PHYSICAL REVIEW A 67, 012303 共2003兲 Efficient distillation beyond qubits Karl Gerd H. Vollbrecht* and Michael M. Wolf† Institute for Mathematical Physics, TU Braunschweig, Braunschweig, Germany 共Received 4 September 2002; published 7 January 2003兲 We provide generalizations of known two-qubit entanglement distillation protocols for arbitrary Hilbert space dimensions. The protocols, which are analogs of the hashing and breeding procedures, are adapted to bipartite quantum states that are diagonal in a basis of maximally entangled states. We show that the obtained rates are optimal, and thus equal to the distillable entanglement, for a (d⫺1)-parameter family of rank deficient states. Methods to improve the rates for other states are discussed. In particular, for isotropic states it is shown that the rate can be improved such that it approaches the relative entropy of entanglement in the limit of large dimensions. DOI: 10.1103/PhysRevA.67.012303 PACS number共s兲: 03.67.⫺a, 03.65.Ta I. INTRODUCTION The possibility of entanglement distillation plays a crucial role in quantum communication and quantum information processing 共cf. 关1兴兲. Together with quantum error correction it enables all the fascinating applications provided by quantum information theory in the presence of a noisy and interacting environment. It provides a method to overcome decoherence without requiring a complete isolation from the environment. The usual abstract way of thinking about entanglement distillation is the following. Two parties, Alice and Bob, situated at distant locations share n copies of a mixed entangled quantum state , which they may have obtained by sending one part of a pure maximally entangled state through a noisy quantum channel. Assume that both parties are able to perform any collective quantum operation, which merely acts locally on their part of the n copies. Moreover, Alice and Bob are connected via a classical channel, such that they can perform arbitrary many rounds of local quantum operations, where each round may depend on the measurement outcomes of all the preceding operations on both sides. The set of operations accessible in this way is called LOCC 共local operations and classical communication兲. It was shown in one of the seminal works from the early years of quantum information theory 关2兴 that under the above conditions Alice and Bob can for certain two-qubit states distill a smaller number m of states ⬘ , which are closer to the maximally entangled state than the initial ones, from a larger number n⭓m of more weakly entangled states . This can be done in such a way that in the limit n→⬁ the output states ⬘ become maximally entangled. The asymptotic ratio m/n is then called the rate of the distillation protocol and the maximally accessible rate under all LOCC protocols is an important measure of entanglement, the distillable entanglement D( ). The latter quantifies in some sense the amount of useful entanglement contained in the state . Up to now the hashing/breeding distillation protocol presented in 关2,3兴, which is adapted to Bell diagonal states of *Electronic address: k.vollbrecht@tu-bs.de † Electronic address: mm.wolf@tu-bs.de 1050-2947/2003/67共1兲/012303共9兲/$20.00 two qubits, is essentially the only protocol leading to a nonzero rate in the asymptotic limit. The present paper is devoted to generalizing these protocols to higher dimensions. We will therefore closely follow the ideas of Refs. 关2,3兴. The protocols are adapted to states that are diagonal in a basis of maximally entangled states or mapped onto such states by a LOCC twirl operation. The main step is to translate the apparent quantum task into a classical problem in such a way that all the operations involved are LOCC. The following results are obtained. 共1兲 We provide an entanglement assisted distillation protocol 共breeding兲 that works for any finite dimension d. It is in this case assumed that Alice and Bob share maximally entangled states initially, which they may have obtained with a different protocol 共e.g., hashing in a prime-dimensional subspace兲 and with a smaller rate. The attained distillation rate is given by log2 d⫺S„T共 兲 …, 共1兲 where S(T( )) is the von Neumann entropy of the twirled state . 共2兲 We show that a hashing protocol exists for prime dimensions d, which does not require any predistilled states. The rate obtained is the same as in Eq. 共1兲. The method can easily be generalized to dimensions that are powers of primes, if one uses a different basis of maximally entangled states. 共3兲 Both protocols, breeding and hashing, are shown to be optimal for a (d⫺1)-parameter family of low rank states. This generalizes the observation of Rains 关4兴 for the case d ⫽2. 