EXPERIMENTAL AND NUMERICAL STUDY OF HYDRODYNAMICS IN A CIRCULATING FLUIDIZED BED SIRPA KALLIO+, JOHANNA AIRAKSINEN+, MATIAS GULDÉN*, ALF HERMANSON*, JUHO PELTOLA‡, JOUNI RITVANEN#, MAIJU SEPPÄLÄ+, SRUJAL SHAH#, VEIKKO TAIVASSALO+ + VTT Technical Research Centre of Finland, P.O.Box 1000, FI-02044 VTT, Finland Åbo Akademi University, Heat Engineering Laboratory, Piispankatu 8, FI-20500 Turku, Finland ‡ Tampere University of Technology, Department of Energy and Process Enginering, P.O.Box 527, FI33101 Tampere, Finland # Lappeenranta University of Technology, Department of Energy and Environmental Technology, P.O.Box 20, FI-53851 Lappeenranta, Finland * sirpa.kallio@vtt.fi, +358 20 7224015 ABSTRACT Fluid dynamics of circulating fluidized beds (CFB) can be computed with different methods. Typically simulations are conducted as transient to fully describe the complicated flow patterns of dense gas-solid suspensions. The computational mesh used in these simulations must be reasonably fine, which in the case of large industrial processes leads to unfeasibly long computations. To improve the modelling capabilities it is necessary to develop faster simulation methods. The most attractive approach seems to be time-averaged modelling facilitating steady-state simulation of a fluidization process. The model development and closure of the time-averaged equations requires transient simulations. A prerequisite for utilisation of the transient results is that the simulations are validated by measurements. For that purpose, a laboratory scale 2D CFB was built at Åbo Akademi University and experiments were carried out. The apparatus and the experiments are described in the present paper. The behaviour of the CFB was video recorded and the videos were analysed to determine the average voidage distribution in the CFB. The pressure distribution in the bed and the circulation rate of solids were also measured. In addition, PIV measurement methods were tested to evaluate the possibilities to analyse the velocities of individual particles and particle clusters. Two experiments done in the laboratory scale 2D CFB were simulated as transient with the Fluent software using the kinetic theory models of granular flow. The time-averaged volume fractions and velocities of gas and particles were determined for the calculation period in the studied cases. The simulation results were compared with measured flow properties, observing a reasonably good agreement. The results were further analysed with the aim to develop time-averaged CFD models. Since CFB simulations usually require a coarse mesh, additional simulations were conducted to evaluate the mesh dependence of the results with the aim to later develop closure relations that take the mesh into account. Keywords: CFB, CFD simulation, experimental, PIV INTRODUCTION Fluid dynamics of circulating fluidized beds (CFB) can be computed with different methods. Typically the simulations are conducted with Eulerian-Eulerian models based on the kinetic theory of granular flow. The simulations are run as transient to fully describe the complicated flow patterns of dense gas-solid suspensions. These models require a fine computational mesh, which in the case of large industrial processes leads to unfeasibly long computations. To improve the modelling capabilities, it is necessary to develop faster simulation methods. The most attractive approach seems to be timeaveraged modelling facilitating steady-state simulation of fluidization. Several attempts to develop models for steady-state simulations, and for coarse-mesh simulations that require similar equation closures, have been presented in the literature. Agrawal et al. (2001) and Andrews et al. (2005) studied the average drag and stress terms through simulations in small domains with periodic boundary conditions. Zhang & VanderHeyden (2002) suggested an added-mass force closure for the correlation between fluctuations of the pressure gradient of the continuous phase and fluctuations of solids volume fraction. De Wilde (2007) analyzed the same term from simulations and accounted also for the drag force in the derivation of a new closure. Zheng et al. (2006) presented a two-scale Reynolds stress turbulence model for gas-particle flows. Anisotropy and the influence of the real CFB