Earth and Planetary Science Letters 146 Ž1997. 401–414 Fractal features in mixing of non-Newtonian and Newtonian mantle convection Arkady Ten a a,b , David A. Yuen a,) , Yu.Yu. Podladchikov c , Tine B. Larsen d , Elizaveta Pachepsky a , Andrei V. Malevsky e Department of Geology and Geophysics, Minnesota Supercomputer Institute, UniÕersity of Minnesota, Minneapolis, MN 55415-1227, USA b Institute of Mineralogy and Petrography, Russian Academy of Science, NoÕosibirsk, 630090, Russia c Geologisches Institut, E.T.H., CH-8092, Zurich, Switzerland ¨ d Danish Lithosphere Center, DK-1350 Copenhagen K, Denmark e Departement de Physique et CERCA, UniÕersite´ de Montreal, Montreal, Que. H3X 2H9, Canada Received 4 September 1996; accepted 9 December 1996 Abstract Mixing processes in mantle convection depend on the rheology. We have investigated the dynamical differences for both non-Newtonian and Newtonian rheologies on convective mixing for similar values of the effective Rayleigh number. A high-resolution grid, consisting of up to 1500 = 3000 bi-cubic splines, was employed for integrating the advection partial differential equation, which governs the passive scalar field carried by the convecting velocity. We show that, for similar magnitudes of the averaged velocities and surface heat flux, the local patterns of mixing are quite different for the two rheologies. There is a greater richness in the scales of the spatial heterogeneities of the passive scalar field exhibited by the non-Newtonian flow. We have employed the box-counting technique for determining the temporal evolution of the fractal dimension, D, passive scalar field of the two rheologies. We have explained theoretically the development of different regimes in the plot of N, the number of boxes, covered by a range of colors in the passive scalar field, and S, the grid size used in the box-counting. Mixing takes place in several stages. There is a transition from a fractal type of mixing, characterized by islands and clusters to the complete homogenization stage. The manifestation of this transition depends on the scales of the observation, and the initial heterogeneity and on the rheology. Newtonian mixing is homogenized earlier for long-wavelength observational scales, while a very long time would transpire before this transition would take place for non-Newtonian rheology. These results show that mixing dynamics in the mantle have properties germane to fluid turbulence and self-similar scaling. Keywords: mantle; mixing; convection; fractals; rheology; models 1. Introduction The process of mixing in fluid flows is of fundamental importance in many areas, ranging from in) Corresponding author. E-mail: davey@krissey.msi.umn.edu dustrial and environmental systems to geophysical and astrophysical processes. Mixing problems are still studied case by case. The effects of shear-thinning rheology on mixing have been studied within the context of time-periodic forcing on cylindrical flows w1x for industrial applications. Some significant 0012-821Xr97r$17.00 Copyright q 1997 Elsevier Science B.V. All rights reserved. PII S 0 0 1 2 - 8 2 1 X Ž 9 6 . 0 0 2 4 4 - 0 402 A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 effects were found in the chaotic advection of a passive tracer in the shear-thinning fluids, in which the viscosity decreases with increasing strain rate w2x. Our interests stem from mantle dynamics and here one must consider the mixing phenomenon in the presence of rheological fluid motions driven by thermal convection. We are interested in mixing from a geophysical standpoint, with mantle convection being the centerpiece. Since upper mantle rheology is likely to be non-Newtonian, we may not avoid the issue of mixing in rheological fluids. In spite of the seeming ubiquity of non-Newtonian rheology in the upper mantle, there is a dearth of studies on mixing in non-Newtonian convection. Recent work by us w3x has shown the possibilities for using a very dense grid for mapping out the complex patterns of passive scalar field driven by time-dependent convection. These passive scalar fields exhibit characteristics of turbulent flows at high Reynolds number. We will present the high-resolution results of the evolution of the passive scalar fields and compare the differences between Newtonian and non-Newtonian mixing. The high spatial resolution, well over 10 3 = 10 3 grid points, allows for a close examination of these issues in mixing with fractal analysis. We will present a simple model of mixing based on the evolution of the fractal dimension and utilize the data from the high-resolution passive scalar fields for testing out the model. 