence of the Ze-IWC relationship on Dm was investigated by Atlas et al. [1995], Brown et al. [1995], Liu and Illingworth [2000], and Sassen et al. [2002]. [18] In the present study, the effect of the particle effective size (De) on the Ze-IWC relationship is investigated, with results shown in Figure 4. Instead of using individual habits, a habit mixture based on the study by Baum et al. [2005a] is assumed, which was derived by comparing the calculated median mass equivalent diameters and IWC from in situ measured PSD with those in situ measurements. For each of the 1119 PSDs, the De is calculated from equation (4). The 1119 values of De range in value from less than 50 mm to greater than 200 mm. Six groups are formed with De ranging from 50 mm to 200 mm at an interval of 25 mm. Two additional groups are formed with De < 50 mm and De > 200 mm. The coefficient a and exponent b for the Ze-IWC relationships are given in Table 1 for the 8 groups of De. [19] The sensitivity of the Ze-IWC relationship to De is shown in Figure 4a. In general, for a given Ze, the IWC increases with decreasing De. In contrast, for a given IWC, Ze increases with increasing De. The slopes of the Ze-IWC relationships are close for Dm > 50 mm but the slope for the smallest value of De is different. The smallest values of De are mostly observed in the CRYSTAL-FACE (Figure 5). The distinct different slope of the Ze-IWC relationship for these ice clouds reveals again the influence of nonsphericity of ice particles on the Ze-IWC relationship. Chepfer et al. [2005] found that the main habits of the ice particles observed in the CRYSTAL-FACE are hexagonal columns. However, the habit mixture derived by Baum et al. [2005a] Figure 3. The relationship between ice water content (IWC) and equivalent radar backscattering reflectivity (Ze) at 94 GHz derived on the basis of all 6 habits discussed previously (black dots are for calculations on the basis of the measured ice particle size distributions). The previously derived (see Figure 1) Ze-IWC relationships for clouds consisting solely of individual habits are superimposed for reference. 4 of 9 D20205 HONG ET AL.: ZE-IWC RELATIONSHIPS FOR ICE CLOUDS Figure 4. The relationships between ice water content (IWC) and equivalent radar backscattering reflectivity (Ze) at 94 GHz for clouds consisting of a mixture of habits for specific ranges of (a) effective particle sizes (De) and (b) cloud temperatures (T). is used to derive the Ze-IWC relationship in the present study. [20] Moreover, the Ze-IWC relationships for De in the range of 50-100 mm and for De > 100 mm have similar slopes. These features are indicated by the values of the coefficient a and exponent b shown in Table 1. The regular dependence of the Ze-IWC relationships on De, except for the smallest De, may be potentially useful for deriving the De from observed Ze for a given IWC or to derive the IWC from the observed Ze for a given De. This result indicates that the vertical distributions of De or IWC could be derived from similar lookup table as Figure 4a. [21] Liu and Illingworth [2000] and Sassen et al. [2002] documented that the inclusion of temperature for retrieving IWC from Ze can improve the accuracy of retrieved IWC. Recently, Boudala et al. [2006] developed a parameterized radar retrieval algorithm of IWC in terms of temperature and D20205 Ze which is based on in situ aircraft measurements. Since cloud temperature is given for each of our PSDs, the dependence of the Ze-IWC relationship on temperature is investigated. Figure 4b shows the Ze-IWC relationships for six groups of temperatures. The coefficient a and exponent b of the Ze-IWC relationships for the six groups are also listed in Table 1. [22] Unlike the systematic effect of De on the Ze-IWC relationship, the effect of temperature on the Ze-IWC relationship shows more variability. While Boudala et al. [2006] suggested that Ze generally increases with increasing temperature for a given IWC; in this study, this feature is generally observed only when Ze are above $10 dBZ. Thus one cannot draw firm conclusions