geometry, both essential for successful description of CFB hydrodynamics, were largely left out in the papers listed above. These topics were, however, addressed in earlier work on steady state modelling done at Lappeenranta University of Technology (LUT) and at Åbo Akademi University (ÅA) in the 90’s but accurate equation closure was not possible at that time. New measurement techniques and computational methods have now made a more elaborate equation closure feasible by providing us detailed data on the fluctuations in velocities and voidage. Transient simulations can now be utilized in development of equation closures. With the objective to develop models for steady state simulation, work is now in progress in a three-year joint project at the authors’research units. A prerequisite for utilisation of the results from transient simulations is validation of the models by measurements. For that purpose, a laboratory scale 2D CFB was built at ÅA and experiments were carried out. The present paper deals with experimental and numerical studies conducted in the joint project, which are related to this laboratory scale circulating fluidized bed at ÅA. EXPERIMENTAL The 2D circulating fluidized bed A 2D CFB unit was constructed at Åbo Akademi University (Guldén, 2008). The height of the riser is 3 m and width 0.4 m. The distance between the riser walls is 0.015 m which renders the bed two-dimensional. The CFB pilot is shown in Figure 1. The 0.4 m wide riser walls, the side walls of the solids separator and the walls of the standpipe are made of polycarbonate plates and the rest of plywood and metal plates. Air distributor consists of 8 equally spaced air nozzles. Solids separation is done in a simple separation box from which particles fall through the return leg into a loop seal consisting of two fluidized 10 cm wide sections. The amount of solids in the loop seal and the solids circulation rate are determined from videos taken of the loop seal region when the gas flow to the loop seal is abruptly cut off. The fluidization air flow rates to the riser and the loop seal are measured and controlled by Bronkhorst High-Tech B.V. Thermal Mass Flow Controllers. Pressure was measured at several locations round the CFB with a custom made manometer. Figure 1. The 2D CFB system: a rough sketch, the 2D CFB, and its lower part with the wind box and the loop seal. The experiments The bed material consisted of spherical glass particles with material density of 2480 kg/m3 and the Sauter mean diameter of 0.385 mm. In the ambient conditions of the experiments, the terminal velocity of an average size particle is 2.9 m/s. Two experiments with superficial gas velocities 3.1 m/s and 3.5 m/s were conducted. The solids mass in the riser was in the two experiments 2.76 kg and 2.50 kg, respectively. In the experiments, a dense vigorously fluctuating bottom region was observed with highest particle concentration in the wall regions. Above the bottom zone, the suspension travelled mainly upwards in form of clusters and more dilute suspension between the clusters. At the side walls clusters were seen to fall down. Fig. 2 illustrates the flow structure at the bed bottom and at 114-145 cm height. A denser wall region with falling clusters is seen at both heights. The figures show long narrow clusters and strands everywhere in the bed. The widths of the narrowest strands observed were about 2 mm. At the higher elevation, solids concentration inside the clusters was significantly lower than in the clusters in the bottom region. The behavior of the CFB at bed bottom and at 114-145 cm height was video recorded in both experiments. From each case a 30 s section of the video was analyzed to estimate the average volume fractions in the studied locations. The estimate was based on a comparison between the local instantaneous grey scale values of the video image with the reference values corresponding to an empty bed and to a packed bed. In the interpretation of the concentration, Beer-Lambert law of absorbance of light was utilized. The reference image corresponding to an empty bed at bed bottom and the reference corresponding to a packed bed higher up were not available. Thus the reference values had to be extrapolated from other regions. Since the lighting conditions were not fully uniform, the