共4兲 We discuss methods for improving the rates for isotropic states. In particular, the projection onto local subspaces will turn out to yield the optimal rate in the limit of large dimensions. Despite the quite considerable effort in the theory of entanglement distillation and its practical relevance, many of the basic questions are yet unanswered. So we know neither a decidable necessary and sufficient criterion for distillability in Hilbert spaces Cd 丢 Cd with d⬎2, nor D( ), even for otherwise simple quantum states . What makes the investigation of distillability so difficult is, on the one hand, the 67 012303-1 ©2003 The American Physical Society PHYSICAL REVIEW A 67, 012303 共2003兲 KARL GERD H.VOLLBRECHT AND MICHAEL M. WOLF asymptotic limit (n→⬁) and, on the other hand, the mathematically intractable set of LOCC operations. However, many partial results have been obtained in various directions, and before we go into the details of the present article we want at least briefly to recall some of them. (a) Distillability. For the case of two qubits it was shown in 关6兴 that every entangled state is distillable. A general necessary condition for the distillability of a state is the fact that its partial transpose T A , defined with respect to a given product basis by 具 i j 兩 T A 兩 kl 典 ⫽ 具 k j 兩 兩 il 典 , has a negative eigenvalue 关5兴. Except for special cases like states on C2 丢 Cn 关6,7兴 and Gaussian states 关8兴, it is, however, unclear whether this condition is sufficient as well. There is some evidence presented in 关7,9兴 that this may not be the case and that there are indeed undistillable states, whose partial transpose is not positive 共NPPT兲. However, it was shown in 关10兴 共see also 关11兴兲 that every NPPT state becomes distillable when adding a certain bound entangled state with positive partial transpose 共PPT兲. Moreover, this activation process was shown to require only an infinitesimal amount of entanglement contained in the additional PPT state 关10兴. (b) Distillation protocols. Up to now, essentially the only mixed state distillation protocol leading to a nonzero rate in the asymptotic limit is the breeding/hashing protocol presented in 关2,3兴, which is adapted to Bell-diagonal states of two qubits. There are, however, several purification schemes that increase the purity and entanglement of a state without yielding a nonzero rate on their own. The best known examples are the recurrence protocols presented in 关2,3兴 共see 关12兴 for the discussion of imperfect operations兲 and 关13兴. These were investigated also for higher dimensions in 关14兴 and 关15兴. In 关16兴 it was shown that these methods can be improved by using more than one source state per target. A systematic generalization of the local unitaries applied in the recurrence method for two-qubit systems was recently provided in 关17兴. A protocol which is analogous to the hashing procedure but uses PPT preserving rather than LOCC operations is described in 关18兴. (c) Distillable entanglement. For pure states the distillable entanglement is equal to the von Neumann entropy of the reduced state 关19兴. For mixed states only bounds are known, which can be calculated for some very special cases 共cf. 关20兴兲. The best known upper bound for the distillable entanglement can be found in 关21兴. A closely related bound, which we will describe in detail later, is given by the relative entropy of entanglement 关4,22兴. (d) Relations to other quantum information tasks. It was already noticed in 关3兴 that a distillation protocol involving only one-way classical communication 共like the hashing protocol兲 corresponds to a quantum error correcting code, and vice versa. Moreover, upper bounds for the distillable entanglement allow one to obtain upper bounds for quantum channel capacities 共cf. 关23兴兲. In particular, the inequality D 1 共 兲 ⭓S 共 trB 关 兴 兲 ⫺S 共 兲 , 共2兲 where D 1 ( ) is the distillable entanglement for one-way communication protocols, implies Shannon-like formulas for quantum capacities, providing the quantum noisy coding theorem 关23兴. The inequality 共2兲 is consistent with the results we obtain in Sec. V. An important application of distillation and purification schemes is also the possibility of factoring out an eavesdropper for secret quantum communication 关13,24兴. This is known as quantum privacy amplification. II. PRELIMINARIES Let us first introduce the preliminaries we need for the distillation protocols described in Secs. III and IV. We begin by characterizing the states for which the protocols are adapted and we will subsequently specify the set of required local operations. A. Basis of maximally entangled states Bases of maximally entangled states 兵 ⌿ kl 其 , k,l 苸 兵 0, . . . ,d⫺1 其 , exist for any Hilbert space H⫽Cd 丢 Cd and correspond to an orthonormal operator basis of d 2 unitary d⫻d matrices 兵 U kl 其 via 兩 ⌿ kl 典 ⬅ 共 1 丢 U kl 兲 兩 ⍀ 典 , 共3兲 with 兩 ⍀ 典 being a maximally entangled state. The latter is in the following chosen to be 兩 ⍀ 典 ⫽ 兩 ⌿ 00典 ⫽1/冑d 兺 d⫺1 j⫽0 兩 j j 典 . A general construction procedure 关25兴 for unitary operator bases involves Latin squares and complex Hadamard matrices and the best known example constructed in this way is of the form d⫺1 U kl ⫽ 兺 r⫽0 rl 兩 k 丣 r 典具 r 兩 , ⫽e 2 i/d , 共4兲 where 丣 means addition modulo d. The set of unitaries in Eq. 共4兲 is orthonormal with respect to the Hilbert-Schmidt scalar product, i.e., tr关 U * i j U kl 兴 ⫽d ␦ ik ␦ jl , and forms a discrete Weyl system since U i j U kl ⫽ jk U i 丣 k, j 丣 l . In the following we will solely use the maximally entangled basis from Eqs. 