from the current analysis that an explicit inclusion of temperature in the Ze-IWC relationship can improve the accuracy of IWC derived from Ze. [23] The effect of temperatures on De has been investigated by numerous groups [e.g., Ou and Liou, 1995; Ou et al., 1995; Wyser, 1998; Garrett et al., 2003]. If De should be a function of temperature, it would make sense to include temperature in the Ze-IWC relationship. The De as a function of temperature for the 1119 measurements during the CRYSTAL-FACE, TRMM, ARM, FIRE-I, are FIRE-II are shown in Figure 5. In general, the De of ice clouds increase with increasing temperatures. However, the relationship between De and temperature shows much variability. This feature is distinctly shown by the evident separation of the measurements in the TRMM campaign. The TRMM measurements came from cirrus anvils, and thus from an environment denoted by high updraft velocities, whereas the other PSDs came from cirrus having much lower updraft velocities. Our analysis suggests that the temperature cannot be included into the Ze-IWC relationship through a common relationship between temperature and De. [24] Because of the pronounced variability in the relationship between De and temperatures, the effect of De on the Ze-IWC relationship for ice clouds is investigated for two temperature ranges with different De ranges. Note that the deriving Ze-IWC relationships do not involving the Table 1. Fitting Coefficient a and Exponent b for the Relationships Between Ice Water Content (IWC) and Equivalent Radar Backscattering Reflectivity (Ze) at 94 GHz for Clouds Consisting of a Mixture of Ice Particle Habitsa IWC =a Zeb Effective particle size, De (mm) Temperature, T (!C) Ice Cloud Properties a b De < 50 50 < De < 75 75 < De < 100 100 < De < 125 125 <De < 150 150 < De < 175 175 < De < 200 200 < De $30 < T < $25 $35 < T < $30 $40 < T < $35 $45 < T < $40 $50 < T < $45 T < $50 0.3121 0.3429 0.2071 0.1073 0.0679 0.0483 0.0405 0.0314 0.0670 0.0714 0.0876 0.1001 0.1242 0.2115 0.6852 0.7930 0.7880 0.8369 0.8797 0.8948 0.8938 0.8701 0.5703 0.5967 0.5374 0.6327 0.6415 0.6470 a The results are provided for a number of ranges of effective particle sizes (De) and cloud temperatures (T). 5 of 9 D20205 HONG ET AL.: ZE-IWC RELATIONSHIPS FOR ICE CLOUDS D20205 IWC relationships for different De ranges, with a size interval of 25 mm are used for the exponent a of the ZeIWC relationship developed for the entire size range of 50– 200 mm. The coefficients a of the Ze-IWC as a function of De based on the mean values of each size bin are shown in Figure 7. A fitting is performed for the relationships between De and the coefficient a in the range of 50 < De < 200 mm. [27] The Ze-IWC relationships for different De, developed for two temperature ranges of $50!C < T < $40!C and $40!C < T < $25!C, are shown in Figure 8. The IWC and Ze calculated from the individual PSDs are also shown in the figure. The relationships among the Ze, IWC, and De reveal again that one of the three parameters can be derived Figure 5. Effective particle sizes (De) of ice clouds as a function of temperature (T) for the set of 1119 individual PSDs obtained from the CRYSTAL-FACE, TRMM, ARM, FIRE-I, and FIRE-II campaigns. temperatures directly. Two temperature ranges of $50!C to $40!C and $40!C to $25!C are used to separate the measured ice cloud PSDs first. The separated PSDs are then used to derive the Ze-IWC relationships for the De in the range of 50 – 150 mm and 50 – 200 mm at the two temperature ranges, respectively. The two temperature ranges and De ranges are chosen in order to have sufficient samples for the analyses. Similarly to the results shown in Figure 4a, the De values are grouped with an interval of 25 mm. The Ze-IWC relationships in Figure 6 show a similar feature as Figure 4a, but for a given temperature range, the dependence of Ze-IWC relationship on De is more pronounced. [25] For the derived Ze-IWC relationships in the two given temperature ranges (Figure 6), the IWC values are compared to those from the Ze-IWC relationships without considering the