2. Mixing by passive scalar field: details of modelling Mixing processes can be monitored by a Lagrangian approach using passive tracers w4–7x from the convective velocity field. The main limitation of the Lagrangian approach is due to its statistical nature, which requires the calculation of many particle trajectories and it is also beset by a global description of the scalar field at large time. We have taken the alternative Eulerian approach of monitoring a passive scalar field by simulating an advection partial differential equation, which allows us to have direct access to the local and global characteristics of the passive scalar field, as well as to information about the gradient of the field. Moreover, one can study by visualization the temporal evolution of this scalar field. We have here neglected the effects of diffusion, which determines the homogenization of the smallest scales of the scalar field. The mixing of a passive scalar field c in the absence of chemical reactions and diffusion is governed by the non-dimensional first-order partial differential equation: Ec Et q U P grad c s 0 Ž 1. where U is a precomputed, time-dependent velocity field taken from a thermal convection calculation. A characteristic-based method w8x with fourth-order spatial and second-order temporal accuracy has been employed for solving the first-order partial differential equation. This solution of c is simply transported along the characteristic curves with the velocity field U w3x. The set of convection equations used to calculate the thermal and velocity fields in a two-dimensional cartesian domain is described elsewhere w9x. They consist of the conservation equations of mass, momentum and energy with the time-dependence present only in the energy equation, because of the infinite Prandtl number nature of the mantle. These solutions were obtained with a similar bi-cubic spline-based method w8x. The flow dynamics are not influenced at all by the passive nature of c , which serves the role of mapping out the structure being advected by the fluid motion. There is no mass flux out of the boundaries because of the impermeable Žvanishing normal velocity. boundary conditions imposed around the box. Reflecting boundary conditions at the vertical edges have been imposed on the horizontal velocity and temperature in the convection simulations w8,9x, as well as a vanishing vertical velocity at the horizontal boundaries. Since the mechanism of mixing produces smallscale features, we have taken the strategy of employing a much denser grid for the scalar c field than for the temperature and velocity field used in the convection simulation. The need for a much denser grid for c is consistent with the physics of passive advection, which is much more chaotic w7x than the convective flow carrying c . The spline functions allow for an accurate interpolation of the velocity field onto a denser grid for integrating Eq. Ž1.. The c fields presented below have been integrated in an A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 aspect ratio two box with up to 1500 = 3000 unequally spaced grid points, as compared to the temperature and velocity fields which have been integrated with 72 unevenly spaced vertical points by 200 uniform grid points along the horizontal direction. The display of the c fields and the fractal analysis have been conducted on this same grid. It should be noted that these simulations and the visualization display have really stretched the present technological capabilities. We had to store and move about 200 Gbytes of data just for the two runs reported here. Visualization was done on a wall consisting of seven million pixels in order to obtain a global moving view of the complex time-dependent field, which contains a wide spectrum of scales. The computations were made in parallel mode using a SGI cluster of Power Challenge workstations. These exceedingly high-resolution grid configurations will unveil the range of multiple scales developed in the evolution of c and will allow us to conduct a statistical characterization of the turbulent-like structures by fractal analysis with high fidelity. We note that laboratory image processing of turbulent mixing w8x with high-performance CCD cameras has captured up to 2 million pixels. Because of the enormous computational and human resources which this problem has required, we have only investigated two rheological cases. These cases are taken from the extended-Boussinesq convection models in which both adiabatic and