共3兲 and 共4兲 or tensor products thereof and denote the first index as the shift and the second as the phase index. B. Symmetric states Symmetric states commuting with a group of local unitaries play an important and paradigmatic role in quantum information theory and in particular in the context of entanglement distillation. The best known examples are Werner states, isotropic states, and Bell-diagonal states. The latter are convex combinations of the four maximally entangled Bell states of two qubits and contain in this case the isotropic states, which for two-qubit systems are in turn equivalent to Werner states. In analogy to the two-qubit case, we will call a state on Cd 丢 Cd Bell diagonal if it can be written as a convex combination of maximally entangled states P i j ⫽ 兩 ⌿ i j 典具 ⌿ i j 兩 . The corresponding symmetry group is given by 012303-2 PHYSICAL REVIEW A 67, 012303 共2003兲 EFFICIENT DISTILLATION BEYOND QUBITS G⫽ 兵 U i, j 丢 U i,⫺ j 其 , 共5兲 which is an Abelian group with the property that its commutant, which is again spanned by G, contains d 2 onedimensional projectors 兵 P i j 其 . Hence, for 兵 i j 其 being convex weights, ⫽ 兺i j i j P i j ⇔ ᭙ g苸G: 关 ,g 兴 ⫽0. 共6兲 Moreover, every nonsymmetric state can be mapped onto a Bell-diagonal state T( ) by means of a discrete twirl operation T共 兲 ⫽ 1 d2 兺 g苸G g * g, 共7兲 which can be implemented by means of local operations and classical communication. Isotropic states, which are completely characterized by their fidelity f ª 具 ⍀ 兩 兩 ⍀ 典 , are a special instance of Belldiagonal states with 00⫽ f and i j ⫽(1⫺ f )/(d 2 ⫺1) for (i, j)⫽(0,0). An isotropic state is entangled and distillable if and only if f ⬎1/d 关14兴. C. Local operations and measurements An essential ingredient for any distillation protocol acting on two-qubit systems is the controlled-NOT 共CNOT兲 operation. One possibility of generalizing this operation to higher dimensions is to use a controlled shift 共CS兲operation 关14兴, which acts as C兩i典 丢 兩 j典⫽兩i典 丢 兩 j 丣 i典, 共8兲 where the first tensor factor is the source and the second the target. It is readily verified that a bilateral controlled shift 共BCS兲 operation, where both parties in a bipartite system apply CS operations locally on a tensor product of two maximally entangled states, acts as 共 C 丢 C 兲 兩 ⌿ i j 典 丢 兩 ⌿ kl 典 ⫽ 兩 ⌿ i, j両l 典 丢 兩 ⌿ k 丣 i,l 典 , 共9兲 where the first tensor product on the left-hand side in Eq. 共9兲 corresponds to the Alice-Bob split, whereas the others correspond to the source-target split. Note that the target state picks up the shift index of the source, i.e., k哫k 丣 i, while the source remains unchanged if and only if l⫽0. If we measure a target state of the form 兩 ⌿ kl 典 in a computational basis, then k is the difference of the measurement outcomes. In this way we can obtain information about the shift index of an unknown source state, if we know the target state: We first apply a BCS operation and then measure the target state in the computational basis. An analogous transformation can be defined for the phase indices, since we can simply interchange the two indices by the following local unitary operation: 共 V 丢 V̄ 兲 P i j 共 V 丢 V̄ 兲 * ⫽ P j,⫺i , V⫽ 1 冑d kl 兩 k 典具 l 兩 . 兺 k,l 共10兲 So we can define a modified bilateral controlled shift 共MBCS兲 operation by first applying a V 丢 V̄ transformation to the source state, followed by a BCS operation on source and target and then undoing the local operation on the source state by a (V 丢 V̄) * rotation. The MBCS operation then acts as P i j 丢 P kl 哫 P i 丣 l, j 丢 P k 丣 j,l , 共11兲 where the second tensor factor corresponds to the target again. Assume now that we have one target state 兩 ⌿ 00典 and n source states with shift indices k 1 , . . . ,k n and phase indices l 1 , . . . ,l n . We now apply s a BCS operations and p a MBCS operations to the ath source and the target. If we then measure the target state again in the computational basis, the difference of the measurement outcomes will be n n a⫽1 a⫽1 共 丣 k a s a 兲 丣 共 丣 l a p a 兲 ⫽: 具 kជ ,sជ 典 丣 具 ជl ,pជ 典 . 共12兲 This enables us to obtain some information about the distribution of the shift and phase indices of the source states without disturbing them. In the following we will organize the shift and phase indices of a sequence of maximally entangled states in a single vector Sជ ª(k 1 , . . . ,k n ,l 1 , . . . ,l n ) and accordingly the mulជ tiplicities of the BCS and MBCS operations in a vector M ជ then belong to ª(s 1 , . . . ,s n ,p 1 , . . . ,p n ). Both Sជ and M 兵 0, . . . ,d⫺1 其 2n , i.e., they are elements of the group Z2n d with addition modulo d. ជ folThe sequence of local operations characterized by M lowed by a measurement of an additionally required target state P 00 thus yields the information ជ ,Sជ 典 ª 具M 2n 丣 M i S i ⫽ 具 kជ ,sជ 典 丣 具 ជl ,pជ 典 共13兲 i⫽1 about a sequence Sជ of maximally entangled states, without disturbing the latter. To complete the list of basic local operations required later on we have still to introduce a generalization of a /2 rotation given by u共 g 兲ª 兺k e i /dk g兩 k 典具 k 兩 , 2 共14兲 where g苸Z is an arbitrary number. We will use this within bilateral operations of the form u(g) 丢 ū(g) and v (g) 丢 v̄ (g), where v (g)ªV * u(g)V. These unitary operations act on a maximally entangled state P kl as 012303-3 关 u 共 g 兲 丢 ū 共 g 兲兴 P kl 关 u 共 g 兲 丢 ū 共 g 兲兴 * ⫽ P k,l両gk , 共15兲 PHYSICAL REVIEW A 67, 012303 共2003兲 KARL GERD H.VOLLBRECHT AND MICHAEL M. WOLF 关v共 g 兲 丢 v̄共 g 兲兴 P kl 关v共 g 兲 丢 v̄共 g 兲兴 * ⫽ P k 丣 gl,l . D. Why primes are special Measurements based on the Z2n d scalar product in Eq. 