Supercond. Sci. Technol. 11 (1998) 1181–1185. Printed in the UK PII: S0953-2048(98)93386-3 The range of giant flux instabilities in the H –T plane in hard superconductors: calculations and experiment V V Chabanenko†, A I D’yachenko†, A V Chabanenko†, M V Zalutsky†, H Szymczak‡, S Piechota‡ and A Nabialek‡ † Physico-Technical Institute, National Academy of Sciences, ul. R. Luxembourg 72, 340114 Donetsk, Ukraine ‡ Institute of Physics, Polish Academy of Science, Al. Lotnikow 32/46, 02-668 Warsaw, Poland Received 2 February 1998 Abstract. We have studied magnetothermal instabilities, giant flux jumps, both theoretically and experimentally. Magnetostriction and magnetization hysteresis loops with flux jumps were calculated over a wide range of experimental parameters employing two critical-state models: the Kim–Anderson model and the exponential model. The influence of the magnetic history on the flux jumps’ magnetostriction and magnetization were investigated for the LaSrCuO single crystal. The shape of the unstable region of the critical state in the temperature–magnetic field plane was constructed from calculations and experimental results. In the Kim–Anderson model H –T diagrams of flux instabilities agree well with experimental results on HTSC single-crystal LaSrCuO and experimental results on LTSC niobium. 1. Introduction When the magnetic field H is ramping, the appearance of a small increase of the temperature leads to a decrease of the value of the critical current density of the hard type II superconductors. In adiabatic conditions this increases dissipation and can lead to ‘thermomagnetic catastrophe’. As a result, giant flux jumps appear and the sample goes to the resistive or normal state. The investigation of flux instabilities in HTSCs is interesting because of the potential applications as well as the importance of gaining a fundamental understanding of the phenomenon. We have studied magnetothermal instabilities both theoretically and experimentally in LaSrCuO. There are a lot of papers devoted to giant flux jumps attributed to the avalanche effect in the flux movement. For our main aim, the build-up of diagrams of the instability range (or flux jump range) of the critical state of type II superconductors (SCs) in the temperature–magnetic field plane and comparison of them with the experimental data, three papers proved to be of importance [1–3]. In [1] Kim–Anderson model analytical expressions for flux jumps in magnetization are given. Another paper [2] is devoted to computation of field dependences of magnetostriction of SCs, but without consideration of flux jumps. The present paper on the basis of a combination c 1998 IOP Publishing Ltd 0953-2048/98/101181+05$19.50 of these approaches to the problem gives the computation of both magnetization M(H ) and magnetostriction 1L(H ) loops with flux jumps. We apply the same criterion of instability as in [1]; however, for our calculations we used numerical computation of the magnetic properties of type II SCs. The algorithm used by us makes it possible to derive these for any analytical dependences of critical current versus magnetic field. In particular we select two very widespread types of j (H ) dependences, the socalled Kim–Anderson model and the exponential model (according to [2] the exponential model is most favourable for describing the measured magnetostriction curves). The analysis of the width of the region of the magnetic fields where the critical state of SCs is unstable, carried out for different temperatures, allowed us to derive calculated H –T diagrams for flux jumps. In the Kim–Anderson model the shape of the unstable region of the critical state in the temperature–magnetic field plane agrees well with our experimental results on HTSC single-crystal LaSrCuO and experimental results [3] on LTSC niobium. 2. H –T diagram of flux instabilities: theory and experiment The influence of the magnetic history on the flux jumps was investigated in the LaSrCuO crystal. Magnetostriction 1181 V V Chabanenko et al and magnetization hysteresis loops with flux jumps were calculated employing two critical-state models: the Kim– Anderson model and the exponential model. 