poor reference values reduced the accuracy of the method. Figure 2. Images from the experiments, from the left: at the bottom at U0=3.1 m/s, at the bottom at U0=3.5 m/s, at 1.14-1.45 m height at U0=3.1 m/s, and at 1.14-1.45 m height at U0=3.5 m/s. Evaluation of the feasibility of PIV as a tool for analysis of solids velocities To get more detailed data for model development and validation, local solids velocities should be measured along with the local voidage. A good method for velocity analysis is Particle Image Velocimetry (PIV) which was tested here to confirm the feasibility of the method. Different imaging methods were tested. In PIV, images of a particle-laden flow are recorded with a short time delay between consecutive frames. The images are then divided into smaller interrogation areas, the intensity profiles of which are crosscorrelated between the consequent frames. The displacement of the particles can be calculated from the correlation peak and translated to velocity. For backlit images the local instantaneous void fraction can be estimated from the Beer-Lambert law on basis of the average gray scale value of the interrogation area. In this study a LaVision ImagerPro HS high speed camera was used with continuous and pulsed lighting. The measurement setup for pulsed light is shown in Fig. 3. The camera has a CMOS sensor with a resolution of 1280x1024 pixels. The maximum recording frequency of the camera at the full resolution is 638 Hz for single-frame and 518 Hz for double-frame images. In the double-frame mode, the two frames to be correlated are recorded with a very short time delay followed by a longer delay before another double frame. In the single-frame mode, images are recorded with even time intervals and each pair of consecutive frames is correlated. Before the cross-correlation the intensities were locally normalized and inverted for the backlit images. Figure 3. The measurement setup for the pulsed light measurements. Pulsed light source To control the exposure in the double-frame mode of the camera, a pulsed light source is needed. Due to the limitations set by the CFB geometry, the light can only be directed from the front or from the behind. Backlighting (light comes from behind) creates a shadow image with the particles in the focus plane sharp and those outside of it blurred. The cross-correlation algorithm weights the sharp particles as they create the highest intensity peaks in the inverted image. However, the method can only be used if the light can penetrate through the suspension. In the CFB this is not the case at the lowest void fractions. Figure 4 shows samples of the recorded images of a 45x34 mm2 window located in the middle of the riser at 130 cm height, and the vector fields calculated from them. Sections c and d in Figure 4 show examples of a situation in which the light doesn't penetrate the clusters and the velocity calculation fails. With frontlighting the light is directed from the direction of the camera. Intensity peaks are generated by the particles closest to the front wall. The velocities of these particles can be determined at any void fraction but these measures only represent the particles right next to the wall. Another drawback is that there is no easy way to estimate the void fraction. The frontlit method can be used to study wall Figure 4. Instantaneous velocity vector fields overlaid on the and those regions th effects original images recorded using a diode-laser backlight. Every 16 of the calculated vectors is displayed. The measurement window is where the backlighting fails marked with red in the schematic on the right. due to low void fractions. In this study a diode-laser was used for its portability. The power of the laser limits the size of the usable measurement window to around 50-80 mm. With these image sizes double-frame imaging has to be used to achieve a short enough time delay between correlated frames. As the maximum pulse length of the laser also decreases as the triggering frequency increases, no time resolution can be obtained and the calculated fields have to be considered as discrete samples. The sampling can be spread over a long period of time without collecting an unreasonable amount of data, making the calculation of representative average fields more