共13兲 play a crucial role in the entanglement distillation protocols discussed in the following. One of the main tasks will ជ such that we thereby be to choose the measurement vector M obtain as much information about the sequence Sជ as possible. In general this can be a highly nontrivial problem. However, ជ randomly if the dimension d is a prime, then choosing M turns out to be a pretty good choice. The reason why this works well only for prime dimensions is that in this case Zd is a field, which means that it is an Abelian group not only with respect to the addition modulo d, but also with respect to the multiplication if we exclude the zero element. That is, for a,b,x苸Zd , a⫽0, every equation of the form 共17兲 b⫽ax mod d has a unique solution for x if and only if d is prime. This leads us to the following lemma. Lemma 1. Let Sជ ⫽Sជ ⬘ be elements of Zm d with d prime. m Given a scalar product 具 xជ ,yជ 典 ª 丣 i⫽1 x i y i and a uniformly ជ 苸Zmd , the probability for distributed random vector M ជ ,Sជ 典 ⫽ 具 M ជ ,Sជ ⬘ 典 is equal to 1/d. 具M ជ 典 ⫽0. Proof. We ask for the probability that 具 Sជ ⫺Sជ ⬘ ,M Since Sជ ⫽Sជ ⬘ , there exists a component x where S x ⫽S x⬘ and we can write ជ 典 ⫽M x 共 S x ⫺S x⬘ 兲 ⫹ 0⬅ 具 Sជ ⫺Sជ ⬘ ,M 兺 M i共 S i ⫺S ⬘i 兲 . i⫽x 共18兲 Assume now that all M i ,i⫽x, are already randomly chosen. Then Eq. 共18兲 has the form of Eq. 共17兲 with x⫽M x , a ⫽(S x ⫺S x⬘ ), and b⫽ 兺 i⫽x M i (S ⬘i ⫺S i ). Since this equation has a unique solution for x and M x is a uniformly distributed random variable, the probability that M x matches the solution is indeed 1/d. 䊏 III. THE BREEDING PROTOCOL The breeding protocol is the preliminary stage of the hashing protocol discussed in the next section. Both are adapted to the distillation of Bell-diagonal states and the main idea is to transform this quantum problem into the classical problem of identifying a word given the probability distribution of the corresponding alphabet and a restricted set of measurements. Assume that Alice and Bob share n copies of a Belldiagonal state , such that 丢 n⫽ 兺 k 1 , . . . ,k n ,l 1 , . . . ,l n P k 1 l 1 丢 ••• 丢 P k n l n ª P Sជ 共16兲 k 1 l 1 ••• k n l n P k 1 l 1 丢 ••• 丢 P k n l n . 共19兲 共20兲 with probability k 1 l 1 ••• k n l n . Note that, if they knew the sequence Sជ ⫽(k 1 , . . . ,k n ,l 1 , . . . ,l n ), they could apply appropriate local unitary operations in order to obtain the stan丢n and thus gain nlog2d dard maximally entangled state P 00 ebits of entanglement. Let us further assume that they have already a sufficiently large set of predistilled maximally entangled states P 00 and that they are able to perform all the local operations such as BCS and MBCS operations described in the previous section. In this case they can utilize the predistilled states for ជ ,Sជ 典 performing local measurements leading to the result 具 M as discussed in Eq. 共13兲 in order to obtain some information about the sequence Sជ . However, every single measurement ជ will destroy one of the predistilled maximally entangled M states, and the task is therefore to identify the sequence Sជ using as few measurements as possible. At this point the quantum task of distillation is transformed into an entirely classical problem: Given an unknown vector Sជ and the possibility of measuring functions of the ជ ,Sជ 典 , how many measurements r do we need to idenform 具 M ជ tify S ? Knowing Sជ , we gained n maximally entangled pairs, but destroyed r, such that the overall gain would be (1 ⫺r/n)log2d ebits per copy. We would need r⫽2n measurements to identify a completely random Sជ 苸Z2n d with independently and uniformly distributed components. So we would destroy more entangled pairs than we gain. Fortunately, however, the set of possible vectors Sជ is not completely random but has a distribution depending on the spectrum of the Bell-diagonal state . In the limit of many copies there exists thus a set of likely sequences containing only 2 nS( ) ⭐d 2n different vectors Sជ with the property that the probability that a vector Sជ is contained within this set of likely sequences approaches 1 in the limit n→⬁ 关26兴. Here S( ) is the von Neumann entropy of the density matrix, which is equal to the Shannon entropy of the spectrum of , i.e., S 共 兲 ⫽⫺ kl log2 kl . 兺 k,l 共21兲 ជ ranNow let Alice and Bob choose each measurement M domly. Then Lemma 1 tells us that if d is prime they can reduce their list of possible sequences by a factor of 1/d after every measurement by deleting every sequence that is not consistent with the obtained result. Since their list initially contains 2 nS( ) possible sequences, r⫽nS( )/log2d measurements are required in order to identify Sជ in the limit of large n. The rate obtained in this way in the asymptotic limit is a lower bound to the 共entanglement assisted兲 distillable entanglement, which is thus An appropriate interpretation of Eq. 