influence from the temperatures (Figure 4a) for different De. The correlations between the two derived IWC are similar, and the average deviations of the two derived IWC with respect to the IWC calculated from the particle size distributions are similar. This indicates again that including temperature for the Ze-IWC relationship does not provide a significant improvement of the accuracy of the IWC from the Ze-IWC that includes cloud temperature. [26] However, Figure 6 also indicates that separating the effects of De and temperatures of ice clouds on the Ze-IWC relationships may be useful for inferring the De from the Ze-IWC relationship. For different De, the exponent b of the Ze-IWC relationships are similar. This agrees well with the results presented by Brown et al. [1995], who showed that the exponents of the Ze-IWC relationships for inverseexponential size distributions of varying scale diameter are the same. Thus the mean values of the exponents for the Ze- Figure 6. The relationships between ice water content (IWC) and equivalent radar backscattering reflectivity (Ze) at 94 GHz for clouds consisting of a mixture of ice particle habits as a function of effective particle size (De) when cloud temperatures (T) are in the range of (a) $50!C to $40!C and (b) $40!C to $25!C. 6 of 9 D20205 HONG ET AL.: ZE-IWC RELATIONSHIPS FOR ICE CLOUDS D20205 [30] The Ze-IWC relationship has been found to be sensitive to the variability in the ice particle spectrum [Atlas et al., 1995; Schneider and Stephens, 1995; Brown et al., 1995; Aydin and Tang, 1997; Liu and Illingworth, 2000; Sassen et al., 2002]. In the present study, on the basis of the 1119 measured measurement particle size distributions, the effect of the particle effective size (De) on the Ze-IWC relationships is investigated by deriving the Ze-IWC relationships for different ranges of De. The IWC generally increases with decreasing De for a given Ze. The dependence of Ze-IWC relationships on De shows a regular feature, which may be potentially useful for estimating De from observed Ze. [31] The effect of temperature on the Ze-IWC relationships reveals that the inclusion of temperature in Ze-IWC relationship has no significant improvement for estimating IWC. This is also revealed by the relationships between Figure 7. Coefficient a of the Ze-IWC relationships as a function of effective particle size (De) when cloud temperatures (T) are in the range of $50!C to $40!C and $40!C to $25!C. from the other two from the previously built lookup tables at different temperature ranges. The two lookup tables for the Ze-IWC relationships with different De at two temperature ranges $50!C < T < $40!C and $40!C < T < $25!C) shown in Figure 8 are used to estimate ice cloud De. The estimated ice cloud De agree well with the De calculated using the ice particle size distributions (Figure 9). The relative errors for the two temperatures ranges of $50!C < T < $40!C and $40!C < T < $25!C are less than 32% and 24%, respectively. The RMS of estimated De are about 8 mm and the correlation coefficients between the estimated ice cloud De and the De calculated using the ice particle size distributions are over 94%. 4. Summary and Conclusions [28] The effect of ice particle habits on Ze-IWC relationships is investigated using six different ice habits including hexagonal solid and hollow columns, plates, 3D bullet rosettes, aggregates, and droxtals. The Ze-IWC relationships for ice clouds composed of these habits are derived by the calculated Ze and IWC from 1119 measured particle size distributions obtained from a variety of field campaigns. The Ze-IWC relationships obtained for these individual habits show distinct differences. For a given Ze, the IWC vary in a factor of 1.5– 2.0 for ice cloud composed of different habits, and in particular, the variations in IWC are larger when the Ze are negative than when the Ze are positive. [29] Rather than using a single habit, a habit mixture from Baum et al. [2005a] is used additionally to derive the Ze-IWC relationships. These Ze-IWC relationships show pronounced scattering, indicating the difficulty in finding a single Ze-IWC relationship for all ice clouds [e.g., Atlas et al., 1995; Aydin and Tang, 1997; Liu and Illingworth, 2000; Sassen et al., 2002; Boudala et al., 2006]. Figure 8. Same as Figure 6 but for the Ze-IWC relationships using the fitting coefficient a as a function of De shown in Figure 7. 