2.1. Critical state Let us consider the pinning-induced magnetization and magnetostriction loops with flux jumps for a specimen having a slab geometry with thickness of L = 2d (−d ≤ x ≤ d). Suppose that the external magnetic field He is applied parallel to the slab face. The magnetic field profile H (x) inside the slab is given by the solutions of the critical state equation dB/dx = −µ0 J (x) (1) where current density |J (x)| ≤ |Jc (x)| and µ0 is the permeability of vacuum. This critical-state equation can be used to determine the magnetization and the magnetostriction when H Hc1 (for YBCO the lower critical field H is of the order of several hundred gauss at T = 0 while the flux jumps are observed at fields µ0 H of the order of several tesla). According to the Kim–Anderson model [4] Jc (B) = ±J0 (T )B0 /(B0 + |B|). (2) Here B0 is a phenomenological parameter and J0 is the critical current density at zero magnetic field B; in HTS materials J0 (T ) ≈ J0 (0)(1 − T /Tc ). Integration of equations (1) and (2) gives B± (x) = B0 − [(B0 − B ∗ )2 ± 2µ0 J0 (x − x ∗ )B0 ]1/2 B(x) < 0 B± (x) = −B0 + [(B0 + B ∗ )2 ± 2µ0 J0 (x − x ∗ )B0 ]1/2 B(x) > 0. (3) The +(−) sign corresponds to domains of vortices where dB/dx > 0 (dB/dx < 0) and the field B ∗ = B(x ∗ ). In the exponential model [5] the critical current density is expressed as follows: Jc (B) = ±J0 exp(−B/B0 ). (4) The sign indicates the flow direction of the current. Integration of equations (1) and (4) provides the local field distribution: B± (x) = B0 ln[exp(B ∗ /B0 ) ± µ0 J0 (x − x ∗ )/B0 ] B(x) > 0 B± (x) = −B0 ln[exp(−B ∗ /B0 ) ± µ0 J0 (x − x ∗ )/B0 ] B(x) < 0. (5) Here the +(−) sign again corresponds to the local field distribution where dB/dx > 0 (dB/dx < 0) and the boundary field B ∗ = B(x ∗ ). The full magnetic field profile in the sample is given by the combination of solutions (3) or (5). The parameters x ∗ and B ∗ are chosen so that the condition µ0 He = B(x = 0) holds and the field B(x) distribution is continuous. The corresponding formulae for x ∗ in the Kim–Anderson model are given in [1]. For the exponential model as well as for any form of j (H ) when the number of jumps becomes very large the use of analytical expressions for x ∗ is not very sensible. 1182 Figure 1. Magnetization and magnetostriction loops with flux jumps; calculation in the Kim–Anderson model. Comparison of the solutions (3) and (5) shows that they are close to each other if B ∗ /B0 1. From the four solutions (3) and (5), all the necessary magnetic field profiles can be constructed [1, 2]. When the value of the magnetic field B(x) is known, the magnetization M and magnetostriction 1L/L0 can be calculated by simple integration: Z d 1L(B)/L0 = −1/(µ0 EL0 ) [Be2 − B 2 (x)] dx (6) 0 Z M(B) = 1/(µ0 d) d B(x) dx − He . (7) 0 Here E is the elastic constant of the material along the x axis and L = 2d. Flux instabilities in hard superconductors Figure 3. Magnetization loops (calculation) which illustrate the influence of the maximal temperature T ∗ reached by the sample during flux jump; T1∗ > T2∗ . |He |). Because of the moving of flux lines, the magnetic field, B(x), in the sample increases by 1B(x). The 1B(x) value has to be calculated from equation (1) in following way. Let xi be the points at which the B(xi ) = Bi values are calculated with the index l ≤ i ≤ n, xl = 0, xn = d and 0 − Bi , B 0 (x) as the initial local field. We put 1B = Bi+1 where i > 1, Bi = B(x = 0) = µ0 He . The critical-state equation (1) gives the conditions: |1B| < µ0 Jc (Bi ) B(xi ) + 1B (8) B(xi+1 ) = B(xi ) + sign(1B)µ0 Jc (Bi ) dx |1B| > µ0 Jc (Bi ) Figure 2. H –T ranges of the flux instability: (a ) experiment on LaSrCuO; (b ) calculation (d = 5 mm, jc = 109 A m−2 , B0 = 2 T; Bp , full penetration field); (c ) experiment [8] on Nb. where dx = xi+1 − xi . Because of exchange with the magnetic field, B(x), the energy per unit volume Q is dissipated in the vicinity of x where Z d [B(x 0 ) − B 0 (x 0 )] dx 0 . (9) Q(x) = Jc (x) x Under local adiabatic conditions one obtains 1T (x) = Q(x)/CV 2.2. Algorithm for numerical calculation of magnetization and magnetostriction loops with flux jumps, instability criterion The instability criterion (under adiabatic conditions) in the case of the Kim–Anderson type of critical current density Jc (B) can be derived analytically [1]. For the exponential model (4) this is not possible and we have used in this case the calculations based on the adiabatic flux–B jump instability criterion. Let the applied field He increase (decrease) by a small amount 1He (|1He | (10) where CV is the specific heat of the superconductor. For YBCO [6], CV (1–26 K) (J cm−3 ) = 2.68 × 10−4 T −2 + 1.01 × 10−4 T + 2.53 × 10−6 T 3 + 7.17 × 10−9 T 5 and CV (26–100 K) (J cm−3 ) = 2.02 × 10−4 T 2 − 7.82 × 10−9 T 4 . The increase of temperature 1T reduces the critical current Jc : 1Jc (x) = (∂Jc /∂T )1T (x). (11) According to the critical-state equations (8), the reduction in Jc leads to a decrease in the shielding ability of the 1183 V V Chabanenko et al conditions of the sample. The critical state conditions (8) for type II SCs allow one to calculate magnetic field profiles in a slab and for any totality of the flux jumps, independently of the magnetic history. 