共19兲 is to say that Alice and Bob share the state 012303-4 D 共 兲 ⭓log2 d⫺S 共 兲 . 共22兲 PHYSICAL REVIEW A 67, 012303 共2003兲 EFFICIENT DISTILLATION BEYOND QUBITS Let us now extend the obtained result, expressed in Eq. 共22兲, from prime dimensions to arbitrary ones. As we have already mentioned, Lemma 1 holds only for primes and cannot be extended. A way out of this dilemma is to use controlled shift operations between Hilbert spaces of different dimensions. The definition looks similar to Eq. 共23兲: surement outcomes, i.e., the final shift index of the target, will be C ⬘兩 i 典 丢 兩 j 典 ª 兩 i 典 丢 兩 j 丣 i 典 , ជ ,Rជ 典 in Eq. 共25兲 is the familiar outcome if The first term 具 M n⫺1 M i M i⫹n⫺1 S 2n the target state is P 00 . The terms ⫺ 兺 i⫽1 ⫹S n correspond to the other possible targets and their back action onto the source states, and the last term gS 2n is due to the initial v (g) 丢 v̄ (g) rotation. Note that in general the outcome also depends on the order in which the different BCS and MBCS operations are carried out. For Eq. 共25兲 first all BCS and then all MBCS operations were applied. With the possibility of measuring functions of the form 共25兲 we will now follow the line of argumentation of the previous section and show that the gain of information is 共asymptotically兲 at least log2d bits per measurement, if the dimension d is prime. Therefore we ask again for the probability that two different sequences Sជ ⫽Sជ ⬘ lead to the same ជ and g measurement outcome under the assumption that M are uniformly distributed random variables. To this end we have to distinguish between three different cases. 共1兲 The two sequences differ only in S n ⫽S n⬘ . This is the trivial case where Sជ and Sជ ⬘ are distinguished with unit probability. 共2兲 Sជ and Sជ ⬘ differ in the phase index of their target, i.e., ជ is already cho⬘ . If we assume in this case that M S 2n ⫽S 2n ជ ;g 兩 Sជ 典 ⫽ 具 M ជ ;g 兩 Sជ ⬘ 典 is of the form sen, then the equation 具 M b⫽ax with g playing the role of x. Hence, the probability that a randomly chosen g matches the right solution is 1/d, if d is prime. 共3兲 Sជ and Sជ ⬘ have a target state with the same phase ⬘ and Rជ ⫽Rជ ⬘ . Then Lemma 1 tells us that index, i.e., S 2n ⫽S 2n ជ distinguishes the two sequences Rជ a randomly chosen M ជ ⬘ with probability 1/d, if d is prime. ⫽R The hashing protocol consists now of several rounds of such measurements, where each round destroys the entanglement of one of the n pairs characterized by Sជ . The relevant part of the system after r rounds is thus described by a vector and the measurements applied to Sជ (r) are in Sជ (r)苸Z2(n⫺r) d ជ (r)苸Z2(n⫺r⫺2) and g(r)苸Zd . Note turn characterized by M d that, given the sequence of measurements, the vector Sជ (r) deterministically depends on Sជ ⫽Sជ (0). The above discussion implies now that the probability 共23兲 with the only difference that i runs from 0 to d⫺1 whereas j runs from 0 to d ⬘ ⫺1, where d ⬘ is now supposed to be a prime with d ⬘ ⭓d. Moreover, the addition in the second ket 共target兲 is modulo d ⬘ . The penalty of the BCS and MBCS operations based on such a controlled shift operation is that the source states after the operation will in general no longer be of the form P kl given by Eqs. 共3兲 and 共4兲. However, they still are, if the target state, acting on Cd ⬘ 丢 Cd ⬘ , has a phase index equal to zero. Then, ⬘ 典 ⫽ 兩 ⌿ i, j 典 丢 兩 ⌿ ⬘k 丣 i,0典 . 共 C ⬘ 丢 C ⬘ 兲 兩 ⌿ i j 典 丢 兩 ⌿ k0 共24兲 In this way we can straightforward generalize the result of Eq. 共22兲 to Bell-diagonal states of arbitrary dimension, just by reshuffling the degrees of freedom of the predistilled maximally entangled states. Hence, the crucial point is that the target states, which are in the case of the breeding protocol the predistilled resources, have prime dimensions. IV. THE HASHING PROTOCOL So far we have assumed that Alice and Bob initially share a set of predistilled maximally entangled states. We took into account this resource when calculating the rate, but, since the additivity of the distillable entanglement is not yet decided for bipartite systems, we might expect a smaller rate for the 共non entanglement assisted兲 distillation rate. The hashing protocol, however, achieves the same asymptotic rate as the previously discussed breeding protocol without requiring additional predistilled states. The main idea, though, is still the same: Alice and Bob identify the sequence Sជ by means of LOCC. The protocol, however, is now a bit more complicated since if we use one of the n states characterized by Sជ 苸Z2n d as target for the BCS and MBCS operations then we have to take into account the back action from the unknown target to the remaining source states. We will in the following choose the nth state characterized by S n and S 2n as the target and consider the remainជ ing n⫺1 states characterized by a vector R ⫽(S 1 , . . . ,S n⫺1 ,S n⫹1 , . . . ,S 2n⫺1 ) as source states. In the first step of the protocol a bilateral v (g) 丢 v̄ (g) rotation with a randomly chosen number g苸 兵 0, . . . ,d⫺1 其 is applied to the target state. This shifts some information about the phase index of the target state into its shift index. ជ 苸Z2n⫺2 is chosen and the two Then a random vector M d parties perform the respective BCS and MBCS operations. After measuring the target state, the difference of the mea- n⫺1 ជ ;g 兩 Sជ 典 ª 具 M ជ ,Rជ 典 ⫺ 具M 兺 i⫽1 M i M i⫹n⫺1 S 2n ⫹S n ⫹gS 2n . 共25兲 r⫺1 ជ 共 r 兲 ;g 共 r 兲 兩 Sជ 共 r 兲 ⫺Sជ 共 r 兲 ⬘ 典 ⫽0 兴 P 关 Sជ 共 r 兲 ⫽Sជ 共 r 兲 ⬘ ᭙ k⫽0 :具M 共26兲 that Sជ (r) and Sជ (r) ⬘ agree on all r measurement results, and thereby remain distinct, is at most d ⫺r , if d is prime. Since we have initially again about 2 nS( ) likely sequences, we 012303-5 PHYSICAL REVIEW A 67, 012303 共2003兲 KARL GERD H.VOLLBRECHT AND MICHAEL M. WOLF need 共in the limit of large n) r⫽nS( )/log2d rounds in order to identify the remaining sequence Sជ (r). This leads us again to the rate in Eq. 共22兲. What if d is not prime? Unfortunately, we cannot extend the result to other dimensions in the way we did in the case of the breeding protocol, since we do not have any target states of prime dimension with zero phase indices. However, if the dimension is a power of a prime d⫽d ⬘ p , then we can easily extend the result for states that are diagonal with respect to a different basis of maximally entangled states, given by P kជ ជl ª p 丢 i⫽1 P kili, 共27兲 1 ⫽ d 丢 C . The 共LOCC兲 twirl operation, which maps an arbitrary state onto a state diagonal in this basis, is given by 哫T 丢 p ( ). The hashing protocol can then be applied in the described manner to pn tensor factors of prime dimension d ⬘ and we obtain again in this way the rate in Eq. 共22兲 for states in d ⫽d ⬘ p dimensions. Moreover, note that isotropic states are diagonal in both bases given by Eqs. 共3兲 and 共4兲 and Eq. 共27兲. V. OPTIMALITY FOR LOW RANK STATES It is well known from the case of two-qubit systems that the hashing/breeding protocol is not optimal in general. However, for a certain (d⫺1)-parameter family of rank deficient states, we will show that the rate obtained is equal to the relative entropy of entanglement. Since the latter is an upper bound to the distillable entanglement, this implies that the protocols are optimal in this case. For d⫽2 this was first noticed by Rains in 关4兴. Consider mixed states of rank smaller than or equal to d: 兺 l兩 l 典具 l兩 , l⫽1 共28兲 which are diagonal with respect to 兩 l 典 ª 兩 ⌿ 0,l 典 ⫽ 共30兲 冋 1 ⫽ 兺 exp d 2 l,r,s ⫽ 1 d 册 2i l 共 r⫺s 兲 兩 r,r 典具 s,s 兩 d 共31兲 d⫺1 兺 r⫽0 兩 r 典具 r 兩 丢 兩 r 典具 r 兩 共32兲 E R 共 兲 ⫽inf 共 tr关 共 log2 ⫺log2 兲兴 兲 , 共33兲 where the infimum is taken over all separable states . Hence, if we choose ⫽ sep , the distillable entanglement is bounded by D 共 兲 ⭐E R 共 兲 ⭐⫺tr关 log2 sep兴 ⫺S 共 兲 . 共34兲 However, ⫺tr关 log2sep兴 ⫽log2d and the rate achieved by the breeding/hashing protocol is thus optimal for every . Strictly speaking, the hashing protocol leads to distillable entanglement and the breeding rate is equal to the distillable entanglement D ⬘ assisted by a maximally entangled resource . The latter can easily be seen by noting that D ⬘ 共 兲 ⫽D 共 丢 兲 ⫺E R 共 兲 ⭐E R 共 丢 兲 ⫺E R 共 兲 ⭐E R 共 兲 . 共35兲 共36兲 That is, the relative entropy of entanglement is an upper bound for the entanglement assisted distillable entanglement as well. VI. IMPROVING THE RATES FOR ISOTROPIC STATES d ⫽ 兺 兩 l 典具 l兩 l⫽1 is evidently a separable state, which is said to be maximally correlated. We will denote this state by sep in the following. An upper bound to the distillable entanglement is given by the relative entropy of entanglement 关4,22兴, which is defined by where P k i l i is a maximally entangled state acting on Cd ⬘ d⬘ d 1 冑d d⫺1 兺 r⫽0 e (2 i/d)rl 兩 rr 典 . 共29兲 The set of these states forms a simplex in Rd⫺1 and has the property that every state except for the barycenter, for which l ⫽1/d, is entangled. To see this, note first that maxl兵l其 is the fully entangled fraction. That is, if not all l are equal, then the fully entangled fraction is larger than 1/d and the corresponding state is thus entangled. On the other hand, if l ⫽1/d, then For a general Bell-diagonal state the protocols introduced are not optimal. In particular, for states with a large entropy the rate is poor or even zero. In order to improve this, one can make use of hybrid protocols, where the first step decreases the entropy while conserving most of the entanglement, and in a second step the hashing/breeding protocol is applied. There are many ways of performing such an entropy decreasing preprocessing. We will in the following discuss two of them for the case of isotropic states: the recurrence method which is well known for qubits 关2,3,13兴 and has already been investigated in 关14,15兴 for d⬎2, and the projection onto local subspaces. For the latter we will show that in the limit of large dimensions the rate approaches the relative entropy of entanglement. Hence, the achieved rate is optimal in that limit. Isotropic states, for which we will discuss both methods in more detail, have the form 012303-6 PHYSICAL REVIEW A 67, 012303 共2003兲 EFFICIENT DISTILLATION BEYOND QUBITS ⫽ f 兩 ⍀ 典具 ⍀ 兩 ⫹ 1⫺ f d 2 ⫺1 共 1⫺ 兩 ⍀ 典具 ⍀ 兩 兲 . 