VOLUME 80, NUMBER 11 PHYSICAL REVIEW LETTERS 16 MARCH 1998 Corrugation Flux Front Instability in Type-II Superconductors F. Bass, B. Ya. Shapiro, and M. Shvartser Institute of Superconductivity, Department of Physics, Bar-Ilan University, Ramat Gan 52900, Israel (Received 16 June 1997) The dynamics of vortex flux entering a superconductor containing immovable flux of the opposite sign (antivortices) is considered. We obtain a solution for a flat moving interface separating the positive and negative flux areas. When the velocity of the positive flux exceeds some critical value, a corrugation instability of the interface develops. [S0031-9007(98)05548-3] PACS numbers: 74.60.Ge The study of magnetic flux penetration into type-II superconducting samples has attracted the attention of many research groups [1]. This interest is motivated by the fact that this phenomenon can be viewed as a prototype of a general class of macroscopic nonlinear dynamic phenomena, as well as by its importance for applications. Traditionally, the magnetic front between the magnetic flux state and the Meissner superconducting state has been considered to be a flat plane [2]. However, recent magneto-optical experiments [3–6] demonstrate that nonuniform flux penetration occurs, in particular, upon exposing a previously magnetized sample to a weak magnetic field of the opposite sign. While at low temperatures, and flux (aligned along the new field) gradually enters the sample and the flux boundary remains flat; the situation changes dramatically at higher temperatures. In particular, in a YBa2 Cu3 O7 bulk superconductor, at temperatures above 47 K, the boundary between the distinct flux areas is strongly perturbed and a magnetic field, of magnitude 120 G, penetrates the sample through a sudden nucleation of magnetic domains [3–5]. This instability exists only in a relatively narrow temperature “window” and has not been observed above 80 K. In superconducting Nb, the structure and growth of the magnetic domain appear similar to that seen for a viscousfingering growth phenomena in solid-liquid systems [7]. The temperature window for the instability in this sample stretches at least from 3 to 7 K [6]. In this paper we report on flux-antiflux dynamics in type-H superconductors. In particular, we find a solution for a flat moving interface separating positive and negative flux areas in a superconductor. We predict that this interface becomes unstable when the flux velocity exceeds some critical value due to the “overheating” of the interface caused by vortex-antivortex annihilation. The growth of the instability gives rise to a nonlinear pattern whose nature remains to be determined. Let us consider the situation when vortex flux enters a sample containing immovable flux of the opposite sign (antivortices). We start with a model of a two-component vortex gas [8] spatially homogeneous along the z-axis, which is valid for the experimentally interesting situation of low magnetic fields. Here, the typical spacing between 0031-9007y98y80(11)y2441(4)$15.00 vortices a0 greatly exceeds the vortex-vortex (or vortexantivortex) interaction radius j. The vortex-vortex repulsion, since it conserves the number of vortices, does not play a significant role, and will be ignored. In this approximation, the vortex-antivortex dynamics obeys the well-known equations of recombination theory [8,9] n1 n2 ≠n1 ! yd 1 1 = ? sn1 ! ­ 0, (1) ≠t t n1 n2 ≠n2 1 ­ 0, (2) ≠t t where n1 and n2 are the vortex and antivortex densities, respectively; t 21 ­ yj is the recombination rate; j is the annihilation cross-section, which is of the order of the co! is the vortex herence length of the superconductor; and y ! velocity. In the creep regime, y is strongly temperature dependent ! ! ­y (3) y FF exps2UyT d , ! where U is the pinning potential; and y FF is the flux velocity in the flux-flow regime. The set of Eqs. (1) and (2) must be completed by the heat transfer equation