convenient. The spatial resolution of the method is around 5 times the diameter of the particles. Continuous light source To get a larger measurement area than the available laser could provide, high frequency fluorescent tubes were used to provide a backlight. Tests showed that with the single frame imaging mode, a 600 Hz imaging frequency and a measurement window over the whole width of the experimental device is a suitable combination. The individual particles are not distinguishable, but the PIV correlation algorithm produced an acceptable solids velocity field except in regions with the lowest voidage. The spatial resolution was around 20 mm. The light source used proved to be slightly inadequate to allow a short enough exposure time to eliminate the motion blur at the highest solids velocities. A more powerful a light source is needed for future measurements. For good average fields the data has to be collected over a long period of time, at least for 20 seconds. Figure 5 shows a sample of a velocity vector field measured over the whole width of the riser just below the solids return inlet. The downward flow near the wall can be seen on the left side, while the incoming solids disturb the wall layer on the right side. Figure 5. Velocity vectors overlaid on the original image, constant backlight. Every 4 th one of the calculated vectors is displayed. The measurement window is marked with red in the schematic on the right. CFD SIMULATION OF THE 2D CFB AND VALIDATION Models used The two experiments conducted in the 2D CFB were simulated with the models based on the kinetic theory of granular flow available in the Fluent 6.3.26 CFD software (Fluent, 2006). The continuity and momentum equations used in the transient simulations can be written for phase q (gas phase denoted by g and solid phase by s) as follows: ∂α q ρ qm ∂α q ρ qmuq , k + =0 ∂t ∂xk (1) ∂α q ρ qm u q ,i ∂t + ∂α q ρ qm u q ,k u q ,i ∂x k ∂p ∂α qτ q ,ik ∂α qτ = −α q + + ∂xi ∂xk ∂x k M + α q ρ qm g i + ( −1) (δ qs +1) q ,ik − ∂p q ∂xi K gs (u g ,i − u s ,i ) δ qs (2) where t is time, x is spatial coordinate, volume fraction, density, u velocity, p gas phase pressure, ps solids pressure, g gravitational acceleration, K drag coefficient, qs Kronecker delta, laminar stress, and M local scale turbulent stress. The granular temperature was obtained from a partial differential equation using the Syamlal et al. (1993) model for granular conductivity. The solid phase granular viscosity was calculated from the model by Syamlal et al. (1993). The solids bulk viscosity and solids pressure were calculated from the formulas by Lun et al. (1984). The k- turbulence model producing the local scale turbulent stress was the version modified for multiphase flows (“dispersed turbulence model”, Fluent (2006)). At the walls, the partial slip model of Johnson and Jackson (1987) was used for the solids with specularity coefficient equal to 0.001 and the free slip boundary condition was used for the gas. For gas-particle interaction, a combination of the Wen & Yu (1966) (at the voidage above 0.8) and Ergun (1952) equations was used. The frictional solids stresses were calculated from the model of Schaeffer (1987). The first-order discretization for time stepping and the second-order spatial discretization were employed. The 2D grid of the simulation consisted of 31648 elements with the mesh spacing of 6.25 mm. The time step in the simulation was 0.2 ms. Air inflow velocity at the bottom was described by a function that reproduces the orifice locations. Simulation results and comparisons with measurements For comparison with measurements, the simulations were first run till a steady state and then for an extra 10 s time period to obtain averages of the velocities and void fractions. Fig. 6 illustrates the typical flow patterns obtained in the simulations and the corresponding time averages at the two fluidization velocities. The flow patterns are similar to the ones observed in the experiments. Due to the coarseness of the computational mesh, however, the simulated clusters are wider, the thinnest ones being 1.5 cm wide. Otherwise the flow structure is correct with a dense bottom bed and dense wall regions with downflow of solids. Figure. 