viscous heating terms are included w9x. The first case ŽA. has a non-Newtonian, temperature-dependent rheology with a power-law index n s 3 and a temperature-dependent viscosity contrast of 300 across the layer. The rheological law, appropriate for mantle rocks w9x, takes the form: e ij s Aexp Ž BT y CZ . t Žny1.t ij Ž 2. where: Z is the depth; A is a material constant; B s 16.1; C s 6.9; the power-law index n s 3; t ij is the deviatoric stress tensor; t is the second-invariant of the deviatoric stress tensor defined by the trace; e ij is the deviatoric strain-rate tensor. The second case ŽB. has a Newtonian Žn s 1., temperature-dependent rheology with B s 5.4 and C s 2.3. Both models have a temperature-dependent viscosity contrast of 300 across the layer and a depth-dependence in the viscosity increasing by a factor of 10. These models 403 also have a depth-dependent thermal expansivity decreasing by a factor of 1r3 across the layer w10x. The surface dissipation number, D w9x, and surface temperatures, To w9x, are 0.05 and 0.1, respectively, for both cases. The volumetrically averaged Rayleigh numbers are about the same in both cases, namely Ra s 3 = 10 6 . Similar surface Nusselt numbers, around 20, are obtained for both cases. We have included the depth-dependent physical properties to maintain some degree of realism for application in mantle convection, while at the same time focusing on the differences between Newtonian and non-Newtonian rheologies. We have chosen these variable viscosity cases as possible end-member cases in studying mixing of strongly time-dependent mantle convection. 3. Evolution of the passive scalar fields In Fig. 1 we show the differences between the passive scalar field, c , and the temperature fields for the Newtonian case. The initial c field was divided into three equal parts with red at the top, green in the middle and blue at the bottom. We have taken as initial conditions the temperature field from an already convecting solution with a growing instability at the top thermal boundary layer. This thermal initial condition is taken from a situation well past the initial transient. There is an infinite number of initial conditions for the c field we could have employed for integrating Eq. Ž1.. We have selected a relatively simple initial condition for c . The inset shows a descending plume Žblack. plunging down and two upwellings Žpurple. along the side boundaries at a time of 13 Myr after the start of the integration of Eq. Ž1.. We have taken a layer depth of 2000 km to dimensionalize the time by the thermal diffusion time associated with this depth. A dimensionless time of 0.001 then corresponds to 127 Myr. Besides having very close Nusselt numbers, the two rheological models also have nearly the same root-mean-squared velocity, which lies in the neighborhood of 900 in non-dimensional units. The entrainment of warm Žgreen. material into the cold Žred. descending plume is clearly revealed in the c field. Another interesting feature is the appearance of a secondary rising instability at the right. There are 404 A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 Fig. 1. A comparison between the passive scalar field and the temperature field Žinset.. The time is 0.001 after the start of integrating Eq. Ž1.. The rheology is Newtonian, temperature and depth dependent with a viscosity contrast due to a temperature of 300 and to a depth of 10. The volumetrically averaged Rayleigh number is around 3 = 10 6 . The spline grid for the temperature field is 72 = 200 points, and 1000 = 1000 points for the c field. For display, the grid has been expanded by interpolation to 1000 = 2000 points. The initial configuration for c has red at the top, green in the middle and blue at the bottom, all evenly distributed. The initial temperature field has been taken from an already convecting solution. many interesting features picked up by the c field, which reveal much more clearly the complicated dynamics. This figure shows why a much higher resolution is required for an accurate description of the c field. For comparison of the two rheologies, we show in Fig. 2 four snapshots of the c field for the Newtonian case and in Fig. 3 four panels portraying the non-Newtonian case. The first two panels describe the initial stages, while the third and fourth panels display the later development. The final times are approximately the same. In order to comprehend better the dynamic differences, one has to look at the animation of the of the c field. The motions of the c field are really different from the evolution of the T