in the form: dQ ≠T (4) ­ k=2 T 1 2 gsT 2 T0 d , ≠t dt where dQ n1 n2 (5) ­ Q0 dt cp t is determined by the energy released by vortex-antivortex annihilation. Here k is the heat coefficient, cp is the heat capacity, T0 is the sample temperature in the absence of flux motion, Q0 ­ f0 Hc1 y2p is the heat released by annihilation of a single vortex-antivortex pair, Hc1 is the lower critical field, f0 is unit flux, and g 21 ­ tR is the characteristic time of temperature relaxation. The set of Eqs. [(1)–(4)] completed by the boundary conditions describes all features of the model. This hydrodynamical approach is correct if we consider variations on a scale much larger when a0 . We start from the plane flux front dynamics when all of the functions described by Eqs. [(1)–(4)] depend © 1998 The American Physical Society 2441 VOLUME 80, NUMBER 11 PHYSICAL REVIEW LETTERS only on the spatial coordinate parallel to the flux-front propagation. In this case the problem becomes one dimensional, as described by the set of equations: n1 n2 ≠n1 ≠ 1 sn1 yd 1 ­ 0; ≠t ≠x t (6) n1 n2 ≠n2 1 ­ 0, ≠t t (7) ≠2 T ≠T n1 n2 ­k 2 1 Q0 2 gsT 2 T0 d , ≠t ≠x cp t (8) and the boundary conditions n1 sx ! 2`d ­ n2 sx ! `d ­ n0 . Working to the leading order in the small parameter dTyT0 , where dT is the temperature growth caused by the vortex-antivortex annihilations during the effective heating time (which cannot exceed the relaxation time tR ), we immediately obtain from Eq. (8) that T ­ T0 . The maximal shift of the temperature dT may be estimated as dT . Q0 n0 tR ytA cp where tA ­ t0 yn0 is the vortexantivortex annihilation time. In this approximation, and neglecting magnetic screening effect, the pair of nonlinear equations (6) and (7) may be solved exactly. In particular, substituting for n2 from Eq. (7) in Eq. (6) and introducing a new variable Z t t 21 n1 sx, t 0 d dt 0 ­ usx, td , (9) z ­x2 n1 sz d ­ n0 1 ; 1 1 exps2n0 z yy0 td n2 sz d ­ n0 exps2n0 z yy0 td , 1 1 exps2n0 z yy0 td n2 sz , y, td ­ n2 sz d 1 Qsz , y, td; T ­ T0 sz d 1 D µ ∂ Dsz , y, td ; y ­ y0 1 1 T0 µ ∂ Dsz , y, td 21 21 t ­ t0 1 1 . T0 (10) (11) y0 ; ysT0 d . (13) (14) Here we neglect the influence of temperature fluctuations on the heat capacity cp and on the relaxation coefficient g, as this does not affect the physical picture. (We implied that U ­ T0 .) Substituting these relations in the initial set of Eqs. (1), (2), (4) we obtain after linearization the following set of equations for the deviations: ∂ µ 2 ≠2 D ≠D y0 ≠D ≠ D 1 2 gD 2 ­k ≠t 2 ≠z ≠y 2 ≠z 2 1 Q0 (12) n1 sz , y, td ­ n1 sz d 1 Csz , y, td; one can transform the pair of equations (6) and (7) to the following single equation: Performing an integration over time and solving the equation obtained by the method of characteristics, we obtain the traveling interface solution: y0 t 2 It is interesting to note that the vortex-antivortex interface moves into the antivortex-filled domain with the velocity y0 y2, the average of the velocity y0 of the moving vortices and the zero velocity of the antivortices. The spatial distributions of vortex and antivortex flux densities overlap, forming an interface region where the vortices of opposite signs coexist. The scale of characteristic width of this region DL may be estimated from Eqs. (11) and (12) as DL . ytyn0 , sn0 jd21 , a02 yj. This is much larger than the intervortex distance a0 , so that there is a macroscopically large area in which the total magnetic induction B ­ f0 sn2 2 n1 d ­ n0 f0 tanhsn0 z yy0 td is suppressed. The vortex velocity sy ~ ,Bd approaches a constant at the interface point where B ! 