共37兲 That is, they are depolarized maximally entangled states depending on a single fidelity parameter f 苸 关 0,1兴 . The twirl operation mapping every state onto an isotropic state has the form 哫 兰 dU(U 丢 Ū) (U 丢 Ū) * , i.e., it is an averaging over the unitary group U(d) with respect to the Haar measure dU. The states in Eq. 共37兲 are entangled 共and distillable兲 if and only if f ⬎1/d 关14兴. A. The recurrence method The recurrence method for higher dimensions and variations thereof has already been discussed in detail in 关14兴 and 关15兴. For completeness, however, we will recall the main steps. The idea is to apply a BCS operation on two copies of the state and then to measure the target state in the computational basis. The source states are kept whenever the measurement outcomes coincide, otherwise they are discarded. The remaining states may then be twirled onto isotropic states again and we can proceed by either iterating the recurrence method or applying the hashing/breeding procedure if the entropy of the remaining states is already sufficiently small, i.e., S( )⬍log2d. We note that, as already mentioned in 关13兴 for d⫽2, the isotropic twirling after each step is not really necessary and in general increases the entropy and therefore decreases the rate of a subsequently applied breeding/hashing protocol. However, it is sufficient to look at the fidelity parameter f in order to see that a recurrence preprocessing improves the rates such that every entangled isotropic state becomes distillable. Straightforward calculation shows that the fidelity f ⬘ after applying the recurrence method once is given by f ⬘⫽ 1⫹ f 关 d f 共 d 2 ⫹d⫺1 兲 ⫺2 兴 d 3 f 2 ⫺2d f ⫹d 2 ⫹d⫺1 , 共38兲 and the probability for equal measurement outcomes is p rec⫽ d 3 f 2 ⫺2d f ⫹d 2 ⫹d⫺1 共 d⫹1 兲 d 共 d⫺1 兲 2 . FIG. 1. Normalized rates for isotropic states of dimension d ⫽7. The upper bound 共thick兲 is given by the relative entropy of entanglement. The hashing rate 共solid兲 can be improved in the region S( )⬃log2d if one first applies one round of the recurrence method 共dotted兲 or locally projects the state onto subspaces of dimension 3 and 4 共dashed兲. In Fig. 1 we have applied the method as described above to an isotropic state of dimension d⫽7. As expected this leads to an improvement of the rate in the region where S( )⬃log2d. B. Projecting onto local subspaces A surprisingly efficient method for improving the distillation rate is to project the initial state locally onto blocks of smaller dimensions and to apply the hashing/breeding protocol to these subspaces. Let 兵 Q i ⫽ 兺 k 兩 k 典具 k 兩 其 be a set of b projectors of dimension q i corresponding to a local projective observable with b outb b q i ⫽d and 兺 i⫽1 Q i ⫽1d . Assume further comes, i.e., 兺 i⫽1 that Alice and Bob have the same observable 兵 Q Ai 其 ⫽ 兵 Q Bi 其 and that they apply the corresponding measurement to an isotropic state . Again the state is kept if the results of the measurements coincide and discarded otherwise. If both parties obtain the same measurement outcome i, which happens with a probability p i⫽ 共39兲 Note that the recurrence method alone does not lead to a nonzero rate since in every round we destroy or discard at least half of the resources 共all the target states兲 and maximally entangled states are obtained only in the limit of infinitely many rounds. However, it holds that f ⬘ ⬎ f and therefore S( ⬘ )⬍S( ) for every entangled isotropic . This means that every entangled isotropic state can be distilled with a nonzero rate by applying sufficiently many rounds of the recurrence protocol followed by hashing/breeding. There are many directions in which the recurrence method can be modified or improved. One could use more than one source state 关16兴, a different bilateral operation 关15兴, neglect the isotropic twirling 关13兴, apply it to other kinds of states 关15兴, or use target and source states with different fidelities. 冉 冊 qi qi 共 1⫺ f 兲 f⫹ 2 q 2i ⫺ , d d 共 d ⫺1 兲 共40兲 the state after the measurement i ⫽(Q Ai 丢 Q Bi ) (Q Ai B 丢 Q i ) * /p i is again an isotropic state on Cq i 丢 Cq i with fidelity 冋 f i⫽ f 冉 冊册 qi qi 共 1⫺ f 兲 1⫺ ⫹ 2 d 共 d ⫺1 兲 d /p i . 共41兲 If we now apply the hashing/breeding protocol to the b blocks, the rate obtained, b 兺 i⫽1 p i max关 0,log2 q i ⫺H 共 i 兲兴 , 共42兲 exceeds log2d⫺H() for some values of f depending on the dimensions 兵 q i 其 of the subspaces. If the dimensions of the 012303-7 PHYSICAL REVIEW A 67, 012303 共2003兲 KARL GERD H.VOLLBRECHT AND MICHAEL M. WOLF Assume that d⫽2 m , i.e., a single state consists of m pairs of qubits, and let the local measurements have m outcomes corresponding to subspaces of equal dimensions q i ⫽2 m /m. We can then estimate the probability of success and the achieved fidelity 关for m⭓(1⫺ f ) ⫺1 ] by FIG. 2. Normalized rates for the case where consists of ten pairs of qubit systems (d⫽2 10) and the overall state is isotropic. The upper bound 共thick兲 is given by the relative entropy of entanglement. The hashing rate 共solid兲 can be significantly improved when projecting onto subspaces of dimension 2 m , m⫽1, . . . ,9. The dashed line is the envelope of the rates obtained