field. One can see the formation of small eddies in the bottom two panels in Fig. 2. Newtonian mixing is primarily dominated by long-wavelength features with two cells and a significant vertical transport component. There is a great deal of mixing by the small eddies. The bottom panel of Fig. 2 shows that, after nearly four overturns, the system is not completely homogenized but is partitioned into different domains, separated by the main descending flow in the middle of the box. In contrast, non-Newtonian mixing takes place in a helter-skelter and meandering fashion and involves the participation by fastscale jets and large-scale coherent structures Žsee the bottom two panels in Fig. 3.. Mixing is less efficient than for Newtonian convection and there are still many islands of unmixed material Žred and blue. left even after 3 overturns, indicating some sort of quenching of the mixing process. Although both rheological flows have similar magnitudes of averaged velocities and surface heat flux, there are significant deviations in the manner of stirring and stretching of the c field displayed by the two rheologies. This finding is not so surprising, because there is firm evidence w13x that non-Newtonian convection tends to generate a jerkier kind of time-dependent fluctuation and more contrasting spatial heterogeneities in the velocity fields than Newtonian convection. These results are different from those found in shear-thinning fluid flows w1x forced by the rotating velocity boundary conditions. There a decrease in the amount of local stretching was found, A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 405 Fig. 2. Temporal evolution of the c field for Newtonian rheology. Same parameter values are used as in Fig. 1. From top to bottom the times are: 9 = 10y4 , 1.2 = 10y3 , 3.7 = 10y3 and 4.0 = 10y3 . 406 A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 Fig. 3. Temporal evolution of the c field for non-Newtonian rheology. The same temperature and depth dependent viscosity contrasts as for the Newtonian case and the power-law index of n s 3. Times are: 7 = 10y4 , 1.3 = 10y3 , 3.0 = 10y3 , and 3.8 = 10y3 . A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 whereas in thermal convection the internal dynamics of the non-Newtonian convection produce the largescale coherent features, giving rise to a somewhat inefficient route for mixing. 4. Fractal analysis of the passive scalar field 4.1. Fractal model deÕelopment and results Fractal analysis can shed light on the distribution of scales in mixing. We have determined the fractal dimension of the high-resolution images representing the c field. The grid points along the horizontal and vertical directions are denoted by nx and ny, respectively. To quantify mixing with time, let us consider a rectangular strip initially at a depth h with a vertical thickness D h and extending horizontally across. Both h and D h are measured in ‘‘grid points units’’. Typically, nx P ny is ( 10 7, nx P D h ( 10 6 . This strip is assigned a ‘‘black’’ color, while the rest of the domain is designated to be ‘‘white’’. As mixing proceeds, the morphology of the initially 407 horizontal strip will become more and more complex. At each time, the resulting black and white pictures are processed by the box counting technique w14x. This processing results in a diagram log ŽN. vs. log ŽS., where N is the minimal w14x number of boxes of size S needed to cover the black color ŽFig. 4.. The box coverage of a black patch of material is illustrated on the right hand side of Fig. 5, where the dotted boxes indicate the presence of some amount of black material in that box with a grid of width S. The ‘‘box-counting’’ fractal dimension Žotherwise known as the Hausdorff or capacity dimension. is given by the slope of the straight segment on the log ŽN. vs. log ŽS. plot. Inspection of the actual box counting results ŽFig. 6. reveals a more complicated pattern. The log ŽN. vs. log ŽS. curves are composed of at least three different linear segments that change their location in time, as mixing proceeds. The trilinear Ž3L. representation of the box-counting results is sketched in Fig. 5. At the finest scales the first linear segment lies below a first crossover scale S1 Ži.e., 1 - S1.. It has a non-fractal slope of 2 and an intercept nx P D h. Fig. 4. Schematic diagram showing the various regimes in mixing from a box-counting perspective. The number of boxes with size S needed to cover an object Žsee black island in the inset. is given by N. Several stages take place with the initial layering, the transient phase