0, justifying our considerations. In particular, this implies that our solution is valid in the interface region even in the presence of magnetic screening [10]. Let us consider the stability of this vortex-antivortex interface with respect to small deviations from its initial plane shape. In this case one can look for solutions of Eqs. (1), (2), (4) in the form 2` ≠2 u ≠2 u n0 ≠ exps2ud 1 y 2 ­ 0. ≠t 2 ≠x≠t t ≠t 16 MARCH 1998 fn 1 sz dQ 1 n2 sz dC 1 n1 sz dn2 sz d sDyT0dg , t0 cp (15) (16) µ ∂ ≠C ≠D ≠D ≠C y0 ≠C n1 sz d fn 1 sz dQ 1 n2 sz dC 2 n1 sz dn2 sz d sDyT0 dg ­ 0, y0 1 1 1 y1 1 y1 1 ≠t 2 ≠z T0 ≠z ≠y ≠y t0 (17) y0 ≠Q fn1 sz dQ 1 n2 sz dC 1 n1 sz dn2 sz d sDyT0 dg ≠Q ­ 0, 2 1 ≠t 2 ≠z t0 2442 (18) VOLUME 80, NUMBER 11 PHYSICAL REVIEW LETTERS ! where we assume that the vortex velocity y also possesses a component parallel to the interface yy sT d, where yy ø y1 f1 1 Dsz , y, tdyT0 g, and y1 ø y0 . It is evident that all of the preparations far from the flux-antiflux interface cannot result in a front instability. Therefore, one can assume that these perturbations must be localized on the boundary. Looking for a solution in the form 0 1 0 1 C Csz , y, t B C B C @ Qsz , y, td A ­ expsvt 1 iky y 2 az 2 y2d @ Q A , D Dsz , y, td (19) we obtain from Eqs. [(15)–(18)] after integration on z a set of equations, and the requirement for the selfconsistency of these leads to the following equation for the dimensionless growth rate: V ­ vt0 yn0 V 3 1 V 2 fsiq 1 1d 1 Aq2 1 g p 2 P p g 1 ∑ ∏ iq Pp V 1 sAq2 2 P p 1 g p d siq 1 1d 1 iqP p 1 1 2 2 iq (20) sAq2 1 g p d ­ 0 , 2 where q­ ky y1 t0 ; n0 t0 g ­g ; n0 p A­ kn0 ; y12 t0 Q0 n02 P­ . 4t0 T0 cp Pp ­ P t0 ; n0 (21) Representing V in the form V ­ V1 1 iV2 , (22) we obtain for V1 in theplimit of g p ø 1y4A p ø 1sq ! 0d (since tA ytR ø 1 and kytA ¿ y1 ¿ kytR ): ∂ µ 1 Pp 1 2 1 q2 2 q4 . (23) V1 ­ p2 4 2g 16g p2 A positive value of V1 implies an instability, and this occurs if P p . 2g p2 . In dimensional variables [see Eq. (21)] this condition reads s 8T0 cp g 2 y0 $ yc ­ . (24) Q0 n03 j 2 For velocities of the flux exceeding this critical value yc there is a band of unstable wave vectors, and a critical length scale defined by the wave vector qc of the fastest growing mode: ∂ µ p P 2 p2 qc ­ 2g 21 . (25) 2g p2 16 MARCH 1998 In dimensional variables we get sy0 $ yc d y1 tR lc ­ 2pykc . q ¿ a0 . 2 fy0 yyc2 2 1g (26) This is just the condition that we need in order to justify using the hydrodynamical approach. Thus, the dynamics of a type-II superconductor, containing vortex flux moving through immovable flux of the opposite sign (anitvortices), strongly depends on the vortex velocity and on the temperature, which may be considered to be the main control parameter of the problem. This dynamics possesses the following most important properties: (1) For a sufficiently small velocity of the vortices on the interface y , yc the flux-antiflux interface propagates with velocity yy2. This fact has an evident physical explanation. Indeed, in the frame moving with velocity yy2, vortices possess velocity yy2, while antivortices have velocity 2yy2 and the flux-antiflux interface is stationary. (2) The characteristic width of the vortex-antivortex coexistence region DL may be macroscopically large DL , a02 yj ¿ a0 , where a0 and j are the intervortex distance and linear cross sections of the vortex-antivortex annihilation, respectively. (3) If the vortex flux velocity exceeds its critical value y0 . yc , then the flux-antiflux interface exhibits an instability. This instability is caused by the vortex-antivortex overheating exceeding the thermal absorption in the sample. This type of instability is well known in plasma physics as the “overheating instability” [11,12]. The critical velocity of this instability, determined by Eq. (24), may be simply obtained in the following manner. The temperature increase during the time tA of a single annihilation event may be estimated as Q0 n0 ycp tA [see Eq. (6)], which must be multiplied by the number dN of the unit events during the heat relaxation time tR , dN , tR ytA . The relaxation caused by the sample lattice is the competing process in the system. The temperature relaxation for time tR may be estimated as T0 ytR . It is evident that the overheating instability arises under the condition DQ tR Q0 n0 T0 ; 2 . 