6. Instantaneous and average solids volume fractions at U0=3.1 m/s (left) and at U0=3.5 m/s. A comparison between measured and simulated solids circulation rates was also done. Both in the experiments and in the simulations, an increase in the fluidization velocity increased the circulation rate. Moreover, solids circulation rates obtained in the simulations were of the same order as measured in the laboratory unit. Gas phase static pressure was measured at several elevations at the wall opposite to the solids return. Figure 7a shows a comparison between the measured and simulated average pressure profiles at the wall. The simulated pressure profile is close to the measured one at the lower fluidization velocity but a clear discrepancy is seen at the higher velocity. From the measured pressure profile, the vertical voidage profile could be estimated. The results are depicted in Fig. 7b together with the average solids volume fraction profile obtained from the simulations. In addition, the average values obtained from the analysis of the videos, taken at two elevations during the experiments, are marked in Figure 7b. In general, the match is reasonably good considering the inaccuracies in both of the experimental methods. a) b) Figure. 7. Comparison of measured and simulated vertical pressure (a) and solid volume fraction (b) profiles in the experiments with fluidization velocities 3.1m/s and 3.5 m/s. From the videos, the average lateral solid volume fraction profiles were determined at 20 cm and 130 cm heights. Figure 8 shows a comparison between the measured and the simulated lateral solids volume fraction profiles. In the profiles determined from the videos there is clear asymmetry. This is very likely caused by the uneven lighting in the experiments combined with the lack of good reference images for fixing the concentration scale. Otherwise the measured and simulated profiles are in good agreement. The thin dense wall region observed in the simulations could also be detected in the experimental results. Figure 8. Comparison of simulated and measured lateral solid volume fraction profiles at 20 cm and 130 cm heights at fluidization velocities 3.1 m/s and 3.5 m/s. From the simulation results, the average lateral velocity profiles could be calculated. Figure 9 shows the profiles obtained in the two simulations at 130 cm height. A downflow region is seen at the walls. This corresponds to the visual observations and the velocity fields determined by PIV. No average velocity profiles were measured at this stage. Figure 9. Lateral profiles of the solids vertical velocity component at fluidization velocities 3.1 m/s and 3.5 m/s determined from the simulations 130 cm height. Simulations of particle mixtures In fluidized bed combustors the solid phase consists of particles with different sizes, densities and compositions. Thus any model used to describe CFB hydrodynamics should also be applicable to mixtures of particles. Experiments are planned to be conducted in the 2D CFB using mixtures of particles to serve as validation of multi-particle models. At this stage, preliminary simulations were done to test the capability of the Fluent software to simulate mixtures. In the first simulation, a single solid phase was divided into two and Fluent was proved to correctly treat this division. Next, different mixtures of two types of particles were simulated. An example of resulting segregation of the two particle sizes is shown in Fig. 10. The results seem reasonable but validation through measurements is required and will be done in the future. a) b) c) d) Figure 10. Simulation results for a particle mixture with 10 mass% of particles with dp=0.650 mm and 90 mass% with dp=0.270 mm. Fluidization velocity U0 = 2 m/s. a) volume fraction of particles with dp=0.650 mm, b) volume fraction of particles with dp=0.270 mm, c) 10 s average volume fraction of particles with dp=0.650 mm, d) 10 s average volume fraction of particles with dp=0.270 mm. TRANSIENT CFD MODELING USING COARSER MESHES As long as time-averaged models are not available, the most feasible alternative to simulate gas-solid flow in a large scale CFB is to use a coarse mesh in a transient simulation and to time-average the results. In coarse mesh simulations information on the local flow structures is lost when the flow gets filtered by the mesh. The lost information must