and the steady-state regime. Both the initial state and the state of complete homogenization are non-fractal with D s 2. Fractal mixing is characterized by a power-law like Žnon-integer exponent. behavior in the log–log plot of N vs. S. 408 A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 Fig. 5. Schematic diagram illustrating the decomposition of the box-counting algorithm into the boundary and interior contributions. The boundary contributions deal with interfaces and increase with time. The interior contributions decrease with time as the object becomes more convoluted Žsee right panel.. This represents the initial layered state. Initially, this segment occupies all scales ŽS1 s ny at t s 0.. S1 decreases in time as mixing destroys the initial layering by stirring up the larger scales. The intermediate linear segment represents the regime of fractal mixing, which spans scales from S1 to S2, and is decreasing in time with a non-integer slope 1 - 2. Fractal mixing implies a strongly uneven distribution of heterogeneity, the presence of ‘‘islands’’ of unmixed fluids of any size in between S1 and S2. The third linear segment is at the coarse end and spans the scales from a second crossover scale, S2, to ny. It has the ‘‘non-fractal’’ slope of 2, the same as the first segment, but with a higher intercept nx P ny. The third segment represents the completely mixed state, in which each box contains at least one black grid point. First, it occurs only at the largest scales, then its width increases with time, as S2 decreases. The destruction of the fractal subrange is caused by widening of the segment. It is natural in fractal scalings to have high and low cutoffs. For a better understanding of the box-counting method, let us introduce N, N b , Ni, which represent the number of boxes of size S needed to cover the black color, its boundary, and its interior, respectively. Furthermore, let us assume: N ( S D , N b ( S D b , Ni ( S Di Ž 3. where D, D b , Di are the ‘‘box’’ fractal dimensions of the black color, its boundary, and its interior, respectively. From geometrical considerations ŽFig. 5., one may expect the following scenario. First, D b is increasing from 1 to D inf , 1 - D inf - 2, while simultaneously D decreases from 2 to D b . Therefore, the slopes of log ŽN. vs. log ŽS. are function of both time and scale. At a fixed scale, the evolution of the local slope of the log ŽN. vs. log ŽS. will start from 2 Žthe initial layering.; then decreases to a minimum, which at this particular instant can be bigger then or equal to the fractal dimension of the border. Finally, it rises back again to D s 2, as a result of complete homogenization ŽFig. 4.. Fractal dimensions were determined by using different sizes of boxes in the box-counting procedure. This will give an idea as to the influences of the sampling size on the time-dependent fractal signatures. Olson et al. w15x have shown numerically for 40,000 particles that the longer wavelength heterogeneities would be well mixed before the smaller scale inhomogeneities. In Figs. 7 and 8 we show the time histories of the monofractals for small and large boxes, respectively. The fractal dimension as a function of time have been constructed from the N ŽS. curves, shown in Fig. 6. We have also verified the accuracy of the monofractal dimension D by conducting a multifractal w16x analysis on the same data w17x. The boxes used in Fig. 7 have the smallest resolution possible for estimating the fractal dimension. The area occupied by the two sizes of boxes is at most 3 = 10y5 times the total area of the image. This small size yields a very high resolution for determining small-scale heterogeneities. At these A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 409 Fig. 6. The dependence of N on S in logarithmic format for several times: Ža. Newtonian rheology; Žb. non-Newtonian rheology. A grid with 1500 = 3000 points has been used for the box-counting analysis. Times are given for the beginning and at the termination of the analysis. Note the erosion with time at the high S end. From the NŽS. curves we then calculate the fractal dimension D with t. The initial thickness of the heterogeneity, used in the box-counting, is about 0.2 times the total thickness of the layer. 