0, tR tA cp tA tR tR ­ g 21 ; tA ­ sn0 yo jd21 , (27) (28) which is equivalent to the criterion defined by Eq. (24). (4) The most rapidly growing mode of instability occurs at wavelength lc . It seems reasonable to guess that patterns emerging from this instability will, at least initially, have a characteristic size of order lc ¿ a0 in which case lc may be macroscopically large. (5) The growth rate of the corrugation instability V1 sqd shows that in the domain of instability the growing modes develop for a wide range of wave vectors. The wave length lm at which V1 vanishes, sets a length scale 2443 VOLUME 80, NUMBER 11 PHYSICAL REVIEW LETTERS FIG. 1. The ratio y0 yyc vs temperature for Nb for which Tc ­ 9 K. A corrugation instability arises only in a comparatively narrow temperature “window” of width DTW determined by the inequality y0 sT0 d . yc sT0 d. for the problem. The set of Eqs. [(23)–(25)] tells us p that lc ­ 2lm , and the minimal wavelength of the instability has the same order as the rapidly growing mode lc . The existence of this length has a very clear physical explanation. It appears as a balance between the excess heat cp DQlm released in the fluctuation region of the size of the order of lm for the time t $ tR and the heat flow sy carried by the vortices and directed along the interface, bringing this heat out from this hot domain due to the temperature gradient. The balance relation gives the condition of instability DQlm . sy1 tR d2 T0 ylm ; sy ­ 2cp sy12 tR d=y T , (29) y12 tR is the diffusion coefficient of the vortices and sliding along the interface and transmitting heat to the lattice. On substituting DQ from Eq. (27) in Eq. (29) we immediately obtain for lm the result of the linear theory of instabilities defined by Eq. (26). (6) The instability appears only in a relatively narrow temperature window determined by the inequality y0 . yc sT0 d. For instance, for an Nb sample with the following parameters: the Fermi energy eF ­ 3 3 104 K; the Fermi momentum pF ­ 107 cm21 ; the super- 2444 16 MARCH 1998 conducting gap D0 ­ 13 K; the critical temperature Tc ­ 9 K, the Debye frequency vD ­ 300 K; the vortex viscosity h ­ 1027 dyn secycm2 ; the intervortex distance a0 ­ 1024 cm; the annihilation cross section j ­ 1025 cm; the Fermi velocity yF ­ 107 cmysec; the ratio UyD0 ­ 1.2; the flux velocity in the flux-flow regime yFF ­ 104 cmysec, where yFF , f0 Jc ych; Jc ­ cf0 n02 j ­ 105 Aycm and using for cp and g their dependence in the low temperature region cp ­ NseF dD0 sD0 y T d3y2 exps2D0 yT d, where NseF d is the DOS at Fermi 2 level and g ­ ge-ph ­ T 3 yvD , we conclude from Eqs. (3) and (24) that the temperature window for flux instability is very similar to that observed experimentally [6] in this material, namely DTW ø 4 K, as can be seen from Fig. 1. We would like to thank Dr. M. Bazilevitch for helpful discussions. This work was supported by the Israel Ministry of Sciences and Arts and German-Israel Foundation. We would also like to thank the Bar-Ilan Minerva Center for Superconductivity for permanent support. [1] R. P. Huebner, Magnetic Flux Structures in Superconductors (Springer-Verlag, Berlin, 1979). [2] C. P. Bean, Rev. Mod. Phys. 36, 31 (1964). [3] V. K. Vlasko-Vlasov et al., Physica (Amsterdam) 222, 361 (1994). [4] T. H. Johansen et al., in High Temperature Superconductors: Synthesis, Processing, and Large-Scale Applications, edited by U. Balachandran, P. J. McGinn, and J. S. Abell (The Minerals, Metals & Materials Society, Warrendale, PA, 1996). [5] M R. Koblichka et al., Europhs. Lett. (to be published). [6] C. A. Duran, P. L. Gammel, R. E. Miller, and D. J. Bishop, Phys. Rev. B 52, 75 (1995). [7] J. S. Langer, Rev. Mod. Phys. 52, 1 (1980). [8] V. V. Bryksin and S. N. Dorogovtsev, Sov. Phys. JETP 77, 791 (1993). [9] E. S. Bakhanova et al., Sov. Phys. JETP 73, 1061 (1991). [10] F. 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