7 of 9 D20205 HONG ET AL.: ZE-IWC RELATIONSHIPS FOR ICE CLOUDS D20205 apply the Ze-IWC relationships derived for different De within given temperature ranges to operational radar retrieval because the information about De (for estimating IWC) or IWC (for estimating De) is needed. However, the information can be provided by observations made by other active and passive sensors. Moreover, these relationships can be used to simulate radar Ze of ice clouds simulated from the weather forecasting, mesoscale, climate models that output IWC, De, and temperatures. [32] Acknowledgments. The authors thank B. T. Draine and P. J. Flatau for providing their well-documented DDA model. The authors also thank the three anonymous reviewers for constructive comments and suggestion. Ping Yang’s research is supported by a National Science Foundation (NSF) grant (ATM-0239605). References Figure 9. Comparison between the estimated De from the Ze-IWC relationships shown in Figure 8 and the De from measured ice particle size distributions for cloud temperatures (T) in the ranges of (a) $50!C to $40!C and (b) $40!C to $25!C. temperatures and De derived from 1119 data sets measured for ice clouds. However, for a given temperature range, the dependence of the Ze-IWC relationship on De is pronounced. This provides an opportunity to obtain De from the Ze-IWC relationship. The Ze-IWC relationship is derived for different De for the two temperature ranges. The dependence of the Ze-IWC relationship on the effective particle size within a given temperature range is pronounced, and may be useful for inferring the cloud effective particle size from a Ze-IWC relationship. It is difficult to Atlas, D., S. Y. Matrosov, A. J. Heymsfield, M.-D. Chou, and D. B. Wolf (1995), Radar and radiation properties of ice clouds, J. Appl. Meteorol., 34, 2329 – 2345. Aydin, K., and C. Tang (1997), Relationships between IWC and polarimetric radar measurands at 94 and 220 GHz for hexagonal columns and plates, J. Atmos. Oceanic Technol., 14, 1055 – 1063. Bailey, M., and J. Hallett (2004), Growth rates and habits of ice crystals between $20! and $70!C, J. Atmos. Sci., 61, 514 – 544. Battaglia, A., O. Sturniolo, and F. Prodi (2001), Analysis of polarization radar returns from ice clouds, Atmos. Res., 59, 231 – 250. Baum, B. A., A. J. Heymsfield, P. Yang, and S. T. Bedka (2005a), Bulk scattering properties for the remote sensing of ice clouds. part I: Microphysical data and models, J. Appl. Meteorol., 44, 1885 – 1895. Baum, B. A., P. Yang, A. J. Heymsfield, S. Platnick, M. D. King, Y.-X. Hu, and S. T. Bedka (2005b), Bulk scattering properties for the remote sensing of ice clouds. part II: Narrowband models, J. Appl. Meteorol., 44, 1896 – 1911. Baum, B. A., P. Yang, S. L. Nasiri, A. K. Heidinger, A. J. Heymsfield, and J. Li (2007), Bulk scattering properties for the remote sensing of ice clouds. part III: High resolution spectral models from 100 to 3250 cm$1, J. Appl. Meteorol. Clim., 46, 423 – 434. Boudala, F., G. Isaac, Q. Fu, and S. G. Cober (2002), Parameterization of effective particle sizes for high latitude clouds, Int. J. Climatol., 22, 1267 – 1284. Boudala, F., G. Isaac, and D. Hudak (2006), Ice water content and precipitation rate as a function of equivalent radar reflectivity and temperature based on in situ observations, J. Geophys. Res., 111(D11), D11202, doi:10.1029/2005JD006499. Brown, P., A. Illingworth, A. Heymsfield, G. McFarquhar, K. Browning, and M. Gosset (1995), The role of spaceborne millimeter-wave radar in the global monitoring of ice cloud, J. Appl. Meteorol., 34, 2346 – 2366. Chepfer, H., V. Noel, P. Minnis, D. Baumgardner, L. Nguyen, G. Raga, M. J. McGill, and P. Yang (2005), Particle habit in tropical ice clouds during CRYSTAL-FACE: Comparison of two remote sensing techniques with in-situ observations, J. Geophys. Res., 110, D16204, doi:10.1029/2004JD005445. Donovan, D.