410 A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 Fig. 7. Fractal dimension D vs. time t for the two rheologies. A small observational scale, S between 2 and 4, is used. The initial thickness is the same as in Fig. 6. Fig. 8. Fractal dimension D vs. t for the two rheologies. A larger observational scale, S, between 16 and 32, is used. The initial thickness is the same as in Fig. 6. A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 scales there is a marked difference in the evolution of D between the Newtonian and non-Newtonian rheologies. The initial D h of the monitored heterogeneity is about 1r5 of the layer. Homogenization is faster for the Newtonian case, as can also be observed in the spatial patterns by comparing Figs. 2 and 3. At this small scale of observation, mixing dynamics for both rheologies remain fractal-like for a long time and no signs are in sight for the transition to the path for complete homogenization. Increasing the area of observation by a factor of 8 ŽFig. 8. has a much greater impact on the Newtonian fractal evolution, as we can now reach the valley in D predicted by the model described above. This valley is now attainable because, at this coarser spatial resolution, we have reached a point where there is a transition from fractal mixing. The rise in D indicates that, for this scale of observation, complete homogenization is on the way. On the other hand, even at this relatively large observational scale, the style of non-Newtonian mixing remains fractallike for a long time. We have studied the influences of a thinner initial vertical thickness in Fig. 9, where we reduced D h by a factor of 3 to about 1r15 of the layer. A thinner 411 initial thickness, corresponding to a smaller-scale initial heterogeneity in the mixing process, causes the fractal dimension for both rheologies to drop sharply close to the theoretical limit of 1.35 w11,12,18x. The thinness of the initial layer is responsible for the dominant contribution by the boundary component of the fractal dimension D b . In this vein we may propose a kind of ‘‘spatial universality’’ in that the temporal evolution of D b does not depend on the initial width D h and the asymptotic limits of D s 1.35 w11,18x or D s 1.33 w19x for the interface boundary are reached. The timescales for reaching the valley D are much smaller than the timescales for the greater initial thickness Žcf. Fig. 8.. This would imply that heterogeneities in the high Rayleigh number regime would drop down precipitously to low values of D, where the boundary contributions would be at a maximum, before rising back up to the route of complete homogenization in the interior. 4.2. Box-counting decomposition Box counting results ŽFig. 6. also show that the initial layering subrange Žfrom 1 to S1. is being Fig. 9. Fractal dimension D vs. t for the two rheologies. The observational scale is the same as for Fig. 8, but the initial thickness has been reduced by a factor of 3. A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 412 destroyed by very fast mixing and is reduced to the first couple of scales. Therefore, as a rough approximation, we may assume a two-segment representation of the plot log ŽN. vs. log ŽS.. In this case, the fractal portion is given by: Ns n P Dh SD , S min - S 2 Ž 4. whereas the segment characterizing complete mixing or homogenization is given by: nxny N s 2 , S 2 - S max Ž 5. s where n x and n y are the grid points along the two directions. Next, we can employ the intersection of these two lines from Eq. Ž3. and Eq. Ž4.; that is, the crossover from fractal mixing to complete homogenization, as a quantitative measure of mixing. This condition then determines a ‘‘mixing scale’’, S mix , which is: 1 S mix s S 2 s ny žD / Ž 2y D . h Ž 6. Thus, the mixing scale S mix decreases in time due to a decrease in D, and it also scales inversely with the initial ‘‘concentration’’ D hrny. Thus, a bigger initial inhomogeneity would be mixed earlier. 4.3. Rheological uniÕersality Our two model runs display a remarkable similarity in DŽt. for such different rheologies. Their time scales cannot be directly compared. However, due to similar ‘‘effective Ra numbers’’ a rough comparison can still be made. The monotonic decrease, the spatial universality ŽFig. 9., and the value of the limiting fractal dimension ŽD s 1.35 " 0.05. are essentially the same. The limiting value of the fractal dimension is controlled by the geometry for the interfaces. One suggests here a universal asymptotic Žfor large time. fractal dimension for any initially planar interface, advected by strongly time-dependent convection. The number D s 1.35 for this limiting universal fractal dimension of the interface does not depend on the rheology. This rheological independence confirms that we are dealing with a turbulent advective subrange of scales, in which the mixing is independent of the rheology and is only affected by advection. The physics of advection and surface growth are known to be mostly controlled by whether the processes is conservative or nonconservative w20x. Sreenivasan et al. w8,15x claimed the value 1.35 Ž2.35 for the 3-D flows. as a universal fractal dimension of the interfaces for a wide variety of the turbulent flows. A value of 1.33 has been derived by Procaccia and Zeitak w19x on different assumptions. 