2.3. Results of calculation and comparison with experiment Figure 4. Magnetostriction loops for different temperatures, LaSrCuO. superconductor by 1HS , where Z d 1HS = − 1Jc (x 0 ) dx 0 . (12) x The magnetic configuration is unstable with respect to a flux jump if 1HS > He [7, 8]. During a flux jump, the temperature inside the sample increases and reaches a maximum value T ∗ < Tc , which is assumed to be independent of the position x inside the sample. The critical current density at T ∗ is Jc (T ∗ ) < Jc (T0 ), where T0 is the temperature of the sample before the flux jump. Therefore, according to the critical-state conditions, the magnetic field configuration is given by the solution of the equations (8) for Jc = Jc (T ∗ ). After the flux jump the temperature inside the sample is returned to the starting value T0 , but the magnetic field profiles in the slab are unchanged, i.e. they are the same as for T = T ∗ . An increase (decrease) of the external field, He , leads to the new magnetic field distributions. It is assumed that the maximum temperature, T ∗ , reached during a jump, which is less than Tc , is the same for all jumps. Generally speaking the T ∗ value is unknown because it depends on microstructure of the sample, sweep rate and the adiabatic 1184 These results and data [1, 2] are used for computer simulations. Magnetostriction and magnetization loops are constructed over a wide range of experimental parameters. In figure 1, one can see an example of theoretically calculated magnetostriction and magnetization hysteresis loops with magnetostriction and magnetization jumps on the basis of the Kim–Anderson model. 1Hfj is the flux instability range of the magnetic field. Similar calculations were performed for different temperatures and were used for the construction of the H –T phase diagram of flux instability (figure 2(b)). The calculations done make it possible to follow the change in the pattern of flux jumps (figure 3) when varying the maximal temperature T ∗ reached by the sample during a jump (or when varying the final depth of flux penetration into the sample). During the experiment a similar result can be, for example, reached by changing the velocity of heat removal from sample surface. However, it is rather difficult to control this parameter in the experiment. Experiments reported here have been performed on an La1.85 Sr0.15 CuO4 single crystal with the fields oriented along the c-axis. The sample had dimensions of 2.15 × 2.24 × 5.42 mm3 , with the c-axis the shortest test axis. The change of length 1L of the sample was measured in the a–b-plane along the longest dimension, using a strain gauge technique. The resistance change of strain gauges was measured by an AC bridge. The magnetic field was swept at a constant cyclic rate of 0.5 T min−1 after the sample was zero-field cooled to the measuring temperature. An onset temperature for superconductivity of 35.5 K was observed in a field of 10 G. Figure 4 shows the manifestation of flux jump instabilities in the virgin magnetization curve for LaSrCuO single crystal. Hirr is the field where M becomes reversible. As can be seen from figures 2(a) and 2(c), the overall pictures of the H –T ranges of flux instability are similar in shape for Nb [3] and LaSrCuO. One can also see a good qualitative agreement between the experimental and the calculated phase diagrams. This shows that the Kim–Anderson model is applicable at large distances away from the irreversibility line for HTSC materials whereas the exponential model is applicable in the vicinity of the irreversibility line. As is clear from both calculation and experiment, the first and third quadrants have significantly fewer flux jumps than the second and fourth quadrants. For example, for the T = 4 K curve (figure 1(a)) and experiment [9], flux jumps are completely absent in the first and third quadrants. According to our calculation, the difference in the frequency of occurrence of the flux jumps in the different quadrants is related to the shape of the flux profiles in the various quadrants. Flux instabilities in hard superconductors References [1] Muller K-H and Andrikidis C 1994 Phys. Rev. B 49 1294 [2] Ikuta H, Kishio K and Kitazawa K 1994 J. Appl. 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