-P., M. Quante, I. Schlimme, and A. Macke (2004), Use of equivalent spheres to model the relation between radar reflectivity and optical extinction of ice cloud particles, Appl. Opt., 43, 4929 – 4940. Foot, J. S. (1988), Some observations of the optical properties of clouds. II: Cirrus, Q. J. R. Meteorol. Soc., 114, 145 – 164. Garrett, T. J., H. Gerber, D. G. Baumgardner, C. H. Twohy, and E. M. Weinstock (2003), Small, highly reflective ice crystals in low-latitude cirrus, Geophys. Res. Lett., 30(21), 2132, doi:10.1029/2003GL018153. Heymsfield, A. J., and C. M. R. Platt (1984), A parameterization of the particle size spectrum of ice clouds in terms of ambient temperature and the ice water content, J. Atmos. Sci., 41, 846 – 855. Heymsfield, A. J., and L. M. Miloshevich (2003), Parameterization for the cross-sectional area and extinction of cirrus and stratiform ice cloud particles, J. Atmos. Sci., 60, 936 – 956. Heymsfield, A. J., A. Bansemer, P. R. Field, S. L. Durden, J. Stith, J. E. Dye, W. Hall, and T. Grainger (2002), Observations and parameterizations of particle size distributions in deep tropical cirrus and stratiform precipitating clouds: Results from in situ observations in TRMM field campaigns, J. Atmos. Sci., 59, 3457 – 3491. Heymsfield, A. J., S. Matrosov, and B. A. Baum (2003), Ice water pathoptical depth relationships for cirrus and precipitating cloud layers, J. Appl. Meteorol., 42, 1369 – 1390. 8 of 9 D20205 HONG ET AL.: ZE-IWC RELATIONSHIPS FOR ICE CLOUDS Heymsfield, A. J., A. Bansemer, C. Schmitt, C. Twohy, and M. R. Poellot (2004), Effective ice particle densities derived from aircraft data, J. Atmos. Sci., 61, 982 – 1003. Heymsfield, A. J., Z. Wang, and S. Matrosov (2005), Improved radar ice water content retrieval algorithms using coincident microphysical and radar measurements, J. Appl. Meteorol., 44, 1391 – 1412. Hong, G. (2007a), Radar backscattering properties of nonspherical ice crystals at 94 GHz, J. Geophys. Res., 112, D22203, doi:10.1029/ 2007JD008839. Hong, G. (2007b), Parameterization of scattering and absorption properties of nonspherical ice crystals at microwave frequencies, J. Geophys. Res., 112, D11208, doi:10.1029/2006JD008364. Hong, G., P. Yang, B.-C. Gao, B. A. Baum, Y. X. Hu, M. D. King, and S. Platnick (2007), High cloud properties from three years of MODIS Terra and Aqua data over the Tropics, J. Appl. Meteor. Climatol., 46, 1840 – 1856. King, M. D., W. P. Menzel, Y. J. Kaufman, D. Tanré, B.-C. Gao, S. Platnick, S. A. Ackerman, L. A. Remer, R. Pincus, and P. A. Hubanks (2003), Cloud and aerosol properties, precipitable water, and profiles of temperature and humidity from MODIS, IEEE Trans. Geosci. Remote Sens., 41, 442 – 458. King, M. D., S. Platnick, P. Yang, G. T. Arnold, M. A. Gray, S. A. Ackerman, and K. N. Liou (2004), Remote sensing of liquid water and ice cloud optical thickness, and effective radius in the arctic: Application of airborne multispectral MAS data, J. Atmos. Ocean. Technol., 21, 857 – 875. King, M. D., S. Platnick, P. A. Hubanks, G. T. Arnold, E. G. Moody, G. Wind, and B. Wind (2006), Collection 005 change summary for the MODIS cloud optical property (06_OD) Algorithm. Kosarev, A. L., and I. P. Mazin (1991), An empirical model of the physical structure of upper layer clouds, Atmos. Res., 26, 213 – 228. Lemke, H. M., and M. Quante (1999), Backscatter characteristics of nonspherical ice crystals: Assessing the potential of polarimetric radar measurements, J. Geophys. Res., 104, 31,739 – 31,752. Liu, C. L., and A. J. Illingworth (2000), Toward more accurate retrievals of ice water content from radar measurements of clouds, Appl. Meteorol., 39, 1130 – 1146. Mace, G., A. J. Heymsfield, and M. R. Poellot (2002), On retrieving the microphysical properties of cirrus clouds using the moments of the millimeter-wavelength Doppler spectrum, J. Geophys. Res., 107(D24), 4815, doi:10.1029/2007JD001308. Macke, A., P.