4.4. Ultimate limit of conÕectiÕe mixing The above discussion suggests that the convection cannot produce complete homogenization from any initial heterogeneity. According to Eq. Ž5., and substituting in the universal value D s 1.35, there is such a limiting scale, S mix : S mix s ny 1.54 žD / h Ž 7. At scales larger than S mix , complete homogenization is possible, but at scales smaller than S mix , there will always be islands of unmixed material. The exponent 1.54 may contain a ‘‘defect’’ from the power-law exponent 3r2, if the value of 1.33 from w19x is employed instead. An obvious candidate for further mixing is molecular diffusion. Thus, we can give a conservative estimate of the complete homogenization time, as the time to remove heterogeneities at the scale S mix by diffusion: t( S 2mix d Ž 8. where d is the molecular diffusion coefficient. However, this estimate could be orders of magnitude inaccurate by underestimating the diffusion rate by the fractal interface. The phenomenon of molecular diffusion enhanced by the turbulent diffusion is well known w18x. 5. Summary and conclusions We have carried out high-resolution numerical simulations of the passive scalar fields carried by velocities developed in non-Newtonian and Newtonian convection. The passive scalar fields exhibit characteristics of high Reynolds number turbulent flows. Visualization of these complex fields has A. Ten et al.r Earth and Planetary Science Letters 146 (1997) 401–414 revealed that there are substantial differences in the spatial patterns between the two rheologies, with the Newtonian flow displaying faster rates of homogenization and the non-Newtonian configuration retaining islands and clusters of heterogeneities and signs of nonlinear quenching of mixing. We have quantified mixing dynamics by using the box-counting technique for evaluating the fractal dimension of the highly resolved passive scalar field. We have developed a model for time-dependent mixing based on the log–log plot of N, the number of the number of boxes covered by a given color, vs. S, the grid size used in the box-counting. The temporal evolution of mixing can be portrayed by the intersection of two segments in this plot. A transition is predicted for a fractal-type of mixing, characterized by the presence of islands and clusters, to homogenization. We have verified this model with numerical simulations. The style of mixing also depends on the scale of observation. We have found that long-wavelength Newtonian heterogeneities would reach this path toward complete mixing much earlier than for large-scale non-Newtonian inhomogeneities. We would expect these rheological differences in mixing to exist also in 3-D, as toroidal excitation would be greater for non-Newtonian rheology w21x. This model makes a number of predictions, which warrant further studies. Among them are the concepts of ‘‘spatial’’ and ‘‘rheological’’ universality. The first idea is concerned with the changes in the scale of mixing, S mix , with time Žsee Eq. Ž6.. and the second proposal deals with the asymptotic limit of D and its independence from rheology. If these statements are corroborated in the future, then we will have demonstrated the important link between fractal features and mixing. Multifractal analysis should be carried out, because it will shed light on the presence of higher fractal dimensions and their predictions on the transport properties in mixing. We must await the next generation of massively parallel computers to make any inroad into this type of mixing problem in three dimensions. Acknowledgements We thank Bobby Bolshoi and Minye Liu for encouragement and discussions and Bill Newman for 413 an enlightening review. E. Pachepsky was supported by a summer internship program of the Minnesota Supercomputer Institute. We are grateful for the technical assistance provided by Y. Itoh and D.M. Reuteler. This research was supported by Cray Research Inc., Ocean Sciences Program of N.S.F., the Danish Research Council, the Geosciences of D.O.E. and the Universitair Stimulerings Fonds of the Vrije Universiteit, Amsterdam, Netherlands. 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