in this way. The dotted curve is the rate one would achieve when considering as a set of ten pairs of qubits, twirling onto isotropic states on C2 丢 C2 , and applying the hashing protocol then on the two-qubit level. blocks are about the same, then an increasing number of blocks leads to a larger 共smaller兲 rate for small 共large兲 f. Figures 1 and 2 show the rates obtained for d⫽7 and for the case where the two parties share 10 pairs of qubits and the overall state is isotropic. For the latter case the rate is already not too far below the relative entropy of entanglement. In fact, the content of the following subsection is to sketch that in the limit of large dimensions d→⬁ the relative distance between these quantities vanishes for all f. C. The limit of large dimensions As we have already mentioned, an upper bound for the distillable entanglement is the relative entropy of entanglement, i.e., the minimal distance between and a separable state measured in terms of the relative entropy S 共 , 兲 ⫽tr关 log2 兴 ⫺tr关 log2 兴 . 共43兲 For entangled isotropic states the nearest separable state is the isotropic state with f ⫽1/d 关21,28,29兴 and the relative entropy of entanglement is thus E R 共 兲 ⫽log2 d⫺ 共 1⫺ f 兲 log2 共 d⫺1 兲 ⫺S 共 f ,1⫺ f 兲 共44兲 for f ⬎1/d and zero otherwise, where S is again the Shannon entropy. Note that in the limit of large dimensions this becomes after normalization E R共 兲 ⫽f. d→⬁ log2 d lim 共45兲 The same limit, however, appears for the distillation rate obtained with the block projection method described in the previous subsection. p i ⭓ p̃ª f ⫺4 ⫺m , m 共46兲 f i ⭓ f̃ ª fm . f m⫹1 共47兲 In the limit of large m, the Eqs. 共46兲 and 共47兲 tell us that we gain m 共almost兲 maximally entangled states of dimension q ⫽2 m /m with probability f /m. Looking at the normalized entanglement as in Eq. 共45兲 leads then indeed to the same limit as for the relative entropy of entanglement. Hence, we 共relatively兲 approach the distillable entanglement in the limit of large dimensions. However, the main reason for this is that the relative entanglement difference of two maximally entangled states in dimensions 2 m /m and 2 m vanishes for m →⬁. Hence, the result is not as deep as it might seem at first glance. Nevertheless, projecting onto blocks of lower dimensions can significantly improve the rates already for finite dimensions as shown in Figs. 1 and 2. VII. CONCLUSION Despite considerable efforts in the theory of entanglement distillation, this field of investigation provides many open questions even on a very basic level. Due to the complexity of the underlying variational problem it is hard to find good upper and lower bounds to the distillable entanglement, not to mention an explicit calculation of this measure of ‘‘useful entanglement.’’ So far, the most important distillation protocol leading to a nonzero rate, and thus to a nontrivial lower bound to the distillable entanglement, has been adapted to Bell-diagonal states of two qubits. Of course, this protocol can also be applied to higher dimensional states either by projecting down to qubits or by interpreting the state as a tensor product of qubits if possible 共compare Fig. 2兲. However, both methods will in general discard most of the entanglement. The present article shows how to generalize the breeding and hashing protocols to higher dimensions. The rates obtained are optimal only for special cases; however, they provide an improved lower bound to the distillable entanglement in general. Both protocols consist of two steps: first the quantum task is translated to a classical problem and then the latter is solved. The classical part of the protocol is already essentially optimal; however, some information and hence entanglement is lost during the ‘‘translation process.’’ We think that the presented results admit further generali 012303-8 PHYSICAL REVIEW A 67, 012303 共2003兲 EFFICIENT DISTILLATION BEYOND QUBITS ACKNOWLEDGMENTS zations toward other classes of states and maybe also with respect to the restriction of the hashing protocols to dimensions that are 共powers of兲 primes. We hope that our work initiates further investigations concerning the distillation of entanglement, including explora tions of the implications from recent work in the field of quantum error correcting codes. The authors would like to thank R. F. Werner, H. Barnum, and D. Schlingemann for valuable discussions. Funding by the European Union project EQUIP 共Contract No. IST-199911053兲 and financial support from the DFG 共Bonn兲 are gratefully acknowledged. 关1兴 G. Alber et al., Quantum Information, Springer Tracts in Modern Physics Vol. 173 共Springer, Berlin, 2001兲. 关2兴 C.H. Bennett, G. Brassard, S. Popescu, B. Schumacher, J. Smolin, and W.K. Wootters, Phys. Rev. Lett. 76, 722 共1996兲. 关3兴 C.H. Bennett, D.P. DiVincenzo, J.A. Smolin, and W.K. Wootters, Phys. Rev. A 54, 3824 共1996兲. 关4兴 E. Rains, e-print quant-ph/9707002. 关5兴 M. Horodecki, P. Horodecki, and R. Horodecki, Phys. Rev. Lett. 80, 5239 共1998兲. 关6兴 M. Horodecki, P. Horodecki, and R. Horodecki, Phys. Rev. Lett. 78, 574 共1997兲. 关7兴 W. 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