-N. Francis, G. M. McFarquhar, and S. Kinne (1998), The role of ice particle shapes and size distributions in the single scattering properties of cirrus clouds, J. Atmos. Sci., 55, 2874 – 2883. Matrosov, S. Y., A. V. Korolev, and A. J. Heymsfield (2002), Profiling cloud mass and particle characteristic size from Doppler radar measurements, J. Atmos. Oceanic Technol., 19, 1003 – 1018. Miloshevich, L. M., and A. J. Heymsfield (1997), A balloon-borne continuous cloud particle replicator for measuring vertical profiles of cloud microphysical properties: Instrument design, performance, and collection efficiency analysis, J. Atmos. Oceanic Technol., 14, 753 – 768. Mishchenko, M. I., J. W. Hovenier, and L. D. Travis (2000), Light Scattering by Nonspherical Particles: Theory, Measurements, and Applications, Academic Press, San Diego. Mitchell, D. L. (1991), Evolution of snow-size spectra in cyclonic storms. part II: Deviations from the exponential form, J. Atmos. Sci., 48, 1885 – 1899. D20205 Okamoto, H. (2002), Information content of the 95 GHz cloud radar signals: Theoretical assessment of effects of non-sphericity and error evaluations of the discrete dipole approximation, J. Geophys. Res., 107(D22), 4628, doi:10.1029/2001JD001386. Ou, S. C., and K. N. Liou (1995), Ice microphysics and climatic temperature perturbations, Atmos. Res., 35, 127 – 138. Ou, S. C., K. N. Liou, Y. Takano, N. X. Rao, Q. Fu, A. J. Heymsfield, L. M. Miloshevich, B. Baum, and S. A. Kinne (1995), Remote sounding of cirrus cloud optical depths and ice crystal sizes from AVHRR data: Verification using FIRE-II-IFO measurements, J. Atmos. Sci., 52, 4143 – 4158. Platnick, S., M. D. King, S. A. Ackerman, W. P. Menzel, B. A. Baum, J. C. Riédi, and R. A. Frey (2003), The MODIS cloud products: Algorithms and examples from Terra, IEEE Trans. Geosci. Remote Sens., 41, 459 – 473. Sassen, K., Z. Wang, V. I. Khvorostyanov, G. L. Stephens, and A. Bennedetti (2002), Cirrus cloud ice water content radar algorithm evaluation using an explicit cloud microphysical model, J. Appl. Meteorol., 41, 620 – 628. Sato, K., and H. Okamoto (2006), Characterization of Ze and LDR of nonspherical and inhomogeneous ice particles for 95-GHz cloud radar: Its implication to microphysical retrievals, J. Geophys. Res., 111, D22213, doi:10.1029/2005JD006959. Schneider, T. L., and G. L. Stephens (1995), Theoretical aspects of modeling backscattering by cirrus ice particles at millimeter wavelengths, J. Atmos. Sci., 52, 4367 – 4385. Shupe, M. D., T. Uttal, and S. Y. Matrosov (2005), Arctic cloud microphysics retrievals from surface-based remote sensors at SHEBA, J. Appl. Meteorol., 44, 1544 – 1562. Stephens, G. L., et al. (2002), The Cloudsat Mission and the A-Train: A new dimension of space-based observations of clouds and precipitation, Bull. Am. Meteorol. Soc., 83, 1771 – 1790. Stith, J. L., J. E. Dye, A. Bansemer, A. J. Heymsfield, D. A. Grainger, W. A. Petersen, and R. Cifelli (2002), Microphysical observations of tropical clouds, J. Appl. Meteorol., 41, 97 – 117. Stith, J. L., J. A. Haggerty, A. J. Heymsfield, and C. A. Grainger (2004), Microphysical characteristics of tropical updrafts in clean conditions, J. Appl. Meteorol., 43, 779 – 794. Wylie, D. P., D. L. Jackson, W. P. Menzel, and J. J. Bates (2005), Trends in global cloud cover in two decades of HIRS observations, J. Clim., 18, 3021 – 3031. Wyser, K. (1998), The effective radius in ice clouds, J. Clim., 11, 1793 – 1802. Yang, P., H. Wei, H.-L. Huang, B. A. Baum, Y. X. Hu, G. W. Kattawar, M. I. Mishchenko, and Q. Fu (2005), Scattering and absorption property database for nonspherical ice particles in the near-through far-infrared spectral region, Appl. Opt., 44, 5512 – 5523. $$$$$$$$$$$$$$$$$$$$$$ B. A. Baum, Space Science and Engineering Center, University of Wisconsin-Madison, 1225 West Dayton St., Madison, WI 53706, USA. A. J. Heymsfield, National Center for Atmospheric Research, 3450 Mitchell Lane, Boulder, CO 80307-3000, USA. G. Hong and P. Yang, Department of Atmospheric Sciences, Texas A&M University, 3150 TAMU College Station, TX 77843, USA. (hong@ariel. met.tamu.edu) 9 of 9