be brought back into the system through closure models to predict the hydrodynamics correctly. This corresponds to what has to be done in time-averaged modelling where all information on time variations of the flow needs to be fed to the model through equation closures. In this study, the effect of mesh size was evaluated by simulating the experiment conducted in the 2D CFB at fluidization velocity 3.1 m/s in three different meshes with spacings 0.625 cm, 2.5 cm and 5 cm. The time step in all simulations was 0.2 ms. The models were the same as used in the validation simulations of the previous section. The only difference is in the description of the gas inlet. With the coarse meshes used here, it is not possible to describe accurately the gas flow through the separate orifices. Thus the entire bottom of the riser was defined as an inlet with a constant gas inflow velocity. In each of the simulations, computations start from a situation where solids are uniformly distributed throughout the riser. After 10-second simulation, a stable solution is reached, with solids leaving the riser from the outlet and entering the bed through the return leg. The mass flow rate of solids entering the system through the return channel is adjusted in such a way that, at any instant of time the mass in the riser remains the same as in the experiment. Averaging is then performed for another 20 seconds. Timeaveraged contours of solid volume fraction and the Favre-averaged gas y velocity for different mesh sizes are shown in Figure 11. Figure 11. Simulations with mesh spacings 0.625 cm, 2.5 cm and 5 cm: a) Time-averaged solid volume fraction and b) Favre-averaged gas y velocity. As seen from Fig. 11a, with the smaller mesh spacing of 0.625 cm, the time averaged solid volume fraction contours shows presence of small scale clusters. When the mesh spacing is increased, the time-averaged solids volume fraction shows a much more uniform distribution and the mesoscale structures of the flow get filtered. This is also seen in Fig. 11b. When the mesh spacing is increased, channelling in the middle of the riser and wider wall layers are observed in the averaged velocity profiles. Thus the simulations show that the results are mesh dependent. To obtain the same results in different meshes, closure equations that take the mesh into account need to be developed. A fine mesh is computationally expensive. For the above gas-solid flow calculations of 30 s real time, the CPU time consumed by a single processor was around 8 hours with the 5 cm mesh spacing, with 2.5 cm mesh spacing it was 14 hours and with 0.625 cm mesh spacing 129 hours. TOWARDS TIME-AVERAGED MODELING A transient simulation in a coarse mesh is one alternative for simulating large CFBs. Long simulation times are required to obtain a representative average flow field through averaging of the transient simulation results. A faster alternative would be to directly compute the average flow field from steady state models. Unfortunately, such models are not available to date. For that purpose, models for CFBs are developed in the current research project. As an initial step in the development, the instantaneous continuity and momentum equations, Equations (1) and (2), are averaged over time. First we need to define the average quantities. A time average, also called Reynolds average, of a variable φ is defined as φ= 1 t + ∆t φ dt ∆t ∫t (3) The instantaneous values can now be written as φ = φ + φ ' . This average is used for the volume fraction q and pressure p. Thus, e.g., α q = α q + α q ' and p = p + p ' , and, consequently, α q ' = 0 and p ' = 0 . A Favre average or a phase-weighted average is defined as follows 〈φ 〉 = α qφ αq (4) Favre averaging is applied on velocities and we denote the average velocity by U q , i ≡ 〈u q ,i 〉 . For the instantaneous velocity we have then u q ,i = U q ,i + u q ,i " . Note that 〈u" q , i 〉 = 0 but practically always u" q ,i ≠ 0 . We obtain now the time-averaged continuity equation for phase q ( ∂α q ρ qm ∂ρ qm α qU q , k + =0 ∂t ∂xk and time-averaged momentum equation for a phase q qm is a constant): (5) ∂α q ρ qmU q,i ∂t + ∂α q ρ qmU q, k U q,i ∂x k = α q ρ qm g i − α q ∂p ′ ∂α qτ q ,ik ∂p + − α q′ ∂x i ∂x k ∂xi (6) + ∂α qτ M ∂x k q ,ik + (−1) (δ qs +1) K gs (u gi − u si ) − ∂ pq ∂xi δ qs − ∂ρ qm α q u q′′, k u q′′,i ∂x k The terms on the right hand side are the gravitation term, pressure term, pressure fluctuation term, laminar stress, turbulent stress, drag force, solid pressure term, and the Reynolds stress term. The gravitation and pressure terms can be calculated from the basic average flow properties but the rest of the terms need to be modelled. To evaluate the importance of the different terms, a long (about 15 min) simulation of the experiment at U0=3.5 m/s was conducted and the computation results were timeaveraged. Fig. 12 shows the terms in the time-averaged balance equation for the solid phase vertical velocity component. The time derivative in the time-averaged equation can be discarded in this case. In order to simplify the comparison of the terms, the convection term in Equation (6) is moved to the right hand side. ∂α s ρ smU s , kU s, y 1: − ∂xk 2 : α s ρ sm g y 3: −αs ∂p ∂x y 4 : − α s′ ∂p′ ∂x y 5: 6: ∂α sτ s , yk ∂xk ∂α sτ M q , yk ∂ xk 7 : K gs (u gy − usy ) 8: − 9: − ∂ ps ∂x y ∂ρ sm α s us′′, k us′′, y ∂xk Figure 12. The different terms in the time-averaged balance equation of the solids vertical velocity component plotted on the riser centre line as a function of height. Although the simulated time period was very long, the average velocities are still not perfectly smooth functions of the spatial coordinates. Consequently, the velocity derivatives are even more restless which is seen in the large spatial variations in the convection term. However, a comparison of the magnitudes of the different terms can still be made. In the upper part of the riser, the largest terms are the drag term and the gravitation term. The Reynolds stress term and the term originating from the correlation between fluctuations in gas phase pressure and solids volume fraction are significant in the bottom region. The turbulent stress term and solid pressure term are small over the whole riser length on the centre line. However, a wider analysis of the terms in the bottom bed showed that solids pressure can be significant in the dense wall regions whereas the turbulent stresses are insignificant everywhere in the CFB. The largest terms to be modelled are the drag forces and the Reynolds stresses. Modelling of the pressure fluctuation term was considered in De Wilde (2007) and a similar approach could be considered also here. The average drag forces have typically been described by means of a correction to the drag coefficient as a function of suspension density, see e.g. Kallio et al. (2008). Analysis of the average drag forces in the transient simulation could be used to modify the earlier drag correction models. In Kallio et al. (2008), the different components of the Reynolds stress tensors were analysed from another transient simulation. An order of magnitude difference was observed between the different components. Thus no assumption of isotropy, as often made in modelling of single phase turbulence, can be made in modelling of turbulence in dense gas-solid flows. The different components need to be modelled separately and preferably through separate transport equations for each Reynolds stress component. Transport equations for the Reynolds stresses of a phase q can be obtained from the averaged momentum equations and they can be written as follows: ∂ρ qm α q u′qi′u′qj′ ∂t + ∂ρ qmU qk α q u′qi′u′qj′ ∂xk = Pq ,ij + Π q ,ij + Dq ,ij + M q ,ij − ε q ,ij + Gg ,ij + Fq ,ij + δ qs S q ,ij (7) where Pq,ij is the production of the Reynolds stresses ∂U q , j ∂U q ,i Pq ,ij = −α q ρ q u"q ,k u"q ,i + u"q ,k u"q , j ∂x k ∂x k q,ij (8) is the pressure-strain covariance (or redistribution) term ∂α u" ∂α u" Π q ,ij = p' q q , j + q q ,i ∂x ∂x j i (9) Dq,ij represents the turbulent, pressure and molecular diffusion Dq ,ij = − ( ∂ α q ρ q u"q,i u"q , j u"q , k + α q p ' u"q ,iδ jk + α q p ' u"q, jδ ik − α qτ q, jk (u" )u"q ,i − α qτ q ,ik (u" )u"q , j ∂xk ) (10) q,ij is the dissipation term ε q ,ij = α qτ q , jk (u" ) ∂u"q ,i ∂xk + α qτ q ,ik (u" ) ∂u"q , j ∂xk (11) Fq,ij is the turbulent mass flux Fq ,ij = u"q ,i ∂α qτ q , jk (U ) ∂xk + u"q , j ∂α qτ q ,ik (U ) ∂xk (12) and Mq,ij arises from the modelling the local scale turbulence M q ,ij = u"q ,i ∂α qτ qM, jk ∂x k + u" q , j ∂α qτ qM,ik (13) ∂x k The phase interaction term Gq,ij reads Gq ,ij = K gs (u ′g′,i u ′s′, j + u ′g′, j u ′s′,i − 2u ′q′,i u ′q′, j ) + (−1) + (−1) (δ qs +1) (δ qs +1) K gs u ′q′,i (U g , j - U s , j ) (14) K gs u ′q′, j (U g ,i - U s ,i ) The two-phase term Ss,ij is S s ,ij = −u"s ,i ∂ps ∂p − u"s , j s ∂x j ∂xi (15) These terms in the balance equation for the vertical normal component of the solid phase Reynolds stress are plotted in Fig. 13 on the centreline of the riser. Here again we see that the simulation is too short to produce smooth averages. As shown in Fig. 13, the largest term is the phase interaction term Gq,ij and a couple of other terms like the production and dissipation terms are also significant. In a time-averaged CFD simulation, only the stress production terms Pq ,ij needs no modelling. All the other terms need to be modelled. Performance and applicability of various modelling alternatives for the Reynolds stresses will next be examined and tested. 5000 1 2 4000 3 4 3000 5 6 2000 7 8 1000 9 10 0 ∂U s, y ∂xk 1 : Ps, yy = −2α s ρ s u"s, k u"s, y 2 : Π s , yy = 2 p' ∂α s u"s , y 4 : Dsp, yy ∂x y ( ∂ α s ρ s u"s, y u"s, y u"s, k ∂x k ∂ = −2 α s p' u"s, y ∂x y 3 : DsT, yy = − 5 : Dsm, yy = 2 ( ) ( ∂ α sτ s , yk (u" )u"s , y ∂xk 6 : Fs, yy = 2u"s, y ) ) ∂α sτ s , yk (U ) ∂x k 7 : ε s , yy = 2α sτ s , yk (u" ) ∂u" s , y ∂x k 8 : Gs , yy = 2K gs (u g′′, y u s′′, y − u s′′, y u′s′, y ) + 2 K gs us′′, y (U g , y - U s , y ) -1000 9 : S s, yy = −2u"s , y -2000 0 0.5 1 1.5 y [m] 2 2.5 3 10 : M s , yy = 2u" s, y ∂p s ∂x y ∂α sτ sM, yk ∂x k Figure 13. The terms in the balance equation for the vertical normal component of the solid phase Reynolds stress [kg/ms3]. CONCLUSIONS Fluid dynamics of circulating fluidized beds (CFB) can be computed with a variety of methods. Typically the simulations are conducted with Eulerian-Eulerian models based on the kinetic theory of granular flow. These models require a fine computational mesh and, in addition, that the simulations are run as transient, which in the case of large industrial processes leads to unfeasibly long computations. To improve the modelling capabilities it is necessary to develop faster simulation methods. The most attractive approach seems to be time-averaged modelling facilitating steady-state simulation of fluidization. An order of magnitude slower but still feasible alternative would be to use a coarse mesh and special mesh-dependent closure equations in a transient simulation. A prerequisite for utilisation of transient simulations in steady-state model development is validation by measurements. Thus, a 0.4 m wide and 3 m high laboratory scale 2D CFB was built at Åbo Akademi University. Experiments were carried out for validation of the CFD simulations. The behaviour of the process was video recorded and the videos were analysed to determine the average voidage distribution in the CFB. The pressure distribution in the bed and the circulation rate of solids were also measured. The measured flow properties were compared with simulation results, observing a reasonably good agreement. In addition, PIV measurements were conducted to evaluate the possibilities to determine the velocities of individual particles and particle clusters. The high speed imaging, together with time resolved velocity fields and void fraction estimates based on the gray scale value, proved to provide an excellent visualization of the velocity of the clusters in the CFB. Results from a long simulation were analysed to evaluate the requirements for the closure of the time-averaged equations. The largest terms to be modelled are the gassolid interaction and the Reynolds stress. 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(1966). Mechanics of fluidization, Chemical Engineering Progress Symposium Series, Vol. 66, pp.100-111 ZENG, ZH.X., ZHOU, L.X. (2006). A two-scale second-order moment particle turbulence model and simulation of dense gas–particle flows in a riser, Powder Tech., Vol. 162, pp. 27-32 ZHANG, D.Z., VANDERHEYDEN, W.B. (2002). The effects of mesoscale structures on the macroscopic momentum equations for two-phase flows, Int. J. of Multiphase Flow, Vol. 28, pp. 805-822 ACKNOWLEDGEMENT The financial support of Tekes, VTT Technical Research Centre of Finland, Fortum Oyj, Foster Wheeler Energia Oy, Neste Oil Oyj and Metso Power Oy is gratefully acknowledged.